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  • Articles  (174)
  • soil  (88)
  • monitoring  (65)
  • Chemical Engineering
  • Fisheries
  • Organic Chemistry
  • Energy, Environment Protection, Nuclear Power Engineering  (174)
  • 1
    ISSN: 1573-0840
    Keywords: acid rain ; photochemical smog ; ground-level ozone ; particulate matter ; modelling ; monitoring ; real-time prediction ; policy application
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering , Geography , Geosciences
    Notes: Abstract Acid rain and photochemical smog are two regionalair-quality issues that have received considerableattention in the last two decades due to their harmfuleffects. Health impacts of particulate matter (PM) inthe atmosphere is another issue of concern. Sulphur dioxide emission controls were introducedin both Canada and the U.S.A. to reduceacid-deposition-related damage. While these emissionreductions have already resulted in reduced sulphatedeposition, based on results from modelling studiesmuch of southeastern Canada is still expected toexperience damaging levels of acid deposition evenafter all currently legislated emission controls arefully implemented. Moreover, there has not been acorresponding reduction in the acidity ofprecipitation. This may be attributable to aconcurrent reduction in base-cation concentration inprecipitation. Models were also developed to understand theformation, transport and diffusion of troposphericozone. The models have been used to provide policyguidance for emission control options to reduceground-level ozone to acceptable limits. In thesummer of 1997 a Canadian pilot project was initiatedto provide real-time forecasts of ground-level ozonein the southeastern part of the province of NewBrunswick in eastern Canada. With the emergence of fine Particulate Matter(PM2.5) as a health concern, efforts are underwayin Canada to develop a “unified'' regional air-qualitymodel that will address the combined impacts ofvarious pollutants in the atmosphere. In this effortthe atmosphere is viewed as a single entity where theimpacts of multiple pollutants are considered at thesame time.
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  • 2
    ISSN: 1573-2959
    Keywords: copper-nickel smelter ; ICP mass spectrometry ; Kola peninsula ; pollution ; soil ; trace elements ; vegetation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Concentrations of 34 elements determined by ICP mass spectrometry were studied in surface soil and vegetation along a north–south gradient through the ‘Pechenganickel’ smelter complex in Kola peninsula, northern Russia. Strong influence from the smelter was evident for Fe, Co, Ni, and Cu, mainly associated with dry deposition of large particles. Also for As, Se, Mo, Sb, Te, Bi, and Pb the smelter or associated sources appeared to be distinct contributors of contamination consisting presumably of smaller particles. Significant but less distinct effects leading to enhanced concentration levels were observed for P, S, V, Cr, Zn, and Tl. In the case of Mn, Rb, Sr, Cs, and Ba the concentrations in vegetation were generally lower near the source, which may be due to cation exchange with protons or heavy metal cations in the soil and subsequent leaching from the root zone. For Li, Be, B, Na, Mg, Al, Ca, Y, Cd, La, Th, and U no particular influence from the smelter complex was observed. Some characteristic differences observed in element concentrations in different plant species and between different years of Pinus sylvestris needles are discussed. The high concentrations observed for many trace elements in the humus horizon indicates that it acts as an active biogeochemical barrier against downward transport of these elements.
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  • 3
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    Environmental monitoring and assessment 64 (2000), S. 583-590 
    ISSN: 1573-2959
    Keywords: biological activity of soil ; constantpressure volumetric respirometer ; flow-through respirometer ; respirometry methods ; soil ; soil respiration
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Among commonly employed methods of fast estimation of the soil biological activity a method of the oxygen consumption determination is used. The main goal of this research was an estimation of a soil respiratory metabolism using the constant pressure volumetric respirometer and also using the flow-through respirometer UNI-RES10.Soil respiration measurements were done using both types of respirometers in temperatures 10, 15, 20, 25, 30 and 35 °C, keeping up the constant humidity. The investigated soil was a soil humus belonged to organic soils from the Dziekanów Leśny field. The soil respiration was also measured for 8 plant communities in Sudeten Mountains with various respiration intensity.After the experiments it was stated that both measuring instruments could be used for the soil metabolism evaluation. Readouts obtained from the UNI-RES10 respirometer are smaller then readouts when using the constant pressure volumetric respirometer. The flow-through respirometers have to be calibrated to obtain results comparable with these from volumetric ones. The volumetric and flow-through respirometry methods are useful for the comparative analysis of metabolism levels.
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  • 4
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    Mitigation and adaptation strategies for global change 5 (2000), S. 189-216 
    ISSN: 1573-1596
    Keywords: certification ; Clean Development Mechanism ; energy efficiency ; evaluation ; global climate change ; greenhouse gas emissions ; joint implementation ; monitoring ; reporting ; verification
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering , Geography
    Notes: Abstract In this paper, we present an overview of guidelinesdeveloped for the monitoring, evaluation, reporting,verification, and certification (MERVC) ofenergy-efficiency projects for climate changemitigation. The monitoring and evaluation ofenergy-efficiency projects is needed to determine moreaccurately their impact on greenhouse gas (GHG)emissions and other attributes, and to ensure that theglobal climate is protected and that countryobligations are met. Reporting, verification andcertification will be needed for addressing therequirements of the Kyoto Protocol. While the cost ofmonitoring and evaluation of energy-efficiencyprojects is expected to be about 5–10% of a project'sbudget, the actual cost of monitoring and evaluationwill vary depending on many factors, including thelevel of precision required for measuring energy andGHG reductions, type of project, and amount of fundingavailable.
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  • 5
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    Environmental monitoring and assessment 64 (2000), S. 379-390 
    ISSN: 1573-2959
    Keywords: monitoring ; research ; CISNet ; environmental stressors
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The U.S. Environmental Protection Agency (EPA), National Oceanic and Atmospheric Administration (NOAA), and National Aeronautics and Space Administration (NASA) have formed a partnership to establish pilot sites for the development of a network known as the Coastal Intensive Site Network (CISNet). CISNet is composed of intensive, long-term monitoring and research sites around the U.S. marine and Great Lakes coasts. In this partnership, EPA and NOAA are funding research and monitoring programs at pilot sites that utilize ecological indicators and investigate the ecological effects of environmental stressors. NASA is funding research aimed at developing a remote sensing capability that will augment or enhance in situresearch and monitoring programs selected by EPA and NOAA. CISNet has three objectives: 1) to develop a sound scientific basis for understanding ecological responses to anthropogenic stresses in coastal environments, including the interaction of exposure, environment/climate, and biological/ecological factors in the response, and the spatial and temporal nature of these interactions, 2) to demonstrate the value of developing data from selected sites intensively monitored to examine the relationships between changes in environmental stressors, including anthropogenic and natural stresses, and ecological response, and 3) to provide intensively monitored sites for development and evaluation of indicators of change in coastal systems.
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  • 6
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    Environmental monitoring and assessment 64 (2000), S. 409-419 
    ISSN: 1573-2959
    Keywords: monitoring ; assessment ; water ; sediment ; bioaccumulation ; toxicity ; pesticides ; mercury ; PCB
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The San Francisco Estuary Regional Monitoring Program for Trace Substances (RMP) began in 1993 and is sponsored by 74 local, state, and federal agencies and companies through their discharge or Bay use permits. The RMP monitors water, sediment, toxicity, and bivalve bioaccumulation at 25 sites in the Bay that are considered to represent "background" conditions. Several major environmental issues have been identified by the RMP. Polychlorinated biphenyls and mercury were often above water quality guidelines, and often occurred in fish tissues above U.S. Environmental Protection Agency (U.S. EPA) screening values. Concentrations do not appear to be decreasing, suggesting continuing inputs. Episodes of aquatic toxicity often occurred following runoff events that transport contaminants into the Bay from urbanized and agricultural portions of the watershed. Sediment toxicity occurred throughout the Bay, and has been correlated with concentrations of specific contaminants (chlordanes, polynuclear aromatic hydrocarbons) at some locations; mixtures of contaminants were probably also important. Since the RMP does not monitor all ecosystem components, assessments of the overall condition of the Bay cannot be made. However, in terms of contamination, the RMP samples suggest that the South Bay, and North Bay sites are moderately contaminated.
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  • 7
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    Environment, development and sustainability 2 (2000), S. 277-304 
    ISSN: 1573-2975
    Keywords: Systems of Knowledge ; Local Knowledge ; Fisheries ; Resource Management
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering , Sociology
    Notes: Abstract During the last 20 years, the existence of rich systems of local knowledge, and their vital support to resource use and management regimes, has been demonstrated in a wide range of biological, physical and geographical domains, such as agriculture, animal husbandry, forestry and agroforestry, medicine, and marine science and fisheries. Local knowledge includes empirical and practical components that are fundamental to sustainable resource management. Among coastal-marine fishers, for example, regular catches and, often, long-term resource sustainment are ensured through the application of knowledge that encompasses empirical information on fish behaviour, marine physical environments, fish habitats and the interactions among ecosystem components, as well as complex fish taxonomies. Local knowledge is therefore an important cultural resource that guides and sustains the operation of customary management systems. The sets of rules that compose a fisheries management system derive directly from local concepts and knowledge of the resources on which the fishery is based. Beyond the practical and the empirical, it is essential to recognise the fundamental socio-cultural importance of local knowledge to any society. It is through knowledge transmission and socialisation that worldviews are constructed, social institutions perpetuated, customary practices established, and social roles defined. In this manner, local knowledge and its transmission, shape society and culture, and culture and society shape knowledge. Local knowledge is of great potential practical value. It can provide an important information base for local resources management, especially in the tropics, where conventionally-used data are usually scarce to non-existent, as well as providing a shortcut to pinpoint essential scientific research needs. To be useful for resources management, however, it must be systematically collected and scientifically verified, before being blended with complementary information derived from Western-based sciences. But local knowledge should not be looked on with only a short-term utilitarian eye. Arguments widely accepted for conserving biodiversity, for example, are also applicable to the intellectual cultural diversity encompassed in local knowledge systems: they should be conserved because their utility may only be revealed at some later date or owing to their intrinsic value as part of the world's global heritage. At least in cultures with a Western liberal tradition, more than lip-service is now being paid to alternative systems of knowledge. The denigration of alternative knowledge systems as backward, inefficient, inferior, and founded on myth and ignorance has recently begun to change. Many such practices are a logical, sophisticated and often still-evolving adaptation to risk, based on generations of empirical experience and arranged according to principles, philosophies and institutions that are radically different from those prevailing in Western scientific circles, and hence all-but incomprehensible to them. But steadfastly held prejudices remain powerful. In this presentation I describe the 'design principles' of local knowledge systems, with particular reference to coastal-marine fishing communities, and their social and practical usefulness. I then examine the economic, ideological and institutional factors that combine to perpetuate the marginalisation and neglect of local knowledge, and discuss some of the requirements for applying local knowledge in modern management.
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  • 8
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    Environmental monitoring and assessment 61 (2000), S. 301-313 
    ISSN: 1573-2959
    Keywords: biological activity ofsoil ; constant-pressure volumetric respirometer ; heavy metals ; respirometry methods ; soil ; soil degradation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A main goal of investigations is to determine could a soilrespiration be an indicator of the soil pollution. In this case a measured levelof the soil oxygen consumption depends of its pollution. It alsomeans that the pollution reduces biological processes in edaphon.Investigated soil samples were taken from polluted andnon-polluted places in the Baix Llobregat near Barcelona (Catalonia, NE Spain). Soil samples were taken from the top ofsoil (0–5 cm) without a litter. Soil analysis were done, determining percentage shares of coarsefragments, coarse sand, fine sand, coarse silt, fine silt, clay,CaCO3, organic matter as well as water pH and conductivityCE (1:5 [mS cm-1]). Also were determined (in mg kg-1)quantities of heavy metals, as Fe, Al, Mn, Zn, Cr, Ni, V, Cu, Cd, Pb.The soil respiration was investigated in temperatures15 and 30 °C and with controlled humidity.The respiration in 30 °C is number of times greater thenin 15 °C both for polluted and non-polluted soils.Particularly high coefficients of correlation between the soilrespiration and soil pollution in polluted soils were obtainedfor Pb: r = 0.75 in 15 °C and r = 0.98 in30 °C; for Ba: 0.90 and 0.57; for V: 0.99 and 0.81. In non-polluted soils highest correlation coefficients are for Pb: r = 0.70 in 15 °C; Fe: 0.60 and 0.72; Al: 0.68 and0.64; Mn: 0.51 and 0.66; Ba: 0.63 and 0.61; Cr: 0.94 and0.70; Ni: 0.64 and 0.65; Cu: 0.69 and 0.48; as well as V: 0.62in 15 °C; and Cd: 0.69 in 15 °C.This way the soil respiration could be a good indicator of the soil pollution.
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  • 9
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    Environmental monitoring and assessment 63 (2000), S. 329-339 
    ISSN: 1573-2959
    Keywords: bioavailable ; lead ; sediment ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract This study determined the spatial distribution of soiland of sediment-associated lead in Iqaluit, Nunavut.Samples were collected from the following areas:outside the built-up area of the town to reflectbackground concentrations; known or potential pointsources of lead, such as the Upper Base, the SylviaGrinnell Dump and the Metal Dump (North 40); andresidential and commercial areas of Iqaluit and Apex,a satellite community. In the laboratory, the 〈63 μm sample fraction was analyzed for total lead andbioavailable lead, estimated by non-residual acidextractable lead content. The research findings revealthat elevated levels of bioavailable lead are presentin the study area. Total lead concentrations generallydo not exceed environmental guidelines. However, leadconcentrations in the Sylvia Grinnell Dump, and Apexand Iqaluit grid areas exceed health-based guidelines.The research concludes that there is not a serioushealth hazard posed by lead levels in the soil andsediment in the study area. However, severalenvironmental (elevated lead levels, bioavailableforms of lead and bare soil surfaces) and behaviouralfactors (vigorous and unsupervised play outside) maycreate a risk of lead exposure.
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  • 10
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    Environmental monitoring and assessment 64 (2000), S. 1-8 
    ISSN: 1573-2959
    Keywords: assessment ; ecology ; estuaries ; indicators ; mid-Atlantic ; monitoring ; scale ; trends ; West
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Management for the future sustainability and integrity of our nation's ecological resources requires concepts and tools for measuring status and trends in these resources at multiple spatial and temporal scales and at multiple levels of biological organization. Key elements of this process are ecologically meaningful indicators and cost-effective monitoring designs. The Environmental Monitoring and Assessment Program (EMAP) advances the science needed for measuring ecosystem condition and trends. Most recently the EMAP approach has been successfully used by participants in the Mid-Atlantic Integrated Assessment (MAIA), including EPA's Office of Research and Development, EPA's Region III, and the States of the Mid-Atlantic. The participants in MAIA have produced a regional landscape atlas, state of the estuaries report, and state of the streams report. The work in MAIA is currently moving from monitoring into the assessment phase. The Western EMAP Pilot (Western Pilot), will be a test of our current MAIA indicators and technology for applicability in western ecosystems. New indicators and designs may be needed in the Western Pilot for assessments at the level of EPA's Regions, of the states, and of the Tribes; these assessments will be done so that they can be combined to provide regional assessments. Our coastal monitoring program in the Western estuaries will also be initiated shortly. Subsequently, this will be expanded to the Gulf and Atlantic coasts to provide the current condition of our national estuaries. By continuing to improve the science of monitoring, EMAP researchers will remove data gaps and allow the unequivocal assessment of the health of the nation's resources.
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  • 11
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    Environmental monitoring and assessment 65 (2000), S. 119-127 
    ISSN: 1573-2959
    Keywords: DOAS ; Differential Optical Absorption Spectroscopy ; urban air quality ; monitoring ; vertical distribution ; ozone
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The concentrations of ozone, NO2 and SO2, measured with a DOAS system 70 m above ground level in the city of Graz were compared with data from conventional ground stations. The dependence of vertical trace-gas distributions on stability categories and time of the day or year was investigated. Concerning the maximum ozone concentrations in summer, the DOAS data are representative for the ground-level situation. In average, the concentrations 70 m above ground are more than twice the ground-level concentrations. It has been shown that beside the reaction with NO, dry deposition is an important sink for ozone near the surface. The DOAS NO2-concentrations are representative for ground-level conditions in summer, except for the morning maximum of NO2. In winter the DOAS NO2-concentrations amount for 73% of the ground level values in average. Concerning the slow reacting trace gas SO2, the DOAS data are always representative for the ground-level conditions.
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  • 12
    ISSN: 1573-2959
    Keywords: mercury ; mining ; monitoring ; aquatic ; acid mine drainage ; floc ; Clear Lake ; remediation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Mercury (Hg) in the aquatic ecosystem of Clear Lake has been documented since the 1970s when fishes were found to have elevated levels of toxic methyl mercury (meHg). Mining practices at the Sulphur Bank Mercury Mine (active intermittently from 1872–1957) along the shoreline of Clear Lake included the bulldozing of waste rock and overburden ore into the shallow nearshore regions of the lake and the creation of steeply sloped piles of waste rock at the water's edge. This process, plus erosion of the waste rock piles, resulted in the accumulation of an estimated 100 metric tons of Hg in Clear Lake. A monitoring program to assess Hg in Clear Lake was established in 1992, and conducted continuously from 1994. Drought conditions in California had persisted for ca. 6 yrs prior to 1992, when the U.S. Environmental Protection Agency (USEPA) remediated the steeply sloped eroding waste rock piles, which appeared to reduce sediment Hg concentrations significantly. In April 1995, a white flocculent material was observed in Clear Lake adjacent to the mine and has been observed every year since, leading to the discovery of ongoing acid mine drainage (AMD), low pH fluids high in Hg and extremely high in sulfate. AMD is now believed to be the most likely cause of elevated meHg in Clear Lake. The discovery of this source of meHg production in Clear Lake, which will significantly influence remedial options, was only made possible by implementation of a diligent monitoring program.
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  • 13
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    Water, air & soil pollution 124 (2000), S. 1-21 
    ISSN: 1573-2932
    Keywords: horizon ; selective extraction ; soil ; trace metal ; vertical distribution
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract To predict the long-term behavior of trace metals in a soilprofile, we studied the vertical distributions of barium, zinc,copper, chromium, nickel, cobalt, lead, and the principalmetals, aluminum, iron and manganese, in three soils withdeveloped horizons obtained from rural areas in Japan. Totalelement analysis and selective extraction tests with variousreagents were conducted to clarify the extractability of themetals at each sampling depth.Soil-b (Dystric Cambisols) had the highest extractability ofelements although the vertical distributions of its traceelements were similar to those of soil-d (Umbric Andosols),which had to lowest metal extractability of the three soils.Soil-KUR (Orthic Acrisols or Dystric Cambisols) was the oldest of the three soils and showed downward movement of some tracemetals (chromium and nickel) and principal elements (Fe and Mn)that was probably induced by long-term weathering.The extractability of manganese, zinc and barium with water washigher than other metals examined in all three soils. Lead andcobalt in soil-b and soil-KUR also were considered to have highextractability under long-term weathering processes. Zinc andlead accumulated near soil surface showed higher extractabilitywith every reagent used than those in deep layers of the three soils.
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  • 14
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    Environmental monitoring and assessment 60 (2000), S. 337-357 
    ISSN: 1573-2959
    Keywords: cellulose ; charcoal kiln ; decomposition ; herb seeds ; moisture ; respiration ; smoke pollution ; soil ; temperature
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Long-term charcoal production in small private charcoal kilns (CK) in Eastern Bieszczady Mts. (SE Poland) can cause local smoke contamination of the ambient forest environment. Responses of model soil systems, contaminated or not contaminated by CK smoke, to contrasting combinations of hydrothermic regimes were compared in laboratory microcosms (respiration of soil community, decomposition rate of soil organic matter and cotton stripes, herb seeds germination were studied). The majority of the obtained data show a markedly higher level of soil biological activity in the CK versus the control series. In some cases CK and control soil systems show different patterns of reactions to the tested combinations of microclimate regime. These phenomena should at least partly be attributed to the effects of CK pollution.
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  • 15
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    Environmental monitoring and assessment 61 (2000), S. 207-229 
    ISSN: 1573-2959
    Keywords: benthos ; birds ; diatoms ; ecologicalindicators ; integrated assessment ; fish ; lakes ; monitoring ; zooplankton
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Biological indicators of communitiestypically reflect a common environmental signalreflecting the general condition of the ecosystem, as well asindividual signals by indicators differentiallysensitive to particular environmental conditions. Wedescribe here a method of integrating and interpretingsuch indicators from 19 New England lakes for fivetaxonomic groups (diatoms, benthos, zooplankton, fish,and birds). Our approach provides a systematicstandardized way to integrate multiple metrics fromdifferent taxonomic groups by addressing four elementscrucial to analyzing data from multiple indicators: covariate control, re-scaling of data, standardizing the sign of responses, and dimensional reduction. We evaluated the biologicalmetrics against individual environmental stressors andagainst multivariate physicochemical metricscharacterizing general anthropogenic stress among thelakes. The method detected a response to variationin the gross environmental condition of the lakes thatwas correlated across taxa and metrics. In addition,a differential response to near shore conditions wasdemonstrated for fish. The success of the approach inthis study lends support to its general application toecological monitoring involving complex data sets.
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  • 16
    ISSN: 1573-2959
    Keywords: monitoring ; ecosystem processes ; conceptual modeling ; indicators ; human impacts
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Monitoring at large geographic scales requires a framework for understanding relationships between components and processes of an ecosystem and the human activities that affect them. We created a conceptual model that is centered on ecosystem processes, considers humans as part of ecosystems, and serves as a framework for selecting attributes for monitoring ecosystems in the Sierra Nevada. The model has three levels: 1) an ecosystem model that identifies five spheres (Atmosphere, Biosphere, Hydrosphere, Lithosphere, Sociocultural), 2) sphere models that identify key ecosystem processes (e.g., photosynthesis), and 3) key process models that identify the "essential elements"that are required for the process to operate (e.g., solar radiation), the human activities ("affectors") that have negative and positive effects on the elements (e.g., air pollution), and the "consequences"of affectors acting on essential elements (e.g., change in primary productivity). We discuss use of the model to select attributes that best reflect the operation and integrity of the ecosystem processes. Model details can be viewed on the web at http://www.r5.fs.fed.us/sncf/spam_report/index.htm(Appendix section).
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  • 17
    ISSN: 1573-3017
    Keywords: authorisation ; field research ; model ecosystems ; monitoring ; pesticides
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract On request of the Dutch government a committee of the Health Council of the Netherlands has reviewed the role that results of field research in its broadest sense (i.e., including multi-species toxicity tests in the laboratory, research on model ecosystems et cetera) can play in ecotoxicological risk assessment for the authorisation of pesticides. The Committee believes that field research can provide valuable additional data about the exposure of non-target organisms and the resultant effects at population, community and ecosystem level. However, it frequently is unclear how these data might be used in reaching a decision about authorisation. To solve this problem, it is necessary to specify what is understood by “unacceptable damage”. Both more clearly formulated protection goals of the government and a better understanding of the ecological significance of effects are needed to clarify this. Furthermore, the Committee points out that the statistical power of field trials must be sufficient to allow for the detection of changes that might be regarded as ecologically relevant. Finally, it recommends keeping a finger on the pulse in relation to authorised pesticides by monitoring their presence in environmental compartments and by investigating their role in suddenly occurring mortality among conspicuous animal species, such as birds, fish and honeybees. This kind of research forms a safety net for substances that have been wrongly authorised.
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  • 18
    ISSN: 1573-2932
    Keywords: acid precipitation ; acid vain ; Atlantic salmon ; LRTAP ; monitoring ; Nova Scotia ; rivers ; toxicity
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The Atlantic salmon (Salmo salar) resource of eastern Canada is impacted by acid rain in the Southern Upland (Atlantic Coast) area of Nova Scotia. Salmon runs in this area have become extinct in 14 rivers, are severely impacted in 20 rivers, and lightly impacted in 15 rivers. Water chemistry and fish communities in nine Southern Upland salmon rivers were studied from 1982 to 1996 as part of the effort to monitor the effects of the emission controlprograms in Canada and the United States. There hasbeen no statistically significant change in total ioncontent of Southern Upland river water, but there wasa significant decline in sulfate levels that was balanced by an increase in organic anions, and declines in calcium and magnesium that were balanced by increases in sodium and potassium. A geochemical scenario is proposed to account for these chemical changes. River water pH levels showed no overall linear trend, but at borderline toxicity sites the year-to-year variations in pH were correlated withchanges in juvenile salmon population densities. Tenfish species were collected, but none showed anysignificant overall time trend in population density.Fish species diversity was positively correlated with pH.
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  • 19
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    Water, air & soil pollution 121 (2000), S. 379-398 
    ISSN: 1573-2932
    Keywords: deciduous woodland ; Meathop Wood ; PAHs ; pasture ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A survey of PAHs in the soils of a mature,mixed-deciduous woodland and the surrounding pasturewas conducted along two transects. PAH `profiles'were not significantly different in the woodland soilcompared with the pasture. ΣPAH concentrations in thewoodland soil were significantly higher than soil fromthe surrounding pasture by a factor of 1.5–3 (P 〈 0.01), indicating enhanced deposition of PAHs to thesoil under the canopy via leaf litter, stemflow and/or through-fall. A deposition `edge effect' was onlyobserved at the windward edge of the canopy where thenumber and density of aerial and basal stems washighest (P 〈 0.05). The influence of predominantwest/south-westerly winds was observable in the lackof an edge effect at the leeward edges, and the higherΣPAH concentrations in the predominantly leewardpasture compared to the windward pasture (P 〈 0.05).
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  • 20
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    Water, air & soil pollution 122 (2000), S. 203-229 
    ISSN: 1573-2932
    Keywords: housedust ; IEUBK model ; metals ; risk assessment ; scanning electron microscopy ; sequential extraction ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Soils and housedusts were collected from three areas of Pribram,an historic metal mining and smelting town in the Czech Republic. The main objectives of the study were: (i) to assessthe influence of physico-chemical form, particle size, soilproperties and contaminant source on Pb bioavailability andexposure risk; (ii) compare the Pb bioavailability data obtainedfrom the mining and smelting areas and assess whether anydifferences observed could be attributed to the factors thoughtto exert an influence. Lead concentrations were highest in thesmelter area. Mining area garden soils also contained elevatedPb concentrations. Solubility of housedust Pb in 0.12 M HCl (asurrogate for stomach acid) was similar in all study areas andwas similar to values reported in the literature. However, 0.12M HCl solubility of garden soil Pb was low in the mining areacompared to the other study areas and compared to other urbanareas. Blood Pb concentrations were also relatively low in themining area compared to the other study areas and the reducedsoil Pb solubility observed in this area was suspected as aninfluencing factor. However, exposure pathways may also beimportant in explaining the differences observed.
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  • 21
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    Water, air & soil pollution 122 (2000), S. 93-103 
    ISSN: 1573-2932
    Keywords: base saturation ; deposition ; forest ecosystems ; monitoring ; regeneration ; soil acidification ; total acid load
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Between 1993 and 1995 a system of six intensive monitoring stations in representative stands of Norway spruce (Picea abies), sessile oak (Quercus robur) and Scots pine (Pinus sylvestris) were installed in forests of Saxony (Germany), they are integrated in the European Level II - Programme. As a complementary system, and in addition to the annual nation-wide forest decline survey, 280 sites within the forest soil condition survey (European Level I - Programme) have been examined since 1992. The results of deposition monitoring show that until 1997 the acidity in precipitation and troughfall still was very high, despite of strong reductions in industrial emissions between 1989 and 1992. The annual fluxes (hydrological year 1996) of sulphur in throughfall ranged between 16 and 77 kg-ha-1, whereas the fluxes of total inorganic N varied between 17 and 46 kg-ha-1. The forest soils show high degrees of acidification with only low base saturation. In most cases the nutrient status of the soils has to be improved in the course of a regeneration programme in order to rebuild more natural forest ecosystems.
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    Water, air & soil pollution 122 (2000), S. 281-297 
    ISSN: 1573-2932
    Keywords: landfill ; leachate ; monitoring ; MSW ; prediction ; refuse
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Parameters such as pH, concentrations of Cl-, turbidity,NH3-N, CODCr and BOD5 (simplified as COD and BODrespectively in the following text) in leachate generated inthe large-scale testing landfill unit and closed landfill unitsat Shanghai Refuse Landfill were monitored from April 1995 toOctober 1998. The mathematical simulation formula between theseparameters and refuse age were established based on the dataobtained from the testing landfill unit and justified by thedata obtained at the closed landfill units from 1989 to 1993.The long-term predictions for the leachate concentrations forthe Landfill were made using the mathematical simulation formulaestablished. It was predicted that the COD and BOD may bereached to the strictest standard for pollution control on municipal solid wastes landfill in China, i.e., COD 〈 100 mg L-1 and BOD 〈 30 mg L-1, after 15 yr natural attenuation. The time predicted for NH3-N concentrations to reach the discharging standard, 15 mg L-1, was found to be at least 23–26 yr or even longer. The predictions for concentrations of Cl-, turbidity, and pH values in leachate are also given. The natural attenuation of Cl- is the slowest and might be decreased to 200 mg Cl- L-1, the agricultural irritation standard, after at least 58 yr.
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    Water, air & soil pollution 123 (2000), S. 159-166 
    ISSN: 1573-2932
    Keywords: coagulation ; Cryptosporidium ; filtration ; Giardia ; monitoring ; turbidity
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The most commonly used water filtration technique involves coagulation and rapid rate filtration, either in conventional plants with flocculation and sedimentation, or in direct filtration plants in which the sedimentation process is omitted. Both versions of coagulation and filtration can be effective for controlling Giardia cysts and Cryptosporidium oocysts, but research done by several investigators has shown that coagulation and filtration must be operated very carefully to attain the best results. When filtered water turbidity is 0.1 ntu or lower, the process is most effective. Careful control of coagulation chemistry and of filtration rate increases, continuous monitoring of filtered water turbidity, and proper management of backwash water are keys to successful filtration.
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    Water, air & soil pollution 119 (2000), S. 139-156 
    ISSN: 1573-2932
    Keywords: aldicarb ; herbicides ; insecticides ; monitoring ; organochlorine ; organophosphate ; surface water
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A survey was conducted of pesticide distribution in the water ofthe upper Jordan basin, due to the importance of its quality asthe main source of drinking water in Israel.A preliminary survey of pesticide distributers and farmersrevealed intensive use of many pesticides in agriculture. Fourof these were selected as targets for monitoring in the surfacewater of the region, at seven sampling stations. The highestresidue found was of aldicarb and its metabolites, with lowercontent of organophosphate and organochlorine insecticides. Noconcentrations reached the maximum levels permitted by the EPAfor drinking water, but recommendations were made, nonetheless,for continuous monitoring of pesticides in the region.Subsequent monitoring (1993–1997) showed a steady decrease in aldicarb residues.
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  • 25
    ISSN: 1573-2932
    Keywords: denitrification ; ferrous iron ; field test ; hypoheiczone ; nitrate removal ; riparian zone ; soil ; stream export
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In regions with intensive agriculture and shallow hydrological systems, headstreams are often polluted with nitrate even at the springs. In North-West France, nitrate concentration was seen to decrease downstream during baseflow conditions when the stream flows on granite, but this does not occur on schist. In order to explain this difference in behaviour, we analysed the groundwaters and surveyed the redox conditions (using a field test for ferrous iron) in near-bank wet meadows as well as in the hyporheic zone. We show that the wet meadow groundwater was denitrified and that oxygen and nitrate were presentaround the stream channel in a wide zone on granite,compared with a very restricted zone on schist. Ongranite, exchanges between the stream and the hyporheic zone are favoured by sandy or peaty material having high hydraulic conductivity. This gives rise to two processes (1) lateral inflow of denitrified water from wet meadows, (2) in the opposite direction, supply of stream nitrate to denitrification sites in the hyporheic zone. In the second case, a high hydraulic conductivity also reduces the water residence time and limits denitrification, resulting in high levels of oxygen and nitrate. On schist, the low hydraulic conductivity prevents an efficientconnection between surface and subsurface waters.
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    Water, air & soil pollution 118 (2000), S. 395-406 
    ISSN: 1573-2932
    Keywords: forest litter ; mapping ; nuclear test ; radioactive contamination ; Russia ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The results of the extensive measurements ofCesium-137 (137Cs) in virgin soils, plants,forest litter and lake bottom sediments of AltayRegion in 1992–1995 are presented. Analyses of thevertical soil profiles indicate that 137Cs ispresent in the upper 5–20 cm of the soil. Crops andthe majority of wild plants show no signs ofcontamination with 137Cs even in areas where soilis contaminated. A regional map of 137Csconcentration is presented, which shows a highlyirregular pattern of radio-cesium deposition from thenuclear tests on the Semipalatinsk Nuclear Polygonbetween 1949 to 1962. This kind of lateraldistribution of 137Cs in Altay virgin topsoilscannot be accounted for only by the distance from thenuclear testing site, on the contrary, it seems to bepredominantly dependent on the weather conditions anda pattern of rainfall at the time of Semipalatinskexplosions. The article discusses the factors causingthe post-precipitation redistribution of 137Cs inthe soil column and demonstrates that forest litter,lichen and lake bottom sediments can be used assensitive indicators of the historical and currentradioactive contamination.
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  • 27
    ISSN: 1573-2932
    Keywords: Everglades ; mercury ; mobility ; peat ; phosphorus ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Soils in the southern half of Water Conservation Area3A are mostly peats with some organic-rich marls. Mercury contents of 64 surface samples over a500 km2 area average 28.7 ng cc-1 (209 ppb drysediment), which is typical of organic-rich soils. High Hg contents in Everglades fish are therefore notcaused by anomalously high soil Hg. Hg contents showno systematic lateral variation, consistent withdeposition from well-mixed atmospheric sources ratherthan nearby point sources or runoff from canals.Cores from 9 sites contain more Hg and P at or nearthe surface than at 20–30 cm depth. Hg and P contentsof individual cores correlate well and define separatebackground and anomalous populations. The subsurfacedistribution of P is determined largely by uptake bysawgrass and other plants. The correlation between Pand Hg suggests that, although atmospheric Hgdeposition has undoubtedly increased in recentdecades, postdepositional mobilization of Hg may beimportant in Everglades soils. This finding, togetherwith recent direct measurements of atmospheric Hgdeposition, indicates that previous estimates of Hgdeposition rates based on Everglades peat cores, whichassumed that Hg is immobile in peat after deposition,have yielded large overestimates.
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    Environmental monitoring and assessment 56 (1999), S. 269-291 
    ISSN: 1573-2959
    Keywords: grid approach ; mapping ; monitoring ; National Forests ; purposive sampling ; random sampling ; statistical inventory
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A forest ecological inventory and monitoring system combining information derived from maps and samples is proposed based on ecosystem regions (Bailey, 1994). The system extends the design of the USDA Forest Service Region 6 Inventory and Monitoring System (R6IMS) in the Pacific Northwest of the United States. The key uses of the information are briefly discussed and expected results are illustrated with examples. The system is flexible, allowing regions based on ecological considerations to be modified. Sampling intensities that are affordable are likely to be insufficient to provide meaningful estimates for key parameters relating to rare and endangered species, watersheds, and other ecological units. Methods are proposed for collecting additional information in follow-up surveys and combining it with relevant information obtained in R6IMS. Near-continuous information on weather and possible pollution variables recorded by instruments at sampling sites is needed to develop meaningful models to understand what is happening in the ecoregions. R6IMS and the proposed additions constitute a dynamic system which will be modified further as data are analyzed.
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    Environmental monitoring and assessment 57 (1999), S. 1-20 
    ISSN: 1573-2959
    Keywords: dissolved oxygen ; EMAP ; estuary ; Gulf of Mexico ; monitoring
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Because deficient dissolved oxygen (DO) levels may have severe detrimental effects on estuarine and marine life, DO has been widely used as an indicator of ecological conditions by environmental monitoring programs. The U.S. EPA's Environmental Monitoring and Assessment Program for Estuaries (EMAP-E) monitored DO conditions in the estuaries of the Gulf of Mexico from 1991 to 1994. DO was measured in two ways: 1) instantaneous profiles from the surface to the bottom were taken during the day, and 2) continuous measurements were taken near the bottom at 15 min intervals for at least 12 h. This information was summarized to assess the spatial distribution and severity of DO conditions in these estuaries. Depending on the criteria used to define hypoxia (DO concentrations usually 〈2 mg L-1 or 〈5 mg L-1) and the method by which DO is measured, we estimate that between 5.2 and 29.3% of the total estuarine area in the Louisianian Province was affected by low DO conditions.
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    Environmental monitoring and assessment 59 (1999), S. 191-209 
    ISSN: 1573-2959
    Keywords: estimation ; geostatistics ; interpolation ; radionuclides ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Many environmental surveys require the implementation of estimation techniques to determine the spatial distribution of the variable being investigated. Traditional methods of interpolation and estimation, for example, inverse distance squared and triangulation often ignore features of the data set such as anisotropy which may have a significant impact on the quality of the estimates produced. Geostatistical techniques may offer an improved method of estimation by modelling the spatial continuity of the variable using semi-variogram analysis. The theoretical model fitted to the semi-variogram is then used in the assignation of weighting factors to the samples surrounding the location to be estimated. This paper outlines the results of a comparison between three common estimation methods, polygonal, triangulation and inverse distance squared and a geostatistical method, in the estimation of soil radionuclide activities. The geostatistical estimation method known as kriging performed best over a range of parameters used to test the performance of the methods. Kriging exhibited the best correlation between actual and estimated values, the narrowest error distribution and the lowest overall estimation error. Polygonal estimation was best at reproducing the data set distribution. Conditional bias was evident in all the methods, low values being over-estimated and high values being under-estimated.
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  • 31
    ISSN: 1573-3017
    Keywords: Swainson's hawk ; monocrotophos ; ecotoxicology ; monitoring ; mortality
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Approximately 6,000 dead Swainson's hawks (Buteo swainsoni) were discovered in the Pampas of Argentina in 1995–96. Subsequent meetings held between Argentine, US, Canadian, and Swiss personnel led to an agreement whereby chemical companies removed the organophosphate (OP) monocrotophos (MCP) from the area where mortalities had occurred in northern La Pampa province. We monitored hawks in the MCP exclusion zone from 28 November 1996 through 25 January 1997. We sampled 133 hawks for exposure to anti-cholinesterase insecticides, 131 of which showed no apparent signs of adverse effects. Two hawks had inhibited ChE that recovered over time. Feather and footwash samples from captured birds were tested for OP residues. One feather sample was positive for dimethoate; no footwash sample was positive for any of the OPs screened. Cholinesterase (ChE) activities from hawks in Argentina were (mean±SE, n=131) 0.674±0.014 total ChE, 0.236±0.006 acetylcholinesterase (AChE), and 0.438±0.013 butyrylcholinesterase (BChE). Mean plasma AChE from Argentine hawks was significantly depressed below North American reference values. Total ChE and BChE activities were not significantly different. Mortality due to OP poisoning was not found in the MCP exclusion zone in northern La Pampa, though it continued outside of the zone where MCP was used, both legally and illegally. Education campaigns and extension efforts, emphasizing the local MCP restrictions, were effective in controlling Swainson's hawk mortalities in the study area where substantial mortality occurred the previous two years.
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    Mitigation and adaptation strategies for global change 4 (1999), S. 43-60 
    ISSN: 1573-1596
    Keywords: carbon offsets ; emission trading ; energy efficiency ; evaluation ; forestry ; global climate change ; greenhouse gas emissions ; joint implementation ; monitoring ; reporting ; verification
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering , Geography
    Notes: Abstract Because of concerns with the growing threat of global climate change from increasing emissions of greenhouse gases, the United States and other countries are implementing, by themselves or in cooperation with one or more other nations, climate change projects. These projects will reduce greenhouse gas (GHG) emissions or sequester carbon, and will also result in non-GHG benefits (i.e., environmental, economic, and social benefits). Monitoring, evaluating, reporting, and verifying (MERV) guidelines are needed for these projects to accurately determine their net GHG, and other, benefits. Implementation of MERV guidelines is also intended to: (1) increase the reliability of data for estimating GHG benefits; (2) provide real-time data so that mid-course corrections can be made; (3) introduce consistency and transparency across project types and reporters; and (4) enhance the credibility of the projects with stakeholders. In this paper, we review the issues involved in MERV activities. We identify several topics that future protocols and guidelines need to address, such as: (1) establishing a credible baseline; (2) accounting for impacts outside project boundaries through leakage; (3) net GHG reductions and other benefits; (4) precision of measurement; (5) MERV frequency and the persistence (sustainability) of savings, emissions reduction, and carbon sequestration; (6) reporting by multiple project participants; (7) verification of GHG reduction credits; (8) uncertainty and risk; (9) institutional capacity in conducting MERV; and (10) the cost of MERV.
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  • 33
    ISSN: 1572-9729
    Keywords: bioremediation ; composting ; petroleum ; soil ; thermophilic
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract The effects of the C/N ratio, CaCO3 and PO4 addition, and temperature profile on reactor-based composting of weathered hydrocarbon-contaminated soil were evaluated in a series of 30-day tests in temperature-controlled mini-composters. Soil containing 17,000 mg (kg dry soil)−1 mineral oil and grease (MOG) was composted with maple leaves and alfalfa. Although the leaves and alfalfa also contained MOG, degradation of contaminated soil derived MOG (total MOG degradation minus MOG degradation in a control with no soil) increased from 0 to 45% as the quantity of co-substrate increased from 0 to 63%. Simulation of biopile conditions (i.e., aeration and addition of mineral salts but no co-substrate) resulted in only 6% MOG degradation. Addition of CaCO3 before composting increased total MOG degradation from 23% to 43%. Total MOG degradation increased with decreasing C/N ratio. At a molar C/N ratio of 17, 43% of the total MOG was degraded in 30 days, while at a C/N ratio of 40 there was no total MOG degradation. When temperatures ranging from 23 to 60 °C were investigated, 50 °C maintained for 29 days resulted in the maximum degradation which was 68% of total initial MOG.
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    Environmental monitoring and assessment 55 (1999), S. 279-298 
    ISSN: 1573-2959
    Keywords: biological indicators ; change ; epilithic lichens ; global climate ; Israel ; monitoring ; Negev desert
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The issue of biological monitoring of the local consequences of anticipated global climate change is considered for the Central Negev Highlands, Israel. Epilithic lichens are suggested as biological monitors. The proposed methodology of such monitoring consists of a sampling scheme, including lichen measurement along transects on flat calcareous rocks, and construction of a trend detection index (TDI). TDI is a sum of lichen species cover with coefficients chosen so as to ensure maximum ability to detect global climate trends. Coefficients have been estimated in a study of lichens along an altitudinal gradient from 500 to 1000 m a.s.l. The gradient study demonstrated that the TDI index is performed better than other integrated indices. Recommendations on this system to monitor climate change with epilthic lichens are given. Measuring, for instance, a hundred transects in fifty plots (two transet per plot scheme) allows one to detect a climate-driven change in the epilithic lichen community corresponding to a 0.8 °C shift in annual mean temperature. Such resolution appears sufficient in view of global warming of 2.5 °C considered by the Intergovernmental Panel on Climate Change as a realistic prediction for the end of the next century.
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    Environmental monitoring and assessment 58 (1999), S. 121-131 
    ISSN: 1573-2959
    Keywords: bioaccumulation ; Italy ; lichens ; soil ; trace elements
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Total concentrations of Al, Ba, Cd, Co, Cr, Cu, Fe, Mn, Mo, Pb, Sr, Ti, V and Zn in the epiphytic lichen Parmelia sulcata and superficial soils from 60 remote sampling sites in Tuscany (central Italy) were determined to evaluate the contribution of soil to the elemental composition of the lichen. The results showed that in the Mediterranean environment, the trace element content of unwashed lichen samples is greatly affected by soil contamination. However, despite the strong correlations between the concentrations of lithogene elements such as Al, Fe and Ti in P. sulcata, lichen levels of these elements were not at all linearly correlated with their concentrations in the soil, suggesting that dust contamination is highly variable and probably dependent on local site characteristics. All methods evaluated to minimize soil contamination indicated Cu, Pb and Zn as elements of atmospheric origin. However, while levels of Pb were similar to those reported for background areas, moderate pollution by Cu and Zn, probably from fertilizers used in agriculture, was revealed. For elements such as Cd and Mo, identified as atmophile, some uncertainty exists due to the fact that they are essential for lichen metabolism and accumulate intracellularly in lichens; they may therefore occur in soluble form in the lichen thallus.
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    Water, air & soil pollution 112 (1999), S. 259-278 
    ISSN: 1573-2932
    Keywords: forest ; municipal sludge ; nitrogen ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Nitrogen dynamics were assessed for a forested site in southern New Hampshire during the first and second growing seasons after surface application of an aerobically-digested, limed, liquid municipal sludge. Sludge was applied in June 1989, at 3.3, 6.9, and 14.5 M ha-1 (or 199, 396, and 740 kg TKN ha-1). Elevated net N mineralization (in situ buried bags) occurred in the organic and upper mineral soil horizons during the first two months after sludge application, but was similar to control levels thereafter. Net N mineralization was negligible at 30 and 60 cm soil depths. Foliar N concentration increased with sludge loading rates. Concentrations of NH4+ and NO3- in soil leachate were low, except in early fall when microbial activity was still high and plant demand was low. In trenched subplots where vegetative uptake was eliminated, NO3- concentrations in soil leachate (60 cm) rose to between 15 and 35 mg N L-1 in the first year and remained high in the second year. Other studies reported higher magnitudes of NO3- leaching from treated plots. These studies and the findings reported here shown the characteristics of the sludge being applied to land are at least as important as the physical and chemical characteristics of the site to which they are to be applied.
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    Water, air & soil pollution 113 (1999), S. 77-95 
    ISSN: 1573-2932
    Keywords: extraction ; hydraulic conductivity ; lead ; soil
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    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Extraction using ethylenediaminetetraacetic acid (EDTA), and other chelates has been demonstrated to be an effective method of removal of Pb from many contaminated soils. However, column leaching of Pb from alkaline soils with EDTA has been problematic due to extremely low soil permeability. The first purpose of this study was to develop batch extraction procedures and methods of analysis of batch extraction data to provide Pb solubility information which can be used to model the column extraction of Pb from soils. The second purpose was to determine the effect of the addition of KOH and CaCl2 to K2H2EDTA extract solution on both hydraulic conductivity and Pb removal. A Pb-contaminated soil sample was collected from an abandoned battery recycling facility. Both batch shaker extractions and column leaching experiments were completed using 5 different EDTA extract solutions. When only CaCl2 was added to EDTA no change in the amount of Pb removed by batch extraction was observed. As expected, lead solubility was observed to decrease as pH was increased by the addition of KOH. However, Pb solubility was only slightly decreased by the addition of both CaCl2 and KOH. The amount of time required to leach 6.0 L of extraction solution through the soil columns varied from 2 to 33 days. The addition of CaCl2 and/or KOH resulted in increased soil hydraulic conductivity relative to the EDTA-only solution. The hydraulic conductivity was related to residual calcium carbonate content, suggesting that dissolution of CaCO3 and subsequent production of CO2 gas in the soil pores was partially responsible for the observed reductions in soil permeability. However, Pb removal was diminished with the addition of CaCl2 and KOH because of the decreased Pb solubility and also kinetic limitations associated with the shorter residence time of the extract solution in the column.
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    Environmental monitoring and assessment 57 (1999), S. 183-194 
    ISSN: 1573-2959
    Keywords: gas chromatography and ultraviolet spectroscopy ; organic compounds ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Samples of compost-amended soil from waste dumping sites in Lagos Metropolis were extracted with dichloromethane (3 × 20 cm3) and the extract was evaporated at 35 °〉C. The residue was extracted with 2,2,4-trimethylpentane, and portions of the solution were applied to a column containing silica gel from which aliphatic and aromatic hydrocarbons were eluted with n-hexane and toluene respectively. Analysis of the n-hexane fraction using gas chromatography showed the presence of a mixture of aliphatic hydrocarbons, ranging from C9 to C25, while ultraviolet analysis of the toluene fraction suggested 1,2-benzanthracene; 2,3-benzphenanthrene, chrysene and pyrene as polyaromatic compounds present in samples analyzed. The crude extracts were highly coloured and viscous. Total extractable organic residues in the 2,2,4-trimethylpentane extracts ranged from 36 to 89 mg g-1 of soil.
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    Environmental monitoring and assessment 59 (1999), S. 47-72 
    ISSN: 1573-2959
    Keywords: flow-normalisation ; long-term trends ; monitoring ; nitrogen ; riverine load ; statistical analysis
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Concern about nitrogen loads in marine environments has drawn attention to the existence and possible causes of long-term trends in nitrogen transport in rivers. The present study was based on data from the Swedish environmental monitoring programme for surface water quality; the continuity of these data is internationally unique. A recently developed semiparametric method was employed to study the development of relationships between runoff and river transport of nitrogen since 1971; the observed relationships were then used to produce time series of flow-normalised transports for 66 sites in 39 river basins. Subsequent statistical analyses of flow-normalised data revealed only few significant downward trends (p ≤0.05) during the time period 1971–1994, and the most pronounced of these downward trends were caused by reduced point emissions of nitrogen. The number of significant upward trends was substantially larger (15 for total-N and 18 for NO3-N). Closer examination of obtained results revealed the following: (i) the most pronounced upward trends were present downstream of lakes, and (ii) observed increases in nitrogen transport coincided in time and space with reduced point emissions of phosphorus or organic matter. This indicated that changes in the retention of nitrogen in lakes were responsible for the upward nitrogen trends. The hypothesis that nitrogen saturation of forest soils has caused a general increase in the riverine export of nitrogen from forested catchments in Sweden was not confirmed. Neither did the results indicate that improved agricultural practices have reduced the export of nitrogen from agricultural catchments.
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    Water, air & soil pollution 114 (1999), S. 121-135 
    ISSN: 1573-2932
    Keywords: acid rain ; aluminium ; groundwater ; mountainousenvironment ; Nordic countries ; precipitates ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Areas a few square metres in size, devoid of higher vegetation other than moss, have been mapped at 600–700 m above sea level in the mountains of the western part of central Norway. The moss is covered by a grey precipitate during dry summer periods. The precipitate has been identified by ICP-AES analysis of HNO3-extract, X-ray diffraction (XRD) and by scanning electron microscopy (SEM) as an aluminium(Al)-hydroxide, probably amorphous Al-hydroxide and diaspore (Al(OH)3), containing 21–25% Al by weight. In comparison, the underlying moraine deposits contain 1.5–3.5% Al by weight. A small spring, where groundwater discharges, is located uphill of each contaminated area. The Al content of the water which emerges from these springs decreases downhill away from the spring and is inversely proportional to the pH. The runoff waters originating at the springs have been modelled using the computer-codes MINTEQA2 and ALCHEMI and are found to be saturated with respect to amorphous Al(OH)3. This study raises the very important question as to what extent a lower pH in the influent meltwater may leach out more aluminium and possibly lead to the formation of larger amounts of precipitate.
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    Water, air & soil pollution 115 (1999), S. 337-346 
    ISSN: 1573-2932
    Keywords: natural organic structures ; pentachlorophenyl adsorption ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The adsorption of pentachlorophenol (PCP) on a soil was studied by equilibrating the soil (with and without its indigenous organic matter) with PCP in the presence and the absence of added natural organic species (benzoic acid, lactic acid, glucuronic acid and catechol). Both the added organic species and the indigenous organic matter were found to enhance PCP adsorption, the enhancement being greater with benzoic acid than with the less hydrophobic lactic acid. Adsorption of these organic species was also enhanced by PCP, suggesting the existence of a co-operative adsorption mechanism.
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    Water, air & soil pollution 114 (1999), S. 171-184 
    ISSN: 1573-2932
    Keywords: cadmium ; plant uptake ; soil ; Salix
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Cadmium concentrations in Salix (willow) shoots are generally high and Salix can therefore potentially remove significant amounts of Cd from soil. The aim of this study was to investigate how long-term Salix cultivation had affected total and plant available Cd concentrations in agricultural soil. The study was made in 8 to 30 yr old plantations. Soil profiles down to 65 cm depth were sampled and conditions within the plantations were compared to those in nearby reference areas. When consideration was given to certain pH differences, concentrations of exchangeable Cd throughout the soil profiles were significantly lower in the Salix stands than in the reference areas. However, the effect on concentrations of total Cd was negligible. The yield levels proved not to be optimal and Cd concentrations in shoots were lower than average in the investigated stands. Data on exchangeable Cd show that uptake occurs throughout the soil profile and the Cd pool involved is thus large. These facts may explain why total concentrations were only slightly influenced. The conclusion reached was that Salix cultivation reduces the amount of plant-available Cd in the soil. However, more investigations are needed to evaluate how this effect can be optimized by choice of clone and other management measures.
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  • 43
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    Water, air & soil pollution 114 (1999), S. 155-170 
    ISSN: 1573-2932
    Keywords: adsorption ; extraction ; herbicide ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The adsorption of herbicides on soil colloids is a major factor determining their mobility, persistence, and activity in soils. Solvent extraction could be a viable option for removing sorbed contaminants in soils. This study evaluated the extractability of three herbicides: 2,4 dichlorophenoxy-acetic acid (2,4-D), 4-chloro-2-methylphenoxypropanoic acid (mecoprop acid or MCPP), and 3,6-dichloro-2-methoxybenzoic acid (dicamba). Three solvents (water, methanol, and iso-propanol) and three methods of extraction (column, batch, and soxhlet) were compared for their efficiencies in removing the herbicides from three soils (loamy sand, silt loam, and silty clay). Both linear and non-linear Freundlich isotherms were used to predict sorption intensity of herbicides on soils subjected to various extraction methods and conditions. High Kdand Kfr, and low N values were obtained for all herbicides in silty clay soil by batch extraction. Methanol was the best solvent removing approximately 97% of all added herbicides from the loamy sand either by column or soxhlet extraction method. Isopropanol ranked second by removing over 90% of all herbicides by soxhelet extraction from all three soils. However, water was ineffective in removing herbicides from any of the soils using any of the three extracting procedures used in this study. In general, the extent of herbicide removal depended on soil type, herbicide concentration, extraction procedure, solvent type and amount, and extraction time.
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  • 44
    ISSN: 1573-2932
    Keywords: dry deposition ; dry deposition velocity ; forest ; monitoring ; surface resistance ; SO2
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In 1990 a project to develop a dry deposition monitoring method of SO2, NH3 and NO2 to Speulder forest in the Netherlands began. Detailed annual deposition fluxes for these gases were measured throughout November 1992 to December 1995. This paper describes the measurement set-up and the analysis of the deposition parameters for SO2. The dry deposition velocity was usually smaller than the maximum Vd, showing a resistance to surface uptake, except for periods when the canopy is wet and surface resistance is negligible. Several methods were tested to estimate annual average fluxes from the gradient measurements. Annual fluxes were estimated by selecting the data for periods fulfilling gradient theory and extending the data by using an inferential method for the other periods. The surface resistance parametrisation used in the inferential method was tested using the selected data and was found to yield systematic larger fluxes of the order of 20%. Annual fluxes were 465 mol ha-1 a-1 in 1992/1993, 460 mol ha-1 a-1 in 1994 and 330 mol ha-1 a-1 in 1995. The uncertainty in the annual flux was estimated to be 25%. The annual average dry deposition velocity was 1.5 cm s-1. No large differences were found in deposition parameters between each of the three years.
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  • 45
    ISSN: 1573-2932
    Keywords: atmospheric deposition ; mining area ; SO2 emission ; soil ; sulfur isotopes ; Sweden
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Mining activities for almost thousand years have caused large S emissions in the Falun area, central Sweden. Since the beginning of the 20th century, the S deposition has decreased considerably. The soil S concentrations and S isotope compositions were analyzed for ΣS and adsorbed SO42- for three soil profiles close to the mining area in order to identify the soil S sources. The δ34S values were found to be different for ΣS and adsorbed SO42- and ranged from –3.7‰ to +2.6‰. In the B-horizon, the observed ΣS δ34S values (and hence calculated δ34S values for organic S) were mostly lower than those of the adsorbed SO42-. In the O-horizon, ΣS showed similar δ34S values as the adsorbed SO42- in the mineral soil. The adsorbed SO42- showed nearly constant δ34S values with depth. The δ34S values in the soils are interpreted to reflect a mixture of historical and modern deposition due to soil S circulation with no or negligible fractionation. The lower δ34S values of organic S in the B-horizon suggests preservation of acid deposition originating from mining activities back in time. The adsorbed SO42- in the mineral soil and the organic S in the O-horizon reflect a response to a new δ34S composition in the atmosphere due to fossil fuel burning during the 20th century.
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  • 46
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    Water, air & soil pollution 115 (1999), S. 321-335 
    ISSN: 1573-2932
    Keywords: grain yield ; irrigation ; refinery waste water ; seed quality ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Field experiments were conducted to evaluate the impact of petrochemical industry waste water on certain physico-chemical properties of soil and on growth, yield and quality of corn (Zea mays L.) and mustard (Brassica juncea L. Czern and Coss). The pH of the waste water was near about neutral but it contained a higher amount of nitrogen, potassium, phosphate, sodium, chloride, calcium, carbonates, bicarbonates and suspended and dissolved solids when compared with fresh water. Soil receiving the waste water showed no significant changes in water soluble salts, electrical conductivity, cation exchange capacity, pH, total organic carbon etc. Moreover, waste water irrigation resulted in increased growth and yield of both the crops. Thus, it may be concluded that the petrochemical industry waste water may be used profitably for the cultivation of corn and mustard.
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  • 47
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    Water, air & soil pollution 110 (1999), S. 421-432 
    ISSN: 1573-2932
    Keywords: calcium ; coal fly ash ; gypsum ; pH ; selenium ; soil ; sulfur ; trace element
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Selenium, a potentially toxic trace element, is present in coal fly ash and is accumulated by plants growing on ash landfills. Application of gypsum (CaSO4·2H2O) can reduce Se accumulation. The persistence of this effect and the efficacy of repeated gypsum applications were investigated in forbs and grasses on a soil-capped, fly ash landfill near Lansing, New York. Gypsum was applied as a top-dressing at a rate of 0 or 11.2 t ha-1 in 1990 to three plots, and one-half of each of these plots received an additional top dressing of gypsum at 11.2 t ha-1 in 1991, producing four treatments – no gypsum, gypsum only in 1990, gypsum only in 1991, and gypsum in both years. Vegetation was harvested in July and October of 1991 and in July of 1992 and analyzed for Se, S, and Ca. Application of gypsum: (1) decreased Se accumulation by forbs and grasses harvested later in the season; (2) decreased Se accumulation in a subsequent year; (3) produced no further decrease when reapplied in a second year; and (4) did not decrease Se accumulation two years after a single application. The decrease in Se accumulation was not due to dilution caused by S fertilization. Variation in Se accumulation was not explained by variation in the pH and Se concentration of the soil and ash.
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  • 48
    ISSN: 1573-2932
    Keywords: bioassays ; bioremediation ; microbiology ; PCP ; soil ; toxicity
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Five bioassays were used to measure toxicity during bioremediation of a soil contaminated with pentachlorophenol (PCP; 335 ppm), polycyclic aromatic hydrocarbons (PAHs; 1225 ppm) and petroleum hydrocarbons (19 125 ppm). Different bioremediation treatments were tested in soil microcosms including amendment with phosphorus and/or PCP-degrading Pseudomonas sp. UG30, either as free cells or encapsulated in κ-carrageenan. Soil toxicity was monitored using the solid-phase Microtox test, SOS-chromotest, lettuce seed germination, earthworm survival and sheep red blood cell (RBC) haemolysis assays. PCP levels were reduced in all treatments after 210 days. The RBC lysis assay, Microtox test and SOS-chromotest indicated reduced toxicity in most of the microcosms by day 210. Trends depicted by lettuce seed germination and earthworm survival LC50 values varied with each treatment. For example, in soil amended with phosphorus, both the seed germination and earthworm survival LC50 data suggested increased soil toxicity. However, for soil treated with encapsulated Pseudomonas sp. UG30 cells, the earthworm survival LC50 data indicated reduced toxicity while seed germination LC50 values showed little change from values obtained prior to bioremediation. Our results show that toxicity trends in a contaminated soil during bioremediation differ according to the assay used.
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  • 49
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    Water, air & soil pollution 109 (1999), S. 163-178 
    ISSN: 1573-2932
    Keywords: cadmium ; copper ; lead ; MSW-biosolids compost ; MSW compost ; soil ; zinc
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The goal of this study was to measure the As, Cu, Fe, Pb and Zn contents of soils amended with municipal solid waste (MSW) and MSW-biosolids compost and to determine the long-term transport of these metals to lower soil horizons. Lead, Cu, Cd and Zn contents in the composts were 3–20 times more concentrated in the compost compared to the soil at the Calverton, NY, U.S.A. farm. As a result, Pb, Cd, Cu and Zn were elevated in the upper 5 cm soil layer following compost application and the metal enrichment was proportional to the amount of compost applied (21–62 Mg ha-1). In addition, Pb, As and Cu contents of the non-compost amended Calverton soils were enriched above the tillage depth (20–25 cm). Cu, Pb and As enrichment was attributed to the historical use of sodium arsenite, lead arsenate and copper sulfate insecticides and fungicides. Results of the metal analyses of soil cores collected 16 and 52 months following compost application showed that Cu, Zn and Pb remained confined to the upper 5 cm soil layer. The low water extractable fraction of these metals in MSW and MSW-biosolids compost was a major factor limiting the transport of these metals to lower soil horizons. In contrast, Cd leaching from the upper 0–5 and 5–10 cm soil layers was continuous over the 52 month study period and was attributed primarily to the presence of soluble Cd in phosphate fertilizer initially applied to the Calverton farm soil.
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  • 50
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    Water, air & soil pollution 111 (1999), S. 171-186 
    ISSN: 1573-2932
    Keywords: denitrification ; microorganisms ; nitrate ; riparian ; soil ; temperate ; vegetation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Excess nitrate (NO3-) in lakes and streams has deleterious effects for environmental and human health. Nitrate concentrations have become problematic in agricultural watersheds due to increased use of fertilizers and improper management of livestock wastes. Research has indicated that the planting and/or preservation of riparian buffer zones can be an effective means of reducing pollution from agricultural fields (Osborne and Kovacic, 1993; Jordan et al., 1992; Simmons et al., 1992). Biological denitrification is the most desirable means of nitrate attenuation as the microbial conversion of NO3- removes nitrate from the watershed in the form of N gases. Despite the inherent value of biological denitrification, a comprehensive review discussing the role of this process in removing nitrate from riparian zones is lacking. In this paper we examine the results and conclusions of past research on the topic of denitrification in riparian zones and make recommendations for future research in this area. The need for subsurface denitrification assays in riparian zones is emphasized.
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  • 51
    ISSN: 1573-2932
    Keywords: analysis ; phase ; selective ; sequential extraction ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Two selective extraction schemes, that commonly known as Tessier's and that used by the Geological Survey of Canada (GSC), are compared. The nominal phases identified include: adsorbed/exchangeable/carbonate, ‘AEC’; amorphous Fe oxyhydroxides (including Mn oxides), ‘amFeox’; organics and sulphides, ‘org/sul’; and residual (silicates and more resistant minerals). Three standard reference soil samples, SRMs 2709, 2710 and 2711, were analysed in triplicate for the elements Ca, Cd, Cu, Fe, Mn, Ni, P, Pb, Ti, V and Zn. Results by both methods agree extremely well for Ca, Mn and Cd, and for Ni and V in SRMs 2709 and 2711. For other elements, there is a strong tendency for a higher percentage to be dissolved earlier in the GSC scheme (in the AEC, amFeox and org/sul phases). Consistently more Fe reports to the amFeox and org/sul phases by the GSC method, otherwise present in the residual phase by the Tessier scheme. Results for P do not compare well, with a much greater proportion of the element being extracted in the amFeox phase by the GSC procedure. Very little P appears to be labile by the Tessier protocol. This paper suggests that more research is needed into the nature of phases purportedly extracted by selective leaches.
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  • 52
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    Water, air & soil pollution 115 (1999), S. 21-70 
    ISSN: 1573-2932
    Keywords: atmospheric transport ; current-use pesticides ; deposition ; field measurements ; long-range transport ; monitoring ; organochlorine pesticides ; pesticides ; rainwater
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Recently, evidence has accumulated that the extensive use of modern pesticides results in their presence in the atmosphere at many places throughout the world. In Europe over 80 current-use pesticides have been detected in rain and 30 in air. Similar observations have been made in North America. The compounds most often looked for and detected are the organochlorine insecticide lindane and triazine herbicides, especially atrazine. However, acetanilide and phenoxyacid herbicides, as well as organophosphorus insecticides have also frequently been found in rain and air. Concentrations in air normally range from a few pg/m3 to many ng/m3. Concentrations in rain generally range from a few ng/L to several µg/L. In fog even higher concentrations are observed. Deposition varies between a few mg/ha/y and more than 1 g/ha/y per compound. However, these estimates are usually based on the collection and analysis of (bulk) precipitation and do not include dry particle deposition and gas exchange. Nevertheless, model calculations, analysis of plant tissue, and first attempts to measure dry deposition in a more representative way, all indicate that total atmospheric deposition probably does not normally exceed a few g/ha/y. So far, little attention has been paid to the presence of transformation products of modern pesticides in the atmosphere, with the exception of those of triazine herbicides, which have been looked for and found frequently. Generally, current-use pesticides are only detected at elevated concentrations in air and rain during the application season. The less volatile and more persistent ones, such as lindane, but to some extent also triazines, are present in the atmosphere in low concentrations throughout the year. In agricultural areas, the presence of modern pesticides in the atmosphere can be explained by the crops grown and pesticides used on them. They are also found in the air and rain in areas where they are not used, sometimes even in remote places, just like their organochlorine predecessors. Concentrations and levels are generally much lower there. These data suggest that current-use pesticides can be transported through the atmosphere over distances of tens to hundreds, and sometimes even more than a thousand kilometres. The relative importance of these atmospheric inputs varies greatly. For mountainous areas and remote lakes and seas, the atmosphere may constitute the sole route of contamination by pesticides. In coastal waters, on the other hand, riverine inputs may prevail. To date, little is known about the ecological significance of these aerial inputs.
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  • 53
    ISSN: 1572-8900
    Keywords: Starch ; PHBV ; PHA ; plastic ; blends ; biodegradation ; soil ; compost
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology , Energy, Environment Protection, Nuclear Power Engineering , Mechanical Engineering, Materials Science, Production Engineering, Mining and Metallurgy, Traffic Engineering, Precision Mechanics
    Notes: Abstract Injection molded specimens were prepared by blending poly (hydroxybutyrate-co-valerate) (PHBV) with cornstarch. Blended formulations incorporated 30% or 50% starch in the presence or absence of poly-(ethylene oxide) (PEO), which enhances the adherence of starch granules to PHBV. These formulations were evaluated for their biodegradability in natural compost by measuring changes in physical and chemical properties over a period of 125 days. The degradation of plastic material, as evidenced by weight loss and deterioration in tensile properties, correlated with the amount of starch present in the blends (neat PHBV 〈 30% starch 〈 50% starch). Incorporation of PEO into starch-PHBV blends had little or no effect on the rate of weight loss. Starch in blends degraded faster than PHBV and it accelerated PHBV degradation. Also, PHBV did not retard starch degradation. After 125 days of exposure to compost, neat PHBV lost 7% of its weight (0.056% weight loss/day), while the PHBV component of a 50% starch blend lost 41% of its weight (0.328% weight loss/day). PHB and PHV moieties within the copolymer degraded at similar rates, regardless of the presence of starch, as determined by 1H-NMR spectroscopy. GPC analyses revealed that, while the number average molecular weight (Mn) of PHBV in all exposed samples decreased, there was no significant difference in this decrease between neat PHBV as opposed to PHBV blended with starch. SEM showed homogeneously distributed starch granules embedded in a PHBV matrix, typical of a filler material. Starch granules were rapidly depleted during exposure to compost, increasing the surface area of the PHBV matrix.
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  • 54
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    Biodegradation 9 (1998), S. 327-336 
    ISSN: 1572-9729
    Keywords: fungi ; organophosphate insecticides ; phosphorus mineralization ; sulfur mineralization ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract Thirteen fungal species isolated from soil treated with pesticides were tested for their ability to mineralize and degrade three organophosphate insecticides currently used in Egypt (Cyolan®, Malathion® and Dursban®) in liquid media free from phosporus (P) and sulfur (S). All fungal species grew successfully on the culture media treated with the three used doses of insecticides (10, 50 and 100 ppm active ingredient) but the growth rate varied with the species, the insecticide and the doses. At 10 ppm level, insecticide degradation expressed in term of organic P mineralization (calculated as % of applied P) was the highest with all fungi tested. Organic P mineralization from pesticides was decreased by increasing the dose used to 50 and 100 ppm. The highest amount of P mineralized was observed with Cyolan® followed by Malathion® whilst P mineralization from Dursban® proceeded very slowly. Aspergillus terreus showed the greatest potential to mineralize organic P followed by A. tamarii, A. niger, Trichoderma harzianum and Penicillium brevicompactum whilst the remaining fungi only moderately mineralized the organic P component of the insecticides tested. Organic sulfur mineralization by the used fungal species paralleled, to some extent, organic P mineralization. The extracellular protein content of culture filtrates in the presence of various doses of insecticides was also decreased by increasing insecticide concentrations. The extracellular protein was significantly correlated with P and S mineralization (r = 0.89** and 0.64**, respectively) whilst correlation with cell dry mass was not significant (r = 0.03 and 0.003) suggesting a direct relationship between pesticide degradation and microbial protein production. The addition of P or S to the growth media enhanced extracellular protein excretion, and increased organic P and S mineralization by the most potent species tested (A. niger, A. tamarii, A. terreus and T. harzianum). This increment was significant in most cases, especially at the higher application rates. The relationship between extracellular protein excretion and organic P and S mineralization from insecticides was highly significant with the addition of inorganic phosphorus (r = 0.96** and 0.83**, respectively) or sulfur (r = 0.85** and 0.89**, respectively) to the growth media.
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  • 55
    ISSN: 1573-2959
    Keywords: risk assessment ; chlorinated compound ; environmental ; marine ; exposure ; aquatic toxicity ; monitoring ; trichloroethylene
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract This risk assessment on trichloroethylene (TRI) was carried out specifically for the marine environment, according to the methodology laid down in the EU risk assessment Regulation (1488/94) and the Guidance Document of the EU New and Existing Substances Regulation (TGD, 1997). The study consists of the collection and evaluation of data on effects and environmental concentrations from analytical monitoring programs in large rivers and estuaries in the North Sea area. The risk is indicated by the ratio of the "predicted environmental concentrations" (PEC) and the "predicted no effect concentrations" (PNEC) for the marine aquatic environment. In total, 19 studies for fish, 30 studies for invertebrates and 14 studies for algae have been evaluated. Both acute and chronic toxicity studies have been taken into account and the appropriate assessment factors have been used to define a PNEC value of 150 µg/l. Most of the available monitoring data apply to rivers and estuaries and were used to calculate PECs. The most recent data (1991-1995) support a typical PEC of 0.1 µg TRI/l water and a worst case PEC of 3.5 µg TRI/l water. The calculated PEC/PNEC ratios give a safety margin of 40 to 1,500 between the predicted no effect concentration and the exposure concentration. Additional evaluation of environmental fate and bioaccumulation characteristics showed that no concern for food chain accumulation is expected.
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  • 56
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    Environmental and ecological statistics 5 (1998), S. 81-91 
    ISSN: 1573-3009
    Keywords: density estimation ; distance sampling ; detection function ; monitoring ; Pollard-Yates
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Line transect sampling is an effective survey method for estimating butterfly densities because it provides unbiased estimates of site-density (provided key assumptions are met), and estimates are comparable among sites. For monitoring Karner blue butterflies in Wisconsin, USA, comparable estimates are required because each year a different selection of sites will be monitored. Annual state-wide indices of species abundance can be derived from the site-surveys and compared to previous year's indices to monitor trends. We advocate that line transect sampling is preferable to Pollard-Yates transects as a survey technique for monitoring Karner blue butter- flies. The Pollard-Yates surveys do not adjust for diferences in site detectability. As a consequence, estimates of among-site from Pollard-Yates surveys can be biased. © Rapid Science 1998
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  • 57
    ISSN: 1573-3017
    Keywords: earthworm ; nickel ; soil ; toxicology ; eisenia veneta
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The toxic effects of nickel on survival, growth, and reproduction of Eisenia veneta were investigated following 4 weeks of exposure to a nickel-chloride spiked loamy sand soil. The ability of a simple earthworm biomarker, the lysosomal membrane stability of coelomocytes, to reflect nickel exposure was also studied. Nickel caused a significant toxic effect on E.veneta at soil concentrations above 85 mg Ni/kg. Reproduction (cocoon production) was the most sensitive parameter being reduced at soil concentrations above 85 mg Ni/kg (EC10 = 85 mg Ni/kg). Survival of adults was only reduced at concentrations above 245 mg Ni/kg, while adult and cocoon wet weight were not affected by soil nickel concentrations up to 700 mg Ni/kg. The lysosomal membrane stability, measured as neutral-red retention time, was reduced at soil nickel concentrations similar to those that reduced reproduction, and demonstrated a dose-response relationship. The neutral-red retention time showed large individual variation for the earthworms within each exposure concentration. It was concluded that the lysosomal membrane stability, measured as neutral red retention time, has a potential role in risk assessment, but care should be taken conducting this test.
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  • 58
    ISSN: 1573-1642
    Keywords: watershed ; water quality ; monitoring ; science education ; environmental data
    Source: Springer Online Journal Archives 1860-2000
    Topics: Architecture, Civil Engineering, Surveying , Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract From 1992 to 1994, Saturday Academy and the Oregon Graduate Institute of Science and Technology instituted the pilot phase of a long-term monitoring program called the Student Watershed Research Project (SWRP). The SWRP program was developed to create and maintain collaboration among eighth through twelfth grade teachers and students, scientists, businesses, governmental agencies, and community members which would couple environmental education with the collection of high quality, reproducible watershed health data. The original authors of this paper set out to evaluate the impacts of the SWRP program in terms of changes in educational attitudes of participants and collection of accurate data. Findings demonstrate that assuring accuracy of student collected data was challenging, that teachers and students benefited greatly from a hands-on research approach to science education, and that such an approach would be difficult without the support of a program like SWRP. The SWRP program is entering its seventh year in the Portland, Oregon and Vancouver, Washington metropolitan areas with approximately half of the pilot phase participants still involved. A Quality Assurance Project Plan has been developed to assure data accuracy. Evaluation student science education attitudes documents improved results on a yearly basis.
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  • 59
    ISSN: 1573-2959
    Keywords: risk assessment ; chlorinated compound ; environmental ; marine ; exposure ; aquatic toxicity ; monitoring ; chloroform
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract This risk assessment on chloroform was carried out specifically for the marine environment, according to the methodology laid down in the EU risk assessment Regulation (1488/94) and the Guidance Document of the EU New and Existing Substances Regulation (TGD, 1997). The study consists of the collection and evaluation of data on effects and environmental concentrations from analytical monitoring programs in large rivers and estuaries in the North Sea area. The risk is indicated by the ratio of the "predicted environmental concentrations" (PEC) and the "predicted no effect concentrations" (PNEC) for the marine aquatic environment. In total, 23 studies for fish, 17 studies for invertebrates and 10 studies for algae have been evaluated. Both acute and chronic toxicity studies have been taken into account and the appropriate assessment factors have been used to define a typical PNEC value of 72 µg/l. Due to limitations of the studies evaluated, a worst PNEC of 1 µg/l could also be used. Most of the available monitoring data apply to rivers and estuaries and were used to calculate PECs. The most recent data (1991-1995) support a typical PEC of 0.2 µg chloroform per litre of water and a worst case PEC of 5 to 11.5 µg chloroform per litre of water. The calculated PEC/PNEC ratios give a safety margin of 6 to 360 between the predicted no effect concentration and the exposure concentrations. A worst case ratio, however, points to a potential risk for sensitive species. Refinement of the assessment is necessary by looking for more data. Additional evaluation of environmental fate and bioaccumulation characteristics showed that no concern is expected for food chain accumulation.
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  • 60
    ISSN: 1573-2959
    Keywords: risk assessment ; chlorinated compound ; environmental ; marine ; exposure ; aquatic toxicity ; monitoring ; tetrachloroethylene
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract This risk assessment on tetrachloroethylene (PER) was carried out specifically for the marine environment, according to the methodology laid down in the EU risk assessment Regulation (1488/94) and the Guidance Document of the EU New and Existing Substances Regulation (TGD, 1997). The study consists of the collection and evaluation of data on effects and environmental concentrations from analytical monitoring programs in large rivers and estuaries in the North Sea area. The risk is indicated by the ratio of the "predicted environmental concentrations" (PEC) and the "predicted no effect concentrations" (PNEC) for the marine aquatic environment. In total, 18 studies for fish, 13 studies for invertebrates and 8 studies for algae have been evaluated. Both acute and chronic toxicity studies have been taken into account and the appropriate assessment factors have been used to define a PNEC value of 51 µg/l. Most of the available monitoring data apply to rivers and estuary waters and were used to calculate PECs. The most recent data (1991-1995) support a typical PEC of 0.2 µg PER/l water and a worst case PEC of 2.5 µg PER/l water. The calculated PEC/PNEC ratios give a safety margin of 20 to 250 between the predicted no effect concentration and the exposure concentration. Additional evaluation of environmental fate and bioaccumulation characteristics showed that no concern is expected for food chain accumulation.
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  • 61
    ISSN: 1573-2932
    Keywords: acidification ; acid rain ; catchment ; China ; geochemistry ; soil ; soil water
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Acid deposition is considered to be a major environmental problem in China, but information about effects on soils and waters is scarce. To contribute to increased knowledge about the problem a small catchment (about 7 ha) in the outskirts of Guiyang, the provincial capital of Guizhou in south-western China, was instrumented for collection of precipitation, throughfall, soil water and stream water. In addition soil samples have been collected and analyzed for key properties. Median pH in the precipitation is 4.40 (quartiles: 4.19 and 4.77) and the median sulfate concentration 228 µeq/L (quartiles: 147 and 334 µeq/L). The dry deposition of both SO2 and alkaline dust is considerable. The sum of wet deposition of sulfate and dry deposition of SO2 has been estimated to about 8.5 gSm-2yr-1. The total S-deposition may be somewhat higher due to dry deposition of sulfate and occult deposition. In soil water, SO4 2- is the major anion, generally ranging from 300 to 2500 µeq/L in the different plots. Calcium is an important cation, but there is also a considerable contribution of aluminum from the soil. In some of the plots the concentrations of inorganic monomeric aluminum (Ali) are typically between 200 and 400 µm. Potential harmful levels of aluminum and/or high Ali/(Ca2+ + Mg2+) molar ratios occur in the catchment, but damages to vegetation have not yet been reported. In most cases exchangeable aluminum accounts for between 75 and 95% of the total effective cation exchange capacity (CECE) in the mineral soils. The aluminum chemistry cannot easily be explained by conventional models as the Gaines-Thomas ion-exchange equation or equilibrium with an Al(OH)3 mineral phase. The stream water is generally less acidic and has considerably lower concentrations of aluminum than the soil water, even though quite acid events have been observed (pH 〈 4.4). The median pH values are 4.9 and 5.0 in the two first order streams and 6.3 in the dam at the lower boarder of the catchment.
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  • 62
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    Water, air & soil pollution 101 (1998), S. 399-410 
    ISSN: 1573-2932
    Keywords: bioavailability ; bush bean ; cadmium ; contamination ; heavy metal ; industrial waste ; mobility ; Phaseolus vulgaris ; sandy soil ; Savannah River Site ; soil ; thallium ; vanadium
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A field study was conducted over a 30 mo period to examine movement of Cd, Tl, and V through the profile of a Coastal Plain soil (Typic Kandiudult) and the availability of these trace metals to bush bean (Phaseolus vulgaris L.) plants. The metals were applied to field plots as dissolved salts and mixed into the surface 7.5 cm. The greatest concentration of all three metals was observed in the surface soils, with a steep decrease occurring down to the 7.5 to 15 cm depth. Thallium was the most mobile of the three metals; approximately 15% of the applied Tl and 〈3% of the applied Cd and V moved below the surface 7.5-cm region during the 30-mo experiment. Extractable concentrations of all three metals in the surface soils decreased significantly (P ≤0.05) during the initial 18 mo after treatment. No further decrease occurred between 18 and 30 mo. The presence of Al- and Fe-oxides and small amounts of clay minerals and organic matter in this highly-weathered, low cation-exchange soil were likely responsible for the retention of the trace metals. Bioavailability, as measured by concentrations and total amounts of metals in root and aboveground tissues of plants, did not change significantly between 18 and 30 mo. These data suggest that bioavailability of Cd, Tl, and V decreased over time as a result of transformation of these elements into unavailable forms and not to leaching. These changes in bioavailability occurred soon after application, becoming negligible after 18 mo.
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  • 63
    ISSN: 1573-2932
    Keywords: catchment ; monitoring ; nitrogen deposition ; nitate leaching ; runoff chemistry ; stream chemistry
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    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Samples were collected from 13 upland sites (main inflow and loch outflow) in the UK along an N deposition gradient of 12-50 kg ha-1 yr-1 to determine the relationship between N deposition and NO3 - concentrations in surface waters. There was no direct correlation between NO3 - leaching and soluble inorganic N deposition at these sites, but a significant relationship with NO3 - was found using a deposition function incorporating dissolved organic carbon (DOC) flux from each catchment. A similar but less significant relationship was found between NO3 - concentration and DOC:DON ratio in runoff water. Catchments showed evidence of N saturation, i.e., when mean NO3 - concentration exceeded 5 µeq L-1, when the mean DOC:DON ratio fell below an approximate value of 25. Five other large loch sites (LLS) with multiple subcatchments were used to test these relationships and for four of these mostly heathland sites the predicted NO3 - concentrations closely matched measured values. At the fifth site, where most subcatchments were forested, the deposition function and DOC:DON ratios gave conflicting predictions and both methods generally underestimated measured NO3 - concentrations. If the capacity of these catchments to retain deposited N is determined by C supply then many upland catchments in the UK may experience increasing NO3 - concentrations in runoff in the future at current or increased levels of N deposition.
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  • 64
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    Water, air & soil pollution 105 (1998), S. 471-480 
    ISSN: 1573-2932
    Keywords: benzo(a)pyrene deposition ; Lithuania ; monitoring ; moss chemistry ; plant tissue chemistry
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Benzo(a)pyrene (BP) has been investigated in bulk atmospheric deposition, moss, needles of pine and some species of vascular plants. At two remote Lithuanian sites, for 1990-1995 the flux of benzo(a)pyrene from the atmosphere to the ground surface varied between 0.3 to 4.8 μg-2 mo-1. Consequently the territory of Lithuania (65,000 km2) yearly was exposed to 624-2574 kg of carcinogen. The distribution of BP in soil and various vascular plant tissues (Trifolium tepens, Elitrygea repens, Thymus serpyllum) indicates that benzo(a)pyrene is assimilated by flora. The concentration of BP is different in various organs of vascular plants and mostly depends on the degree of soil pollution. More than 300 samples of moss, mostly Hylocomium splendens and Pleurozium schreberi were analyzed for BP. From 3.1 to 896.0 μg kg-1 of BP were measured in the moss samples. The flux of BP to the ground surface correlates well with its concentration in moss. A map of BP flux across Lithuania was created.
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  • 65
    ISSN: 1573-2959
    Keywords: risk assessment ; chlorinated compound ; marine ; environmental ; exposure ; aquatic toxicity ; monitoring
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract This risk assessment on 1,1,2-trichloroethane (T112) was carried out specifically for the marine environment, according to the methodology laid down in the EU risk assessment Regulation (1488/94) and the Guidance Document of the EU New and Existing Substances Regulation (TGD, 1997). The study consists of the collection and evaluation of data on effects and environmental concentrations from analytical monitoring programs in large rivers and estuaries in the North Sea area. The risk is indicated by the ratio of the "predicted environmental concentrations" (PEC) and the "predicted no effect concentrations" (PNEC) for the marine aquatic environment. In total, 22 studies for fish, 45 studies for invertebrates and 9 studies for algae have been evaluated. Both acute and chronic toxicity studies have been taken into account and the appropriate assessment factors have been used to define a PNEC value of 300 µg/l. Most of the available monitoring data apply to rivers and estuaries and were used to calculate PECs. The most recent data (1991-1995) support a typical PEC of 0.01 µg T112/l water and a worst case PEC of 5 µg T112/l water. The calculated PEC/PNEC ratios give a safety margin of 60 to 30,000 between the predicted no effect concentration and the exposure concentration. Additional evaluation of environmental fate and bioaccumulation characteristics showed that no concern is expected for food chain accumulation.
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  • 66
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    Environmental monitoring and assessment 53 (1998), S. 279-295 
    ISSN: 1573-2959
    Keywords: acidification ; dry and wet deposition ; euthrophication ; monitoring
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A monitoring station for atmospheric deposition was designed and constructed. Three such stations were applied in a pilot project for a year on three sites (Speulder forest in The Netherlands, Auchencorth in Scotland and Melpitz in Germany) in different regions in Europe to estimate local inputs and to validate deposition models which are currently used or developed to estimate ecosystem specific deposition in Europe. Fluxes at Auchencorth Moss are lowest for all components, except for those much influenced by the sea as a source. As Melpitz is located far away from seas, these components are lowest at this site. Wet deposition is the dominant source of input at Auchencorth, whereas at Speulder forest, through its roughness and pollution climate, dry deposition is dominant. At this site dry deposition velocities are highest. Melpitz is a polluted site. Particularly sulphur deposition is high. It is recommended to equip several locations in Europe with intensive deposition monitoring methods. Such a network will be an extension of existing monitoring programmes on air pollution, such as that run by Eurepean Monitoring and Evaluation Programme for the long-range transmission of air pollutants in Europe (EMEP). The intensive monitoring locations should be selected based on pollution climates and type of vegetation, common in Europe.
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  • 67
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    Environmental monitoring and assessment 53 (1998), S. 395-399 
    ISSN: 1573-2959
    Keywords: risk assessment ; chlorinated compound ; marine ; environmental ; exposure ; aquatic toxicity ; monitoring
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A voluntary programme on risk assessment for chlorinated chemicals was initiated by Euro Chlor (the European Chlorine Producers Federation). The study was targeted on the marine environment, starting with the North Sea, and the methodology used was based on the European Union risk assessment principles. Details of the method used are described in this paper. A first set of five compounds is published in this special issue: chloroform, 1,2-dichloroethane, 1,1,2-trichloroethane, trichloroethylene, tetrachloroethylene.
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  • 68
    ISSN: 1573-2959
    Keywords: risk assessment ; chlorinated compound ; environmental ; marine ; exposure ; aquatic toxicity ; monitoring ; 1,2-dichloroethane
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract This risk assessment on 1,2-dichloroethane (EDC) was carried out specifically for the marine environment, according to the methodology laid down in the EU risk assessment Regulation (1488/94) and the Guidance Document of the EU New and Existing Substances Regulation (TGD, 1997). The study consists of the collection and evaluation of data on effects and environmental concentrations from analytical monitoring programs in large rivers and estuaries in the North Sea area. The risk is indicated by the ratio of the "predicted environmental concentrations" (PEC) and the "predicted no effect concentrations" (PNEC) for the marine aquatic environment. In total, 21 studies for fish, 17 studies for invertebrates and 7 studies for algae have been evaluated. Both acute and chronic toxicity studies have been taken into account and the appropriate assessment factors have been used to define a PNEC value of 1100 µg/l. Most of the available monitoring data apply to rivers and estuaries and were used to calculate PECs. The most recent data (1991-1995) support a typical PEC of 0.5 µg EDC/l and a worst case PEC of 6.4 µg EDC/l. The calculated PEC/PNEC ratios give a safety margin of 170 to 2200 between the predicted no effect concentration and the exposure concentration. Additional evaluation of environmental fate and bioaccumulation characteristics showed that no concern is expected for food chain accumulation.
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  • 69
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    Water, air & soil pollution 102 (1998), S. 221-238 
    ISSN: 1573-2932
    Keywords: contaminated ; EDTA ; lead ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Lead contamination of soils is a common problem throughout the world. Laboratory batch test and bench scale experiments have shown that EDTA can be used to remove lead from contaminated soils. However, due to the high cost and laborious task associated with actual environmental remediation of a lead contaminated soil, there is a need to be able to predict the outcome of a remediation process in advance in order to optimize the process and minimize the cost. This paper describes the development and validation of a computer model which can be used to simulate the removal of lead from a contaminated soil column using EDTA as the chelating agent. The model is able to simulate the lead removal from soil based on equilibrium as well as kinetic dissolution of Pb. The comparison of the simulated results with actual lead concentrations both in effluent and soil shows that the model can predict the lead removal process with reasonable accuracy.
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  • 70
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    Water, air & soil pollution 102 (1998), S. 415-425 
    ISSN: 1573-2932
    Keywords: factor score ; Kriging ; soil ; trace element
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The abundances of copper, lead, zinc, nickel, chromium, cobalt, mercury, vanadium, and manganese in eighty three surface soil samples collected from Shenzhen area were determined. The correlation among element contents and the factors affecting the contents were studied using principle component analysis. The factor scores of the first two components were analyzed as regionalized variables using variogram analysis and Kriging. The interpolated factor scores were then mapped to show the common features in spatial distribution of a set of elements with similar geochemical behavior. It was demonstrated that the spatial distribution patterns of parent material in the area are the primary factor governing the spatial variation of the elements.
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  • 71
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    Water, air & soil pollution 103 (1998), S. 357-373 
    ISSN: 1573-2932
    Keywords: fluoride pollution ; ionic strength ; pH ; soil ; sorption
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Fluoride (F) accumulation and transport in soil columns near the aluminium smelter at Årdal in Western Norway are studied together with fluoride sorption capacity, and the effect of pH and ionic strength on F solubility in soil. Unpolluted soil columns of 50 cm height placed at different distances from the smelter (1–0 km) accumulated from 0.27 g F m-2 to 1.5 g F m-2 during a 5 months period. Fluoride accumulation was high in the upper 0–10 cm of the soil columns where 50–90% of the accumulated F was found. Laboratory sorption experiments showed that the sorption of added F in the Ah-horizons increased with increased distance from the smelter at Årdal, in accordance with decreasing previous pollution from the smelter. The B-horizons sorbed considerably more F than the Ah-horizons, due to higher content of Al-oxides/hydroxides. Maximum sorption of F occurred at pH 4.8–5.5. Fluoride solubility increased with increased ionic strength. Continued deposition of F may increase the availability to plants and soil organisms. Leaching of F from soil to groundwater or surface water will be strongly dependent on the presence and thickness of a B-horizon, and probably also on underlying horizons.
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  • 72
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    Water, air & soil pollution 103 (1998), S. 375-388 
    ISSN: 1573-2932
    Keywords: aluminium fluoride complexes ; fluoride pollution ; organic matter ; pH ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The effect of fluoride (F) on pH and solubility of organic matter (TOC), aluminium (Al), iron (Fe), calcium (Ca), magnesium (Mg) and potassium (K) in soil samples collected near an aluminium smelter in Norway was studied. Increased addition of F to the soil samples led to an increase in pH and concentrations of TOC, Al and Fe in solution. Most of the F and Al in solution were in the forms of ALFx-complexes. K solubility decreased in some soil samples, but there were no consistent effect on the solubility of Ca or Mg. The effect of NaF addition was significantly different from equimolar NaCl-treatments. The concentrations of Al, Fe, TOC and the pH-values were lower, while the concentrations of K, Mg and Ca were higher in the NaCl-treatments than in the NaF-treatments. The results from the experiment imply that F-pollution of soil induces breakdown of Al- and Fe-oxides/hydroxides and solubilize organic material in the soil. This may influence the availability of potentially toxic elements, such as AIFx-complexes, to microorganisms and plant roots.
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  • 73
    ISSN: 1573-2932
    Keywords: base metal mining ; biota ; metal pollution ; sediment ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Soil, aquatic biota (moss: Brachythecium rivulare; aquatic macrophytes: Juncus effusus, Potamogeton crispus; fish: Salmo trutta fario, Anguilla anguilla, Phoxinus phoxinus, Chelon labrosus) and sediment samples from the Urumea river valley were analysed for metals by acid digestion and atomic absorption spectroscopy. The sediments show the presence of metal pollution (Cd: 2.5–24 mg kg-1; Pb: 125–1,150 mg kg-1; Zn: 125–2,500 mg kg-1) because mining and industrial wastes. A selective retention of dense minerals in dam sediments contributes to the load of metal, but interstitial water analysis (Cd: 〈0.02–0.1 mg L-1; Pb: 0.3–1.0 mg L-1; Zn: 〈0.05–0.6 mg L-1) shows that precipitation equilibrium controls their mobilisation. Biota samples show evidence of metal accumulation, moss reaching 1,100 mg kg-1 in lead and 6,800 mg kg-1 in zinc. Soil from the valley is polluted by both, river carried material and industrial sources (Cd: 1.0–4.0 mg kg-1; Pb: 26–1,120 mg kg-1; Zn: 105–1,390 mg kg-1/math〉), but they are used, indistinctly, for farming and pasture.
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  • 74
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    Water, air & soil pollution 106 (1998), S. 111-122 
    ISSN: 1573-2932
    Keywords: silicone ; silanol ; environmental ; biodegradation ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Dimethylsilanediol (DMSD) is the ultimate hydrolysis product of silicone (polydimethylsiloxane = PDMS) polymer in soil. Our previous paper showed that it would volatilize from soil, and the present study investigates the importance of microbial degradation in removing DMSD from soil. DMSD (14C-labeled) was thus incubated (1 mg kg-1) for 30 wk at 25 °C in soils from a permanent grass field, a corn field, a deciduous woodland, and a pine woodland. Release of14 CO2 varied from 0.4 to 1.6% wk-1. For 3 of the soils, 14CO2 increased with higher microbial biomass, while organisms in the deciduous woodland soil were more active in degrading DMSD than organisms in the other soils. After 30 weeks, most of the remaining 14C in the soil had moved from freely available water extractable to less available acid and base extractable fractions. Similar incubations with 2% plant litter showed extensive transfer of the DMSD into the litter layer. Incubations with a microbial inhibitor showed less DMSD degradation, while cold storage of soils almost completely stopped degradation. These results suggest that microbial degradation is an important mechanism of DMSD loss from soil.
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  • 75
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    Water, air & soil pollution 108 (1998), S. 129-148 
    ISSN: 1573-2932
    Keywords: biodegradation ; leaching ; soil ; triazine
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The purpose of this study was to investigate the fate of triazines and their metabolites in the unsaturated zone in the field conditions during a period from the spring sowings to the autumn tillages. The study was performed upon two soils treated for corn culture during the year 1992. The investigations were presented after the wet weather by subsurface drainage and surface runoff. Throughout the 6 months survey, the relative importance of the triazines is by decreasing order: atrazine 〉 simazine 〉 desethylatrazine (DEA). After the application, the herbicides were only found in the first 40 cm of the soil during the dry period of the cultivation. They were dragged towards the depth by percolation water mainly during the first water infiltrations when the drains were set in again in autumn or winter. The losses of herbicides after the cultivation cycle (october) expressed as a ratio of the initial input ranged from 40 to 73% for the atrazine and from 40 to 44% for the simazine and depended on the importance of the application amount. In autumn and winter, the losses originating in percolation were higher than those due to volatilization and/or degradation (abiotic and biodegradation), as the soil conditions were unpropicious to the formation of non-extractable residues.
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  • 76
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    Water, air & soil pollution 108 (1998), S. 51-68 
    ISSN: 1573-2932
    Keywords: Crustacea ; growth ; heavy metals ; monitoring
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The dynamics of lead (Pb) and cadmium (Cd) accumulation in juvenile Porcellio scaber were studied over 6 months after exposing them to three different concentrations of lead and cadmium in their food. Subsequently the ability of P. scaber to eliminate lead and cadmium was studied over two months. Growth was measured to determine whether metal contamination leads to physiological stress in the animals. The accumulation of Pb and Cd in P. scaber shows two different phases. Up to the age of 2–3 months the assimilation exceeds the rate of growth and leads to rapidly increasing concentrations. After 3 months the rate of accumulation is proportional to the rate of growth and the heavy metal concentrations remain on a stabilized level. P. scaber was able to eliminate about 40% of the assimilated lead within 2 weeks but there was no elimination of Cd within 7 weeks. Contaminated P. scaber shows significant growth reduction. The physiological response of P. scaber to heavy metal contamination is discussed.
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  • 77
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    Water, air & soil pollution 108 (1998), S. 391-409 
    ISSN: 1573-2932
    Keywords: contamination ; lead ; migration ; partitioning ; soil ; zinc
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The chemical partitioning of lead and zinc is described in contaminated soils and underlying strata at historical lead smelting sites. Sections of soil-rock cores from eight sites of age 200 to c.1900 yr were analysed using a sequential extraction procedure. Of the total amount of lead and zinc present in soils, only a small proportion is in a readily mobile form. However, this proportion increases significantly as the pH falls below 5 and for lead reaches 37% in soils at Bole A. A high proportion of lead in soils appears to be associated with the carbonate and specifically adsorbed phase. It is suggested that this is partly due to the formation of cerussite (PbCO3) in soils contaminated with calcareous slag wastes. Lead present in the residual phase in contaminated soils may be related to the presence of the element in silicate slag particles. Rapid migration of lead to a depth of 5.6 m in sandstone at Bole A was related to its high solubility in the acidic soils and rock at this site. Comparable migration at Bole C proceeds by a different mechanism, possibly with lead in association with Fe-Mn oxides and slag particles. In clay infill in fractured sandstone at Bole A, anthropogenic lead present at a depth of 4.4 m was extracted predominantly in the fraction representing Fe-Mn oxides.
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  • 78
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    Water, air & soil pollution 106 (1998), S. 425-445 
    ISSN: 1573-2932
    Keywords: crops ; crop-yield ; effect ; environment ; freshwater ; irrigation ; leachate ; salinity ; sodicity ; soil ; wastewater ; water-quality
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract An investigation was carried out at pilot scale to test the feasibility of using the effluent of a rotating biological contactors (RBC) unit treating wastewater generated from a university campus. The objective of the study was to cerefully monitor the impact of wastewater irrigation on the soil, percolating water, crop growth and the pathogenic condition within the immediate vicinity of wastewater application. Experimental plots with three crops: alfalfa, radish and tomato were irrigated with fresh and waste waters. The irrigation water was applied by sprinklers. Each crop was given two sub-treatments: with fertilizer and without fertilizer. The physical and chemical properties of the soil, the crop yields, and subsurface drainage were measured. In most of the cases, the yields resulted from the uses of wastewater with fertilizer were compatible with those of the uses of freshwater with fertilizer. The washings of tomato fruits grown with wastewater were analyzed for fecal coliforms. It appeared that the fruit skins were free of viable fecal coliforms 24 hours after the wastewater application. Subsurface drainage analyses did not show any alarming levels of constituents irrespective of the source of the water: wastewater or freshwater. The wastewater irrigation applied for a season had no significant effect on a silty loam soil. With wastewater irrigation, slught changes in the soil porosity and salinity were observed.
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  • 79
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    Water, air & soil pollution 101 (1998), S. 45-67 
    ISSN: 1573-2932
    Keywords: Bacteria ; biodiversity ; chemically-contaminated ; ecology ; microorganisms ; molecular ; PCR ; soil ; toxic
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Microorganisms isolated from soil are sources of known and new microorganisms and genetic material. This review examines general principles of soil bacterial biodiversity, limitations in sampling soils, and examples of bacterial diversity in chemically-contaminated soils. Both conventional and molecular methods used to assess microbial biodiversity in soils will be addressed as well as selected examples of the effects of organic and inorganic pollutants on soil microbial diversity.
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  • 80
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    Water, air & soil pollution 103 (1998), S. 91-100 
    ISSN: 1573-2932
    Keywords: airborne particulate matter ; drinking water ; gas chromatography ; gas chromatography-mass spectrometry ; industrial-urban area ; PAH occurrence ; sewage sludge ; soil ; solid phase extraction
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The Polycyclic Aromatic Hydrocarbons (PAHs) pollution state of the chosen town (Zabrze) of Upper Silesia, the most industrialised region in Poland, was presented. Zabrze is a town of medium size, having population twenty times bigger than a medium town polulation in Poland. In this study we determined the qualitative and quantitative composition of PAHs fraction separated from the following elements of environment: suspended dust, drinking water, soil and sewage sludge. The following analytical techniques were used: Soxhlet Extraction, Solid Phase Extraction, Gas Chromatography-Mass Spectrometry, Capillary Gas Chromatography and High Performance Liquid Chromatography. The results confirmed the significant state of examined region pollution. They stated the exceed of contents B(a)P in suspended dust. The soils in that place were heavily polluted with PAHs, about 4000 µg · kg-1 for the sum of PAHs. The total contents of PAHs in sewage sludge of Zabrze did not exceed the analogous contents published for West European sewage sludge treatment plants and the level of determined PAHs in drinking water did not show any claims.
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  • 81
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    Water, air & soil pollution 105 (1998), S. 217-226 
    ISSN: 1573-2932
    Keywords: California ; monitoring ; nitrate export ; Sierra Nevada ; stream water chemistry ; sulfate export ; watershed
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Based on studies of high-elevation, Sierra Nevada catchments during the period from 1983 through 1996, we describe temporal variations in the concentrations of NO3 - and SO4 2- in surface waters. During snowmelt, some catchments had a pattern of NO3 - increase to a plateau between the start of snowmelt and some weeks before runoff peaked, and a decline as runoff increased to its maximum. In other catchments, NO3 - concentrations peaked during the autumn and winter. Long-term trends in surface water chemistry were evident in only two catchments: an increase in SO4 2- concentrations in surface waters of the Ruby Lake basin, and a lowering of annual maxima and minima of NO3 - concentrations at Emerald Lake. From October 1987 through April 1994, SO4 2- concentrations increased from about 6 µeq L-1 to about 12 µeq L-1 in Ruby Lake, and in Emerald Lake, NO3 - maxima declined by 25-50 %.
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  • 82
    ISSN: 1572-9729
    Keywords: Desulfomonile tiedjei ; soil ; PCR ; reductive dechlorination
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract The aim of this work was to test the feasibility ofintroducing an anaerobic microbial reductivedechlorination activity into non sterile soil slurrymicrocosms by inoculation with the pure anaerobicbacterial strain Desulfomonile tiedjei, which iscapable of dechlorinating 3-chlorobenzoate tobenzoate. To show that the bacterium was establishedin the microcosms we followed the expression of thereductive dechlorination activity and a molecularprobe based on PCR amplification of the 16S rDNA genewas developed. However, the success of PCRamplification of the 16S rDNA gene depends on the DNAextraction and purification methodologies applied, asshown through the use of several protocols. In thisstudy we report a DNA extraction and purificationmethod which generates sufficient and very clean DNAsuitable for PCR amplification of the D. tiedjei16S rDNA gene. The threshold of detection was about5.103 bacteria per gram of soil slurry.Introduction of D. tiedjei in soil slurrymicrocosms proved successful since 3-chlorobenzoatedechlorination activity was established with thisbacterium in microcosms normally devoid of thisdechlorination capacity. Indeed, the addition of D. tiedjei to microcosms supplemented with acetateplus formate as cosubstrate, at their respectiveconcentrations of 5 and 6 mM, led to a totalbiotransformation of 2.5 mM of 3-chlorobenzoate within12 days. After complete 3-chlorobenzoatedechlorination, the 16S rDNA gene of this bacteriumwas specifically detected only in the inoculatedmicrocosms as shown by PCR amplification followed byrestriction mapping confirmation.
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  • 83
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    Biodegradation 8 (1997), S. 349-356 
    ISSN: 1572-9729
    Keywords: biodegradation ; bioremediation ; acclimation ; Everglades ; mineralization ; nitrophenol ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract The Everglades in South Florida are a unique ecologicalsystem. As a result of the widespread use of pesticides andherbicides in agricultural areas upstream from these wetlands,there is a serious potential for pollution problems in theEverglades. The purpose of this study was to evaluate theability of indigenous microbial populations to degradexenobiotic organic compounds introduced by agricultural andother activities. Such biodegradation may facilitate theremediation of contaminated soils and water in the Everglades.The model compound selected in this study is 4-nitrophenol, achemical commonly used in the manufacture of pesticides. Themineralization of 4-nitrophenol at various concentrations wasstudied in soils collected from the Everglades. Atconcentrations of 10 and 100 µg/g soil, considerablemineralization occurred within a week. At a higherconcentration, i.e., 10 mg/g soil, however, no mineralizationof 4-nitrophenol occurred over a 4-month period; such a highconcentration apparently produced an inhibitory effect. Therate and extent of 4-nitrophenol mineralization was enhancedon inoculation with previously isolated nitrophenol-degradingmicroorganisms. The maximum mineralization extent measured,however, was less than 30% suggesting conversion to biomassand/or unidentified intermediate products. These resultsindicate the potential for natural mechanisms to mitigate theadverse effects of xenobiotic pollutants in a complex systemsuch as the Everglades.
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  • 84
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    Mitigation and adaptation strategies for global change 2 (1997), S. 101-115 
    ISSN: 1573-1596
    Keywords: Carbon dioxide ; costs ; forests ; Joint Implementation ; mitigation ; monitoring ; policies
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering , Geography
    Notes: Abstract Forest sector mitigation options can be grouped into three categories: (1) management for carbon (C) conservation, (2) management for C storage, and (3) management for C substitution. The paper provides background information on the technical potential for C conservation and sequestration worldwide and the average costs of achieving it. It reviews policy measures that have been successfully applied at regional and project levels toward the reduction of atmospheric greenhouse gases. It also describes both national programs and jointly implemented international activities. The monitoring methods, and the items to monitor, differ across these categories. Remote sensing is a good approach for the monitoring of C conservation, but not for C substitution, which requires estimation of the fossil fuels that would be displaced and the continued monitoring of electricity generation sources. C storage, on the other hand, includes C in products which may be traded internationally. Their monitoring will require that bi- or multi-lateral protocols be set up for this purpose.
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  • 85
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    Mitigation and adaptation strategies for global change 2 (1997), S. 191-202 
    ISSN: 1573-1596
    Keywords: Carbon storage ; Joint Implementation ; monitoring ; remote sensing
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering , Geography
    Notes: Abstract Adequate monitoring of carbon sequestered by forestry activities is essential to the future of forestry as a climate change mitigation option. A wide range of approaches has been taken to monitor changes in forest carbon attributable to project activities. This paper describes simple, least-cost/least-precision methods, remote sensing, periodic carbon inventories, and traditional research methods. Periodic carbon inventories are the preferred approach because they are cost-effective, provide measurements with known levels of precision, and allow the monitoring of other values such as biodiversity and commercial timber volumes. Verification of monitoring estimates is discussed as an auditing process designed to evaluate reported carbon sequestration values. The limitations of remote sensing for biomass determination and the potential for changes in monitoring approaches due to improvements in technology are briefly reviewed.
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  • 86
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    Mitigation and adaptation strategies for global change 2 (1997), S. 231-246 
    ISSN: 1573-1596
    Keywords: Farm forestry ; carbon sequestration ; monitoring ; evaluation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering , Geography
    Notes: Abstract In Mexico an estimated 4.5 × 106ha are available for farm forestry, while up to 6.1 × 106 ha could be saved from deforestation by making shifting agriculture more productive and sustainable. Various farm forestry systems are technically, socially, and economically viable, including live fences, coffee with shade trees, plantations, tree enrichment of fallows, and taungya, with a C-sequestration potential varying from 17.6 to 176.3 Mg C ha−1. A self-reporting system with on-site spot checks is presented for the monitoring and evaluation (M&E), and will be tested in a farm forestry C-sequestration pilot project, to begin in Chiapas, Mexico, in 1997. The M&E procedure will facilitate the collection of field data at low cost, help ensure that the systems continue to address the needs of farmers, and give farmers an understanding of the value of the service that they are providing.
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  • 87
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    Mitigation and adaptation strategies for global change 2 (1997), S. 101-115 
    ISSN: 1573-1596
    Keywords: Carbon dioxide ; costs ; forests ; Joint Implementation ; mitigation ; monitoring ; policies
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering , Geography
    Notes: Abstract Forest sector mitigation options can be grouped into three categories: (1) management for carbon (C) conservation, (2) management for C storage, and (3) management for C substitution. The paper provides background information on the technical potential for C conservation and sequestration worldwide and the average costs of achieving it. It reviews policy measures that have been successfully applied at regional and project levels toward the reduction of atmosphere greenhouse gases. It also describes both national programs and jointly implemented international activities. The monitoring methods, and the items to monitor, differ across these categories. Remote sensing is a good approach for the monitoring of C conservation, but not for C substitution, which requires estimation of the fossil fuels that would be displaced and the continued monitoring of electricity generation sources. C storage, on the other hand, includes C in products which may be traded internationally. Their monitoring will require that bi- or multi-lateral protocols be set up for this purpose.
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  • 88
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    Mitigation and adaptation strategies for global change 2 (1997), S. 231-246 
    ISSN: 1573-1596
    Keywords: Farm forestry ; carbon sequestration ; monitoring ; evaluation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering , Geography
    Notes: Abstract In Mexico an estimated 4.5×106ha are available for farm forestry, while up to 6.1×106ha could be saved from deforestation by making shifting agriculture more productive and sustainable. Various farm forestry systems are technically, socially, and economically viable, including live fences, coffee with shade trees, plantations, tree enrichment of fallows, and taungya, with a C-sequestration potential varying from 17.6 to 176.3 Mg C ha−1. A self-reporting system with on-site spot checks is presented for the monitoring and evaluation (M&E), and will be tested in a farm forestry C-sequestration pilot project, to begin in Chiapas, Mexico, in 1997. The M&E procedure will facilitate the collection of field data at low cost, help ensure that the systems continue to address the needs of farmers, and give farmers an understanding of the value of the service that they are providing.
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  • 89
    ISSN: 1573-2932
    Keywords: petrochemicals ; adsorption ; soil ; multi-components ; fixed-column-reactor ; experiment ; breakthrough
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Present-day massive exploration, extraction, transport, and use of petrochemicals pose a real threat of continuous or occasional accidental contamination of precious groundwater. However, the knowledge of the pathways and mechanisms involved in the transport, retention, and degradation of such chemicals once they are within the soil matrix is very limited. One of the important means of petrochemical retention in the soil is through the process of chemical adsorption onto the soil. An investigation was conducted to observe the adsorption phenomena of several components of petrochemicals (benzene, toluene, and xylene) solved in hexane utilizing the columnar continuous plug-flow configuration of a fixed bed of sands. Three types of soils were investigated for the time variation of the adsorption of the organic chemicals. The results are the indicative values of the adsoption of the principal components of petrochemicals in paacked-soil-bed subjected to tortuous seepage flow conditions of the fluids. The adsorption results are presented in the form of breakthrough curves. The paper includes the analytical methodology of UV spectroscopy which was utilized to measure the concentrations of various chemical components of the petrochemical mixture.
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  • 90
    ISSN: 1573-2932
    Keywords: soil ; pollution ; heavy metals ; smelters ; factoranalysis
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A combined statistical and computergraphic approach is proposed for apportionment and attribution of soil contaminants in complex areas. The field test site lies north of Swansea, south Wales and contains two major pollutant sources, an active nickel refiner and (4 km away) the site of major base metal smelting in the nineteenth century (the Lower Swansea Valley reclamation study area). Soil samples (70 samples, 0–15 cm) were collected on a regular grid of 1000 m interval. They were extracted using 0.05 M diammonium EDTA and the extracts analysed for Cd, Co, Cu, Fe, Mn, Ni, Pb and Zn. Soil pH and %organic content were also determined. Factor analysis yielded three groups which explained 73.8% of the data variance (1: Cd, Cu, %OM, Pb, Zn, Ni; 2: Cd, Zn, Mn, pH; 3: Cu, Mn, Co, Ni, Fe). Isoline plots were classifiable into the same three groups. It was concluded that factor 3 contained those elements associated with smelter emissions, factor 1 with contamination from the Lower Swansea Valley and in factor 2 pedogenetic processes control the occurrence of the elements.
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  • 91
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    Water, air & soil pollution 94 (1997), S. 163-180 
    ISSN: 1573-2932
    Keywords: acid deposition ; liming ; catchment ; lake ; water chemistry ; fish ; soil ; model
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In June 1983 a whole-catchment liming experiment was conducted at Tjønnstrond, southernmost Norway, to test the utility of terrestrial liming as a technique to restore fish populations in remote lakes with short water-retention times. Tjønnstrond consists of 2 small ponds of 3.0 and 1.5 ha in area which drain a 25-ha catchment. The area is located at about 650–700 meters above sea-level in sparse and unproductive forests of spruce, pine and birch with abundant peatlands. A dose of 3 ton/ha of powdered limestone were spread by helicopter to the terrestrial area. No limestone was added to the ponds themselves. The ponds were subsequently stocked with brown and brook trout. Liming caused large and immediate changes in surface water chemistry; pH increased from 4.5 to 7.0, Ca increased from 40 to 200 μeq/L, ANC increased from –30 to +70 μeq/L, and reactive-Al decreased from about 10 to 3 μmol/L. During the subsequent 11 years the chemical composition of runoff has decreased gradually back towards the acidic pre-treatment situation. The major trends in concentrations of runoff Ca, ANC, pH, Al and NO3 in runoff are all well simulated by the acidification model MAGIC. Neither the measured data nor the MAGIC simulations indicate significant changes in any other major ion as a result of liming. The soils at Tjønnstrond in 1992 contained significantly higher amounts of exchangeable Ca relative to those at the untreated reference catchment Storgama. In 1992 about 75% of the added Ca remains in the soil as exchangeable Ca, 15% has been lost in runoff, and 10% is unaccounted for. The whole-catchment liming experiment at Tjønnstrond clearly demonstrates that this liming technique produces a long-term stable and favourable water quality for fish. Brown trout in both ponds in 1994 have good condition factors, which indicate that the fish are not stressed by marginal water quality due to re-acidification. The water quality is still adequate after 11 years and 〉20 water renewals. Concentrations of H+ and inorganic Al have gradually increased and approach levels toxic to trout, but the toxicity of these are offset by the continued elevated Ca concentrations. Reduced sulphate deposition during the last 4 years (1990–94) has also helped to slow and even reverse the rate of reacidification. The experiment at Tjønnstrond demonstrates that for this type of upland, remote terrain typical of large areas of southern Norway, terrestrial liming offers a suitable mitigation technique for treating acidified surface waters with short retention times.
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  • 92
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    Environmental and ecological statistics 4 (1997), S. 49-64 
    ISSN: 1573-3009
    Keywords: soil ; pollution ; threshold ; geostatistics ; indicators ; kriging ; risk ; Swiss Jura
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The probability that the concentrations of toxic substances in soil or other medium exceed tolerablemaxima at any unsampled place can be estimated by indicator geostatistics. The method is developed and used to estimate and map the risk of contamination by cadmium, copper and lead in the topsoil of a 14.5 km 2 region in the Swiss Jura. It combines both direct measurements of metal concentrations and thecalibration of a geological map, and it shows that the risk of toxicity is least on Argovian rocks. Two approaches are proposed to divide a region into safe' and 'hazardous' zones on the basis of probability maps. The first declares as contaminated all places where the risk of contamination exceeds a given threshold. The second approach first evaluates the financial costs that might result from a wrongdeclaration, after which the site is allocated to a class so as to minimize that cost. The risk of exposure for humans and animals is generally greater for contaminated agricultural land than for forest soil, and so land use is taken into account in both procedures.
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  • 93
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    Environmental and ecological statistics 4 (1997), S. 131-152 
    ISSN: 1573-3009
    Keywords: biodiversity ; geographic information systems ; geostatistics ; monitoring ; response surfaces ; spatial analysis
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Echelons provide an objective approach to prospecting for areas of potential concern in synoptic regional monitoring of a surface variable. Echelons can be regarded informally as stacked hill forms. The strategy is to identify regions of the surface which are elevated relative to surroundings (Relative ELEVATIONS or RELEVATIONS). These are areas which would continue to expand as islands with receding (virtual) floodwaters. Levels where islands would merge are critical elevations which delimit echelons in the vertical dimension. Families of echelons consist of surface sectors constituting separate islands for deeper waters that merge as water level declines. Pits which would hold water are disregarded in such a progression, but a complementary analysis of pits is obtained using the surface as a virtual mould to cast a counter-surface (bathymetric analysis). An echelon tree is a family tree of echelons with peaks as terminals and the lowest level as root. An echelon tree thus provides a dendrogram representation of surface topology which enables graph theoretic analysis and comparison of surface structures. Echelon top view maps show echelon cover sectors on the base plane. An echelon table summarizes characteristics of echelons as instances or cases of hill form surface structure. Determination of echelons requires only ordinal strength for the surface variable, and is thus appropriate for environmental indices as well as measurements. Since echelons are inherent in a surface rather than perceptual, they provide a basis for computer-intelligent understanding of surfaces. Echelons are given for broad-scale mammalian species richness in Pennsylvania.
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  • 94
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    Mitigation and adaptation strategies for global change 2 (1997), S. 191-202 
    ISSN: 1573-1596
    Keywords: Carbon storage ; Joint Implementation ; monitoring ; remote sensing
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering , Geography
    Notes: Abstract Adequate monitoring of carbon sequestered by forestry activities is essential to the future of forestry as a climate change mitigation option. A wide range of approaches has been taken to monitor changes in forest carbon attributable to project activities. This paper describes simple, least-cost/least-precision methods, remote sensing, periodic carbon inventories, and traditional research methods. Periodic carbon inventories are the preferred approach because they are cost-effective, provide measurements with known levels of precision, and allow the monitoring of other values such as biodiversity and commercial timber volumes. Verification of monitoring estimates is discussed as an auditing process designed to evaluate reported carbon sequestration values. The limitations of remote sensing for biomass determination and the potential for changes in monitoring approaches due to improvements in technology are briefly reviewed.
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  • 95
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    Journal of fusion energy 16 (1997), S. 231-236 
    ISSN: 1572-9591
    Keywords: Dust ; radioactive inventory ; removal ; monitoring
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In the future fusion reactor, dust control may become more important for safety, than for existing fusion facilities. Some estimations show more than hundreds kg/yr dust will be generated from the plasma facing materials in the vacuum vessel. If we consider continuously operating plant, dust should be monitored and removed during the operation time. Optical monitoring methods and electrostatic removal methods are useful approaches to accomplish this. An investigation of the development of the dust removal system for a fusion reactor is reported in this paper.
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  • 96
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    Water, air & soil pollution 96 (1997), S. 61-71 
    ISSN: 1573-2932
    Keywords: allotment gardens ; dustfall ; ground water ; heavy metals ; oil refinery ; soil ; vegetables
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In the period 1984–1990 the following vegetables were grown: red beet, carrot and parsley in four allotment gardens of Płock city (Central Poland), situated near the refinery and petrochemical works. Cadmium, lead, copper, chromium, zinc and manganese concentrations were determined in the leaves and roots of vegetables. The heavy metal accumulation in the soil, dustfall (measure of air pollution), and ground water was determined. The quality of the vegetable yield, notably of the leaves, was low. This was mainly due to the excessive chromium and cadmium content in the leaves. Accumulation of heavy metals was relatively low in the soil, rather high in the ground water and variable in the dust.
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  • 97
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    Water, air & soil pollution 96 (1997), S. 61-71 
    ISSN: 1573-2932
    Keywords: allotment gardens ; dustfall ; ground water ; heavy metals ; oil refinery ; soil ; vegetables
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In the period 1984–1990 the following vegetables were grown: red beet, carrot and parsley in four allotment gardens of Płock city (Central Poland), situated near the refinery and petrochemical works. Cadmium, lead, copper, chromium, zinc and manganese concentrations were determined in the leaves and roots of vegetables. The heavy metal accumulation in the soil, dustfall (measure of air pollution), and ground water was determined. The quality of the vegetable yield, notably of the leaves, was low. This was mainly due to the excessive chromium and cadmium content in the leaves. Accumulation of heavy metals was relatively low in the soil, rather high in the ground water and variable in the dust.
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  • 98
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    Water, air & soil pollution 94 (1997), S. 59-69 
    ISSN: 1573-2932
    Keywords: fly-ash particles ; ombrotrophic peats ; air pollution history ; monitoring
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The movement of fly-ash particles in a sequence ofSphagnum moss was studied in laboratory experiments and field investigations. The data obtained in the laboratory show that only 0.8% of particles, placed on the surface of a 6–10 cm thickSphagnum layer, were washed out with water (700–750 mm) during the 241 days of the experiment. The majority of added particles were fixed in the upper part (90% in 1–3 cm) of the moss layer. A SEM study indicates that sorption is slightly species-dependent due to the micromorphological parameters of theSphagnum species. The storage of particles bySphagnum mosses allows the use of natural sequences to study the history of atmospheric pollution. The distribution of particles in the upper part of moss layers in Viru Bog (50 km east of Tallinn, North Estonia) shows good agreement with the known air pollution history in Tallinn.
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  • 99
    ISSN: 1573-2932
    Keywords: soil ; pollution ; heavy metals ; smelters ; factor analysis
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A combined statistical and computergraphic approach is proposed for apportionment and attribution of soil contaminants in complex areas. The field test site lies north of Swansea, south Wales and contains two major pollutant sources, an active nickel refiner and (4 km away) the site of major base metal smelting in the nineteenth century (the Lower Swansea Valley reclamation study area). Soil samples (70 samples, 0–15 cm) were collected on a regular grid of 1000 m interval. They were extracted using 0.05 M diammonium EDTA and the extracts analysed for Cd, Co, Cu, Fe, Mn, Ni, Pb and Zn. Soil pH and %organic content were also determined. Factor analysis yielded three groups which explained 73.8% of the data variance (1: Cd, Cu, %OM, Pb, Zn, Ni; 2: Cd, Zn, Mn, pH; 3: Cu, Mn, Co, Ni, Fe). Isoline plots were classifiable into the same three groups. It was concluded that factor 3 contained those elements associated with smelter emissions, factor 1 with contamination from the Lower Swansea Valley and in factor 2 pedogenetic processes control the occurrence of the elements.
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  • 100
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    Water, air & soil pollution 94 (1997), S. 225-245 
    ISSN: 1573-2932
    Keywords: acid precipitation ; Quebec ; lakewater quality ; acidification and recovery ; monitoring
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A total of 51 lakes in southern Quebec, Canada, were sampled between 1985 and 1993 to study changes in water chemistry following reductions in SO2 emissions (main precursor of acid precipitation). Time series analysis of precipitation chemistry revealed significant reductions in concentrations and deposition of SO4 2- from 1981 to 1992 in southern Quebec as well as reductions in concentrations and deposition of base cations (Ca2+, Mg2+), NO3 - and H+ in the western section of the study area. Reductions in atmospheric inputs of SO4 2- have resulted in decreased lakewater SO4 2- concentrations in the majority of the lakes in our study, although only a small fraction (9 of 37 lakes used in the temporal analysis) have improved significantly in terms of acidity status (pH, acid neutralizing capacity – ANC). The main response of the lakes to decreased SO4 2- is a decrease in base cations (Ca2++Mg2+), which was observed in 17 of 37 lakes. Seventeen lakes also showed significant increases in dissolved organic carbon (DOC) over the period of study. The resulting increases in organic acidity as well as the decrease in base cations could both play a role in delaying the recovery of our lakes.
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