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Collision induced fragmentation of small ionic argon clusters (2002)

Barat, M. ; Brenot, J. C. ; Fayeton, J. A. ; [et al.]

College Park, Md. : American Institute of Physics (AIP)

The Journal of Chemical Physics 117 (2002), S. 1497-1506

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ISSN: 1089-7690

Source: AIP Digital Archive

Topics: Physics , Chemistry and Pharmacology

Notes: The mechanisms of collision induced fragmentation of small Arn+ (n=2–9) clusters are investigated in the 100 eV center-of-mass energy range. The velocity vectors of the fragments are measured in a multicoincidence experiment for two- and three-body fragmentation. The relative role of the two basic dynamics, electronic transitions, and momentum transfer in binary collisions is evaluated. The structure of the clusters deeply influences the type of mechanism. This is clearly the case of Ar3+ for which a specific impulsive process called "diatom" mechanism plays an important part in the fragmentation of one isomer. © 2002 American Institute of Physics.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1063/1.1485067

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