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Measurement of the rotational spectra of OH+ and OD+ by laser magnetic resonance (1986)

Gruebele, M. H. W. ; Müller, R. P. ; Saykally, R. J.

College Park, Md. : American Institute of Physics (AIP)

The Journal of Chemical Physics 84 (1986), S. 2489-2496

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ISSN: 1089-7690

Source: AIP Digital Archive

Topics: Physics , Chemistry and Pharmacology

Notes: Far IR rotational transitions between the four lowest rotational levels in the X 3Σ− vibronic ground states of OH+ and OD+ have been observed by laser magnetic resonance spectroscopy. Ground state molecular constants, including the three g factors, have been determined and employed in the calculation of a Born–Oppenheimer equilibrium geometry. The centrifugal distortion of the spin-rotation interaction is found to have a significant effect on the determination of other molecular constants. Hyperfine splittings have been resolved and analyzed for OH+, but could not be observed in OD+ spectra with a 6 MHz collision-broadened linewidth.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1063/1.450368

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