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  • Articles  (481)
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  • 01. Atmosphere::01.01. Atmosphere::01.01.07. Volcanic effects
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  • Springer  (481)
  • American Geophysical Union
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  • 1990-1994  (208)
  • 1980-1984  (176)
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  • Articles  (481)
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  • 1
    Electronic Resource
    Electronic Resource
    Polymerization of acrylamide initiated by Ce(IV)-lactic acid redox system (1983)
    Springer
    Colloid & polymer science 261 (1983), S. 188-189 
    Details
    ISSN: 1435-1536
    Keywords: Polymerization ; kinetics ; redox polymerization ; acrylamide
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology , Mechanical Engineering, Materials Science, Production Engineering, Mining and Metallurgy, Traffic Engineering, Precision Mechanics
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01410701
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  • 2
    Electronic Resource
    Electronic Resource
    Influence of specimen thickness on isothermal crystallization kinetics. A theoretical analysis (1984)
    Springer
    Colloid & polymer science 262 (1984), S. 366-373 
    Details
    ISSN: 1435-1536
    Keywords: kinetics ; isothermal crystallization ; polymer ; spherulite ; differential scanning calorimetry
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology , Mechanical Engineering, Materials Science, Production Engineering, Mining and Metallurgy, Traffic Engineering, Precision Mechanics
    Notes: Abstract In the DSC technique, isothermal crystallization experiments are usually performed on thin flat specimens, but their interpretation generally uses theories developed for an unbounded volume. In this paper, isothermal crystallization of spherical entities in the volume limited by two parallel infinite planes is considered. Our model, derived from Avrami's theory, gives an analytical expression for the transformed volume fraction as a function of time. It is shown that the influence of thickness becomes important when thickness becomes of the order of or smaller than the average spherulite radius. The main effects of a decreasing thickness are a slower crystallization kinetics and a decrease in the Avrami exponent. These results can be used to interpret experimental data obtained in isothermal polymer crystallization.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01410254
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  • 3
    Electronic Resource
    Electronic Resource
    The effect of TiO2 on the kinetics of polyamide 6 crystallization (1983)
    Springer
    Colloid & polymer science 261 (1983), S. 621-625 
    Details
    ISSN: 1435-1536
    Keywords: Polyamide 6 ; crystallisation ; kinetics ; titania
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology , Mechanical Engineering, Materials Science, Production Engineering, Mining and Metallurgy, Traffic Engineering, Precision Mechanics
    Notes: Abstract The kinetics of isothermal and nonisothermal crystallization of polyamide-6 (PA6) containing titania was studied by means of DSC. It was found thatTiO 2 causes an acceleration in the crystallization of polyamide-6 and lowers the value of the Avrami exponent,n. The presence of TiO2 does not affect equilibrium melting pointT m 0 , glass temperatureT g, or surface free energiesσ e andσ of the basal and lateral surfaces.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01415030
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  • 4
    Electronic Resource
    Electronic Resource
    Proceedings: Ad Hoc Mathematical Fire Modeling Working Group (1984)
    Springer
    Fire technology 20 (1984), S. 47-63 
    Details
    ISSN: 1572-8099
    Keywords: Extinguishment ; fire modeling ; mass loss ; heat release ; char ; reflash ; sprinklers ; radiant flux ; kinetics ; reaction rate ; heat loss ; ash ; latent heat ; spray density ; extinguishing agents
    Source: Springer Online Journal Archives 1860-2000
    Topics: Architecture, Civil Engineering, Surveying
    Notes: Abstract The Ad Hoc Mathematical Fire Modeling Working Group was organized about seven years ago to facilitate voluntary cooperation and coordination in developing mathematical fire modeling capability. The group has a steering committee of representatives of agencies that support fire modeling and related research. These include the National Bureau of Standards' Center for Fire Research, Factory Mutual Research Corp., the Naval Research Laboratory, NASA, and the Federal Aviation Agency. The Group holds plenary meetings when it seems desirable to do so (about once each 1 1/2 years), and workshops on topical subjects. Three workshops were held in 1983. Normally, Group meetings are held before or after other meetings at which a number of interested personnel would likely be present. Minutes are mailed to those who attended and to others (including European and Japanese personnel) who have indicated interest. This workshop was arranged by Ron Alpert of Factory Mutual Research Corp. and held at their facilities at Norwood, MA, in November 1983.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF02384150
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  • 5
    Electronic Resource
    Electronic Resource
    Effects of pressure on the kinetics of the dehydration of carbonic acid and the hydrolysis of CO2 in aqueous solution (1982)
    Springer
    Journal of solution chemistry 11 (1982), S. 339-346 
    Details
    ISSN: 1572-8927
    Keywords: Carbon dioxide ; hydrolysis ; aqueous solution ; kinetics ; activation volume
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology
    Notes: Abstract The pressure dependence of the dehydration reaction of H2CO3 was measured in acidic aqueous solution for pressures up to 1 kbar using a high-pressure stopped-flow instrument. The corresponding volume of activation was found to be 6.4±0.4 cm3-mol−1 at 25°C and 0.5 ionic strength. Volume equation calculations result in a value of −9.9±1.9cm3-mol−1 for the volume of activation for the hydrolysis of CO2 under the same conditions. For the first time, the reaction mechanism can be interpreted in terms of dissociative and associative modes, respectively. These data are used to construct an overall reaction volume profile.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00649292
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  • 6
    Electronic Resource
    Electronic Resource
    Thermodynamic parameters of coupled chemical reactions from temperature jump relaxation amplitudes (1981)
    Springer
    Journal of solution chemistry 10 (1981), S. 39-50 
    Details
    ISSN: 1572-8927
    Keywords: Temperature jump ; kinetics ; thermodynamics ; TRIS ; iminodiacetic acid ; magnesium ion ; phenol red
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology
    Notes: Abstract Equations describing the temperature jump amplitudes associated with a system of two coupled reactions (TRIS-phenol red) as well as the ternary system (Mg2+-iminodiacetic acid-phenol red) are presented. The termodynamic parameters calculated from experimentally measured temperature perturbation amplitudes using a multiparametric curve fitting procedure are found to be in good agreement with those determined from pH- and costant rate thermometric titrations. For phenol red, pK I =7.55, ΔH I =3.45 kcal, and for Mg2+ iminodiacetic acid, log K M =2.84, ΔH M =3.25 kcal, were obtained. It is shown that this method can be used to determine accurate thermodynamic enthalpy changes over a narrow temperature interval of less than 1.0°C from a single experiment requiring about 50 μl of sample solution.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00652779
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  • 7
    Electronic Resource
    Electronic Resource
    Rate and thermodynamic studies of the interaction between water and iso-butyl cellosolve by ultrasonic methods (1983)
    Springer
    Journal of solution chemistry 12 (1983), S. 771-781 
    Details
    ISSN: 1572-8927
    Keywords: Ultrasonics ; kinetics ; aqueous solution ; iso-butyl cellosolve
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology
    Notes: Abstract Ultrasonic absorption and velocity measurements in aqueous solution of iso-butyl cellosolve (ethylene glycol iso-butyl ether) as a function of the concentration are reported. The two relaxational absorptions have been attributed to the perturbation of the equilibria expressed by AB⇌A+B and Aα(1/n)An where A is the solute, B is the solvent, AB is the complex and A n is the solute aggregate. The rate constants for each step have been determined. From the concentration dependence of the maximum excess absorption per wave length, the enthalpy change and the volume change for the reaction between the solute and the solvent have been determined for aqueous solutions of butyl cellosolve (ethylene glycol n-butyl ether), iso-butyl cellosolve and propyl cellosolve (ethylene glycol n-propyl ether). The results are consistent with a hydrogen bonding reaction. The effect of the ethers on water structure are considered and it is clear that the fraction of water molecules which can hydrogen bond to the solute decreases with the increasing hydrophobicity of the solute.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00653180
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  • 8
    Electronic Resource
    Electronic Resource
    The kinetics of the solvolysis of chloropentacyanocobaltate(III) ions in water containing 2-methoxyethanol or diethylene glycol: A contrast with the effect of more hydrophobic cosolvents (1994)
    Springer
    Journal of solution chemistry 23 (1994), S. 1089-1100 
    Details
    ISSN: 1572-8927
    Keywords: Solvolysis ; kinetics ; aqueous solvent mixtures ; Co(III) complexes
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology
    Notes: Abstract The kinetics of the solvolysis of [Co(CN)5Cl]3− have been investigated in water +2-methoxyethanol and water + diethylene glycol mixtures. Although the addition of these linear hydrophilic cosolvent molecules to water produces curvature in the variation of log(rate constant) with the reciprocal of the dielectric constant, their effect on the enthalpy and entropy of activation is minimal, unlike the effect of hydrophobic cosolvents. The application of a Gibbs energy cycle to the solvolysis in water and in the mixtures using either solvent-sorting or TATB values for the Gibbs energy of transfer of the chloride ion between water and the mixture shows that the relative stability of the emergent solvated Co(III) ion in the transition state compared to that of Co(CN)5Cl3− in the initial state increases with increasing content of cosolvent in the mixture. By comparing the effects of other cosolvents on the solvolysis, this differential increase in the relative stabilities of the two species increases with the degree of hydrophobicity of the cosolvent.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00976258
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  • 9
    Electronic Resource
    Electronic Resource
    The effects of aqueous solvent structure on the mutarotation kinetics of glucose (1977)
    Springer
    Journal of solution chemistry 6 (1977), S. 203-216 
    Details
    ISSN: 1572-8927
    Keywords: Glucose ; kinetics ; mixed solvent ; kinetic isotope effect ; enthalpy of activation ; entropy of activation ; tetrahydrofuran ; tert-butanol ; mutarotation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology
    Notes: Abstract The mutarotation rates of glucose in aqueous mixtures of tetrahydrofuran andtert-butanol in the mole fraction (xi) range 0〈xi〈0.2 have been measured at 5° intervals in the range 5–35°C. The kinetic deuterium isotope effects have been determined for the same solvent compositions at 25 and 35°C. A statistical analysis of the Arrhenius plots indicates that the experimental errors, although small, are too large for the establishment of any compensation behavior between ΔH
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00646739
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  • 10
    Electronic Resource
    Electronic Resource
    Kinetics of the solvolysis oftrans-dichlorotetra-(4-t-butylpyridine)-cobalt(III) ions in water +t-butyl alcohol mixtures (1990)
    Springer
    Journal of solution chemistry 19 (1990), S. 1073-1084 
    Details
    ISSN: 1572-8927
    Keywords: Solvolysis ; kinetics ; mixtures of water+cosolvent
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology
    Notes: Abstract Rates of solvolysis of the complex cation [Co(4tBupy)4Cl2]+ have been determined in mixtures of water with the hydrophobic solvent, t-butyl alcohol. The solvent composition at which the extremum is found in the variation of the enthalpy ΔH* and the entropy ΔS* of activation correlates well with the extremum in the variation of the relative partial molar volume of t-butyl alcohol in the mixture and the straight line found for the variation of ΔH* with ΔS* is coincident with the same plot for water + 2-propanol mixtures. A free energy cycle is applied to the process initial state (C n+) going to the transition state [M(n+1)+...Cl−] in water and in the mixture using free energies of transfer of the individual ionic species, ΔG t o (i), from water into the mixture. Values for ΔG t o (i) are derived from the solvent sorting method and from the TATB/TPTB method: using data from either method, changes in solvent structure on going from water into the mixture are found to stabilize the cation in the transition state, M(n+1)+, more than in the initial state, C n+. This is compared with the application of the free energy cycle to the solvolysis of complexes [Co(Rpy)4Cl2]+ and [Coen2LCl]+ in mixtures of water with methanol, 2-propanol or t-butyl alcohol: the above conclusion regarding the relative stabilization of the cations holds for all these complexes in their solvolyses in water+alcohol mixtures using values of ΔG t o (Cl−) from either source.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00649452
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  • 11
    Electronic Resource
    Electronic Resource
    Effect of ionic interactions on the rates of reduction of Cu(II) with H2O2 in aqueous solutions (1992)
    Springer
    Journal of solution chemistry 21 (1992), S. 1271-1287 
    Details
    ISSN: 1572-8927
    Keywords: Cu(II) ; kinetics ; reduction ; temperature dependence ; H2O2, NaCl, NaBr, NaClO4
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology
    Notes: Abstract The rates of reduction of Cu(II) with H2O2 have been measured in NaCl and NaBr solutions and mixtures with NaClO4 as a function of pH (6 to 9), temperature (5 to 45°C) and ionic composition (0.1 to 6M). The effect of pH on the rates was found to be independent of temperature and ionic composition. The rates increased as a function of [H+] raised to the power of 1.3 to 1.6. Speciation calculations indicate that this pH dependence can be attributed to Cu(OH)2 being the reactive species. The rate constants in NaCl and NaBr and mixtures with NaClO4 were independent of ionic strength, but proportional to the halide concentration raised to the power of 2.0 (0.2 to 2.6M). These results can be attributed to Cu(OH)2Cl 2 2− being the reactive species to reduction with H2O2. The Cu(I) halide complexes formed from the reduction are not easily oxidized with O2 or H2O2. The faster rates in Br− solutions, which form stronger complexes with Cu+, support this contention. Measurements made in NaCl with added NaHCO3, NaB(OH)4 EDTA, NTA and glycine were also made. These measurements indicate that the CuL complexes (L=B(OH) 4 − , CO 3 2− , EDTA, NTA, and glycine) are not very reactive to reduction with H2O2. The addition of Mg2+ or Ca2+ caused the rates to increase due to the formation of MgL or CaL complexes and the resultant release of reactive Cu2+.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00667222
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  • 12
    Electronic Resource
    Electronic Resource
    Thermodynamics of coupled reactions by the method of dynamic titration: the Nickel(II)-salicylate ion system (1994)
    Springer
    Journal of solution chemistry 23 (1994), S. 483-500 
    Details
    ISSN: 1572-8927
    Keywords: Thermodynamics ; kinetics ; chemical relaxation ; temperature-jump ; amplitudes
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology
    Notes: Abstract Amplitudes of chemical relaxation signals can provide useful information as to the thermodynamics of coupled chemical reactions. The temperature-jump technique has been used to investigate the thermodynamic behavior of the Nickel(II)-3,5-dinitrosalicylate system in buffer solution, where complex formation steps are coupled to proton transfer steps. The analysis of the relaxation curves is based on the transformation of a set of coupled elementary reactions into a set of uncoupled ‘normal reactions.’ By analogy with classical titrations, the experiments have been performed by changing the metal ion concentration at constant ligand concentration and pH. Each measured amplitude is associated in this way to a point of a ‘dynamic titration’ and a procedure is formulated by which the values of the equilibrium constants and enthalpies of the normal reactions are simultaneously obtained by simple linear plots. From the dependence of these parameters on suitable functions of the concentrations of the reactants the values of ΔG° and ΔH° of the individual steps are derived. It is shown that the addition of a buffer (instead of an indicator) influences the stoichiometric coefficients of the normal reaction in such a way that measurable amplitudes are produced in systems that, as the presently investigated, in unbuffered solution would remain insensitive to the external perturbation. The circumstances under which the dynamic method offers advantages over the classical techniques are discussed.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00972614
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  • 13
    Electronic Resource
    Electronic Resource
    Solvent effects on the acid-catalyzed hydrolysis of tetramethylurea (1976)
    Springer
    Journal of solution chemistry 5 (1976), S. 163-169 
    Details
    ISSN: 1572-8927
    Keywords: Solvent effects ; tetramethylurea ; hydrolysis ; hydrogen bonding ; kinetics
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology
    Notes: Abstract Tetramethylurea was hydrolyzed in aqueous hydrochloric acid at temperatures of 80, 90, and 100°C. All reactions were carried out in an excess of both tetramethylurea and water, with first-order dependence on acid concentration being observed. As the concentration of water was increased, the rate of hydrolysis decreased until equimolar amounts of water and tetramethylurea were present. Subsequent addition of water had no effect on the observed rate.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00654333
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  • 14
    Electronic Resource
    Electronic Resource
    A method to determine the relative value of the barriers of carbon chain growth and termination in Fischer-Tropsch synthesis: elementary reaction kinetics for chain growth (1993)
    Springer
    Catalysis letters 19 (1993), S. 93-97 
    Details
    ISSN: 1572-879X
    Keywords: Fischer-Tropsch synthesis ; reaction activation barrier ; carbon chain growth and termination ; kinetics
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology
    Notes: Abstract A method is established, by which the difference of the reaction activation barriers of carbon chain growth and termination in Fischer-Tropsch (FT) synthesis can be determined from experiments. A FT synthesis is carried out on Fe/Zn catalyst. We apply the method to analyze the experimental result and obtain the difference of reaction activation barriers of carbon chain growth and termination of α-olefins on the catalyst.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00765205
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  • 15
    Electronic Resource
    Electronic Resource
    Kinetics and mechanisms of the low-temperature degradation of cellulose (1994)
    Springer
    Cellulose 1 (1994), S. 26-56 
    Details
    ISSN: 1572-882X
    Keywords: low-temperature degradation ; kinetics ; mechanisms ; electrical insulation ; transformers
    Source: Springer Online Journal Archives 1860-2000
    Topics: Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition , Process Engineering, Biotechnology, Nutrition Technology
    Notes: Abstract A critical review is given of the degradation of cellulose in the low-temperature region (below about 300°C) of power transformer operation. The large number of kinetic studies, under a variety of environmental conditions from Kraft paper in insulating oil, to cotton and paper in oxygen, are considered in terms of a first-order polymer chain scission model. In many cases, the data are replotted to suit the model. A common activation energy of 111±6 kjmol−1 is calculated and it is shown that the pre-exponential factor, rather than the activation energy, is sensitive to the oxidizing nature of the environment and the susceptibility to degradation of the material. The chemical mechanisms of degradation are reviewed, and conclusions and recommendations are made regarding chemical condition monitoring and life prediction of electrical insulation.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00818797
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  • 16
    Electronic Resource
    Electronic Resource
    Oxidation of carbidic carbon on a rhodium surface (1994)
    Springer
    Catalysis letters 27 (1994), S. 79-90 
    Details
    ISSN: 1572-879X
    Keywords: kinetics ; carbon ; oxygen ; recombination ; rhodium ; surface characterisation ; XPS ; AES
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology
    Notes: Abstract Different mechanisms of atomic carbon and oxygen recombination on a rhodium surface are studied with Auger electron spectroscopy (AES) and X-ray photoelectron spectroscopy (XPS). The kinetics of adsorbed carbidic carbon oxidation (carbon coverageθ c ≈ 0.1–0.3 ML) by gas-phase oxygen that proceeds by a Langmuir-Hinshelwood reaction mechanism, provides the value of the activation energy for recombination (E rec ⇂t ≈ 170±20 kJ/mol).E rec ⇂t depends slightly on the carbon coverage. An Eley-Rideal type of reaction was observed for adsorbed oxygen and atomic gas-phase carbon recombination which occurs in a dynamic regime. The low value found for the activation energy (near zero) is consistent with the mechanism that this exothermic reaction is too fast for energy dissipation into the substrate; the energy is mainly transferred into translational, vibrational and rotational energy of CO.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00806980
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  • 17
    Electronic Resource
    Electronic Resource
    Enthalpies of reaction and reaction rates by flow microcalorimetry: Ester hydrolysis in basic medium (1980)
    Springer
    Journal of solution chemistry 9 (1980), S. 59-73 
    Details
    ISSN: 1572-8927
    Keywords: Enthalpies of reaction ; heats of reaction ; kinetics ; ester hydrolysis ; microcalorimetry
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology
    Notes: Abstract The conditions under which the Picker flow microcalorimeter can be used to measure enthalpies and rates of reactions were investigated. For this purpose, systematic studies were made of the enthalpies of neutralization of HCl, HBr, HNO 3 , acetic, proprionic, and butyric acids with NaOH, enthalpies of hydrolysis of methyl and ethyl acetate with NaOH, and the reaction rates of the ester hydrolysis with NaOH. The general procedure and various sources of error are discussed and it is concluded that enthalpies of slow reactions can be measured to about 1% when the calorimeter is operated in the quasi-isothermal mode and the reaction rates to about 3% when operated in the quasi-adiabatic mode.
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    URL: http://dx.doi.org/10.1007/BF00650137
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  • 18
    Electronic Resource
    Electronic Resource
    Dynamics and self-organization of catalytic systems (1994)
    Springer
    Topics in catalysis 1 (1994), S. 305-314 
    Details
    ISSN: 1572-9028
    Keywords: non-Langmuir ; kinetics ; non-linear dynamics ; oscillations ; chaos ; self-organization
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology
    Notes: Abstract The kinetics of a catalytic reaction is frequently formulated in terms of simple concepts of the Langmuir type. Apart from limitations arising from the non-uniformity of the catalyst's surface and from the coverage dependence of the rate “constants”, several other complications may come into play. These may arise on the “quantum level” where energy flow between the various degrees of freedom may cause failure of simple transition state theory, as well as on the “continuum level” where formulation of rate equations in terms of coupled non-linear differential equations may give rise to a rich scenario of spatio-temporal self-organization, including kinetic oscillations, chaos, and formation of concentration patterns. Several of these phenomena are illustrated by selected examples.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01492284
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  • 19
    Electronic Resource
    Electronic Resource
    The polymerization of sickle hemoglobin in solutions and cells (1993)
    Springer
    Cellular and molecular life sciences 49 (1993), S. 110-117 
    Details
    ISSN: 1420-9071
    Keywords: Polymerization ; sickle hemoglobin ; sickle cell disease ; kinetics ; thermodynamics ; polymer domains ; nucleation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Medicine
    Notes: Abstract The polymerization of sickle hemoglobin occurs by the same mechanisms in solutions and in cells, and involves the formation of 14 stranded fibers from hemoglobin molecules which have assumed a deoxy quaternary structure. The fibers form via two types of highly concentration-dependent nucleation processes: homogeneous nucleation in solutions with hemoglobin activity above a critical activity, and heterogeneous nucleation in similarly supersaturated solutions which also contain hemoglobin polymers. The latter pathway is dominant, and creates polymer arrays called domains. The individual polymers bend, but also cross-link, and the resulting mass behaves as a solid. The concentration of polymerized hemoglobin increases exponentially unless clamped by rate limiting effects such as oxygen delivery.
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    URL: http://dx.doi.org/10.1007/BF01989414
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  • 20
    Electronic Resource
    Electronic Resource
    The influence of sulfur dioxide on propane oxidation activity over supported platinum and palladium (1994)
    Springer
    Catalysis letters 30 (1994), S. 41-51 
    Details
    ISSN: 1572-879X
    Keywords: propane ; oxidation ; platinum ; palladium ; sulfur dioxide ; alumina ; zirconia ; activity ; acidity ; kinetics
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology
    Notes: Abstract Earlier studies have shown that sulfur dioxide and metal-support interaction can strongly influence propane oxidation over platinum. In particular, oxidation activity is enhanced when platinum is supported on sulfated γ-alumina or zirconia compared to γ-alumina. Therefore, it is of interest to compare the performance of palladium under the same experimental conditions. Four model catalysts were examined: Pt/γ-alumina, Pt/zirconia, Pd/γ-alumina and Pd/zirconia. The metal loading was kept at or below 0.05 wt% to emphasize changes in activity attributable to metal-support interaction. Reaction rates were measured with and without sulfur dioxide. Surface sulfation was analyzed by measuring acid strength and evaluating spectra obtained by Fourier-transform infrared spectroscopy. In contrast to platinum, sulfation does not promote propane oxidation on Pd/γ-alumina, and Pd/zirconia is less active than Pd/γ-alumina.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00813671
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  • 21
    Electronic Resource
    Electronic Resource
    Kinetics of the gas-solid heterogeneous photocatalytic oxidation of trichloroethylene by near UV illuminated titanium dioxide (1990)
    Springer
    Catalysis letters 4 (1990), S. 345-354 
    Details
    ISSN: 1572-879X
    Keywords: Ultraviolet heterogeneous photocatalysis ; oxidation ; trichloroethylene ; titania ; kinetics
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology
    Notes: Abstract Kinetics of the gas/solid heterogeneous photocatalytic oxidation of dilute trichloroethylene (TCE) vapors by ultraviolet-illuminated titanium dioxide have been determined using a fixed-bed dynamic photoreactor. Reaction rate dependences on inlet TCE, oxygen and water vapor concentrations were found to consist of both reactant sensitive and insensitive regions. In the reactant sensitive regions, measured limiting apparent reaction rate orders for TCE, oxygen and water vapor are 0.8, 1.7 and — 3, respectively. Water vapor in the reactant stream lowersinitial reaction rates relative to corresponding water free conditions, but is required to sustain photocatalytic activity for extended periods of time.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00765320
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  • 22
    Electronic Resource
    Electronic Resource
    Group theory and experiments on helical and linear distributed feedback gas lasers (1984)
    Springer
    Applied physics 33 (1984), S. 115-131 
    Details
    ISSN: 1432-0649
    Keywords: 02.20 ; 42.55 ; 42.60D
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract This study puts forward the concept of helical distributed feedback (DFB) lasers. The basic features of this new type of laser are derived by group theoretical considerations on cylindrical, circular linear periodic, and helical waveguide and laser structures. It is demonstrated that not only linear periodic structures but also helical structures show Bragg and DFB effects. Microwave and far-infrared experiments on passive helical metal waveguides reveal Bragg resonances in transmission. These results initiated the first experimental realization of a helical DFB gas laser, i.e. an optically pumped 496μm CH3F laser with a helical metal waveguide of a pitch close to 250μm. This helical DFB laser shows higher-mode selectivity than the corresponding linear DFB laser. Finally, we show that the concept of helical DFB also applies to dye lasers with internal DFB incorporated by a mixture of the dye with a cholesteric liquid crystal.
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    Submillimetre laser lines from CH3OH pumped by a13C18O2 pump laser: Observations and assignments (1984)
    Springer
    Applied physics 34 (1984), S. 17-21 
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    Keywords: 42.55
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    Notes: Abstract Twenty-four new optically pumped submillimetre laser lines have been observed when CH3OH is excited using a13C18O2 pump laser. Four of these lines have been assigned to transitions involving the CO stretching band. In addition to these lines, a further six new lines have been observed when pumping with12C18O2 and13C16O2 lasers. One of these lines has been assigned to a transition involving the CO stretching band. The observation of infrared-infrared double resonance signals in CH3OH has allowed the prediction of a further six laser lines which should be excited using a13C18O2 pump laser.
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    Coherent effects in inverse compton scattering in the high frequency region (1984)
    Springer
    Applied physics 34 (1984), S. 221-228 
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    Keywords: 42.55 ; 41
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    Topics: Physics
    Notes: Abstract The conditions under which a cooperative emission from different friges occurs in the scattering between a relativistic electron beam and two interfering laser beams are discussed. In particular, the conditions to have an electron grating are discussed.
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    Bistability and passive Q-switching of a CO2 laser with saturable absorber (1984)
    Springer
    Applied physics 35 (1984), S. 77-82 
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    Keywords: 42.55 ; 42.65
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    Notes: Abstract The coexistence of bistability and repetitive passive Q-switching of a CO2 laser with a gaseous saturable absorber has been investigated experimentally. With CH3F as the saturable absorber bistability has been observed simultaneously with passive Q-switching, whereas with CH3OH either one of these phenomena can only exist, as demonstrated for the first time. The measured features of both systems can be explained qualitatively by rate-equation theory.
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    Optically pumped submillimetre laser action in formaldoxime and ammonia (1984)
    Springer
    Applied physics 35 (1984), S. 127-129 
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    Notes: Abstract Strong submillimetre laser action has been obtained on five lines of a new laser gas, formaldoxime. Several new emission lines have also been produced by isotopic CO2 laser pumping of14NH3 and15NH3. One of these lines at 102.9 μm is a rotation-inversion transition in the 2v 2 state, and is the first example of cw laser action in such a highly excited state.
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    Amplified spontaneous emission in short-pulse excimer amplifiers (1990)
    Springer
    Applied physics 51 (1990), S. 71-74 
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    Keywords: 42.60 ; 42.55
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    Notes: Abstract We have found a simple analytical expression which describes the relation between amplified spontaneous emission (ASE) and small-signal gain in short-pulse amplifiers. It is also shown that the contrast of the short pulse to the ASE is weakly dependent on the saturation of the ASE, and influenced mainly by the saturation of the short pulse. The theoretical considerations were verified by measurements.
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    Stepwise photoionization of complex organic molecules in the gas phase induced by UV laser radiation (1982)
    Springer
    Applied physics 27 (1982), S. 57-61 
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    Keywords: 33 ; 82.50 ; 42.55
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    Notes: Abstract We measured the photoionization cross-sections of anthracene, 1,2-benzanthracene,p-terphenyl, and 2,5-diphenylfuran molecules excited to the singlet and triplet electronic states intermediate in the stepwise two-photon ionization process at 266 nm (all compounds) and at 355, 391 and 417 nm (anthracene).
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    Origin of laser-output noise of cataphoretic HeSe+ lasers (1982)
    Springer
    Applied physics 28 (1982), S. 373-381 
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    Keywords: 42.55 ; 42.80 ; 52
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    Notes: Abstract We investigated noise and fluctuations of the output power of cataphoretic HeSe+ lasers in positive column plasma. Direct coupling of laser output power noise and fluctuations of the local population inversion was found. An investigation of the positive column plasma showed moving striations being responsible for the gain fluctuations. Whereas the local plasma properties are dominated by high frequency striations in the 100 kHz range, integrated quantities such as laser gain per pass are most strongly influenced by low-frequency waves with a continuous noise spectrum below 200 kHz. External modulation of the discharge voltage or current at a frequency near thehf striations reduces laser noise and increases laser output power.
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    Lifetime, photostability, and chemical structure of IR heptamethine cyanine dyes absorbing beyond 1 μm (1982)
    Springer
    Applied physics 29 (1982), S. 15-18 
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    Keywords: 32 ; 42.55
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    Notes: Abstract Optical absorption,S 1 lifetime, and photostability are investigated for a series of heptamethine ir dyes and related to chemical structure. The high photostability of several dyes and the large range ofS 1 lifetimes make these dyes very interesting for ir dye lasers and for ir mode-locked laser systems.
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    Strong far-infrared laser action in carbonyl fluoride and vinyl fluoride (1982)
    Springer
    Applied physics 29 (1982), S. 13-14 
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    Notes: Abstract Intense far-infrared laser action is reported for carbonyl fluoride and vinyl fluoride. Eleven new lines with wavelengths between 339 μm≦λ≦538 μm were obtained by optically pumping carbonyl fluoride with numerous lines of the 10.4 μm band of a cw CO2 laser. Twenty-three lines with wavelengths in the range 172 μm≦λ≦783 μm were detected when pumping the recently discovered efficient FIR laser molecule vinyl fluoride. In addition, three very weak new lines were found using 1.1-difluoroethylen.
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    Temporal analysis of a mode-locked Nd-glass laser by four-wave mixing (1982)
    Springer
    Applied physics 29 (1982), S. 263-267 
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    Keywords: 42.55 ; 42.65 ; 42.80
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    Notes: Abstract The duration, shape, and background intensity level of pulses of a passively modelocked Nd-glass laser are determined by noncollinear phase-matched four-photon frequency mixing of time-separated fundamental and second-harmonic pulses in a KI crystal. The pulse shape is found to be slightly asymmetric with slower trailing than rising parts. The background intensity level before and behind the main pulse is about 5¢10−6 the peak pulse intensity.
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    New FIR laser lines from optically pumped DCOF (1983)
    Springer
    Applied physics 30 (1983), S. 1-4 
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    Keywords: 33 ; 42.55
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    Notes: Abstract Twenty FIR laser lines with wavelengths between 146 and 2000 μm have been observed from deuterated formyl fluoride (DCOF) optically pumped with isotopic CO2 lasers. Tunable diode laser measurements on thev 4 band of DCOF were combined with earlier high precision spectroscopic data on thev 3 andv 4 bands, and enabled identification of the transitions responsible for 9 of the new FIR lines.
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    Theory of synchronously pumped dye lasers (1983)
    Springer
    Applied physics 30 (1983), S. 135-142 
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    Notes: Abstract An analysis of cw synchronously pumped dye lasers is presented. Under the assumption that the cavity (tuning element) bandwidth is much wider than the bandwidth of the transform limited pulses generated, the pulse forming dynamics is rigorously treated. It is shown that for a finite mismatch between the lengths of the dye and the pump lasers, a steady-state pulse develops in the dye laser cavity with a conserved pulseshape. The characteristics (energy, shape, peak power, duration) of these pulses of ultimate width are quantitatively determined as a function of cavity mismatch. An analytical solution for the pulse envelope is determined, which yieldsI(t)∝Sech2(t/t p ) to a good approximation.
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    The effect of added nitrogen on multiphoton absorption by ammonia (1983)
    Springer
    Applied physics 32 (1983), S. 75-78 
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    Notes: Abstract Multiphoton absorption (MPA) of the CO2 laser 9 μmR(30) line (pulse width 60 ns, FWHM) by NH3 and NH3/N2 mixtures was studied as a function of gas composition, pressure and laser fluence (Φ). MPA occurs for Φ smaller than those that have been used for optically pumped NH3/N2 lasers; consequently a simple two-level absorption model will not adequately describe laser action in these systems. The photon energy deposited in NH3/N2 mixtures can be calculated from the MPA cross-section and the fluence dependence of the illumination geometry. An examination of the efficiency of conversion of this absorbed energy to the reported radiant energy of optically pumped NH3/N2 lasers shows an optimum value which depends on pressure, and gas composition.
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    Power enhancement of the cw 12.08 μm NH3 Raman laser with the addition of H2/He buffer gases (1983)
    Springer
    Applied physics 32 (1983), S. 105-111 
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    Notes: Abstract The effects of H2, He, and N2 buffer gases on the efficiency of the cw 12.08 μm NH3 Raman laser are studied experimentally. The laser output power is increased by nearly 60% with the addition of H2 or He, which we essentially attribute to the high thermal conductivity of these buffer gases. In the optimum conditions (NH3/H2:1/1 mixture with 0.35 Torr partial pressure of NH3) 3.3 W output power at 12.08 μm is obtained which corresponds to 11% power conversion efficiency.
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    A cw uv copper hollow cathode laser in the 260 nm region (1983)
    Springer
    Applied physics 32 (1983), S. 127-135 
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    Keywords: 42.55 ; 42.60
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    Notes: Abstract A cw uv copper hollow cathode laser is described, which could be operated for a longer time duration with an output power of 7 mW in the 260 nm region. A double-cathode configuration with a protection for the mirrors from metal-vapour deposition is presented. Characteristics of the laser output power, the spontaneous emission, and the ion densities in the negative glow were measured as depending on the discharge current, the neon gas pressure, and the size of the cathode slit. The observed saturation of the laser output power at high discharge current (1 A/cm2) and the optimum slot size are discussed.
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    CW and pulsed FIR-CO2 hybrid laser with improved efficiency and amplitude stability at short FIR wavelengths (1984)
    Springer
    Applied physics 33 (1984), S. 23-27 
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    Notes: Abstract For the first time stable cw output of a FIR-CO2 hybrid laser has been achieved at wavelengths shorter than 300 μm. Due to the saturable absorber characteristic of the FIR laser gas, cw or pulsed emission is observed on both, the CO2 and the FIR laser output, depending on the operating conditions. Results are reported on different resonant lines in CH3OH and the 67 μm Raman line in NH3. The good efficiency of this laser is also demonstrated by the excitation of two new emission lines in CH3OH, namely 49 and 56 μm, pumped by 9R(22) and 9R(24), respectively.
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    The effect of triplet quenchers on vapor-phase dye-laser performance (1984)
    Springer
    Applied physics 34 (1984), S. 83-86 
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    Keywords: 33.50 ; 34.50 ; 42.55
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    Notes: Abstract An XeF pumped vapor phase POPOP dye laser with a pulse duration of 300 ns was obtained when trans-stilbene was used as triplet quencher. An energy conversion efficiency of 7,5% with a peak power efficiency of 12% was measured.
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    New cw fir laser emissions from CO2 laser-pumped vinyl bromide (1984)
    Springer
    Applied physics 34 (1984), S. 175-177 
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    Notes: Abstract 47 new cw far-infrared laser lines with wavelenths between 453 and 2356 μm have been obtained by optically pumping vinyl bromide (C2H3Br) by a CO2 laser. A significant portion of these lines has wavelengths longer than 750 μm.
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    Small-signal gain of Free Electron Laser in a resonator Gaussian mode (1984)
    Springer
    Applied physics 35 (1984), S. 163-166 
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    Notes: Abstract We present an analytical expression for the small-signal gain of a Free Electron Laser (FEL) in the presence of a Gaussian mode. To describe the electron beam evolution we use the one-dimensional (1-d) Vlasov equation. Our perturbation result, valid for small values of the parameterq (length of the undulatorL divided by the Rayleigh rangeZ R), can be extrapolated to values ofq≈4÷5.
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    611.8 nm single-mode He-Ne laser (1990)
    Springer
    Applied physics 51 (1990), S. 292-294 
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    Notes: Abstract The conditions for optimum 611.8 nm laser operation are obtained and a convenient method for indicating 3.39 µm suppression is proposed. Single longitudinal mode 611.8 nm generation is obtained using higher gas-mixture pressure and application of an axial magnetic field. Several milliwatt monomode output power and 0.75 multimode-to-monomode power conversion coefficients are obtained without an internal iodine cell. A comparison of the experimental results with a single-mode laser theory is given.
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    Performance of internal-mirror frequency-stabilized He-Ne lasers emitting green, yellow or orange light (1990)
    Springer
    Applied physics 51 (1990), S. 421-426 
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    Notes: Abstract A comprehensive control system has been developed for the stabilization of internalmirror He-Ne lasers to their power envelopes. It is designed particularly for use with lasers emitting at 552, 505, or 490 THz (543, 594, 612 nm). The aim has been to combine convenience in routine operation with good day-to-day resettability and minimal frequency drift during a day. The lasers are observed to emit in up to four modes simultaneously and their tuning behaviour is highly alignment-sensitive. They also tend to flip between modes having orthogonal linear planes of polarization. Reliable control of polarization and mode frequency are possible using permanent magnets and active length control through thermal expansion. The stabilized single-frequency outputs have frequency drifts of about 2×10−8 per year, and powers of between 150 μW and 850 μW.
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    Output and picosecond amplification characteristics of an efficient and high-power discharge excimer laser (1991)
    Springer
    Applied physics 52 (1991), S. 1-7 
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    Notes: Abstract Improvements in output pulse energy and efficiency of a conventional capacitor-transfer-type discharge excimer laser with automatic preionization have been achieved by extending the discharge volume and resulting moderate pumping of the active medium. The discharge laser produces a pulse energy of more than 1 J for XeCl, KrF, and ArF lasers in square beams of about 2×2 cm2, and the maximum overall efficiency observed is 2.9% for XeCl, 3.2% for KrF and 1.8% for ArF. The laser device has been involved in a picosecond (∼ 32 ps) XeCl laser amplification system, and was operated as an amplifier at a repetitive frequency of 10 Hz. Saturation fluence for XeCl laser was measured to be 1.4 mJ/cm2, and the picosecond pulse energy of ∼40 mJ was extracted from the amplifier.
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    Investigation of vibrational relaxation of excimers (1991)
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    Applied physics 52 (1991), S. 22-26 
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    Notes: Abstract The excimer vibtational relaxation have been studied in the diffusional approximation, and stationary substantially non-equilibrium populations of high vibrational levels have been found. New formulae have been derived for quantum yield of UV lasing. Taking into account the vibrational relaxation the new effect of far-IR radiation amplification in the active media of excimer lasers is predicted.
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    New far infrared laser lines from 13CH2F2 and frequency measurements (1991)
    Springer
    Applied physics 52 (1991), S. 32-35 
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    Notes: Abstract We report new FIR laser lines from 13CH2F2 molecules optically pumped by a waveguide CO2 laser. The increased tunability (300 MHz) with respect to a conventional CO2 laser allows the pumping of 13CH2F2 vibrational transitions of large offset. 34 new laser lines have been discovered, ranging from 113.1 μm to 491.4 μm in wavelength, thus increasing the number of known FIR laser lines from this important molecule to 99. For all the new lines and many (36) of those known previously, precise offset measurements through the transferred Lamb-dip technique were performed. The frequency of six new laser lines was also directly measured by heterodyne detection with known laser lines.
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    New FIR laser lines from CD3OD optically pumped by a CO2 waveguide laser (1991)
    Springer
    Applied physics 52 (1991), S. 36-41 
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    Notes: Abstract In this work we report new FIR laser lines from CD3OD optically pumped by a CO2 waveguide laser. The wide tunability of this laser (290 MHz) makes it possible to pump absorption lines with large frequency offset relative to the CO2 laser line center, which are not possible by using conventional CO2 lasers. As a consequence 19 new laser lines have been discovered, ranging from 38.0 μm to 455.2 μm in wavelength. For all lines, precise frequency offset measurements between the CO2 line center and the center of the absorber CD3OD line were performed using the transferred Lamb-dip technique. We also present direct Doppler-free offset measurements of infrared absorption, obtained within the FIR laser cavity itself, using optoacoustic detection.
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    Nonlinear mirror based on raman interactions (1991)
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    Applied physics 52 (1991), S. 96-101 
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    Notes: Abstract We analyze a nonlinear mirror based on Raman interactions. The mirror is a combination of a Raman-active medium and a tetrachroic mirror. The reflections of the nonlinear mirror at two input frequencies differing by the Raman shift are calculated and its properties and possible applications are discussed.
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    Negative feedback using a nonlinear mirror for the generation of a long train of short light pulses (1991)
    Springer
    Applied physics 52 (1991), S. 158-162 
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    Notes: Abstract A nonlinear mirror is used to provide a passive negative feedback in an actively mode-locked pulsed Nd:YAG laser. Trains of 250 ps pulses with a total length of up to 50 microseconds were generated. The train duration is limited only by the flashlamp pump pulse length.
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    Diagnostics of a Compact Discharge-Pumped XeCl Laser with BCl3 Halogen Donor (1991)
    Springer
    Applied physics 52 (1991), S. 234-243 
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    Keywords: 42.55 ; 52.65 ; 52.80
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    Notes: Abstract The results of a comprehensive study of a compact UV-preionized XeCl laser are presented. The subjects of this study were: discharge voltage and current measurements, dye laser probing of the active medium, and the mass spectrometry of gas mixture degradation products. It is shown that the gas lifetime was significantly improved when the laser was operated with BCl3 as a halogen donor instead of commonly used HCl. By the dye laser absorption and gain probing, the temporal and spatial dependences of the densities for several plasma components, Ne*, Xe*, Xe+*, Cl−, XeCl* and of ground state boron atoms were measured. Some aspects of plasma kinetics for uniform and constricted phases of the discharge are discussed. By the mass spectrometry of gas mixture degradation products on long-term operation of the laser device several gaseous (N2, O2, CO2, H2O, C2H4) and solid (NiCl2, H3BO3) products were detected in the laser chamber. NH4Cl was determined to be a stable fraction of the deposits on optics surfaces. The reasons for the improvement of gas lifetime for BCl3-containing gas mixtures are discussed.
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    Simultaneous oscillation on UV and IR transitions of the copper ion laser (1991)
    Springer
    Applied physics 52 (1991), S. 323-325 
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    ISSN: 1432-0649
    Keywords: 42.55 ; 52.25
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract Simultaneous oscillation of UV (248–270 nm) and IR lines (773–785 nm) in the copper ion laser with helical hollow cathode has been observed using high reflectivity combination mirrors. The output power characteristics of these laser lines are measured as functions of the discharge current and fill-gas pressure. A total laser power of about 100 mW with equal UV and IR contributions was obtained.
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    Infrared recombination lasers pumped by low energy Nd: YAG and excimer lasers (1992)
    Springer
    Applied physics 54 (1992), S. 234-238 
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    Keywords: 42.55 ; 42.60B ; 52.50J
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    Topics: Physics
    Notes: Abstract 24 infrared laser lines on atomic and ionic transitions have been observed in recombining plasmas by vaporizing and ionizing Cd, Pb, Sn, Zn, and Mg with low energy Nd:YAG or excimer pump-lasers. For operation and optimization of the recombination lasers separated plasma spots and a plasma confinement have been used. The operation of shorter wavelength systems by isoelectronic scaling is discussed.
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    Elimination of variables in simple laser equations (1992)
    Springer
    Applied physics 55 (1992), S. 117-120 
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    Keywords: 42.55 ; 42.65 ; 02
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    Notes: Abstract The usual way of obtaining rate equations (RE) and a single equation for the field amplitude (EFA) from the semiclassical laser equations (Lorenz-Haken model) is reexamined by undertaking a systematic elimination procedure developed in synergetics. The RE and EFA are justified in the case 1 (γ⊥≫γ∥, κ) and case 2 (γ⊥, γ∥≫κ), respectively. We show that, because the eliminated variable happens to contain a considerable contribution from an unstable mode, the usual elimination technique in the case 3 (γ⊥, κγ∥) leads to an inconsistency. As important by-products we obtain the RE and EFA for arbitrary cavity relaxation constant (κ). Some remarks are given on the direct elimination technique in the non-diagonal representation in the study of instabilities.
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    Polarization and power characteristics of pulsed dye lasers with transverse pumping (1992)
    Springer
    Applied physics 55 (1992), S. 494-500 
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    Topics: Physics
    Notes: Abstract Starting from the classical theory on molecular luminescence in liquids, rate equation for two-polarization-mode laser oscillation under transverse pumping with intense excitation have been set forth neglecting the influence of orientational relaxation of the dye molecules. Hence, the laser output power and polarization under different configurations have been obtained. The results show that the dye laser is partially polarized even when the pump beam is unpolarized and no polarizing elements exist in the cavity. If we define a reference plane consisting of the axes of the pump beam and the dye laser, the laser system has to adopt the plane perpendicular to the reference plane as the polarization direction in order to yield a highly efficient, linearly polarized laser output. Experiments on a copper-vapor laser pumped dye laser verified these analytical results.
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    Simultaneous detection of atomic and molecular hydrogen using a tunable ArF excimer laser (1993)
    Springer
    Applied physics 56 (1993), S. 229-234 
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    Keywords: 42.55
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    Topics: Physics
    Notes: Abstract We report preliminary experiments which demonstrate the simultaneous detection of both atomic and molecular hydrogen using a single tunable ArF laser. The tunable ArF laser was modified to lase simultaneously at two wavelengths by the addition of a second grating to the oscillator stage as in earlier work by Ketterle et al. for KrF operation. To our knowledge, this is the first demonstration of dual-wavelength capability with a tunable ArF excimer. The H atom diagnostic utilized tunable ArF excimer laser output at 193.29 nm which was Raman shifted in D2 (first Stokes) to generate 205.14 nm radiation which then excited the H atom to its (3s, 3d) states via a two-photon transition. Fluorescence was detected at 656 nm on the (3s, 3d) → 2p transition. The second wavelength from the tunable excimer was used to excite several rovibronic LIF transitions of hydrogen molecule via two-photon absorption on the E 1Σ g + ⇐ X 1Σ g + (2,0) band. Fluorescence occurs at 750 nm and 830 nm on the (E 1Σ g + ⇒ B 1Σ g + ) transitions.
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    Nonlinear behaviour of atomic fluorescence in mercury vapours following double-resonance laser excitation (1994)
    Springer
    Applied physics 58 (1994), S. 303-307 
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    Keywords: 32.00 ; 42.55 ; 42.65
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    Topics: Physics
    Notes: Abstract When mercury atoms, present with a buffer gas (N2 or Ar) in a quartz cell or in a graphite furnace are excited into the 73 S 1 level by means of two pulsed dye lasers tuned at 253.652 nm (61 S o → 63 P 1) and 435.835 nm (63 P 1 → 73 S 1), a laser-like, collimated emission is observed along the axis of the cell at the green mercury line (73 S 1 → 63 P 2), 546.074 nm). This radiation exhibits a pronounced non-linear dependence upon the number density of the mercury atoms in the cell. This behaviour is interpreted as being due to amplified spontaneous emission (ASE), which occurs as a result of the transient population inversion between the 7s 3 S 1 and 6p 3 P 2 o levels. The parameters governing the population inversion can be deduced by applying a rate equation analysis to the atomic system. A time-resolved observation of both ASE and spontaneous fluorescence signals confirms the totally different characteristics of the two emission processes.
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    Orange, red and deep-red flashlamp-pumped Pr3+:LiYF4 laser with improved output energy and efficiency (1994)
    Springer
    Applied physics 58 (1994), S. 421-424 
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    ISSN: 1432-0649
    Keywords: 42.60.Lh ; 42.55 ; 42.70
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    Topics: Physics
    Notes: Abstract Three laser transitions (607.2 nm, 639.5 nm, 720.9 nm) in a flashlamp-pumped Pr3+:LiYF4 laser at room temperature are investigated. Cerium ions (Ce3+) doped into the fused-quartz envelope of the flashlamp efficiently transfer strong UV radiation from pumping light into the absorption region of Pr3+ ions (λ = 420−480 nm), so that the slope efficiency of all three laser emissions could be increased by almost 100% compared to excitation with a pure quartz flashlamp. At a pump energy of 30 J the output energy of these three laser emissions reached 4.7 mJ, 87 mJ and 30 mJ.
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    A magnetically stabilized coaxial laser discharge (1981)
    Springer
    Applied physics 26 (1981), S. 161-167 
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    Keywords: 52.80 ; 42.55
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    Notes: Abstract A new magnetic discharge stabilization technique for coaxial laser systems is described. The approach utilizes crosses electric and magnetic fields to create and maintain a large and rapidly rotating plasma volume which does not experience glow-to-arc transitions. Very high cw specific discharge power loadings have been achieved even without the benefit of external gas cooling or circulation. Performance is insensitive to gas composition and pressure such that high power coaxial discharges have been run in CO2 laser gas mixtures up to several hundred torr. Stable cw discharges have also been obtained in mixtures containing several torr of SF6. The technique appears to be readily scalable to give very large excited volumes in systems with comparatively small overall physical dimensions.
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    Population inversion in thallium by flashlamp-photodissociation of TII (1983)
    Springer
    Applied physics 32 (1983), S. 83-84 
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    Keywords: 42.55 ; 33.80
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    Notes: Abstract A population inversion between the 62 P 3/2 and 62 P 1/2 state of thallium has been achieved for the first time by incoherent photodissociation of TII. This is accomplished by using wall-ablating flashlamps of short risetime and appropriate light filtering. The inversion lasts about 4 μs and is terminated by quenching collisions.
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    The vibrational relaxation time constant for theB v=0 level of XeCl (1983)
    Springer
    Applied physics 32 (1983), S. 193-198 
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    Keywords: 42.55 ; 33 ; 82.50
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    Topics: Physics
    Notes: Abstract The vibrational relaxation time constant for theB v=0 vibrational level of XeCl* has been investigated by observing the coupling between theB v=1 andB v=0 vibrational levels under saturated lasing conditions. Based on this observation, estimates of the expected extraction efficiency from theB-state have been made.
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    Transverse mode dynamics in a free-electron laser (1984)
    Springer
    Applied physics 33 (1984), S. 9-16 
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    Keywords: 42.60 ; 42.20 ; 42.55
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    Notes: Abstract We derive the most general equations of motion for the electrons and the electromagnetic field in a free-electron laser including the effects of diffraction and pulse propagation. The field evolution is expressed in terms of the amplitudes and phases of a complete set of transverse modes. The analytic solution is given in the small-signal regime, where the theory is shown to be in excellent agreement with a recent experiment at Orsay.
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    Pressure dependence of laser oscillation and superfluorescent emission from an optically pumped CF4 laser (1984)
    Springer
    Applied physics 34 (1984), S. 37-41 
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    Keywords: 42.55
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    Topics: Physics
    Notes: Abstract Experiments on pressure dependence of a CF4 laser have been carried out to elucidate dynamic characteristics of CF4 molecules pumped by CO2 lasers. The results are followed by a model calculation which characterizes collisional quenching of the energy levels related to the stimulated emission. The enhancement of the laser output induced by buffer-gas addition, which was found under specific conditions, is discussed in relation to the competition between laser and superfluorescent emissions.
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    Long wavelength operation of a CW CO-laser up to 8.18 μm (1981)
    Springer
    Applied physics 26 (1981), S. 73-76 
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    Keywords: 07 ; 42.55
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    Topics: Physics
    Notes: Abstract A liquid nitrogen cooled cw CO-Laser is described, with which laser action up to 8.18 μm (v=36→35) has been achieved.
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    Design criteria and operating characteristics of a single-mode pulsed dye laser (1981)
    Springer
    Applied physics 26 (1981), S. 141-146 
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    Notes: Abstract We have designed and tested a pulsed single-mode dye laser for spectroscopy experiments. The dye laser is pumped by a 6 kHz copper vapor laser to produce up to 230 mW average power at over 5% efficiency in a nearly diffraction limited beam. The dye laser pulse closely resembles the 30 ns pump pulse. Using an electronic servo loop, the 60 MHz wide line can be scanned, without mode hopping, through the 16 GHz permitted by the travel on the piezo driven mirror mount.
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    Free electron laser (1982)
    Springer
    Applied physics 28 (1982), S. 150-154 
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    Keywords: 42.55
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    Further study of continuous-wave CO flame chemical laser of the CS2/O2/N2O type (1983)
    Springer
    Applied physics 30 (1983), S. 29-33 
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    Keywords: 42.55 ; 42.60
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    Topics: Physics
    Notes: Abstract This report describes an experimental examination of the output characteristics of the continuous-wave (cw) carbon monoxide flame chemical laser (FCL) of the CS2/O2/N2O type in case of small CS2/O2 reactants ratios (tipically CS2/O2≦1/10). A linear burner which gives a homogeneous and stable flame was used during the experimental study. The measurements of temperature distribution in CS2/O2 as well as CS2/O2/N2O flames show maximum temperatures of 1040 and 890 K, respectively. The addition of nitrous oxide (N2O) leads to dramatically enhanced output laser power caused primarily by V−V transfer processes. A chemical efficiency, based on the reaction O+CS→CO*+S, of 3% was achieved. The spectral composition of the CO FCL of the CS2/O2/N2O type shows lasing in the region from 5.130 to 5.586 μm. Experimental results were obtained with a nondispersive optical cavity.
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    FIR NH3 cascade laser excited by a Q-switch laser (1983)
    Springer
    Applied physics 31 (1983), S. 5-8 
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    Keywords: 42.55
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    Notes: Abstract Short FIR laser pulses of high repetition rate are obtained by pumping NH3 with the pulses of a passively Q-switched IR laser. The two cascade laser transitions observed show coupled relaxation oscillations. The pulse shapes and delay times are qualitatively in agreement with a four-level rate-equation model.
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    Surface spectroscopy (1982)
    Springer
    Applied physics 28 (1982), S. 229-232 
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    Keywords: 82.65 ; 68 ; 36.40 ; 78 ; 42.55
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    Guided waves and IR lasers (1982)
    Springer
    Applied physics 28 (1982), S. 283-289 
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    Keywords: 85.60 ; 42.80 ; 42.55 ; 33
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    Intense laser generation from an atomic-fluorine laser (1984)
    Springer
    Applied physics 33 (1984), S. 235-238 
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    Notes: Abstract An intensive generation of radiation from a discharge-pumped atomic-fluorine gas laser is reported. A peak power exceeding 330 kW and a total energy of more than 2 mJ is obtained for a number of lines in the red, using a NF3∶He (1∶100) gas mixture at total pressure of 500 Torr. The circuitry optimization is described and the conditions for effective operation of the atomic-fluorine laser are discussed. The temporal and the spectral characteristics of the laser emission are also presented.
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    Free electron laser (1982)
    Springer
    Applied physics 29 (1982), S. 157-158 
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    Keywords: 42.60 ; 42.55
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    New lasers and laser schemes (1982)
    Springer
    Applied physics 29 (1982), S. 143-148 
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    Keywords: 42.60 ; 42.55
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    Notes: Conclusion We have demonstrated the existence of an anomalous polarization coupling mechanism present in the injection locked TEA CO2 laser. As a direct consequence of this work, a new injection technique has been formulated which permits efficient injection coupling and maximises energy extraction whilst eliminating the detrimental optical feedback effects to which other injection locking systems are prone.
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    Energy transfer in slab dye lasers (1984)
    Springer
    Applied physics 35 (1984), S. 71-75 
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    Keywords: 42.60 ; 42.55 ; 42.72
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    Topics: Physics
    Notes: Abstract A simple model of the energy transfer between a booster dye and the active dye in a flashlamp pumped planar waveguide dye laser is described. Analytical results are compared with experiments for several dyes in the 600–650 nm region. A twofold increase of laser output was found at a wavelength (630 nm) which is of particular interest for several applications.
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    Self-phase locking in lasers with homogeneously broadened emission lines (1984)
    Springer
    Applied physics 33 (1984), S. 187-193 
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    Keywords: 42.50 ; 42.55 ; 42.60
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    Notes: Abstract It is shown by numerical analysis based on Lamb's equations of motion, that standing-wave lasers with purely homogeneously broadened emission lines exhibit regular multimode oscillations. Specifically, modes lying far from the line centre are quenched due to mode competition, and the amplitudes of the oscillating modes approach steady-state values. The stabilization of the amplitudes is normally accompanied, or followed, by an evolution of the phases towards a phase-locked regime, where the relative phasesψ n = 2φ n −φ n + 1 −φ n − 1 [φ n phase in then th mode, defined by (6)] attain either the value 0 or ± π. The build-up times for the relative phases are found to vary over a wide range.
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    Improved gain on the Cl2(D′3 П g −A′3 П u ) transition at 258 nm by halogen donor mixing (1984)
    Springer
    Applied physics 35 (1984), S. 11-15 
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    Keywords: 42.55
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    Notes: Abstract The temporal development of the small-signal gain on the Cl2(D′−A′) transition at 258 nm has been investigated by means of an amplified spontaneous emission (ASE) technique. For electron beam pumped He/Cl2 mixtures, the gain appears only at the end of the pumping pulse, whereas for He/Cl2/CCl4 mixtures the temporal gain profile coincides with the fluorescence pulse, and the maximum gain coefficient increases by about a factor of two. The observed effects are due to the mixing of both halogen donors and can be explained by considering the quenching of theD′-state by electrons.
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    Theory of the synchronously pumped picosecond dye laser (1982)
    Springer
    Applied physics 27 (1982), S. 27-37 
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    Keywords: 42.55 ; 42.60
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    Notes: Abstract The circulation of a synchronously mode locked dye laser pulse in a linear cavity configuration containing a dye cell as an active medium and a bandwidth-limiting element is treated. The condition that the pulse shape reproduces after each cavity round-trip provides a nonlinear integro-differential equation for the steady-state pulse shape. For the solution of this equation an approximate method, not limited to small pulse energies, is given and the pulse duration, intensity, energy, asymmetry of the pulse shape, stable regions and other interesting parameters are discussed.
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    The He/Cl2 laser at 258 nm (1982)
    Springer
    Applied physics 27 (1982), S. 49-55 
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    Keywords: 42.55 ; 34 ; 33
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    Notes: Abstract Lasing from e-beam pumped He/Cl2 mixtures at 258 nm was investigated in a longitudinal pumping geometry. Time dependence, output powers and energies as well as the spectral composition of the laser pulses were determined for different experimental conditions. Optical gain was observed for eight transitions around 258 nm. The fine structure results from isotopic splitting and contributions from different vibrational states. No bottle-necking occurs. However, saturation and absorption by excited states limited the total output power to 6MW and the output energies to 200 mJ. A simple kinetic model is proposed that reproduces the larger number of experimental data quite sufficiently.
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    A one joule, XeCl pumped dye laser (1981)
    Springer
    Applied physics 26 (1981), S. 31-32 
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    Notes: Abstract A 4 J XeCl (308 nm) laser has been used to produce ∼ 1 J of dye laser output from selected dyes whose lasing wavelengths sample the spectral range from 330 to 600 nm.
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    Resonant pumping far-infrared NH3 laser (1981)
    Springer
    Applied physics 26 (1981), S. 33-36 
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    Keywords: 42.55 ; 33 ; 34
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    Notes: Abstract A far-infrared (FIR) NH3 laser was resonantly pumped with a line-tunable infrared (IR) NH3 laser. The number of the observed FIR laser lines amounted to 33. Most of them belonged toaR(J,K) rotation-inversion transition in (0, 1, 0, 0) vibrational state. The line tunability of sealed-off FIR NH3 laser was almost achieved in 90, 115, 150, and 220 μm wavelength regions by the selective line tuning of the pumping IR NH3 laser.
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    Ultra-violet excited laser emission in Na2 (1982)
    Springer
    Applied physics 29 (1982), S. 195-200 
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    Keywords: 42.55 ; 35
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    Notes: Abstract Laser emission at different wavelengths in the range of 903–914 nm and around 2.5 μm has been observed upon excitation of Na2 by uv radiation from an excimer laser at 351 nm and an excimer pumped dye laser in this wavelength range. The emission is attributed to a cascade emission $$C^1 \Pi _u \to 2^1 \sum _g^ + $$ followed by $$2^1 \sum _g^ + \to A^1 \sum _u^ + $$ . In addition, coupled with the laser emission around 910 nm, broad-band fluorescence peaking around 855.5 nm is observed which, eventually, may be the first observation of the $$b^3 \sum _g^ + \to x^3 \sum _u^ + $$ bound-free transition in Na2.
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    Theory of passively mode-locked cw dye lasers (1982)
    Springer
    Applied physics 27 (1982), S. 105-113 
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    ISSN: 1432-0649
    Keywords: 42.55 ; 42.60
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The circulation of an ultrashort light pulse in a continuously pumped modelocked dye laser with a linear cavity configuration containing the active dye, the saturable absorber and a bandwidth-limiting elements is treated. The steady-state condition that the pulse shape reproduces after each cavity round-trip leads to a nonlinear integro-differential equation for this pulse shape. An approximate method for the solution of this equation not limited to the case of low laser gain and small pulse energies is given. The stable single pulse region and characteristic pulse parameters, as energy, duration, intensity and asymmetry, are considered in dependence on the laser parameters.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00697557
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    On the theory of electron motion due to superposed em waves and its application to the free-electron laser with linear polarization (1982)
    Springer
    Applied physics 28 (1982), S. 15-20 
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    ISSN: 1432-0649
    Keywords: 42.55 ; 41
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The relativistic motion of a charged particle in an electromagnetic field depending only on one coordinate is shown to be exactly equivalent to the unidimensional motion of a particle having a time and space-varying mass. By means of the averaged Lagrangian method an approximate solution is obtained for the relativistic electron motion in two oppositely moving waves of any polarization, one of them being weaker than the other one, thus generalizing the results previously obtained for circular polarization. A comparison with numerical calculations shows a good agreement. A pendulum-like motion in an effective periodic potential is shown to exist not only for two waves of the same frequency, but more generally when the frequency of the weaker wave is an odd harmonic of the frequency of the stronger one.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00693886
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  • 83
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    A subpicosecond dye laser pumped by a xenon ion laser (1984)
    Springer
    Applied physics 34 (1984), S. 191-192 
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    ISSN: 1432-0649
    Keywords: 42.55 ; 42.60
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract A pulsed xenon ion laser has been used to pump a rhodamine 6G dye laser utilizing a ring resonator. The dye laser has been passively mode-locked; a pulsewidth of 0.5 ps and a 50 kW peak power have been obtained.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00697634
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  • 84
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    Novel quantum-electronics phenomena and devices (1982)
    Springer
    Applied physics 29 (1982), S. 152-156 
    Details
    ISSN: 1432-0649
    Keywords: 42.80 ; 42.55
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00688656
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  • 85
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    Theory of active-passive mode-locking of solid-state lasers using a nonlinear mirror (1990)
    Springer
    Applied physics 50 (1990), S. 409-413 
    Details
    ISSN: 1432-0649
    Keywords: 42.65 ; 42.55
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The theory of active-passive mode-locked solid-state lasers is developed where the passive mode-locking is achieved by a nonlinear mirror. Steady-state cw numerical solutions are analyzed in detail for the case of a Nd: YAG laser. The steady-state pulse duration can be reduced by an order of magnitude as compared to the pure active mode-locking regime.
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    URL: http://dx.doi.org/10.1007/BF00325094
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  • 86
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    Optimization of the UV CuII laser (1981)
    Springer
    Applied physics 26 (1981), S. 49-56 
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    ISSN: 1432-0649
    Keywords: 42.55 ; 52.80
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The cw output power of the uv CuII laser has been optimized with respect to the hollow cathode geometry, the discharge current, the fill gas pressure and the resonator mirror parameters. A maximum laser output power of 900 mW for multiline operation at 248.6, 259.1, 260.0, and 270.3 nm was achieved with 100 A discharge current, 260 V voltage and 16 mbar fillgas pressure, when a hollow cathode of 1.2 m length and 2×6 mm2 cross section was employed. The single-pass pain gl has been estimated to 7%. A hollow cathode cross section of 1.5×4.5 mm2 is suggested as an optimum geometry. In addition, some investigations on the mechanism of the laser power decay in Ne−Cu-discharges are presented.
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    URL: http://dx.doi.org/10.1007/BF00702687
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  • 87
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    Single picosecond-pulse generation in a mode-locked oscillator and regenerative amplifier system (1981)
    Springer
    Applied physics 26 (1981), S. 239-242 
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    ISSN: 1432-0649
    Keywords: 42.55
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract A mode-locked Nd-glass laser oscillator with intra-cavity pulse selection by a Pockels cell shutter is described. A regenerative amplifier system with a saturable absorber is used to shorten the selected light pulses from the master oscillator. Pulses were shortened from 8 ps to 1 ps.
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    URL: http://dx.doi.org/10.1007/BF00692544
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  • 88
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    Electron dynamics in free electron laser resonator modes (1982)
    Springer
    Applied physics 29 (1982), S. 101-109 
    Details
    ISSN: 1432-0649
    Keywords: 42.50 ; 42.55 ; 52.60
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract We study the electron phase-space evolution and gain in free electron lasers whose short-wavelength radiation has Gaussian spherial wavefronts. Several free electron laser designs are considered: the undulator, the tapered wavelength undulator, and the optical klystron. We find that the gain spectrum is no longer proportional to the slope of the forward spontaneous emission spectrum, and we determine the design of the Gaussian mode which maximizes the energy extraction from the electron beam.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00692771
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  • 89
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    Detection of atomic oxygen in flames by absorption spectroscopy (1994)
    Springer
    Applied physics 59 (1994), S. 543-546 
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    ISSN: 1432-0649
    Keywords: 32.20 ; 42.55 ; 82.80
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The absolute concentration of atomic oxygen in an atmospheric pressure hydrogen/air flame has been measured using Intracavity Laser Spectroscopy (ICLS) based on a dye laser pumped by an argon-ion laser. Absorptions at the highly forbidden transitions at 630.030 nm and 636.380 nm were observed at an equivalent optical length of up to 10 km. The relatively low intensity of the dye laser avoids photochemical interferences that are inherent to some other methods for detecting atomic oxygen. The detection sensitivity is about 6 × 1014 atom/cm3 and can be improved with better flame and laser stabilization.
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    URL: http://dx.doi.org/10.1007/BF01082398
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  • 90
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    IR and FIR spectroscopy of 13CD3OH around the 10P(22) and 10P(24) CO2 laser lines: New FIR laser emissions, frequency measurements and assignments (1992)
    Springer
    Applied physics 54 (1992), S. 24-28 
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    ISSN: 1432-0649
    Keywords: 42.55
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract By using high resolution infrared Fourier transform data on 13CD3OH and the 10P(22) and 10P(24) lines of a waveguide CO2 laser to optically pump this methanol isotope, eight new FIR laser lines were observed. The frequencies of five laser lines were directly measured by heterodyne detection with already known laser lines. Particularly interesting are the lines pumped by the 10P(24) line, since a triade of emissions could be completely assigned.
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    URL: http://dx.doi.org/10.1007/BF00331730
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  • 91
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    Repetitive passive Q-switching and bistability in lasers with saturable absorbers (1983)
    Springer
    Applied physics 30 (1983), S. 57-77 
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    ISSN: 1432-0649
    Keywords: 42.55 ; 42.65
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract We report detailed experimental data on the passive Q-switching operation in a CO2 laser with CH3I saturable absorber, and on the transient behaviour in the near-Q-switching situation. Under suitable operating conditions, we found bistability in the output power. In some cases, we observed the simultaneous presence of bistability and passive Q-switching. The theoretical part of the paper starts from the four-level model of laser with saturable absorber, as formulated by other authors. By adiabatically eliminating the variables of the resonant levels, we reduce the problem to a set of three differential equations, from which we derive explicit analytical conditions for the rise of passive Q-switching. These conditions turn out to be in good qualitative and partially quantitative agreement with our experimental findings as well as with other experimental data previously obtained by other authors. Finally we classify the possible combinations of passive Q-switching and bistability that one can find in this type of experiments.
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    URL: http://dx.doi.org/10.1007/BF00688479
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  • 92
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    Dye stability under excimer-laser pumping (1983)
    Springer
    Applied physics 30 (1983), S. 109-116 
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    ISSN: 1432-0649
    Keywords: 33 ; 42.55
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The stability of polymethine dyes under XeCl laser excitation has been investigated. (For these dyes emitting in the ir the difference between absorbed and emitted photoenergy is 2 eV.) The stability was measured in an amplifier device operating in the saturated regime. While the influence on dye concentration is negligible, the fluence dependence shows the importance of two photon absorptions. A meausure for the stability is the number of photons which can be emitted per dye molecule before the dye solution has degraded to 50% of the initial value. This value is in the range of 150–280. The stability is clearly related to the formation of photoproducts absorbing at the pump and the laser wavelength. A model starting from the change in the dye solution absorption spectra is in very good agreement with the observed energy decays.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00695464
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  • 93
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    Optimum gain length for pulsed dye laser amplifiers (1990)
    Springer
    Applied physics 50 (1990), S. 133-136 
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    ISSN: 1432-0649
    Keywords: 42.55 ; 42.60d
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract It is shown analytically that for a pulsed dye laser amplifier, transversely pumped by a short duration pulsed laser, there exists an optimum gain length of the amplifier at dye laser wavelengths at which ground state absorption does not vanish. Thus, if the available pump power is distributed over this gain length, the extraction efficiency and the saturated gain of the amplifier reaches a maximum. The dependence of the extraction efficiency and gain on the amplifier length is strongly affected by the nonlinear absorption of the dye laser arising from excited state absorption, subsequent to ground state absorption.
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    URL: http://dx.doi.org/10.1007/BF00331908
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  • 94
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    A new blue-green XeF (C→A) excimer laser amplifier concept (1984)
    Springer
    Applied physics 35 (1984), S. 227-231 
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    ISSN: 1432-0649
    Keywords: 42.55 ; 42.60
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The feasibility of using the electrically excited XeF(C»A) excimer medium as an efficient wideband amplifier in the blue-green region of the spectrum has been investigated. Calculations show that for an intense blue-green optical flux input the amplification characteristics of XeF(C»A) improve, as a result of both bleaching of the pump induced absorbers and by additional production of XeF(C) level population. The removal of one of the major absorbing species, Xe** in the XeF (C»A) laser mixture by means of a pulsed ruby laser probe beam has been demonstrated.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00693931
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  • 95
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    Laser induced lasing in CS2 vapor (1992)
    Springer
    Applied physics 54 (1992), S. 221-226 
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    ISSN: 1432-0649
    Keywords: 42.50 ; 42.55 ; 42.55H
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract When CS2, contained in a tube at pressures ranging from 350 to 450 mTorr, was optically excited by a pulsed laser at a wavelength of 343.6 nm to the J=29, v=(0, 10, 0), R 3 B 2 state (i.e., the Σ=0 component of the a 3 A 2 state), six coherent emissions were observed along the same axis from both ends of the tube. These emissions possess the characteristics of the pump laser, such as linewidth, pulse duration and polarization, but do not need a cavity to gain amplification. The emissions terminate on the high vibrational states of the ground electronic state. A time delay between the pump laser and the emissions was observed. The emission intensity depends non-linearly on the CS2 pressure and exhibits a third order power dependence. A cooperative stimulated emission model is proposed to explain this phenomenon.
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    URL: http://dx.doi.org/10.1007/BF00325506
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    Output power enhancement of the 632.8 nm monomode He-Ne/I2-laser (1992)
    Springer
    Applied physics 54 (1992), S. 307-308 
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    ISSN: 1432-0649
    Keywords: 42.55 ; 42.60
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract For the He-Ne/I2-laser, a stable monomode operation has been realized when the tube pressure exceeds a certain level. An output power of more than 1 mW has been obtained at the 632.8 nm laser transition. Within the monomode tuning range of the laser, the d, e, f, g, and h, i, j iodine hyperfine components of the R(127) line of the 11–5 band of the B 3 II + 0u−X 1Σ+ 0g electronic transition have been observed. The mode selection method used makes it possible to increase the contrast of the iodine hyperfine components.
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    URL: http://dx.doi.org/10.1007/BF00325197
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  • 97
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    Theory of passive mode-locking of CW dye lasers with contacted and non-contacted absorbers (1981)
    Springer
    Applied physics 26 (1981), S. 197-202 
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    ISSN: 1432-0649
    Keywords: 42.55
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract A theoretical treatment of the influence of a saturable absorber in close contact with a highly reflecting mirror on a light pulse is given. The shaping of a Gaussian pulse during a single passage through such an absorber is calculated for various absorber lengths. The influence of absorber position and length on the pulse parameters and the stability of a continuously pumped dye laser are investigated. The shortest pulses and the most favourable operation conditions of the laser are to be expected in the case of a short contacted saturable absorber.
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    URL: http://dx.doi.org/10.1007/BF00692447
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  • 98
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    Waveguide CW 118.6 μm H2O laser (1982)
    Springer
    Applied physics 27 (1982), S. 123-128 
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    ISSN: 1432-0649
    Keywords: 42.55 ; 42.60
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract This paper reports results of an experimental study of a cw 118.6 μm H2O waveguide laser. The laser cavity is a 3 cm inner diameter, 3.2 m long Pyrex tube, with plane reflectors against its ends, one of them being a copper mesh coupler. The active medium is a H2O:H2 gas mixture. Successive optimizations lead to a reliable output power of 50 mW, for the EH11 mode. The power density is the highest ever reported, and the stability is such that the power drifts by less than 2% per hour. This laser is competitive with the optically pumped 118.8 μm CH3OH laser.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00694636
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  • 99
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    Picosecond pulse transmission in germanium of various thicknesses (1982)
    Springer
    Applied physics 27 (1982), S. 201-205 
    Details
    ISSN: 1432-0649
    Keywords: 42.10 ; 42.55 ; 78.20
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The transmission of ultrashort pulses from a mode-locked Nd: glass laser in germanium of various thicknesses (3 to 8 μm) has been measured as a function of incident irradiance. Transmission is seen to increase with irradiance level in all samples. The degree of enhancement is greater for the thcker samples. At high excitation levels, thinner samples show a peaking of transmission, which does not occur in a thick sample. Taking the sample as composed of thin elements, the parameters characterizing the photoexcited electron-hole plasma have been found by assuming homogeneous excitation within each element. Theoretical curves thus obtained give good quantitative account of the experimental results. Peaking of transmission is seen to due to a balance between absorption enhancement in the front portion of the sample and absorption reduction in the back.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00697442
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  • 100
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    Optically pumped14NH3 laser and its stark tuning at 10.78 μm (1982)
    Springer
    Applied physics 28 (1982), S. 55-62 
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    ISSN: 1432-0649
    Keywords: 33 ; 42.55
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract Infrared (ir) emissions from a TEA-CO2-laser-pumped NH3 laser are reported. Superfluorescent emissions and selective single-line oscillations have been obtained in the range from 11 to 13 μm. The results make possible the design of a NH3 Stark cell allowing a 1 GHz shift of the 10.78 μm NH3 emission line.
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    URL: http://dx.doi.org/10.1007/BF00693893
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