Publication Date:
2015-04-02
Description:
The impact of different boundary layer source regions in Asia on the chemical composition of the Asian monsoon anticyclone, considering its intraseasonal variability in 2012, is analysed by CLaMS simulations using artificial emission tracers. Our simulations show that the Asian monsoon anticyclone is highly variable in location and shape and oscillates between 2 states: first a symmetric anticyclone and second, an asymmetric anticyclone either elongated or split in two smaller anticyclones. A maximum in the distribution of air originating from Indian/Chinese boundary layer sources is usually found in the core of the symmetric anticyclone, in contrast the asymmetric state is characterised by a double peak structure in the horizontal distribution of air originating from India and China. The simulated horizontal distribution of artificial emission tracers for India/China is in agreement with patterns found in satellite measurements of O3 and CO by the Aura Microwave Limb Sounder (MLS). The contribution of different boundary source regions to the Asian monsoon anticyclone strongly depends on its intraseasonal variability and is therefore more complex than hitherto believed, but in general the highest contributions are from North India and Southeast Asia at 380 K. In the early (June to mid-July) and late (mid-August to October) period of the monsoon 2012, contributions of emissions from Southeast Asia are highest and in the intervening period (≈ mid-July to mid-August) emissions from North India have the largest impact. Further, our simulations confirm that the thermal tropopause above the anticyclone constitutes a vertical transport barrier. Enhanced contributions of emission tracers for Asia are found at the northern flank of the Asian monsoon anticyclone between double tropopauses indicating an isentropic transport from the anticyclone into the lowermost stratosphere. After the breakup of the anticyclone, significant contributions of air masses originating in India/China are sill found over Asia in September/October. In addition, these air masses spread out within the mid-latitudes of the Northern Hemisphere and in the tropics at around 380 K. Moreover, air masses from Southeast Asia experienced diabatic upward transport in the tropics and subsequently isentropic poleward transport occurs at around 380 K with the result that the extratropical lowermost stratosphere is flooded by end of September with air masses originating in Southeast Asia. Our results demonstrate that emissions from Asia have a significant impact on the chemical compositions of the lowermost stratosphere of the Northern Hemisphere in particular after the end of the monsoon season in September/October 2012.
Electronic ISSN:
1680-7375
Topics:
Geosciences
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