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Enhanced ordering of water at hydrophobic surfaces (2014)

American Institute of Physics (AIP)

In: Journal of Chemical Physics

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Publication Date: 2014-02-08

Description: We study the properties of water molecules adjacent to a hydrophobic molecular layer with vibrational sum-frequency generation spectroscopy. We find that the water molecules at D 2 O/hexane, D 2 O/heptane, and D 2 O/polydimethylsiloxane interfaces show an enhanced ordering and stronger hydrogen-bond interactions than the water molecules at a D 2 O/air interface. With increasing temperature (up to 80 °C) the water structure becomes significantly less ordered and the hydrogen bonds become weaker.

Print ISSN: 0021-9606

Electronic ISSN: 1089-7690

Topics: Chemistry and Pharmacology , Physics

Published by American Institute of Physics (AIP)

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