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Hole and antihole profiles in nonphotochemical hole-burned spectra (1989)

Lee, In-Ja ; Hayes, John M. ; Small, Gerald J.

College Park, Md. : American Institute of Physics (AIP)

The Journal of Chemical Physics 91 (1989), S. 3463-3469

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ISSN: 1089-7690

Source: AIP Digital Archive

Topics: Physics , Chemistry and Pharmacology

Notes: The shapes of the real-phonon and pseudophonon sideband holes (PSBH) which occur in hole-burned spectra in amorphous solids are both wavelength and burn time dependent. The theory previously proposed to simulate hole shapes in the short burn time limit is extended to examine the PSBH shapes at arbitrary times and at different burn wavelengths. The simulated spectra are compared with experimental data for tetraphenyl porphin in polystyrene. It is also shown how the simulated spectra may be used to deconvolve the antihole spectrum from the hole spectrum.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1063/1.456875

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