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Line mixing in the ν1 and 2ν2 isotropic Raman Q-branch of CO2 perturbed by argon and helium (1999)

Boulet, C. ; Bouanich, J.-P. ; Hartmann, J.-M.

College Park, Md. : American Institute of Physics (AIP)

The Journal of Chemical Physics 111 (1999), S. 9315-9324

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ISSN: 1089-7690

Source: AIP Digital Archive

Topics: Physics , Chemistry and Pharmacology

Notes: The shapes of the ν1 and 2ν2 isotropic Raman Q-branch of CO2 perturbed by argon and helium have been measured by Stimulated Raman Spectroscopy (SRS) or coherent anti-Stokes Raman Spectroscopy (CARS) techniques. The data have been successfully analyzed with an energy corrected sudden (ECS) approximation model based on basic rates determined independently. Finally comparison of the present data with time resolved double resonance experiments allows us to discuss the physical origin of the two empirical constants which account for the shift and broadening of the branch due to vibrational effects. © 1999 American Institute of Physics.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1063/1.480031

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