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  • 1
    Electronic Resource
    Electronic Resource
    Solvent influence on the magnetic field effect of polymethylene-linked photogenerated radical ion pairs (1989)
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 91 (1989), S. 4098-4105 
    Details
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: The solvent viscosity and polarity dependence of the magnetic field effect in polymethylene-linked radical ion pairs, which were generated by photoinduced intramolecular electron transfer in compounds of the type pyrene–(CH2)n–N,N-dimethylaniline, has been studied. A stochastic Liouville equation is used, in which the dynamics of the polymethylene chain, the spin Hamiltonian as a function of the varying radical distance (exchange interaction), and a distance-dependent back electron transfer rate are incorporated. The results are compared with predictions made on the basis of the (static) subensemble approximation.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1063/1.457624
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