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  • American Institute of Physics (AIP)  (10)
  • Springer Nature  (9)
  • Wiley-Blackwell  (5)
  • American Geophysical Union (AGU)
  • 1995-1999  (6)
  • 1990-1994  (9)
  • 1975-1979  (9)
  • 1
    Electronic Resource
    Electronic Resource
    State-to-state vibrational energy transfer in DF(v=1–3) (1990)
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 93 (1990), S. 3207-3214 
    Details
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: Overtone vibration–laser double resonance studies of DF(v=1–3) energy transfer yield self-relaxation rate constants for v=1, 2 and 3 of k1=(0.37±0.06)×10−12 cm3 mol−1 s−1, k2=(22.0±2.0)×10−12 cm3 mol−1 s−1, and k3=(17.0±1.8)×10−12 cm3 mol−1 s−1, respectively. The approach also directly measures the relative importance of vibration-to-vibration (V–V) and vibration-to-translation-and-rotation (V–T,R) energy transfer. The fraction of DF(v) molecules relaxing by V–V energy transfer is 1.1±0.1 and 0.72±0.10 for v=2 and v=3, respectively. Essentially all of the vibrational energy transfer in v=2 occurs via the V–V mechanism. The slower relaxation of DF(v=3) compared to DF(v=2), in contrast to simple scaling law predictions, reflects the decreasing influence of the V–V mechanism, even though it is still the primary relaxation pathway for DF(v=3). Comparison with HF self-relaxation qualitatively indicates that V–R energy transfer is important in V–T,R relaxation of DF(v=1).
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1063/1.458853
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  • 2
    Electronic Resource
    Electronic Resource
    Finite-dimensional behavior in dissipative partial differential equations (1995)
    Woodbury, NY : American Institute of Physics (AIP)
    Chaos 5 (1995), S. 330-345 
    Details
    ISSN: 1089-7682
    Source: AIP Digital Archive
    Topics: Physics
    Notes: Dissipative partial differential equations have applications throughout the sciences: models of turbulence in fluids, chemical reactions, and morphogenesis in biology can all be written in a general form which allows them to be subjected to a unified analysis. Recent results on these equations show that in many cases they are not as complex as they initially appear, and can be converted into a set of ordinary differential equations. However, most of the relevant references present a bewildering array of terms which can obscure the simple underlying ideas. The main purpose of this paper is to introduce this terminology, motivated by several major results, slowly and by example. Detailed proofs are omitted, but it is hoped that this approach will give a good understanding of and intuitive feel for the subject without recourse to technicalities. Nevertheless, sufficient mathematical detail is included to allow application of these results to many examples. © 1995 American Institute of Physics.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1063/1.166081
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  • 3
    Electronic Resource
    Electronic Resource
    New vapor phase spontaneous Raman spectrometer (1992)
    [S.l.] : American Institute of Physics (AIP)
    Review of Scientific Instruments 63 (1992), S. 3280-3284 
    Details
    ISSN: 1089-7623
    Source: AIP Digital Archive
    Topics: Physics , Electrical Engineering, Measurement and Control Technology
    Notes: A highly sensitive, spontaneous Raman spectrometer designed for the study of vapors and other low-density samples is discussed. The high sensitivity is achieved by means of the novel combination of a multipass light cell and a high-temperature gasdynamic focusing system. A complete description of the apparatus is given, along with the results of a sensitivity test in ambient air, as well as results demonstrating gasdynamic focusing of a vapor and Raman transitions in such a sample.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1063/1.1142537
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  • 4
    Electronic Resource
    Electronic Resource
    Imaging nanometer-thick patterned self-assembled monolayers via second-harmonic generation microscopy (1997)
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 81 (1997), S. 2051-2054 
    Details
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: We have used the inherent surface sensitivity of second-harmonic generation to develop an instrument for nonlinear optical microscopy of surfaces and interfaces. This optical technique is ideal for imaging nanometer-thick, chromophoric self-assembled monolayers (SAMs), which have been patterned using photolithographic techniques. In this paper, we demonstrate the application of second-harmonic generation microscopy to patterned SAMs of the noncentrosymmetric molecule calixarene and discuss the resolution and sensitivity limits of the technique. © 1997 American Institute of Physics.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1063/1.364284
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  • 5
    Electronic Resource
    Electronic Resource
    Instrumentation and cell design for in situ studies of electrode surfaces using x-ray synchrotron radiation : Proceedings of the 4th international conference on synchrotron radiation instrumentation (1992)
    [S.l.] : American Institute of Physics (AIP)
    Review of Scientific Instruments 63 (1992), S. 950-955 
    Details
    ISSN: 1089-7623
    Source: AIP Digital Archive
    Topics: Physics , Electrical Engineering, Measurement and Control Technology
    Notes: As an integral part of a program to develop x-ray techniques for in situ structural studies of electrode surfaces, a series of experiments has been carried out using x-ray diffraction (XRD) and x-ray absorption spectroscopy (XAS) at the Daresbury SRS. These studies, which involve continuous control of the electrode potential and the need to probe the electrode surface with synchrotron radiation, demand careful attention to cell design. Three types of experiment are described in order to illustrate possible approaches to cell design and the versatility of in situ x-ray techniques.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1063/1.1143789
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  • 6
    Electronic Resource
    Electronic Resource
    The DIII-D lithium beam edge diagnostic system (abstract) : Proceedings of the 9th topical conference on high temperature plasma diagnostics (1992)
    [S.l.] : American Institute of Physics (AIP)
    Review of Scientific Instruments 63 (1992), S. 4940-4940 
    Details
    ISSN: 1089-7623
    Source: AIP Digital Archive
    Topics: Physics , Electrical Engineering, Measurement and Control Technology
    Notes: We are installing a diagnostic system based on a neutral lithium beam to investigate plasma behavior in the edge region of DIII-D discharges [D. M. Thomas et al., Rev. Sci. Instrum. 61, 3040 (1990]. The system will provide neutral equivalent current densities of several mA/cm2 at beam energies from 5 to 30 keV, sufficient to penetrate several centimeters past the last closed flux surface in most of the DIII-D operating regime. Fluorescence of the beam atoms is induced by collisions with plasma particles and is a sensitive measure of the edge density behavior. The emitted 670.8-nm fluorescence is collected and coupled via fiber optics to a multichannel high-speed data acquisition system based on silicon diode detectors. Because of the favorable atomic properties of lithium (i.e., high electron impact excitation cross section, resonance wavelength well separated from Hα) we should be able to study density fluctuations in this region from an analysis of the associated fluctuations in the beam fluorescence. A description of the installed diagnostic, test stand measurements of intrinsic beam fluctuations and any initial operating experience on DIII-D will be presented. This work supported by U. S. Department of Energy Grant No. DE-FG03-90ER5408 and Contract DE-AC03-89ER51114, which support does not constitute an endorsement by DOE of views expressed in this publication.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1063/1.1143502
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  • 7
    Electronic Resource
    Electronic Resource
    A CO2 laser tangential imaging system for CDX-U (abstract) : Proceedings of the 9th topical conference on high temperature plasma diagnostics (1992)
    [S.l.] : American Institute of Physics (AIP)
    Review of Scientific Instruments 63 (1992), S. 4983-4983 
    Details
    ISSN: 1089-7623
    Source: AIP Digital Archive
    Topics: Physics , Electrical Engineering, Measurement and Control Technology
    Notes: In a previous paper [R. Nazikian and B. Grek, Rev. Sci. Instrum. 61, 2899 (1990)], it was shown that tangential imaging provides a powerful new technique for rendering two-dimensional images of local density fluctuations in toroidal plasma devices. The technique consists of projecting a CO2 laser beam tangent to magnetic field lines at the plasma midplane and using phase contrast or other related optical methods for imaging line integral density fluctuations. In this paper we present recent progress in the development of such an imaging system for CDX-U. The interferometer makes use of a novel variation on the Zernike phase contrast method for detecting phase variations impressed on laser beams propagating through random media. This work supported by Department of Energy contract No. DE-AC02-76-CHO-3073.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1063/1.1143519
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  • 8
    Electronic Resource
    Electronic Resource
    A spectroscopic study of CaOCH3 using the pump/probe microwave and the molecular beam/optical Stark techniques (1998)
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 109 (1998), S. 5283-5289 
    Details
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: The Stark effect on the qR22(0,0.5) (ν=17 682.9251 cm−1) and qP11(0,1.5) (ν=17 682.1966 cm−1) branch features of the (0,0) B 2A1–X 2A1 band system of calcium methoxide, CaOCH3, was measured and analyzed to give the magnitude of the permanent electronic dipole moments, |μ|, of 1.58(8) D and 1.21(5) D for the X 2A1 and B 2A1 states, respectively. The dipole moments are compared with other monovalent calcium compounds and those predicted from a simple electrostatic model. Pure rotational transitions in the X 2A1 state were recorded using the pump/probe microwave-optical double resonance technique. The proton magnetic hyperfine splitting pattern confirms a C3v symmetry of the ground electronic state. The determined Fermi contact and dipolar parameters are: aF=−0.421(27) MHz; Taa=1.070(45) MHz, and |Tbb−Tcc|=0.292(47) MHz. The latter parameter is associated with the lifting of the K-degeneracy of this symmetric top molecule and mixing the I0=1/2 and I0=3/2 levels. © 1998 American Institute of Physics.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1063/1.477146
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  • 9
    Electronic Resource
    Electronic Resource
    The permanent electric dipole moments of chromium and vanadium mononitride: CrN and VN (1999)
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 110 (1999), S. 881-889 
    Details
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: The Pe(1), F″=2.5 branch feature of the (0,0) D 3Π0e–X 3Δ1 band system of 51VN was recorded as a function of an applied static electric field. The resultant Stark splitting and shifts were analyzed giving values of 3.07(7) D and 6.1(4) D for the X 3Δ1 and D 3Π0e states, respectively, for the magnitude of the permanent electric dipole moment, |μ|. Similarly, the Ree(0.5) branch feature of the (0,0) A 4Π3/2–X 4Σ− band system of 52CrN was recorded as a function of an applied static electric field and analyzed to produce |μ| values of 2.31(4) D and 5.42(2) D for the X 4Σ− and A 4Π3/2 states, respectively. In order to facilitate the dipole moment determinations for 52CrN it was necessary to record and analyze the field free spectrum of the (0,0) A 4Π3/2–X 4Σ− subband system. A comparison of the dipole moments for the first row monoxides and mononitrides is made and trends are discussed with reference to a molecular orbital correlation scheme. © 1999 American Institute of Physics.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1063/1.478055
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  • 10
    Electronic Resource
    Electronic Resource
    High resolution spectroscopy of BaCH3(X˜ 2A1): Fine and hyperfine structure analysis (1998)
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 108 (1998), S. 2703-2711 
    Details
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: The pure rotational spectrum of BaCH3(X˜ 2A1) in its ground vibrational state has been recorded using millimeter/submillimeter direct absorption techniques, the first spectroscopic information obtained for this molecule. The radical was created using Broida-type oven/d.c. discharge methods by the reaction of barium vapor and Sn(CH3)4. Twenty-eight rotational transitions of the main isotopomer 138BaCH3 were recorded, as well as five for 136BaCH3 and three for the 137BaCH3 species. Being a prolate symmetric top, K ladder structure was observed in all transitions for BaCH3, as well as fine structure splittings which arise from the unpaired electron in the molecule. For the 137Ba isotopomer, hyperfine interactions were also resolved, arising from the spin of the barium nucleus. The complete data set has been analyzed with a 2A Hamiltonian, and rotational, spin-rotational, and magnetic hyperfine/nuclear quadrupole parameters accurately determined. The fine and hyperfine structure constants established from this study suggest a predominantly ionic bond for BaCH3, but with a considerable covalent component. Structural parameters for BaCH3 derived in this work are consistent with those of other alkaline earth monomethyl species. © 1998 American Institute of Physics.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1063/1.475662
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