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  • Articles  (256)
  • heavy metals  (118)
  • nitrogen  (78)
  • mercury  (63)
  • Energy, Environment Protection, Nuclear Power Engineering  (256)
  • 1
    Electronic Resource
    Electronic Resource
    Application of an ion mobility detector in radiation stimulated plasma chemistry
    Amsterdam : Elsevier
    Radiation Physics and Chemistry 42 (1993), S. 993-996 
    Details
    ISSN: 0969-806X
    Keywords: acceleration ; argon ; beta particles ; drift ; electric field ; electrons ; excited states ; ion mobility ; ions mobility ; nitrogen ; reactive species
    Source: Elsevier Journal Backfiles on ScienceDirect 1907 - 2002
    Topics: Chemistry and Pharmacology , Energy, Environment Protection, Nuclear Power Engineering , Physics
    Type of Medium: Electronic Resource
    URL: http://linkinghub.elsevier.com/retrieve/pii/0969-806X(93)90419-U
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  • 2
    Electronic Resource
    Electronic Resource
    Distribution and coassociations of selected metals in seals of the Antarctic
    Amsterdam : Elsevier
    Environmental Pollution 83 (1994), S. 341-349 
    Details
    ISSN: 0269-7491
    Keywords: Antarctica ; distribution ; heavy metals ; inter-metal correlation ; seals
    Source: Elsevier Journal Backfiles on ScienceDirect 1907 - 2002
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1016/0269-7491(94)90156-2
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  • 3
    Electronic Resource
    Electronic Resource
    Mercury and selenium in arctic and coastal seals off the coast of Norway
    Amsterdam : Elsevier
    Environmental Pollution 85 (1994), S. 153-160 
    Details
    ISSN: 0269-7491
    Keywords: grey seal ; harbour seal ; harp seal ; mercury ; ringed seal ; selenium
    Source: Elsevier Journal Backfiles on ScienceDirect 1907 - 2002
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1016/0269-7491(94)90081-7
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  • 4
    Electronic Resource
    Electronic Resource
    Iron content and its relations to the sulphur and titanium contents of epiphytic and terricolous lichens and pine bark in Finland
    Amsterdam : Elsevier
    Environmental Pollution 84 (1994), S. 131-138 
    Details
    ISSN: 0269-7491
    Keywords: air pollution ; bioindicators ; element ratios ; geochemical relations ; heavy metals
    Source: Elsevier Journal Backfiles on ScienceDirect 1907 - 2002
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1016/0269-7491(94)90095-7
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  • 5
    Electronic Resource
    Electronic Resource
    Heavy metal concentrations in sediments from Manila Bay, Philippines and inflowing rivers
    Amsterdam : Elsevier
    Environmental Pollution 86 (1994), S. 83-88 
    Details
    ISSN: 0269-7491
    Keywords: Manila Bay ; heavy metals ; historical trend of pollution ; marine sediment ; riverine sediment
    Source: Elsevier Journal Backfiles on ScienceDirect 1907 - 2002
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1016/0269-7491(94)90009-4
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  • 6
    Electronic Resource
    Electronic Resource
    A Risk Assessment for Consumers of Mourning Doves (1998)
    Springer
    Risk analysis 18 (1998), S. 563-573 
    Details
    ISSN: 1539-6924
    Keywords: Risk assessment ; mourning doves ; hunting ; radionuclides ; heavy metals ; lead shot ; cesium
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Recreational and subsistence hunters and anglers consume a wide range of species, including birds, mammals, fish and shellfish, some of which represent significant exposure pathways for environmental toxic agents. This study focuses on the Department of Energy's (DOE's) Savannah River Site (SRS), a former nuclear weapons production facility in South Carolina. The potential risk of contaminant intake from consuming mourning doves (Zenaida macroura), the most popular United States game bird, was examined under various risk scenarios. For all of these scenarios we used the mean tissue concentration of six metals (lead, mercury, cadmium, selenium, chromium, manganese) and radiocesium, in doves collected on and near SRS. We also estimated risk to a child consuming doves that had the maximum contaminant level. We used the cancer slope factor for radiocesium, the Environmental Protection Agencies Uptake/Biokinetic model for lead, and published reference doses for the other metals. As a result of our risk assessments we recommend management of water levels in contaminated reservoirs so that lake bed sediments are not exposed to use by gamebirds and other terrestrial wildlife. Particularly, measures should be taken to insure that the hunting public does not have access to such a site. Our data also indicate that doves on popular hunting areas are exposed to excess lead, suggesting that banning lead shot for doves, as has been done for waterfowl, is desirable.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/B:RIAN.0000005931.39844.35
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  • 7
    Electronic Resource
    Electronic Resource
    Influence of Prenatal Mercury Exposure Upon Scholastic and Psychological Test Performance: Benchmark Analysis of a New Zealand Cohort (1998)
    Springer
    Risk analysis 18 (1998), S. 701-713 
    Details
    ISSN: 1539-6924
    Keywords: Benchmark ; mercury ; risk assessment ; epidemiology
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract This paper presents benchmark (BMD) calculations and additional regression analyses of data from a study in which scores from 26 scholastic and psychological tests administered to 237 6- and 7-year-old New Zealand children were correlated with the mercury concentration in their mothers' hair during pregnancy. The original analyses of five test scores found an association between high prenatal mercury exposure and decreased test performance, using category variables for mercury exposure. Our regression analyses, which utilized the actual hair mercury level, did not find significant associations between mercury and children's test scores. However, this finding was highly influenced by a single child whose mother's mercury hair level (86 mg/kg) was more than four times that of any other mother. When that child was omitted, results were more indicative of a mercury effect and scores on six tests were significantly associated with the mothers' hair mercury level. BMDs calculated from five tests ranged from 32 to 73 mg/kg hair mercury, and corresponding BMDLs (95% lower limits on BMDs) ranged from 17 to 24 mg/kg. When the child with the highest mercury level was omitted, BMDs ranged from 13 to 21 mg/kg, and corresponding BMDLs ranged from 7.4 to 10 mg/kg.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/B:RIAN.0000005917.52151.e6
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  • 8
    Electronic Resource
    Electronic Resource
    Interactions of bacteria with cadmium (1992)
    Springer
    Biodegradation 3 (1992), S. 161-170 
    Details
    ISSN: 1572-9729
    Keywords: bioremediation ; cadmium ; heavy metals
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract Cadmium pollution arises mainly from contamination of minerals used in agriculture and from industrial processes. The usual situation is of large volumes of soil and water that are contaminated with low — but significant — concentrations of cadmium. Therefore, detoxification of the polluted water and soil involves the concentration of the metal, or binding it in a way that makes it biologically inert. Cadmium is one of the more toxic metals, that is also carcinogenic and teratogenic. Its effects are short term, even acute (diseases like Itai-itai), or long term. The long term effects are intensified due to the fact that cadmium accumulates in the body. This paper describes a study involving several hundred cadmium-resistant bacterial isolates. These bacteria could be divided into three groups—the largest group consisted of bacteria resistant to cadmium by effluxing it from the cells. The bacteria of the other two groups were capable of binding cadmium or of detoxifying it. We concentrated on one strain that could bind cadmium very efficiently, depending on the bacterial biomass and on the pH. This strain could effectively remove cadmium from contaminated water and soil.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00129081
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  • 9
    Electronic Resource
    Electronic Resource
    An integrated algal sulphate reducing high rate ponding process for the treatment of acid mine drainage wastewaters (1998)
    Springer
    Biodegradation 9 (1998), S. 247-257 
    Details
    ISSN: 1572-9729
    Keywords: acid mine drainage ; algae ; heavy metals ; high rate algal ponds ; sulphate reducing bacteria ; waste stabilisation ponds
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract Acid mine drainage pollution may be associated with large water volume flows and exceptionally long periods of time over which the drainage may require treatment. While the use and role of sulphate reducing bacteria has been demonstrated in active treatment systems for acid mine drainage remediation, reactor size requirement and the cost and availability of the carbon and electron donor source are factors which constrain process development. Little attention has focussed on the use of waste stabilisation ponding processes for acid mine drainage treatment. Wastewater ponding is a mature technology for the treatment of large water volumes and its use as a basis for appropriate reactor design for acid mine drainage treatment is described including high rates of sulphate reduction and the precipitation of metal sulphides. Together with the co-disposal of organic wastes, algal biomass is generated as an independent carbon source for SRB production. Treatment of tannery effluent in a custom-designed high rate algal ponding process, and its use as a carbon source in the generation and precipitation of metal sulphides, has been demonstrated through piloting to the implementation of a full-scale process.The treatment of both mine drainage and zinc refinery wastewaters are reported. A complementary role for microalgal production in the generation of alkalinity and bioadsorptive removal of metals has been utilised and an Integrated 'Algal Sulphate Reducing Ponding Process for the Treatment of Acidic and Metal Wastewaters' (ASPAM) has been described.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1008352008353
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  • 10
    Electronic Resource
    Electronic Resource
    Aboveground nitrogen and phosphorus use by five plantation-grown trees with different leaf longevities (1991)
    Springer
    Biodegradation 14 (1991), S. 167-191 
    Details
    ISSN: 1572-9729
    Keywords: leaf longevity ; nitrogen ; nutrient use efficiency ; phosphorus ; requirement ; retranslocation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract Aboveground nitrogen (N) and phosphorus (P) requirement, retranslocation and use efficiency were determined for 28-year-old red oak (Quercus rubra L.), European larch (Larix decidua Miller), white pine (Pinus strobes L.), red pine (Pinus resinosa Ait.) and Norway spruce (Picea abies (L) Karst.) plantations on a similar soil in southwestern Wisconsin. Annual aboveground N and P requirements (kg/ha/yr) totaled 126 and 13 for red oak, 86 and 9 for European larch, 80 and 9 for white pine, 38 and 6 for red pine, and 81 and 13 for Norway spruce, respectively. Nitrogen and P retranslocation from current foliage ranged from 81 and 72%, respectively, for European larch, whereas red pine retranslocated the smallest amount of N (13%) and Norway spruce retranslocated the smallest amount of P (18%). In three evergreen species, uptake accounted for 72 to 74% of annual N requirement whereas for two deciduous species retranslocation accounted for 76 to 77% of the annual N requirement. Nitrogen and P use (ANPP/uptake) was more efficient in deciduous species than evergreen species. The results from this common garden experiment demonstrate that differences in N and P cycling among species may result from intrinsic characteristics (e.g. leaf longevity) rather than environmental conditions.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00000806
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  • 11
    Electronic Resource
    Electronic Resource
    A ground water nitrogen budget for a headwater swamp in an area of permanent ground water discharge (1991)
    Springer
    Biodegradation 14 (1991), S. 209-224 
    Details
    ISSN: 1572-9729
    Keywords: ground water ; hydrology ; nitrogen ; mass balance ; nutrient retention ; swamp
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract Ground water inputs and outputs of N were studied for a small ground water discharge swamp situated in a headwater drainage basin in southern Ontario, Canada. Darcy's equation with data for piezometers was used to measure inputs of shallow local ground water at the swamp margin and deep regional ground water beneath the swamp. Ground water flux was also quantified by measuring ground water discharge to the outlet stream draining the swamp in combination with a chemical mixing model to separate shallow and deep ground water components based on chloride differences. Estimates of shallow ground water flux determined by these two approaches agreed closely however, the piezometer data seriously underestimated the deep ground water input to the swamp. An average ground water input-output budget of total N (TN) total organic nitrogen (TON) ammonium (NH4 +-N) and nitrate (NO3 --N) was estimated for stream base flow periods which occurred on an average of 328 days each year during 1986–1990. Approximately 90% of the annual NO3 --N input was contributed by shallow ground water at the swamp margin. Deep ground water represented about 65% of the total ground water input and a similar proportion of TON and NH4 +-N inputs. Annual ground water NO3 --N inputs and outputs were similar whereas NH4 +-N retention was 4 kg ha-1 representing about 68% of annual ground water input. Annual TON inputs in ground water exceeded outputs by 7.7 kg ha (27%). The capacity of the swamp to regulate ground water N fluxes was influenced by the N chemistry of ground water inputs and the hydrologic pathways of transport within the swamp.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00000808
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  • 12
    Electronic Resource
    Electronic Resource
    Sulfur metabolism in higher plants: potential for phytoremediation (1998)
    Springer
    Biodegradation 9 (1998), S. 311-318 
    Details
    ISSN: 1572-9729
    Keywords: glucosinolates ; gypsum ; heavy metals ; phyto-extraction ; phytoremediation ; sulfate
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract Sulfur is a major nutrient for all organisms. Plant species have a high biodiversity in uptake, metabolization and accumulation of sulfur so that there are potentials to use plants for phytoremediation of sulfur-enriched sites. A survey of soils enriched with sulfur either naturally or by human activities shows that a surplus of sulfur is mostly accompanied with a surplus of other chemical elements which may limit phytoremediation because these co-occurring elements are more toxic to plants than sulfur. In addition, the accumulation of the other elements makes the plant material (phyto-extraction) less suitable for the use as fodder and for human consumption.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1008250827209
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  • 13
    Electronic Resource
    Electronic Resource
    Prospects for in vivo NMR methods in xenobiotic research in plants (1998)
    Springer
    Biodegradation 9 (1998), S. 411-422 
    Details
    ISSN: 1572-9729
    Keywords: agrochemicals ; heavy metals ; NMR imaging ; NMR spectroscopy ; subcellular compartmentation xenobiotic metabolism
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract The application of non-invasive nuclear magnetic resonance (NMR) methods in xenobiotic research is reviewed in relation to: (i) the characterisation of the effects of xenobiotics on the metabolism of plants and plant cell suspensions; (ii) the direct detection of xenobiotics and their degradation products in vivo; and (iii) the spatial localisation of xenobiotics and their derivatives at the subcellular and tissue levels. Novel information has been generated by in vivo NMR studies of both agrochemicals and heavy metals, but a lack of generality in the methods makes it difficult to extrapolate from one successful application to the next. In vivo NMR spectroscopy is shown to be informative when a xenobiotic perturbs metabolic pathways that are accessible to the technique, and it is useful for probing the partitioning of paramagnetic metal ions between the cytoplasm and the vacuole. The successful application of 19F NMR to the analysis of plant tissue extracts also suggests that in vivo 19F NMR spectroscopy may have a role in biotransformation studies of fluorinated xenobiotics. In contrast NMR imaging techniques have been little used for xenobiotic research in plants, and while the method has been shown to be capable of monitoring the uptake and translocation of paramagnetic ions in plants, the potential use of high resolution 1H and 19F NMR imaging for mapping agrochemicals in tissues is still in its infancy.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1008372107739
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  • 14
    Electronic Resource
    Electronic Resource
    Heavy metal bioavailability in a soil affected by mineral sulphides contamination following the mine spillage at Aznalcóllar (Spain) (2003)
    Springer
    Biodegradation 14 (2003), S. 199-205 
    Details
    ISSN: 1572-9729
    Keywords: bioremediation ; heavy metals ; metal availability ; organic matter ; pyrite ; sulphide oxidation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract A field experiment, lasting 14 months, was carried out in order to assess the effect of organic amendment and lime addition on the bioavailability of heavy metals in contaminated soils. The experiment took place in a soil affected by acid, highly toxic pyritic waste from the Aznalcóllar mine (Seville, Spain) in April 1998. The following treatments were applied (3 plots per treatment): cow manure, a mature compost, lime (to plots having pH 〈 4), and control without amendment. During the study two crops of Brassica juncea were grown, with two additions of each organic amendment. Throughout the study, the evolution of soil pH, total and available (DTPA-extractable) heavy metals content (Zn, Cu, Mn, Fe, Pb and Cd), electrical conductivity (EC), soluble sulphates and plant growth and heavy metal uptake were followed. The study indicates that: (1) soil acidification, due to the oxidation of metallic sulphides in the soil, increased heavy metal bioavailability; (2) liming succeeded in controlling the soil acidification; and (3) the organic materials generally promoted fixation of heavy metals in non-available soil fractions, with Cu bioavailability being particularly affected by the organic treatments.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1024288505979
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  • 15
    Electronic Resource
    Electronic Resource
    Soil chemistry change in a lowland english deciduous Woodland 1974–1991 (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 677-682 
    Details
    ISSN: 1573-2932
    Keywords: soils ; acidification ; ancient woodland ; nitrogen ; environmental change
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract This study outlines the results of analysis of soil samples collected from fixed quadrats located in a regular pattern across Wytham Wood. Oxfordshire, England. The site contains plots of mixed deciduous ancient woodland and more recent plantations. A previous soil study was undertaken in 1974 and samples archived. Soils were resampled in 1991 and some re-analysis of the 1974 samples was undertaken. Soils were of a wide range in types from sands to gravels with a pH range of 3.0–7.0. Results showed some decline in pH in lower horizons, but most striking was a large increase in soil nitrogen for all horizons and soil types.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00476907
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  • 16
    Electronic Resource
    Electronic Resource
    Deposition gradients and foliar and soil leachate concentrations of air pollutants in Scots pine stands of S.-E. Finland and the Karelian Isthmus, N.-W. Russia (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1263-1268 
    Details
    ISSN: 1573-2932
    Keywords: air pollution ; sulphur ; nitrogen ; base cations ; throughfall ; Scots pine ; needle elements ; soil leachate ; N.-W. Russia
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Bulk precipitation and throughfall analyses in 50–100-year-old Scots pine stands revealed decreasing sulphur, nitrogen, calcium and magnesium deposition gradients, which extend from the St. Petersburg-Leningrad region and N.-E. Estonia to S.-E. Finland. The Ca and Mg deposition alleviate the acidifying effect of sulphur and nitrogen. The Scots pine canopies acted as a sink for ammonium and nitrate, while the canopy interactions increased sulphur, calcium and magnesium content in throughfall. Foliar S, N and Ca concentrations correlated positively with the corresponding deposition loads. In contrast, low foliar magnesium concentrations were detected in the vicinity of St. Petersburg. The results indicate that the sulphur and calcium deposition may have increased soil leachate S and Ca concentrations in the most polluted Scots pine stands.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00477155
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  • 17
    Electronic Resource
    Electronic Resource
    Cost-Effective Nutrient Reductions to the Baltic Sea (1997)
    Springer
    Environmental and resource economics 10 (1997), S. 341-362 
    Details
    ISSN: 1573-1502
    Keywords: Baltic Sea ; eutrophication ; nitrogen ; phosphorus ; cost effective
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering , Economics
    Notes: Abstract Due to eutrophication caused by heavy loads of nitrogen and phosphorus, the biological conditions of the Baltic Sea have been disturbed: large sea bottom areas without any biological life, low stocks of cods, and toxic blue green algaes. It is recognized that the nitrogen and phosphorus loads to the Baltic Sea must be reduced by 50% in order to restore the sea. The main purpose of this paper is to calculate cost effective nitrogen and phosphorus reductions to the Baltic Sea from the nine countries surrounding the Baltic Sea. The results show a significant difference in minimum costs of decreasing nitrogen and phosphorus loads to the Sea: approximately 12 000 millions of SEK per year and 3 000 millions of SEK respectively for reductions by 50%. It is also shown that a change from a policy of cost-effective nutrient reductions to a policy where each country reduces the nutrient loads by 50% increase total costs for both nitrogen and phosphorus reductions by about 300%. The results are, however, sensitive to several of the underlying assumptions and should therefore be interpreted with much caution.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1026497515871
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  • 18
    Electronic Resource
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    Sulphur and nitrogen deposition in Norway, status and trends (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 623-628 
    Details
    ISSN: 1573-2932
    Keywords: monitoring ; deposition ; sulphur ; nitrogen
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The total deposition of sulphur (S) and nitrogen (N) components in Norway during the period 1988–1992 has been estimated on the basis of measurement data of air- and precipitation chemistry from the national monitoring network. There are large regional variations in depositions with highest values in the southwestern part of Norway. Time series analysis of annual mean concentrations of sulphur dioxide (SO2) and sulphate (SO4 −−) in air, non marine SO4 −−, nitrate (NO3 −) and ammonium (NH4 +) in precipitation, shows a significant reduction in the S concentrations both in air and precipitation. In precipitation the concentrations are reduced by 30–45 percent in Southern Norway and 45–55 percent in Central and Northern Norway. Even larger reductions are observed in air concentrations with 50–65 percent reduction in Southern Norway and 65–88 percent reduction further north. For N components there are generally no significant trends in concentration levels nor in precipitation or air. The observed trends are comparable with reported trends in emission.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00476898
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  • 19
    Electronic Resource
    Electronic Resource
    Soil sensitivity due to acid and heavy metal deposition in East Central Europe (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 737-742 
    Details
    ISSN: 1573-2932
    Keywords: acid deposition ; heavy metals ; cadmium ; soil contamination
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Simultaneous soil acidification and deposition of heavy metals is a major concern for forest and agricultural soils of the Black Triangle region of East Central Europe including southern former East Germany, northern Bohemia of the Czech Republic, and southern Poland. The objective of this project was to develop historical and future projections of acid and heavy metal deposition to soils (As, Cd, Pb, Zn) and to produce a preliminary map of soil sensitivity to cadmium pollution and uptake by crops. Ultimately, we wish to assess the relative hazard and recovery times of soils to metals deposition in the region. Emission and deposition data bases obtained from several models developed at IIASA were linked using the Geographical Information System ARC/INFO to produce soil maps of sensitivity to cadmium mobility based on metals deposition, soil type, soil texture, organic matter content, and acid deposition. RAINS 6.1 (Alcamo et al., 1990) was utilized to produce maps of acid deposition for EMEP grids (150 km x 150 km). The largest amount of acid load is deposited in southern East Germany. Sulfur deposition in that area was 10–12 gS/m2/yr in 1990, and S+N deposition exceeded 8000 eq/ha/yr. But the “hot spot” for metals deposition is further to the east, in the Silesia area of southern Poland. The TRACE2 trajectory model of Alcamo, Bartnicki, and Olendrzynski (1992) was used to estimate cumulative metals deposition since 1955 with scenarios to 2010. Pb has improved over Europe since 1970 when depositions in the Ruhr River Valley of West Germany exceeded 60 mg/m2/yr. But cadmium deposition in southern Poland (Katowice and Krakow) has now accumulated to 60–70 mg/m2 by atmospheric deposition alone. During base case simulations from 1955–87, approximately 1.8 mg/kg Pb and 0.12 mg/kg Cd have been added to the mixed plow-layer of ∼30 cm. If these emissions continue indefinitely, the accumulation of metals will become problematic for agriculture and the food chain.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00476917
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  • 20
    Electronic Resource
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    Perch mercury content is related to acidity and color of 26 Russian lakes (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 823-828 
    Details
    ISSN: 1573-2932
    Keywords: fish ; mercury ; lake chemistry ; biomagnification
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract We determined mercury in fish (perch Perca fluviatilis) from 26 Russian lakes in three regions over four years. The lakes ranged in size from 2 to 395,000 ha, in pH from 4.5 to 10.0, and in color from 3 to 190 hazen. Sixteen lakes were drainage lakes, with permanent outlets, and 10 were seepage lakes, with no permanent inlets or outlets. The lakes were generally located in forested regions with little or no human habitation in the watershed. The three regions were geologically distinct: Precambrian Shield granitic bedrock covered with thin soil; Triassic bedrock covered with thick glacial tills; and Triassic bedrock covered with thin sediments. At each lake water samples were collected and analyzed for pH, add neutralizing capacity (ANC), major cations, and anions. Dissolved mercury species were estimated with a thermodynamic equilibrium model (MINTEQA2). Mercury content of dorsal muscle varied from 0.04 to 1.0 μg/g wet weight, and was linearly related to calculated HgCH3Cl (r20.68, p〈0.001). Lake HgCH3Cl, in turn, was related to lake pH (r2=0.86, p〈0.001). Stepwise multiple regression selected lake HgCH3Cl and color as the factors most highly related to fish mercury content, with the model accounting for 75% of the variation.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00476931
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  • 21
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    Indirect effects of N and S deposition on a Norway spruce ecosystem. An update of findings within the Skogaby project (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1613-1622 
    Details
    ISSN: 1573-2932
    Keywords: Deposition ; ecosystem ; nitrogen ; Norway spruce ; nutrient cycling ; production ; root function ; sulphur
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In this paper we try to interpret results from different investigations where an ecosystem with Norway spruce was manipulated with increased N and S deposition via the soil system. The site, in Skogaby in Southwest Sweden, had 1989–93 an annual deposition of 9 kg NH4-N; 7 kg NO3-N and 20 kg SO4-S ha−1. The stand was treated during 6 years with 100 kg N and 114 kg S ha− y−1 in the form of ammonium sulphate (NS treatment). The stand reacted with increased above ground production of 31% after 3 years of treatment. The uptake above ground of N was 155 kg ha−1 higher than in the control. Those trends were even stronger after 6 years of treatment. There were no decreases in the uptake of P, K, Ca or Mg (but for B) after 3 or 6 years of NS-treatment. Needle macro nutrient concentrations in relation to N decreased for several nutrients due to dilution effects. As result of the NS treatment pH increased markedly in the litter layer, and less, but significantly, in the humus layer. A decrease in pH value by about 0.3 units was found in the rest of the soil profile down to 50 cm. Dry mass of needle litter fall and litter layer both increased as a result of 6 years of NS-treatment. After three years of treatment 77–80% of all living fine roots in both control and NS treatment were found in the humus layer and the upper 10 cm of the mineral soil. The amount of living fine roots in the humus layer of NS-treated trees decreased to about one third of the control, and the amount of dead fine roots increased by 150% compared with untreated trees after 6 years of treatment. It is argued that the decreased amount of living and increased amount of dead fine roots not necessarily are indications of decreased root vitality. It can also be explained by increased root turnover rate and decreased decomposition rates of N rich new and old fine root litter. No inorganic N was leached from the control plots whereas the NS treated plots started to leach NO3 the second year of treatment. During 1989–1993 a total of 44 kg NO3-N and 30 kg NH4-N per ha was lost from the system which means that 88% of the N supplied was retained by the ecosystem. At first SO4 was adsorbed in the soil, but after five years of treatment the output was almost equal to the input.
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    URL: http://dx.doi.org/10.1007/BF00477211
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    Development and application of a reactive plume model for mercury emissions (1995)
    Springer
    Water, air & soil pollution 80 (1995), S. 325-335 
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    ISSN: 1573-2932
    Keywords: Atmospheric chemistry ; mercury ; plume model
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A reactive plume model that includes atmospheric chemical reactions of mercury was developed. The model simulates advective transport with the mean wind flow; horizontal and vertical turbulent diffusion; gas phase; aqueous-phase and particulate chemistry; cloud microphysics; wet deposition and dry deposition. The model was applied to the simulation of clear sky, non-precipitating cloud and precipitating cloud scenarios. No significant mercury chemistry occurs in the absence of droplets. In clouds, Hg(II) is reduced to Hg(0) with more reduction taking place in precipitating clouds than in non-precipitating clouds.
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    URL: http://dx.doi.org/10.1007/BF01189682
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    Denuder-based techniques for sampling, separation and analysis of gaseous and participate mercury in air (1995)
    Springer
    Water, air & soil pollution 80 (1995), S. 1209-1216 
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    ISSN: 1573-2932
    Keywords: gaseous ; particulate ; mercury ; sampling ; silver ; gold ; denuder
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A denuder-based method for sampling and separating gaseous and participate mercury in the air is described. Two different denuder configurations developed in Vilnius, Lithuania (silver) and in Gothenburg, Sweden (gold) are compared. Data were acquired at different sampling locations around the cities of Vilnius and Gothenburg. The concentration of particulate Hg was found to be 0.04 to 0.40 ng m−3 in the Vilnius region, and 0.11 to 0.57 ng m−3 in the Gothenburg region. Intel-calibration results for the silver and gold denuders are presented. The results obtained by the two different denuder configurations and sampling set-ups display satisfactory agreement.
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    URL: http://dx.doi.org/10.1007/BF01189784
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    Acid deposition: Perspectives in time and space (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 15-24 
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    ISSN: 1573-2932
    Keywords: Acid deposition ; global change ; Asia ; fertilizer ; nitrogen ; sulfur
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Most acid-deposition investigations have been concerned with the impact of nitrogen oxides (NOx) and sulfur dioxide (SO2) emissions on Europe and North America. This paper examines three issues beyond this central focus. Major conclusions are 1) ammonia (NH3) emissions and subsequent nitrogen (N) accumulation in terrestrial ecosystems have the potential to generate significant acidification in terrestrial and aquatic ecosystems; 2) sulfur (S) and N accumulation in environmental reservoirs will not only result in significant and extensive acidification but will also impact the earth's radiation balance, tropospheric oxidizing capacity, ecosystem nutrient balance and groundwater quality; and 3) future emissions will substantially increase in the developing world, especially in Asia. By 2020, Asian emissions of SO2, NOx and NH3 will be equal to or greater than the combined emissions from Europe and North America.
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    URL: http://dx.doi.org/10.1007/BF00483685
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    Global forest systems: An uncertain response to atmospheric pollutants and global climate change? (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 101-110 
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    ISSN: 1573-2932
    Keywords: carbon ; nitrogen ; sulfur ; biogeochemistry ; mitigation ; global change
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Forest systems cover more than 4.1×109 ha of the Earth's land area. The future response and feedbacks of forest systems to atmospheric pollutants and projected climate change may be significant. Boreal, temperate and tropical forest systems play a prominent role in carbon (C), nitrogen (N) and sulfur (S) biogeochemical cycles at regional and global scales. The timing and magnitude of future changes in forest systems will depend on environmental factors such as a changing global climate, an accumulation of CO2 in the atmosphere, and increase global mineralization of nutrients such as N and S. The interactive effects of all these factors on the world's forest regions are complex and not intuitively obvious and are likely to differ among geographic regions. Although the potential effects of some atmospheric pollutants on forest systems have been observed or simulated, large uncertainty exists in our ability to project future forest distribution, composition and productivity under transient or nontransient global climate change scenarios. The potential to manage and adapt forests to future global environmental conditions varies widely among nations. Mitigation practices, such as liming or fertilization to ameliorate excess NOx or SOx or forest management to sequester CO2 are now being applied in selected nations worldwide.
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    URL: http://dx.doi.org/10.1007/BF00483692
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    Nutrient balance in Scots pine (Pinus sylvestris L.) forest. 2. Effects of plant growth and N-deposition on soil solution and leachate chemistry in a lysimeter experiment (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1149-1154 
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    ISSN: 1573-2932
    Keywords: forest soil ; leaching ; lysimeter ; nitrogen
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Three years of N application to a Cambic arenosol (Typic Udorthent) in two lysimeter series, one with and one without young saplings of Pinus sylvestris L. have produced significant changes in soil solution and leachate chemistry. An application of 30 kg N/ha*yr−1 significantly increased NO3 − leaching from the soil. This N load was also sufficient to significantly increase the mobility of the phyto-toxic elements Al3+ and Mn2+, likewise to increase leaching of the important plant nutrients Ca2+, Mg2+ and K+. At a N load of 90 kg N/ha*yr−1 significant increase in NH4 + leaching was observed, but total leaching of NH4 + was still very low compared to NO3 − leaching. No significant treatment effects were found for SO4 2−, Fe2+ and Cl− in the leachate. Trees grown in the lysimeters buffered the acidifying effect of N application and increased the leachate pH by 0.2 pH units compared to lysimeters without trees.
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    Effects of nitrogen load to the forest floor in sitka spruce stands (Picea sitchensis) as affected by difference in deposition and spruce aphid infestations (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1173-1178 
    Details
    ISSN: 1573-2932
    Keywords: sitka spruce ; nitrogen ; deposition ; leaching ; proton production ; green spruce aphid
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Studies of biogeochemical cycling and soil acidification have been carried out in even aged stands of Norway spruce, sitka spruce, Douglas fir, beech and oak under the frame of “The Element Cycling Project”. Deposition of excess nitrogen to forests is important as a potential acidifying input. In Denmark, reduced vitality in Norway spruce has promoted extensive planting of sitka spruce. However, several spruce aphid infestations have caused defoliation in many sitka spruce stands. The objectives of this study were to evaluate the effects of deposition and increased litterfall due to spruce aphid infestations on nitrogen transformations in the forest floor in sitka spruce stands on different soil types. The deposition of throughfall nitrogen range from 19 to 35 kg/ha/year. Fluxes of nitrogen in litterfall ranged from 21 to 77 kg/ha/year, whereas nitrogen leaching range from 1 to 57 kg/ha/year. Leaching was lowest at the infertile sites, but increased with magnitude of deposition and aphid infestations. Proton production according to the nitrogen transformations was largest at the fertile site most often affected by infestations. Huge amounts of bird droppings, honey dew and input of easily available nutrients by canopy leaching probably induced litter decomposition and formation of NO 3 − in the soil water.
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    URL: http://dx.doi.org/10.1007/BF00477140
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    Elevational trends in the fluxes of sulphur and nitrogen in throughfall in the Southern Appalachian Mountains: Some surprising results (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2265-2270 
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    ISSN: 1573-2932
    Keywords: atmospheric deposition ; high elevation forests ; foliar uptake ; cloudwater ; nitrogen ; sulphur
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract From 1986–1989, a team of scientists measured atmospheric concentrations and fluxes in precipitation and throughfall, and modeled dry and cloudwater deposition in a spruce-fir forest of the Great Smoky Mountains National Park which is located in the Southern Appalachian Region of the United States. The work was part of the Integrated Forest Study (IFS) conducted at 12 forests in N. America and Europe. The spruce-fir forest at 1740 m consistently received the highest total deposition rates (∼2200, 1200, and 700 eq ha−1 yr−1 for SO4 2−, NO3 −, and NH4 +). During the summers of 1989 and 1990 we used multiple samplers to measure hydrologie, SO4 2−, and NO3 − fluxes in rain and throughfall events beneath spruce forests above (1940 m) and below (1720 m) cloud base. Throughfall was used to estimate total deposition using relationships determined during the IFS. Although the SO4 2− fluxes increased with elevation by a factor of ∼2 due to higher cloudwater interception at 1940 m, the NO3 − fluxes decreased with elevation by ∼30%. To investigate further, we began year round measurements of fluxes of all major ions in throughfall below spruce-fir forests at 1740 m and at 1920 m in 1993–1994. The fluxes of most ions showed a 10–50% increase with elevation due to the ∼70 cm yr−1 cloudwater input at 1920 m. However, total inorganic nitrogen exhibited a 40% lower flux in throughfall at 1920 m than at 1740 m suggesting either higher dry deposition to trees at 1740 m or much higher canopy uptake of nitrogen by trees at 1920 m. Differential canopy absorption of N by trees at different elevations would have significant consequences for the use of throughfall N fluxes to estimate deposition. We used artificial trees to understand the foliar interactions of N.
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    URL: http://dx.doi.org/10.1007/BF01186171
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    Sulphur and nitrogen input to the Ratanica forested catchment (Carpathian Foothills, southern Poland) (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1765-1770 
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    ISSN: 1573-2932
    Keywords: nitrogen ; sulphur ; input ; forested catchment
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The study covers 1991–1994 concentrations of SO2 and NO2 in the air, concentrations of sulphur and nitrogen in bulk precipitation, throughfall and stemflow as well as input of S and N to the Ratanica forested catchment (S. Poland), which is exposed to moderate anthropogenic pollution are presented. There was high input of sulphur (26 kg ha−1) and nitrogen (24 kg ha−1) to the catchment, mainly in NH4+ (18 kg ha−1). The significant contribution of NH4 + connected with intensive agriculture in surrounding fields has led to eutrophication of the ecosystem.
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    URL: http://dx.doi.org/10.1007/BF00477235
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    Biogeochemistry of a forested watershed in the central Adirondack Mountains: Temporal changes and mass balances (1996)
    Springer
    Water, air & soil pollution 88 (1996), S. 355-369 
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    ISSN: 1573-2932
    Keywords: atmospheric deposition ; ecosystem ; hydrology ; nitrogen ; sulfur
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Information on atmospheric inputs, water chemistry and hydrology were combined to evaluate elemental mass balances and assess temporal changes in elemental transport from 1983 through 1992 for the Arbutus Lake watershed. This watershed is located within a northern hardwood ecosystem at the Huntington Forest within the central Adirondack Mountains of New York (USA). Changes in water chemistry, including increasing NO3 − concentrations (1.1 μmol c , L−1 yr-1), have been detected during this study period. Starting in 1991 hydrological flow has been measured from Arbutus Lake and these measurements were compared with predicted flow using the BROOK2 hydrological simulation model. The model adequately (r2=0.79) simulated flow from this catchment and was used to estimate drainage for earlier periods when direct hydrological measurements were not available. Modeled drainage water losses coupled with estimates of wet and dry atmospheric deposition were used to calculate solute budgets. Export of SO4 2− (831 mol c ha−1 yr−1) from the greater Arbutus Lake watershed exceeded estimates of atmospheric deposition in an adjacent hardwood stand suggesting an additional source of S. These large drainage losses of SO4 2− also contributed to the drainage fluxes of basic cations (Ca2+, Mg2+, K+ and Na+). Most of the atmospheric inputs of inorganic N were retained (average of 74% of wet precipitation and 85% total deposition) in the watershed. There were differences among years (56 to 228 mol ha−1 yr−1) in drainage water losses of N with greatest losses occurring during a warm, wet period (1989–1991).
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    URL: http://dx.doi.org/10.1007/BF00294111
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    Chemical characteristics of leachate from pulp and paper mill residuals used to reclaim a sandy soil (1996)
    Springer
    Water, air & soil pollution 89 (1996), S. 167-187 
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    ISSN: 1573-2932
    Keywords: Pulp and paper mill sludge ; nitrogen ; DOC ; heavy metals ; water quality
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Primary sludge, secondary sludge, and wood ash from a pulp and paper mill were combined with sand to create a synthetic topsoil (C:N ratio of 18:1) to restore an abandoned gravel pit. Synthetic topsoil was applied to field microcosms at rates equivalent to 0, 2170, 4341, or 6511 kg N/ha; each was seeded with grass. Fifteen chemical constituents in leachate were measured during two field seasons. Cadmium, Ni and Zn were mobilized rapidly by soil disturbance. Chloride and SO4-S eluted rapidly from the sludge along with Na. Nitrate leached with Ca late in each field season when sludge N-mineralization and nitrification exceeded plant uptake and microbial immobilization. Ammonium elution was negligible. Dissolved organic carbon (DOC) was mobilized by decomposition of organic matter in the sludge, as were Mg and K. Copper eluted with DOC, probably as an organic ligand. Lead and ortho-P were below our detection limits. We concluded that a synthetic topsoil with a 30:1 C:N ratio applied at a rate of 2100-4300 kg N/ha should provide adequate plant nutrition while minimizing water quality hazards.
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    Mercury concentrations in forest trees from Slovakia (1996)
    Springer
    Water, air & soil pollution 89 (1996), S. 267-275 
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    ISSN: 1573-2932
    Keywords: mercury ; forest trees ; biomonitors ; contaminants
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The concentration of mercury has been determined in assimilation organs of forest trees from 10 main industrial regions of Slovakia, four mountain forests and one military area and compared with concentration of mercury from 1356 permanent monitoring plots of Slovakia. The mercury concentration ranges for 2 yr old needles of Picea abies Karst. were (in mg kg−1): 1.249–4.402 (Rudnany iron ore mines), 0.013–0.749 (nine other industrial regions), 0.021–0.737 (four mountain forests) and 0.053–0.538 (military area). The mercury content in the soil (0–5 cm) from a mercury smelting plant ranged from 9.9 to 130 mg kg−1, and the moss Pleurozium schreberi contained 3.8–9.1 mg kg−1. The values obtained were compared with the available literature data.
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    URL: http://dx.doi.org/10.1007/BF00171636
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    Feasibility of a counter-current extraction procedure for the removal of heavy metals from contaminated soils (1996)
    Springer
    Water, air & soil pollution 89 (1996), S. 317-335 
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    ISSN: 1573-2932
    Keywords: Soil remediation ; extraction ; heavy metals
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Effective remediation and sanitation technologies for soils contaminated with heavy metals are limited. We investigated the feasibility of a counter-current metal extraction procedure for the removal of selected heavy metals (Cd, Cu, Ph, and Zn) from two contaminated soils. The process involved a decarbonation (removal of carbonates), acid solubilisation, washing, and liming step. Results from batch equilibration experiments simulating the counter-current process showed more than 85% of the Cd present to be removed. Removal efficiencies for Cu and Pb were limited to approximately 15%, this mainly due to resorption of these elements during the decarbonation step. As most Zn was found to be present in a more difficult acid-extractable solid phase, its extractability accounted for only 25%. While reaction (pH) conditions of both decarbonation and solubilisation determined removal efficiencies, washing the extracted soil with deionized water only slightly increased the amount of metals removed. Metal distribution among solid phases — exchangeable, carbonate, reducible, organically bound, and residual — was affected by the different treatments. The amount of metals contained in the exchangeable and residual fractions determined their extractability. Except for Cu, the reducible and organically bound fractions were less important. After solubilisation 13 to 70% of the metals were present in an exchangeable solid phase. This implicates that washing the solubilized soil with a salt may increase the extractability of metals, especially for Zn and Pb. Based on our results the process is critically evaluated and possibilities for optimization formulated.
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    MODELLING LEACHING OF INORGANIC Hg(II) IN A SCANDINAVIAN IRON-HUMUS PODZOL - VALIDATION AND LONG-TERM LEACHING UNDER VARIOUS DEPOSITION RATES (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 301-320 
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    ISSN: 1573-2932
    Keywords: acid rain ; batch experiment ; Freundlich isotherm ; lysimeter experiment ; mercury ; simulation model
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Increasing mercury contents are reported from freshwater systems and fish in northern Europe and North America. Mercury input from soils is a major source with the leaching being affected by increased atmospheric mercury deposition compared to pre-industrial times and by other environmental conditions such as acid rain. The results of a mathematical model-calculation of vertical inorganic Hg(II) leaching in a Scandinavian iron-humus podzol under different atmospheric input rates of mercury are presented. Leaching under background rain conditions was calculated to be considerably stronger than under acid rain conditions. Increasing fractions of deposited soluble or solute atmospheric mercury were leached from the O f(h)-horizon with decreasing soil content of soluble mercury under acid rain conditions; this effect was less pronounced under background rain conditions. The steady state concentrations of soluble mercury of the upper soil horizons were calculated and compared with the actual concentrations of total (= soluble + insoluble mercury) and extractable (= estimate of soluble) mercury measured in these horizons. The results indicate that even if the deposition of airborne mercury to soil is strongly reduced, the total mercury content of the soil decreases only slowly. It may take decades or even centuries before a new steady state concentration of total mercury is established in the soil. The decrease of the mercury concentration in the O f(h)-horizon is probably largely dependent on the turnover of organic matter, binding most of the deposited airborne mercury in an insoluble form. Hence, present day mercury leaching is likely to be dominated by mercury deposited during former times and temporarily retained in an insoluble form in the organic matter.
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    URL: http://dx.doi.org/10.1023/A:1026476921969
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    The role of humic substances in the aqueous mobilization of mercury from contaminated floodplain soils (1996)
    Springer
    Water, air & soil pollution 90 (1996), S. 507-520 
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    ISSN: 1573-2932
    Keywords: mercury ; foodplains ; humic substances ; complexation ; speciation ; mobilization ; risk assessment ; water solubility
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The water-mobilizability of mercury from contaminated floodplain soils of the river Elbe in Northern Germany was evaluated by batch extraction experiments. It was shown that only a small amount of the total mercury present (about 1% per extraction) can be mobilized by water. This mercury is transported entirely in the form of a complex bound to humic acids (HA); particulates and fulvic acids (FA) did not seem to contribute to the process. It could not be removed from the HA even at pH 1, indicating an extremely strong complexation e.g. by sulfur-containing ligands. Furthermore, the influence of pH on the mobilization was investigated. It was found that in the range of natural pH-values, there was no observable effect of pH on the mobilization of either mercury or dissolved organic carbon (DOC). This surprising finding is explained by an unexpectedly high buffering capacity of the humics, both in the acidic and in the alkaline region. Only at extreme pH-values there was deviation from this behaviour. In contrast to other heavy metals, the amount of mobilized mercury decreases at pH 〈 3; and at pH 〉 12, an increased mobilization of mercury was observed because the humics are mobilized completely, accompanied by the total amount of mercury bound to them.
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    Forms of Cu, Ni, and Zn in soils of sudbury, ontario and the metal concentrations in plants (1996)
    Springer
    Water, air & soil pollution 90 (1996), S. 531-542 
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    ISSN: 1573-2932
    Keywords: heavy metals ; smelting ; soil contamination ; plant contamination
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Forms of Cu, Ni, and Zn in the contaminated soils of the Sudbury mining/smelting district were studied to assess metal mobility and plant availability. Soil, tufted grass (Deschampsia caespitosa (L.) Beauv.), tickle grass (Agrostis scabra Willd.), dwarf birch (Betula pumila L. var. glandulifera Regel) and white birch (Betula paprifera Marsh.) leaf and twig samples were taken from 20 locations around three Cu-Ni smelters. The sampling sites were collected to cover a wide range of soil pH and soil Cu and Ni concentrations. The water-soluble, exchangeable, sodium acetate-soluble, and total concentrations of the metals in the soils were analyzed. The soils were contaminated with Cu and Ni up to 2000 µg g−1. Zinc concentrations were also elevated in some samples above the normal soil level of 100 µg g−1. The mobility of Cu and Zn, expressed as the proportion of metals in Fl and F2 forms, increased with soil pH decrease. A strong positive correlation was found between the soil exchangeable (F2) Ni and the soil pH. Concentrations of Cu and Ni in birch twigs showed a good linear relationship with exchangeable forms of the metals in soils. A highly significant correlation was also found between total Ni in soils and the metal content of the twigs. No significant correlation was found between Zn concentrations in the soils and plants. Birch twigs are a good indicator (better than leaves) of Cu and Ni contamination of the Sudbury soils. The mobile forms of Cu and Ni and low pH seem to be the main factors that will control the success of revegetation. Strong variability of the soil metal mobility requires any reclamation effort be site-specific.
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    URL: http://dx.doi.org/10.1007/BF00282667
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    Solubility of heavy metals in a contaminated soil: Effects of redox potential and pH (1996)
    Springer
    Water, air & soil pollution 90 (1996), S. 543-556 
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    ISSN: 1573-2932
    Keywords: heavy metals ; solubility ; redox potential ; pH ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract To assess the mobilities of Pb, Cd, and Zn from a contaminated soil, the effects of redox potential and pH value on metal solubilities were investigated. Both redox potential and pH were found to greatly affect heavy metal solubility in the soil. Results showed that the soil suspension under continuous oxygen aeration for 21 days resulted in increases of redox potential from 290 to 440 mV and pH value from 6.9 to 7.0, respectively. Soluble concentrations of Pb, Cd, and Zn varied with time, and were all lower than 1 mg kg−1. When the soil suspension was aerated with nitrogen, final redox potential was −140 mV and pH value of 7.1. The soluble metal concentrations were slightly higher than those aerated with oxygen. The equilibrium solubility experiments were conducted under three different pH values (3.3, 5.0, 8.0) and three redox potential (325, 0, −100 mV). Results showed that metals were sparingly soluble under alkaline conditions (pH = 8.0). Metal solubilities were higher when under slightly acidic conditions (pH = 5.0), and increased drastically when pH was kept at 3.3. When solubilities were compared under same pH values, it was observed that metal solubilities increased as redox potential decreased. Generally speaking, acidic and reducing conditions were most favorable for metal solubilization, and the effect of pH was more significant than that of redox potential. It was proposed that heavy metals were mostly adsorbed onto Fe-Mn oxyhydroxides. The pH-dependent metal adsorption reaction and the dissolution of Fe-Mn oxyhydroxides under reducing conditions was the mechanism controlling the release of heavy metals from soils.
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    URL: http://dx.doi.org/10.1007/BF00282668
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    Global mercury pollution and the role of gold mining: An overview (1997)
    Springer
    Water, air & soil pollution 97 (1997), S. 205-207 
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    ISSN: 1573-2932
    Keywords: mercury ; gold mining ; ecosystems ; methyl-Hg ; cycling ; global sources
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract As described by Jemelov and Ramel (1995), the Scientific Committee on Problems of the Environment (SCOPE) sponsored an investigation of Hg in ecosystems with special emphasis on tropical regions. In these regions small-scale gold mining activities have occupied about 10 million people worldwide who use Hg for extracting gold.
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    Determination of atmospheric mercury during the North sea experiment (1997)
    Springer
    Water, air & soil pollution 97 (1997), S. 257-263 
    Details
    ISSN: 1573-2932
    Keywords: mercury ; atmosphere ; rainwater ; marine
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Total gaseous mercury (TGM) and rainwater were collected on board of two research vessels (F. S. ALKOR and R.V. BELGICA) positioned 200 km apart in the center of the North Sea during the North Sea Experiment, September 1991. On the F. S. ALKOR (up-wind ship) TGM concentrations ranged from 0.7 to 2.6 ng·m−3 with an average of 1.5 ng m−3 and on the R. V. BELGICA (down-wind ship) TGM ranged from 0.7 to 1.9 ng·m−3 with an average of 1.2 ng·m−3. An average 20% decrease is observed from the up-wind to the down wind ship. which may largely be affected by entrainment into the free troposphere. An overall removal (entrainment) velocity of 0.95 cm·s−1 was calculated for the whole experiment. The average removal velocity was 0.5 cm·s−1 for dry periods and varied between 1 to 5 cm·s−1 during rain events. Rainwater concentrations varied between 5 and 25 ng·1−1. Based on these data an annual wet deposition flux of 1.08 ng Hg cm−2 yr1− was estimated for the North Sea.
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    URL: http://dx.doi.org/10.1007/BF02407464
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    Sediment Accumulation of Nutrients (N, P) in the Eastern Gulf of Finland (Baltic Sea) (1997)
    Springer
    Water, air & soil pollution 99 (1997), S. 477-486 
    Details
    ISSN: 1573-2932
    Keywords: sediment ; nitrogen ; phosphorus ; organic matter ; cluster analysis ; Gulf of Finland ; estuaries
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Dry weight (DW), ignition loss (IL) and concentrations of total nitrogen (TN) and total phosphorus (TP) of the sediment surface layer (0 to 10 cm, 1 cm slices) were analyzed from 20 sites in the eastern Gulf of Finland. The distance of the sampling sites from the mouth of the River Neva explained the nutrient concentrations of the sediments well, while the effect of water depth was negligible. The increase of TN and the decrease of TP along the transect from the river mouth towards the open Gulf were caused by the diminishing share of allochthonous material supplied from the River Neva. The mean TN concentration of the different accumulation areas was about 40 % higher in the sediment surface than in the deeper layer (9 to 10 cm). The corresponding difference for TP varied from 53 to 56 %. The results suggest considerable netflux of nutrients from sediment to water. The net sediment accumulation of nutrients were estimated as 6.0 g m-2 a-1 of N and 1.7 g m-2 a-1 of P corresponding 22 000 t a-1 of N and 6 100 t a-1 of P for the whole eastern Gulf.
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    URL: http://dx.doi.org/10.1023/A:1018399625103
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    Sulphur and heavy metal concentrations in Scots pine bark in northern Finland and the Kola peninsula (1997)
    Springer
    Water, air & soil pollution 93 (1997), S. 395-408 
    Details
    ISSN: 1573-2932
    Keywords: air pollution ; pine bark ; sulphur ; pH ; conductivity ; heavy metals
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Sulphur and heavy metal deposition in northern Finland (= in Lapland) and the Kola Peninsula were surveyed using Scots pine bark samples. Sulphur concentrations in bark close to the Kola smelters were on an average twice as high as on the Finnish side of the border. The Cu and Ni concentrations near the smelters were almost 100-fold the mean values in northern Finland. There was a marked decrease in the sulphur and heavy metal concentrations with increasing distance from the emission sources. The effects of emission from the Kola Peninsula were evident in Finland only close to the border, especially in the eastern parts of Inari (NE corner of Lapland) where the Cu and Ni concentrations were 2- to 6-fold those in western Lapland. The sulphur and heavy metal concentrations in most of northern Finland were low. However were the concentrations of Cr in bark in the SW corner of Lapland considerably high, due to the emissions from the Tornio refined steel plants.
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    The influence of heavy metals on carbon dioxide evolution from a typic xerochrept soil (1997)
    Springer
    Water, air & soil pollution 93 (1997), S. 409-417 
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    ISSN: 1573-2932
    Keywords: CO2 evolution ; heavy metals ; loading effect ; metal equivalent
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In a laboratory study the effects on soil respiration of trace metals (Ni, Cd, Cu, Mn, Pb, Zn) added at loading rates ranging from 0 to 1000μg g−1 were determined. Differences in toxicity with respect to the type of metal salt added were also evaluated. The inhibitory effect on soil respiration differed considerably among the heavy metals and increased with the increasing loading rate. No linear relationships were found between the degree of inhibition and the levels of total and available metals. Toxicity evaluation at 20 and 50% inhibition of soil respiration showed Cu as the most toxic and Mn as the most tolerable metal. A ‘metal equivalent’ was calculated as the sum of the amounts of the available metals weighted to their relative toxicity with respect to the least toxic one: Mn equivalent=Mn+1.9Pb+2.1Ni+2.5Zn+6.7Cd+6.7Cu. The ionic potential of the heavy metals was found to be positively related to the percent inhibition of soil respiration. Chlorides and sulphates appeared to depress soil respiration more than nitrates, the latter counter-balancing the toxic effect of the heavy metals.
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    HEAVY METAL CONTAMINATED SOILS IN AN OLD INDUSTRIAL AREA OF WALES, GREAT BRITAIN: SOURCE IDENTIFICATION THROUGH STATISTICAL DATA INTERPRETATION (1997)
    Springer
    Water, air & soil pollution 94 (1997), S. 85-98 
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    ISSN: 1573-2932
    Keywords: soil ; pollution ; heavy metals ; smelters ; factoranalysis
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A combined statistical and computergraphic approach is proposed for apportionment and attribution of soil contaminants in complex areas. The field test site lies north of Swansea, south Wales and contains two major pollutant sources, an active nickel refiner and (4 km away) the site of major base metal smelting in the nineteenth century (the Lower Swansea Valley reclamation study area). Soil samples (70 samples, 0–15 cm) were collected on a regular grid of 1000 m interval. They were extracted using 0.05 M diammonium EDTA and the extracts analysed for Cd, Co, Cu, Fe, Mn, Ni, Pb and Zn. Soil pH and %organic content were also determined. Factor analysis yielded three groups which explained 73.8% of the data variance (1: Cd, Cu, %OM, Pb, Zn, Ni; 2: Cd, Zn, Mn, pH; 3: Cu, Mn, Co, Ni, Fe). Isoline plots were classifiable into the same three groups. It was concluded that factor 3 contained those elements associated with smelter emissions, factor 1 with contamination from the Lower Swansea Valley and in factor 2 pedogenetic processes control the occurrence of the elements.
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    URL: http://dx.doi.org/10.1023/A:1026478427782
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    TOTAL MERCURY AND METHYLMERCURY IN SEDIMENTS AND IN THE POLYCHAETE NEREIS DIVERSICOLOR AT GROOT BUITENSCHOOR (SCHELDT ESTUARY, BELGIUM) (1997)
    Springer
    Water, air & soil pollution 94 (1997), S. 109-123 
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    ISSN: 1573-2932
    Keywords: mercury ; methylmercury ; sediment ; polychaete ; Nereis diversicolor ; methylation ; bioaccumulation ; Scheldt estuary
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Total mercury (Hg) and methylmercury (MeHg) concentrations were determined in sediments and in the polychaete worm Nereis diversicolor at 13 stations of a brackish water intertidal mudflat of the Scheldt estuary. Hg and MeHg concentrations in sediments ranged from 144 to 1192 ng g−1 dw and from 0.8 to 6 ng g−1 dw, respectively. Both Hg and MeHg concentrations increased with an increase of organic matter (OM) content and fine grain fraction. In contrast, Hg accumulation by N. diversicolor was significantly (p 〈 0.05) higher at stations with sandy sediments (mean value: 125 ng g−1 dw) than at stations with muddy sediments (mean value, 80 ng g−1), probably because Hg availability for bioaccumulation at muddy stations was reduced by high OM content of the muddy sediments. MeHg accounted for an average of 0.7% of the total Hg in sediments and 18% of the total Hg in N. diversicolor. Seasonal variations significantly affected Hg concentrations in sediments and MeHg in N. diversicolor. Total Hg concentrations in sediments were significantly (p 〈 0.05) higher in autumn and winter than in spring and summer whereas MeHg concentrations were lowest in winter compared to the other seasons. On the other hand, total Hg concentrations in the worms were lowest in spring whereas MeHg concentrations were significantly (p 〈 0.01) higher in spring and summer than in autumn and winter.
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    Comparison of two reagents, sodium pyrophosphate and sodium hydroxide, in the extraction of labile metal organic complexes (1997)
    Springer
    Water, air & soil pollution 99 (1997), S. 217-223 
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    ISSN: 1573-2932
    Keywords: selective leach ; organic ; humic ; fulvic ; analysis ; mercury ; zinc
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The international reference lake sediment, LKSD-4, was used to compare Hg, organic C and Zn extracted from its ‘soluble organic’ phase by two commonly used reagents: 0.1 M Na4P2O7 solution at pH 10 and 0.5 M NaOH solution at pH 12. While recoveries of Hg and Zn by 0.1 M Na4P2O7 are not affected by changes in sample weight to reagent volume ratio (W/V) or contact time, those by NaOH show a marked dependency. In general, the NaOH leach extracts more organic C and Hg from LKSD-4 but less Zn. Over the range of conditions studied, the NaOH-based method extracted 4.7–9.8% C, 27–103 ng g−1 Hg and 19–69 μg g−1 Zn from LKSD-4, compared to 2.3–2.8% C, 17–24 ng g−1 Hg and 64–72 μg g−1 Zn by the Na4P2O7 leach. Clearly, different groups of organic substances are being dissolved by these two reagents and therefore a comparison of data from different laboratories becomes meaningless. This paper suggests that more research is needed into the exactNature of metal-organic associations extracted by selective leaches and into associated artifacts of extraction such as readsorption phenomena.
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    Pollutant exchange at the water/sediment interface in the venice canals (1997)
    Springer
    Water, air & soil pollution 99 (1997), S. 255-263 
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    ISSN: 1573-2932
    Keywords: heavy metals ; sediments ; pollution ; resuspension ; release processes ; bioavailability ; anthropogenic ; metal ; residual inetal ; geochemical phases
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The space-time distribution of some pollutants (Cu, Ph, Zn, Cd, Fe, Mn, V, Ni, Cr) in the sludge of the canals of Venice was studied. The contamination levels were comparable to, or higher, than those measured in the most polluted sediments of the Lagoon of Venice Sediments were collected by two different sampling techniques I ) collection of sediment cores (upper 5 cm) by a syringe-type corer, 2) collection by traps, placed on the bottom of the canal Traps pennitted the sampling of sediments essentially resuspended by overlying water turbulence This sediment fraction is subjected to variations of its physicochemical parameters (principally change of redox conditions) and therefore to pollutant exchange at the water/sediment interface The metals principally exchanged during sediment resuspension were Cd, Pb, Zn and Cu These metals have principally an anthropogenic origin and are bound to the most labile geochemical phases of the sediment (such as sulphides), which can be oxidised during sediment resuspension, releasing metals into the water Fe, Cr and Ni were only partially exchanged, while Mn and V were generally not exchanged, a significant fraction of these metals is of natural origin and is bound to the most refractory phases of the sediment.
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    Benthic fluxes of dissolved inorganic carbon, nutrients and oxygen in the Gulf of Trieste (Northern Adriatic) (1997)
    Springer
    Water, air & soil pollution 99 (1997), S. 305-314 
    Details
    ISSN: 1573-2932
    Keywords: Adriatic Sea ; nutrients ; benthic fluxes ; carbon ; nitrogen ; silicon ; phosphorus ; budgets
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Benthic fluxes of dissolved inorganic N, Si and P nutrients, alkalinity, dissolved inorganic C (DIC), and O2 from sediments in the Gulf of Trieste (northern Adriatic, Italy) were measured monthly in the period September 1995 – August 1996 using in situ incubated light benthic chambers. The highest efluxes of DIC, NH4 +, PO4 3−, Si(OH)4, and NO3 − influxes encountered in late summer — early autumn were the consequence of degradation of benthic microalgae, and in autumn mostly of sedimented phytoplankton. High NO3 − efflux was observed in spring. Only NH4 + and Si(OH)4 fluxes were significantly correlated with temperature. This correlation suggests that the rate of downward input and the quality and quantity of sedimentary organic matter (autochthonous and allochthonous) were superimposed on the temperature fluctuations. High DIC, NH4 + and Si(OH)4 effluxes observed in July 1996 were due to the late spring — early summer degradation of sedimentary organic matter produced by benthic microalgae, while the autumn phytoplankton bloom was quickly reflected in enhanced benthic fluxes due to higher temperature. Significant correlations between NH4 +, PO4 3− and Si(OH)4 fluxes suggested their parallel regeneration and utilization at the sediment-water interface. The nutrient fluxes were linked to O2 consumption, suggesting that aerobic oxidation processes were important at the sediment-water interface in the Gulf. The N, P and Si nutrients released from sediment pore waters are probably utilized in benthic microalgal and bottom-water primary production. This indicates that pelagic and benthic communities in the central part of the Gulf of Trieste function relatively independently of each other.
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    LONG-TERM TRANSFORMATIONS AND REDISTRIBUTION OF POTENTIALLY TOXIC HEAVY METALS IN ARID-ZONE SOILS INCUBATED: I. UNDER SATURATED CONDITIONS (1997)
    Springer
    Water, air & soil pollution 95 (1997), S. 399-423 
    Details
    ISSN: 1573-2932
    Keywords: fractionation ; redistribution ; saturation ; kinetics ; heavy metals
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Solid-phase transformations of Cd, Cu, Cr, Ni and Zn, added as soluble salts at several levels to two arid-zone soils, were studied over a period of one year. The soils were maintained under a saturated-paste regime and sampled periodically. A selective sequential dissolution procedure was employed to determine the changes in metal distribution among six operationally defined solid-phase fractions. A function, Uts was introduced to measure the fractional attainment of equilibrium of the soils following a perturbation. The direction and rate of redistribution of the added metals in the soils were affected by the nature of the metal, the soil properties and the metal loading level. Cd added to the soils was transferred from the exchangeable (EXC) into the carbonate (CARB) fraction. When soluble Cu, Cr, Ni and Zn were added at low loading levels, metals were transferred from the reducible oxides(RO) bound and easily reducible oxides (ERO) bound fractions and the EXC fraction, into the CARB fraction. However, at the higher loading level, metals were transferred from the EXC and CARB fractions into the organic matter bound (OM), ERO and RO fractions. The Uts function approached lower values as incubation continued but remained removed from 1. The overall flux of metals among fractions was the combined result of the readjustment of the metals in the native soil to changing conditions due to saturation, and the transfer of added soluble metals to the less labile fractions.
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    Effect of copper smelting air pollution on the mites (ACARI) associated with young scots pine forests polluted by a copper smelting works at Głogów, Poland. II. Soil mites (1997)
    Springer
    Water, air & soil pollution 97 (1997), S. 287-302 
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    ISSN: 1573-2932
    Keywords: Acari ; bioindicators ; Gamasida ; heavy metals ; Oribatida ; Scots pine forest
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The soil mites were investigated in the areas covered with dead needles in young Scots pine forests (plant associationLeucobryo-Pinetum), polluted by a copper smelting works at Głogów, and in a control plot. The concentration of heavy metals, mainly copper and lead, was the lowest in the control plot, and increased towards the pollution source. A high concentration of these metals reduced the density of mites and species number of Oribatida and Gamasida, while small concentrations were associated with the increasing abundance of mites and species number of Oribatida. Among mites, the following categories were distinguished: a) sensitive to heavy metals, b) sensitive to a high concentration, but tolerant of small concentrations, and c) tolerant of these metals. The changed vertical distribution of mites in the most polluted soil was also observed, due to accumulation of heavy metals in the Of/h horizon.
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    Monitoring nitrogen pollution from sugarcane runoff using15N analysis (1997)
    Springer
    Water, air & soil pollution 98 (1997), S. 389-399 
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    ISSN: 1573-2932
    Keywords: fertilizer ; nitrogen ; pollution ; runoff ; stable isotopes ; sugarcane
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In many forested wetlands of Louisiana, surface water quality is being deteriorated by nutrient input from adjacent agricultural production area. This field study assesses the input of fertilizer N, applied to sugarcane fields, to forested wetlands. The potential use of natural abundance variations in15N/14N ratios for identification and tracing surface water N sources (NH 4 + - and NO 3 − -N) was evaluated. Runoff and surface water samples were collected from sugarcane fields and bordering forested wetlands (6 stations) over a 16 month period and analyzed for NH 4 + -N, NO 3 − -N, and associated NH 4 + -δ 15N and NO 3 − -δ 15N ratios. FertilizerN draining into adjacent forested wetland was estimated to be only a small fraction of the amount applied. Concentrations of NH 4 + - and NO 3 − -N in the collected water samples were low and ranged from 0.02 to 1.79 mg L−1. Isotopic analysis revealed NH 4 + -δ 15N and NO 3 − -δ 15N means were distinctive and may have the potential to be used as tracers of N contamination. The mean NH 4 + -δ 15N value was +18.6±7.1‰ and the NO 3 − -δ 15N mean was +8.3±3.1‰. Anomalously high NO 3 − -δ 15N values (〉30‰) were attributed to denitrification.
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    Accumulation of inorganic and organic pollutants by biofilms in the aquatic environment (1997)
    Springer
    Water, air & soil pollution 99 (1997), S. 651-659 
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    ISSN: 1573-2932
    Keywords: River sediments ; biofilms ; organic micropollutants ; heavy metals ; temporal variations ; biosorption ; accumulation processes
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In a partly urbanized catchment to the south of Trier, Germany, short term variations in river sediment compounds as well as the bioaccumulation of pollutants on surface associated microbial coatings (biofilms) were investigated weekly during a period of six months. Concentrations of selected heavy metals (Cu, Zn, Pb), polycyclic aromatic hydrocarbons (PAH), polychlorinated biphenyls (PCB) and for microbial characterisation protein, carbohydrate and uronic acid were analyzed. Sorption processes on biofilms were determined by temporal variations in pollutants and microbial parameters and through the comparison of sorbed substances in biofilms and sediments. The results show, that sorption events on biofilms play an important and dynamic role in spring and summer for transport and accumulation of the investigated pollutants in the aquatic environment. The amount of pollutants sorbed on sediment particles is not only dependent on the particulate bound or solved pollutants in the river water, but is strongly controlled by the changing conditions of the biofilms.
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    The Influence of Age on Cadmium Concentrations in Seabirds (1998)
    Springer
    Environmental monitoring and assessment 50 (1998), S. 159-171 
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    ISSN: 1573-2959
    Keywords: age ; biomonitoring ; heavy metals ; seabirds
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The effects of age on cadmium concentrations was investigated in Cory's shearwater, Calonectris diomedea, Lesser black-backed gull, Larus fuscus, and great skuas, Catharacta skua. There was no evidence for the continued accumulation of cadmium with increasing adult age. Adult shearwaters did have higher concentrations of cadmium compared to young fledglings, but there was no significant difference between cadmium concentrations in adult and sub-adult gulls. In addition, the sample of great skuas were of known age (3–22 yrs old) and showed no evidence of increasing cadmium concentrations with adult age in liver or kidney. However, it is possible that age accumulation of cadmium in great skuas was masked by individual dietary preferences overriding the effects of increasing age. It is often assumed that cadmium concentrations continue to accumulate with increasing adult age, but seabirds may have evolved some as yet unknown mechanism for excretion or more rapid turnover of cadmium than previously thought. The implications of this for the use of seabirds as biomonitors is discussed.
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    Studies on the Uptake of Heavy Metals by Various Plant Species on Chromite Minespoils in Sub-tropical Regions of India (1999)
    Springer
    Environmental monitoring and assessment 55 (1999), S. 389-399 
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    ISSN: 1573-2959
    Keywords: accumulation ; heavy metals ; mine spoils ; vegetation ; soil-plant relationships
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The presence of heavy metals (Cr, Ni and Fe) in soil and accumulated by herbs, shrubs and trees regenerated naturally on the minewaste-dumps of Sukinda chromite mines (TISCO sector) were investigated. There was significant correlationship between Cr and Fe in the soil where a tree species (Catunaregam spinosa) occurred. Guazuma ulmifolia and Diospyros montana also did show significant correlation between leaf, stem and soil for Cr, Ni and Fe. Among the shrubs (Calotropis gigantea, Chromolaena odorata, Phyllanthus reticulatus and Woodfordia fruticosa) significant and positive correlations were obtained for Cr and Ni in soil and iron and nickel in leaf and chromium and nickel in stem. Among the annual herbs, whole plant of tephrosia purpurea and Borrevia articularis showed significant and positive correlation with chromium and nickel with the maximum correlation coefficient value. It was concluded that the above information would be useful in revegetation programmes in subtropical regions having seasonal rainfall.
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    Metals in Feathers of Bonin Petrel, Christmas Shearwater, Wedge-Tailed Shearwater, and Red-Tailed Tropicbird in the Hawaian Islands, Northern Pacific (1999)
    Springer
    Environmental monitoring and assessment 59 (1999), S. 343-358 
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    ISSN: 1573-2959
    Keywords: birds ; environmental pollutants ; heavy metals
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Levels of environmental pollutants are usually higher in mainland and coastal areas than in offshore or oceanic islands due to higher inputs from agricultural and industrial sources. Levels of heavy metals are usually higher in adult than in young birds, because they have had longer to accumulate metals in their tissues, and/or because they may eat larger, more contaminated, prey. We examined the levels of arsenic, cadmium, chromium, lead, manganese, mercury, and selenium in the adults and young of Bonin petrel (Pterodroma hypoleuca), Christmas shearwater (Puffinus nativitatis) and red-tailed tropicbird (Phaethon rubricauda) on Midway Atoll, and adult wedge-tailed shearwater (Puffinus pacificus) on Midway Atoll and on Manana Island (off Oahu) in the northern Pacific. All birds were analyzed individually except for Christmas Shearwater chicks where samples were pooled to obtain sufficient quantities for analysis. Significant (p〈0.05) age-related differences were found for mercury, selenium, manganese and chromium in Bonin petrels, for selenium and mercury in Christmas shearwaters, and for chromium and mercury in Red-tailed Tropicbirds. Lead approached significance for all three species. Adults had higher levels than young except for chromium and manganese in the petrels and arsenic in all three species. There were significant interspecific differences in concentrations of all metals except arsenic for the adults nesting on Midway. Christmas shearwaters had the highest levels of all metals except mercury and chromium. Bonin petrels, the smallest species examined, had mercury levels that were over three times higher than any of the adults of the other three species. For wedge-tailed shearwaters, levels of chromium and lead were significantly higher, and manganese and selenium were lower on Midway than Manana. Knowledge of the foraging ranges and habits of these far-ranging seabirds is inadequately known, but does not currently explain the observed differences among species. We could not find a consistent pattern of differences between the burrow nesting species (Bonin petrel, Wedge-tailed shearwater) and the surface nesting tropicbirds. There was no consistent pairwise correlation between any metals across all species.
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    Heavy Metal Tolerance in Chromogenic and Non-Chromogenic Marine Bacteria from Arabian Gulf (1999)
    Springer
    Environmental monitoring and assessment 59 (1999), S. 321-330 
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    ISSN: 1573-2959
    Keywords: agar diffusion assay ; Arabian Gulf ; chromogenic bacteria ; heavy metals ; toxicity
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A simple method – direct agar diffusion assay – was optimised for rapid assessment of heavy metal toxicity to marine chromogenic and non-chromogenic bacteria. The procedure involved spotting of a 10 microliter test solution on the seeded agar plate and incubation of the plates at 30°C to accelerate bacterial growth. Under optimum conditions, test results were obtainable within 12–18 hr instead of 96 hr incubation time generally required for a marine bacterial assay by conventional agar plate methods. A range of sixteen heavy metals, each at 5 different concentrations was tested. Toxicity was demonstrated by the formation of a clear zone of growth inhibition around the point of application. Toxicity of tested chemicals could be easily demonstrated at concentrations as low as 0.1 μg per spot on the agar plate. A dose dependent relation between metal concentration (μg/spot) and the diameter of the clear zone on agar plate was observed, suggesting potential of this method as an easy and economical tool in quantitative toxicology studies.
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    Mercury dynamics in young Common Tern (Sterna hirundo) chicks from a polluted environment (1993)
    Springer
    Ecotoxicology 2 (1993), S. 33-40 
    Details
    ISSN: 1573-3017
    Keywords: mercury ; body distribution ; feather concentrations ; body burden ; tern chicks
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: We studied mercury concentrations and amounts in tissues of 19 starved young Common Tern chicks (median age 4 days) and in eggs from the same colony. Concentrations and burden were similar between eggs and newly hatched chicks. Mercury concentrations were highest in down, which contained at least 38% of the body mercury. The mercury burden of the whole body and of the tissues as well as the concentration in down increased with age and body mass, indicating the importance of down as an elimination pathway. Conversion ratios between mercury concentrations in tissues and the whole chick body varied according to the contamination level.
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    URL: http://dx.doi.org/10.1007/BF00058212
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    Allozymes Reflect the Population-Level Effect of Mercury: Simulations of the Mosquitofish (Gambusia holbrooki Girard) GPI-2 Response (1998)
    Springer
    Ecotoxicology 7 (1998), S. 141-150 
    Details
    ISSN: 1573-3017
    Keywords: fish ; mercury ; natural selection ; allozyme ; population
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Measurements of the differential tolerance between enzyme genotypes and shifts in allozyme frequencies in populations from contaminated habitats have prompted the use of allozymes as markers of population-level toxicant effects. However, such studies often do not consider other factors that influence allele frequencies, including natural clines, migration, the intensity and specificity of selection and toxicant-induced genetic bottlenecks. In addition, selection components other than survival are not included. Consequently, the associated conclusions remain speculative. To assess this approach rigorously, a simulation study was conducted with the mosquitofish (Gambusia holbrooki) GPI-2 locus. Laboratory studies have shown the GPI-238/38 homozygote at this locus to be less tolerant than other genotypes during acute exposure to mercury. The GPI-2100/100 genotype has also been shown to have a reproductive disadvantage at lower mercury concentrations. Simple and then more complex models were used to quantify the relative effects of viability selection, random genetic drift and migration on the GPI-238 allele frequency. Simulations were also performed to assess the contribution of sexual and fecundity selection. A simple population model suggested that viability selection plays a greater role than does mortality-driven, genetic drift in the decrease of the sensitive allele under the conditions of this study. A more complex, stochastic model indicated that no significant mortality-driven drift was taking place in this system. In both models, migration mitigated the effect of selection. Sexual and fecundity selection had little effect on the allele frequencies in these simulations. We conclude that, provided the system under study is clearly understood, shifts in allele frequency can indicate the population-level effects of pollutants.
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    URL: http://dx.doi.org/10.1023/A:1014352226686
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    Litter decomposition and nitrogen mineralization in oak stands along an urban-rural land use gradient (1997)
    Springer
    Urban ecosystems 1 (1997), S. 117-131 
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    ISSN: 1573-1642
    Keywords: decomposition ; heavy metals ; litterbags ; nitrification ; nitrogen mineralization ; urbanization
    Source: Springer Online Journal Archives 1860-2000
    Topics: Architecture, Civil Engineering, Surveying , Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract We investigated litter mass loss and soil nitrogen (N)-transformation rates in oak stands along a 130-km, urban-rural transect originating in New York City to examine the relationship between changes in these parameters and previously documented differences in soil temperature, heavy metal and total salt concentrations, and soil biota. Reference litter from a rural site was placed in litterbags, and rates of mass loss and changes in N concentration in litter residues were measured over a 6-month period. Net N-mineralization and nitrification rates were measured in A horizon soils using laboratory incubations under constant moisture and temperature. Both mass loss (76%) and N release (65%) from litterbags reached their maximum in urban stands, whereas net N-mineralization rates were 2.3-fold higher than in rural A horizon soils. Litter fragmentation by earthworms and higher soil temperatures are potential causes of the higher mass loss rates observed in urban stands. The higher releases of N measured in the urban litterbags could be a result of their faster mass loss rates, exogenous inputs of N from atmospheric deposition, a relatively low heterotrophic demand for N, or a combination of these factors. The results of this study suggest that in comparison with rural stands, urban forests are characterized by comparatively high rates of litter decomposition, and may also be characterized by comparatively high rates of N mineralization. Additional studies are needed to test whether these effects are common to urban environments in general.
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    Sources, sinks, and fluxes of nutrients (N + P) in a small highly modified urban estuary in southern California (2000)
    Springer
    Urban ecosystems 4 (2000), S. 125-144 
    Details
    ISSN: 1573-1642
    Keywords: nitrogen ; phosphorus ; macroalgae ; estuary ; anthropogenic
    Source: Springer Online Journal Archives 1860-2000
    Topics: Architecture, Civil Engineering, Surveying , Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Our objective was to begin to investigate sources, sinks, and flux rates of nitrogen (N) and phosphorus (P) in Famosa Slough, a small (12 ha) highly modified urban estuary in San Diego, California, U.S.A. The hydrology of Famosa Slough has been modified by culverts that dampen tidal influence and seasonal runoff from two urban watersheds, each of which has been implicated as a nutrient source that generates nuisance algal blooms. In 1995 and 1996, the ranges of nutrients measured in the water column were extremely wide; upper values exceeded those in other estuaries identified as eutrophic. Average dissolved inorganic nitrogen ranged from 2 to 250 μM, while dissolved inorganic phosphorus ranged from 〈1 to 15 μM. Nutrient content of the water changed rapidly both spatially and temporally depending on the tides and rainfall. While tidal water dominated this system, especially in the dry season, our results indicate that Famosa Slough's small watershed, not the larger watershed of the San Diego River, was the major source of nutrients during rainfall. Sediment nutrients were also high (∼3 mg N g dry wt−1 and 0.600 mg P g dry wt−1). Short-term flux studies suggest that the large accumulations of opportunistic green macroalgae commonly found in this estuary, and possibly the sediments, may act as a large and rapid sink for nutrients during times of high nutrient supply. We suggest that small, shallow estuaries in urban settings may have more complex and rapid nutrient dynamics than those found in larger systems.
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    URL: http://dx.doi.org/10.1023/A:1011359311384
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    Seasonal and spatial patterns of S, Ca, and N dynamics of a Northern Hardwood forest ecosystem (1992)
    Springer
    Biodegradation 17 (1992), S. 165-189 
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    ISSN: 1572-9729
    Keywords: calcium ; fine roots ; nitrogen ; northern hardwood ; nutrient dynamics ; seasonality ; soils ; sulfur ; vegetation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract Seasonal dynamics of S, Ca and N were examined at the Huntington Forest, a northern hardwood ecosystem in the central Adirondacks of New York for a period of 34 months (1985–1988). Solute concentrations and fluxes in bulk precipitation, throughfall (TF) and leachates from the forest floor, E horizon and B horizon were quantified. Both above and below-ground elemental fluxes mediated by vegetation (e.g. uptake, litter inputs, and fine roots production) were also determined. The roles of abiotic and biotic processes were ascertained based on both changes in solute concentrations through the strata of the ecosystem as well as differences between dormant and growing seasons. Concentrations of SO4 2−, NO3 −, NH4 + and Ca2+ were greater in TF than precipitation. Forest floor leachates had greater concentrations of SO4 2−, NO3 − + NH4 + and Ca2+ (9, 6 and 77 µeq L−1, respectively) than TF. There were differences in concentrations of ions in leachates from the forest floor between the dormant and growing seasons presumably due to vegetation uptake and microbial immobilization. Concentrations and fluxes of NO3 − and NH; were greatest in early spring followed by a rapid decline which coincided with a demand for N by vegetation in late spring. Vegetation uptake (44.7 kg N ha−1 yr−1 ) could account for the low leaching rates of N03 −. Within the mineral soil, changes with soil depth and the absence of seasonal patterns suggest that cation exchange (Ca+) or anion sorption (SO4 2−) are primarily responsible for regulating solute concentrations. The increase in SO4 2− concentration after leachates passed through the mineral soil may be attributed to desorption of sulfate that was adsorbed during an earlier period when SO4 2− concentrations would have been greater due to elevated S inputs.
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    Nitrogen mass balances and denitrification rates in central Ontario Lakes (1993)
    Springer
    Biodegradation 20 (1993), S. 195-212 
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    ISSN: 1572-9729
    Keywords: denitrification ; lake ; mass balance ; nitrogen
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract Nitrogen mass balances for seven unproductive lakes and 20 forested catchments in central Ontario were measured between 1977 and 1989. Average annual lake denitrification rates calculated with the N/P ratio method were strongly correlated with summer anoxic factor (extent of surficial sediment anoxia) whereas denitrification rates calculated with a210Pb sediment N accumulation method were poorly correlated with the anoxic factor suggesting that the N/P method is superior. Substantial denitrification occurred in all lakes — an average of 36% of TN inputs or 75% of the net gain. On a regional area-weighted basis, 67% of bulk atmospheric TN deposition was stored or denitrified terrestrially, 12% was denitrified in lakes, 4% was stored in lake sediments, and 17% was exported from lakes. N/P ratios were generally less in streams than in precipitation suggesting preferential N retention in catchments, whereas the N/P ratios in lake outputs were slightly higher than lake input ratios, suggesting preferential P retention in lakes. This is consistent with the notion that P-limited lakes can exist adjacent to N-limited forests.
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    Effect of nitrogen and phosphorus addition on phenanthrene biodegradation in four soils (1999)
    Springer
    Biodegradation 10 (1999), S. 43-50 
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    ISSN: 1572-9729
    Keywords: biodegradation ; nitrogen ; nutrients ; phenanthrene ; phosphorus
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract Phenanthrene mineralization rates were found to vary widely among four soils; differences in soil nutrient levels was one hypothesis to explain this variation. To test this hypothesis, phenanthrene mineralization rates were measured in these soils with, and without, added nitrogen and phosphorus. Mineralization rates either remained unchanged or were depressed by the addition of nitrogen and phosphorus. Phenanthrene degradation rates remained unchanged in the soil which had the highest indigenous levels of nitrogen and phosphorus and which showed the largest increase in phosphorus levels after nutrients were added. The soils in which degradation rates were depressed had lower initial phosphorus concentrations and showed much smaller or no measurable increase in phosphorus levels after nutrients were added to the soils. To understand the response of phenanthrene degradation rates to added nitrogen and phosphorus, it may be necessary to consider the bioavailability of added nutrients and nutrient induced changes in microbial metabolism and ecology.
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    Nitrogen inputs to a marine embayment: the importance of groundwater (1990)
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    Biodegradation 10 (1990), S. 309-328 
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    ISSN: 1572-9729
    Keywords: estuaries ; groundwater ; nitrogen ; nitrogen cycle ; nitrogen loading
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract We examined the importance of nitrogen inputs from groundwater and runoff in a small coastal marine cove on Cape Cod, MA, USA. We evaluated groundwater inputs by three different methods: a water budget, assuming discharge equals recharge; direct measurements of discharge using bell jars; and a budget of water and salt at the mouth of the Cove over several tidal cycles. The lowest estimates were obtained by using a water budget and the highest estimates were obtained using a budget of water and salt at the Cove mouth. Overall there was more than a five fold difference in the freshwater inputs calculated by using these methods. Nitrogen in groundwater appears to be largely derived from on site septic systems. Average nitrate concentrations were highest in the region where building density was greatest. Nitrate in groundwater appeared to behave conservatively in sandy sediments where groundwater flow rates were high (〉 11/m2/h), indicating that denitrification was not substantially reducing external nitrogen loading to the Cove. Nitrogen inputs from groundwater were approximately 300 mmol-N/m3/y of Cove water. Road runoff contributed an additional 60 mmol/m3/y. Total nitrogen inputs from groundwater and road runoff to this cove were similar in magnitude to river dominated estuaries in urbanized areas in the United States.
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    The anthropic catchment-ecosystem concept: An Irish example (1985)
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    Human ecology 13 (1985), S. 209-240 
    Details
    ISSN: 1572-9915
    Keywords: catchment-ecosystem ; nutrient-budget ; anthropogenic inputs ; nitrogen ; phosphorus ; eutrophication ; agricultural policies
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Ethnic Sciences
    Notes: Abstract The catchment-ecosystem concept is adapted to investigate the nutrient-budget of the highly-modified Colebrooke drainage basin in Northern Ireland. Anthropogenic inputs, mainly manures and fertilizers, account for 86% of the nitrogen and 96% of the phosphorus added to the catchment. These inputs greatly exceed the streamflow outputs, thereby indicating that the flow of nutrients is dominated by agriculture. This is explained by the transformation of traditional mixed farming into more intensive livestock production and is linked to policies encouraging increased agricultural production, amalgamation of farms, afforestation, rural depopulation, and urbanization. Substantial increases in the Nand Poutput of the catchment and further eutrophication of the recipient lake, Lough Erne, are predicted without the implementation of policies to reduce agricultural nutrient losses.
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    Long term effects of enhanced nitrogen deposition on a lowland dry heath in southern Britain (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1701-1706 
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    ISSN: 1573-2932
    Keywords: nitrogen ; heathland ; Calluna vulgaris ; critical load ; growth ; litter production
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Experimental additions of ammonium sulphate to a nitrogen-poor dry heathland have been carried out since 1989. There are four nitrogen treatments: a control (receiving artificial rain only), a low treatment which receives an additional 7.7 kg N ha−1 yr−1, a high treatment receiving 15.4 kg N ha−1 yr−1 and an alternating treatment which receives either the control or the high nitrogen additions, in alternate years. The estimated background deposition at the study site is 13–18 kg N ha−1 yr−1, a value similar to the critical load that has been suggested for the conversion of lowland heath to grassland. Over the past 5 years there have been significant stimulations in shoot growth, flowering, canopy density and litter production. Flowering, in particular, strongly reflects nitrogen additions in the alternating treatment. Current models of the response of dry Calluna heathlaud to enhanced nitrogen deposition suggest that higher tissue nitrogen levels will occur and will be accompanied by heightened sensitivity to secondary stresses. This may in turn lead to canopy breakdown and replacement by grassland. The application of nitrogen at deposition rates only slightly in excess of the critical load over five years has produced small, non-significant increases in shoot nitrogen content. However, there is clear evidence of a large positive effect on shoot growth, flowering, litter production and canopy density of Calluna. The observation of these responses at the application rates used in this study supports the current proposals for critical loads of nitrogen for lowland heaths.
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    Copper in Scots pine forests around a heavy-metal smelter in south-western Finland (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1727-1732 
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    ISSN: 1573-2932
    Keywords: copper ; element flux ; heavy metals ; Pinus ; soil pollution ; understorey vegetation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Distribution and fluxes of copper within Pinus sylvestris stands were studied during 1992–1994 along a heavy-metal pollution gradient in south-western Finland. The stands are situated at distances of 0.5, 4 and 8 km from a copper-nickel smelter that started operating in 1945 at Harjavalta. According to the results, copper concentrations in the soil, in the understorey vegetation and in the trees increased steeply towards the smelter. Almost 50 years' accumulation of heavy metals in the soil has caused direct toxic effects to soil microbes, thus decreasing decomposition and nutrient mineralisation. During the past few years, sulphur and heavy metal emissions from the copper and nickel smelter have been radically decreased. However, the heavy metals which have been accumulating in the soil for decades continue to affect the vegetation for a long time through soil processes. Consequently, long-term accumulation in the soil has to be taken into account when determining the critical loads of forest ecosystems for heavy metals.
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    Reducing the contribution of ammonia to nitrogen deposition across Europe (1995)
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    Water, air & soil pollution 85 (1995), S. 1891-1896 
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    ISSN: 1573-2932
    Keywords: emissions ; nitrogen ; ammonia ; agriculture ; integrated assessment modelling ; abatement strategies
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract European emissions of reduced nitrogen, arising principally from agriculture, are comparable with those of oxidised nitrogen from mobile and stationary combustion sources. It is therefore important to include ammonia emissions in working towards a new protocol on nitrogen under the programme of the UN Economic Commission for Europe on the control of transboundary air pollution. However the nature of the sources and the subsequent atmospheric transport and chemistry are very different from other acidifying pollutants. This paper describes work in hand under the MARACCAS project to compare agricultural activities in different European countries and to assess the applicability and efficacy of potential abatement measures. The aim is to derive abatement costs for each country relating successive emission reductions to the costs of achieving them, to be used by the UN ECE Task Force on Integrated Assessment Modelling (TFIAM) — in particular with our Abatement Strategies Assessment Model, ASAM. The paper will also address the large uncertainties involved in integrated assessment modelling with respect to ammonia, and suggest how these may be allowed for in deriving cost-effective abatement strategies.
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    Critical loads of acidity and nitrogen, based on multiple criteria for different swedish ecosystems (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2375-2380 
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    ISSN: 1573-2932
    Keywords: Critical load ; acidity ; nitrogen ; Norway spruce ; Scots pine ; ground vegetation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The critical loads of acidity and nitrogen has been mapped for Swedish forest soils, using data from the Swedish Forest Inventory. The Swedish critical load map used in negotiations has been based on a number of ecological receptors. For terrestrial ecosystems criteria based on no adverse effect on growth, soil stability and groundwater quality was used. For surface waters, stream and lake biology was used as indicators for setting limits to acidification. A reduction of 75% of the acidity deposition in relation to 1988 is required in order to protect 95% of the forest resource in Sweden from effects of soil acidification. A reduction of 50% of the nitrogen deposition is required to avoid exceedance in more than 5% of the area. The mapping work was carried out by using the PROFILE model.
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    Calculation and mapping of critical loads of s, n and acidity on ecosystems of the Northern Asia (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2395-2400 
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    ISSN: 1573-2932
    Keywords: critical loads ; nitrogen ; sulphur ; northern Asia
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract On the basis of modified simple steady state mass-balance equations, the critical loads for nutrient and acidifying nitrogen as well as for sulphur and acidity have been calculated for various ecosystems of northern Asia using simplified expert-modelling GIS and grid cells 150×150 km. The minimal values of critical loads of nitrogen, CL(N), (〈50eq/ha/yr) were shown for arctic and subarctic ecosystems and the maximal ones (〉300eq/ha/yr) for ecosystems of chernozemic and chernozem-like soils in southern Siberia and the Far East. The minimal values of critical loads of sulphur, CL(S), as well as acidity were shown predominantly in the northern part of east Siberia and in the Kamchatka peninsula and the maximal ones for ecosystems having neutral and alcaline soils. The corresponding exceedances were indicated for many regions of the northern part of Asia with maximal values for regions of Ural mountains, frontery of Kazakhstan, Altai, lower Yenisei river flow, Far East, Sakhalin and South-Kurilean islands.
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    Uncertainty analysis of critical loads for terrestrial ecosystems in Russia (1995)
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    Water, air & soil pollution 85 (1995), S. 2559-2564 
    Details
    ISSN: 1573-2932
    Keywords: uncertainty analysis ; computed critical loads ; nitrogen ; sulpher ; acidity
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The goal of this study is to give a comprehensive and quantitative estimation of the uncertainty of computed in different scale nitrogen (N) and sulphur (S) critical loads (CL) values for terrestrial ecosystems of the Northern Asia, European part and the North-Western regions of Russia. The CL values are used to set goals for future deposition rates of acidifying compounds so that the environment is protected. In this research CL values for terrestrial ecosystems are determined using the expert-modelling geoinformation system (EM GIS) approach. UNCSAM software package is used as the tool for uncertainty analysis. The analysis presented here focuses on the estimation and effect of the input source uncertainties and sensitivities on the CL values in various regions under study. In spite of the region, nitrogen uptake by vegetation, nitrogen leaching from terrestrial ecosystems and the difference between deposition and uptake by plants of base cations (BC) are the most influential factors for all terrestrial ecosystems of Russia.
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    Spatial variability in emissions reduction strategies for sulphur and nitrogen in the UK (1995)
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    Water, air & soil pollution 85 (1995), S. 2619-2624 
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    ISSN: 1573-2932
    Keywords: sulphur ; nitrogen ; critical loads function ; emissions reductions
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The roles of sulphur (S) and nitrogen (N) in causing critical loads exceedance across the UK show considerable spatial variability at the present time. Over much of lowland Britain it appears that the environment can only be protected by reducing N deposition, whilst in upland areas (e.g. most of Scotland and Wales) reductions in S deposition are the primary requirement. Using the Hull Acid Rain Model (HARM) the effects of current and possible future emissions control legislation on critical loads exceedance can be explored. Based on HARM output, the implementation of the UNECE Sulphur Protocol (1994) will bring about a substantial reduction in the amount of S being deposited in the UK, especially in central and southern parts of the country. Some areas will remain where additional reductions in S are required. Over most of the country, however, the need to reduce N deposition will become paramount. The changing contributions and significance of non-UK sources can be estimated.
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    Increasing role of nitrogen in the acidification of surface waters in the Adirondack Mountains, New York (1997)
    Springer
    Water, air & soil pollution 95 (1997), S. 313-336 
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    ISSN: 1573-2932
    Keywords: nitrogen ; acidification ; Adirondack Mountains ; atmospheric deposition
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Assessments of the aquatic effects of acidic deposition have focused on sulfur, as have recent efforts to control the emissions of acidifying compounds. Nitrogen dynamics were excluded from most acidic deposition modeling studies because it was believed that terrestrial ecosystems strongly retain N and because modeling N is a more formidable task than modeling S due to the influence of complex biological processes on N cycling. Re-examination of available data for the Adirondack Mountains of New York suggests that N deposition may be contributing to both chronic and episodic acidification of freshwaters to a greater extent than is generally believed. Previous research concluded that N has played a limited role in acidification processes in these lakes, based on regional averages of chronic chemistry. However, it is now known that historic acidification responses have been spatially variable within the Adirondack Mountains and that the declines in lakewater pH have been less than previously believed. Lakewater NO3 − concentrations are commonly in the range of 5 to 25 μeq L−1 on a chronic basis in portions of the Adirondack region that have experienced significant chronic acidification. These NO3 − concentrations correspond in magnitude to inferred historical acidification. Furthermore, the relative importance of NO3 − as an agent of acidification increases dramatically during snowmelt when conditions are most toxic to fish. The consequence of not addressing N in formulating acidification recovery strategies for the Adirondacks includes the likelihood that we will overestimate the response of surface water to the mandated sulfur emissions reductions.
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    Effects of enhanced supplies of nitrogen and sulphur on rhizosphere and soil chemistry in a Norway spruce stand in SW Sweden (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1777-1782 
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    ISSN: 1573-2932
    Keywords: aluminium ; base cations ; bulk soil ; nitrogen ; rhizosphere soil ; sulphur
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Rhizophere and bulk soil chemistry were investigated in a Norway spruce stand in SW Sweden. The rhizosphere and bulk soil chemistry in water extracts in control plots (C) and plots repeatedly treated with ammonium sulphate (NS) were compared. Treatment regime was started in 1988. Cylindrical core samples of the LFH-layer and mineral soil layers were collected in 1992 and used for water extract analyses. Samples of soil from LFH-layer and mineral soil layers were taken in 1991 and 1993 for determination of CEC and base saturation. Soil pH and NH4-N, NO3-N and SO4-S, Al, Ca, K and Mg concentrations in water extracts were measured for rhizosphere and bulk soils. The pH-values of bulk and rhizosphere soils in NS plots decreased compared with those in control plots, whereas concentrations of NH4-N, NO3-N, SO4-S, base cations and Al in water extract increased. In both bulk and rhizosphere soils the concentration of NH4-N was much higher than that of NO3-N. A significant difference in the pH and Mg concentration of bulk and rhizosphere soil between the treated and control plots was found only in the 0–10 cm layer. For all layers, there was a significant difference in NH4-N concentrations in the bulk and rhizosphere soil between the NS treatment and control plots. Concentrations of exchangeable base cations and the base saturation level in the LFH-layer decreased in the NS plots. The concentration of extractable SO4-S increased in the NS plots. The NS treatment enhanced the amount of litter in L-layer, owing to increases in needle biomass and litterfall but led to losses of base cations, mainly K and Mg, from LFH-layer. It was concluded that the NS treatment displaced cations from exchangeable sites in the LFH-layer leading to higher concentrations of these elements in both rhizosphere and bulk soil.
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    Behaviour of sulphur and nitrogen compounds measured at marine stations Lista and Säby in Scandinavia (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2039-2044 
    Details
    ISSN: 1573-2932
    Keywords: sulphur ; nitrogen ; Scandinavia ; long distance transport ; elemental tracers
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Long distance transport of various air pollutants has been studied at two Scandinavian coastal sites. The measuring period has covered one year divided into 4 campaigns. Seasonal variations for sulphur and nitrogen compounds as well as anthropogenically emitted metals are reported. Concentrations of Pb and Zn as well as the ratio of V/Ni concentrations have been used to trace sulphuric episodes. Covariation of anthropogenic pollutants for the two sites is demonstrated.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01186134
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    Modelling leaching of inorganic Hg(II) in a Scandinavian iron-humus podzol — validation and long-term leaching under various deposition rates (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 301-320 
    Details
    ISSN: 1573-2932
    Keywords: acid rain ; batch experiment ; Freundlich isotherm ; lysimeter experiment ; mercury ; simulation model
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Increasing mercury contents are reported from freshwater systems and fish in northern Europe and North America. Mercury input from soils is a major source with the leaching being affected by increased atmospheric mercury deposition compared to pre-industrial times and by other environmental conditions such as acid rain. The results of a mathematical model-calculation of vertical inorganic Hg(II) leaching in a Scandinavian iron-humus podzol under different atmospheric input rates of mercury are presented. Leaching under background rain conditions was calculated to be considerably stronger than under acid rain conditions. Increasing fractions of deposited soluble or solute atmospheric mercury were leached from the O f(h)-horizon with decreasing soil content of soluble mercury under acid rain conditions; this effect was less pronounced under background rain conditions. The steady state concentrations of soluble mercury of the upper soil horizons were calculated and compared with the actual concentrations of total (= soluble + insoluble mercury) and extractable (= estimate of soluble) mercury measured in these horizons. The results indicate that even if the deposition of airborne mercury to soil is strongly reduced, the total mercury content of the soil decreases only slowly. It may take decades or even centuries before a new steady state concentration of total mercury is established in the soil. The decrease of the mercury concentration in the O f(h)-horizon is probably largely dependent on the turnover of organic matter, binding most of the deposited airborne mercury in an insoluble form. Hence, present day mercury leaching is likely to be dominated by mercury deposited during former times and temporarily retained in an insoluble form in the organic matter.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF02407211
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    Variations in sulphur and nitrogen foliar concentration of deciduous and conifers vegetation in Slovakia (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 329-345 
    Details
    ISSN: 1573-2932
    Keywords: beech ; biomonitoring ; nitrogen ; solid particles ; spruce ; sulphur
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The foliage contents of Stotal and Ntotal were determined in 405 Permanent monitoring plots in four National Parks and sixteen Landscape Protection Areas and were compared with 1483 Permanent monitoring plots on Slovakia. The foliage content of S ranged from 0.72 to 6.77 g kg−1 in hardwoods and from 0.98 to 4.3 g kg−1 in softwoods. A critical increase was determined in one National Park and in four Landscape Protection Areas. The foliage content of N ranged from 9.7 to 48.7 g kg−1 in softwoods, and from 7.8 to 51.4 g kg−1 in hardwoods. An insufficient level of N was determined in one Landscape Protection Area and a critical increase in four Landscape Protection Areas. The sulphur to nitrogen ratio ranged from 0.08 to 0.176 in softwoods, and from 0.078 to 0.253 in hardwoods. The foliage surface on hitherto explored four National Parks and sixteen Landscape Protection Areas in network 4×4 km was covered by all categories of rigid fallout particles. Fly-ash from coal combustion were observed each of National Parks and Landscape Protection Areas by scanning electron microscopy. Mycelia and spore, mineral matters, sand and soil particles were present on all National Parks and Landscape Protection Areas. Particles derived from aluminium production were observed at three Landscape Protection Areas. Particles derived from cement production and from lime works were observed at two National Parks and six Landscape Protection Areas. Particles derived from ferrous metals industry were observed at each of National Parks and Landscape Protection Areas and particles typical for other technologies were present in three of National Parks and twelve Landscape Protection Areas.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF02407213
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    HEAVY METALS IN ALLOTMENT GARDENS CLOSE TO AN OIL REFINERY IN PŁOCK (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 61-71 
    Details
    ISSN: 1573-2932
    Keywords: allotment gardens ; dustfall ; ground water ; heavy metals ; oil refinery ; soil ; vegetables
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In the period 1984–1990 the following vegetables were grown: red beet, carrot and parsley in four allotment gardens of Płock city (Central Poland), situated near the refinery and petrochemical works. Cadmium, lead, copper, chromium, zinc and manganese concentrations were determined in the leaves and roots of vegetables. The heavy metal accumulation in the soil, dustfall (measure of air pollution), and ground water was determined. The quality of the vegetable yield, notably of the leaves, was low. This was mainly due to the excessive chromium and cadmium content in the leaves. Accumulation of heavy metals was relatively low in the soil, rather high in the ground water and variable in the dust.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1026402218990
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    VARIATIONS IN SULPHUR AND NITROGEN FOLIAR CONCENTRATION OF DECIDUOUS AND CONIFERS VEGETATION IN SLOVAKIA (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 329-345 
    Details
    ISSN: 1573-2932
    Keywords: beech ; biomonitoring ; nitrogen ; solid particles ; spruce ; sulphur
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The foliage contents of Stotal and Ntotal were determined in 405 Permanent monitoring plots in four National Parks and sixteen Landscape Protection Areas and were compared with 1483 Permanent monitoring plots on Slovakia. The foliage content of S ranged from 0.72 to 6.77 g kg-1 in hardwoods and from 0.98 to 4.3 g kg-1 in softwoods. A critical increase was determined in one National Park and in four Landscape Protection Areas. The foliage content of N ranged from 9.7 to 48.7 g kg-1 in softwoods, and from 7.8 to 51.4 g kg -1 in hardwoods. An insufficient level of N was determined in one Landscape Protection Area and a critical increase in four Landscape Protection Areas. The sulphur to nitrogen ratio ranged from 0.08 to 0.176 in softwoods, and from 0.078 to 0.253 in hardwoods. The foliage surface on hitherto explored four National Parks and sixteen Landscape Protection Areas in network 4 × 4 km was covered by all categories of rigid fall-out particles. Fly-ash from coal combustion were observed each of National Parks and Landscape Protection Areas by scanning electron microscopy. Mycelia and spore, mineral matters, sand and soil particles were present on all National Parks and Landscape Protection Areas. Particles derived from aluminium production were observed at three Landscape Protection Areas. Particles derived from cement production and from lime works were observed at two National Parks and six Landscape Protection Areas. Particles derived from ferrous metals industry were observed at each of National Parks and Landscape Protection Areas and particles typical for other technologies were present in three of National Parks and twelve Landscape Protection Areas.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1026422606600
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    ACCUMULATION OF CADMIUM AND ZINC FROM DIFFUSE IMMISSION ON ACID SANDY SOILS, AS A FUNCTION OF SOIL COMPOSITION (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 1-16 
    Details
    ISSN: 1573-2932
    Keywords: heavy metals ; pollution ; sandy soils ; zinc smelter
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Sandy soils, in the border area of Belgium and the Netherlands (the Kempen region), are heavily contaminated by atmospheric deposition of cadmium and zinc from nearby smelters. Groundwater contamination by leaching from these low retention soils is subject of study. There are reports of high cadmium and zinc concentrations in groundwater in the area, but in most cases the direct sources are unknown. In an attempt to predict present or future risk of groundwater contamination by soil leaching, metal binding processes (retardation) were studied that are specific for these soil types under the existing acidifying conditions. From four fields nine contaminated profiles were sampled and analyzed for cadmium and zinc. Average concentrations of 131 μg g-1 zinc and 1.6 μg g-1 cadmium with maximum values of 2989 μg g-1 respectively 16.3 μg g-1 were found. In addition pH and contents of organic matter, aluminium, iron, and manganese were determined. The relative importance of these soil parameters for metal retardation is derived from the profiles. The data show that organic matter is the most important soil component for binding cadmium and zinc. Adsorption of cadmium and zinc on aluminium, iron and manganese (hydr) oxides appears to be of minor importance at low pH (〈5.5).
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1019297625144
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    Accumulation of cadmium and zinc from diffuse immission on acid sandy soils, as a function of soil composition (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 1-16 
    Details
    ISSN: 1573-2932
    Keywords: heavy metals ; pollution ; sandy soils ; zinc smelter
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Sandy soils, in the border area of Belgium and the Netherlands (the Kempen region), are heavily contaminated by atmospheric deposition of cadmium and zinc from nearby smelters. Groundwater contamination by leaching from these low retention soils is subject of study. There are reports of high cadmium and zinc concentrations in groundwater in the area, but in most cases the direct sources are unknown. In an attempt to predict present or future risk of groundwater contamination by soil leaching, metal binding processes (retardation) were studied that are specific for these soil types under the existing acidifying conditions. From four fields nine contaminated profiles were sampled and analyzed for cadmium and zinc. Average concentrations of 131μg g−1 zinc and 1.6μg g−1 cadmium with maximum values of 2989μg g−1 respectively 16.3μg g−1 were found. In addition pH and contents of organic matter, aluminium, iron, and manganese were determined. The relative importance of these soil parameters for metal retardation is derived from the profiles. The data show that organic matter is the most important soil component for binding cadmium and zinc. Adsorption of cadmium and zinc on aluminium, iron and manganese (hydr) oxides appears to be of minor importance at low pH (〈5.5).
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF02407193
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    Partitioning of heavy metals in podzol soils contaminated by mine drainage waters, Dalarna, Sweden (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 39-59 
    Details
    ISSN: 1573-2932
    Keywords: acid mine drainage ; heavy metals ; jarosite ; soils ; Sweden
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The discharge of acidic mine drainage waters onto a hillslope in Dalarna, central Sweden, has lead to the contamination of the podzol soils with Cu, Fe, Ni, Pb, Zn and sulfate. Samples from contaminated and reference soils have been collected for chemical and mineralogical analyses. Jarosite is identified by x-ray diffraction analysis as a precipitate in the upper horizons (A, E, B) of the contaminated soils, where the soil acidity (pHKCl∼2.6) promotes jarosite stability. The sequential chemical extraction of soil samples indicates that, in the reference A horizon, Cu, Pb, Ni and Zn are bound primarily to cation exchange sites and organic matter. In the A horizon of the contaminated soils closest to the rock dump, metal partitioning is dominated by the Fe oxide fractions, despite the high organic matter content; Pb is almost completely bound to crystalline Fe oxides, possibly adsorbed to Fe oxides or occuring in a jarosite solid solution. In the reference B and C horizons, Cu, Ni and Zn are primarily adsorbed/coprecipitated in the Fe oxide fractions, while Pb remains with a large fraction bound to organic matter. In the Fe-rich B horizon of the contaminated soils, the partitioning of the metals in cation exchange sites and to organic matter has greatly increased relative to the reference soils, resulting from the mobilization of organo-metal complexes down the profile.
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    URL: http://dx.doi.org/10.1007/BF02407195
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    Heavy metals in allotment gardens close to an oil refinery in Płock (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 61-71 
    Details
    ISSN: 1573-2932
    Keywords: allotment gardens ; dustfall ; ground water ; heavy metals ; oil refinery ; soil ; vegetables
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In the period 1984–1990 the following vegetables were grown: red beet, carrot and parsley in four allotment gardens of Płock city (Central Poland), situated near the refinery and petrochemical works. Cadmium, lead, copper, chromium, zinc and manganese concentrations were determined in the leaves and roots of vegetables. The heavy metal accumulation in the soil, dustfall (measure of air pollution), and ground water was determined. The quality of the vegetable yield, notably of the leaves, was low. This was mainly due to the excessive chromium and cadmium content in the leaves. Accumulation of heavy metals was relatively low in the soil, rather high in the ground water and variable in the dust.
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    URL: http://dx.doi.org/10.1007/BF02407196
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    Mercury from Combustion Sources: A Review of the Chemical Species Emitted and Their Transport in the Atmosphere (1997)
    Springer
    Water, air & soil pollution 98 (1997), S. 241-254 
    Details
    ISSN: 1573-2932
    Keywords: coal ; deposition ; emission ; mercury ; municipal solidwaste
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Different species of mercury have different physical/chemical properties and thus behave quite differently in air pollution control equipment and in the atmosphere. In general, emissions of mercury from coal combustion sources are approximately 20–50% elemental mercury (Hg°) and 50–80% divalent mercury (Hg(II)), which may be predominantly HgCl2. Emissions of mercury from waste incinerators are approximately 10–20% Hg° and 75–85% Hg(II). The partitioning of mercury in flue gas between the elemental and divalent forms may be dependent on the concentration of particulate carbon, HCl and other pollutants in the stack emissions. The emission of mercury from combustion facilities depends on the species in the exhaust stream and the type of air pollution control equipment used at the source. Air pollution control equipment for mercury removal at combustion facilities includes activated carbon injection, sodium sulfide injection and wet lime/limestone flue gas desulfurization. While Hg(II) is water-soluble and may be removed from the atmosphere by wet and dry deposition close to combustion sources, the combination of a high vapor pressure and low water-solubility facilitate the long-range transport of Hg° in the atmosphere. Background mercury in the atmosphere is predominantly Hg°. Elemental mercury is eventually removed from the atmosphere by dry deposition onto surfaces and by wet deposition after oxidation to water- soluble, divalent mercury.
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    URL: http://dx.doi.org/10.1023/A:1026429911010
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    MONITORING NITROGEN POLLUTION FROM SUGARCANE RUNOFF USING 15N ANALYSIS (1997)
    Springer
    Water, air & soil pollution 98 (1997), S. 389-399 
    Details
    ISSN: 1573-2932
    Keywords: fertilizer ; nitrogen ; pollution ; runoff ; stable isotopes ; sugarcane
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In many forested wetlands of Louisiana, surface water quality is being deteriorated by nutrient input from adjacent agricultural production areas. This field study assesses the input of fertilizer N, applied to sugarcane fields, to forested wetlands. The potential use of natural abundance variations in 15N14N ratios for identification and tracing surface water N sources (NH 4 + - and NO3 --N) was evaluated. Runoff and surface water samples were collected from sugarcane fields and bordering forested wetlands (6 stations) over a 16 month period and analyzed for NH 4 + -N, NO 3 - -N, and associated NH 4 + -δ15N and NO 3 - -δ15N ratios. Fertilizer N draining into adjacent forested wetland was estimated to be only a small fraction of the amount applied. Concentrations of NH 4 + - and NO 3 - -N in the collected water samples were low and ranged from 0.02 to 1.79 mg L-1. Isotopic analysis revealed NH 4 + -δ15N and NO 3 - -δ15N means were distinctive and may have the potential to be used as tracers of N contamination. The mean NH 4 + -δ15N value was +18.6 ± 7.1‰ and the NO 3 - -δ15N mean was +8.3 ± 3.1‰. Anomalously high NO 3 - -δ15N values (〉30‰) were attributed to denitrification.
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    URL: http://dx.doi.org/10.1023/A:1026483228623
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    Mercury from combustion sources: A review of the chemical species emitted and their transport in the atmosphere (1997)
    Springer
    Water, air & soil pollution 98 (1997), S. 241-254 
    Details
    ISSN: 1573-2932
    Keywords: coal ; deposition ; emission ; mercury ; municipal solid waste
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Different species of mercury have different physical/chemical properties and thus behave quite differently in air pollution control equipment and in the atmosphere. In general, emissions of mercury from coal combustion sources are approximately 20–50% elemental mercury (Hg°) and 50–80% divalent mercury (Hg(II)), which may be predominantly HgCl2. Emissions of mercury from waste incinerators are approximately 10–20% Hg° and 75–85% Hg(II). The partitioning of mercury in flue gas between the elemental and divalent forms may be dependent on the concentration of particulate carbon, HCl and other pollutants in the stack emissions. The emission of mercury from combustion facilities depends on the species in the exhaust stream and the type of air pollution control equipment used at the source. Air pollution control equipment for mercury removal at combustion facilities includes activated carbon injection, sodium sulfide infection and wet lime/limestone flue gas desulfurization. While Hg(II) is water-soluble and may be removed from the atmosphere by wet and dry deposition close to combustion sources, the combination of a high vapor pressure and low water-solubility facilitate the long-range transport of Hg° in the atmosphere. Background mercury in the atmosphere is predominantly Hg°. Elemental mercury is eventually removed from the atmosphere by dry deposition onto surfaces and by wet deposition after oxidation to water-soluble, divalent mercury.
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    URL: http://dx.doi.org/10.1007/BF02047037
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    Spatial and Temporal Variability of Total Non-Residual Heavy Metals Content in Stream Sediments from the Suquia River System, Cordoba, Argentina (1997)
    Springer
    Water, air & soil pollution 93 (1997), S. 303-319 
    Details
    ISSN: 1573-2932
    Keywords: heavy metals ; TNR ; stream sediments ; Suquía River
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The Suquía is a semiarid (rainfall, 700-900 mm y-1), medium-size (7700 km2) riversystem located in central Argentina. Its mountainous upper catchment includes pristine areas aswell as a variety of human settlements and a reservoir lake. A large city (Córdoba, ca. 1.3million inhabitants) and a terminal hypersaline lake are included in the middle and lower basin.Total non-residual (TNR) heavy metals (Pb, Cu, Ni, Zn, Mn, and Fe) have been determined inriver bed sediments in two seasons (spring and autumn), seeking to establish the factors whichcontrol the temporal and spatial variability. The major findings were: a) concentrations of TNRmetals were, in general, higher during springtime than during autumn, particularly downstreamfrom the city of Córdoba; b) organic matter played a significant role as a controlling factorwherever it defined reducing conditions, lowering the concentrations of Mn and Fe hydrousoxides; c) a higher organic load (e.g., downstream the city) and more pronounced reducingconditions could be the causes for the increased Fe concentration, probably precipitated assulfides; d) organic matter exhibited a closer correlation with some TNR metals in autumn,probably caused by a larger capacity for complexation in the biologically-processed organicdebris; and, e) the existence of pristine areas in the drainage basin allowed for the calculation ofenrichment factors (EF) which show the significance of several environmental impacts in theSuquía system.
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    URL: http://dx.doi.org/10.1023/A:1022113330970
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    Sulphur and Heavy Metal Concentrations in Scots Pine Bark in Northern Finland and the Kola Peninsula (1997)
    Springer
    Water, air & soil pollution 93 (1997), S. 395-408 
    Details
    ISSN: 1573-2932
    Keywords: air pollution ; pine bark ; sulphur ; pH ; conductivity ; heavy metals
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Sulphur and heavy metal deposition in northern Finland (= in Lapland) and the Kola Peninsulawere surveyed using Scots pine bark samples. Sulphur concentrations in bark close to the Kolasmelters were on an average twice as high as on the Finnish side of the border. The Cu and Niconcentrations near the smelters were almost 100-fold the mean values in northern Finland. Therewas a marked decrease in the sulphur and heavy metal concentrations with increasing distancefrom the emission sources. The effects of emissions from the Kola Peninsula were evident inFinland only close to the border, especially in the eastern parts of Inari (NE corner of Lapland)where the Cu and Ni concentrations were 2- to 6-fold those in western Lapland. The sulphur andheavy metal concentrations in most of northern Finland were low. However were theconcentrations of Cr in bark in the SW corner of Lapland considerably high, due to the emissionsfrom the Tornio refined steel plants.
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    URL: http://dx.doi.org/10.1023/A:1022160930526
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    The Influence of Heavy Metals on Carbon Dioxide Evolution from a Typic Xerochrept Soil (1997)
    Springer
    Water, air & soil pollution 93 (1997), S. 409-417 
    Details
    ISSN: 1573-2932
    Keywords: CO2 evolution ; heavy metals ; loading effect ; metal equivalent
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In a laboratory study the effects on soil respiration of trace metals (Ni, Cd, Cu, Mn, Pb, Zn)added at loading rates ranging from 0 to 1000 µg g-1 were determined. Differences intoxicity with respect to the type of metal salt added were also evaluated. The inhibitory effect onsoil respiration differed considerably among the heavy metals and increased with the increasingloading rate. No linear relationships were found between the degree of inhibition and the levels oftotal and available metals. Toxicity evaluation at 20 and 50% inhibition of soil respiration showedCu as the most toxic and Mn as the most tolerable metal. A ‘metal equivalent’ was calculated asthe sum of the amounts of the available metals weighted to their relative toxicity with respect tothe least toxic one: Mn equivalent = Mn + 1.9Pb + 2.1Ni + 2.5Zn + 6.7Cd + 6.7Cu. The ionicpotential of the heavy metals was found to be positively related to the percent inhibition of soilrespiration. Chlorides and sulphates appeared to depress soil respiration more than nitrates, thelatter counter-balancing the toxic effect of the heavy metals.
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    URL: http://dx.doi.org/10.1023/A:1022111323406
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  • 89
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    Ash from Cereal and Rape Straw Used for Heat Production: Liming Effect and Contents of Plant Nutrients and Heavy Metals (1997)
    Springer
    Water, air & soil pollution 93 (1997), S. 93-108 
    Details
    ISSN: 1573-2932
    Keywords: straw ash ; ashes ; bottom ash ; fly ash ; biofuel ; cereal straw ; rape straw ; straw combustion ; fertilizer ; plant nutrients ; heavy metals
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The composition of 79 samples of straw ash from seven heating plants in Sweden wasanalysed with the aim of evaluating straw ash as a fertilizer and liming agent. The variation in ashcomposition was explained mainly by ash fraction (bottom ash vs. fly ash) and straw type (wheat,barley, rye, rape) but also by heating plant. Compared with concentrations of Zn, Pb and Cd inbottom ash, levels in fly ash were 10-90 times higher. Fly ash also contained more Cu and Kcompared with bottom ash. The Cd/P ratio was 0.03 in bottom ash and 0.6 g Cd/kg P in fly ash.Ash from rape straw had a higher Ca content and liming effect compared with ash from cerealstraw; e.g., the liming effect of rape ash was more than three times higher than that of wheat ash.The liming effect varied between 3.5 and 44% CaO and depended mainly on the Ca content. Theaverage P content was 1.7% (0.2-4.4%), with slightly higher concentration in rape ash than inwheat ash. The potential for using straw ash as a fertilizer and liming agent is discussed. Compared withcommercial fertilizers the use of bottom ash as a P fertilizer results in a lower addition of Cd.However, the total heavy metal content of straw ash poses a potential problem.
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    URL: http://dx.doi.org/10.1023/A:1022179708289
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    Spatial and temporal variability of total non-residual heavy metals content in stream sediments from the Suquia River system, Cordoba, Argentina (1997)
    Springer
    Water, air & soil pollution 93 (1997), S. 303-319 
    Details
    ISSN: 1573-2932
    Keywords: heavy metals ; TNR ; stream sediments ; Suquía River
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The Suquía is a semiarid (rainfall, 700–900 mm y−1), medium-size (7700 km2) river system located in central Argentina. Its mountainous upper catchment includes pristine areas as well as a variety of human settlements and a reservoir lake. A large city (Córdoba, ca. 1.3 million inhabitants) and a terminal hypersaline lake are included in the middle and lower basin. Total non-residual (TNR) heavy metals (Pb, Cu, Ni, Zn, Mn, and Fe) have been determined in river bed sediments in two seasons (spring and autumn), seeking to establish the factors which control the temporal and spatial variability. The major findings were: a) concentrations of TNR metals were, in general, higher during springtime than during autumn, particularly downstream from the city of Córdoba; b) organic matter played a significant role as a controlling factor wherever it defined reducing conditions, lowering the concentrations of Mn and Fe hydrous oxides; c) a higher organic load (e.g., downstream the city) and more pronounced reducing conditions could be the causes for the increased Fe concentration, probably precipitated as sulfides; d) organic matter exhibited a closer correlation with some TNR metals in autumn, probably caused by a larger capacity for complexation in the biologically-processed organic debris; and, e) the existence of pristine areas in the drainage basin allowed for the calculation of enrichment factors (EF) which show the significance of several environmental impacts in the Suquía system.
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    URL: http://dx.doi.org/10.1007/BF02404763
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    Heavy metal contaminated soils in an old industrial area of Wales, Great Britain: Source identification through statistical data interpretation (1997)
    Springer
    Water, air & soil pollution 94 (1997), S. 85-98 
    Details
    ISSN: 1573-2932
    Keywords: soil ; pollution ; heavy metals ; smelters ; factor analysis
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A combined statistical and computergraphic approach is proposed for apportionment and attribution of soil contaminants in complex areas. The field test site lies north of Swansea, south Wales and contains two major pollutant sources, an active nickel refiner and (4 km away) the site of major base metal smelting in the nineteenth century (the Lower Swansea Valley reclamation study area). Soil samples (70 samples, 0–15 cm) were collected on a regular grid of 1000 m interval. They were extracted using 0.05 M diammonium EDTA and the extracts analysed for Cd, Co, Cu, Fe, Mn, Ni, Pb and Zn. Soil pH and %organic content were also determined. Factor analysis yielded three groups which explained 73.8% of the data variance (1: Cd, Cu, %OM, Pb, Zn, Ni; 2: Cd, Zn, Mn, pH; 3: Cu, Mn, Co, Ni, Fe). Isoline plots were classifiable into the same three groups. It was concluded that factor 3 contained those elements associated with smelter emissions, factor 1 with contamination from the Lower Swansea Valley and in factor 2 pedogenetic processes control the occurrence of the elements.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF02407095
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  • 92
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    INCREASED CADMIUM AVAILABILITY TO CROPS ON A SEWAGE-SLUDGE AMENDED SOIL (1997)
    Springer
    Water, air & soil pollution 94 (1997), S. 361-372 
    Details
    ISSN: 1573-2932
    Keywords: heavy metals ; contamination ; mobilization ; cadmium ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Analysis of spatial distribution of sewage-sludge born cadmium on the experimental plot revealed positive correlation of total cadmium and organic matter. Soil pH fluctuated randomly on the field. ‘Bioavailable’ concentrations, as determined by NH4-acetate extraction, were closely correlated to the total cadmium levels, and only negligible effects of pH and/or organic matter fluctuations were recorded. Desorption model using modified Freundlich isotherm was applied to predict risks of cadmium solubilization at different conditions. Simulations revealed that the organic matter content within the ranges found at the experimental field cannot support a proper immobilization of cadmium at pH-range observed at the field. The phenomenon was explained by ineffective care for the soil in the past.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1026407720823
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  • 93
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    Increased cadmium availability to crops on a sewage-sludge amended soil (1997)
    Springer
    Water, air & soil pollution 94 (1997), S. 361-372 
    Details
    ISSN: 1573-2932
    Keywords: heavy metals ; contamination ; mobilization ; cadmium ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Analysis of spatial distribution of sewage-sludge born cadmium on the experimental plot revealed positive correlation of total cadmium and organic matter. Soil pH fluctuated randomly on the field. ‘Bioavailable’ concentrations, as determined by NH4-acetate extraction, were closely correlated to the total cadmium levels, and only negligible effects of pH and/or organic matter fluctuations were recorded. Desorption model using modified Freundlich isotherm was applied to predict risks of cadmium solubilization at different conditions. Simulations revealed that the organic matter content within the ranges found at the experimental field cannot support a proper immobilization of cadmium at pH-range observed at the field. The phenomenon was explained by ineffective care for the soil in the past.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF02406068
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  • 94
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    Sediment accumulation of nutrients (N, P) in the eastern Gulf of Finland (Baltic Sea) (1997)
    Springer
    Water, air & soil pollution 99 (1997), S. 477-486 
    Details
    ISSN: 1573-2932
    Keywords: sediment ; nitrogen ; phosphorus ; organic matter ; cluster analysis ; Gulf of Finland ; estuaries
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Dry weight (DW), ignition loss (IL) and concentrations of total nitrogen (TN) and total phosphorus (TP) of the sediment surface layer (0 to 10 cm, 1 cm slices) were analyzed from 20 sites in the eastern Gulf of Finland. The distance of the sampling sites from the mouth of the River Neva explained the nutrient concentrations of the sediments well, while the effect of water depth was negligible. The increase of TN and the decrease of TP along the transect from the river mouth towards the open Gulf were caused by the diminishing share of allochthonous material supplied from the River Neva. The mean TN concentration of the different accumulation areas was about 40 % higher in the sediment surface than in the deeper layer (9 to 10 cm). The corresponding difference for TP varied from 53 to 56 %. The results suggest considerable netflux of nutrients from sediment to water. The net sediment accumulation of nutrients were estimated as 6.0 g m−2 a−1 of N and 1.7 g m−2 a−1 of P corresponding 22 000 t a− of N and 6 100 t a−1 of P for the whole eastern Gulf.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF02406887
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  • 95
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    Bivalves and heavy metals in polluted sediments: A chemometric approach (1997)
    Springer
    Water, air & soil pollution 99 (1997), S. 615-622 
    Details
    ISSN: 1573-2932
    Keywords: Near-shore sediments ; heavy metals ; bioindicators ; bivalves ; benthic populations ; multivariate analysis ; multiple regression analysis ; predictive models
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Copper, lead, cadmium, zinc, chromium, manganese, iron and nickel were determined in near-shore sediments in the harbour of Trieste (Northern Adriatic), in an area highly exposed to urban and industrial wastes, where severe alteration of benthic population was observed. A typical bivalve of this area,Corbula gibba, was used as bioindicator of sea-bottom pollution. Multivariate statistical analysis of the chemical data interpret concentrations and distributions of heavy metals in these sediments, attesting anthropogenic source for Cu, Pb, Cd and Zn. Using labile fractions of heavy metals in sediments as ‘predictors’, and length or bionnass of the bivalve as dependent variables, we obtained, by a multiple regression procedure, a predictive model showing the influence of metals on this benthic organism of this polluted area.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF02406900
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  • 96
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    INCREASING ROLE OF NITROGEN IN THE ACIDIFICATION OF SURFACE WATERS IN THE ADIRONDACK MOUNTAINS, NEW YORK (1997)
    Springer
    Water, air & soil pollution 95 (1997), S. 313-336 
    Details
    ISSN: 1573-2932
    Keywords: nitrogen ; acidification ; Adirondack Mountains ; atmospheric deposition
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Assessments of the aquatic effects of acidic deposition have focused on sulfur, as have recent efforts to control the emissions of acidifying compounds. Nitrogen dynamics were excluded from most acidic deposition modeling studies because it was believed that terrestrial ecosystems strongly retain N and because modeling N is a more formidable task than modeling S due to the influence of complex biological processes on N cycling. Re-examination of available data for the Adirondack Mountains of New York suggests that N deposition may be contributing to both chronic and episodic acidification of freshwaters to a greater extent than is generally believed. Previous research concluded that N has played a limited role in acidification processes in these lakes, based on regional averages of chronic chemistry. However, it is now known that historic acidification responses have been spatially variable within the Adirondack Mountains and that the declines in lakewater pH have been less than previously believed. Lakewater NO3 - concentrations are commonly in the range of 5 to 25 μeq L-1 on a chronic basis in portions of the Adirondack region that have experienced significant chronic acidification. These NO3 - concentrations correspond in magnitude to inferred historical acidification. Furthermore, the relative importance of NO3 - as an agent of acidification increases dramatically during snowmelt when conditions are most toxic to fish. The consequence of not addressing N in formulating acidification recovery strategies for the Adirondacks includes the likelihood that we will overestimate the response of surface water to the mandated sulfur emissions reductions.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1026422031266
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  • 97
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    MERCURY ACCUMULATION IN DEVILS LAKE, NORTH DAKOTA – EFFECTS OF ENVIRONMENTAL VARIATION IN CLOSED-BASIN LAKES ON MERCURY CHRONOLOGIES (1997)
    Springer
    Water, air & soil pollution 98 (1997), S. 275-296 
    Details
    ISSN: 1573-2932
    Keywords: mercury ; mercury accumulation ; mercury deposition ; North Dakota ; saline lakes ; sediment cores
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Sediment cores were collected from lakes in the Devils Lake Basin in North Dakota to determine if mercury (Hg) accumulation chronologies from sediment-core data are good indicators of variations in Hg accumulation rates in saline lakes. Sediment cores from Creel Bay and Main Bay, Devils Lake were selected for detailed analysis and interpretation. The maximum Hg concentration in the Creel Bay core was 0.15 micrograms per gram at 8 to 9 centimeters. The maximum Hg concentration in the Main Bay core was 0.07 micrograms per gram at 5 to 7 centimeters. The general decreases in Hg concentrations with depth are attributed to historic variations in atmospheric Hg deposition rate. Hg stratigraphies combined with210 Pb and 137Cs dating analyses yield Hg chronologies that indicate a general increase in Hg accumulation rates in Devils Lake since the middle of the 19th century. Mean modern Hg accumulation rates in Creel Bay were 4.9 nanograms per square centimeter per year, and rates in Main Bay were 1.8 nanograms per square centimeter per year. Mean preindustrial Hg accumulation rates in Creel Bay were 1.2 nanograms per square centimeter per year, and rates in Main Bay were 1.6 nanograms per square centimeter per year. Relatively low Hg concentrations in recent sediments in the Devils Lake Basin, along with similarities in Hg accumulation rates between lakes in the Devils Lake Basin and other lakes in the northern interior of North America, indicate that local sources of Hg are not important sources of Hg. Results of the study indicate that accurate Hg chronologies are discernible in sediment cores collected from saline lakes. However, spatial and temporal variations in lake level and water chemistry common to saline lakes make interpretation of radioisotopic and geochemical chronologies difficult. Hg geochemistry in Devils Lake, and presumably in other saline lakes, is dynamic. The results of this study indicate that the absolute amount of sediment transported to Devils Lake, along with the associated Hg and total organic carbon, and the distribution of sedimentation patterns in Devils Lake may be affected by changing lake levels.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1026415001754
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  • 98
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    Heavy Metal Content in Xylem Sap (Vitis Vinifera) from Mining and Smelting Areas (1998)
    Springer
    Environmental monitoring and assessment 50 (1998), S. 189-200 
    Details
    ISSN: 1573-2959
    Keywords: grapevines ; heavy metals ; mining ; smelting ; xylem sap
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract No data are available on the content of heavy metals in the xylem sap of grapevines growing in contaminated areas. The aim of this work was to obtain data on the concentration of Pb, Zn, Cd and Cu in the xylem sap of grapevine (Vitis vinifera) cultivar Monica (ungrafted), growing near contaminated sites: a smelter, an abandoned and an active mine, and to investigate relationships between xylem sap mineral composition and the heavy metal content of the soil. The concentrations of Pb, Zn, Cd and Cu in the sap were enhanced compared to that of the soil, ranging from 4.3 to 611.4 µg Pb $$g_{d.wt.}^{ - 1} $$]〉$$ , 801 to 6176 µg Zn $$g_{d.wt.}^{ - 1} $$]〉$$ , 2.5 to 45 µg Cd $$g_{d.wt.}^{ - 1} $$]〉$$ and 19.8 to 161 µg Cu $$g_{d.wt.}^{ - 1} $$]〉$$ . Dry matter of xylem sap was significantly related to the heavy metals content in xylem saps, but no significant relationship between the metals in sap and total and DTPA/TEA extractable metal fraction in soil was found.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1005854213903
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  • 99
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    An Overview of Contaminant-Related Issues Identified by Monitoring in San Francisco Bay (2000)
    Springer
    Environmental monitoring and assessment 64 (2000), S. 409-419 
    Details
    ISSN: 1573-2959
    Keywords: monitoring ; assessment ; water ; sediment ; bioaccumulation ; toxicity ; pesticides ; mercury ; PCB
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The San Francisco Estuary Regional Monitoring Program for Trace Substances (RMP) began in 1993 and is sponsored by 74 local, state, and federal agencies and companies through their discharge or Bay use permits. The RMP monitors water, sediment, toxicity, and bivalve bioaccumulation at 25 sites in the Bay that are considered to represent "background" conditions. Several major environmental issues have been identified by the RMP. Polychlorinated biphenyls and mercury were often above water quality guidelines, and often occurred in fish tissues above U.S. Environmental Protection Agency (U.S. EPA) screening values. Concentrations do not appear to be decreasing, suggesting continuing inputs. Episodes of aquatic toxicity often occurred following runoff events that transport contaminants into the Bay from urbanized and agricultural portions of the watershed. Sediment toxicity occurred throughout the Bay, and has been correlated with concentrations of specific contaminants (chlordanes, polynuclear aromatic hydrocarbons) at some locations; mixtures of contaminants were probably also important. Since the RMP does not monitor all ecosystem components, assessments of the overall condition of the Bay cannot be made. However, in terms of contamination, the RMP samples suggest that the South Bay, and North Bay sites are moderately contaminated.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1006459605924
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  • 100
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    Contrasting effects of sewage sludge and commercial fertilizer on egg to adult development of two herbivorous insect species (1994)
    Springer
    Ecotoxicology 3 (1994), S. 94-109 
    Details
    ISSN: 1573-3017
    Keywords: heavy metals ; old-fields ; municipal sludge ; blackfaced leafhopper ; Graminella nigrifrons ; Cicadellidae ; cabbage looper moth ; Noctuidae ; Trichoplusia ni
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Municipal sewage sludge containing heavy metals had a toxic effect on the development of the cabbage looper, Trichoplusia ni (Lepidoptera: Noctuidae), one of two herbivorous insects commonly found in an Ohio old-field which had been subjected to long-term sewage sludge application. Soils were removed in 1992 from an old-field following 11 years of heavy nutrient enrichment (1978 to 1988) with applications of either sewage sludge (Milorganite®) containing heavy metal contaminants or urea-phosphate fertilizer. Egg to adult development rate and survival of the blackfaced leafhopper, Graminella nigrifrons (Homoptera: Cicadellidae), and the cabbage looper was determined on maize (leafhopper) and broccoli (looper) seedlings grown in soils from sludge-treated, fertilizer-treated, or untreated control plots of the old-field. Fertilizer and sludgetreated soils had higher levels of N. P and organic matter, and a lower pH than the untreated control soils, while sludge-treated soils contained significantly higher concentrations of Cd, Cu, Pb, and Zn. Maize appeared to be unaffected by the three soil treatments, and survival and rate of egg to adult development of the leafhopper was not affected. Broccoli seedlings grown in both the high nutrient fertilizer and sludge soils were greener and larger than broccoli grown in control soils. However, the cabbage looper had significant larval and pupal mortality (25 to 40%) and prolonged egg to adult development on sludge-grown broccoli compared to control and fertilizer treatments. As assimilation into the food chain of heavy metals and other organic pollutants, such as PCBs, is in part a function of the interaction of soil chemistry and type of plant, the application of municipal sludges to old-fields needs to be carefully monitored, as contaminants may have significant developmental and behavioural effects on some secondary links in the old-field food chain.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00143408
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