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Intermolecular spectral densities of liquids: A quantitative comparison of time-domain and frequency-domain techniques (1996)

Cong, Peijun ; Simon, John D. ; She, C. Y.

College Park, Md. : American Institute of Physics (AIP)

The Journal of Chemical Physics 104 (1996), S. 962-966

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ISSN: 1089-7690

Source: AIP Digital Archive

Topics: Physics , Chemistry and Pharmacology

Notes: Intermolecular spectral densities measured by two independent experimental techniques, time-domain optical-heterodyne-detected Raman-induced-Kerr-effect spectroscopy (OHD-RIKES) and frequency-domain stimulated gain spectroscopy (SGS), for three molecular liquids (benzene, carbon disulfide, and chloroform) are compared. The agreement in the high-frequency (interaction-induced) portion of the spectrum (20–150 cm−1) is quantitative. The relative merits between time-domain and frequency-domain coherent light-scattering techniques are discussed. © 1996 American Institute of Physics.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1063/1.470819

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