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  • 551.9  (18)
  • ddc:320  (17)
  • English  (35)
  • Romanian
  • 2020-2022  (35)
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  • 1
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    Evolution of Magmatism in the New Hebrides Island Arc and in Initial Back-Arc Rifting, SW Pacific (2021)
    Details
    Publication Date: 2021-07-26
    Description: We present new geochemical and isotopic data for rock samples from two island arc volcanoes, Erromango and Vulcan Seamount, and from a 500 m thick stratigraphic profile of lava flows exposed on the SW flank of Vate Trough back-arc rift of the New Hebrides Island Arc (NHIA). The basalts from the SW rift flank of Vate Trough have ages of ~0.5 Ma but are geochemically similar to those erupting along the active back-arc rift. The weak subduction component in the back-arc basalts implies formation by decompression melting during early rifting and rifting initiation by tectonic processes rather than by lithosphere weakening by arc magma. Melting beneath Vate Trough is probably caused by chemically heterogeneous and hot mantle that flows in from the North Fiji Basin in the east. The melting zone beneath Vate Trough back-arc is separate from that of the arc front, but a weak slab component suggests fluid transport from the slab. Immobile incompatible element ratios in South NHIA lavas overlap with those of the Vate Trough depleted back-arc basalts, suggesting that enriched mantle components are depleted by back-arc melting during mantle flow. The slab component varies from hydrous melts of subducted sediments in the Central NHIA to fluids from altered basalts in the South NHIA. The volcanism of Erromango shows constant compositions for 5 million years, that is, there is no sign for variable depletion of the mantle or for a change of slab components due to collision of the D'Entrecasteaux Ridge as in lava successions further north.
    Keywords: 551.9 ; subduction zone ; back-arc basalt ; sediment subduction
    Language: English
    Type: article
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  • 2
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    Sampling soil water along the pF curve for δ2H and δ18O analysis (2021)
    Details
    Publication Date: 2021-07-23
    Description: Soil water stable isotopes are widely used across disciplines (e.g., hydrology, ecology, soil science, and biogeochemistry). However, the full potential of stables isotopes as a tool for characterizing the origin, flow path, transport processes and residence times of water in different eco-, hydro-, and geological compartments has not yet been exploited. This is mainly due to the large variety of different methods for pore water extraction. While recent work has shown that matric potential affects the equilibrium fractionation, little work has examined how different water retention characteristics might affect the sampled water isotopic composition. Here, we present a simple laboratory experiment with two well-studied standard soils differing in their physico-chemical properties (e.g., clayey loam and silty sand). Samples were sieved, oven-dried and spiked with water of known isotopic composition to full saturation. For investigating the effect of water retention characteristics on the extracted water isotopic composition, we used pressure extractors to sample isotopically labelled soil water along the pF curve. After pressure extraction, we further extracted the soil samples via cryogenic vacuum extraction. The null hypothesis guiding our work was that water held at different tensions shows the same isotopic composition. Our results showed that the sampled soil water differed isotopically from the introduced isotopic label over time and sequentially along the pF curve. Our and previous studies suggest caution in interpreting isotope results of extracted soil water and a need to better characterize processes that govern isotope fractionation with respect to soil water retention characteristics. In the future, knowledge about soil water retention characteristics with respect to soil water isotopic composition could be applied to predict soil water fractionation effects under natural and non-stationary conditions. In this regard, isotope retention characteristics as an analog to water retention characteristics have been proposed as a way forward since matric potential affects the equilibrium fractionation between the bound water and the water vapour.
    Keywords: 551.9 ; pF value ; soil water isotopes ; soil water pool ; δ2H and δ18O analysis
    Language: English
    Type: article
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  • 3
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    Cryptic metasomatic agent measured in situ in Variscan mantle rocks: Melt inclusions in garnet of eclogite, Granulitgebirge, Germany (2021)
    Details
    Publication Date: 2021-07-26
    Description: Garnet of eclogite (formerly termed garnet clinopyroxenite) hosted in lenses of orogenic garnet peridotite from the Granulitgebirge, NW Bohemian Massif, contains unique inclusions of granitic melt, now either glassy or crystallized. Analysed glasses and re-homogenized inclusions are hydrous, peraluminous, and enriched in highly incompatible elements characteristic of the continental crust such as Cs, Li, B, Pb, Rb, Th, and U. The original melt thus represents a pristine, chemically evolved metasomatic agent, which infiltrated the mantle via deep continental subduction during the Variscan orogeny. The bulk chemical composition of the studied eclogites is similar to that of Fe-rich basalt and the enrichment in LILE and U suggest a subduction-related component. All these geochemical features confirm metasomatism. In comparison with many other garnet+clinopyroxene-bearing lenses in peridotites of the Bohemian Massif, the studied samples from Rubinberg and Klatschmühle are more akin to eclogite than pyroxenites, as reflected in high jadeite content in clinopyroxene, relatively low Mg, Cr, and Ni but relatively high Ti. However, trace elements of both bulk rock and individual mineral phases show also important differences making these samples rather unique. Metasomatism involving a melt requiring a trace element pattern very similar to the composition reported here has been suggested for the source region of rocks of the so-called durbachite suite, that is, ultrapotassic melanosyenites, which are found throughout the high-grade Variscan basement. Moreover, the Th, U, Pb, Nb, Ta, and Ti patterns of these newly studied melt inclusions (MI) strongly resemble those observed for peridotite and its enclosed pyroxenite from the T-7 borehole (Staré, České Středhoři Mountains) in N Bohemia. This suggests that a similar kind of crustal-derived melt also occurred here. This study of granitic MI in eclogites from peridotites has provided the first direct characterization of a preserved metasomatic melt, possibly responsible for the metasomatism of several parts of the mantle in the Variscides.
    Keywords: 551.9 ; clinopyroxenite ; eclogite ; melt inclusions ; metasomatism ; orogenic peridotite
    Language: English
    Type: article
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  • 4
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    The Preparation and Preliminary Characterisation of Three Synthetic Andesite Reference Glass Materials (ARM-1, ARM-2, ARM-3) for In Situ Microanalysis (2021)
    Details
    Publication Date: 2021-07-27
    Description: Three synthetic reference glasses were prepared by directly fusing and stirring 3.8 kg of high-purity oxide powders to provide reference materials for microanalytical work. These glasses have andesitic major compositions and are doped with fifty-four trace elements in nearly identical abundance (500, 50, 5 µg g−1) using oxide powders or element solutions, and are named ARM-1, 2 and 3, respectively. We further document that sector-field (SF) ICP-MS (Element 2 or Element XR) is capable of sweeping seventy-seven isotopes (from 7Li to 238U, a total of sixty-eight elements) in 1 s and, thus, is able to quantify up to sixty-eight elements by laser sampling. Micro- and bulk analyses indicate that the glasses are homogeneous with respect to major and trace elements. This paper provides preliminary data for the ARM glasses using a variety of analytical techniques (EPMA, XRF, ICP-OES, ICP-MS, LA-Q-ICP-MS and LA-SF-ICP-MS) performed in ten laboratories. Discrepancies in the data of V, Cr, Ni and Tl exist, mainly caused by analytical limitations. Preliminary reference and information values for fifty-six elements were calculated with uncertainties [2 relative standard error (RSE)] estimated in the range of 1–20%.
    Keywords: 551.9 ; glass reference materials ; microanalysis ; sector-field ICP-MS ; LA-ICP-MS ; multiple-element quantification
    Language: English
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  • 5
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    Implications of Reactions Between SO2 and Basaltic Glasses for the Mineralogy of Planetary Crusts (2021)
    Details
    Publication Date: 2021-07-27
    Description: Basalts are ubiquitous in volcanic systems on several planetary bodies, including the Earth, Mars, Venus, and Jupiter's moon Io, and are commonly associated with sulfur dioxide (SO2) degassing. We present the results of an experimental study of reactions between SO2 and basaltic glasses. We examined Fe-free basalt, and Fe-bearing tholeiitic and alkali basalts with a range of Fe3+/Fetotal (0.05 to 0.79) that encompass the oxygen fugacities proposed for most terrestrial planetary bodies. Tholeiitic and alkali basalts were exposed to SO2 at 600, 700, and 800 °C for 1 hr and 24 hr. Surface coatings formed on the reacted basalts; these contain CaSO4, MgSO4, Na2SO4, Na2Ca(SO4)2, Fe2O3, Fe3O4, Fe-Ti-(Al)-oxides, and TiO2. Additionally, the SO2-basalt reaction drives nucleation of crystalline phases in the substrate to form pyroxenes and possible Fe-oxides. A silica-rich layer forms between the substrate and sulfate coatings. More oxidized basalts may readily react with SO2 to form coatings dominated by large Ca-sulfate and oxide grains. On less oxidized basalts (NNO−1.5 to NNO−5), reactions with SO2 will form thin, fine-grained aggregates of sulfates; such materials are less readily detected by spectroscopy and spectrometry techniques. In contrast, in very reduced basalts (lower than NNO−5), typical of the Moon and Mercury, SO2 is typically a negligible component in the magmatic gas, and sulfides are more likely.
    Keywords: 552.26 ; 551.9 ; gas-solid reaction ; sulfur dioxide ; planetary crust ; sulfate ; volcanology ; geochemistry
    Language: English
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  • 6
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    NanoSr – A New Carbonate Microanalytical Reference Material for In Situ Strontium Isotope Analysis (2021)
    Details
    Publication Date: 2021-07-23
    Description: The in situ measurement of Sr isotopes in carbonates by MC-ICP-MS is limited by the availability of suitable microanalytical reference materials (RMs), which match the samples of interest. Whereas several well-characterised carbonate reference materials for Sr mass fractions 〉 1000 µg g−1 are available, there is a lack of well-characterised carbonate microanalytical RMs with lower Sr mass fractions. Here, we present a new synthetic carbonate nanopowder RM with a Sr mass fraction of ca. 500 µg g−1 suitable for microanalytical Sr isotope research (‘NanoSr’). NanoSr was analysed by both solution-based and in situ techniques. Element mass fractions were determined using EPMA (Ca mass fraction), as well as laser ablation and solution ICP-MS in different laboratories. The 87Sr/86Sr ratio was determined by well-established bulk methods for Sr isotope measurements and is 0.70756 ± 0.00003 (2s). The Sr isotope microhomogeneity of the material was determined by LA-MC-ICP-MS, which resulted in 87Sr/86Sr ratios of 0.70753 ± 0.00007 (2s) and 0.70757 ± 0.00006 (2s), respectively, in agreement with the solution data within uncertainties. Thus, this new reference material is well suited to monitor and correct microanalytical Sr isotope measurements of low-Sr, low-REE carbonate samples. NanoSr is available from the corresponding author.
    Keywords: 551.9 ; strontium isotopes ; laser ablation ; reference material ; calcium carbonate ; nanopowder ; MC-ICP-MS
    Language: English
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  • 7
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    Intercalibration of Mg Isotope Delta Scales and Realisation of SI Traceability for Mg Isotope Amount Ratios and Isotope Delta Values (2021)
    Details
    Publication Date: 2021-07-21
    Description: The continuous improvement of analytical procedures using multi-collector technologies in ICP-mass spectrometry has led to an increased demand for isotope standards with improved homogeneity and reduced measurement uncertainty. For magnesium, this has led to a variety of available standards with different quality levels ranging from artefact standards to isotope reference materials certified for absolute isotope ratios. This required an intercalibration of all standards and reference materials, which we present in this interlaboratory comparison study. The materials Cambridge1, DSM3, ERM-AE143, ERM-AE144, ERM-AE145, IRMM-009 and NIST SRM 980 were cross-calibrated with expanded measurement uncertainties (95% confidence level) of less than 0.030‰ for the δ25/24Mg values and less than 0.037‰ for the δ26/24Mg values. Thus, comparability of all magnesium isotope delta (δ) measurements based on these standards and reference materials is established. Further, ERM-AE143 anchors all magnesium δ-scales to absolute isotope ratios and therefore establishes SI traceability, here traceability to the SI base unit mole. This applies especially to the DSM3 scale, which is proposed to be maintained. With ERM-AE144 and ERM-AE145, which are product and educt of a sublimation–condensation process, for the first time a set of isotope reference materials is available with a published value for the apparent triple isotope fractionation exponent θapp, the fractionation relationship ln α(25/24Mg)/ln α(26/24Mg).
    Keywords: 551.9 ; delta scale ; traceability ; scale anchor ; absolute isotope ratio ; comparability ; triple isotope fractionation
    Language: English
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  • 8
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    Driving towards transformation? To what extent does global climate governance promote decarbonisation of land transport? (2021)
    Details
    Publication Date: 2021-05-21
    Description: This article aims to analyse the potential for international climate governance to promote the decarbonisation of land transport. It first summarises challenges and barriers that impede the transformation of the sector. On this basis, the article discusses how international governance could potentially assist with overcoming these barriers and mobilising potentials. Subsequently, the article analyses to what extent existing international governance institutions deliver on the potential identified. The analysis finds that while there is a large number of international institutions trying to promote the decarbonisation of land transport, none of them emerge saliently as hubs or core institutions. There is a substantial amount of activity to generate and disseminate knowledge and learning, but the potential for providing guidance and signal, setting rules, providing transparency/accountability and means of implementation could be further exploited. The article concludes with suggestions on how international governance may be strengthened.
    Keywords: ddc:320
    Repository Name: Wuppertal Institut für Klima, Umwelt, Energie
    Language: English
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  • 9
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    Guiding the transformation : the role of global climate governance as a facilitator of the transition of unsustainable socio-technical systems (2021)
    Details
    Publication Date: 2021-05-18
    Description: Climate change is a transformation challenge. It requires the transformation of a patchwork of independent socio-technical systems. These complex systems have their own specific challenges and path dependencies. Lukas Hermwille introduces a perspective on socio-technical complexity to the study of global climate governance and asks what governance arrangements on the international level, in particular the United Nations Framework Convention of Climate Change (UNFCCC) and its Paris Agreement, can offer to facilitate and foster the required transformational change. His work shows the importance of the discursive power of global climate governance, shifting the expectations and visions of the future of key actors and, as a corollary, changing their investment decisions of today towards a more sustainable future.
    Keywords: ddc:320
    Repository Name: Wuppertal Institut für Klima, Umwelt, Energie
    Language: English
    Type: doctoralthesis , doc-type:doctoralThesis
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  • 10
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    Hardwired towards transformation? : Assessing global climate governance for power sector decarbonization (2020)
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    Publication Date: 2021-05-21
    Description: Fully decarbonising global power supply is essential to meet the objectives of the Paris Agreement. A wide range of inter- and transnational governance institutions exist that work towards the transformation of the power sector. But are these governance efforts sufficient to address the challenges? To address this question the article first identifies governance needs on the basis of systemic sector-specific transformation challenges and discusses the potential for international governance to address them. Second, the paper surveys existing inter- and transnational institutions and assess to what extent they exploit the potential of international governance. The analysis shows that many of the governance needs are already being satisfied to some extent, particularly with respect to the deployment of renewable energy. It also shows that a significant blind spot remains: the phase-out of fossil fuels for electricity generation. The detailed analysis enables us to identify options for enhancing the governance landscape.
    Keywords: ddc:320
    Repository Name: Wuppertal Institut für Klima, Umwelt, Energie
    Language: English
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  • 11
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    Design options for the global stocktake : lessons from other review processes (2020)
    Wuppertal : Wuppertal Institut für Klima, Umwelt, Energie
    Details
    Publication Date: 2021-04-20
    Description: While the Paris Agreement (PA) has enshrined ambitious long-term objectives, the current actions of the Parties to the Agreement fall far short of these goals. The Global Stocktake (GST), established in Art. 14 of the PA, may help narrow this gap between ambition and action: its purpose is to review the implementation of the PA and to assess the collective progress of the international community towards Paris goals. While some general modalities on how to conduct the GST have been adopted, the details are still to be determined. The objective of this report is to analyze existing international regimes as regards their review processes, the contribution of these review processes to various governance functions and, finally, to derive lessons for the GST. Processes analyzed include: the design of the upcoming Global Stocktake itself, the Talanoa Dialogue (TD) which is the direct precursor of the GST, the Agenda 2030 High-Level Political Forum (HLPF), which features a regular stocktaking process focused on progress toward the Sustainable Development Goals (SDGs), the review processes of the UN human rights system (UNHRS) and the review processes and assessment panels of the Montreal Protocol (MP). The analysis of each review process is organised in four section: (1) political background and context, (2) technical and organisational details of the processes, (3) interface between the political and technical processes, and (4) how the review processes contribute to achieving the objectives of the respective regime, particularly governance functions of the regime (guidance and signal, transparency and accountability, and knowledge and learning).
    Keywords: ddc:320
    Repository Name: Wuppertal Institut für Klima, Umwelt, Energie
    Language: English
    Type: workingpaper , doc-type:workingPaper
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  • 12
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    A sectoral perspective on global climate governance : analytical foundation (2021)
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    Publication Date: 2021-05-21
    Description: This article develops a sectoral approach to the analysis of global climate governance. This approach advances the assessment of global climate governance by focusing on complexes of intergovernmental and transnational institutions co-governing key socio-technical sectoral systems. The actual and potential contribution of these sectoral institutional complexes to advancing decarbonization can be assessed according to five key governance functions: (1) providing guidance and signal to actors, (2) setting rules to facilitate collective action, (3) enhancing transparency and accountability, (4) offering support (finance, technology, capacity-building), and (5) promoting knowledge and learning. On this basis, we can assess the potential of international cooperation to address the challenges specific sectoral systems face in the climate transition as well as the extent to which existing sectoral institutional complexes deliver on this potential. This provides a solid starting point for developing options for filling identified gaps and enhancing the effectiveness of global climate governance.
    Keywords: ddc:320
    Repository Name: Wuppertal Institut für Klima, Umwelt, Energie
    Language: English
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  • 13
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    Climate ambition and sustainable development for a new decade : a catalytic framework (2021)
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    Publication Date: 2021-07-28
    Description: This paper examines the Global Climate Action Agenda (GCAA) and discusses options to improve sub- and non-state involvement in post-2020 climate governance. A framework that stimulates sub- and non-state action is a necessary complement to national governmental action, as the latter falls short of achieving low-carbon and climate-resilient development as envisaged in the Paris Agreement. Applying design principles for an ideal-type orchestration framework, we review literature and gather expert judgements to assess whether the GCAA has been collaborative, comprehensive, evaluative and catalytic. Results show that there has been greater coordination among orchestrators, for instance in the organization of events. However, mobilization efforts remain event-driven and too little effort is invested in understanding the progress of sub- and non-state action. Data collection has improved, although more sophisticated indicators are needed to evaluate climate and sustainable development impacts. Finally, the GCAA has recorded more action, but relatively little by actors in developing countries. As the world seeks to recover from the COVID-19 crisis and enters a new decade of climate action, the GCAA could make a vital contribution in challenging times by helping governments keep and enhance climate commitments; strengthening capacity for sub- and non-state action; enabling accountability; and realizing sustainable development.
    Keywords: ddc:320
    Repository Name: Wuppertal Institut für Klima, Umwelt, Energie
    Language: English
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  • 14
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    Enough? The role of sufficiency in European energy and climate plans (2021)
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    Publication Date: 2021-08-06
    Description: Energy sufficiency is one of the three energy sustainability strategies, next to energy efficiency and renewable energies. We analyse to what extent European governments follow this strategy, by conducting a systematic document analysis of all available European National Energy and Climate Plans (NECPs) and Long-Term Strategies (LTSs). We collect and categorise a total of 230 sufficiency-related policy measures, finding large differences between countries. We find most sufficiency policies in the transport sector, when classifying also modal shift policies to change the service quality of transport as sufficiency policies. Types of sufficiency policy instruments vary considerably from sector to sector, for instance the focus on financial incentives and fiscal instruments in the mobility sector, information in the building sector, and financial incentive/tax instruments in cross-sectoral application. Regulatory instruments currently play a minor role for sufficiency policy in the national energy and climate plans of EU member states. Similar to energy efficiency in recent decades, sufficiency still largely referred to as micro-level individual behaviour change or necessary exogenous trends that will need to take place. It is not treated yet as a genuine field of policy action to provide the necessary framework for enabling societal change.
    Keywords: ddc:320
    Repository Name: Wuppertal Institut für Klima, Umwelt, Energie
    Language: English
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  • 15
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    Grounding social foundations for integrated assessment models of climate change (2020)
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    Publication Date: 2021-05-18
    Description: Integrated assessment models (IAMs) are commonly used by decision makers in order to derive climate policies. IAMs are currently based on climate-economics interactions, whereas the role of social system has been highlighted to be of prime importance on the implementation of climate policies. Beyond existing IAMs, we argue that it is therefore urgent to increase efforts in the integration of social processes within IAMs. For achieving such a challenge, we present some promising avenues of research based on the social branches of economics. We finally present the potential implications yielded by such social IAMs.
    Keywords: ddc:320
    Repository Name: Wuppertal Institut für Klima, Umwelt, Energie
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  • 16
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    Vertical integration in a multi-level governance system using the example of the German resource efficiency programme (2020)
    Abingdon : Routledge
    Details
    Publication Date: 2020-12-09
    Description: The ultimate goal of German Resource Efficiency Programme (ProgRess) is to make the extraction and use of natural resources more sustainable and reduce associated environmental pollution as much as possible. By doing this - also with responsibility towards future generations - the programme should create a prerequisite for securing a long-term high quality of life. To bring the policy approaches formulated in ProgRess to reality, efforts to implement resource efficiency measures have to be increased at all levels - from international to regional to local. The chapter intends to provide an impetus for the current debate on ProgRess policy development. The chapter identifies, analyses and describes deficits and possibilities of vertical integration of the German programme in particular and derives recommendations for action which may also serve as indications for other strategies. The following sections are based on results of the advisory report "Vertical integration of the national resource efficiency programme ProgRess (VertRess)", conducted by the German Institute of Urban Affairs (Difu) and the Wuppertal Institute for Climate, Environment and Energy on behalf of the German Environmental Agency (UBA) and the Federal Ministry of the Environment, Nature Conservation and Nuclear Safety (BMU).
    Keywords: ddc:320
    Repository Name: Wuppertal Institut für Klima, Umwelt, Energie
    Language: English
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  • 17
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    A sectoral perspective on international climate governance : key findings and research priorities (2021)
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    Publication Date: 2021-05-21
    Description: This concluding article derives six major findings from the contributions to this special issue. First, the barriers and challenges to decarbonisation vary significantly across sectoral systems. Second, and similarly, the need and potential for the five functions of international governance institutions to contribute to effective climate protection also vary widely. Third, while the pattern is uneven, there is a general undersupply of international climate governance. Fourth, the sectoral analyses confirm that the UNFCCC and Paris Agreement play an important overarching role but remain limited in advancing effective sectoral governance. Fifth, while non-environmental institutions may present important barriers to decarbonisation, more synergistic effects are possible. Sixth, our sectoral approach provides a sound basis on which to identify sector-specific policy options. The paper then offers reflections on the merits and limitations of the sectoral approach, before identifying avenues for future research to further advance the agenda.
    Keywords: ddc:320
    Repository Name: Wuppertal Institut für Klima, Umwelt, Energie
    Language: English
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  • 18
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    Bridging the ambition gap : the situation-ambition approach for crediting baselines under article 6.4 (2020)
    Details
    Publication Date: 2021-05-18
    Keywords: ddc:320
    Repository Name: Wuppertal Institut für Klima, Umwelt, Energie
    Language: English
    Type: contributiontoperiodical , doc-type:contributionToPeriodical
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  • 19
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    Near-Complete Local Reduction of Arctic Stratospheric Ozone by Severe Chemical Loss in Spring 2020 (2021)
    Details
    Publication Date: 2021-09-27
    Description: In the Antarctic ozone hole, ozone mixing ratios have been decreasing to extremely low values of 0.01–0.1 ppm in nearly all spring seasons since the late 1980s, corresponding to 95–99% local chemical loss. In contrast, Arctic ozone loss has been much more limited and mixing ratios have never before fallen below 0.5 ppm. In Arctic spring 2020, however, ozonesonde measurements in the most depleted parts of the polar vortex show a highly depleted layer, with ozone loss averaged over sondes peaking at 93% at 18 km. Typical minimum mixing ratios of 0.2 ppm were observed, with individual profiles showing values as low as 0.13 ppm (96% loss). The reason for the unprecedented chemical loss was an unusually strong, long-lasting, and cold polar vortex, showing that for individual winters the effect of the slow decline of ozone-depleting substances on ozone depletion may be counteracted by low temperatures.
    Keywords: 551.9 ; ozone ; stratosphere ; ozone loss ; Arctic ; ozone hole ; temperature
    Language: English
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  • 20
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    Vortex-Wide Detection of Large Aspherical NAT Particles in the Arctic Winter 2011/12 Stratosphere (2021)
    Details
    Publication Date: 2021-09-27
    Description: Micron-sized HNO3-containing particles in polar stratospheric clouds are known to denitrify the polar winter stratosphere and support chemical ozone loss. We show that populations of nitric acid trihydrate (NAT) particles with volume-equivalent median radii of 3–7 μm can be detected vortex-wide by means of infrared limb sounding. Key for detection are the applied optical characteristics of highly aspherical particles consisting of the β-NAT phase. Spectroscopic signatures and ambient conditions of detected populations show that these particles play a key role in denitrification of the Arctic winter stratosphere. Complementary gas-phase HNO3 observations indicate collocated highly efficient HNO3 sequestration within days and are consistent with measured spectral signals of populations of large NAT particles. High amounts of condensed gas-phase equivalent HNO3 exceeding 10 ppbv and long persistence of detected populations, despite expected gravitational settling, imply that our understanding of the particles is incomplete.
    Keywords: 551.9 ; polar winter ; stratosphere ; denitrification ; nitric acid trihydrate ; infrared limb sounding
    Language: English
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  • 21
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    Sources of Uncertainty in Regional and Global Terrestrial CO2 Exchange Estimates (2021)
    Details
    Publication Date: 2021-09-27
    Description: The Global Carbon Budget 2018 (GCB2018) estimated by the atmospheric CO 2 growth rate, fossil fuel emissions, and modeled (bottom-up) land and ocean fluxes cannot be fully closed, leading to a “budget imbalance,” highlighting uncertainties in GCB components. However, no systematic analysis has been performed on which regions or processes contribute to this term. To obtain deeper insight on the sources of uncertainty in global and regional carbon budgets, we analyzed differences in Net Biome Productivity (NBP) for all possible combinations of bottom-up and top-down data sets in GCB2018: (i) 16 dynamic global vegetation models (DGVMs), and (ii) 5 atmospheric inversions that match the atmospheric CO 2 growth rate. We find that the global mismatch between the two ensembles matches well the GCB2018 budget imbalance, with Brazil, Southeast Asia, and Oceania as the largest contributors. Differences between DGVMs dominate global mismatches, while at regional scale differences between inversions contribute the most to uncertainty. At both global and regional scales, disagreement on NBP interannual variability between the two approaches explains a large fraction of differences. We attribute this mismatch to distinct responses to El Niño–Southern Oscillation variability between DGVMs and inversions and to uncertainties in land use change emissions, especially in South America and Southeast Asia. We identify key needs to reduce uncertainty in carbon budgets: reducing uncertainty in atmospheric inversions (e.g., through more observations in the tropics) and in land use change fluxes, including more land use processes and evaluating land use transitions (e.g., using high-resolution remote-sensing), and, finally, improving tropical hydroecological processes and fire representation within DGVMs.
    Keywords: 551.9 ; atmospheric inversions ; global carbon budget ; dynamic global vegetation models ; carbon cycle
    Language: English
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    Seasonality of Organic Matter Degradation Regulates Nutrient and Metal Net Fluxes in a High Energy Sandy Beach (2021)
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    Publication Date: 2021-10-12
    Description: During seawater circulation in permeable intertidal sands, organic matter degradation alters the composition of percolating fluids and remineralization products discharge into surficial waters. Concurrently, coastal seawater nutrient and organic matter composition change seasonally due to variations in pelagic productivity. To assess seasonal changes in organic matter degradation in the intertidal zone of a high energy beach (Spiekeroog Island, southern North Sea, Germany), we analyzed shallow pore waters for major redox constituents (oxygen [O2], manganese [Mn], and iron [Fe]) and inorganic nitrogen species (nitrite [NO2−], nitrate [NO3−], and ammonium [NH4+]) in March, August, and October. Surface water samples from a local time series station were used to monitor seasonal changes in pelagic productivity. O2 and NO3− were the dominating pore water constituents in March and October. Dissolved Mn, Fe, and NH4+ were more widely distributed in August. Seasonal changes in seawater temperature as well as organic matter and nitrate supply by seawater were assumed to affect microbial rates and degradation pathways. Pore water and seawater variability led to seasonally changing constituent effluxes to surface waters. Mn, Fe, and NH4+ effluxes are minimal in March and reached their maximum in August. Furthermore, the intertidal sands switched from a net dissolved inorganic nitrogen sink in March to a net source in August. In conclusion, seasonal effects on intertidal pore water biogeochemistry affect constituent fluxes across the sediment-water interface. The seasonality of the beach bioreactor must be considered when fluxes are extrapolated to annual timescales.
    Keywords: 551.9 ; submarine groundwater discharge ; subterranean estuary ; oxygen ; nitrogen ; manganese ; iron
    Language: English
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    Could oxalate-extractable phosphorus replace phosphorus fractionation schemes in soil phosphorus prospections?—A case study in the prehistoric Milseburg hillfort (Germany) (2021)
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    Publication Date: 2021-10-14
    Description: A geoarchaeological soil phosphorus (P) prospection is used to identify a gate within the prehistoric rampart of the Milseburg hillfort (Hesse, Germany). This study compares the application of a P fractionation scheme and P extraction with ammonium-oxalate. We hypothesized that oxalate-extractable P (P-ox) and the related degree of P saturation (DPS) could replace the more expensive and time-consuming fractionation schemes for geoarchaeological investigations. Comparing the results, the P fractionation helped to verify the existence of another section of the prehistoric ramparts and to identify the location of a gate within it. It also helped to discover the archaeologically relevant soil depths in the investigated area. This information could not be retrieved from the P-ox data alone. Soil P-ox contents and DPS values are relatively unspecific with regard to prehistoric land use. However, DPS at least indicates settled versus unsettled areas. Still, the results of the P fractionation more clearly delineate Iron Age land use areas including settlement, non-settlement, rampart, and rampart gap (probable gate). Thus, in geoarchaeological contexts, this method seems to be preferable to a singular P-ox extraction. However, for better results, P-ox determination could be integrated into a P fractionation scheme.
    Keywords: 551.9 ; 631.4 ; Milseburg ; oxalate-extractable phosphorus ; phosphorus fractionation ; phosphorus saturation ; soil phosphorus prospection
    Language: English
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    How Important is Denitrification in Riparian Zones? Combining End-Member Mixing and Isotope Modeling to Quantify Nitrate Removal from Riparian Groundwater (2021)
    Details
    Publication Date: 2021-10-14
    Description: Riparian zones are important buffer zones for streams as they are hotspots of nitrate transformation and removal in agricultural catchments. However, mixing of water from different sources and various transformation processes can complicate the quantification of nitrate turnover in riparian zones. In this study, we analyzed nitrate concentration and isotope data in riparian groundwater along a 2-km stream section in central Germany. We developed a mathematical model combining end-member mixing and isotope modeling to account for mixing of river water and groundwater and quantify nitrate transformation in riparian groundwater. This enabled us to explicitly determine the extent of denitrification (as process leading to permanent nitrate removal from riparian groundwater) and transient nitrate removal by additional processes associated with negligible isotope fractionation (e.g., plant uptake and microbial assimilation) and to perform an extensive uncertainty analysis. Based on the nitrogen isotope data of nitrate, the simulations suggest a mean removal of up to 27% by additional processes and only about 12% by denitrification. Nitrate removal from riparian groundwater by additional processes exceeded denitrification particularly in winter and at larger distance from the river, underlining the role of the river as organic carbon source. This highlights that nitrate consumption by additional processes predominates at the field site, implying that a substantial fraction of agricultural nitrogen input is not permanently removed but rather retained in the riparian zone. Overall, our model represents a useful tool to better compare nitrogen retention to permanent nitrogen removal in riparian zones at various temporal and spatial scales.
    Keywords: 551.9 ; denitrification ; riparian zones ; nitrate ; isotope analysis ; mixing model ; eutrophication
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    Sediment Properties Drive Spatial Variability of Potential Methane Production and Oxidation in Small Streams (2021)
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    Publication Date: 2021-10-14
    Description: Emissions of the potent greenhouse gas methane (CH4) from streams and rivers are a significant component of global freshwater methane emissions. The distribution of CH4 production and oxidation within stream sections and in vertical sediment profiles is not well understood, and the environmental controls on CH4 production and emission in such systems create a significant challenge for assessing larger-scale dynamics. Here we investigate factors driving the spatial variability of sediment potential methane production (PMP) and potential methane oxidation (PMO) in a temperate stream network in Germany. PMP was highly variable, ranging from 5 × 10−4 to 28.58 μg CH4 gDW−1 d−1 and PMO ranged from 0.43 μg CH4 gDW−1 d−1 to 14.41 μg CH4 gDW−1 d−1. Important drivers of spatial variability of PMP and PMO in the sediments of the stream main-stem were related to fine sediment fraction and organic carbon content. At smaller spatial scale, that is, in a sub-catchment stream section, the drivers were more complex and included sediment nitrogen and organic carbon content, as well as porewater dissolved organic carbon, dissolved organic matter quality, and metal concentrations. As with reservoirs and impounded rivers, fine sediment deposition and organic carbon content were found to be key controls on the spatial variability of CH4 production and oxidation. These findings enhance our understanding of CH4 dynamics, improve the potential for identifying CH4 production hotspots in small streams, and provide a potential means for upscaling emission rates in larger-scale assessments.
    Keywords: 551.9 ; carbon cycle ; streams ; methane ; sediment ; porewater ; grain size
    Language: English
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    Stable Carbon Isotope Studies of CH4 Dynamics Via Water and Plant Pathways in a Tropical Thai Paddy: Insights Into Diel CH4 Transportation (2021)
    Details
    Publication Date: 2021-10-14
    Description: Separate evaluation of methane (CH4) emission dynamics (e.g., oxidation, production, and transportation) at the soil-plant-atmosphere and soil-water-atmosphere interfaces has been limited in tropical rice paddies, but it is crucial for comprehending the entire CH4 cycles. We investigated CH4 oxidation, production, and transportation through plant and water pathways during the reproductive stage in a tropical Thailand rice paddy field using natural abundance carbon stable isotope ratios (δ13CH4 and δ13CO2). Mass balance equations using δ13CH4 and δ13CO2 in soil gases indicated that CH4 oxidation in the planted soil exceeded those in the interrow soil due to oxygen supply through rice roots. In addition, at 1–11 cm depth acetate fermentation was the dominant process in the planted soil, whereas in the interrow soil the dominant process was H2/CO2 reduction. The water pathway showed a significant negative correlation between CH4 flux and released δ13CH4 over 24 hr, driven by a diel change in episodic ebullition, steady ebullition, and diffusion, all due to diel changes in soil temperature and atmospheric pressure. In contrast, the plant pathway showed a significant positive relationship between CH4 flux and emitted δ13CH4 throughout one day. A comparison of the diel change in emitted δ13CH4 between the water and plant pathways showed that the rice plants transported CH4 in soil bubbles without any large isotopic fractionation. The diel change in the plant-mediated CH4 transportation was mainly controlled by diel changes in soil bubble expansion and CH4 diffusion through plants, which were probably regulated by diel changes in soil temperature and atmospheric pressure.
    Keywords: 551.9 ; CH4 ; carbon stable isotopes ; rice paddy ; plant pathway ; water pathway ; diel CH4 transportation
    Language: English
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    Influence of Ocean Circulation and Benthic Exchange on Deep Northwest Atlantic Nd Isotope Records During the Past 30,000 Years (2021)
    Details
    Publication Date: 2021-10-01
    Description: Neodymium (Nd) isotopes extracted from authigenic sediment phases are increasingly used as a proxy for past variations in water mass provenance. To better constrain the controls of water mass provenance and nonconservative effects on the archived Nd isotope signal, we present a new depth transect of Nd isotope reconstructions from the Blake Bahama Outer Ridge along the North American continental margin covering the past 30 ka. We investigated five sediment cores that lie directly within the main flow path of the Deep Western Boundary Current, a major advection route of North Atlantic Deep Water. We found offsets between core tops and seawater Nd isotopic compositions that are observed elsewhere in the Northwest Atlantic. A possible explanation for this is the earlier suggested redistribution of sediment by nepheloid layers at intermediate as well as abyssal depths, transporting material downslope and along the continental margin. These processes potentially contributed to Nd isotope excursions recorded in Northwest Atlantic sediment cores during the Bølling-Allerød and early Holocene. An Atlantic-wide comparison of Nd isotope records shows that the early Holocene excursions had an additional contribution from conservative advection of unradiogenic dissolved Nd. Nevertheless, the trends of the Nd isotope records are in general agreement with previous reconstructions of water mass provenance from the entire Atlantic and also reveal millennial-scale changes during the last deglaciation in temporal high resolution, which have rarely been reported before. Further, the new records confirm that during cold periods the Northwest Atlantic was bathed by an increased contribution of southern sourced water.
    Keywords: 551.9 ; neodymium isotopes ; deglaciation ; water masses ; Last Glacial Maximum ; benthic exchange
    Language: English
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    Effects of Temperature and Light on Methane Production of Widespread Marine Phytoplankton (2021)
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    Publication Date: 2021-12-01
    Description: Methane (CH4) production in the ocean surface mixed layer is a widespread but still largely unexplained phenomenon. In this context marine algae have recently been described as a possible source of CH4 in surface waters. In the present study we investigated the effects of temperature and light intensity (including daylength) on CH4 formation from three widespread marine algal species Emiliania huxleyi, Phaeocystis globosa, and Chrysochromulina sp. Rates of E. huxleyi increased by 210% when temperature increased in a range from 10°C to 21.5°C, while a further increase in temperature (up to 23.8°C) showed reduction of CH4 production rates. Our results clearly showed that CH4 formation of E. huxleyi is controlled by light: When light intensity increased from 30 to 2,670 μmol m−2 s−1, CH4 emission rates increased continuously by almost 1 order of magnitude and was more than 1 order of magnitude higher when the daylength (light period) was extended from 6/18 hr light-dark cycle to continuous light. Furthermore, light intensity is also an important factor controlling CH4 emissions of Chrysochromulina sp. and P. globosa and could therefore be a species-independent regulator of phytoplankton CH4 production. Based on our results, we might conclude that extensive blooms of E. huxleyi could act as a main regional source of CH4 in surface water, since blooming of E. huxleyi is related to the seasonal increase in both light and temperature, which also stimulate CH4 production. Under typical global change scenarios, E. huxleyi will increase its CH4 production in the future.
    Keywords: 551.9 ; 557.7 ; marine phytoplacton ; CH4 production ; temperature influence ; light intensity influence ; daylength influence
    Language: English
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    Governance policies for a "just transition" : a case study in the Rhineland lignite mining district (2021)
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    Publication Date: 2021-12-10
    Description: This paper develops policy measures for a "just transition" based on a case study conducted in Germany's Rhineland lignite mining district. Semi-structured guided interviews served as the methodological approach. Expert interviews were conducted with representatives of citizen initiatives, trade unions and the Federal State of North Rhine-Westphalia. The results reveal the need for policy measures in different areas: First, employees working for subcontractors of the lignite industry have a high risk of losing their jobs because there are virtually no support policies for them. Second, there needs to be more input by civic initiatives regarding the process of structural change. And last, land needs to be prevented from becoming a scarce resource in the Rhineland area due to current mining legislation. We use an actor-centred institutionalist framework to derive governance approaches in line with the needs of various stakeholders.
    Keywords: ddc:320
    Repository Name: Wuppertal Institut für Klima, Umwelt, Energie
    Language: English
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    Caught in between : credibility and feasibility of the voluntary carbon market post-2020 (2021)
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    Publication Date: 2021-11-11
    Description: On the one hand, a large number of companies have committed to achieve net zero emissions and many of them foresee to offset some remaining emissions with carbon credits, suggesting a surge of future demand. Yet, the supply side of the voluntary carbon market is struggling to align its business model with the new legal architecture of the Paris Agreement. This article juxtaposes these two perspectives. It provides an overview of the plans of 482 major companies with some form of neutrality/net zero pledge and traces the struggle on the supply side of the voluntary carbon market to come up with a viable business model that ensures environmental integrity and contributes to achieving the objectives of the Paris Agreement. Our analysis finds that if carbon credits are used to offset remaining emissions against neutrality objectives, these credits need to be accounted against the host countries' Nationally Determined Contributions (NDCs) to ensure environmental integrity. Yet, operationalizing this approach is challenging and will require innovative solutions and political support. Key policy insights: There is a growing mismatch between the faith placed in carbon credits by private sector companies and the continued quest for a common position of the main suppliers of the voluntary carbon market. The voluntary carbon market has not yet found a way to align itself with the new legal architecture of the Paris Agreement in a credible and legitimate way. Public policy support at the national and international level will be needed to operationalize a robust approach for the market’s future activities.
    Keywords: ddc:320
    Repository Name: Wuppertal Institut für Klima, Umwelt, Energie
    Language: English
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    Presentation of the 5Ds in energy policy : a policy paper to show how Germany can regain its role as a pioneer in energy policy (2021)
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    Publication Date: 2021-11-11
    Description: The widely recognised Energiewende, ("energy transition") in Germany has lost its original momentum. We therefore address the question of how the transition process to a new energy system can be reignited. To do so, we developed the "5Ds approach", which lays the groundwork for a process analysis and the identification of important catalysts and barriers. Focusing on the five major fields required for the energy transition, we analyse the effects of: (1) Decarbonisation: How can efficiency and renewable energies be expanded successfully? (2) Digitalisation: Which digital solutions facilitate this conversion and would be suitable as sustainable business models? (3) Decentralisation: How can potential decentralised energy and efficiency opportunities be developed? (4) Democratisation: How can participation be strengthened in order to foster acceptance (and prevent "yellow vest" protests, etc.)? (5) Diversification of service: Which services can make significant contributions in the context of flexible power generation, demand-side management, storage and grids? Our paper comes to the conclusion that German policy efforts in the "5D" fields have been implemented very differently. Particularly with regard to democratisation, the opportunities for genuine participation among the different social actors must be further strengthened to get the Energiewende back on track. New market models are needed to meet the challenges of the energy transition and to increase the performance of "5D" through economic incentives.
    Keywords: ddc:320
    Repository Name: Wuppertal Institut für Klima, Umwelt, Energie
    Language: English
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    Evidence-based narratives in European research programming (2021)
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    Publication Date: 2021-11-11
    Description: The article introduces and exemplifies the approach of evidence-based narratives (EBN). The methodology is a product of co-design between policy-making and science, generating robust intelligence for evidence-based policy-making in the Directorate General for Research and Innovation of the European Commission (DG RTD) under the condition of high uncertainty and fragmented evidence. The EBN transdisciplinary approach tackles practical problems of future-oriented policy-making, in this case in the area of programming for research and innovation addressing the Grand Societal Challenge related to climate change and natural resources. Between 2013 and 2018, the EU-funded RECREATE project developed 20 EBNs in a co-development process between scientists and policy-makers. All EBNs are supported with evidence about the underlying innovation system applying the technological innovation systems (TIS) framework. Each TIS analysis features the innovation, its current state of market diffusion and a description of the innovation investment case. Indicators include potential future market sizes, effects on employment and environmental and social benefits. Based on the innovation and TIS function analyses, the EBNs offer policy recommendations. The article ends with a critical discussion of the EBN approach.
    Keywords: ddc:320
    Repository Name: Wuppertal Institut für Klima, Umwelt, Energie
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    Harnessing international climate governance to drive a sustainable recovery from the COVID-19 pandemic (2020)
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    Publication Date: 2021-11-23
    Description: The impacts of the COVID-19 crisis and the global response to it will co-determine the future of climate policy. The recovery packages responding to the impacts of the pandemic may either help to chart a new sustainable course, or they will further cement existing high-emission pathways and thwart the achievement of the Paris Agreement objectives. This article discusses how international climate governance may help align the recovery packages with the climate agenda. For this purpose, the article investigates five key governance functions through which international institutions may contribute: send guidance and signals, establish rules and standards, provide transparency and accountability, organize the provision of means of implementation, and promote collective learning. Reflecting on these functions, the article finds that the process under the United Nations Framework Convention on Climate Change (UNFCCC), together with other international institutions, could promote sustainable recovery in several ways.
    Keywords: ddc:320
    Repository Name: Wuppertal Institut für Klima, Umwelt, Energie
    Language: English
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    Unlocking green financing for building energy retrofit : a survey in the western China (2020)
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    Publication Date: 2021-12-07
    Description: Energy service companies (ESCOs) play crucial role in building energy efficiency retrofit sector. However limited access to green financing has prevented ESCOs in their expansions in China. This paper, based on a survey of 469 samples and on-site visiting to and interviewing relevant 50 actors of ESCOs, financial institutions and local housing authorities, identifies main barriers of accessing to green financing at both systemic policy level and operational meso and micro level in China, and analyzes good practices at local level that overcome the barriers. The paper concludes that, although there are barriers existing at the policy level in China, substantial attentions and priorities should be given to take actions for overcoming the barriers existed at the operational meso and micro level. The paper suggests that the good practices of capacity building for ESCOs and local financial sector, intensifying participation of intermediate organizations or facilitators and diversifying financial sources and funding mechanisms and models that emerge from the local level should be disseminated in China.
    Keywords: ddc:320
    Repository Name: Wuppertal Institut für Klima, Umwelt, Energie
    Language: English
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    Silicon Isotopes in an EMIC's Ocean: Sensitivity to Runoff, Iron Supply, and Climate (2021)
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    Publication Date: 2021-10-26
    Description: The isotopic composition of Si in biogenic silica (BSi), such as opal buried in the oceans' sediments, has changed over time. Paleorecords suggest that the isotopic composition, described in terms of δ30Si, was generally much lower during glacial times than today. There is consensus that this variability is attributable to differing environmental conditions at the respective time of BSi production and sedimentation. The detailed links between environmental conditions and the isotopic composition of BSi in the sediments remain, however, poorly constrained. In this study, we explore the effects of a suite of offset boundary conditions during the Last Glacial Maximum (LGM) on the isotopic composition of BSi archived in sediments in an Earth System Model of intermediate complexity (EMIC). Our model results suggest that a change in the isotopic composition of Si supply to the glacial ocean is sufficient to explain the observed overall low(er) glacial δ30Si in BSi. All other processes explored trigger model responses of either wrong sign or magnitude or are inconsistent with a recent estimate of bottom water oxygenation in the Atlantic Sector of the Southern Ocean. Caveats, mainly associated with generic uncertainties in today's pelagic biogeochemical modules, remain.
    Keywords: 551.9 ; 551.9 ; Earth System Model ; silicon isotopes ; Last Glacial Maximum ; biogeochemical modeling ; ocean ; sediment
    Language: English
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