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  • 04. Solid Earth::04.08. Volcanology::04.08.01. Gases  (43)
  • 04. Solid Earth::04.08. Volcanology::04.08.99. General or miscellaneous
  • American Geophysical Union  (27)
  • INGV  (25)
  • Annual Reviews
  • 2005-2009  (52)
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  • 1
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    Investigation into magma degassing at Nyiragongo volcano, Democratic Republic of the Congo (2008)
    American Geophysical Union
    Details
    Publication Date: 2021-01-27
    Description: We report the first combined measurements of the composition and flux of gas emitted from Nyiragongo volcano by ground-based remote-sensing techniques. Ultraviolet spectroscopic measurements made in May/June 2005 and January 2006 indicate average SO2 emission rates of 38 kg s−1 and 23 kg s−1, respectively. Open-path Fourier transform infrared spectroscopic measurements obtained in May/June 2005, January 2006, and June 2007 indicate average molar proportions of 70, 24, 4.6, 0.87, 0.26, 0.11, and 0.0016% for H2O, CO2, SO2, CO, HCl, HF, and OCS, respectively. The composition of the plume was remarkably similar in 2005, 2006, and 2007, with little temporal variation in proportions of CO2, SO2, and CO, in particular, on the scale of seconds or days or even between the three field campaigns that span a period of 24 months. This stability persisted despite a wide range of degassing behaviors on the surface of the summit crater's lava lake (including discrete strombolian bursts and lava fountains) and variations in the SO2 emission rate. We explain these observations by a regime of steady state degassing in which bubbles nucleate and ascend in chemical equilibrium with the convecting magma. Short-term (seconds to minutes) temporal fluctuations in the SO2–HCl–HF composition were observed, and these are attributed to shallow degassing processes.
    Description: Published
    Description: Q02017
    Description: 1.2. TTC - Sorveglianza geochimica delle aree vulcaniche attive
    Description: JCR Journal
    Description: reserved
    Keywords: Nyiragongo ; volcanic gas emissions ; FTIR ; DOAS ; remote sensing ; spectroscopy ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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  • 2
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    Monitoring of fumarole discharge and CO2 soil degassing in the Azores: contribution to volcanic surveillance and public health risk assessment (2006)
    INGV
    Details
    Publication Date: 2020-11-12
    Description: Fluid geochemistry monitoring in the Azores involves the regular sampling and analysis of gas discharges from fumaroles and measurements of CO2 diffuse soil gas emissions. Main degassing areas under monitoring are associated with hydrothermal systems of active central volcanoes in S. Miguel, Terceira and Graciosa islands. Fumarole discharge analysis since 1991 show that apart from steam these gas emissions are CO2 dominated with H2S, H2, CH4 and N2 in minor amounts. Mapping of CO2 diffuse soil emissions in S. Miguel Island lead to the conclusion that some inhabited areas are located within hazard-zones. At Furnas village, inside Furnas volcano caldera, about 62% of the 896 houses are within the CO2 anomaly, 5% being in areas of moderate to high risk. At Ribeira Seca, on the north flank of Fogo volcano, few family houses were evacuated when CO2 concentrations in the air reached 8 mol%. To assess and analyse the CO2 soil flux emissions, continuous monitoring stations were installed in S. Miguel (2), Terceira and Graciosa islands. The statistical analysis of the data showed that some meteorological parameters influence the CO2 flux. The average of CO2 flux in S. Miguel stations ranges from 250 g/m2/d at Furnas volcano to 530 g/m2/d at Fogo volcano. At Terceira Island it is about 330 g/m2/d and at Graciosa 4400 g/m2/d.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: volcanology ; geochemistry ; soil degassing ; monitoring ; risk ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring
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  • 3
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    Local stresses, dyke arrest and surface deformation in volcanic edificesand rift zones (2006)
    INGV
    Details
    Publication Date: 2021-06-15
    Description: Field studies indicate that nearly all eruptions in volcanic edifices and rift zones are supplied with magma through fractures (dykes) that are opened by magmatic overpressure. While (inferred) dyke injections are frequent during unrest periods, volcanic eruptions are, in comparison, infrequent, suggesting that most dykes become arrested at certain depths in the crust, in agreement with field studies. The frequency of dyke arrest can be partly explained by the numerical models presented here which indicate that volcanic edifices and rift zones consisting of rocks of contrasting mechanical properties, such as soft pyroclastic layers and stiff lava flows, commonly develop local stress fields that encourage dyke arrest. During unrest, surface deformation studies are routinely used to infer the geometries of arrested dykes, and some models (using homogeneous, isotropic half-spaces) infer large grabens to be induced by such dykes. Our results, however, show that the dyke-tip tensile stresses are normally much greater than the induced surface stresses, making it difficult to explain how a dyke can induce surface stresses in excess of the tensile (or shear) strength while the same strength is not exceeded at the (arrested) dyke tip. Also, arrested dyke tips in eroded or active rift zones are normally not associated with dyke-induced grabens or normal faults, and some dykes arrested within a few metres of the surface do not generate faults or grabens. The numerical models show that abrupt changes in Young's moduli(stiffnesses), layers with relatively high dyke-normal compressive stresses (stress barriers), and weak horizontal contacts may make the dyke-induced surface tensile stresses too small for significant fault or graben formation to occur in rift zones or volcanic edifices. Also, these small surface stresses may have no simple relation to the dyke geometry or the depth to its tip. Thus, for a layered crust with weak contacts, straightforward inversion of surface geodetic data may lead to unreliable geometries of arrested dykes in active rift zones and volcanic edifices.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: dyke injection ; dyke arrest ; crustalstresses ; crustal layering ; surface deformation ; volcanic hazard ; 04. Solid Earth::04.08. Volcanology::04.08.99. General or miscellaneous ; 04. Solid Earth::04.08. Volcanology::04.08.05. Volcanic rocks
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  • 4
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    S, Cl and F degassing as an indicator of volcanic dynamics: The 2001 eruption of Mount Etna (2005)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: The recent eruption of Mount Etna (July 2001) offered the opportunity to analyze magma-derived volatiles emitted during preand syn-eruptive phases, and to verify whether their composition is affected by changes in volcanic dynamics. This paper presents the results of analyses of F, Cl and S in the volcanic plume collected by filter-packs, and interprets variations in the composition based on contrasting solubility in magmas. A Rayleigh-type degassing mechanism was used to fit the acquired data and to estimate Henryâ s solubility constant ratios in Etnean basalt. This model provided insights into the dynamics of the volcano. Abundances of sulfur and halogens in eruptive plumes may help predict the temporal evolution of an ongoing effusive eruption.
    Description: -Gruppo Nazionale per la Vulcanologia.
    Description: Published
    Description: 1559
    Description: partially_open
    Keywords: magmatic degassing ; acidic gases ; plume chemistry ; 01. Atmosphere::01.01. Atmosphere::01.01.07. Volcanic effects ; 04. Solid Earth::04.04. Geology::04.04.12. Fluid Geochemistry ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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  • 5
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    Real-time measurement of volcanic H2S and SO2 concentrations by UV spectroscopy (2006)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: Sulphur speciation in volcanic gases acts as a major redox buffer, and H2S/SO2 ratios represent a valuable indicator of magmatic conditions and interactions between magmatic and hydrothermal fluids. However, measurement of H2S/SO2 even by direct sampling techniques, is not straightforward. We report here on application of a small ultraviolet spectrometer for real-time field measurement of H2S and SO2 concentrations, using open-path and extractive configurations. The device was tested at fumaroles on Solfatara and Vulcano, Italy, in November 2002. H2S concentrations of up to 220ppmm(400 ppmv) were measured directly above the Bocca Grande fumarole at Solfatara, and H2S/SO2 molar ratios of 2 and 2.4, respectively, were determined for the ‘F11’ and ‘F0’ fumaroles at Vulcano. In comparison with other optical techniques capable of multiple volcanic gas measurements, such as laser and FTIR spectroscopy, this approach is considerably simpler and cheaper, with the potential for autonomous, sustained hightime resolution operation.
    Description: Published
    Description: 1652
    Description: partially_open
    Keywords: Remote monitoring ; Plume chemistry ; sulphur species ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring ; 04. Solid Earth::04.08. Volcanology::04.08.07. Instruments and techniques
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  • 6
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    The changing face of Mount Etna’s summit area documented with Lidar technology (2008)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: Morphostructural data derived from Lidar (Light detection and ranging) surveys carried out on Mount Etna in 2005 and 2007 are compared with earlier aerophotogrammetric surveys in 1986 and 1998. These data render an unprecedentedly clear and quantitative image of morphostructural and volumetric changes that have affected the summit area of the volcano in the past two decades and permit the production of a new topographic map. The computed volume gain during the 1986–2007 period amounts to 112 ± 12 106 m3, at a mean annual rate of 5.3 106 m3. The comparison of the various surveys furthermore emphasizes the levels of accuracy and resolution of the different techniques applied. The Lidar technology used in 2007 allows production of high-precision maps in near-real-time, facilitating work concerning environmental hazards such as numerical simulations of, e.g., lava flows.
    Description: Published
    Description: L09305
    Description: 1.5. TTC - Sorveglianza dell'attività eruttiva dei vulcani
    Description: 1.10. TTC - Telerilevamento
    Description: JCR Journal
    Description: partially_open
    Keywords: Lidar ; Etna ; morphostructural changes ; lava flows ; 04. Solid Earth::04.08. Volcanology::04.08.99. General or miscellaneous
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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  • 7
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    Continuous monitoring of soil CO2 flux on Mt. Etna:The 2004–2005 eruption and the role of regional tectonics and volcano tectonics. (2008)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: The soil CO2 flux on Mt. Etna as recorded by the ETNAGAS network (an automatic system for measuring soil CO2 flux and meteorological parameters) started to increase strongly about 5 months prior to the onset of the 2004–2005 eruption and decreased a few months before the end of the eruption. Time delays in the occurrences of anomalies in soil CO2 flux at different sites in the geochemical network constrain the relationship between soil CO2 flux distributions and the tectonic framework of Etna volcano. The anomalies observed before the 2004–2005 eruption support the intrusion of new undegassed magma into the upper feeding system of the volcano (〈20 km below sea level). Magma subsequently rose slowly in the volcano conduits, thereby triggering the onset of the 2004–2005 eruption. The time delays in the occurrences of anomalies in combination with spectral analysis indicate the importance of tectonic and volcanotectonic structures in driving the ascent of deep gases within the crust. Moreover, greatest amplitude pulsations of the low-frequency components of the CO2 flux signals were correlated with the paroxystic activities of the 2004–2005 eruption. This study confirms that CO2 flux variation is a useful indicator for volcanic activity in the surveillance of the Mt. Etna and similar basaltic volcanoes.
    Description: Dipartimento Protezione Civile Ministero degli Interni
    Description: Published
    Description: B09206
    Description: 1.5. TTC - Sorveglianza dell'attività eruttiva dei vulcani
    Description: JCR Journal
    Description: reserved
    Keywords: CO2 flux ; Continuous monitoring of soil CO2 flux ; 04. Solid Earth::04.04. Geology::04.04.12. Fluid Geochemistry ; 04. Solid Earth::04.07. Tectonophysics::04.07.07. Tectonics ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring ; 05. General::05.02. Data dissemination::05.02.03. Volcanic eruptions
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  • 8
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    Intercomparison of volcanic gas monitoring methodologies performed on Vulcano Island, Italy (2005)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: Volcanic gas emissions from fumaroles on the rim of La Fossa crater, Vulcano Island, Italy, were measured simultaneously using direct sampling (for H2O, CO2, total sulfur, HCl and HF), filter packs (for SO2, HCl, HF) and short-path active-mode FTIR measurements (for H2O, CO2,SO2, HCl and HF) in an intercomparison study in May 2002. The results show that Cl/F ratios were in good agreement between all three methods, and that FTIR and direct sampling determined comparable proportions of CO2 and H2O. Amounts of total S observed in direct sampling data were approximately double the amounts of SO2 measured with filter packs and FTIR. This difference could be attributed either to the fact FTIR and filter packs do not measure reduced sulfur species (e.g., H2S) or to sublimation of elemental S upon exit from the fumarole, after collection by direct sampling but before detection with FTIR and filter packs.
    Description: Published
    Description: L02610
    Description: partially_open
    Keywords: volcanic gas techniques ; gas geochemistry ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring ; 04. Solid Earth::04.08. Volcanology::04.08.07. Instruments and techniques
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  • 9
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    Molecular and isotopic composition of free hydrocarbon gases from Sicily, Italy (2005)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: Chemical and isotopic data have been used as geochemical tracers for a genetic characterization of hydrocarbon gases from a total of eleven manifestations located in Eastern and Central-Southern Sicily (Italy). The molecular analysis shows that almost all the samples are enriched in methane (up to 93.2% Vol.), with the exception of four gas samples collected around Mt. Etna showing high mantle-derived CO2 content. Methane isotope signatures suggest that these are thermogenic gases or a mixture between thermogenic gases and microbial gases. Although samples from some mud volcanoes in Southern Sicily (Macalube di Aragona) show isotope signatures consistent with a mixing model between thermogenic and microbial, by combining the molecular compositions (C1/(C2 + C3))and the methane isotope ratios (d13C1), such a process seems to be excluded. Therefore, the occurrence of secondary post-genetic processes should be invoked. Two main hypotheses have been considered: the first hypothesis includes that the gas is produced by microbial activity and altered post-genetically by microbial oxidation of methane, while according to the second hypothesis thermogenic gas have modified their molecular ratios due to vertical migration.
    Description: Published
    Description: L06607
    Description: partially_open
    Keywords: Isotopic composition/chemistry ; Organic geochemistry ; 03. Hydrosphere::03.04. Chemical and biological::03.04.06. Hydrothermal systems ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 05. General::05.02. Data dissemination::05.02.01. Geochemical data
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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  • 10
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    Emission of bromine and iodine from Mount Etna volcano (2005)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: Constraining fluxes of volcanic bromine and iodine to the atmosphere is important given the significant role these species play in ozone depletion. However, very few such measurements have been made hitherto, such that global volcanic fluxes are poorly constrained. Here we extend the data set of volcanic Br and I degassing by reporting the first measurements of bromine and iodine emissions from Mount Etna. These data were obtained using filter packs and contemporaneous ultraviolet spectroscopic SO2 flux measurements, resulting in time-averaged emission rates of 0.7 kt yr 1 and 0.01 kt yr 1 for Br and I, respectively, from April to October 2004, from which we estimate global Br and I fluxes of order 13 (range, 3â 40) and 0.11 (range, 0.04â 6.6) kt yr 1. Observed changes in plume composition highlight the coherent geochemical behavior of HCl, HF, HBr, and HI during magmatic degassing, and strong fractionation of these species with respect to SO2.
    Description: Published
    Description: Q08008
    Description: partially_open
    Keywords: bromine and iodine in volcanic gases ; halogen atmospheric chemistry ; volcanic degassing ; volcanic plumes ; 01. Atmosphere::01.01. Atmosphere::01.01.07. Volcanic effects ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring
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  • 11
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    Accurate measurement of volcanic SO2 flux: Determination of plume transport speed and integrated SO2 concentration with a single device (2005)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: Ground-based measurements of volcanic sulfur dioxide fluxes are important indicators of volcanic activity, with application in hazard assessment, and understanding the impacts of volcanic emissions upon the environment and climate. These data are obtained by making traverses underneath the volcanic plume a few kilometers from source with an ultraviolet spectrometer, measuring integrated SO2 concentrations across the plume’s cross section, and multiplying by the plume’s transport speed. However, plume velocities are usually derived from ground-based anemometers, located many kilometers from the traverse route and hundreds of meters below plume altitude, complicating the experimental design and introducing large flux (can be 〉100%) errors. Here we present the first report of a single instrument capable of (accurate) volcanic SO2 flux measurements. This device records integrated SO2 concentrations and plume heights during traverses. Between traverses, two in-plume SO2 time series are measured from underneath the plume with the instrument, corresponding to zenith and inclined (user-specified angle from vertical in the direction of the volcano) fields of view, respectively. The distance between the points of intersection of the two views with the plume is found on the basis of the determined plume height, and the two signals are cross-correlated to determine the lag between them, enabling accurate derivation of the wind speed. We present flux data (with errors ±12%) obtained in this way at Mt. Etna during July 2004.
    Description: Published
    Description: Q02003
    Description: partially_open
    Keywords: DOAS ; volcanic SO2 emissions. ; 01. Atmosphere::01.01. Atmosphere::01.01.07. Volcanic effects ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring ; 04. Solid Earth::04.08. Volcanology::04.08.07. Instruments and techniques ; 04. Solid Earth::04.08. Volcanology::04.08.08. Volcanic risk
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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  • 12
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    Best-fit results from application of a thermo-rheological model for channelized lava flow to high spatial resolution morphological data (2007)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: The FLOWGO thermo-rheological model links heat loss, core cooling, crystallization, rheology and flow dynamics for lava flowing in a channel. We fit this model to laser altimeter (LIDAR) derived channel width data, as well as effusion rate and flow velocity measurements, to produce a best-fit prediction of thermal and rheological conditions for lava flowing in a ~1.6 km long channel active on Mt. Etna (Italy) on 16th September 2004. Using, as a starting condition for the model, the mean channel width over the first 100 m (6 m) and a depth of 1 m we obtain an initial velocity and instantaneous effusion rate of 0.3–0.6 m/s and ~3 m3/s, respectively. This compares with field- and LIDAR-derived values of 0.4 m/s and 1–4 m3/s. The best fit between model-output and LIDAR-measured channel widths comes from a hybrid run in which the proximal section of the channel is characterised by poorly insulated flow and the medial-distal section by well-insulated flow. This best-fit model implies that flow conditions evolve down-channel, where hot crusts on a free flowing channel maximise heat losses across the proximal section, whereas thick, stable, mature crusts of ′a′a clinker reduce heat losses across the medial-distal section. This results in core cooling per unit distance that decreases from ~0.02–0.015°C m−1 across the proximal section, to ~0.005°C m−1 across the medial-distal section. This produces an increase in core viscosity from ~3800 Pa s at the vent to ~8000 Pa s across the distal section.
    Description: Published
    Description: L01301
    Description: 3.6. Fisica del vulcanismo
    Description: 3.5. Geologia e storia dei sistemi vulcanici
    Description: JCR Journal
    Description: reserved
    Keywords: Kava Channel ; LIDAR ; thermal modeling ; 04. Solid Earth::04.08. Volcanology::04.08.99. General or miscellaneous
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  • 13
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    Deformation and eruptions at Mt. Etna (Italy): A lesson from 15 years of observations (2009)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: Volcanoes deform as a consequence of the rise and storage of magma; once magma reaches a critical pressure, an eruption occurs. However, how the edifice deformation relates to its eruptive behavior is poorly known. Here, we produce a joint interpretation of spaceborne InSAR deformation measurements and volcanic activity at Mt. Etna (Italy), between 1992 and 2006. We distinguish two volcano-tectonic behaviors. Between 1993 and 2000, Etna inflated with a starting deformation rate of 1 cm yr 1 that progressively reduced with time, nearly vanishing between 1998 and 2000; moreover, low-eruptive rate summit eruptions occurred, punctuated by lava fountains. Between 2001 and 2005, Etna deflated, feeding higher-eruptive rate flank eruptions, along with large displacements of the entire East-flank. These two behaviors, we suggest, result from the higher rate of magma stored between 1993 and June 2001, which triggered the emplacement of the dike responsible for the 2001 and 2002–2003 eruptions. Our results clearly show that the joint interpretation of volcano deformation and stored magma rates may be crucial in identifying impending volcanic eruptions.
    Description: This work was partly funded by INGV and the Italian DPC and was supported by ASI, the Preview Project and CRdC-AMRA. DPC-INGV Flank project providing the funds for the publication fees.
    Description: Published
    Description: L02309
    Description: 1.2. TTC - Sorveglianza geochimica delle aree vulcaniche attive
    Description: 1.5. TTC - Sorveglianza dell'attività eruttiva dei vulcani
    Description: 1.10. TTC - Telerilevamento
    Description: 3.6. Fisica del vulcanismo
    Description: 4.3. TTC - Scenari di pericolosità vulcanica
    Description: 4.5. Degassamento naturale
    Description: JCR Journal
    Description: partially_open
    Keywords: deformation ; eruptions ; Mt. Etna ; eruptive cycle ; InSAR ; 04. Solid Earth::04.01. Earth Interior::04.01.99. General or miscellaneous ; 04. Solid Earth::04.01. Earth Interior::04.01.02. Geological and geophysical evidences of deep processes ; 04. Solid Earth::04.03. Geodesy::04.03.99. General or miscellaneous ; 04. Solid Earth::04.03. Geodesy::04.03.06. Measurements and monitoring ; 04. Solid Earth::04.03. Geodesy::04.03.07. Satellite geodesy ; 04. Solid Earth::04.04. Geology::04.04.99. General or miscellaneous ; 04. Solid Earth::04.04. Geology::04.04.09. Structural geology ; 04. Solid Earth::04.04. Geology::04.04.12. Fluid Geochemistry ; 04. Solid Earth::04.07. Tectonophysics::04.07.99. General or miscellaneous ; 04. Solid Earth::04.07. Tectonophysics::04.07.02. Geodynamics ; 04. Solid Earth::04.07. Tectonophysics::04.07.07. Tectonics ; 04. Solid Earth::04.08. Volcanology::04.08.99. General or miscellaneous ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.03. Magmas ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring ; 04. Solid Earth::04.08. Volcanology::04.08.07. Instruments and techniques ; 04. Solid Earth::04.08. Volcanology::04.08.08. Volcanic risk ; 05. General::05.02. Data dissemination::05.02.03. Volcanic eruptions
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  • 14
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    Gas Flux Rate and Migration of the Magma Column (2008)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: The 2002–2003 effusive eruption of Stromboli volcano represents an excellent opportunity to investigate the transition from effusive to explosive activity at an open-conduit basaltic system, when activity migrated from effusive vents, at the base of the craters, to summit explosions. The transition is investigated here through the analysis of very long period seismicity, delay times between infrasonic and thermal onsets of explosions, and SO2 flux recorded during a 1-year period. The synergy of the multiple geophysical observations points to a magma-driven migration of the magma column. Here the increased magma supply at the eruption onset lead to opening of effusive fissures, which draining the magma in the shallow conduit caused the decrease of the magma level. The decrease of the magma supply at the end of the effusion lead to sealing of effusive fissures, upraise of the magma level within the conduit, and reestablishment of explosive activity from the summit vents.
    Description: Unpublished
    Description: 11
    Description: 1.2. TTC - Sorveglianza geochimica delle aree vulcaniche attive
    Description: 1.10. TTC - Telerilevamento
    Description: 3.6. Fisica del vulcanismo
    Description: reserved
    Keywords: Stromboli ; SO2 Flux ; Magma column ; Infrasound ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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  • 15
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    Volcanic plume monitoring at Mount Etna by diffusive (passive) sampling (2005)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: This paper reports the use of diffusive tubes in determining HF, HCl, and SO2 in the volcanic plume of Mount Etna in an attempt to highlight the potential of this method in studying volcanoes. In a first application a network of 18 diffusive tubes was installed on Etna flanks, aimed at evaluating the atmospheric dispersion of the volcanic plume on a local scale. Results showed a monotonic decrease in volatile air concentrations with distance from the craters (HF from 0.15 to 〈0.003 mmol m3, HCl from 2 to 〈0.01 mmol m3, and SO2 from 11 to 0.04 mmol m3), revealing the prevalently volcanic contribution. Matching of SO2/HCl and HCl/HF volatile ratios with contemporaneous measurements at the summit craters validated the use of diffusive tubes in tracing the chemical features of a volcanic plume from remote locations. A first tentative assessment of dry deposition rates of volcanogenic acidic gases was also made, yielding 2.5 74 t d1 (SO2), 0.6 17 t d1 (HCl), and 0.02 0.6 t d1 (HF) and revealing the potential environmental impact of gas emissions. In a second experiment, carried out during the recent October 2002 to February 2003 eruption of Etna, diffusive tubes provided a continuous record of the chemical composition of the eruptive plume from a safe distance of 1 km from the vents, thus considerably decreasing the risks involved in sampling. This highlighted a clear time decrease in SO2 concentrations and SO2/HCl ratios, which was interpreted as due to progressive exhaustion of volatile degassing and eruption energy.
    Description: Published
    Description: D21308
    Description: partially_open
    Keywords: volcanic plumes ; impact of volcanic emissions ; sulfur and halogens chemistry ; 04. Solid Earth::04.03. Geodesy::04.03.06. Measurements and monitoring ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring ; 05. General::05.02. Data dissemination::05.02.03. Volcanic eruptions
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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  • 16
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    Volcanic gas emissions from the summit craters and flanks of Mt. Etna, 1987-2000 (2005)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: In the last 13 years gas emissions from both the summit and the flanks of Mount Etna volcano have been monitored using remote sensing techniques (COSPEC, and FTIR since 2000) and on-site monitoring devices. The SO2 flux variations (600 to 25,000 Mg/day) indicated: (i) low values coinciding with deep seismicity prior to eruptions or/and preceding increases in summit volcanic activity; (ii) increasing trends tracking the ascent of fresh magma within the shallow feeding system and whose rate seems proportional to the speed of magma rise; (iii) decreasing trends related to progressive degassing of magma batches; (iv) an imbalance between the amount of magma erupted and that which contributed the SO2 emission (~ 13 % of the degassing magma having been erupted during the studied period), implying that magma degassing is dominantly intrusive; (v) a seasonal component, probably due to variations in solar zenith angle, meteorological parameters and, possibly, tidal forces.FTIR monitoring allowed to recognize significant variations of SO2/HCl and SO2/HF ratios in the volcanic plume which, combined with COSPEC data, provided new insight into the dynamics of ascent and degassing of discrete magma bodies. Strong variations in CO2-rich soil degassing are interpreted as markers of gradual magma ascent from great depth (〉10 km) to the upper (〈5 km) feeding system of Mt. Etna. These changes appear to precede increases in SO2 plume flux at the craters and, so, provide additional constraints upon the interpretation of COSPEC data and the modeling of magma rise at that volcano.
    Description: Published
    Description: 111-128
    Description: partially_open
    Keywords: Gas emissions ; Mt. Etna ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: book chapter
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  • 17
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    Nitrogen isotopes in thermal fluids of a forearc region (Jalisco Block, Mexico): evidence for heavy nitrogen from continental crust (2005)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: The Jalisco Block (JB) is a geologically and tectonically complex part of northwestern Mexico characterized by active subduction-type volcanism, rifting, and old stable structures. Thermal springs and groups of springs are widely distributed over JB. Bubbling gas from seven thermal springs located within different tectonic environments of the JB was analyzed for He, 20Ne, and N2 concentrations and d15N ratios. All gases are N2-dominant (〉84%) with the exception of one sample (Rio´ Purificacio´n), which has a significant CH4 content (about 50%). All collected gas samples are relatively high in He, up to 1500 ppm vol and with 3He/4He values ranging from 0.6 to 4.5 Ra. All measured nitrogen isotope ratios are heavier than air with d15N values ranging from 0.5 to 5.0%. The relative N2 excess with respect to air-saturated water computed on the basis of N2 and 20Ne contents indicates the contribution of a nonatmospheric N2 source. All the samples show a good correlation between d15N and the relative excess of N2 with d15N +5.3% for the maximum N2 excess of 100%. Due to a presumed lack of seafloor sediment involved in the subduction process, such a d15N positive value seems to reflect the addition to the fluids of a heavy nitrogen originating from metamorphism processes of rocks occurring within the overlying continental crust.
    Description: Published
    Description: 1-9
    Description: partially_open
    Keywords: bubbling gases ; forearc region ; Jalisco Block-Mexico ; nitrogen isotopes ; subduction-related volcanism ; 03. Hydrosphere::03.04. Chemical and biological::03.04.05. Gases ; 03. Hydrosphere::03.04. Chemical and biological::03.04.06. Hydrothermal systems ; 04. Solid Earth::04.07. Tectonophysics::04.07.06. Subduction related processes ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 05. General::05.02. Data dissemination::05.02.01. Geochemical data
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  • 18
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    Chemical mapping of a fumarolic field: La Fossa Crater, Vulcano Island (Aeolian Islands, Italy) (2005)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: The performance of a newly-developed portable gas analyzer, capable of real-time measurement of CO2, SO2 and H2S concentrations in volcanic gases, was tested at La Fossa Crater, Vulcano Island. The gas analyzer was used to acquire about 3000 determinations over the fumarolic field, allowing the definition of its chemical structure and heterogeneity. Our high-resolution analysis reveals that, in December 2004, the La Fossa fumarolic field was characterized by an oxidized inner core (SO2/H2S ratios of 3), and by more reducing conditions on its northern edge (SO2/H2S ratios of 1; range: 0.2–3.3). CO2/(SO2+H2S) molar ratios averaged 35 ± 21, with overlapping compositions for rim and inner crater fumaroles. S-poor compositions (CO2/(SO2+H2S) 50) characterized the field margins, probably due to deposition of native sulfur. Based on the above data and an SO2 flux of 18 ± 3 t.d-1, we estimate CO2 and H2S output rates from the volcano of 420 ± 250 and 4 ± 2 t.d-1, respectively.
    Description: Published
    Description: L13309
    Description: partially_open
    Keywords: electrochemical sensors ; fumarolic gases ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring ; 04. Solid Earth::04.08. Volcanology::04.08.07. Instruments and techniques
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    Type: article
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  • 19
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    Sliding episodes during the 2002–2003 Stromboli lava effusion: Insights from seismic, volcanic, and statistical data analysis (2008)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: Repeated phenomena of flank instability accompanied the 28 December 2002 to 21 July 2003 eruption of Stromboli volcano. The major episodes were two tsunamigenic landslides on 30 December 2002, 2 d after the volcano unrest. After 30 December, sliding processes remodeled the area affected by slope instability.We propose analyses of 565 sliding episodes taking place from December 2002 to February 2003.We try to shed light on their main seismic features and links with the ongoing seismic and volcanic activity using variogram analysis as well. A characterization of the seismic signals in the time and frequency domains is presented for 185 sliding episodes. Their frequency content is between 1 Hz and 7 Hz. On the basis of the dominant peaks and shape of the spectrum, we identify three subclasses of signals, one of which has significant energy below 2 Hz. Low-frequency signatures were also found in the seismic records of the landslides of 30 December, which affected the aerial and submarine northwestern flank of the volcano. Accordingly, we surmise that spectral analysis might provide evidence of sliding phenomena with submarine runouts.We find no evidence of sliding processes induced by earthquakes. Additionally, a negative statistical correlation between sliding episodes and explosion quakes is highlighted by variogram analysis. Variograms indicate a persistent behavior, memory, of the flank instability from 5 to 10 d.We interpret the climax in the occurrence rate of the sliding processes between 24 and 29 January 2003 as the result of favorable conditions to slope instability due to the emplacement of NW-SE aligned, dike-fed vents located near the scarp of the landslide area. Afterward, the stabilizing effect of the lava flows over the northwestern flank of the volcano limited erosive phenomena to the unstable, loose slope not covered by lava.
    Description: This work was supported financially by Istituto Nazionale di Geofisica e Vulcanologia and Dipartimento per la Protezione Civile, project INGV-DPC V4/02.
    Description: Published
    Description: Q04022
    Description: 1.4. TTC - Sorveglianza sismologica delle aree vulcaniche attive
    Description: 1.5. TTC - Sorveglianza dell'attività eruttiva dei vulcani
    Description: 3.6. Fisica del vulcanismo
    Description: JCR Journal
    Description: reserved
    Keywords: rockfalls ; seismicity ; volcanoes ; volcano collapses ; Stromboli ; 04. Solid Earth::04.06. Seismology::04.06.99. General or miscellaneous ; 04. Solid Earth::04.06. Seismology::04.06.08. Volcano seismology ; 04. Solid Earth::04.07. Tectonophysics::04.07.99. General or miscellaneous ; 04. Solid Earth::04.08. Volcanology::04.08.99. General or miscellaneous ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring ; 04. Solid Earth::04.08. Volcanology::04.08.07. Instruments and techniques ; 05. General::05.02. Data dissemination::05.02.03. Volcanic eruptions
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  • 20
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    Variation of H2O/CO2 and CO2/SO2 ratios of volcanic gases discharged by continuous degassing of Mount Etna volcano, Italy (2008)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: We applied the Multi-GAS technique to measure compositions of the volcanic plumes continuously discharged from summit craters of Voragine, Northeast and Bocca Nuova at Mount Etna, in an attempt to estimate compositions of the source volcanic gases. The estimated CO2/SO2 and H2O/CO2 ratios of the volcanic gases show a large variation ranging from 0.6 to 30 and from 1 to 18, respectively. This variability overlaps with the compositional range of dissolved volatiles in melt inclusions and their coexisting bubbles in a magma chamber and can be caused by the low-pressure degassing of a magma with variable bubble content ranging from 0.3 to 15 wt.%. The variable bubble content in the magma is likely a result of supply of deep-derived CO2-rich gas phase to the chamber and subsequent bubble-magma differentiation by bubble ascent in the magma chamber. In contrast, the variation of volcanic gas composition can also be caused by changes of degassing pressure (gas–magma separation pressure), ranging from 0 to 100 MPa, as a result of changes in the depth of the top of the convecting magma in volcanic conduits. Both mechanisms can cause similar compositional variations. However, the two mechanisms will result in contrasting correlations between the SO2 emission rates and the gas compositions that can be examined by parallel observations of the emission rates and compositions in the future.
    Description: Published
    Description: B09203
    Description: 1.2. TTC - Sorveglianza geochimica delle aree vulcaniche attive
    Description: 4.5. Degassamento naturale
    Description: JCR Journal
    Description: reserved
    Keywords: Plume ; gas ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring
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  • 21
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    Unmanned aerial vehicle measurements of volcanic carbon dioxide fluxes (2008)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: We report the first measurements of volcanic gases with an unmanned aerial vehicle (UAV). The data were collected at La Fossa crater, Vulcano, Italy, during April 2007, with a helicopter UAV of 3 kg payload, carrying an ultraviolet spectrometer for remotely sensing the SO2 flux (8.5 Mg d 1), and an infrared spectrometer, and electrochemical sensor assembly for measuring the plume CO2/SO2 ratio; by multiplying these data we compute a CO2 flux of 170 Mg d 1. Given the deeper exsolution of carbon dioxide from magma, and its lower solubility in hydro-thermal systems, relative to SO2, the ability to remotely measure CO2 fluxes is significant, with promise to provide more profound geochemical insights, and earlier eruption forecasts, than possible with SO2 fluxes alone: the most ubiquitous current source of remotely sensed volcanic gas data.
    Description: Published
    Description: L06303
    Description: 1.2. TTC - Sorveglianza geochimica delle aree vulcaniche attive
    Description: JCR Journal
    Description: reserved
    Keywords: Plume measurements ; carbon dioxide fluxes ; 04. Solid Earth::04.04. Geology::04.04.12. Fluid Geochemistry ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring ; 04. Solid Earth::04.08. Volcanology::04.08.07. Instruments and techniques
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  • 22
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    Anomalous magmatic degassing prior to the 5th April 2003 paroxysm on Stromboli (2005)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: A major explosion occurred at Stromboli on April 5 2003, being the most powerful event over a period of exceptional eruptive activity lasting from December to July. Here, we describe results from a network of diffusive tubes set up on the Stromboli’s summit area, aimed at a characterisation of plume composition (SO2, HCl, HF) prior to and after April 5. Data analysis revealed anomalous sulphur degassing 2–3 days before the event, when SO2/HCl ratios (9) significantly higher than those typical of quiescent degassing (1) were recorded. We interpret this exceptional plume signature as an evidence of S-rich magmas ascending in the shallow plumbing system, and propose high SO2/HCl as a potential precursor of major explosions on the volcano. The post-April 5 phase was characterised by time-decreasing SO2/HCl and SO2/HF plume ratios, ascribed to declining magma feeding as a prelude to restoration of ‘‘normal’’ Strombolian activity.
    Description: Published
    Description: L14607
    Description: partially_open
    Keywords: magmatic degassing ; paroxysm ; Stromboli ; 04. Solid Earth::04.03. Geodesy::04.03.06. Measurements and monitoring ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring ; 05. General::05.02. Data dissemination::05.02.03. Volcanic eruptions
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  • 23
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    Evidence of a recent input of magmatic gases into the quiescent volcanic edifice of Panarea, Aeolian Islands, Italy (2005)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: On 2nd/3rd November 2002, a huge amount of gas, mainly composed of CO2, was suddenly released from the sea bottom off the coast of Panarea, producing a ‘‘crater’’20 by 10 meters wide and 7 meters deep. The gas output was estimated to be 109 l/d, two orders of magnitude higher than that measured in the 1980s. The anomalous degassing rate lasted for some weeks, slowly decreasing to an almost constant rate of about 4 x 107 l/d after two months. The geothermo- barometric estimations revealed an increase of both the temperature and pressure in the geothermal system feeding the sampled vents. The 3He/4He ratios were similar to those measured in nearby Stromboli. We have monitored the area for the last two decades, and based on our intensive and extensive geochemical measurements, have ascertained that the geothermal reservoir has lost its steady state. We maintain that a new magmatic input caused these phenomena.
    Description: - Istituto Nazionale di Geofisica e Vulcanologia, Osservatorio Vesuviano, Naples, Italy. - Istituto Nazionale di Geofisica e Vulcanologia, Sezione di Palermo, Palermo, Italy. - Dipartimento Chimica e Fisica della Terra ed Applicazioni, Palermo, Italy.
    Description: Published
    Description: L07619
    Description: partially_open
    Keywords: Submarine degassing ; magmatic fluids ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.04. Thermodynamics ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring ; 05. General::05.02. Data dissemination::05.02.01. Geochemical data ; 04. Solid Earth::04.08. Volcanology::04.08.08. Volcanic risk
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  • 24
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    Evidence of deep magma degassing and ascent by geochemistry of peripheral gas emissions at Mount Etna (Italy): Assessment of the magmatic reservoir pressure (2005)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: Five gas discharges in the area of Mount Etna volcano (Italy) and in the near Hyblean plateau have been monitored since 1996. All the emissions displayed low contributions from crustal fluids, whereas magmatic gases were the main component. Selective dissolution of these gases into hydrothermal aquifers has been recognized and modeled, allowing us to calculate the original composition of the magma-released gases. The inferred composition of the magmatic gases exhibits synchronous variations of He/Ne and He/CO2 ratios, which are coherent with the magma degassing process. On the basis of numerical simulations of volatile degassing from Etnean basalts we have computed the initial and final pressures of the magma batches feeding the emissions. We thus can define the levels of the Etna plumbing system where magmas are stored. Pressure values were around 360 and 160 MPa for initial and final stages, respectively, meaning related depths of about 10 and 3 km below sea level, matching those obtained by geophysical investigations for the deep and shallow magma reservoirs. In addition, we have been able to recognize episodes of magma migration from the deeper reservoir toward the shallow one. An important magma injection into the shallow storage volume was detected during the onset of the 2001 eruption (17 July). No further injection had taken place during this period until September 2001, providing a possible reason for the quick exhaustion of the eruption. In view of this we suggest that the sampled emissions are a powerful geochemical tool to investigate the Etna’s plumbing system and its magma dynamics, as well as the development of eruptive events.
    Description: Published
    Description: 2463
    Description: partially_open
    Keywords: gas geochemistry ; magma degassing ; modeling ; 04. Solid Earth::04.04. Geology::04.04.12. Fluid Geochemistry ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.03. Magmas ; 04. Solid Earth::04.08. Volcanology::04.08.04. Thermodynamics ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring
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  • 25
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    Mount Etna: Geochemical signals of magma ascent and unusually extensive plumbing system (2005)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: Five years of gas monitoring from selected sites suggest that Mt Etna’s plumbing system is much more extensive than previously reported. It extends at least 40 km SW from the volcano’s boundary along the NE-SW regional fault, where it discharges about 200 tons/day of gas, containing helium with mantle-type isotopic composition. Synchronous variations of 3He/4He isotopic ratios in gas sampled at sites located 60 kilometers apart have allowed us to detect pulses of ascending magma in the plumbing system, thus providing a powerful tool for eruption forecasting. Following summer 2001 eruption, the still increasing trend of the 3He/4He ratios indicates that magma storage is even now occurring at a shallow depth. Hence, the volcano maintains a high capacity to re-erupt within the next few months.
    Description: Published
    Description: 1057
    Description: partially_open
    Keywords: helium isotopes ; geochemical monitoring ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.03. Magmas ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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  • 26
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    Link between major flank slip and 2002–2003 eruption at Mt. Etna (Italy) (2008)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: The 2002–2003 Etna eruption is studied through earthquake distributions and surface fracturing. In September 2002, earthquake-induced surface rupture (sinistral offset 0.48 m) occurred along the E-W striking Pernicana Fault (PF), on the NE flank. In late October, a flank eruption accompanied further ( 0.77 m) surface rupturing, reaching a total sinistral offset of 1.25 m; the deformation then propagated for 18 km eastwards to the coastline (sinistral offset 0.03 m) and southwards, along the NW-SE striking Timpe (dextral offset 0.04 m) and, later, Trecastagni faults (dextral offset 0.035 m). Seismicity (〈4 km bsl) on the E flank accompanied surface fracturing: fault plane solutions indicate an overall ESEWNWextension direction, consistent with ESE slip of the E flank also revealed by ground fractures. A three-stage model of flank slip is proposed: inception (September earthquake), climax (accelerated slip and eruption) and propagation (E and S migration of the deformation).
    Description: Published
    Description: 2286
    Description: 1.5. TTC - Sorveglianza dell'attività eruttiva dei vulcani
    Description: 3.2. Tettonica attiva
    Description: 3.5. Geologia e storia dei sistemi vulcanici
    Description: 3.6. Fisica del vulcanismo
    Description: 4.3. TTC - Scenari di pericolosità vulcanica
    Description: JCR Journal
    Description: reserved
    Keywords: volcano seismology ; surface fracturing ; flank slip ; eruption ; Etna ; 04. Solid Earth::04.01. Earth Interior::04.01.99. General or miscellaneous ; 04. Solid Earth::04.01. Earth Interior::04.01.02. Geological and geophysical evidences of deep processes ; 04. Solid Earth::04.02. Exploration geophysics::04.02.99. General or miscellaneous ; 04. Solid Earth::04.04. Geology::04.04.99. General or miscellaneous ; 04. Solid Earth::04.04. Geology::04.04.09. Structural geology ; 04. Solid Earth::04.06. Seismology::04.06.99. General or miscellaneous ; 04. Solid Earth::04.06. Seismology::04.06.01. Earthquake faults: properties and evolution ; 04. Solid Earth::04.06. Seismology::04.06.02. Earthquake interactions and probability ; 04. Solid Earth::04.06. Seismology::04.06.08. Volcano seismology ; 04. Solid Earth::04.06. Seismology::04.06.11. Seismic risk ; 04. Solid Earth::04.07. Tectonophysics::04.07.99. General or miscellaneous ; 04. Solid Earth::04.07. Tectonophysics::04.07.02. Geodynamics ; 04. Solid Earth::04.07. Tectonophysics::04.07.05. Stress ; 04. Solid Earth::04.07. Tectonophysics::04.07.07. Tectonics ; 04. Solid Earth::04.08. Volcanology::04.08.99. General or miscellaneous ; 04. Solid Earth::04.08. Volcanology::04.08.03. Magmas ; 04. Solid Earth::04.08. Volcanology::04.08.05. Volcanic rocks ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring ; 04. Solid Earth::04.08. Volcanology::04.08.08. Volcanic risk ; 05. General::05.02. Data dissemination::05.02.03. Volcanic eruptions
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  • 27
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    Scanning tomography of SO2 distribution in a volcanic gas plume (2008)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: Two-dimensional cross sections of the sulphur dioxide (SO2) distribution in the volcanic gas plume of Mt. Etna were reconstructed using tomographic techniques. The data for these projections were generated by a network of five automated scanning spectrometers, positioned on the flanks of the volcano. These measure slant-column amounts of SO2 at 105 different angles, every four minutes. Stable wind conditions allow the plume to be monitored on 82% of days. A time-series of plume cross sections was computed, revealing the potential of this method to track variations in plume position and structure on timescales of minutes to hours, a result of potential importance for air traffic and civil defence in case of eruption, when copious amounts of fine ash can be transported.
    Description: Published
    Description: L17811
    Description: 1.2. TTC - Sorveglianza geochimica delle aree vulcaniche attive
    Description: JCR Journal
    Description: reserved
    Keywords: tomography ; SO2 ; DOAS ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring ; 04. Solid Earth::04.08. Volcanology::04.08.07. Instruments and techniques
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  • 28
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    Noble gas solubility in silicate melts:a review of experimentation and theory, and implications regarding magma degassing processes (2006)
    INGV
    Details
    Publication Date: 2019-11-04
    Description: Noble gas solubility in silicate melts and glasses has gained a crucial role in Earth Sciences investigations and in the studies of non-crystalline materials on a micro to a macro-scale. Due to their special geochemical features, noble gases are in fact ideal tracers of magma degassing. Their inert nature also allows them to be used to probe the structure of silicate melts. Owing to the development of modern high pressure and temperature technologies, a large number of experimental investigations have been performed on this subject in recent times. This paper reviews the related literature, and tries to define our present state of knowledge, the problems encountered in the experimental procedures and the theoretical questions which remain unresolved. Throughout the manuscript I will also try to show how the thermodynamic and structural interpretations of the growing experimental dataset are greatly improving our understanding of the dissolution mechanisms, although there are still several points under discussion. Our improved capability of predicting noble gas solubilities in conditions closer to those found in magma has allowed scientists to develop quantitative models of magma degassing, which provide constraints on a number of questions of geological impact. Despite these recent improvements, noble gas solubility in more complex systems involving the main volatiles in magmas, is poorly known and a lot of work must be done. Expertise from other fields would be extremely valuable to upcoming research, thus focus should be placed on the structural aspects and the practical and commercial interests of the study of noble gas solubility.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: noble gases ; solubility ; degassing ; silicate melts ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases
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  • 29
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    A model of sulphur solubility for hydrous mafic melts: application to the determination of magmatic fluid compositions of Italian volcanoes (2006)
    INGV
    Details
    Publication Date: 2019-11-04
    Description: We present an empirical model of sulphur solubility that allows us to calculate f S2 if P, T, fO2 and the melt composition, including H2O and S, are known. The model is calibrated against three main experimental data bases consisting in both dry and hydrous silicate melts. Its prime goal is to calculate the f S2 of hydrous basalts that currently lack experimental constraints of their sulphur solubility behaviour. Application of the model to Stromboli, Vesuvius, Vulcano and Etna eruptive products shows that the primitive magmas found at these volcanoes record f S2 in the range 0.1-1 bar. In contrast, at all volcanoes the magmatic evolution is marked by dramatic variations in f S2 that spreads over up to 9 orders of magnitude. The f S2 can either increase during differentiation or decrease during decompression to shallow reservoirs, and seems to be related to closed versus open conduit conditions, respectively. The calculated f S2 shows that the Italian magmas are undersaturated in a FeS melt, except during closed conduit conditions, in which case differentiation may eventually reach conditions of sulphide melt saturation. The knowledge of f S2, fO2 and fH2O allows us to calculate the fluid phase composition coexisting with magmas at depth in the C-O-H-S system. Calculated fluids show a wide range in composition, with CO2 mole fractions of up to 0.97. Except at shallow levels, the fluid phase is generally dominated by CO2 and H2O species, the mole fractions of SO2 and H2S rarely exceeding 0.05 each. The comparison between calculated fluid compositions and volcanic gases shows that such an approach should provide constraints on both the depth and mode of degassing, as well as on the amount of free fluid in magma reservoirs. Under the assumption of a single step separation of the gas phase in a closed-system condition, the application to Stromboli and Etna suggests that the main reservoirs feeding the eruptions and persistent volcanic plumes at these volcanoes might contain as much as 5 wt% of a free fluid phase. Consideration of the magma budget needed to balance the amounts of volatiles emitted in the light of these results shows that the amount of nonerupted magma could be overestimated by as much as one order of magnitude.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: sulphur ; hydrous basalts ; volcanic gas ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.03. Magmas ; 04. Solid Earth::04.08. Volcanology::04.08.07. Instruments and techniques
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    Volatile diffusion in silicate melts and its effects on melt inclusions (2006)
    INGV
    Details
    Publication Date: 2019-11-04
    Description: A compendium of diffusion measurements and their Arrhenius equations for water, carbon dioxide, sulfur, fluorine, and chlorine in silicate melts similar in composition to natural igneous rocks is presented. Water diffusion in silicic melts is well studied and understood, however little data exists for melts of intermediate to basic compositions. The data demonstrate that both the water concentration and the anhydrous melt composition affect the diffusion coefficient of water. Carbon dioxide diffusion appears only weakly dependent, at most, on the volatilefree melt composition and no effect of carbon dioxide concentration has been observed, although few experiments have been performed. Based upon one study, the addition of water to rhyolitic melts increases carbon dioxide diffusion by orders of magnitude to values similar to that of 6 wt% water. Sulfur diffusion in intermediate to silicic melts depends upon the anhydrous melt composition and the water concentration. In water-bearing silicic melts sulfur diffuses 2 to 3 orders of magnitude slower than water. Chlorine diffusion is affected by both water concentration and anhydrous melt composition; its values are typically between those of water and sulfur. Information on fluorine diffusion is rare, but the volatile-free melt composition exerts a strong control on its diffusion. At the present time the diffusion of water, carbon dioxide, sulfur and chlorine can be estimated in silicic melts at magmatic temperatures. The diffusion of water and carbon dioxide in basic to intermediate melts is only known at a limited set of temperatures and compositions. The diffusion data for rhyolitic melts at 800°C together with a standard model for the enrichment of incompatible elements in front of growing crystals demonstrate that rapid crystal growth, greater than 10-10 ms-1, can significantly increase the volatile concentrations at the crystal-melt interface and that any of that melt trapped by the formation of melt inclusions may not be representative of the bulk melt. However, basaltic melt inclusions trapped at 1300°C are more likely to contain bulk melt concentrations of water and carbon dioxide.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: diffusion ; silicate melts ; volatiles ; water ; carbon dioxide ; sulfur ; fluorine ; igneous processes ; chlorine ; melt inclusion ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.03. Magmas
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    Constraining the dynamics of volcanic eruptions by characterization of pumice textures (2006)
    INGV
    Details
    Publication Date: 2019-11-04
    Description: We have characterized the textures of pumice clasts from Phlegraean Fields to gain insights into the conduit flow-dynamics of alkaline explosive eruptions. Vesicularities, vesicle number densities, and vesicle sizes and shapes were measured to obtain the bulk and groundmass properties of the juvenile fraction of Campanian Ignimbrite (CI) and Agnano Monte Spina (AMS) eruptions. The results report the coexistence of three end-member pumice types in the deposits of both eruptions, 1) microvesicular, 2) tube and 3) expanded, which differ according to clast morphology and the macro- to microscopic vesicle texture. Vesicularities (0.85-0.94 for CI, 0.51-0.91 for AMS) and vesicle number densities (2-4×105 cm-2 in CI, 3×105-106 cm-2 in AMS) span quite a wide range in all the three pumice types. Overall, tube pumices exhibit the highest bulk (0.89) and groundmass (CI 0.85, AMS 0.82) average vesicle volume fractions but the lowest average vesicle number densities (CI 2×105, AMS 4×105 cm-2). Comparison with textures of calc-alkaline pumices has revealed many similarities and points to a common origin and distribution of the products from both magma compositions within the volcanic conduit. In addition, the results of the textural analysis were interpreted in the light of the conduit flow modeling of Phlegraean Fields eruptions. The comparison of textural observations with results from simulations of conduit magma ascent has exhibited a good agreement between measured and numerically calculated vesicularities for both compositions, helping to constrain the overall dynamics of alkaline versus calc-alkaline eruptions.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: Phlegraean Fields ; Plinian eruptions ; vesicle textures ; magma ascent dynamics ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.05. Volcanic rocks ; 04. Solid Earth::04.08. Volcanology::04.08.07. Instruments and techniques
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    Determination of volatiles in volcanic rocks and minerals with a Directly Coupled Evolved Gas Analyzing System (DEGAS) -Part I: Interpretation of degassing profiles (DEGAS-profiles) of minerals and rocks on the basis of melting experiments (2006)
    INGV
    Details
    Publication Date: 2019-11-04
    Description: Volatile components in magma strongly influence many physical properties of melts and minerals. The temperature resolved degassing analysis of volcanic crystalline and vitreous rocks gives detailed information about volatile compounds in the melt. Aspecial high-temperature mass-spectrometry device in combination with a thermo-balance allows a quantitative determination of different volatile species. It enables a differentiation between the primary gas content in the magma and the gas released from decomposition of secondary alteration products. The gas release profiles give the following indications: i) during the littoral explosions of Pahoehoe lava the content of volatiles is not changed by interaction with air or sea water; ii) the degassing profiles of vitreous black sand verify the primary content of volatiles in the erupted melt, only CO2 was detected; iii) the oxygen release profile gives significant indications for oxygen undersaturation of the erupted magma; iv) remelting of black sand in air at 1450°C for 0.45 h causes an oxygen saturation of the basaltic melt; v) remelting of black sand in argon atmosphere confirms the oxygen undersaturation of the melt; vi) remelting of black sand-black shale mixtures affects a significant change in the degassing profiles, especially in CO2-release. With the first investigations we can demonstrate that gas release curves of volcanic rocks are qualified for a) detection of the primary gas content of erupted magma; b) detection of alteration processes of the igneous glass; c) detection of contamination of the magma with adjacent rocks.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: volatiles ; magmatic rocks ; basaltic glass ; degassing ; Hawaiian lava ; remelting ; blacksand ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.03. Magmas
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    Geochemical modeling of magmatic gas scrubbing (2006)
    INGV
    Details
    Publication Date: 2019-11-04
    Description: The EQ3/6 software package, version 7.2 was successfully used to model scrubbing of magmatic gas by pure water at 0.1 MPa, in the liquid and liquid-plus-gas regions. Some post-calculations were necessary to account for gas separation effects. In these post-calculations, redox potential was considered to be fixed by precipitation of crystalline a-sulfur, a ubiquitous and precocious process. As geochemical modeling is constrained by conservation of enthalpy upon water-gas mixing, the enthalpies of the gas species of interest were reviewed, adopting as reference state the liquid phase at the triple point. Our results confirm that significant emissions of highly acidic gas species (SO2(g), HCl(g), and HF(g)) are prevented by scrubbing, until dry conditions are established, at least locally. Nevertheless important outgassing of HCl(g) can take place from acid, HCl-rich brines. Moreover, these findings support the rule of thumb which is generally used to distinguish SO2-, HCl-, and HF-bearing magmatic gases from SO2-, HCl-, and HF-free hydrothermal gases.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: magmatic gas ; magma degassing ; hydrothermalsystem ; crater lake ; meteoric water ; scrubbing ; reaction path modeling ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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    Novel laser-based techniques for monitoring of volcanoes (2006)
    INGV
    Details
    Publication Date: 2019-11-04
    Description: An overview of novel laser techniques suitable for volcanic monitoring, based on different kinds of infrared laser sources, is presented. Their main advantages and drawbacks are discussed focusing on the achievable sensitivity and precision levels in analysis of gaseous species. Some of the most recent experimental results obtained in laboratory development as well as in field tests of home-built laser spectrometers are reported. New perspectives in optical devices aimed at geochemical and geophysical applications are also considered.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: diode laser ; absorption spectroscopy ; optical fiber ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.07. Instruments and techniques
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    Vapour-phase crystallisation of silica from SiF4-bearing volcanic gases (2006)
    INGV
    Details
    Publication Date: 2019-11-04
    Description: Thermodynamic modelling of magmatic gases shows that SiF4 may be an important F-bearing species at the high pressures typical of magma reservoirs. Upon decompression during degassing, SiF4 will react with water vapour to form HF and silica. Common magmatic gases of high-T fumaroles seem to contain too little SiF4 to be a significant source of silica, except if extremely large amounts of gas percolate through a small volume of rock, as is the case in lava domes. Only if fluorine contents of the gases exceed 1 mol% detectable amounts of silica may be formed, but such high fluorine contents have not yet been observed in natural gases. Alternatively, silica may be formed by heating of cool SiF4-rich gases circulating in cooling lava bodies. We suggest that these mechanisms may be responsible for the deposition of crystalline silica, most probably cristobalite, observed in vesicles in lavas from Lewotolo volcano (Eastern Sunda Arc, Indonesia). Silica occurs as vapour-crystallised patches in vesicles, and is sometimes associated with F-phlogopite, which further supports F-rich conditions during deposition. Because of the connection between F-rich conditions and high-K volcanism, we propose that late-stage gaseous transport and deposition of silica may be more widespread in K-rich volcanoes than elsewhere, and long-term exposure to ash from eruptions of such volcanoes could therefore carry an increased risk for respiratory diseases. The dependence of SiF4/HF on temperature reported here differs from the current calibration used for temperature measurements of fumarolic gases by remote sensing techniques, and we suggest an updated calibration.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: SiF4 ; vapour crystallisation ; silica ; degassing ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.04. Thermodynamics
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    Numerical model of gas dispersion emitted from volcanic sources (2006)
    INGV
    Details
    Publication Date: 2019-11-04
    Description: An Eulerian model for passive gas dispersion based on the K-theory for turbulent diffusion, coupled with a mass consistent wind model is presented. The procedure can be used to forecast gas concentration over large and complex terrains. The input to the model includes the topography, wind measurements from meteorological stations, atmospheric stability information and gas flow rate from the ground sources. Here, this model is applied to study the distribution of the CO2 discharged from the hot sources of the Solfatara Volcano, Naples, Italy, where the input data were measured during a 15 day campaign in June 2001 carried out to test an Eddy Covariance (EC) station by Osservatorio Vesuviano-INGV, Naples.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: gas dispersion ; volcanic gas ; K-theory ; computer model ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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    Assessment of motion-induced fluidization of dense pyroclastic gravity currents (2006)
    INGV
    Details
    Publication Date: 2019-11-04
    Description: The paper addresses some fundamental aspects of the dynamics of dense granular flows down inclines relevant to pyroclastic density currents. A simple mechanistic framework is presented to analyze the dynamics of the frontal zone, with a focus on the establishment of conditions that promote air entrainment at the head of the current and motion-induced self-fluidization of the flow. The one-dimensional momentum balance on the current along the incline is considered under the hypothesis of strongly turbulent flow and pseudo-homogeneous behaviour of the two-phase gas-solid flow. Departures from one-dimensional flow in the frontal region are also analyzed and provide the key to the assessment of air cross-flow and fluidization of the solids in the head of the current. The conditions for the establishment of steady motion of pyroclastic flows down an incline, in either the fluidized or «dry» granular states, are examined.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: pyroclastic flow ; fluidization ; gravity current ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases
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    Measurements of 220Rn and 222Rn and CO2 emissions in soil and fumarole gases on Mt. Etna volcano (Italy): Implications for gas transport and shallow ground fracture (2008)
    American Geophysical Union
    Details
    Publication Date: 2020-02-24
    Description: Measurements of 220Rn and 222Rn activity and of CO2 flux in soil and fumaroles were carried out on Mount Etna volcano in 2005–2006, both in its summit area and along active faults on its flanks. We observe an empirical relationship between (220Rn/222Rn) and CO2 efflux. The higher the flux of CO2, the lower the ratio between 220Rn and 222Rn. Deep sources of gas are characterized by high 222Rn activity and high CO2 efflux, whereas shallow sources are indicated by high 220Rn activity and relatively low CO2 efflux. Excess 220Rn highlights sites of ongoing shallow rock fracturing that could be affected by collapse, as in the case of the rim of an active vent. Depletion both in 220Rn and in CO2 seems to be representative of residual degassing along recently active eruptive vents.
    Description: This work was funded by the Istituto Nazionale di Geofisica e Vulcanologia (S.G., M.N.) and by the Dipartimento per la Protezione Civile (Italy), projects V3_6/28-Etna (M.N.) and V5/08-Diffuse degassing in Italy (S.G.), and NSF EAR 063824101 (K.W.W.S.).
    Description: Published
    Description: Q10001
    Description: 1.2. TTC - Sorveglianza geochimica delle aree vulcaniche attive
    Description: 4.5. Degassamento naturale
    Description: JCR Journal
    Description: reserved
    Keywords: radon ; thoron ; carbon dioxide ; rock stress ; gas transport ; Mount Etna ; 04. Solid Earth::04.08. Volcanology::04.08.99. General or miscellaneous ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring ; 05. General::05.02. Data dissemination::05.02.01. Geochemical data
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    Thermo-rheological magma control on the impact of highly fluid lava flows at Mt. Nyiragongo (2007)
    American Geophysical Union
    Details
    Publication Date: 2020-05-29
    Description: In January 2002 Mount Nyiragongo erupted foiditic lavas that covered the Southern volcano flank devastating vast urban areas. Lava flows originated from vents at different heights on the eruptive fissure displayed different velocities, from tens of km/h at the highest vents to slow-advance (0.1–1 km/h) in Goma town several km away from the volcano. To understand the different behavior of lava flows and their threat to the local population, we undertook a multidisciplinary study involving textural and rheological measurements and numerical simulations of heat transfer during magma ascent. We demonstrate that pre-eruptive cooling and syn-eruptive undercooling of magma determined the different rheological behavior of lava flows erupted from vents at diverse heights. Venting at lower altitudes is expected to produce viscous, slowly advancing lavas, although development of fluid, faster flows should be included among possible future eruptive scenarios.
    Description: Published
    Description: L06301
    Description: 3.6. Fisica del vulcanismo
    Description: JCR Journal
    Description: reserved
    Keywords: Nyiragongo volcano ; textural and rheological measurements ; numerical simulations ; 04. Solid Earth::04.08. Volcanology::04.08.99. General or miscellaneous
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    Formation processes of the 1909 Tarumai and the 1944 Usu lava domesin Hokkaido, Japan (2006)
    INGV
    Details
    Publication Date: 2019-11-04
    Description: The formation of the two particular lava domes in Hokkaido, Japan is described and interpreted mainly from geophysical viewpoints. The 1909 eruption of Tarumai volcano was not violent but produced a lava dome over four days. The growth rate of the dome is discussed under the assumption that the lava flow was viscous and plastic fluid during its effusion. By Hagen-Poiseuilles Law, the length of the conduit of the lava dome is rather ambiguously determined as a function of viscosity of the magma and diameter of the conduit. The 1944 Usu dome extruded as a parasitic cone of Usu volcano, not in the crater, but in a flat cornfield at the foot of the volcano. From the beginning to the end for more than 17 months, seismometric and geodetic observations of the dome activity were carried out by several pioneering geophysicists. Utilizing their data, pseudo growth curves of the dome at each stage can be drawn. The lava ascended rather uniformly, causing uplift of the ground surface until half-solidified lava reached the surface six months after the deformation began. Thereafter, the lava dome added lateral displacements and finally achieved its onion structure. These two lava domes are of contrasting character, one is andesitic and formed quickly while the other is dacitic and formed slowly, but both of them behaved as viscous and plastic flows during effusion. It is concluded that both the lava domes formed by uplift of magma forced to flow through the conduits, analogous to squeezing toothpaste out of a tube.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: lava domes ; Tarumai volcano ; Usu volcano ; squeeze of magma ; growth rate of domes ; Hagen-Poiseuille's Law ; 04. Solid Earth::04.08. Volcanology::04.08.99. General or miscellaneous
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    Acid-base properties and structons: towards a structural model for predicting the thermodynamic properties of silicate melts (2006)
    INGV
    Details
    Publication Date: 2019-11-04
    Description: Phase equilibrium relationships in igneous systems can be estimated using empirical mathematical models based on multi-component regular solution formulae. Although these provide useable results within the fitted region, they can give very misleading values outside the compositional range of curve fitting. Moreover, they usually give poor estimates of the well-characterized melting relations of simple systems and do not relate to the large body of thermodynamic activity data available in the metallurgical literature, nor to spectroscopic, diffraction or computational models of silicate melt properties. The aim of this paper is to extend previous acid-base models of silicate melts and to use a quasi-chemical model to calculate the activities of quasi-chemical silicate mixing units, or structons, from combinations of the oxo-species used in quasi-chemical and polymer models to calculate oxide activities in metallurgy.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: silicate melt ; acid-base ; oxide melt ; thermodynamic properties ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.04. Thermodynamics
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    Chemical interactions and configurational disorder in silicate melts (2006)
    INGV
    Details
    Publication Date: 2019-11-04
    Description: The Thermodynamics of quasi-chemical and polymeric models are briefly reviewed. It is shown that the two classes are mutually consistent, and that opportune conversion of the existing quasi-chemical parameterization of binary interactions in MO-SiO2 joins to polymeric models may be afforded without substantial loss of precision. It is then shown that polymeric models are extremely useful in deciphering the structural and reactive properties of silicate melts and glasses. They not only allow the Lux-Flood character of the dissolved oxides to be established, but also discriminate subordinate strain energy contributions to the Gibbs free energy of mixing from the dominant chemical interaction terms. This discrimination means that important information on the short-, medium- and long-range periodicity of this class of substances can be retrieved from thermodynamic analysis. Lastly, it is suggested that an important step forward in deciphering the complex topology of the inhomogeneity ranges observed at high SiO2 content can be performed by applying SCMF theory and, particularly, Matsen-Schick spectral analysis, hitherto applied only to rubberlike materials.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: silicate melts ; structure ; entropy ; unmixing ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.04. Thermodynamics
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    Polymerisation, basicity, oxidation state and their role in ionic modelling of silicate melts (2006)
    INGV
    Details
    Publication Date: 2019-11-04
    Description: In order to describe and quantify the reactivity of silicate melts, the ionic notation provided by the Temkin formalism has been historically accepted, giving rise to the study of melt chemical equilibria in terms of completely dissociated ionic species. Indeed, ionic modelling of melts works properly as long as the true extension of the anionic matrix is known. This information may be attained in the framework of the Toop-Samis (1962a,b) model, through a parameterisation of the acid-base properties of the dissolved oxides. Moreover, by combining the polymeric model of Toop and Samis with the «group basicity» concept of Duffy and Ingram (1973, 1974a,b, 1976) the bulk optical basicity (Duffy and Ingram, 1971; Duffy, 1992) of molten silicates and glasses can be split into two distinct contributions, i.e. the basicity of the dissolved basic oxides and the basicity of the polymeric units. Application to practical cases, such as the assessment of the oxidation state of iron, require bridging of the energetic gap between the standard state of completely dissociated component (Temkin standard state) and the standard state of pure melt component at P and T of interest. On this basis it is possible to set up a preliminary model for iron speciation in both anhydrous and hydrous aluminosilicate melts. In the case of hydrous melts, I introduce both acidic and basic dissociation of the water component, requiring the combined occurrence of H+ cations, OH- free anions and, to a very minor extent, of T-OH groups. The amphoteric behaviour of water revealed by this study is therefore in line with the earlier prediction of Fraser (1975).
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: polymerisation ; basicity ; oxidationstate ; water speciation ; Temkin model ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.04. Thermodynamics
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    Fe in magma - An overview (2006)
    INGV
    Details
    Publication Date: 2019-11-04
    Description: The strong influence of physical conditions during magma formation on Fe equilibria offers a large variety of possibilities to deduce these conditions from Fe-bearing phases and phase assemblages found in magmatic rocks. Conditions of magma genesis and their evolution are of major interest for the understanding of volcanic eruptions. A brief overview on the most common methods used is given together with potential problems and limitations. Fe equilibria are not only sensitive to changes in intensive parameters (especially T and fO2) and extensive parameters like composition also have major effects, so that direct application of experimentally calibrated equilibria to natural systems is not always possible. Best estimates for pre-eruptive conditions are certainly achieved by studies that relate field observations directly to experimental observations for the composition of interest using as many constraints as possible (phase stability relations, Fe-Ti oxides, Fe partitioning between phases, Fe oxidation state in glass etc.). Local structural environment of Fe in silicate melts is an important parameter that is needed to understand the relationship between melt transport properties and melt structure. Assignment of Fe co-ordination and its relationship to the oxidation state seems not to be straightforward. In addition, there is considerable evidence that the co-ordination of Fe in glass differs from that in the melt, which has to be taken into account when linking melt structure to physical properties of silicate melts at T and P.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: iron ; silicate melt ; redox conditions ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.03. Magmas ; 04. Solid Earth::04.08. Volcanology::04.08.04. Thermodynamics
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    Chlorine solubility in evolved alkaline magmas (2006)
    INGV
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    Publication Date: 2019-11-04
    Description: Experimental studies of Cl solubility in trachytic to phonolitic melts provide insights into the capacity of alkaline magmas to transport Cl from depth to the earths surface and atmosphere, and information on Cl solubility variations with pressure, temperature and melt or fluid composition is crucial for understanding the reasons for variations in Cl emissions at active volcanoes. This paper provides a brief review of Cl solubility experiments conducted on a range of trachytic to phonolitic melt compositions. Depending on the experimental conditions the melts studied were in equilibrium with either a Cl-bearing aqueous fluid or a subcritical assemblage of low- Cl aqueous fluid + Cl-rich brine. The nature of the fluid phase(s) was identified by examination of fluid inclusions present in run product glasses and the fluid bulk composition was calculated by mass balance. Chlorine concentrations in the glass increase with increasing Cl molality in the fluid phase until a plateau in Cl concentration is reached when melt coexists with aqueous fluid + brine. With fluids of similar Cl molality, higher Cl concentrations are observed in peralkaline phonolitic melts compared with peraluminous phonolitic melts; overall the Cl concentrations observed in phonolitic and trachytic melts are approximately twice those found in calcalkaline rhyolitic melts under similar conditions. The observed negative pressure dependence of Cl solubility implies that Cl contents of melts may actually increase during magma decompression if the magma coexists with aqueous fluid and Cl-rich brine (assuming melt-vapor equilibrium is maintained). The high Cl contents (approaching 1 wt% Cl) observed in some melts/glasses from the Vesuvius and Campi Flegrei areas suggest saturation with a Cl-rich brine prior to eruption.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: alkaline magmas ; solubility ; chlorine ; supercritical fluid ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.03. Magmas
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    Solubility of C-O-H mixturesin natural melts: new experimental data and application range of recent models (2006)
    INGV
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    Publication Date: 2019-11-04
    Description: The effect of pressure, temperature, and melt composition on CO2 and H2O solubilities in aluminosilicate melts, coexisting with CO2-H2O fluids, is discussed on the basis of previously published and new experimental data. The datasets have been chosen so that CO2 and H2O are the main fluid components and the conclusions are only valid for relatively oxidizing conditions. The most important parameters controlling the solubilities of H2O and CO2 are pressure and composition of melt and fluid. On the other hand, the effect of temperature on volatile solubilities is relatively small. At pressures up to 200 MPa, intermediate compositions such as dacite, in which both molecular CO2 and carbonate species can be dissolved, show higher volatile solubilities than rhyolite and basalt. At higher pressures (0.5 to 1 GPa), basaltic melts can incorporate higher amounts of carbon dioxide (by a factor of 2 to 3) than rhyolitic and dacitic melts. Henrian behavior is observed only for CO2 solubility in equilibrium with H2O-CO2 fluids at pressures 〈100 MPa, whereas at higher pressures CO2 solubility varies nonlinearly with CO2 fugacity. The positive deviation from linearity with almost constant CO2 solubility at low water activity indicates that dissolved water strongly enhances the solubility of CO2. Water always shows non-Henrian solubility behavior because of its complex dissolution mechanism (incorporation of OH-groups and H2O molecules in the melt). The model of Newman and Lowenstern (2002), in which ideal mixing between volatiles in both fluid and melt phases is assumed, reproduces adequately the experimental data for rhyolitic and basaltic compositions at pressures below 200 MPa but shows noticeable disagreement at higher pressures, especially for basalt. The empirical model of Liu et al. (2004) is applicable to rhyolitic melts in a wide range of pressure (0-500 MPa) and temperature (700- 1200°C) but cannot be used for other melt compositions. The thermodynamic approach of Papale (1999) allows to calculate the effect of melt composition on volatile solubilities but needs an update to account for more recent experimental data. A disadvantage of this model is that it is not available as a program code. The review indicates a crucial need of new experimental data for scarcely investigated field of pressures and fluid compositions and new models describing evident non-ideality of H-C-O fluid solubility in silicate melts at high pressures.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: CO2 ; H2O ; solubility ; mixed fluid ; silicate melt ; experimental data ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.03. Magmas
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    Numerical simulation of explosive volcanic eruptions from the conduit flow to global atmospheric scales (2006)
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    Publication Date: 2019-11-04
    Description: Volcanic eruptions are unsteady multiphase phenomena, which encompass many inter-related processes across the whole range of scales from molecular and microscopic to macroscopic, synoptic and global. We provide an overview of recent advances in numerical modelling of volcanic effects, from conduit and eruption column processes to those on the Earth s climate. Conduit flow models examine ascent dynamics and multiphase processes like fragmentation, chemical reactions and mass transfer below the Earth surface. Other models simulate atmospheric dispersal of the erupted gas-particle mixture, focusing on rapid processes occurring in the jet, the lower convective regions, and pyroclastic density currents. The ascending eruption column and intrusive gravity current generated by it, as well as sedimentation and ash dispersal from those flows in the immediate environment of the volcano are examined with modular and generic models. These apply simplifications to the equations describing the system depending on the specific focus of scrutiny. The atmospheric dispersion of volcanic clouds is simulated by ash tracking models. These are inadequate for the first hours of spreading in many cases but focus on long-range prediction of ash location to prevent hazardous aircraft - ash encounters. The climate impact is investigated with global models. All processes and effects of explosive eruptions cannot be simulated by a single model, due to the complexity and hugely contrasting spatial and temporal scales involved. There is now the opportunity to establish a closer integration between different models and to develop the first comprehensive description of explosive eruptions and of their effects on the ground, in the atmosphere, and on the global climate.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: numerical modeling ; explosive volcanic eruptions ; conduit flow ; multiphase flow simulation ; stratospheric sulfate aerosol ; 01. Atmosphere::01.01. Atmosphere::01.01.07. Volcanic effects ; 04. Solid Earth::04.08. Volcanology::04.08.99. General or miscellaneous ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases
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    Exploiting ground-based optical sensing technologies for volcanic gas surveillance (2006)
    INGV
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    Publication Date: 2019-11-04
    Description: Measurements of volcanic gas composition and flux are crucial to probing and understanding a range of magmatic, hydrothermal and atmospheric interactions. The value of optical remote sensing methods has been recognised in this field for more than thirty years but several recent developments promise a new era of volcanic gas surveillance. This could see much higher time- and space-resolved data-sets, sustained at individual volcanoes even during eruptive episodes. We provide here an overview of these optical methods and their application to ground-based volcano monitoring, covering passive and active measurements in the ultraviolet and infrared spectral regions. We hope thereby to promote the use of such devices, and to stimulate development of new optical techniques for volcanological research and monitoring.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: volcano monitoring ; volcano plumes ; IR and UV spectoscopy ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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    Isotopically light carbon dioxide in nitrogen rich gases: the gas distribution pattern in the French Massif Central, the Eifel and the western Eger Rift (2006)
    INGV
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    Publication Date: 2019-11-04
    Description: Based on characteristics of the distribution pattern of the western Eger Rift spring gases, a distribution pattern is presented for the gases of the French Massif Central. The central parts of these areas with ascending magmatic CO2 are characterised by high gas fluxes, high CO2 contents of up to 99.99 vol% and isotopially heavy CO2. In the peripheries, the decrease of d13C values of CO2 and CO2 contents in the gas phase is compensated by a rise in N2 contents. It can be demonstrated that gas fractionation in contrary to mixtures with isotopically light biogenic or crustal CO2 controls the distribution pattern of gas composition and isotopic composition of CO2 in these spring gases. Dissolution of CO2 results in formation of HCO3 causing isotope fractionation of CO2 and an enrichment of N2 in the gas phase. With multiple equilibrations, values of about 17 or lower are obtained. The scale of gas alteration depends on the gas flux and the gas-water ratios respectively and can result in N2-rich gases. Essential for the interpretation are gas flux measurements with mass balances derived for most of the springs. Without such mass balances it is not possible to discriminate between mixture and fractionation. The processes of isotopic and chemical solubility fractionations evidently control the gas distribution pattern in other regions as well.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: Eger Rift ; French Massif Central ; Eifel ; carbon dioxide ; gas fractionation ; isotope composition ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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    Radon, water chemistry and pollution check by volatile organic compounds in springs around Popocatepetl volcano, Mexico (2006)
    INGV
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    Publication Date: 2019-11-04
    Description: Popocatepetl volcano is a high-risk active volcano in Central Mexico where the highest population density in the country is settled. Radon in the soil and groundwater together with water chemistry from samples of nearby springs were analysed as a function of the 2002-2003 volcanic activity. The measurements of soil radon indicated fluctuations related to both the meteorological and sporadic explosive events. Groundwater radon showed essential differences in concentration due to the specific characteristics of the studied springs. Water chemistry showed also stability along the monitoring period. No anthropogenic pollution from Volatile Organic Compounds (VOCs) was observed. An overview of the soil radon behaviour as a function of the volcanic activity in the period 1994-2002 is also discussed.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: soil radon ; water chemistry ; volcanic activity ; 04. Solid Earth::04.08. Volcanology::04.08.99. General or miscellaneous
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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    Gas radon emission related to geodynamic activity on Mt. Etna (2006)
    INGV
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    Publication Date: 2019-11-04
    Description: We report preliminary observations on possible correlations between anomalies of subsoil radon concentration and geodynamical events on Mt. Etna. In recent years several studies have been carried out on radon as a precursor of geophysical events, most of them performed either on tectonic or volcanic areas. The peculiarity of our investigation lies on the choice of the etnean region, in which tectonic and volcanic features are both present. In order to characterize Mt. Etna features by investigating radon gas in soil, two stations were located along the NE-SW direction on Mt. Etna. Each of the two stations is fitted with a radon detector, a 3D seismic station and a meteorological station. Differences in the radon concentration trend in the data from north and south flanks could be linked to different faulting mechanisms and then to different mechanisms of radon uprising. The increase in soil radon concentration could be related to both seismic and volcanic events.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: radon ; geodynamical precursor ; Mt. Etna ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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    The November 2002 degassing event at Panarea Island (Italy): five months of geochemical monitoring (2006)
    INGV
    Details
    Publication Date: 2024-05-09
    Description: On 3rd November 2002, at about 3 km off-shore of Panarea Island (Aeolian Islands, Southern Italy), a series of gas vents suddenly and violently opened from the seafloor at the depth of 10-15 m, with an unusually high gas flux and superimposing on the already existing submarine fumarolic field. Starting from the 12th November 2002 a discontinuous geochemical monitoring program was carried out. The emissions consisted in an emulsion whose liquid phase derived from condensation of an uprising vapor phase occurring close to the fluid outlets without significant contamination by seawater. The whole composition of the fluids was basically H2O- and CO2-dominated, with minor amounts of typical «hydrothermal» components (such as H2S, H2, CO and light hydrocarbons), atmospheric-related compounds, and characterized by the occurrence of a significant magmatic gas fraction (mostly represented by SO2, HCl and HF). According to the observed temporal variability of the fluid compositions, between November and December 2002 the hydrothermal feeding system was controlled by oxidizing conditions due to the input of magmatic gases. The magmatic degassing phenomena showed a transient nature, as testified by the almost complete disappearance of the magmatic markers in a couple of months and by the restoration, since January 2003, of the chemical features of the existing hydrothermal system. The most striking feature of the evolution of the «Panarea degassing event» was the relatively rapid restoration of the typical reducing conditions of a stationary hydrothermal system, in which the FeO/Fe1.5O redox pair of the rock mineral phases has turned to be the dominating redox controlling system.
    Description: Published
    Description: JCR Journal
    Description: open
    Keywords: Aeolian Islands ; Panarea ; submarine fumaroles ; gas chemistry ; geochemical monitoring ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring
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