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  • Articles  (98)
  • acidification  (98)
  • Energy, Environment Protection, Nuclear Power Engineering  (98)
  • 1
    Electronic Resource
    Electronic Resource
    Agriculture's share in the emission of trace gases affecting the climate and some cause-oriented proposals for sufficiently reducing this share
    Amsterdam : Elsevier
    Environmental Pollution 83 (1994), S. 95-111 
    Details
    ISSN: 0269-7491
    Keywords: acidification ; agriculture ; climate change ; eutrophication ; greenhouse gases
    Source: Elsevier Journal Backfiles on ScienceDirect 1907 - 2002
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1016/0269-7491(94)90027-2
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  • 2
    Electronic Resource
    Electronic Resource
    Dolomite limits acidification of a biofilter degrading dimethyl sulphide (1999)
    Springer
    Biodegradation 10 (1999), S. 399-404 
    Details
    ISSN: 1572-9729
    Keywords: acidification ; biofilter ; dimethyl sulphide ; dolomite ; inoculation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract The applicability of dolomite particlesto control acidificationin a Hyphomicrobium MS3inoculated biofilter removingdimethyl sulphide (Me2S) wasstudied. While direct inoculationof the dolomite particles with theliquid microbial culture was notsuccessful, start-up ofMe2S-degradation in thebiofilter was observed when thedolomite particles were mixed with33% (wt/wt) of Hyphomicrobium MS3-inoculatedcompost or wood bark material.Under optimal conditions, anelimination capacity (EC) of 1680~g Me2S m-3 d-1 wasobtained for the compost/dolomitebiofilter. Contrary to a wood barkor compost biofilter, no reductionin activity due to acidificationwas observed in these biofiltersover a 235 day period because ofthe micro environmentneutralisation of the microbialmetabolite H2SO4 with thecarbonate in the dolomite material.However, performance of thebiofilter decreased when themoisture content of the mixedcompost/dolomite material droppedbelow 15%. Next to this, nutrientlimitation resulted in a gradualdecrease of the EC andsupplementation of a nitrogensource was a prerequisite to obtaina long-term high EC (〉 250 gMe2S m-3 d-1) forMe2S. In relation to thisnitrogen supplementation, it wasobserved that stable ECs forMe2S were obtained when thisnutrient was dosed to the biofilterat a Me2S-C/NH4Cl-Nratio of about 10.Abbreviations:DW – dry weight,EC – elimination capacity,Me2S – dimethyl sulphide,OL – organic loading rate,VS - volatile solids
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1008345609743
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  • 3
    Electronic Resource
    Electronic Resource
    Deposition Monitoring in Europe (1998)
    Springer
    Environmental monitoring and assessment 53 (1998), S. 279-295 
    Details
    ISSN: 1573-2959
    Keywords: acidification ; dry and wet deposition ; euthrophication ; monitoring
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A monitoring station for atmospheric deposition was designed and constructed. Three such stations were applied in a pilot project for a year on three sites (Speulder forest in The Netherlands, Auchencorth in Scotland and Melpitz in Germany) in different regions in Europe to estimate local inputs and to validate deposition models which are currently used or developed to estimate ecosystem specific deposition in Europe. Fluxes at Auchencorth Moss are lowest for all components, except for those much influenced by the sea as a source. As Melpitz is located far away from seas, these components are lowest at this site. Wet deposition is the dominant source of input at Auchencorth, whereas at Speulder forest, through its roughness and pollution climate, dry deposition is dominant. At this site dry deposition velocities are highest. Melpitz is a polluted site. Particularly sulphur deposition is high. It is recommended to equip several locations in Europe with intensive deposition monitoring methods. Such a network will be an extension of existing monitoring programmes on air pollution, such as that run by Eurepean Monitoring and Evaluation Programme for the long-range transmission of air pollutants in Europe (EMEP). The intensive monitoring locations should be selected based on pollution climates and type of vegetation, common in Europe.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1005818820053
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  • 4
    Electronic Resource
    Electronic Resource
    Transboundary air pollution and soil acidification: A dynamic analysis of an acid rain game between Finland and the USSR (1992)
    Springer
    Environmental and resource economics 2 (1992), S. 161-181 
    Details
    ISSN: 1573-1502
    Keywords: Pollution contron ; acidification ; acid rain game ; transboundary air pollution
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering , Economics
    Notes: Abstract Transboundary air pollution is analysed as a dynamic game between Finland and the nearby areas of the Soviet Union. Sulphur emissions are used as the environmental control variables and the acidities of the soils as the state variables. Acidification is consequently considered to be a stock pollutant having long-lasting harmful effects on the environment. The state dynamics consist of two relationships: first, of a sulphur transportation model between the regions and, second, of a model describing how the quality of the soil is affected by sulphur deposition. The countries are assumed to be interested in maximizing the net benefits from pollution control as measured by the impacts on the values of forest growth net of the abatement costs. Cooperative and noncooperative solutions of the game are compared to assess the benefits of bilateral cooperation. Using empirical estimates of abatement costs, acidification dynamics and impacts on forest growth it is shown that cooperation is beneficial to Finland but not to the Soviet Union. Consequently, Finland has to offer monetary compensation to induce her neighbor to invest in environmental protection.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00338241
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  • 5
    Electronic Resource
    Electronic Resource
    Towards a sustainable and efficient use of manure in agriculture: The Dutch case (1991)
    Springer
    Environmental and resource economics 1 (1991), S. 313-332 
    Details
    ISSN: 1573-1502
    Keywords: Manure problem ; nutrient policy ; nutrient surplus ; regulatory levy ; sustainability ; agriculture ; intensive livestock sector ; acidification ; groundwater pollution ; eutrophication
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering , Economics
    Notes: Abstract Rapid increases in livestock production in the Netherlands have changed manure from a valuable input into a mere waste product. This is especially true for the southern and eastern parts of the country, where specialized pig and poultry farms have concentrated on sandy soils. As these farms generally own very little land, they largely depend on imported feedstuffs. As a consequence, manure is applied to the land in such large quantities that serious environmental problems have resulted: (1) eutrophication of surface water by phosphate emissions; (2) pollution of groundwater by nitrate emissions; and (3) acidification by ammonia emissions. In the last few years the Dutch government has developed a manure policy to counteract these effects. Our analysis of that policy has revealed at least three fundamental defects, which render the manure policy ineffective and inefficient. In this paper proposals are made to remove the defects in current manure policy. Much attention is paid to the problem of designing a mixture of policy instruments which is both effective as well as efficient in limiting the environmental problems caused by manure. It is shown that the use of financial incentives in regulation can substantially improve the efficiency of the manure policy. Finally, the main economic consequences of the proposed policy are examined for the public sector as well as for the agricultural sector.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00367923
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  • 6
    Electronic Resource
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    The Impact of Simulated Acid Rain on Soil Leachate and Xylem Chemistry in a Jack Pine (Pinus Banksiana Lamb.) Stand in Northern Ontario, Canada (1999)
    Springer
    Water, air & soil pollution 111 (1999), S. 89-108 
    Details
    ISSN: 1573-2932
    Keywords: acidification ; base cations ; dendrochemistry ; forest decline ; Jack pine (Pinus banksiana Lamb.)
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The impact of simulated acid rain on soil leachate and xylem chemistry in a young Jack pine (Pinus banksiana Lamb.) stand in the boreal forest of northern Ontario was evaluated. Permanent plots (5 × 2 m) were established in 1981 which were sprayed twice monthly with simulated acid rain, adjusted to pH 5.6, 4.0, 3.5, 3.0 or 2.5 with a 2:1 molar ratio of sulphuric (H2SO4) to nitric acid (HNO3) in addition to ambient rainfall. Sprays were applied between June and September for 5 yr. Unsprayed plots were also monitored. The pH of soil leachate collected between 1981–1985 was reduced significantly by the acid sprays and concentrations of sulphate (SO42-), nitrate (NO3-), calcium (Ca), magnesium (Mg), aluminium (Al), manganese (Mn), and zinc (Zn) increased in the A, B and C horizons. The soil recovered rapidly from the spray treatments, although residual effects were found in soil leachate samples collected during 1986–1987, particularly in the C horizon. Trees receiving spray acidified to pH 2.5 had higher concentrations of Ca, Mn, Cd and Rb in tree-rings formed between 1981–1985 compared to trees receiving spray acidified to pH 4.0 or to trees receiving ambient rainfall alone. Some of the changes in soil chemistry resulting from the application of acidic sprays are reflected in the chemistry of Jack pine tree rings and these chemical signals in tree rings may be used as indicators of soil acidification.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1005007518586
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  • 7
    Electronic Resource
    Electronic Resource
    Effects of Water Chemistry and Habitat on the Density of Young Brown Trout Salmo trutta in Acidic Streams (1999)
    Springer
    Water, air & soil pollution 112 (1999), S. 85-106 
    Details
    ISSN: 1573-2932
    Keywords: acidification ; Brown trout ; calcium ; density ; juveniles ; streams
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract We examined the relationship between young brown trout ( Salmo trutta) density in lake tributaries, and water chemistry and habitat variables. The study was carried out during the autumn in three acidic, softwater river systems in western and southwestern Norway; Gaular and Vikedal (1987–1993) and Bjerkreim (1988–1993). The streams had mean calcium concentrations of 0.35 mg L-1 (Gaular), 0.52 mg L-1 (Vikedal) and 0.84 mg L-1 (Bjerkreim). The concentration of inorganic Al was generally low, with mean values of 8.40 (Gaular), 22.22 (Vikedal) and 43.36 μg L-1 (Bjerkreim). In multiple regressions that involved different water chemistry variables, brown trout density correlated best with calcium concentration and with a combination of calcium and pH; the Ca2+:H+ ratio. In Vikedal and Gaular, calcium explained 51 and 57%, respectively, of the variability in brown trout densities. Althoug alkalinity exhibited the best correlation with brown trout density in Bjerkreim ( r2=0.33), it was similar to that of the model that included all major ions plus pH. The Ca2+:H+ ratio had a larger effect for variability in brown trout density in Gaular (r2=0.66) than calcium alone. In Vikedal and Bjerkreim, the Ca2+:H+ ratio also correlated with brown trout density, but considerably less than in Gaular. The predictive power of habitat variables was much lower than that of water chemistry; the single most important factors were altitude in Gaular (r2=0.22), mean water temperature in Vikedal (r2=0.11) and depth SD (index of heterogeneity) in Bjerkreim (r2=0.07). Models that included both habitat and water chemistry variables showed that the density of young brown trout was predicted primarily by calcium concentrations in Gaular (r2=0.75) and Vikedal (r2=0.54), as opposed to pH in Bjerkreim (r2=0.25). Habitat had low effect in all three river systems (r2=0.01–0.04). The final model explained 86, 68 and 32%, respectively, of the variability in brown trout density in the three catchments. Thus, water chemistry variables seem to be factors that limit the density of young brown trout in acidic softwater streams.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1005068404832
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  • 8
    Electronic Resource
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    Effects of acid anion additions (trifluoroacetate and bromide) on soil solution chemistry of a northern hardwood forest soil (1999)
    Springer
    Water, air & soil pollution 116 (1999), S. 479-499 
    Details
    ISSN: 1573-2932
    Keywords: acidification ; base cations ; bromide ; forest ecosystems ; mobile anion ; soil solution ; TFA ; trifluoroacetate
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Experimental plots within the Hubbard Brook Experimental Forest, NH, were treated with sodium trifluoroacetate (TFA) and lithium bromide (Br), to study the impact of TFA alone and in the presence of increased anion concentrations (e.g. acid deposition) on the soil solution chemistry of a northern hardwood forest soil. Trifluoroacetate is a major atmospheric degradation product of replacement compounds of chlorofluorocarbons (CFC) and Br is widely used as a hydrologic tracer. Calculated drainage losses via soil water flow were less than 60% of inputs, added during the summer, and TFA and Br were temporarily retained in the soil until fall. The initial indication of an acid input of the treatments (HTFA, HBr) in the Bs2 horizon, which reflects stream water chemistry as well, was an increase of base cations in the soil solution, decreasing the soil's acid neutralizing capacity. Thereafter, trifluoroacetate and Br concentrations peaked after the peak in base cations, synchronous with peaks in H+ and Al concentrations. Organic anions, nitrate and chloride played the major role in accompaning base cations out of the solum. Sulfate retention at soil adsorption sites was increased by the presence of TFA and Br, reducing its role as a mobile anion of base cations in this experiment. Relative retention of anions for the whole profile of this northern hardwood forest soil was estimated by correlation analyses and input-output balances in decreasing order on an equivalant basis: SO4 〉 TFA = Br ≥ Cl 〉 NO3 〉 organic anions. Recovery from acid additions were recorded within several weeks after the treatments were stopped. Evaluating the impact of added chemical compounds to soils must be considered within the context of linkages among element cycles and pools.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1005124305408
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  • 9
    Electronic Resource
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    Regional Patterns of Streamwater Acidity and Catchment Afforestation in Galloway, SW Scotland (2000)
    Springer
    Water, air & soil pollution 120 (2000), S. 47-70 
    Details
    ISSN: 1573-2932
    Keywords: acidification ; afforestation ; catchments ; geology
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract This paper investigates the regional relationships between highflow water chemistry and conifer forest cover in 95 streamsspread over an area of approximately 2000 km2 in Galloway,south-west Scotland, paying particular attention to the use ofdetailed catchment area data. Catchment forest data areextracted from a 30 m resolution tree height map derived fromsatellite imagery; geology data from a digital geology map; andaltitude and slope data from a 50 m resolution Digital TerrainModel (DTM). The results show that over the entire region pHlevels are lower with increasing catchment afforestation whilstaluminium concentrations are higher. Concentrations of sulphate arealso higher with increasing afforestation, which suggests thatconifers play a primary role in increasing the acidity levels ofstreams by exacerbating aerial acid deposition in the entireregion.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1005257410074
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  • 10
    Electronic Resource
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    Predicting Freshwater Critical Loads of Acidification at the Catchment Scale: An Empirical Model (1998)
    Springer
    Water, air & soil pollution 105 (1998), S. 31-41 
    Details
    ISSN: 1573-2932
    Keywords: acidification ; catchments ; freshwater critical loads ; predictive model ; Scotland ; statistical modeling
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Current applications of the critical loads concept are geared primarily toward targeting emission control strategies at a national and international level. Maps of critical loads for freshwaters have been produced in grid form based on water samples of representative sites within each grid square. However, the water chemistry data required to calculate freshwater critical loads are not always readily available at a national level and maps are therefore limited to catchments where such data exist. This paper describes the development of an approach that uses nationally available secondary data to predict freshwater critical loads for catchments lacking the appropriate water chemistry information. An empirical statistical model is calibrated using data from 78 catchments throughout Scotland. Water chemistry for each catchment has been determined. Each catchment is characterized according to a number of attributes. Redundancy analysis of these data shows clear relationships between catchment attributes and the critical load derived from the water chemistry. The key variables that explain most of the variation in critical load relate to soil, geology and land use within the catchment. Using these variables as predictors in a regression analysis, the critical load can be predicted across a broad gradient of sensitivity (R2 adj=0.81). The predictive power of the model was maintained when different combinations of explanatory variables were used. This accords the approach a degree of flexibility in that model parameterization can be geared toward availability of secondary data. There are limitations with the model as presently calibrated. However, the approach offers considerable scope for environmental managers to undertake national inventories of catchment sensitivity and specific assessments of individual catchments.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1005085021429
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  • 11
    Electronic Resource
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    Magic, Safe and Smart Model Applications at Integrated Monitoring Sites: Effects of Emission Reduction Scenarios (1998)
    Springer
    Water, air & soil pollution 105 (1998), S. 21-30 
    Details
    ISSN: 1573-2932
    Keywords: acidification ; emission ; MAGIC ; model ; nitrogen ; SAFE ; SMART ; sulfur
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Three well-known dynamic acidification models (MAGIC, SAFE, SMART) were applied to data sets from five Integrated Monitoring sites in Europe. The calibrated models were used in a policy-oriented framework to predict the long-term soil acidification of these background forest sites, given different scenarios of future deposition of S and N. Emphasis was put on deriving realistic site-specific scenarios for the model applications. The deposition was calculated with EMEP transfer matrices and official emissions for the target years 2000, 2005 and 2010. The alternatives for S deposition were current reduction plans and maximum feasible reductions. For N, the NOx and NHy depositions were frozen at the present level. For NOx, a reduction scenario of flat 30% reduction from present deposition also was utilized to demonstrate the possible effects of such a measure. The three models yielded generally consistent results. The ‘Best prediction’-scenario (including the effects of the second UN/ECE protocol for reductions of SO2 emissions and present level for NOx-emissions), resulted in many cases in a stabilization of soil acidification, although significant improvements were not always shown. With the exception of one site, the ‘Maximum Feasible Reductions’ scenario always resulted in significant improvements. Dynamic models are needed as a complement to steady-state techniques for estimating critical loads and assessing emission reduction policies, where adequate data are available.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1005099930089
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  • 12
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    The Prediction of Nitrate Leaching with the First-Order Acidity Balance (FAB) Model for Upland Catchment in Great Britain (1998)
    Springer
    Water, air & soil pollution 105 (1998), S. 205-215 
    Details
    ISSN: 1573-2932
    Keywords: acidification ; catchment ; first-order acidity model ; nitrate leaching ; predictive model
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The relative contribution of N deposition to the acidification of freshwaters in Great Britain has increased over the last few years as S deposition has fallen in line with reduced emissions. In certain high deposition areas of Great Britain, NO3 --based acidity can equal or exceed the contribution of SO4 2--based acidity in some upland waters. Here we apply the first-order acidity balance model (FAB) to predict the maximum N leaching from 13 study catchments at future steady state. Using mean water chemistry and catchment soils data, along with long-term default values for N sink processes, we predict NO3-N leaching at much higher rates than currently are being measured in surface waters, with a mean increase of 10.5 kg ha-1 yr-1. As a result, mean acid neutralizing capacity would decline to less than 0 meq L-1 at 4 sites. While there are uncertainties associated with model parameterization relating to the short-term storage of N within catchment soils and vegetation, model outputs do indicate much greater leaching of N at some time in the future as steady-state is achieved.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1005064416885
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  • 13
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    Recent Temporal Patterns in the Chemistry of Small, Acid-sensitive Lakes in Central Ontario, Canada (1998)
    Springer
    Water, air & soil pollution 105 (1998), S. 343-351 
    Details
    ISSN: 1573-2932
    Keywords: acidification ; decreasing SO2 emissions ; lake water chemistry ; Ontario ; sulfate deposition
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract We monitored the chemistry of 603 small water bodies in three acid-sensitive regions of central Ontario, Canada (Algoma n=235, Muskoka n=216, Sudbury n=152) between 1988-1996 to determine whether they have responded to recent SO2 emission reductions, and whether any chemical changes were related to lake characteristics. During the study, 27-56% of lakes declined in SO4 2- concentrations, 41-57% declined in base cation concentrations, but only 26-28% increased in pH or ANC (acidity status). Increases in pH were greatest in lakes with low ANC, but had weak relationships to lake color or volume. No consistent trends were observed for DOC, NO3 - or TP concentrations. Clearly, the long-term biological recovery of these sensitive aquatic ecosystems will depend on interactions among several environmental stressors, including acidification.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1005076719611
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  • 14
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    Effects of Atmospheric Sea-Salt Deposition on Soils and Freshwaters in Northeast Scotland (1998)
    Springer
    Water, air & soil pollution 105 (1998), S. 83-94 
    Details
    ISSN: 1573-2932
    Keywords: acidification ; river water chemistry ; sea salt deposition ; Scotland ; soil solution chemistry
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The majority of Scottish upland soils are particularly sensitive to acid deposition because of their low weathering rates. The compositions of the exchangeable base cations of such soils in the United Kingdom are dominated by sea salt inputs rather than by mineral weathering inputs of base cations. Catchments with low mineral weathering rates are also those particularly susceptible to freshwater acidification. Therefore, catchments exhibiting a high sea salt effect should also exhibit the most acid waters under base flow and storm flow conditions. A field evaluation study based on 61 catchments in NE Scotland has shown that this is indeed the case. River water pH under both base flow and high flow conditions is correlated stronhly with the relative contribution of Na+ to the sum of Ca2+, Mg2+ and Na+. From these results, an attempt is being made to produce a quantitative signature of weathering for the soils within the catchment upstream of the sampling point. Representative soil samples from the LFH, AE, B and C horizons and on 4 different parent materials have been obtained from the surrounding catchments to validate the above results for associated soil solutions. Sampling took place on upland moorland podzols under Calluna vulgaris. Tension lysimeters were used to sample the soil solutions so that their chemistry could be compared with that of the relevant river water.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1005090518219
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  • 15
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    Proton Budgets of Forest Ecosystems on Volcanogenous Regosols in Hokkaido, Northern Japan (1998)
    Springer
    Water, air & soil pollution 105 (1998), S. 63-72 
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    ISSN: 1573-2932
    Keywords: acidification ; atmospheric deposition ; forest canopy ; Japan ; leaching ; proton budgets
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The proton budgets of deciduous and coniferous forest ecosystems on volcanogenous regosols in Hokkaido, northern Japan, were studied by measuring the biogeochemical fluxes (atmospheric deposition, canopy leaching, vegetation uptake and leaching from soil) at each site during a three year period. The proton budgets were developed for individual compartments of the ecosystem: vegetation canopy, organic and mineral soil layers. At both sites, atmospheric S deposition was the dominant proton source in the vegetation canopy. In organic horizons, dissociation of weak acids (bicarbonate and/or organic acids) and vegetation uptake of base cations were the dominant proton sources, and the net mineralization of base cations was the dominant proton sink. Atmospheric acid deposition was almost neutralized in the forest canopy and organic horizon. At both sites, weathering and/or ion exchange of base cations and protonation of weak acids (mainly bicarbonate) were the dominant proton sinks in the mineral soil. In both organic and mineral soil, internal proton sources (mainly vegetation uptake of base cations and dissociation of weak acids) exceeded external proton sources, indicating that acid deposition was not the main driving force of soil acidification in the studied forest ecosystems.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1005086400473
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  • 16
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    Integrated Assessment of Soil Chemical Status. 2. Application of a Regionalized Model to 622 Forested Sites in Switzerland (1998)
    Springer
    Water, air & soil pollution 105 (1998), S. 11-20 
    Details
    ISSN: 1573-2932
    Keywords: acidification ; recovery ; forest soils ; regional dynamic modeling ; Switzerland
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A regionalized version of the dynamic, process-oriented, multi-layer soil chemistry model SAFE was applied to 622 forest sites in Switzerland to assess effects of acidifying atmospheric deposition on the soil chemistry between 1850 and 2050. Simulation indicates that the present day chemical status of Swiss soils is a result of the last 50 years of acid deposition. Indicative soil parameters such as soil solution pH, acid neutralizing capacity, total Al concentration, base cation to total A1 molar ratio and base saturation consistently deteriorate since the beginning of the 1950s, when acid loads start to increase. The simulated adverse evolution of soil chemistry persists until some time between 1975 and 2010, and apart from being site-dependent, the turning-point is also dependent on which parameter is considered at which soil depth.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1005055020945
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  • 17
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    Acidification of Freshwater Wetlands: Combined Effects of Non-Airborne Sulfur Pollution and Desiccation (1998)
    Springer
    Water, air & soil pollution 105 (1998), S. 95-106 
    Details
    ISSN: 1573-2932
    Keywords: sulfur ; sulfate ; desiccation ; acidification ; nutrients ; water quality ; pollution ; wetlands
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In recent decades, SO4 2- concentrations have increased in groundwater and surface water of freshwater wetlands. For many minerotrophic peatlands, S originating from SO4 2--polluted groundwater and surface water is a more significant source of SO4 2- than the actual atmospheric deposition of S compounds. Lowered groundwater tables in wetlands, as a result of either natural or anthropogenic desiccation, may cause acidification because of concomitant geochemical oxidation processes. The impact of the enhanced availability of reduced S compounds, due to preceding SO4 2- pollution, on these processes was tested in a mesocosm experiment, using soil cores including vegetation from a mesotrophic wet meadow. The soils had been maintained in waterlogged condition for seven months, using two environmentally relevant SO4 2- concentrations (2 and 4 mmol L-1). The groundwater table was reduced in two successive steps: 10 cm below soil surface, and complete desiccation. Control pretreated soils did not show a decrease in soil pH during desiccation, due to adequate buffering by bicarbonate. However, both SO4 2--pretreated groups showed a significant drop in pH (from 6.5 to 4.5) caused by additional sulfide oxidation, leading to high SO4 2- concentrations (10 and 16 mmol L-1, respectively). Cation exchange and acidification-related solubilization processes induced the mobiliztation of base cations and potentially phytotoxic metals like Al. Nutrient concentrations in soil moisture were influenced strongly by SO4 2- pretreatment, showing distinct patterns for P, N and K. Therefore, S polluted groundwater and surface water may severely increase the sensitivity of wetlands to desiccation. The results are discussed in relation to wetland management.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1005083526455
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  • 18
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    Modeling the Concentration of Aluminum in Surface Waters (1998)
    Springer
    Water, air & soil pollution 105 (1998), S. 643-659 
    Details
    ISSN: 1573-2932
    Keywords: acid deposition ; acidification ; aluminium ; modeling
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Although the increased mobilization of aluminum from soils to surface waters is widely recognized as one of the most important ecological effects of acidic deposition, lumped-parameter mathematical models of acidification response typically overestimate the change in Al concentration under changing deposition by a considerable margin. The assumption of equilibrium with gibbsite (Al(OH)3) in the MAGIC model and other models of acid-base chemistry is shown to be inconsistent with measured values for a large variety of lake and stream databases. A modified algorithm for predicting Al concentration, based on empirical relationships evident in field data, provided superior estimates of changes in Al concentration in three long-term monitoring data sets and under experimental conditions at two experimental watershed manipulation sites.
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    URL: http://dx.doi.org/10.1023/A:1004957426629
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    Assessment of the Exposure and Loads of Acidifying and Eutrophying Pollutants and Ozone, as well as their Harmful Influence on the Vitality of the Trees and the Speulder Forest Ecosystem as a Whole (1998)
    Springer
    Water, air & soil pollution 105 (1998), S. 539-571 
    Details
    ISSN: 1573-2932
    Keywords: acidification ; assessment ; eutrophication ; Speulder forest ; vitality
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Within the framework of the Dutch Priority Program on Acidification, 10 yr of research was conducted in a Douglas fir stand at Speulder forest. Research was conducted to establish the loads and levels of acidifying and eutrophying pollutants and ozone, to determine forest vitality characteristics and follow growth parameters and nutrient status in time and to determine the effects of reduction of loads and levels by manipulation experiments. Results indicate that during the last 20 yr critical levels for air pollutants have hardly been exceeded except for ozone, which slightly affected assimilation. Elevated nitrogen deposition has caused several adverse effects including (i) inhibited mycorrhizal development, leading to a decreased base cation and phosphorus uptake; (ii) elevated foliage/root (fine and coarse) ratios, making the forest more sensitive to drought and windthrow; (iii) elevated nitrogen and arginine concentrations in the foliage, associated with relative base cation and phosphorus deficiency, and (iv) elevated nitrate leaching polluting the groundwater. High inputs of acidity have caused elevated ratios of Al to base cations, affecting fine root (uptake) and depletion of the readily available Al pool, thus affecting the long-term sustainability. Despite these effects, forest vitality, in terms of defoliation/discoloration, is reasonable and forest growth even increased in response to nitrogen. The exceedances of critical loads for nitrogen and acidity, however, implies a (large) risk for the long-term sustainability of the Speulder forest.
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    URL: http://dx.doi.org/10.1023/A:1004961610700
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    Trends in the Chemistry of Acidified Bohemian Lakes from 1984 to 1995: I. Major Solutes (1998)
    Springer
    Water, air & soil pollution 108 (1998), S. 107-127 
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    ISSN: 1573-2932
    Keywords: acid deposition ; acidification ; base cations ; Bohemian lakes ; chloride ; Czech Republic ; lake water ; nitrate ; pH ; reversibility ; sulphate ; temporal changes
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Temporal changes in major solute concentrations in six Czech Republic lakes were monitored during the period 1984–1995. Four chronically-acidic lakes had decreasing concentrations of strong-acid anions (CSA = SO4 2- + NO3 - + Cl-), at rates of 3.0 to 9.0 μeq L-1 yr-1. Decreases in SO4 2-, NO3 -, and Cl- (at rates up to 5.1 μeq L-1 yr-1, 3.2 μeq L-1 yr-1, and 0.6 μeq L-1 yr-1, respectively) occurred. The response to the decrease in deposition of S was rapid and annual decline of SO4 2- in lake water was directly proportional to SO4 2- concentrations in the acidified lakes. Changes in NO3 - concentrations were modified by biological consumption within the lakes. The decline in CSA was accompanied in the four most acidic lakes by decreases in AlT, increases in pH at rates of 0.011 to 0.016 pH yr- 1, and decreases of Ca2+ and Mg2+ (but not Na+) in three lakes. The acid neutralizing capacity (ANC) increased significantly in all six lakes. Increases in base cation concentrations (CB = Ca2+ + Na+ + Mg2+ + K+) were the principal contributing factor to ANC increases in the two lakes with positive ANC, whereas decrease in CSA was the major factor in ANC increases in the four chronically-acidic lakes. The continued chemical recovery of these lakes depends on the uncertain trends in N deposition, the cycling of N in the lakes and their catchments, and the magnitude of the future decrease in S deposition.
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    URL: http://dx.doi.org/10.1023/A:1005064829981
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    Trends in Water Chemistry of Acidified Bohemian Lakes from 1984 to 1995: II. Trace Elements and Aluminum (1998)
    Springer
    Water, air & soil pollution 108 (1998), S. 425-443 
    Details
    ISSN: 1573-2932
    Keywords: acidic deposition ; acidification ; aluminum ; atmosphericdeposition ; Bohemia ; Czech Republic ; fluoride ; lake ; trace metal ; trace element ; reversibility ; restoration
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The concentrations of Al, Be, Cd, Cu, F, Fe, Mn, Pb, and Zn were monitored in five glacial lakes and one man-made lake in the southwestern part of the Czech Republic. The lakes had median pHs of 4.4 to 6.5 during 1984 to 1995. Decreases in the concentrations of Mn and Pb occurred in five acidified lakes. The concentrations of AlT, Be, Cd, and F decreased in the four chronically acidified lakes, Zn decreased in two lakes. Concentrations of Cu and Fe remained unchanged. The decreases in Be, Mn, and Zn concentrations were proportional to the decrease in CSA (CSA = SO4 2- + NO3 -+ Cl-); decreases in AlT, Cd, and Pb concentrations were proportionately higher, while F was lower. The greater decrease in the Pb concentrations (61 to 79%, at a rate up to 0.15 μg L-1yr-1) was caused by pronounced decreases in deposition of Pb derived from mobile sources. The decrease of AlT concentrations was dominated by a decrease in Al3+, whose concentration decreased by 51 to 86%. The concentrations of complexes Al(OH)2+, Al(OH)2 +, AlF2+, and AlH3SiO4 2+ also decreased. The decrease in the concentrations of inorganic forms of Al (Ali) compensated 65% of the decrease in CSA. The Cd concentrations were highly variable in the years 1986 to 1988 because of variable amounts of accumulation on particles.
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    URL: http://dx.doi.org/10.1023/A:1005007627334
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    The Impact of Simulated Acid Rain and Fertilizer Application on a Mature Sugar Maple (Acer Saccharum Marsh.) Forstt in Central Ontario Canada (1999)
    Springer
    Water, air & soil pollution 109 (1999), S. 17-39 
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    ISSN: 1573-2932
    Keywords: acidification ; fertilizer ; forest decline ; sugar maple
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The effects of two year's addition of simulated acid precipitation, with and without added fertilizer, on mycorrhizae, litter decomposition and soil and tree chemistry in a sugar maple (Acer saccharum Marsh.) dominated forest were investigated. The forest floor beneath mature sugar maple trees was irrigated at monthly intervals between May and September with local lake water acidified to pH 3, pH 4 or untreated lakewater of pH 4.9. In addition, a commercial organic slow-release fertilizer (Maple Gro) was added to the soil prior to irrigation with pH 3 spray. Trees to which no experimental spray was applied were also included as controls. Eight trees were used for each of the five treatments. Application of the acid spray alone did not acidify surface soil nor cause visible symptoms of decline in trees. The pH of the soil solution and soil leachate was increased by addition of acidified lakewater. An increase in the concentration of sulphate (SO4 2-), calcium (Ca), and magnesium (Mg) in soil leachate was only recorded in plots irrigated with water acidified to pH 3 + Maple Gro. The initial rate of litter decomposition tended to be higher following application of the acid sprays, although mycorrhizal infection of sugar maple roots was reduced in the pH 3 and pH 4 treatments. Concentrations of zinc (Zn), chromium (Cr) and nickel (Ni) were highest in wood formed during the period irrigated with water acidified to pH 3. Foliar nitrogen (N) concentrations tended to be higher in all irrigated treatments, although there were no differences between treatment in any of the other nutrients measured in foliage after two years of treatment. It is concluded that the application of simulated acid rain under field conditions results in a complex interaction of events which are not reproduced in pot trials and must be fully understood before the impact of acid rain on sugar maple forests can be evaluated.
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    URL: http://dx.doi.org/10.1023/A:1005077230678
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    Atmospheric Pollution in a Tropical Rain Forest: Effects of Deposition Upon Biosphere and Hydrosphere I. Concentrations of Chemicals (2000)
    Springer
    Water, air & soil pollution 121 (2000), S. 59-78 
    Details
    ISSN: 1573-2932
    Keywords: acidification ; air pollution ; Brazil ; Cubatão ; precipitation ; Serra do Mar ; tropical rain forest
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The effects of atmospheric deposition upon elementcycling and turnover in three rain forest ecosystems ofthe Serra do Mar, a mountain range along the atlanticcoast of Brazil, have been investigated as part of aninterdisciplinary German-Brazilian research project ondispersion, transformation and deposition of airpollutants in the vicinity the industrial complex ofCubatão, State of São Paulo. The projectincluded on-site measurements from 1991 to 1995, fieldexperiments and mathematical modelling with the goalof providing damage evaluation and risk assessment,and elucidating damage mechanisms with respect tosoils and vegetation. The role of the `Soil Module'sub-project reported here was to assess atmosphericdeposition and fluxes with precipitation and soilwater, and to investigate possible soil changesinduced by atmospheric deposition as well asbiological effects of pollutants via the soil path.Part I of this paper deals with concentrations ofchemicals in precipitation, soil water, surface waterand in litter. Part II will cover fluxes of chemicalsand element budgets.Three sites were chosen which differed significantlywith respect to pollution impact. Annual averages ofionic concentrations in precipitation found in openfield and below the tree canopy amounted to 5 and10 mg L-1, respectively, for sulfate-S, 0.4 and0.7 mg L-1 for nitrate, 0.65 and 1.1 mg L-1 for fluoride,1.8 and 2.6 mg L-1 for ammonium-N, 0.76 and 2.3 mg L-1for Mg, and 3.5 and 7.5 mg L-1 for Ca at the mostpolluted site. The relatively `clean' reference siteattained 1/3 to 1/9 of these averages, thus clearlyreflecting the difference in air pollution load.Chemical composition in the liquid phase is completelychanged when precipitation infiltrates the soilprofile. Nitrate concentration increases by the factor5 to 20. A clear increase is also found for sulfateand chloride. Concentration changes during ecosystempassage of seepage are interpreted in relation tochemical reactions taking place in differentcompartments. They are characterized by an almostcomplete retention of ammonium and some retention ofsulfate in the upper soil layers, and at the mostpolluted site by mobilization of Al from soil mineralsand very high leaching of nitrate as a consequence ofnitirification of organic matter.
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    URL: http://dx.doi.org/10.1023/A:1005249615589
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    Condition factor and whole-body sodium concentrations in a freshwater fish: Evidence for acidification stress and possible ionoregulatory over-compensation (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 377-382 
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    ISSN: 1573-2932
    Keywords: Rhinichthys atratulus ; condition factor ; whole-body sodium ; Shenandoah National Park ; acidification
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Condition factor, “K”, was measured for 1202 blacknose dace (Rhinichthys atratulus) from three streams in Shenandoah National Park (USA) of different acid neutralizing capacities (ANCs). “K” is a ratio of weight standardized to length; it is an indication of the health of the individuals in a population. R. atratulus condition factor in the low-ANC stream was found to be significantly lower (11%) than that of dace measured for fish from the intermediate- and high-ANC streams. This difference, according to the results of related investigations, is likely to be biologically significant. Whole-body sodium concentrations were measured as an additional test of sublethal stress in these streams. During summer base flow conditions, mean whole-body sodium concentrations of adult R. atratulus maintained in cages were found to be highest in the low-ANC stream and lowest in the high-ANC stream. The lower condition factor of dace in the low-ANC stream may be related to whole-body sodium concentration and ion regulation. Ion regulation in the low-ANC stream may be more metabolically costly because of chronic sublethal pH stress. R. atratulus may maintain high body Na+ concentrations in low ANC- and ionic strength waters in order to provide a buffer against large episodic pH depressions. The metabolic cost of this ionoregulatory over-compensation may necessitate the diversion of energy from somatic growth and explain the poorer condition of fish from such waters.
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    URL: http://dx.doi.org/10.1007/BF00476858
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    Losses and recoveries of fish populations in acidified lakes of southern Finland in the last decade (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 315-320 
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    ISSN: 1573-2932
    Keywords: Fish populations ; perch ; roach ; growth ; reproduction ; water chemistry ; acidification ; recover
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Acid-induced fish damage in small lakes in southern Finland was studied in a fish status survey of eighty lakes from 1985–1987. Later, twenty of these lakes were selected for further monitoring. A sampling of these lakes from 1988–1989 showed that the decrease in some perch (Perca fluviatilis L.) and roach (Rutilus rutilus L.) populations still continued. The results from the same lakes in 1992 showed that successful reproduction had taken place with many of the perch populations that had been close to extinction in 1985. In contrast, no signs of recovery in the roach populations were detected. The explanation for the appearance of new cohorts of perch could have been the decrease in acid deposition but the exceptional hydrological conditions of winters in the early 1990s may also have affected them. The different responses of the perch and roach populations were interpreted as a consequence of the different sensitivity of these two species to acidification. Even a slight improvement in the water quality has resulted in the appearance of strong new year-classes of perch, but not of roach. Therefore, more improvement in water quality is needed until a sensitive species like roach can reproduce again.
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    URL: http://dx.doi.org/10.1007/BF00476848
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    Long-term trends in stream chemistry and biology in North-East Scotland: Evidence for recovery (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 689-694 
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    ISSN: 1573-2932
    Keywords: reversibility ; recovery ; long-term trends ; hydrochemistry ; acidification ; macroinvertebrates ; Scotland
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Since 1983 stream chemistry and macroinvertebrate ecology were monitored in ten streams draining the eastern Cairngorms. All streams have exhibited a decline in sulphate concentrations in response to reduced acid deposition; in the more acidic systems this has been reflected by a parallel increase in acid neutralizing capacity (ANC). In some streams this coincides with an increase in the abundance of acid-sensitive mayflies which may provide evidence for biological recovery. In the most chronically acidified systems no increased abundance has been observed despite significant increases in ANC. This suggests that further reductions in deposition and sufficient time for a reversal of soil acidification is required before any biotic recovery occurs.
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    URL: http://dx.doi.org/10.1007/BF00476909
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    Responses of phyto- and zooplankton to liming in a small acidified humic lake (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 943-948 
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    ISSN: 1573-2932
    Keywords: acidification ; liming ; phytoplankton ; zooplankton ; humic lake
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Liming resulted in an immediate and transitory decrease of plankton biomass and phytoplankton primary production in the limed part of an acidified humic lake. In the longer term liming has changed species composition and dominance of phyto- and zooplankton. Due to increased transparency and improved oxygen conditions plankton biomass peaked deeper in the water column after liming. During the three years post-liming period phyto- and zooplankton communities have changed less than reported in several other studies. This is largely because liming was carried out well before the collapse of perch population, which has controlled zooplankton both in the pre- and post-treatment period.
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    URL: http://dx.doi.org/10.1007/BF00476951
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    Assessment of the economic costs of damage caused by air-pollution (1995)
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    Water, air & soil pollution 85 (1995), S. 2583-2588 
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    ISSN: 1573-2932
    Keywords: Air pollution ; external costs ; economic instruments ; health ; building materials ; acidification
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Cost-benefit analysis is one of the fundamental tools for the development of economic instruments for pollution control. The costs of various abatement measures are reasonably well characterised. However, assessment of the economic costs of pollutant impacts is less well developed. This paper reports on two studies carried out for DGXII of the European Commission, the ExternE-Project and the Green Accounting Research Project. Both studies have been performed by international, multi-disciplinary research teams. Analysis of the effects of emissions of PM10, SO2, NOx and VOCs (as ozone precursors) has included assessment of human health, materials, crops and other terrestrial ecosystems, and freshwater fisheries. The analysis follows the ‘impact pathway’ approach, linking dose-response functions, valuation data and other models. It differs significantly to earlier ‘top-down’ approaches that made only very limited use of the wealth of scientific data available. Most success has been achieved in analysis of impacts on human health, building materials and crops. Significant uncertainties exist for these receptors, though these have been identified and are now being addressed. Assessment of impacts on other receptors, perhaps most notably forests, is more limited. The methodology is particularly applicable for analysis of impacts on receptors for which the critical loads approach is not appropriate.
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    URL: http://dx.doi.org/10.1007/BF01186223
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    Testing, improvement, and confirmation of a watershed model of acid-base chemistry (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2607-2612 
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    ISSN: 1573-2932
    Keywords: acidification ; model testing ; modeling ; acid deposition
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Strategies to control the emission of atmospheric pollutants such as sulfur and nitrogen, are generally based in large part on projections using models that simulate the influence of sulfur and/or nitrogen deposition on the acid-base chemistry of surface waters. One of the principal models used throughout Europe and North America for such assessment is the Model of Acidification of Groundwater in Catchments (MAGIC). All watershed models are simplified representations of reality, and as such require careful testing to establish their veracity prior to use for making policy projections. This is particularly true where the use of these model projections has the potential for serious environmental or economic consequences. During the past five years, we have tested the MAGIC model in a large variety of settings and under quite varying environmental conditions. This work has included comparing model hindcast simulations with diatom-inferences of historical acidification, sensitivity analyses to examine the response of the model to alternative assumptions and formulations, and detailed testing of model forecasts by comparing simulated chemistry with the results of catchment-scale and plot-scale experimental acidification and deacidification. Our analyses have elucidated a number of potentially-important deficiencies in model structure and method of application. These have resulted in changes to the model and its calibration procedures. Our work has included in-depth evaluation of issues related to regional aggregation of soils data, background sulfur deposition, natural organic acidity, and aluminum mobilization. The result has been an improved and more thoroughly-tested version of MAGIC. The process we have followed to improve and confirm the MAGIC model has been iterative and time consuming. It required the availability of large volumes of data from experimental manipulation and paleolimnological studies. We believe that such model testing and confirmation efforts should be a critical prerequisite for regional or national assessment activities that are based largely on the results of environmental models.
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    The difference in brown trout (Salmo Trutta L.) blood composition from acidic and limed sites of two rivers in Western Norway (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 203-210 
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    ISSN: 1573-2932
    Keywords: acidification ; blood ; environment ; fish
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Certain blood morphology parameters: red blood cell (RBC) sizes; percentage of polymorphonuclear leukocytes and ratio polychromatocyte/RBC in Brown trout (Salmo trutta L.) from acidified water (mean pH value 4.94) and limed water (mean pH value 5.66) were investigated. The sizes of RBC long axises were significantly larger in fish from acidic environment than from limed condition (14.37 and 12.96μm respectively). The percentage of polymorphonuclear cells (7.86 and 3.32) and polychromatocyte/RBC ratio (0.079 and 0.019) were also significantly larger in fish from the acidified environment. Blood morphology parameters are concluded to be usefull for testing and detection of long-term acidic stress in fish in nature.
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    URL: http://dx.doi.org/10.1007/BF02407205
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    Studies of Soils, Soil Water and Stream Water at a Small Catchment near Guiyang, China (1998)
    Springer
    Water, air & soil pollution 101 (1998), S. 137-162 
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    ISSN: 1573-2932
    Keywords: acidification ; acid rain ; catchment ; China ; geochemistry ; soil ; soil water
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Acid deposition is considered to be a major environmental problem in China, but information about effects on soils and waters is scarce. To contribute to increased knowledge about the problem a small catchment (about 7 ha) in the outskirts of Guiyang, the provincial capital of Guizhou in south-western China, was instrumented for collection of precipitation, throughfall, soil water and stream water. In addition soil samples have been collected and analyzed for key properties. Median pH in the precipitation is 4.40 (quartiles: 4.19 and 4.77) and the median sulfate concentration 228 µeq/L (quartiles: 147 and 334 µeq/L). The dry deposition of both SO2 and alkaline dust is considerable. The sum of wet deposition of sulfate and dry deposition of SO2 has been estimated to about 8.5 gSm-2yr-1. The total S-deposition may be somewhat higher due to dry deposition of sulfate and occult deposition. In soil water, SO4 2- is the major anion, generally ranging from 300 to 2500 µeq/L in the different plots. Calcium is an important cation, but there is also a considerable contribution of aluminum from the soil. In some of the plots the concentrations of inorganic monomeric aluminum (Ali) are typically between 200 and 400 µm. Potential harmful levels of aluminum and/or high Ali/(Ca2+ + Mg2+) molar ratios occur in the catchment, but damages to vegetation have not yet been reported. In most cases exchangeable aluminum accounts for between 75 and 95% of the total effective cation exchange capacity (CECE) in the mineral soils. The aluminum chemistry cannot easily be explained by conventional models as the Gaines-Thomas ion-exchange equation or equilibrium with an Al(OH)3 mineral phase. The stream water is generally less acidic and has considerably lower concentrations of aluminum than the soil water, even though quite acid events have been observed (pH 〈 4.4). The median pH values are 4.9 and 5.0 in the two first order streams and 6.3 in the dam at the lower boarder of the catchment.
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    Atmospheric Pollution in a Tropical Rain Forest: Effects of Deposition Upon Biosphere and Hydrosphere II. Fluxes of Chemicals and Element Budgets (2000)
    Springer
    Water, air & soil pollution 121 (2000), S. 79-92 
    Details
    ISSN: 1573-2932
    Keywords: acidification ; air pollution ; atmospheric deposition ; Brazil ; Cubatão ; element fluxes ; element budgets ; Serra do Mar ; tropical rain forest
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Three rain forest ecosystems in the Serra do Mar, theatlantic coastal mountain range of Brazil, have beeninvestigated in the frame of an interdisciplinaryGerman-Brazilian research project on dispersion,transformation and deposition of air pollutants in andaround the industrial area of Cubatão. Part I ofthis paper gives a description of the overall goals ofthe project, the area of investigation, and thematerials and methods used. It reports on the resultsof the field measurements conducted from 1991 to 1995,covering concentrations of chemicals in precipitation,soil water, surface water and litter fluxes. In thepresent paper, part II, the element fluxes arepresented with calculated concentrations in thetransport media (precipitation, seepage water,litterfall) and their respective flow rates. Elementbudgets for the ecosystem and for the soil compartmentare interpreted with respect to turnover of chemicals,including nutrients, in forest vegetation, and toprocesses of soil acidification.The forests under investigation are characterized bya very high input from the atmosphere. Between 100 and200 kg S ha-1 are annually carried into soil byprecipitation in the form of sulfate, 20 to 70 kg ofnitrogen mainly in the form of ammonium, 3 to 24 kg offluoride. Input of ammonium and organic bound nitrogenis followed by nitrification in the top soil. At themost polluted site, nitrate output with seepageamounts to 300 kg N ha-1 yr-1, sulfate output tomore than 400 kg S. Soil acidification associated withturnover of sulfur and nitrogen is followed by therelease of aluminum from soil minerals, and leachingof ionic forms of Al (up to 280 kg Al ha-1annually). Transfer of aluminum ions to groundwaterand surface water can have serious ecologicaleffects. Alkalinity is consumed, and the water issubject to acidification.
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    URL: http://dx.doi.org/10.1023/A:1005201732427
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    Reconstructing Historic Atmospheric Deposition and Nutrient Uptake from Present Day Values Using MAKEDEP (1998)
    Springer
    Water, air & soil pollution 104 (1998), S. 269-283 
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    ISSN: 1573-2932
    Keywords: acidification ; air pollution ; modelling
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A model, MAKEDEP, was developed for reconstructing historic atmospheric deposition and nutrient uptake for forests using present day values. Deposition is reconstructed by separation of wet deposition and throughfall into five different categories. Dry deposition is assumed to depend linearly on needle biomass. Non-marine deposition is scaled using general European emission and deposition trends for sulphur, nitrate and ammonia. Historic nutrient uptake is reconstructed using current biomass and nutrient content, a logistic forest growth curve and information on historic land use.
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    URL: http://dx.doi.org/10.1023/A:1004958027188
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    Macroinvertebrate-Inferred Stream-Water Acidity in North Eastern Finland Along a Sulphur Deposition Gradient (1998)
    Springer
    Water, air & soil pollution 104 (1998), S. 223-236 
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    ISSN: 1573-2932
    Keywords: acidification ; bioindicators ; macroinvertebrates ; streams
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Recently developed weighted averaging (WA) models and widely used tolerance-limit approaches for inferring stream minimum pH from macroinvertebrates were tested in northeastern Finnish Lapland. Surface waters there are threatened by large sulphur emissions in the Russian Kola Peninsula. The modelled sulphur deposition increases from west to east approximately parallel to longitude. The effect of deposition on stream minimum pH was assessed by relating the macroinvertebrate-inferred stream minimum pH to longitude. In a test set of 17 streams, the minimum pH inferred from pooled invertebrate samples of three seasons by WA models showed a strong correlation (r = 0.67–0.72) with the minimum pH (range 6.3–7.1) observed during the spring snow-melt period. The relationship was slightly weaker (r = 0.59–0.69) using autumn samples only. The tolerance-limit approaches assigned the streams into the correct acidity class, but the inferred pH was not related to the observed minimum pH. This further demonstrates the superiority of the WA approach, especially in detecting early signs of acidification. The minimum pH inferred by WA from autumn assemblages of 37 streams along the deposition gradient showed a significant negative correlation with longitude, suggesting that the emissions from the Kola region contribute to low pH events in streams of northeastern Finnish Lapland. The results demonstrate the potential of bioassessment and monitoring using invertebrates in detecting impacts and changes that could remain unnoticed by conventional water quality-analyses.
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    URL: http://dx.doi.org/10.1023/A:1004974123457
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    Al:Pe projects: Water chemistry and critical loads (1995)
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    Water, air & soil pollution 85 (1995), S. 493-498 
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    ISSN: 1573-2932
    Keywords: remote lakes ; water chemistry ; critical load ; acidification
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Water chemistry data on which all the investigations in the AL:PE 1 (Acidification of Mountain Lakes: Palaeolimnology and Ecology) and AL:PE 2 (Remote Mountain Lakes as Indicators of Air Pollution and Climate Change) projects are based, are available for 28 lakes in U.K. (Scotland), Italy, Norway and France (AL:PE 1) and in Svalbard (Norway), Ireland, Austria, Spain, Portugal, Poland, Slovakia, Slovenia and Russia (AL:PE 2). The results show high sulphate concentrations in some mountain lakes in all the countries. Nitrate and sulphate concentrations have different distribution patterns among the sites. A gradient in acidification from north (Norway) to central Europe (via U.K. to Italy) is identified for the AL:PE lakes by means of multivariate data analysis. Critical loads and their exceedance are calculated, where sufficient information is available, both according to the leaching of S, and of S plus N from the catchment. The pattern of critical load exceedance demonstrates an increasing importance of nitrate from Norway via U.K. to Italy. Leaching of N was of considerable importance to the acidification of lakes in the Italian Alps. The projects receive financial support from the European Union.
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    URL: http://dx.doi.org/10.1007/BF00476877
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    Acid stress and extinction of a spring-spawning fish population (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 383-388 
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    ISSN: 1573-2932
    Keywords: acidification ; fish population extinctions ; physiological stress
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Investigation of Heeney Lake, 21.7 ha, revealed a small population of white sucker, Catostomus commersoni. Only four age-classes were represented in this normally abundant and long-lived species. By 1984 only one new age-class had been recruited into the population. As these fish spawned in the outlet stream in early spring, the potential toxicity of these waters was assessed at two snow-melt events. Rainbow trout, Oncorhynchus mykiss, of hatchery origin were held in the outlet stream as pH declined from 6.5 to 4.7 during a snow melt, late February. Trout showed a loss of 19% in plasma Na and 24% in Cl concurrent with gill Al concentration increasing from 10 to 250 μg'g−1 dry wt. At the mid-April snow melt, pH fell to 4.1, and rainbow trout held in the outlet showed a decline in plasma sodium of 42% and gill Al increased from 10 to 415 μg'g−1 dry wt. Control rainbow trout held in Harp L. at pH 6.3 showed no significant change in plasma and muscle ion concentrations, or in gill Al concentration. White sucker from nearby waters were held in Heeney Lake outlet, late April, and muscle Na and Cl declined significantly as gill Al concentration increased from 11 to 50 μg'g−1 dry wt during 48 hr exposure. White sucker hekl in Heeney L. outlet, mid-May, showed no significant change in plasma ions. No white sucker have been captured in Heeney L. since 1984 and the population is presumed to be extinct. Acid deposition has declined in recent years but lake and stream pH have not recovered and fish populations may still decline or disappear.
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    Have emission reductions led to improvements in water quality at Loch Dee in Galloway? (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 695-700 
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    ISSN: 1573-2932
    Keywords: monitoring ; acidification ; coniferous afforestation ; rainfall chemistry ; water chemistry
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A comprehensive study began in 1980, at the Loch Dee catchment (south west Scotland), to study the effects of acidification and coniferous afforestation on streamwater ecology. When the project started, acid emissions were high but have since declined and stabilised. Average rainfall pH did not change significantly during the study period but total sulphate concentrations declined by 30%. The Loch Dee basin has three main subcatchments. Almost 70% of the Green Burn subcatchment was planted with Sitka spruce, between 1973 and 1975 and canopy closure has occurred at lower altitudes. Comparison of the water chemistry of the Green Burn and the Dargall Lane was done with cusum plots. The pH in the Green Burn has fallen relative to the Dargall Lane, whereas total and non-marine sulphate concentrations have remained unchanged over the last 10 years.
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    Soil solution chemistry and element budgets of three Scots pine ecosystems along a deposition gradient in north-eastern Germany (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1197-1202 
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    ISSN: 1573-2932
    Keywords: Scots pine ; Pinus sylvestris ; deposition ; element budget ; soil solution ; soil chemistry ; alkaline dust ; pH ; acidification ; sulfur release
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Since 1993 we are studying three Scots pine ecosystems along a deposition gradient in north-eastern Germany (formerly GDR). Dramatic reductions of pollutant emissions are reported for the period since 1989/90. S-deposition is high at the sites Roesa and Taura (25 kg S ha−1yr−1) compared to Neuglobsow. Inputs of basic cations, especially Ca, by alkaline dust immissions decrease in the order Roesa 〉 Taura 〉 Neuglobsow. The soil solution data show high concentrations of Ca and SO4 at Roesa decreasing drastically along the deposition gradient. The elevated pH values reflect the impact of alkaline dust deposition particularly in the organic surface layer at Roesa. The site Taura received less base cation deposition and is marked by the lowest pH values throughout the soil profile combined with increased Al concentrations in the solution of the mineral soil. Thus, the composition of the soil solutions clearly reflects the different deposition regimes of the past. The element budgets show that large amounts of base cations, sulfur, and, at Taura, also aluminum are actually released from the soils that were previously stored.
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    Options for liming rivers to ameliorate acidity — A UK perspective (1995)
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    Water, air & soil pollution 85 (1995), S. 1009-1014 
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    ISSN: 1573-2932
    Keywords: Liming ; acidification ; costs ; benefits ; Salmo salar ; Salmo trutta
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The options for large scale liming of river systems are reviewed with particular reference to the River Tywi in Wales, a major salmonid river with a reservoir in the upper catchment. For hydrological source area liming the cost of lime transport is high due to remoteness and inaccessibility. The concern of potential damage to wetland mires of conservation value is considered. Re-treatment intervals are expected to be 5–10 years, but results from sub-catchment experiments indicate that treatment longevity and the pattern of ecological recovery are uncertain. Flow-related dosing systems for rivers avoid impacts on wetlands but would treat only the main river. Reliability may be problematical though the reservoir provides a margin of safety against system failure. Reservoirs can be limed to treat the main river outflow. This avoids the problems of power supply. For the River Tywi, the financial costs of both direct treatment methods are lower than for catchment liming and comparable with estimates of the economic benefit to the fishery. The system currently operated on the Tywi is reservoir treatment. Results from the first 3 years demonstrate colonization of the main river by acid intolerant invertebrate taxa and clear increases in populations of juvenile Atlantic salmon, Salmo salar L. and sea/brown trout. Salmo trutta L.
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    Silvicultural use of wood ashes — Effects on the nutrient and heavy metal balance in a pine (Pinus sylvestris, L) forest soil (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1039-1044 
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    ISSN: 1573-2932
    Keywords: pine ; recycling ; amelioration ; vitalization ; acidification
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In a sustainable forestry recirculation of nutrients through the application of ashes from forest residues can be an essential way to guarantee healthy and vital forests. Wood ashes can also be regarded as a measure against soil acidification. Wood ashes were applied at various rates to the soil in a 35 years old pine (Pinus sylvestris, L) stand at Ringamåla in Blekinge, South Sweden. The experiments started in 1984. The different treatments gave a clear effect on soil chemistry with decreased acidity and aluminum ion concentrations. The base saturation increased in both mor and upper mineral soil layers. Generally no significant increases were found in soil concentrations of heavy metals, except for Cu which increased significantly in the mor layer. Also the extractable Mn concentration increased, in spite of the increased pH in the soil after application of ashes. In order to achieve a biological circulation of nutrients through ash application without polluting the environment, it is of ultimate importance that the wood chips used in power plants and other furnaces have a low concentration of heavy metals and other pollutants.
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    Methods for treating acid groundwater results and evaluation of long-term tests (1995)
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    Water, air & soil pollution 85 (1995), S. 1849-1854 
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    ISSN: 1573-2932
    Keywords: acidification ; groundwater ; countermeasures ; liming ; filters
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Acid groundwater can corrode plumbing systems and solubilize metals in the soil or in the plumbing systems. Since the soluble forms of some metals are toxic, concerns regarding the effects of groundwater acidification on human health have been raised. A number of new methods for treating acidified groundwater have been developed and tested during the last decade. In addition conventional filter devices have been tested and evaluated. Seven methods of in situ alkalization, i.e. treatment of the soil around the well with an alkalizer, have been tested for 1–8 years. These methods involve the application of limestone or slaked lime in the recharge area of the well or in/near the well. Target values set for the tests were: pH〉6,5 and alkalinity 〉60 mg/l. Almost all of these methods have led to improvements in water quality, but in some cases target values were not reached. Most of the treatments have resulted in significant reductions in iron and aluminium contents in drinking water. Eight types of more conventional devices for processing acidified well water have been tested for a couple of years. These de-acidification filters are installed indoors or in some cases inside the well. The majority of them performed well, providing acceptable values of pH and alkalinity under normal water flows. However,after periods of more intense water flushing, some of the filters showed a decreased capacity to neutralize the water. Inexpensive types of equipment, e.g. some of the filters placed inside the well, performed just as well as the more expensive types.
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    A palaeolimnological assessment of the impact of acid deposition on surface waters in North-West Scotland, a region of high sea-salt inputs (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2425-2430 
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    ISSN: 1573-2932
    Keywords: Surface waters ; north-west Scotland ; acidification ; critical loads ; sea-salts ; palaeolimnology ; diatoms
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Recent critical loads assessments suggest that sensitive surface waters in the north-west of Scotland have acidified, whereas earlier surveys indicate little chemical or biological evidence of acidification. It has been suggested that regionally high sea-salt inputs are affecting either critical loads calculations or the susceptibility of surface waters to acidification. We use palaeolimnological techniques to test the hypothesis that the critical load exceedances in north-west Scotland are real. Pre-industrial and present day loch-water pH are inferred from diatom assemblages in sediment cores from 21 lochs in order to estimate recent pH change. The results indicate consistent post-1800 declines in loch-water pH, although the magnitude of this decline is small (〈0.4 pH unit) and in most cases within the error of the technique. It is concluded that although slight acidification might have taken place, this has not been of sufficient magnitude to significantly effect most biological communities (e.g. higher plants, invertebrates and fish).
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    Predicting freshwater critical loads from national data on geology, soils and land use (1995)
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    Water, air & soil pollution 85 (1995), S. 2443-2448 
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    ISSN: 1573-2932
    Keywords: critical loads ; freshwaters ; geology ; soil ; land use ; sensitivity ; acidification ; catchments
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Using information on geology, soils and land use, a map has been generated for Great Britain which indicates five classes of sensitivity of surface waters to acidification. This map has been used for designing sampling strategies for mapping critical loads of acidity for freshwaters. This paper evaluates the freshwater sensitivity map using a data set of water chemistry collected as part of the UK critical loads programme. Discriminant analysis was used to predict five critical load classes from information on geology and soil sensitivity for freshwater sites. This showed geology and soil information can correctly predict approximately 50% of all critical loads classes. In addition, 77% of sites fall within one critical loads class of that predicted. Predictions may be improved by including other variables eg altitude and geographical location. Differences between lake, stream and reservoir sites are also examined. Ranges of critical loads values were determined for each of the five classes of surface water sensitivity. While a trend in critical load values was evident between classes, there was significant overlap. A simplified sensitivity map with only three classes related more closely to critical loads values. The paper demonstrates the usefulness of the surface water sensitivity map for assessing acidification at a national scale, but highlights the difficulties of predicting critical loads for individual sensitive catchments using national data.
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    Application of the critical loads approach in South Africa (1995)
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    Water, air & soil pollution 85 (1995), S. 2577-2582 
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    ISSN: 1573-2932
    Keywords: South Africa ; Eastern Transvaal ; Mpumalanga ; critical loads ; acidification
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract South Africa is the most industrialised country in southern Africa and stands at some risk from negative pollution impacts. To the authors' knowledge, this paper presents the first attempt to apply the critical loads approach on the African continent; although sensitivity mapping has been performed for Africa and the rest of the world (Kuylerstierna et al, this conference). Actual sulphate and base cation deposition loads in Mpumalanga (formerly the Eastern Transvaal province of South Africa) were mapped from 16 monitoring sites. The region is characterised by long, dry periods with little rain, high evaporation (up to 8 mm per day) and low run-off (15% of MAP). Provisional critical load and exceedance maps were produced for the surface waters using the Steady-State Water Chemistry Model and the Diatom model. Maps of soil sensitivity to acid deposition, based on bedrock lithology, soil chemical characteristics and land cover, were produced. A weathering rate of 0.39–0.86 keq/ha/year was calculated for the most sensitive sites and taken as the critical load, based on the assumption that the weathering rate represents the buffering ability of the system. The critical loads were contrasted with measures of actual deposition to examine potential scenario's for critical load exceedances. Akey factor in refining the sensitivity maps, and allowing estimation of the critical loads, is the accurate calculation of weathering rates under the warmer and more arid environmental conditions prevalent in South Africa. In a developing country such as South Africa, where research resources are limited, the critical loads approach is a valuable means of assessing the risk of potential impacts of atmospheric deposition.
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    The effect of pH and atmospheric deposition on concentrations of trace elements in acidified freshwaters: A statistical approach (1996)
    Springer
    Water, air & soil pollution 88 (1996), S. 227-246 
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    ISSN: 1573-2932
    Keywords: trace elements ; trace metals ; freshwaters ; median concentrations ; acidification ; atmospheric deposition ; effect of pH ; surface waters ; mobilization ; Czech Republic
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A statistical evaluation of 5 338 analysis of freshwaters from little polluted stream basins in the Czech Republic indicated a relationship between the Pb, Cu, Zn, Cd, Be, As, Mn, Sr, F− and Fe concentrations and the pH, over a range of pH 3.6 to 9.6. Except for Sr, the median concentrations of all the trace metals increase with decreasing pH, but the increase never extends over the whole studied acidic range (pH 3.6 to 7.0). Acid deposition related mobilization of Mn and Be into freshwaters explains the sharp increase in their concentrations with decreasing pH. Cadmium and Zn are also mobilized n strongly acidic environment. The concentrations of Be, As, F− and Mn in strongly acidic waters and those of Zn and Cd in weakly acidic ones are considerably higher in areas receiving a higher atmospheric loading. For Be and Mn, the higher concentrations are caused by higher acid deposition rates, while for As and F−, the concentrations are probably greater due to higher atmospheric deposition of these elements over more intensely acontaminated areas of the Czech Republic. In extremely acidic waters (pH 〈 4.2), the concentrations of Mn, Be, Cd, Zn and Al no longer increase with decreasing pH; on the contrary, those of Mn and Be actually decrease. This seems to be primarily caused by a decrease in their concentrations within the surface horizons of soils and vegetation induced by prolonged leaching. The Cd and Zn concentrations are independent of pH over an interval of pH 5.4 to 6.0 and thus the increase in the mean concentrations of Cd and Zn with decreasing pH involves two separate stages, at pH 〉 6.0 and at pH 〈 5.4. The concentrations of Cu in acid freshwaters are controlled by both the presence of high molecular weight organics plus biota uptake and by their atmospheric deposition levels; the concentrations of As and Pb are in addition controlled by sorption on Fe - oxyhydroxides. These elements accumulate in the topsoil, even under conditions of severe acidification. The surprisingly lower concentrations of Pb and Cu were found in acidic waters of more contaminated areas.
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    Thinner eggshells of dipper (Cinclus cinclus) eggs from an acidified area compared to a non-acidified area in Norway (1997)
    Springer
    Water, air & soil pollution 93 (1997), S. 255-266 
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    ISSN: 1573-2932
    Keywords: Ratcliffe index ; egg size ; acidification
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Eggs of dippersCinclus cinclus from a chronically acidified area in Southern Norway were compared with eggs from a non-acidified area in Central Norway. There were no differences in egg size, as measured by volume, weight, length and calculated surface area, between the two areas. Eggshells were 7.0% lighter and 6.1% thinner, as measured by the Ratcliffe index and 7.0% as measured by the eggshell index (shell weight/surface area) in Southern Norway than in Central Norway. The Ratcliffe and eggshell indices were highly correlated. Scanning electron micrographs showed that the palisade layer of eggshells of eggs from the acidified area was 10.7% thinner than that of eggshells of eggs from the non-acidified area. Eggshell vapour permeability was not significantly influenced by area. Since the moderately lower thickness in Southern Norway was not accompanied by higher vapour permeability, this indicates that the reduced eggshell thickness did not cause desiccation of dipper eggs in the acidified area. The possibility of underestimating the environmental effects of acidification on dippers is discussed.
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    Increasing role of nitrogen in the acidification of surface waters in the Adirondack Mountains, New York (1997)
    Springer
    Water, air & soil pollution 95 (1997), S. 313-336 
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    ISSN: 1573-2932
    Keywords: nitrogen ; acidification ; Adirondack Mountains ; atmospheric deposition
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Assessments of the aquatic effects of acidic deposition have focused on sulfur, as have recent efforts to control the emissions of acidifying compounds. Nitrogen dynamics were excluded from most acidic deposition modeling studies because it was believed that terrestrial ecosystems strongly retain N and because modeling N is a more formidable task than modeling S due to the influence of complex biological processes on N cycling. Re-examination of available data for the Adirondack Mountains of New York suggests that N deposition may be contributing to both chronic and episodic acidification of freshwaters to a greater extent than is generally believed. Previous research concluded that N has played a limited role in acidification processes in these lakes, based on regional averages of chronic chemistry. However, it is now known that historic acidification responses have been spatially variable within the Adirondack Mountains and that the declines in lakewater pH have been less than previously believed. Lakewater NO3 − concentrations are commonly in the range of 5 to 25 μeq L−1 on a chronic basis in portions of the Adirondack region that have experienced significant chronic acidification. These NO3 − concentrations correspond in magnitude to inferred historical acidification. Furthermore, the relative importance of NO3 − as an agent of acidification increases dramatically during snowmelt when conditions are most toxic to fish. The consequence of not addressing N in formulating acidification recovery strategies for the Adirondacks includes the likelihood that we will overestimate the response of surface water to the mandated sulfur emissions reductions.
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    The Impact of Nitrogen on Forest Soils and Feedbacks on tree Growth (1999)
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    Water, air & soil pollution 116 (1999), S. 65-74 
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    ISSN: 1573-2932
    Keywords: Forests ; N deposition ; soil nitrogen transformations ; nitrification ; tree growth ; acidification ; BC/A1 ratio ; 15N
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The effects of pollutant nitrogen on forest soils and the potential feedbacks on tree growth are discussed using data from recent plot and catchment manipulation studies. Results indicate that N applied to the soil affects both soil N transformations and base cation status in some forest soils. Whilst reductions in tree growth are infrequently reported, a greater understanding of the effect of increased N deposition on soil N transformations, and associated changes in soil acidification and nutritional balance, is essential if sensitive stands are to identified. In particular, the factors controlling soil N accumulation rates and thus the onset of nitrate leaching are not clearly understood with increased nitrogen availability potentially increasing nitrogen accumulation due to abiotic fixation and lignolytic enzyme suppression, whilst the onset of nitrification as the C/N ratio of forest floor material declines, may reduce N retention efficiency. The switch from increased to decreased tree growth rate in response to N additions in some experiments highlights the need for long-term studies as a necessary component of future research.
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    URL: http://dx.doi.org/10.1023/A:1005209622313
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    Effects of Acidification Due to Emissions from the Kola Peninsula on Fish Populations in Lakes Near the Russian Border in Northern Norway (1998)
    Springer
    Water, air & soil pollution 102 (1998), S. 17-36 
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    ISSN: 1573-2932
    Keywords: northern Norway ; lakes ; acidification ; brown trout ; Arctic charr
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In this paper we document the effects of acidification on fish populations in lakes in Sør-Varanger near the Russian border in northern Norway. We used questionnaires in order to assess the current status and distribution of different fish species, and conducted test-fishing to determine relative abundance (CPUE-T) and age structure. Acidification of surface waters in this area is due to emissions of SO2 from smelters on the Kola Peninsula in Russia (Nikel and Zapoljarnij) between 10 and 30 km from the Norwegian border. Sulphur deposition in Sør-Varanger ranges from 0.6 to 2.0 g S m-2 yr-1, which is similar to levels in the most acidified areas in southern Norway. However, a dominant fraction of the acidic deposition reaches the ground in particulate form during summer and autumn. Coastal areas in Sør-Varanger receive small amounts of precipitation; the annual mean is 580 mm. We obtained fish status from 401 lakes, about 40% of all lakes larger than 3 ha, which were inhabited by 236 and 293 populations of Arctic charr (Salvelinus alpinus) and brown trout (Salmo trutta), respectively. The extent of fish damage was small as only three populations of Arctic charr were lost, while three populations of Arctic charr and eight populations of brown trout were at various stages of reduction. Damaged and lost fish populations were identified in smaller lakes at relatively high elevations (172–349 m) in six areas in the Jarfjord Mountains, covering a land area of 30.0 km2. Most of the damage probably occurred during the 1970s and 1980s. In lakes that supported or had supported Arctic charr and brown trout, we found a significant relationship between CPUE-T, and acid neutralizing capacity (ANC) and pH, and also between alkalinity and the concentration of inorganic Al for brown trout. In both species, the catch of fish in age groups 1+ and 2+ (CPUE-R) increased significantly with CPUE-T. Affected populations typically exhibited irregular age composition, and age-classes were missing, indicating that reductions in fish populations were due to recruitment failure. The limited fish damage is related to relatively good catchment resistance to acidic inputs, small amounts of wet deposition as well as precipitation. These conditions result in low accumulation of acidic compounds, producing less acidic run-off waters and few episodes of unfavourable water quality.
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    Effects of environmental stress on forest crown condition in Europe. Part I: Hypotheses and approach to the study (2000)
    Springer
    Water, air & soil pollution 119 (2000), S. 317-333 
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    ISSN: 1573-2932
    Keywords: acid deposition ; acidification ; air pollution ; critical load ; defoliation ; drought ; meteorological stress ; N deposition ; nitrogen oxides ; ozone ; sulphur
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract This paper is the first in a series of four,describing the hypothesis and approach of acorrelative study between observed data on crowncondition in Europe, monitored since 1986 at asystematic 16 × 16 km grid, and site-specificestimations of various natural and anthropogenicstress factors. The study was based on the hypothesisthat forests respond to various natural andanthropogenic stress factors, whose contributiondepend on the geographic region considered. In view ofthis hypothesis, major stand and site characteristics,chemical soil composition, meteorological stressfactors (temperature and drought stress indices) andair pollution stress (concentrations and/ordepositions of SOx, NOy, NHx andO3) were included as predictor variables. Theresponse variables considered were actual defoliationand changes/trends in defoliation for five major treespecies. The spatial distribution of the averagedefoliation during the period 1986–1995 shows highdefoliation in Central Europe and in parts ofScandinavia and of Southern Europe. There are,however, sharp changes at country borders, which aredue to methodological differences between countries.The spatial distribution of the calculated trends showa distinct cluster of large deterioration in parts ofCentral and Eastern Europe and in Spain and a ratherscattered pattern of positive and negative trends for most of Europe, indicating that other factors than airpollution only have a strong impact on defoliation.The limitations of the study are discussed in view ofthe quality of the considered response and predictor variables.
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    Gradual reduction and extinction of fish populations in acid lakes (1995)
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    Water, air & soil pollution 85 (1995), S. 389-394 
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    ISSN: 1573-2932
    Keywords: fish community ; colonization ; extinction ; acidification ; temporal patterns
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Fish communities in four lakes sampled over several years were compared against a reference data set of forty-nine lakes in south-central Ontario. Two of the temporal-comparison lakes (Crosson and Grindstone) exhibit significant changes in their fish communities relative to the reference set. This was due to the extirpation of various fish species (white sucker Catostomus commersoni, lake trout Salvelinus namaycush, and blacknose shiner Notropis heterolepis) during the intervening years. A control lake in the temporal comparison (Poorhouse) showed little change in species composition over time and no loss of species. The fourth temporal lake, Plastic Lake, also showed little change likely as a consequence of the previously documented extinctions in this lake. White suckers within Crosson Lake have demonstrated intermittent recruitment and a 89% reduction in population abundance due to acid-induced reproductive constraints in their spawning stream. Similar conditions contributed to the loss of sucker populations and additional species in Grindstone and Plastic Lakes also. Various species in many of the lakes represent metapopulations. Given the barriers imposed by outflow drainage conditions, these accelerated rates of local extinctions have not been balanced by colonizations from other lakes within the watershed. As a consequence the underlying fish communities have been changed and will remain so without active rehabilitation.
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    Resilience of macroinvertebrate communities in acidified and limed streams (1995)
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    Water, air & soil pollution 85 (1995), S. 413-418 
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    ISSN: 1573-2932
    Keywords: Macroinvertebrates ; resilience ; recovery ; acidification ; Sweden ; liming ; streams ; species richness
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Benthic macroinvertebrate communities in 13 acidified South Swedish streams were sampled in 1981. The same localities were revisited in 1994 when most of the streams had been limed. Untreated streams were used as references. Species richness and proportion of predators increased between the two years. The differences are probably due to the warm and dry summer in 1994. However, the proportions of acid-sensitive species in various groups of streams were about the same the two years, indicating that liming had an insignificant effect on the return of these species. The resilience of the bottom fauna may be attributable to biotic conditions or the failure of the practiced liming methods to maintain healthy chemical conditions.
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    Survival of brook trout (Salvelinus fontinalis) embryos and fry in streams of different acid sensitivity in Shenandoah National Park, USA (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 445-450 
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    ISSN: 1573-2932
    Keywords: Brook trout ; acidification ; Virginia ; early life history
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Shenandoah National Park receives more atmospheric sulfate loading than any other USA national park. pH has been gradually declining in low-ANC streams for more than 10 years. We have completed four 1-to-3 month-long field bioassays in three streams differing in acid neutralizing capacity (ANC), using a total of 18,000 hatchery brook trout eyed-eggs through fry. In three of the four bioassays, embryos/fry showed poorer survivorship in the low-ANC stream, compared to the high-ANC stream. Substantial mortalities occurred under different hydrological conditions, including steady rain plus significant rain events (fall 1992), low rainfall followed by a significant rain event (spring 1993), and steady light rain and snowmelt with no large rain events (spring 1994). In a fourth bioassay (fall 1993), poor survivorship occurred in all three streams due to drought conditions. Trout placed in the intermediate-ANC stream showed variable survivorship, in two bioassays as high as in the high-ANC stream, and in one bioassay as poor as in the low-ANC stream. Baseflow ANC in the intermediate-ANC stream is 40–100 ueq/L, and pH never falls below 6.0. However, during episodes, pH in this stream sometimes fluctuates rapidly in the range of 6.0 to 7.0, and this fluctuation itself may be a source of physiological stress.
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    The role of sea-salts in enhancing and mitigating surface water acidity (1995)
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    Water, air & soil pollution 85 (1995), S. 553-558 
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    ISSN: 1573-2932
    Keywords: Sea-salts ; acidification ; Scottish catchments ; aluminium ; salmonids
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Enhancement of the acidity of fresh waters due to sea-salt “episodes” has been reported in western regions of Scotland, Ireland and Norway and eastern regions of Canada and the United States of America. In all cases these short-term pH depressions have been ascribed to cation-exchange processes in catchment soils whereby sodium ions displace acidic cations (H+, Al3+) resulting in a lowering of the Na/Cl ratio in run-off water. Studies of sea-salt episodes in different catchment types of similar sensitivity in Scotland show significant variations in chemical responses, especially in terms of acidification status. Catchments with high background salt content, in a low sulphur deposition area, show only a small increase in acidity with negligible aluminium release and most of the sodium retention matched by Ca and Mg release. Catchments in intermediate deposition areas, with low background salt levels, exhibit smaller sodium retention with increased leaching of acidity and labile aluminium. High non-marine S deposition sites, with intermediate background salt levels, reveal high levels of acidity and aluminium leaching associated with some calcium leaching and evidence of Mg retention. Mitigation of acidification occurs at sites with high background sea-salt levels (eg north west Scotland) where acidic deposition is selectively retained in catchment soils. Non-marine sulphate values in run-off are therefore much lower (often producing negative values) than those predicted from current S deposition values. Consequently such sites are presently producing false exceedances of freshwater Critical Loads when current S deposition values are used. Future reductions in S deposition will probably affect the adsorption characteristics at these sites with consequent effects on sulphate leaching.
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    Do stream invertebrates accumulate aluminium at low pH conditions? (1995)
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    Water, air & soil pollution 85 (1995), S. 407-412 
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    ISSN: 1573-2932
    Keywords: Stream ; acidification ; aluminium ; invertebrates ; insects ; accumulation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Acidified surface waters often show elevated aluminium (Al) levels, detrimental to fish and some invertebrates. Whether Al can accumulate in benthic invertebrates, with time and/or along the food chain, is not clear. To test this, benthic invertebrates, representing different functional feeding groups, were collected in spring from streams, with different acidity and Al concentrations. Weight-specific Al content was determined with an AAS. At localities with pH ≈ 4, high Al contents (≈ 1 mg inorg-Al g−1 af dw) were found in shredders and/or deposit feeders (Asellus aquaticus, Nemoura sp., and limnephilids), while the predator Isoperla grammatica contained only ≈ 0.3 mg Al g−1, and the “filtering predator” Plectrocnemia conspersa almost no Al. Also at pH ≈ 6 Nemoura sp. and limnephilids showed significantly higher Al contents than did the predators Isoperla grammatica and Rhyacophila nubila, Al concentrations of the animals were often higher at pH 4 than at pH 6. Thus, no evidence of any food chain accumulation (or biomagnification) of Al could be validated. Accordingly, this study gives no support that the high concentrations of Al in fish and birds are due to their feeding on benthic invertebrates at low pH conditions. It was also found that animals that inhabit and/or consume benthic detritus as food contain highest Al levels.
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    The decline of fauna in small streams in the Swedish mountain range (1995)
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    Water, air & soil pollution 85 (1995), S. 419-424 
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    ISSN: 1573-2932
    Keywords: acidification ; acid episodes ; critical load ; mountain ; streams ; benthic fauna ; fish
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Investigations in the southern part of the Scandinavian mountain range have shown a direct correlation between snowpack pH and the lowest pH in small streams. In streams with catchments 〈100 km2 a snowpack pH below 4.8 resulted in a stream pH below 5.5. As the snowpack pH in the southern mountain range is 4.0–4.6, lower values to the south and at high altitudes, large areas are affected by acid deposition. The acidity of the snowpack is released almost directly into the streams during thaw, due to the large snowpack, rapid thaw, steep terrain and thin soils. The acidification of the snow has lead to an extensive fauna depletion, especially in smaller streams without upstream lakes. The abundance of benthos in acidified streams in the municipality of Härjedalen (11.000 km2) is today only one tenth of the abundance before acidification. Fish populations have declined to the same extent, and several acid-sensitive species have been lost. It is concluded that mountain streams and fauna are extremely sensitive to acidification, and that even large reductions of emissions will be insufficient.
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    Modelling geochemistry and Lake pH since glaciation at Lake Gårdsjön (1995)
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    Water, air & soil pollution 85 (1995), S. 713-718 
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    ISSN: 1573-2932
    Keywords: Weathering ; mineral ; soil ; acidification ; geochemistry ; surface water
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The soil acidification model SAFE was modified to calculate historical changes in geochemistry and runoff since the last glaciation ended at the Lake Gårdsjön F1 catchment 12 000 B.P. Changes in runoff pH and ANC, soil weathering rate, soil mineralogy, soil texture and base saturation was also calculated. The changes in mineralogy compared favorable to data. Modeled historic weathering rates were slightly higher than data suggest, while present weathering rate was somewhat to low, 37 mmolc m−2 yr−1. The weathering rate was very high immediately after the last glaciation, and decreased as the smaller particles were consumed by weathering. The calculated runoff pH follows the pattern of the paleo-inferred pH. SAFE suggests a natural depletion of base cations in the C-layer.
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    Changes in trace element speciation in kola north surface waters during snow melt (1995)
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    Water, air & soil pollution 85 (1995), S. 731-736 
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    ISSN: 1573-2932
    Keywords: acidification ; surface water ; pollution ; species ; metals
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The powerful mass-flow of melt water during the brief period of spring thaw provides a surge of pollutants and causes extremely toxic short term conditions. Together with the increase in total metal concentrations during this period, a redistribution in metal speciation occurs that increases the proportion of more toxic forms. Concentrations of ion-exchangeable fractions of nickel (Ni), copper (Cu), aluminium (Al), and manganese (Mn) show strong negative correlations with pH. The sum of complex metal species shows a strong positive correlation with total organic carbon (TOC). A data analysis model based on relationships observed between key parameters and metal behaviour together with gidrological data allowed an assessmrnt of the metal impact on waterbodies from accumulated airborne pollution (Ni, Cu) as well as from accelerated leaching from watersheds (Al, Mn).
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    Pathways of chemical recovery in acidified, metal-contaminated lakes near Sudbury, Ontario, Canada (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 797-803 
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    ISSN: 1573-2932
    Keywords: acidification ; recovery ; copper ; nickel ; lake ; rate ; alkalinity
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract This paper describes the recovery pathways of two lakes situated near the Coniston nickel-copper smelter. These lakes were exposed to very intense airborne pollution, including SO2, H2SO4, Ni and Cu, during the 60 year operation of the smelter. After the closure of the Coniston smelter in 1972 and the subsequent improvement in air quality, the water quality in both lakes began to improve. Despite their proximity and exposure to similar inputs, the lakes differed both in the rate and magnitude of recovery. This study demonstrates the capacity of lakes to recover from chemical stresses over a very short period. Changes in Cu and Ni concentration could be predicted, while changes in pH, measured as H+, could not. The reasons for this discrepancy as well as the processes and lake parameters that control chemical recovery are discussed.
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    Lake and watershed neutralization strategies (1995)
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    Water, air & soil pollution 85 (1995), S. 889-894 
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    ISSN: 1573-2932
    Keywords: acidification ; acid neutralizing capacity ; calcite ; fish ; liming ; mitigation ; ecosystems
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The Experimental Watershed Liming Study (EWLS) evaluated the application of CaCO3, to a forested watershed to mitigate the acidification of surface water. During October 1989, 6.9 Mg CaCC3/ha was applied by helicopter to two subcatchments of about 50% (102.5 ha) of the Woods Lake watershed area. The EWLS team investigated the response to treatment of soils (chemistry and microbial processes), vegetation, wetland, stream and lake waters, and phytoplankton and fish, and applied the Integrated Lake Watershed Acidification (ILWAS) model in predicting a watershed treatment duration of up to 50 years. Observations showed a gradual change in pH, acid neutralizing capacity (ANC) and Ca2+ in the water column; direct lake additions of CaCO3 (three different times) were characterized by abrupt changes following base addition and subsequent rapid reacidification. Moreover, the watershed treatment eliminated the snowmelt acidification of the near-shore region of the lake observed during direct lake treatments. Positive ANC water in the tributary and near-shore area improved conditions for fish reproduction and for a viable fish population. Budgets for 12-month periods before and after the watershed treatment showed that the lake shifted from a source of ANC to a sink due to retention of elevated inputs of Ca2+ from the watershed CaCO3 application.
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    Soil chemistry change in a lowland english deciduous Woodland 1974–1991 (1995)
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    Water, air & soil pollution 85 (1995), S. 677-682 
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    ISSN: 1573-2932
    Keywords: soils ; acidification ; ancient woodland ; nitrogen ; environmental change
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract This study outlines the results of analysis of soil samples collected from fixed quadrats located in a regular pattern across Wytham Wood. Oxfordshire, England. The site contains plots of mixed deciduous ancient woodland and more recent plantations. A previous soil study was undertaken in 1974 and samples archived. Soils were resampled in 1991 and some re-analysis of the 1974 samples was undertaken. Soils were of a wide range in types from sands to gravels with a pH range of 3.0–7.0. Results showed some decline in pH in lower horizons, but most striking was a large increase in soil nitrogen for all horizons and soil types.
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    Groundwater acidification at Birkenes, southern Norway: Comparing trends of chemical composition of precipitation, throughfall, soilwater and groundwater (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1861-1866 
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    ISSN: 1573-2932
    Keywords: acidification ; buffering ; groundwater ; monitoring ; precipitation ; seasalt ; soil ; soilwater ; throughfall
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Chemical time trends for precipitation, throughfall, and soilwater (1986–1992), and groundwater (1980–1993) at Birkenes, southern Norway, are compared to gain insights into possible causes for the recent increase in groundwater acidification there. Precipitation and throughfall trends do not show evidence for an increase in anthropogenic acids (e.g. sulphate), but seasalt deposition (e.g. chloride) has been marginally greater in 1990–1992 than in most previous years on record. Soilwater composition partly indicates increasing acidification in recent years (pH, Al and ANC), but hardness and sulphate content are decreasing. Soilwater ANC became negative in 1989, revealing a lasting deficit in its potential to buffer acidity. Groundwater shows clear signs of intensifying acidification (pH, Al, ANC, hardness and sulphate), and this may result partly from climatic conditions (mild winters, ‘seasalt episodes’) and partly from the deterioration of an acid buffering system within the soil cover. Acidification via sulphate deposition certainly is not a direct cause. The declining hardness of soilwater suggests that the ion-exchange buffer in the soil may have ceased to function properly. The necessity for obtaining long-term time-series of water chemistry is underscored by this study.
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    Acidifying emissions in The Netherlands (1995)
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    Water, air & soil pollution 85 (1995), S. 1909-1914 
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    ISSN: 1573-2932
    Keywords: Emissions ; acidification ; SO2 ; NOX ; NH3 ; Netherlands
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The emission of acidifying compounds to air in the Netherlands, expressed as acidifying equivalents, consisted in 1992 mainly of NOX (45%), NH3 (35%) and SO2 (20%). Transportation, agriculture and large combustion plants each contributed about 30% to the national total emission of acidifying compounds. The emissions from transportation activities mainly consisted of NOX, while in agriculture NH3 emission strongly dominated. Combustion processes in large combustion plants resulted both in SO2 emissions (especially from refineries) and NOX emissions (especially from public power plants). The total emission of acidifying substances decreases steadily in the Netherlands. The emission in 1992 was 24% lower than in 1985. It is expected to decrease further in future. The emission levels in 1992 and 1993 still are more than twice as high as the emission objective for the year 2000, set by Dutch environmental policy.
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    Developing optimal abatement strategies for the effects of sulphur and nitrogen deposition at European scale (1995)
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    Water, air & soil pollution 85 (1995), S. 2601-2606 
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    ISSN: 1573-2932
    Keywords: Integrated Assessment Modelling ; eutrophication ; acidification
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Integrated Assessment Models were successfully used to provide input to the negotiations for the Oslo Protocol on Further Reductions of Sulphur Emissions, finalized within the United Nations Economic Commission for Europe Convention on Long-range Transboundary Air Pollution in Oslo in June 1994. The techniques developed within this framework will be extended now to the simultaneous analysis of sulphur and nitrogen deposition. In addition to acidification, atmospheric deposition of nitrogen contributes to eutrophication of certain ecosystems, through a nutrient effect, and originates from the long-range transport of emissions of both oxidised and reduced nitrogen (NOx and NH3). Modelling reductions in nitrogen deposition thus introduces a need to establish multi-pollutant multi-effect modelling techniques. This paper investigates the development of a model set up to examine reductions of these pollutants in an economically and environmentally efficient manner. The control of nitrogen deposition encompasses action across several economic sectors, particularly the power, transport and agricultural sectors. Combining sulphur and nitrogen deposition limits on a European scale will require a flexible modelling approach and the issues governing possible approaches are presented.
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    Squeezed soil-pore solutes — A comparison to lysimeter samples and percolation experiments (1996)
    Springer
    Water, air & soil pollution 89 (1996), S. 189-204 
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    ISSN: 1573-2932
    Keywords: Concentration depth profiles ; weathering reactions ; acidification ; cation exchange ; aluminium solubility ; aluminium sulphate minerals ; distribution of trace metals
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract This paper presents data on the chemical composition of soil pore fluids that have been obtained by a high-pressure squeezing technique and lysimeter sampling. Cation-exchange capacity has been calculated from cations extracted by a simple percolation method. All pore water concentrations are greatly influenced by the pH in solution. Most pore water concentrations do not simply parallel the corresponding mineralogical and chemical composition of the solids. The depth of the acidification front, as determined by analysis of samples obtained by percolation, is much better reflected in the chemical composition of the squeezed soil pore fluids than in the lysimeter samples. Distinct gradients are seen in Al concentration. In the B-horizons, concentrations of Al are close to the solubility of gibbsite. The pore water concentration profiles of Si and K apparently indicate dissolution of K-silicates, in particular K-feldspar. Contrary to the squeezed pore solutions the sulphate maximum concentration in the soil profile is not recorded by lysimeter samples. Mineral saturation indices show that pore solutions by squeezing are close to the saturation concentrations for K-jarosite and K-alunite. Sulphur-rich phases from the soil are compatible with mixtures of alunite jarosite, zaherite, basaluminite, and hydrobasaluminite. In the upper soil horizons the liquid/solid ratios [calculated as: concentration in solution (µg/ml) * solution fraction in solids (ml/g)/concentration in solids (µg/g)] increase in the order Ph 〈 OC ≈ Zn 〈 Cd and range from 10−6 to 10−3, indicating that Ph is most strongly held and still accumulates in the organic top soil. In the underlying deeper mineral horizons the ratios for Pb, Zn, and Cd decrease by one order of magnitude.
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    INCREASING ROLE OF NITROGEN IN THE ACIDIFICATION OF SURFACE WATERS IN THE ADIRONDACK MOUNTAINS, NEW YORK (1997)
    Springer
    Water, air & soil pollution 95 (1997), S. 313-336 
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    ISSN: 1573-2932
    Keywords: nitrogen ; acidification ; Adirondack Mountains ; atmospheric deposition
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Assessments of the aquatic effects of acidic deposition have focused on sulfur, as have recent efforts to control the emissions of acidifying compounds. Nitrogen dynamics were excluded from most acidic deposition modeling studies because it was believed that terrestrial ecosystems strongly retain N and because modeling N is a more formidable task than modeling S due to the influence of complex biological processes on N cycling. Re-examination of available data for the Adirondack Mountains of New York suggests that N deposition may be contributing to both chronic and episodic acidification of freshwaters to a greater extent than is generally believed. Previous research concluded that N has played a limited role in acidification processes in these lakes, based on regional averages of chronic chemistry. However, it is now known that historic acidification responses have been spatially variable within the Adirondack Mountains and that the declines in lakewater pH have been less than previously believed. Lakewater NO3 - concentrations are commonly in the range of 5 to 25 μeq L-1 on a chronic basis in portions of the Adirondack region that have experienced significant chronic acidification. These NO3 - concentrations correspond in magnitude to inferred historical acidification. Furthermore, the relative importance of NO3 - as an agent of acidification increases dramatically during snowmelt when conditions are most toxic to fish. The consequence of not addressing N in formulating acidification recovery strategies for the Adirondacks includes the likelihood that we will overestimate the response of surface water to the mandated sulfur emissions reductions.
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    Living in a Dusty World: Airborne Dust as a Key Factor for Alpine Lakes (1999)
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    Water, air & soil pollution 112 (1999), S. 217-227 
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    ISSN: 1573-2932
    Keywords: acidification ; dust deposition ; high mountain lakes
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract For a long time studies on precipitation and lake-water chemistry have focussed on the deposition of strong acids. Dust in snow and rain was analyzed much less intensively, but recent findings suggest that it may be the missing link which explains why many low-alkalinity lakes in the Alps and the Pyrenees did not become acidic and nutrient levels are seasonally high, whereas lakes in areas which are rarely influenced by dust depositions, for instance in Scandinavia, have acidified. Beside being a dominant factor for nutrient inputs to oceans, rain forests and remote lakes, dust can also play a major role in global warming and cooling, and it may significantly contribute to soil formation at mountain sites in the Mediterranean. I suggest that future changes in dust deposition and warming will be key factors for the development of alpine lakes.
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    Biotic Effects in Planktonic Crustacean Communities in Acifified Swedish Forest Lakes after Liming (1998)
    Springer
    Water, air & soil pollution 101 (1998), S. 257-288 
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    ISSN: 1573-2932
    Keywords: acidification ; forest lakes ; lime treatment ; planktonic crustaceans
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In Sweden, approximately 16 000 of a total of about 85 000 lakes have been acidified due to acidic deposition. Of these about 8000 have been treated with limestone powder in order to detoxify the acidified waters and protect sensitive fauna. The present study was performed in ten lakes in the southern part of the country. The lakes belong to four different catchments and were in different stages of acidification at the time of lime treatment. The composition of the zooplankton and fish communities also differed and three lakes were empty of fish at the beginning of the studies. Quantitative sampling of planktonic crustaceans was performed during the ice free season between 1976–87 in five of the lakes and between 1977–87 in the other five. After treatment the pH increased significantly in all lakes except one. The average number of crustacean taxa found per sampling occasion increased in all lakes. Increases were statistically significant in four of the lakes. In the lakes empty of fish, increased abundances of chaoborids inhibited, by predation, the increase of species richness. Species richness increased after the introduction of fish and the subsequent reduction of the chaoborids. At the end of the study, more taxa were found in the limed study lakes than in non-treated west coast lakes with an alkalinity of 0.04–0.10 meq L-1. Most species normally occurring in oligotrophic forest lakes were found. It was shown that the water quality after liming made the occurrence of sensitive species possible and that predation from fish and interactions within the zooplankton assemblage were of great importance to the species composition and structure of the zooplankton community.
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    URL: http://dx.doi.org/10.1023/A:1004901320524
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    Weathering Processes in a Lignite Mine Spoil Treated with a CaCo3-Rich Waste Slurry under Two Moisture Programmes (2000)
    Springer
    Water, air & soil pollution 119 (2000), S. 59-74 
    Details
    ISSN: 1573-2932
    Keywords: acidification ; chemical weathering ; liming ; mine spoil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Chemical processes affecting the acidity of asulphide-rich lignite mine spoil treated with high orlow doses of a CaCO3-rich industrial waste slurrywere studied in the laboratory under two moistureprogrammes (cycles of alternate waterlogging anddrying, and percolation) so as to determine the slurrydose neutralizing spoil acidity and the possibledetrimental effects of high doses. The most importantacidity-reducing process was the dissolution ofapplied calcium carbonate, and CaCO3 consumptionwas greater under percolation conditions than underwaterlogging and drying conditions. The most importantacidity-increasing process was the oxidation ofsulphides, which was again more intense underpercolation. Under waterlogging and drying conditions,the formation of hydroxysulphates may also havecontributed to acidification.
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    URL: http://dx.doi.org/10.1023/A:1005187317167
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    Terrestrial ecosystem sensitivity to acid deposition in South China (2000)
    Springer
    Water, air & soil pollution 118 (2000), S. 231-244 
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    ISSN: 1573-2932
    Keywords: acidification ; air pollution ; critical loads ; ecological factors
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Ecosystem sensitivity to acid deposition can be a basis for thederivation of cost-effective strategies to sulfur and nitrogenpollutant control, consequently is widely concerned around theworld. In the article, the relative sensitivity of terrestrialecosystem to acid deposition in South China is assessed andmapped using a new sensitivity classification system suitable tosubtropical ecosystem. The result shows that the distribution ofecosystem sensitivity to acid deposition in South China isalmost zonal, on the whole, sensitivity increases from the northand west to the south and east. The most sensitive areas are thenorthwest and southeast of Zhejiang province, the central partof Fujian province, and the northeast of Guangdong province andGuangxi Zhuang Autonomous Region, which are all in the old acidsoil areas with high precipitation and coniferous forests. Theresulting distribution of sensitive regions is different othermaps, including the sensitivity map which is implemented in theRAINS-Asia model.
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    URL: http://dx.doi.org/10.1023/A:1005139719658
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    Acidification of Solid and Solution Phases at Greater Depths (〉 150 cm) at Solling Spruce Site (2000)
    Springer
    Water, air & soil pollution 120 (2000), S. 89-105 
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    ISSN: 1573-2932
    Keywords: acidification ; cation exchange ; denitrification ; element fluxes ; lysimetry ; proton buffering ; silicateweathering ; Solling
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The acidification of the soil and percolation water at soildepths from 150 to 500 cm was studied at the Solling spruce sitefrom 1991 to 1996. NH4Cl exchangeable cations of the fineearth and bedrock fractions were obtained from different depthsand the soil solution composition was monitored at 150, 200,300, 400 and 500 cm depths using seven suction lysimeters at each depth.In the seepage water collected from 150 and 200 cm depth, pHvalues decreased in the period 1991 to 1996, but no significantchanges were observed in solutions collected below 200 cm depth.Element budgets of Al and Mb (Na, K, Mg, Ca) cationsindicated that buffering by exchange of Al with Mb cationsoccurred mainly in surface 200 cm soil depth. High variabilities in concentrations of SO4 (at 150 cm) andMa (Al, Mn, H, Fe) cations (at 300 and 500 cm) wereobserved. High variabilities in Ma cations could beassigned to one of the lysimeters at each depththat extracted low pH solutions. The amount of exchangeablecations in the fine earth and the bedrock fractions indicatedthat the acidification front (exchangeable Mb cations 〈 80equivalent percent) had occurred to soil depth of more than 360cm, but the extent of acidification that might have occurred inthe preindustrial period is not known. In both fine earth andbedrock fractions, depthwise changes of exchangeable Ma andMb cations were quite similar, suggesting that rockfractions have contributed to proton buffering not only bysilicate weathering but also by cation exchange.
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    The Effect of River Liming on the Trace Metal Budgets of a Down Stream Lake (1998)
    Springer
    Water, air & soil pollution 104 (1998), S. 57-75 
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    ISSN: 1573-2932
    Keywords: acidification ; liming ; trace metals
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Sediment cores from two lakes, connected by a limed river, were analyzed for organic matter, calcium (Ca), iron (Fe), manganese (Mn), zinc (Zn), copper (Cu), lead (Pb), cadmium (Cd), and ion exchange capacity. The distribution of trace metals in the pristine upper lake is governed primarily by changes in the long distance atmospheric transported pollutants. In the lake down stream of the liming station the distribution of trace metals in sediments deposited before liming started (1985) is similar to that in the pristine lake. Liming of the connecting river raises the pH value by about 1.8 units from 5.1 enhancing the accumulation rate of trace metals in the downstream lake. Iron enriched acid insoluble particles are likely to be important carriers of trace metals. The liming agent itself is the most important source for Pb, while increased accumulation of Zn and Cd is caused primarily by enhanced scavenging of dissolved metals. For Cu the two sources are of about equal importance.
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    URL: http://dx.doi.org/10.1023/A:1004955216612
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    Direct and indirect air pollution effects on materials including cultural monuments (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 153-165 
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    ISSN: 1573-2932
    Keywords: air pollutants ; effect on materials ; acidification ; cultural monuments ; sulphur dioxide ; nitrogen oxides ; ozone ; economic calculations
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Damage caused to materials exposed in the atmosphere constitutes one of the most important direct effects of acidifying air pollutants. Systematic field and laboratory investigations performed in the recent decade in many countries have contributed to a considerable increase in the knowledge on the mechanisms of the effects of pollutants, on the quantification of damage and on the assessment of the cost of damage. Beside the very important role of SO2 for several materials also studies of the direct or synergistic effect of NOx and O3 have contributed to the understanding of the complex pollution effects. Even if there are still considerable gaps of knowledge it seems that NOx and O3 may contribute in an important way to the deterioration of several materials also in indoor environments which are important for i.a. electronic equipment, storage conditions and museums. Important knowledge has been gained from the International Cooperation Project within UK ECE which is an extensive field exposure on 39 test sites. Dose-response relations have been obtained after 4-year exposure showing the effect of dry and wet deposition on corrosion of several material groups. Also the effect of micro- and mesoclimate on corrosion of building materials like plaster and bricks in different positions on buildings and locations within an urban area has been subject to systematic studies. Results from the studies are used i.a. for assessment of so called acceptable corrosion levels and for mapping areas where the levels are exceeded at different pollution scenarios, as well as for calculation of economic damage. Based on model studies for some city areas tentative calculations of damage cost have been performed for the European region. The indirect effects consist of increased corrosion due to water and soil acidification which are of importance in geologically sensitive areas. Structures which are in contact with soil and water represent a very great capital investment and are of vital importance to the community.
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    URL: http://dx.doi.org/10.1007/BF00483697
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    The role of nitrogen in acidification of Tatra Mountains lakes (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 481-486 
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    ISSN: 1573-2932
    Keywords: critical loads ; nitrogen deposition ; sulphur deposition ; acidification ; mountain lakes ; Tatra National Park
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract An overall level as well as seasonal changes of acidification of Tatra Mountains surface waters have been studied. Measurements carried out in the Tatra Mountains National Park were concentrated on two lakes: Dlugi Staw and Zielony Staw, situated in the crystalline, granitic part of the mountains. These lakes differ from each other in altitude (1784 m and 1632 m a.s.l. respectively) as well as in quantity and variety of flora and fauna living in and around them. The wet deposition of acidifying compounds of sulphur and nitrogen, and their seasonal variability in the area of the lakes were measured and compared with the critical loads of sulphur and nitrogen for these lakes and their catchments. Results showed that the critical loads of both sulphur and nitrogen in Dlugi Staw were exceeded all over the year and in Zielony Staw the acid deposition was roughly equal to critical load. A surprisingly high concentration of nitrogen compounds in acid deposition, well above the absorption ability of both the lakes and their catchments were ascertained. Nitrogen retention coefficients calculated for the lakes were as follows: Dlugi Staw — approximately 10%, Zielony Staw — approximately 50%. Seasonal variability in nitrate ions concentration in the lakes' waters reflected their prominent acidification caused by nitrogen compounds corresponding to stages 2 and 3 in the scale proposed recently by Stoddard (Stoddard, 1994).
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    Trends in surface water acidification at ecological monitoring sites in southeastern Canada (1981–1993) (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 577-582 
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    ISSN: 1573-2932
    Keywords: acidification ; water chemistry ; statistical trends ; monitoring ; recovery
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Atmospheric deposition and surface water chemistry have been monitored intensively at 5 geologically “sensitive” sites in southeastern Canada. The sites receive differing acid inputs that span the entire range found in Canada. Surface water data collected at 9 stations from 1981 to 1993 for SO 4 2− , NO 3 − , Alkalinity, DOC, pH, Ca2+ and Mg2+ have been analyzed to detect monotonic trends. Similarities between the temporal patterns and trends for SO 4 2− in deposition and surface water suggest that they are strongly linked at our sites. Our 13-year datasets showed significant negative SO 4 2− trends at the 3 Ontario sites and a positive trend in Nova Scotia. A climatically-induced SO 4 2− increase in northwestern Ontario has been reversed. Mobilization and export of adsorbed SO 4 2− and/or reoxidized S from the basins of central Ontario sites is delaying their recovery. Two of our 9 stations (in Quebec and central Ontario) are continuing to acidify. The 2 Nova Scotia stations have the highest DOC levels and both exhibit a decreasing trend. Ionic compensation for declining SO 4 2− varies from station to station, sometimes involving an Alk increase, sometimes a base cation decrease, and sometimes more complex combinations. Additional factors (e.g. climatic variation) also influence variable trends, and data records longer than those presently available will be needed to unequivocally verify acidification recovery.
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    Acidification in Norway — Status and trends (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 629-634 
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    ISSN: 1573-2932
    Keywords: acidification ; monitoring ; calibrated catchments ; lakes ; rivers ; ground water
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Surface and ground water monitoring in Norway is designed to give a regional coverage with most of the stations in areas with acidification and some stations in unpolluted areas that give background values. Surface water (weekly sampling) and precipitation (daily measurement) are monitored at 6 calibrated catchments, 5 located in southern Norway and 1 in northernmost Norway close to the Russian border. Ground water (weekly sampling) is monitored in 4 reservoirs in Southern Norway. 73 lakes located all over Norway are surveyed each fall. Nineteen rivers in western and southern Norway are monitored by monthly sampling. All sites are considered sensitive to acidification and are chosen to minimise the effects of anthropogenic catchment based impacts. Results from the monitoring over the period 1980–1994 show that there is a reduction of sulphate of about 25–35% in surface waters which is related to a 30–45% reduction in sulphate concentration in precipitation. An improvement in water quality as measured as increase in ANC has only been apparent since 1990. Due to heavy seasalt episodes in the most coastal catchments like Birkenes and the rivers in western Norway, there has been no improvement of ANC since 1980. Deposition of nitrogen has not changed over the last 10 years, and there is no change in the levels of nitrate in the monitored surface waters.
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    The “shenandoah national park: Fish in sensitive habitats” (SNP: FISH) project. An integrated assessment of fish community responses to stream acidification (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 309-314 
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    ISSN: 1573-2932
    Keywords: acidification ; Virginia ; fish response
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The “Shenandoah National Park: Fish in Sensitive Habitats” (SNP:FISH) project is a response to declining pH and acid neutralizing capacity in Shenandoah National Park (SNP) streams. SNP receives more atmospheric sulfate than any other USA national park, and pH had decreased to the point where early negative effects on fish were expected. SNP provides the opportunity to study the early stages of acidification effects on fish. Three different classes of geological formations yield streams with low-ANC (0 μEq/L), intermediate-ANC (60–100 μEq/L) or high-ANC (150–200 μEq/L) waters in SNP. This allows a comparison of responses across a water quality gradient in a small geographic area receiving similar deposition. Both chronic and episodic acidification occur in SNP streams. Biological effects are apparent in fish species richness, population density, condition factor, age, size, and bioassay survival. A primary project objective was to provide the necessary data for development and testing models for forecasting changes in fish communities resulting from changes in stream chemistry. Monitored variables include several which are predictive of acidification effects on SNP fish communities.
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    URL: http://dx.doi.org/10.1007/BF00476847
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    A field study on the influence of soil ph on trace element levels in spring wheat (Triticum aestivum), potatoes (Solanum tuberosum) and carrots (Daucus carota) (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 835-840 
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    ISSN: 1573-2932
    Keywords: acidification ; arable soils ; trace elements (Cd, Ni, Zn, Cu, Mn, Cr, Al, Se) ; plant uptake ; field study
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Soil pH is one of the main factors influencing the solubility and availability of trace elements in arable soils. Thus pH can affect the trace element contents of agricultural crops and thereby indirectly influence human health. The aim of this study was to determine Cd, Ni, Zn, Cu, Mn, Cr, Al and Se contents in spring wheat, potatoes and carrots (Cd, Ni and Zn) and estimate their correlations with certain soil factors (surface and subsurface soil pH and organic matter content) governing the plant availability of these elements. Commercial fields were sampled in Sweden in order to cover a wide range of soil types with respect to pH, soil texture and organic matter content. Concentrations of Zn, Mn, Ni (grain) and Cd (straw) in spring wheat (n=43); Cd, Ni, Zn, Mn, Cu and Al in potatoes (n=69); and Cd, Ni and Zn in carrots (n=36) showed significant negative correlations with surface soil pH (0–25 cm). The Se content of potatoes and Cr content of spring wheat straw were positively correlated with soil pH. Stepwise multiple regressions including a combination of soil pHs (0–25 and 25–50 cm) and organic matter contents (0–25 cm) showed that the organic matter content as well as the surface and subsurface soil pH significantly influenced concentrations of several trace elements in one or more of the studied crops. It was concluded that, if acid deposition together with other acidifying processes (fertilisation, harvest of biomass, etc.) are not balanced by a sufficient amount of liming there might be a decrease in the pH of arable soils, which, in turn will lead to decreased levels of Se in edible crops but an overall increase concentrations of other trace elements.
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    URL: http://dx.doi.org/10.1007/BF00476933
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    The consequences of liming a highly acidified catchment in central Scotland (1995)
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    Water, air & soil pollution 85 (1995), S. 1015-1020 
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    ISSN: 1573-2932
    Keywords: acidification ; liming ; catchment ; fish ; Scotland
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Research during the mid 1980s identified acidified, forested catchments in central Scotland whose hydrochemistry was not capable of supporting native fish populations. Calcium concentrations were around 20 μeq l−1, less than the suggested critical value of 50 μeq l−1, with hydrogen concentrations around 70 μeq l−1, greater than the critical value of about 30 μeq l−1. Limestone was applied by aerial application to the source areas of selected streams in 1990 with around 5% (15 ha) of the total catchment area of 270 ha treated at 10 tonnes ha−1. Stream monitoring, carried out over the period 1989–1995, showed an immediate response to liming followed by a progressive decline. Calcium values were elevated to 〉150 μeq l−1 and hydrogen concentrations reduced to 20 μeq l−1, reverting in time towards pre-liming values. Although salmonid survival was improved during low flow conditions in summer, only a few fry survived to the autumn as acid episodes increased, and these were subsequently lost from the system during the winter period. Budget calculations indicated losses of around 30% of the applied calcium during the first four years. Studies on the vegetation and soils revealed a greater than expected penetration of calcium to depth (10–20 cm) in the soil profile. Results suggest that source area liming at this rate has had minimal effects on the vegetation and by increasing the proportion of the catchment limed to 15% could have a much greater success in reducing the frequency of biologically damaging episodes.
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    An integrated analysis of sulfur emissions, acid deposition and climate change (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1539-1550 
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    ISSN: 1573-2932
    Keywords: acidification ; air pollution impacts ; climate change ; global change ; integrated modeling ; sulfur deposition
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract This paper presents one of the first integrated analyses of acidification and climate change on a geographically-detailed basis, and the first linkage of integrated models for acid deposition (RAINS) and for climate change (IMAGE 2). Emphasis in this paper is on Europe. Trends in driving forces of emissions are used to compute anthropogenic SO2 emissions in 13 world regions. These emissions are translated into regional patterns of sulfur deposition in Europe and global patterns of sulfate aerosols using source-receptor matrices. Changes in climate are then computed based on changes in sulfate and greenhouse gases. Finally, we compute ecosystem areas affected by acid deposition and climate change based on exceedances of critical loads and changes in potential vegetation. Using this framework, information from global and regional integrated models can be used to link sulfur emissions with both their global and regional consequences. Preliminary calculations indicate that the size of European area affected by climate change in 2100 (58%) will be about the same as that affected by acid deposition in 1990. By the mid 21st century, about 14% of Europe's area may be affected by both acid deposition and climate change. Also, reducing sulfur emissions in Europe will have both the desirable impact of reducing the area affected by acid deposition, and the undesirable impact of enhancing climate warming in Europe and thus increasing the area affected by climate change. However, for the scenarios in this paper, the desirable impact of reducing sulfur emissions greatly outweighs its undesirable impact.
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    Modelling ”clean rain” treatments in acidified soils-EXMAN project results (1995)
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    Water, air & soil pollution 85 (1995), S. 1807-1812 
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    ISSN: 1573-2932
    Keywords: Modelling ; experimental manipulation ; acidification ; recovery
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The SAFE dynamic model was applied to a ”clean rain” roof experiment performed within the EXMAN project. In the experiment ambient throughfall was removed and replaced with artificial ”clean throughfall”. Input of S, N and H to the forest ecosystem was reduced by 75–100%. The results of the modelling show, that the time scales of model predictions and experiments are the same. The change in base cation flux was well reproduced, while the simulation of changes in aluminum flux was less successful. pH stayed constant in the experiment as well as in the calculations.
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    Ecosystem recovery after emission reductions: Sudbury, Canada (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1783-1788 
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    ISSN: 1573-2932
    Keywords: recovery ; smelter ; acidification ; copper ; nickel
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A case history is presented describing the ecosystem changes that accompanied the nearly 90% reduction of SO2 and metal particulate emissions from Sudbury smelters during the past 25 years. The instances of severe ground-level fumigations that caused acute damage to vegetation in an area of approximately 1,000 km2 have been nearly completely eliminated. Significant improvements in water quality have also occurred in many of the estimated 7,000 acid-damaged lakes. Several species of acid-sensitive phytoplankton, Zooplankton and insects have invaded lakes where improvements have occurred. Epiphytic lichens have reinvaded the former “lichen desert” that once extended out 7 km from the smelters. Sensitive species such as Evernia mesomorpha and Usnea hirta now exist throughout the area. The vascular plant communities have been relatively slow to recover in the most severely damaged terrestrial areas. Metal-tolerant grasses (e.g. Agrostis scabra. Deschampsia caespitosa) were the first species to invade the barrens. Acid- and metal-contamination of soil, severe microclimate conditions, and the damaging effects of insect pests appear to delay recovery of terrestrial ecosystems. Recovery rates of aquatic ecosystems are also affected by a suite of physical, chemical and biotic interactions and many lakes remain severely damaged.
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    Long-term modelling of airborne pollution within the Northern Hemisphere (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2051-2056 
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    ISSN: 1573-2932
    Keywords: acidification ; air pollution ; air pollution modelling
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A long-term modelling (1991–1994) of oxidised sulphur, bound nitrogen and some heavy metals has been carried out by MSC-E/EMEP for the Northern Hemisphere. The transport unit of the model is an Eulerian scheme which could be classified as Pseudo-Lagrangian one. Vertical distribution described by means of Gaussian approximation and the exchange with the free troposphere are taken into account. Vertical movement is calculated proceeding from local mixing conditions, state of the surface, its height (topography) etc. The chemical unit for acid compounds contains 25 reactions and 14 compounds including sulphur and nitrogen compounds peroxyacetylnitrate, tropospheric ozone, volatile hydrocarbons (but methane) are considered as a whole via ozone creation potential. The model time step is 1 hour, meteorological data (winds, temperature, precipitation etc.) cover 6-hour intervals. The model results show that very significant part of the Arctic and West Asian acid pollution is produced by European countries. On the whole the Arctic pollution by SOx, NOx and NHx comes from sources of Old World. The main source of sulphur pollution is located in Russia and of nitrogen compound — in Central and Northern Europe. About 50% SOx, 70% NOx and 40% NHx deposition in Central Asia and Kazakhstan is-imported from external sources. A similar situation is observed in European and Asian parts of Russia.
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    Mapping base cation deposition in Europe on a 10 × 20 km grid (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2389-2394 
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    ISSN: 1573-2932
    Keywords: atmospheric deposition ; base cations ; Europe ; acidification
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Atmospheric deposition of base cations in Europe is mapped on a 10×20 km grid using the inferential modeling technique. Deposition fields are found to resemble the geographic variability of sources, climate and land use. In large parts of southern Europe, more than 50% of the potential acid deposition is found counteracted by deposition of base cations. In central and northwestern Europe, however, base cation deposition usually amounts less than 25% of the acid input. An uncertainty analysis to assess the quality of the base cation deposition maps revealed that for an average grid cell the deviation from the estimated value can be as large as 140%.
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    URL: http://dx.doi.org/10.1007/BF01186191
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    Critical loads — A valuable catchment management tool? (1995)
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    Water, air & soil pollution 85 (1995), S. 2485-2490 
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    ISSN: 1573-2932
    Keywords: Critical loads ; water ; catchment assessments ; forestry ; acidification
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Planning advice for forest planting in acid sensitive areas suggests that, where calculated critical loads for acidity are exceeded at a catchment level, new conifer planting may not be appropriate. In south west Scotland, acid waters are currently found in areas where critical loads are not exceeded. The rivers Cree and Bladnoch show a decline in pH of about one unit since 1970, when major afforestation of the headwaters began. No equivalent decline in pH was observed in the adjacent Water of Luce, although it receives similar inputs and has similar geology and soils. Little of the Luce catchment is afforested. Recent surveys of water quality, invertebrate fauna and salmonid fish reveal a picture of widespread acid conditions, impoverished benthos and absence of young salmon. 25 streams (total catchment 〉150km2) recorded pH 〈4.5 in high flow conditions. Critical loads for acidity were 〉1.5keqha−1yr−1 for 12 and 〉2keqha−1yr−1 for 6 of the 25 streams. Published deposition data suggested that one stream with pH 〈4.5 and 7 streams with pH 〈 5 were in areas where critical load was not exceeded. In 22 catchments, forestry was a major land use. To be effective as planning and management tools, systems must be robust and easy to operate. Critical load exceedance calculations remain research tools at the catchment level where deposition data is generally inadequate. The uncertainties inherent in critical load exceedances render them sources of argument and not beacons of enlightenment.
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    URL: http://dx.doi.org/10.1007/BF01186207
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    Watershed base-cation cycle dynamics modeled over forest regrowth in a Central Appalachian ecosystem (1996)
    Springer
    Water, air & soil pollution 89 (1996), S. 1-22 
    Details
    ISSN: 1573-2932
    Keywords: biogeochemistry ; watershed ; watershed analysis ; model ; budget ; input-output ; base cations ; dynamics ; weathering ; forest floor ; nutrient cycles ; soil ; acidification ; depletion ; ecosystem
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Watershed ecosystem analysis has been used to study aspects of nutrient cycles in many regions of the US. Here we quantify watershed input-output budgets and intrasystem cycling of the base cations Ca, K and Mg in a montane Virginia ecosystem. The intrasystem fluxes of uptake, return, canopy leaching and mineralization were simulated over the period of forest aggradation. A forest-dynamics model, based on previous models, was created to model biotically-driven fluxes at this site; biomass nutrient concentrations were parameterized with a field study. A two-year watershed mass-balance study was then conducted to estimate geologic fluxes for comparison with modeled biotic fluxes. Results show the major biotic fluxes to be much greater, highlighting the importance of considering biomass dynamics in ecosystem nutrient-cycling studies. Mineralization from forest-floor biomass compartments proved to be an increasingly important avenue for internal recycling during aggradation. Accumulation of base cations in biomass also corresponded to a production of H+ in soil at three times the H+ levels in atmospheric deposition at this location. Such high levels of base removal in soils could exceed weathering rates and may result in a depletion of bases from the soil exchange complex.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00300418
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  • 87
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    Influence of organic acids on model projections of lake acidification (1996)
    Springer
    Water, air & soil pollution 91 (1996), S. 271-282 
    Details
    ISSN: 1573-2932
    Keywords: acidification ; diatom ; model ; organic acids
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract We employed three mathematical models to make quantitative estimates of the pH of 33 statistically-selected lakes in the Adirondack mountains, New York (USA) prior to the Industrial Revolution (1840). The models included 1) the MAGIC watershed acidification model, 2) a paleolimnological model of diatom-inferred pH, and 3) the MAGIC model modified to incorporate an empirically-based model of natural organic acidity. Application of approaches 2) and 3) yielded consistent estimates of pre-industrial Adirondack lakewater pH. However, when the organic acid model was not included, MAGIC calculations and diatom-inferred values showed poor agreement. MAGIC projections of lakewater pH 50 years into the future, under differing atmospheric deposition scenarios, were also sensitive to inclusion of the organic acid model. MAGIC predicted greater recovery in response to reduced deposition when organic acids were not considered. These results suggest that failure to consider the pH buffering of naturally-occurring organic acidity will often result in biased projections which overemphasize the response of lakewater pH to changes in atmospheric inputs of strong acid.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00666263
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  • 88
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    Terrestrial ecosystem sensitivity to acidic deposition in developing countries (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2319-2324 
    Details
    ISSN: 1573-2932
    Keywords: sensitivity ; buffering ; acidification ; vegetation effects ; soil ; Al toxicity ; GIS ; mapping ; nutrient
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Acidic deposition is considered a problem in Europe and North America but the potential for ecosystem damage from this pollution is also increasing rapidly in many developing countries. It is therefore important to assess current and future risks of ecosystem effects due to acidic deposition in these areas. It is possible to indicate risk areas by linking an assessment of sensitivity to net acidic input rates derived from deposition estimates for sulphur and nitrogen compounds and base cations. A method to assess and map a relative scale of terrestrial ecosystem sensitivity using international datasets is presented. The assessment relies on the determination of buffering mechanisms that prevent effects related to acidic deposition. Land-cover data, edaphic and climate datasets are combined using a GIS. Large areas are assessed as highly sensitive to acidic deposition in tropical regions of Asia, South and Central America and Africa, and also in the Boreal forests of northern Asia. Sensitive areas cover forest and non-forest ecosystems and some areas of agricultural production. Critical loads are not evaluated in this project but initial estimates will be applied to sensitivity classes at a further stage which will allow estimation of areas at risk by comparison with deposition.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01186180
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  • 89
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    Thinner Eggshells of Dipper (Cinclus Cinclus) Eggs from an Acidified Area Compared to a Non-Acidified Area in Norway (1997)
    Springer
    Water, air & soil pollution 93 (1997), S. 255-266 
    Details
    ISSN: 1573-2932
    Keywords: Ratcliffe index ; egg size ; acidification
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Eggs of dippers Cinclus cinclus from a chronically acidified area in Southern Norway werecompared with eggs from a non-acidified area in Central Norway. There were no differences inegg size, as measured by volume, weight, length and calculated surface area, between the twoareas. Eggshells were 7.0% lighter and 6.1% thinner, as measured by the Ratcliffe index and 7.0%as measured by the eggshell index (shell weight/surface area) in Southern Norway than in CentralNorway. The Ratcliffe and eggshell indices were highly correlated. Scanning electron micrographsshowed that the palisade layer of eggshells of eggs from the acidified area was 10.7% thinner thanthat of eggshells of eggs from the non-acidified area. Eggshell vapour permeability was notsignificantly influenced by area. Since the moderately lower thickness in Southern Norway wasnot accompanied by higher vapour permeability, this indicates that the reduced eggshell thicknessdid not cause desiccation of dipper eggs in the acidified area. The possibility of underestimatingthe environmental effects of acidification on dippers is discussed.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1022110321515
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    Integrated Assessment: an emerging methodology for complex issues (1998)
    Springer
    Environmental modeling and assessment 3 (1998), S. 19-29 
    Details
    ISSN: 1573-2967
    Keywords: acidification ; LRTAP ; integrated environmental assessment
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Over recent years Integrated Assessment (IA) has been presented as a new and innovative approach to modern decision making. In this paper we explore some of the key features that we consider characterise IA; we present IA as a framework that allows a flexible approach to uncertainty in decision making and to which a broad palette of expertise can contribute. The example of the development of an international agreement to reduce acidic deposition is used to illustrate the current practical status of an IA. The scientific process leading to this agreement has previously been described as IA but we argue that, although it marks a change from traditional approaches, further progress is still required to satisfy the requirements for a successful and durable IA.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1019042201713
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  • 91
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    The Bioaccumulation of Mercury in Aquatic Organisms from Two Similar Lakes with Differing pH (1999)
    Springer
    Ecotoxicology 8 (1999), S. 49-56 
    Details
    ISSN: 1573-3017
    Keywords: mercury ; methylmercury ; fish ; acidification ; biomagnification
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Two small drainage lakes of similar surface area (0.4–0.6 km 2 ) and depth, and situated in close proximity to one another (about 9 km apart) in the Muskoka-Haliburton district of rural Ontario, Canada were chosen to investigate the effects of differing pH on Hg accumulation in fish and other biota. Blue Chalk Lake is circumneutral (pH = 6.3–6.9) with an average dissolved organic carbon (DOC) concentration of 2.69 mg/L; Plastic Lake is acidic (pH = 5.2–5.6) with a similar DOC level (2.72 mg/L). Neither lake is an impoundment, and neither receives inputs from point-source urban or industrial waste emissions. Surficial (top 4 cm) sediments and various aquatic biota, including crayfish (Orconectes virilis)], and 5 species of fish [brown bullhead (Ictalurus nebulosus), creek chub (Semotilus atromaculatus), pumpkinseed sunfish (Lepomis gibbosus), yellow perch (Perca flavenscens) and rock bass (Ambloplites rupestris)] were sampled for Hg analysis. Only creek chub and pumpkinseed occurred in both lakes. Significant size (length) vs. Hg-concentration relationships were observed for brown bullhead, pumpkinseed, yellow perch and rock bass, but not for crayfish nor for creek chub in either lake. Rock bass had the highest mean Hg concentration (1.02 ± 0.98 μg/g dry wt.). Pumpkinseed from Plastic Lake had the highest overall rate of accumulation with increasing size. Several individual pumpkinseed and rock bass sampled from the acidic Plastic Lake had Hg concentrations equal to or greater than levels reported to be hazardous to breeding piscivorous birds, such as common loons (Gavia immer), whereas no fish from Blue Chalk approached this threshold (0.3 μg/g wet wt). This study illustrates the importance of within-lake parameters, particularly pH, and species trophic level, in determining Hg accumulation in fish in lakes of similar size that receive similar atmospheric Hg inputs.
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    URL: http://dx.doi.org/10.1023/A:1008936910823
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  • 92
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    Assessing the effects of domestic and international energy scenarios and emission reduction strategies on acidification in Finland (1999)
    Springer
    Environmental modeling and assessment 4 (1999), S. 103-113 
    Details
    ISSN: 1573-2967
    Keywords: critical loads ; acidification ; area exceeded ; integrated assessment ; emission scenarios ; sulfur oxides ; nitrogen oxides ; ammonia ; deposition modeling
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract An integrated model system was developed and used to assess the effects of alternative energy production scenarios and reduction policies on acidification of lakes and forest soils in Finland. The analysis covered different energy scenarios and resulting emissions of sulfur oxides and nitrogen oxides in Finland, as well as ammonia emissions with various control requirements. In addition, emission reduction scenarios of varied ambition levels in the bordering areas of Finland and in other parts of Europe were included in the analysis. The impacts of the different scenarios were quantified with exceedances of critical loads for acidification and with the total areas where the critical loads are exceeded. The possibilities for reducing the areas with critical load exceedances with national or bilateral measures were investigated. The differences in areas at risk, if depositions from domestic and nearby sources are estimated with a regional model and point-source databases or with a continental scale model and coarser-scale emission data, were analyzed. The reasons for the differences and the implications for national-level assessment are discussed.
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    URL: http://dx.doi.org/10.1023/A:1019099814434
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  • 93
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    Weathering processes under various moisture conditions in a lignite mine spoil from as pontes (N.W. Spain) (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 347-366 
    Details
    ISSN: 1573-2932
    Keywords: acidification ; chemical weathering ; hydroxysulfates formation ; mine spoil ; sulfides oxidation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Processes contributing to acid release/consumption during weathering of a lignite mine spoil (2.3% w/w S as sulfides) from As Pontes (N.W. Spain) were studied under three moisture conditions (at field capacity or under alternate wetting-drying or forced percolation), which were simulated in laboratory experiments. Oxidation of sulfides to sulfates was favoured under all three moisture conditions, releasing most acid in spoil kept at field capacity. Hydroxysulfates formed in spoil kept at field capacity or under alternate wetting-drying conditions, thereby contributing to acid release. Acid consumption by dissolution of clay minerals, especially micas, was favoured under all three moisture conditions, but was particularly intense in spoil at field capacity. Dissolution of aluminium oxides was also favoured under all the moisture conditions studied.
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    URL: http://dx.doi.org/10.1007/BF02407214
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    INFLUENCE OF PEATLANDS ON THE ACIDITY OF LAKES IN NORTHEASTERN ALBERTA, CANADA (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 17-38 
    Details
    ISSN: 1573-2932
    Keywords: acid-sensitive lakes ; acidification ; organics peatlands ; Sphagnum
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract About a third of the lakes surveyed in the Birch Mountains Upland of northeastern Alberta, Canada, have pH below 7.0; 25% have alkalinities below 10 mg/L identifying them as acid-sensitive following criteria established by the National Research Council of Canada (1981). Lakes in this region vary greatly as to surface area and depth. Watersheds also vary in area and in amount of peatland cover. Peatlands in the form of peat plateaus and collapse scars, continental bogs, treed and open fens, and shallow organic deposits cover over 50% of some watersheds. Surface water chemistries of these peatlands form three distinct classes: bogs, poor fens and shallow organic deposits. The acidity of certain lakes in this northern area is best explained by effects from high cover of Sphagnum-dominated peatlands in surrounding watersheds. Due to greater flow-through, poor fens appear to be more important than bogs in affecting the acidity of associated lakes.
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    URL: http://dx.doi.org/10.1023/A:1026433231110
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    THE DIFFERENCE IN BROWN TROUT (SALMO TRUTTA L.) BLOOD COMPOSITION FROM ACIDIC AND LIMED SITES OF TWO RIVERS IN WESTERN NORWAY (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 203-210 
    Details
    ISSN: 1573-2932
    Keywords: acidification ; blood ; environment ; fish
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Certain blood morphology parameters: red blood cell (RBC) sizes; percentage of polymorphonuclear leukocytes and ratio polychromatocyte/RBC in Brown trout (Salmo trutta L.) from acidified water (mean pH value 4.94) and limed water (mean pH value 5.66) were investigated. The sizes of RBC long axises were significantly larger in fish from acidic environment than from limed condition (14.37 and 12.96 μm respectively). The percentage of polymorhonuclear cells (7.86 and 3.32) and polychromatocyte/RBC ratio (0.079 and 0.019) were also significantly larger in fish from the acidified environment. Blood morphology parameters are concluded to be usefull for testing and detection of long-term acidic stress in fish in nature.
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    URL: http://dx.doi.org/10.1023/A:1026404417464
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  • 96
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    WEATHERING PROCESSES UNDER VARIOUS MOISTURE CONDITIONS IN A LIGNITE MINE SPOIL FROM AS PONTES (N.W. SPAIN) (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 347-366 
    Details
    ISSN: 1573-2932
    Keywords: acidification ; chemical weathering ; hydroxysulfates formation ; mine spoil ; sulfides oxidation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Processes contributing to acid release/consumption during weathering of a lignite mine spoil (2.3% w/w S as sulfides) from As Pontes (N.W. Spain) were studied under three moisture conditions (at field capacity or under alternate wetting-drying or forced percolation), which were simulated in laboratory experiments. Oxidation of sulfides to sulfates was favoured under all three moisture conditions, releasing most acid in spoil kept at field capacity. Hydroxysulfates formed in spoil kept at field capacity or under alternate wetting-drying conditions, thereby contributing to acid release. Acid consumption by dissolution of clay minerals, especially micas, was favoured under all three moisture conditions, but was particularly intense in spoil at field capacity. Dissolution of aluminium oxides was also favoured under all the moisture conditions studied.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1026448611666
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  • 97
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    Influence of Peatlands on the acidity of lakes in northeastern Alberta, Canada (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 17-38 
    Details
    ISSN: 1573-2932
    Keywords: acid-sensitive lakes ; acidification ; organics peatlands ; Sphagnum
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract About a third of the lakes surveyed in the Birch Mountains Upland of northeastern Alberta, Canada, have pH below 7.0; 25% have alkalinities below 10 mg/L identifying them as acid-sensitive following criteria established by the National Research Council of Canada (1981). Lakes in this region vary greatly as to surface area and depth. Watersheds also vary in area and in amount of peatland cover. Peatlands in the form of peat plateaus and collapse scars, continental bogs, treed and open fens, and shallow organic deposits cover over 50% of some watersheds. Surface water chemistries of these peatlands form three distinct classes: bogs, poor fens and shallow organic deposits. The acidity of certain lakes in this northern area is best explained by effects from high cover ofSphagnum-dominated peatlands in surrounding watersheds. Due to greater flow-through, poor fens appear to be more important than bogs in affecting the acidity of associated lakes.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF02407194
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    THE EFFECT OF EL NIÑO-RELATED DROUGHT ON THE RECOVERY OF ACIDIFIED LAKES (1997)
    Springer
    Environmental monitoring and assessment 46 (1997), S. 105-111 
    Details
    ISSN: 1573-2959
    Keywords: acidification ; El Niño ; global change ; Southern Oscillation (SOI) Index ; sulphate
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Although SO2 emissions and deposition rates havedeclined substantially since the implementation of sulphuremission control programmes in North America [1], recovery(measured as decreases in $${\text{SO}}_{\text{4}}^{{\text{2 - }}} $$ concentrations) of affected lakes in central Ontario has been much less substantial thananticipated based on the decrease in deposition. The slowrecovery is attributed to the reoxidation and release of storedsulphur in catchments. Reduced sulphur retained in previousyears when sulphur deposition was higher is exposed to air andoxidized during severe droughts, then exported duringsubsequent wet periods. Elevated stream $${\text{SO}}_{\text{4}}^{{\text{2 - }}} $$ concentrations and export rates occur in the autumns of yearswith prolonged severe droughts, particularly in catchments withextensive wetlands. Drought in our study catchments occurred inyears following strong El Niño events. When the SouthernOscillation Index (SOI) was strongly negative (1976–77, 1982–83,1986–87, 1991–92, 1993–94) the frequency of occurrence ofdrought the following summer in small catchments with shallowoverburden was extremely high. A lake‘s rate of recovery fromacidification depends upon the amount of excess reduced Sthat has been stored in anoxic zones in the catchment (largely afunction of the extent of wetlands) during years of elevated Sdeposition rates, and the frequency and severity of droughts. Iflong-term changes in global or regional climate alter thefrequency or magnitude of El Niño-related droughts, therecovery of acidified lakes will be affected.
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    URL: http://dx.doi.org/10.1023/A:1005740002952
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