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  • Articles  (32)
  • American Institute of Physics (AIP)
  • Blackwell Publishing Ltd
  • Cambridge University Press
  • 2015-2019  (12)
  • 1975-1979  (20)
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  • Articles  (32)
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  • 1
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    Optimization of an exchange-correlation density functional for water (2016)
    American Institute of Physics (AIP)
    Details
    Publication Date: 2016-06-10
    Description: We describe a method, that we call data projection onto parameter space (DPPS), to optimize an energy functional of the electron density, so that it reproduces a dataset of experimental magnitudes. Our scheme, based on Bayes theorem, constrains the optimized functional not to depart unphysically from existing ab initio functionals. The resulting functional maximizes the probability of being the “correct” parameterization of a given functional form, in the sense of Bayes theory. The application of DPPS to water sheds new light on why density functional theory has performed rather poorly for liquid water, on what improvements are needed, and on the intrinsic limitations of the generalized gradient approximation to electron exchange and correlation. Finally, we present tests of our water-optimized functional, that we call vdW-DF-w, showing that it performs very well for a variety of condensed water systems.
    Print ISSN: 0021-9606
    Electronic ISSN: 1089-7690
    Topics: Chemistry and Pharmacology , Physics
    Published by American Institute of Physics (AIP)
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  • 2
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    Characterizing solid-state ignition of runaway chemical reactions in Ni-Al nanoscale multilayers under uniform heating (2015)
    American Institute of Physics (AIP)
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    Publication Date: 2015-10-08
    Description: Nanoscale layers of nickel and aluminum can mix rapidly to produce runaway reactions. While self-propagating high temperature synthesis reactions have been observed for decades, the solid-state ignition of these reactions has been challenging to study. Particularly elusive is characterization of the low-temperature chemical mixing that occurs just prior to the ignition of the runaway reaction. Characterization can be challenging due to inhomogeneous microstructures, uncontrollable heat losses, and the nonuniform distribution of heat throughout the material prior to ignition. To reduce the impact of these variables, we heat multilayered Ni/Al foils in a highly uniform manner and report ignition temperatures as low as 245 °C for heating rates ranging from 2000 °C/s to 50 000 °C/s. Igniting in this way reveals that there are four stages before the reaction is complete: heating to an ignition temperature, low temperature solid-state mixing, a separate high temperature solid-state mixing, and liquid-state mixing. Multiple bilayer spacings, heating rates, and heating times are compared to show that the ignition temperature is a function of the bilayer spacing. A symmetric numerical diffusion model is used to show that there is very little chemical mixing in the first 10 ms of heating but significant mixing after 50 ms. These predictions suggest that ignition temperatures should increase for the slowest heating rates but this trend could not be identified clearly. The modeling was also used to examine the kinetic parameters governing the early stages of solid-state diffusion and suggest that grain boundary diffusion is dominant.
    Print ISSN: 0021-8979
    Electronic ISSN: 1089-7550
    Topics: Physics
    Published by American Institute of Physics (AIP)
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  • 3
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    The creation of large-volume, gradient-free warm dense matter with an x-ray free-electron laser (2015)
    American Institute of Physics (AIP)
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    Publication Date: 2015-03-25
    Description: The efficiency and uniformity of heating induced by hard x-ray free-electron laser pulse is investigated for 0.5  μ m silver foils using the X-ray Pump Probe instrument at the Linac Coherent Light Source facility. Intense 8.9 keV x-ray pulses of 60 fs duration deposit energy predominantly via inner-shell ionization to create a non-equilibrium Ag solid density plasma. The x-ray pulses are focused to 14 × 17  μ m 2 by means of beryllium lenses and by varying the total beam energy, the energy deposition is varied over a range of irradiances from 4.4 to 6.5 × 10 15  W/cm 2 . Two time-and-space resolved interferometers simultaneously probed the expansion of the front and rear sample surfaces and find evidence of a nearly symmetric expansion pointing to the uniformity of energy deposition over the full target thickness. The experimental results are compared with two different hydrodynamic simulations of the sample expansion. The agreement between experimental and theoretical results yields an estimate of the temperature evolution as a function of x-ray irradiance that varies from 8 to 10 eV for the x-ray irradiances studied.
    Print ISSN: 1070-664X
    Electronic ISSN: 1089-7674
    Topics: Physics
    Published by American Institute of Physics (AIP)
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  • 4
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    Lake-level variability in Salar de Coipasa, Bolivia during the past ∼40,000 yr (2018)
    Cambridge University Press
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    Publication Date: 2018
    Description: 〈div data-abstract-type="normal"〉〈p〉Various paleoclimatic records have been used to reconstruct the hydrologic history of the Altiplano, relating this history to past variability of the South American summer monsoon. Prior studies of the southern Altiplano, the location of the world’s largest salt flat, the Salar de Uyuni, and its neighbor, the Salar de Coipasa, generally agree in their reconstructions of the climate history of the past ∼24 ka. Some studies, however, have highly divergent climatic records and interpretations of earlier periods. In this study, lake-level variation was reconstructed from a ∼14-m-long sediment core from the Salar de Coipasa. These sediments span the last ∼40 ka. Lacustrine sediment accumulation was apparently continuous in the basin from ∼40 to 6 ka, with dry or very shallow conditions afterward. The fossil diatom stratigraphy and geochemical data (δ〈span〉13〈/span〉C, δ〈span〉15〈/span〉N, %Ca, C/N) indicate fluctuations in lake level from shallow to moderately deep, with the deepest conditions correlative with the Heinrich-1 and Younger Dryas events. The stratigraphy shows a continuous lake of variable depth and salinity during the last glacial maximum and latter stages of Marine Oxygen Isotope Stage 3 and is consistent with environmental inferences and the original chronology of a drill core from Salar de Uyuni.〈/p〉〈/div〉
    Print ISSN: 0033-5894
    Electronic ISSN: 1096-0287
    Topics: Geography , Geosciences
    Published by Cambridge University Press
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  • 5
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    p+-doping analysis of laser fired contacts for silicon solar cells by Kelvin probe force microscopy (2016)
    American Institute of Physics (AIP)
    Details
    Publication Date: 2016-03-15
    Description: Local rear contacts for silicon passivated emitter and rear contact solar cells can be established by point-wise treating an Al layer with laser radiation and thereby establishing an electrical contact between Al and Si bulk through the dielectric passivation layer. In this laser fired contacts (LFC) process, Al can establish a few μ m thick p + -doped Si region below the metal/Si interface and forms in this way a local back surface field which reduces carrier recombination at the contacts. In this work, the applicability of Kelvin probe force microscopy (KPFM) to the investigation of LFCs considering the p + -doping distribution is demonstrated. The method is based on atomic force microscopy and enables the evaluation of the lateral 2D Fermi-level characteristics at sub-micrometer resolution. The distribution of the electrical potential and therefore the local hole concentration in and around the laser fired region can be measured. KPFM is performed on mechanically polished cross-sections of p + -doped Si regions formed by the LFC process. The sample preparation is of great importance because the KPFM signal is very surface sensitive. Furthermore, the measurement is responsive to sample illumination and the height of the applied voltage between tip and sample. With other measurement techniques like micro-Raman spectroscopy, electrochemical capacitance-voltage, and energy dispersive X-ray analysis, a high local hole concentration in the range of 10 19  cm −3 is demonstrated in the laser fired region. This provides, in combination with the high spatial resolution of the doping distribution measured by KPFM, a promising approach for microscopic understanding and further optimization of the LFC process.
    Print ISSN: 0021-8979
    Electronic ISSN: 1089-7550
    Topics: Physics
    Published by American Institute of Physics (AIP)
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  • 6
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    PEDOT:PSS emitters on multicrystalline silicon thin-film absorbers for hybrid solar cells (2015)
    American Institute of Physics (AIP)
    Details
    Publication Date: 2015-02-26
    Description: We fabricated an efficient hybrid solar cell by spin coating poly(3,4-ethylene-dioxythiophene):polystyrenesulfonate (PEDOT:PSS) on planar multicrystalline Si (mc-Si) thin films. The only 5  μ m thin Si absorber layers were prepared by diode laser crystallization of amorphous Si deposited by electron beam evaporation on glass. On these absorber layers, we studied the effect of SiO x and Al 2 O 3 terminated Si surfaces. The short circuit density and power conversion efficiency (PCE) of the mc-Si/Al 2 O 3 /PEDOT:PSS solar cell increase from 20.6 to 25.4 mA/cm 2 and from 7.3% to 10.3%, respectively, as compared to the mc-Si/SiO x /PEDOT:PSS cell. Al 2 O 3 lowers the interface recombination and improves the adhesion of the polymer film on the hydrophobic mc-Si thin film. Open circuit voltages up to 604 mV were reached. This study demonstrates the highest PCE so far of a hybrid solar cell with a planar thin film Si absorber.
    Print ISSN: 0003-6951
    Electronic ISSN: 1077-3118
    Topics: Physics
    Published by American Institute of Physics (AIP)
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  • 7
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    On the wave structure of the wall region of a turbulent boundary layer (1975)
    Cambridge University Press
    Details
    Publication Date: 1975-07-29
    Description: Following the ideas suggested by Landahl (1967, 1975), some model calculations of the fluctuating velocity field in the wall region of a turbulent boundary layer have been carried out. It was assumed that the turbulent stresses are generated intermittently on small scales in time and space owing to bursting-type motions. The Reynolds-stress distribution during bursting periods and the mean velocity profile were assumed to be known, and the linear large-scale response to a random system of bursts was computed using an idealized model for the joint probability distribution in time and space of the occurrence of bursts. Computed energy spectra of the streamwise velocity fluctuations display scales in the spanwise and streamwise directions and time which are in good agreement with measurements by Morrison, Bullock & Kronauer (1971). However, the wavenumber band-widths of the computed spectra are narrower than those of the measured ones. This discrepancy is probably due to the crudeness of the model employed for the Reynolds stress during bursting. © 1975, Cambridge University Press. All rights reserved.
    Print ISSN: 0022-1120
    Electronic ISSN: 1469-7645
    Topics: Mechanical Engineering, Materials Science, Production Engineering, Mining and Metallurgy, Traffic Engineering, Precision Mechanics , Physics
    Published by Cambridge University Press
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  • 8
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    The Permafrost Young Researchers Network (PYRN) is getting older: The past, present, and future of our evolving community (2019)
    Cambridge University Press
    Details
    Publication Date: 2019-02-07
    Description: A lasting legacy of the International Polar Year (IPY) 2007–2008 was the promotion of the Permafrost Young Researchers Network (PYRN), initially an IPY outreach and education activity by the International Permafrost Association (IPA). With the momentum of IPY, PYRN developed into a thriving network that still connects young permafrost scientists, engineers, and researchers from other disciplines. This research note summarises (1) PYRN’s development since 2005 and the IPY’s role, (2) the first 2015 PYRN census and survey results, and (3) PYRN’s future plans to improve international and interdisciplinary exchange between young researchers. The review concludes that PYRN is an established network within the polar research community that has continually developed since 2005. PYRN’s successful activities were largely fostered by IPY. With 〉200 of the 1200 registered members active and engaged, PYRN is capitalising on the availability of social media tools and rising to meet environmental challenges while maintaining its role as a successful network honouring the legacy of IPY.
    Print ISSN: 0032-2474
    Electronic ISSN: 1475-3057
    Topics: Ethnic Sciences , Geography
    Published by Cambridge University Press
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  • 9
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    “Frozen-Ground Cartoons”: Permafrost comics as an innovative tool for polar outreach, education, and engagement (2018)
    Cambridge University Press
    Details
    Publication Date: 2018-09-01
    Description: Permafrost occupies 20 million square kilometres of Earth’s high-latitude and high-altitude landscapes. These regions are sensitive to climate change and human activities; hence, permafrost research is of considerable scientific and societal importance. However, the results of this research are generally not known by the general public. Communicating scientific concepts is an increasingly important task in the research world. Different ways to engage learners and incorporate narratives in teaching materials exist, yet they are generally underused. Here we report on an international scientific outreach project called “Frozen-Ground Cartoons”, which aims at making permafrost science accessible and fun for students, teachers, and parents through the creation of comic strips. We present the context in which the project was initiated, as well as recent education and outreach activities. The future phases of the project primarily involve a series of augmented reality materials, such as maps, photos, videos, and 3D drawings. With this project we aim to foster understanding of permafrost research among broader audiences, inspire future permafrost researchers, and raise public and science community awareness of polar science, education, outreach, and engagement.
    Print ISSN: 0032-2474
    Electronic ISSN: 1475-3057
    Topics: Ethnic Sciences , Geography
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  • 10
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    A ~6000 yr diatom record of mid- to late Holocene fluctuations in the level of Lago Wiñaymarca, Lake Titicaca (Peru/Bolivia) (2017)
    Cambridge University Press
    Details
    Publication Date: 2017-08-02
    Description: A multidecadal-scale lake-level reconstruction for Lago Wiñaymarca, the southern basin of Lake Titicaca, has been generated from diatom species abundance data. These data suggest that ~6500 cal yr BP Lago Wiñaymarca was dry, as indicated by a sediment unconformity. At ~4400 cal yr BP, the basin began to fill, as indicated by the dominance of shallow epiphytic species. It remained somewhat saline with extensive wetlands and abundant aquatic plants until ~3800 cal yr BP, when epiphytic species were replaced by planktic saline-indifferent species, suggesting a saline shallow lake. Wiñaymarca remained a relatively shallow lake that fluctuated on a multidecadal scale until ~1250 cal yr BP, when freshwater planktic species increased, suggesting a rise in lake level with a concomitant decrease in salinity. The lake became gradually fresher, dominated by deep, freshwater species from ~850 cal yr BP. By ~80 cal yr BP, saline-tolerant species were rare, and the lake was dominated by freshwater planktic diatoms, resembling the fresh and deep lake of today. These results reveal a more dynamic and chronologically specific record of lake-level fluctuations and associated ecological conditions that provide important new data for paleoclimatologists and archaeologists, to better understand human-environmental dynamics during the mid- to late Holocene.
    Print ISSN: 0033-5894
    Electronic ISSN: 1096-0287
    Topics: Geography , Geosciences
    Published by Cambridge University Press
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