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    Phase-only laser control in the weak-field limit: Two-pulse control of IBr photofragmentation revisited (2016)
    American Institute of Physics (AIP)
    Details
    Publication Date: 2016-01-07
    Description: We demonstrate theoretically that laser-induced coherent quantum interference control of asymptotic states of dissociating molecules is possible, starting from a single vibrational eigenstate, after the interaction with two laser pulses—at a fixed time delay—both operating in the weak-field limit. Thus, phase dependence in the interaction with the second fixed-energy phase-modulated pulse persists after the pulse is over. This is illustrated for the nonadiabatic process: I + Br * ←IBr → I + Br, where the relative yield of excited Br * can be changed by pure phase modulation. Furthermore, a strong frequency dependence of the branching ratio is observed and related to the re-crossing dynamics of the avoided crossing in the above-mentioned process.
    Print ISSN: 0021-9606
    Electronic ISSN: 1089-7690
    Topics: Chemistry and Pharmacology , Physics
    Published by American Institute of Physics (AIP)
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