ALBERT

Note: Contents: 1 General Introduction. - 1.1 The Climate System. - 1.2 The Atmosphere. - 1.3 Energy Budget and Atmospheric Composition. - 1.4 The Water Cycle. - 1.5 Aerosols and Climate Change. - 1.6 Outline of this Textbook. - References. - Further Reading (Textbooks and Articles. - 2 Atmospheric Aerosols. - 2.1 Definitions. - 2.2 Sources of Aerosols and Aerosol Precursors. - 2.2.1 Marine Aerosols. - 2.2.2 Desert Dust. - 2.2.3 Volcanic Aerosols. - 2.2.4 Biogenic Aerosols. - 2.2.5 Biomass Burning Aerosols. - 2.2.6 Aerosols from Fossil Fuel Combustion. - 2.3 Spatial and Temporal Aerosol Distributions. - 2.4 Aerosol-Cloud-Radiation Interactions. - 2.5 Climate Effects of Aerosols. - References. - Further Reading (Textbooks and Articles). - 3 Physical, Chemical and Optical Aerosol Properties. - 3.1 Fine, Accumulation and Coarse Modes. - 3.2 Size Distribution. - 3.3 Chemical Composition. - 3.3.1 Aerosol Mixture. - 3.3.2 Inorganic Aerosols. - 3.3.3 Black Carbon Aerosols. - 3.3.4 Organic Aerosols. - 3.3.5 Geographic Distribution of Aerosol Chemical Composition. - 3.4 Refractive Index. - 3.5 Deliquescence, Efflorescence and Hysteresis. - 3.6 Definition of Aerosol Optical Properties. - 3.6.1 Absorption and Scattering Cross Sections. - 3.6.2 Phase Function. - 3.6.3 Upscatter Fractions. - 3.7 Calculation of Aerosol Optical Properties. - 3.7.1 Mie Theory. - 3. 7.2 Extinction, Scattering and Absorption. - 3.7.3 Optical Depth and Angström Coefficient. - 3.8 Optical Properties of Nonspherical Aerosols. - 3.9 Aerosols and Atmospheric Visibility. - References. - Further Reading (Textbooks and Articles). - 4 Aerosol Modelling. - 4.1 Introduction. - 4.2 Emissions. - 4.2.1 Generalities. - 4.2.2 Fossil Fuels, Biofuels, and Other Anthropogenic Sources. - 4.2.3 Vegetation Fires. - 4.2.4 Sea Spray. - 4.2.5 Desert Dust. - 4.2.6 Dimethylsulphide. - 4.2.7 Biogenic Volatile Organic Compounds. - 4.2.8 Volcanoes. - 4.2.9 Resuspension. - 4.3 Atmospheric Processes. - 4.3.1 Nucleation. - 4.3.2 Condensation of Semi-Volatile Compounds. - 4.3.3 Coagulation. - 4.3.4 In-Cloud Aerosol Production. - 4.3.5 Wet Deposition. - 4.3.6 Dry Deposition. - 4.3.7 Sedimentation. - 4.3.8 Aerosol Transport. - 4.4 Modelling Approaches. - 4.4.1 Bulk Approach. - 4.4.2 Sectional Approach. - 4.4.3 Modal Approach. - 4.5 Example: The Sulphur Budget. - References. - Further Reading (Textbooks and Articles). - 5 Interactions of Radiation with Matter and Atmospheric Radiative Transfer. - 5.1 Introduction. - 5.2 Electromagnetic Radiation. - 5.2.1 Generalities. - 5.2.2 Definitions. - 5.3 Interactions of Radiation with Matter. - 5.3.1 Matter, Energy and Spectral Lines. - 5.3.2 Intensity of Spectral Lines. - 5.3.3 Spectral Line Profiles. - 5.3.4 Processes of lnteractions of Radiation with Matter. - 5.4 Modelling of the Interaction Processes. - 5.4.1 Molecular Absorption Coefficient. - 5.4.2 Scattering Phase Function. - 5.4.3 Molecular Scattering. - 5.4.4 Absorption and Scattering by Aerosols. - 5.4.5 Thermal Emission. - 5.5 Atmospheric Radiative Transfer. - 5.5.1 Equation of Radiative Transfer. - 5.5.2 Extinction Only. - 5.5.3 Scattering Medium. - 5.5.4 Plane-Parallel Atmosphere. - 5.5.5 Resolution of the Equation of Radiative Transfer. - 5.6 Absorption Bands, Energy, and Actinic Fluxes. - 5.6.1 Main Molecular Absorption Bands in the Atmosphere. - 5.6.2 Radiative Flux. - 5.6.3 Two-Flux Method. - 5.6.4 Stefan-Boltzmann Law. - 5.6.5 Radiative Budget. - 5.6.6 Actinic Fluxes. - 5.6.7 Polarization of Radiation. - References. - Further Reading (Textbooks and Articles). - 6 In Situ and Remote Sensing Measurements of Aerosols. - 6.1 Introduction to Aerosol Remote Sensing. - 6.2 Passive Remote Sensing: Measurement of the Extinction. - 6.2.1 General Principles. - 6.2.2 Ground-Based Photometry. - 6.2.3 Spaceborne Occultation Measurements. - 6.2.4 Retrieval of Aerosol Size Distribution. - 6.3 Passive Remote Sensing: Measurement of the Scattering. - 6.3.1 General Principles. - 6.3.2 Ground-Based Measurement of Scattered Radiation. - 6.3.3 Spaceborne Measurements of Scattered Radiation. - 6.4 Measurement of Infrared Radiation. - 6.4.1 General Principles. - 6.4.2 Spaceborne Nadir Measurement of Infrared Radiation. - 6.4.3 Spaceborne Limb Measurement of Infrared Radiation. - 6.5 Active Remote Sensing: Lidar. - 6.5.1 General Principles. - 6.5.2 The Lidar Equation. - 6.5.3 Raman Lidar. - 6.6 In Situ Aerosol Measurements. - 6.6.1 Measurement of Aerosol Concentrations. - 6.6.2 Measurement of Aerosol Chemical Composition. - 6.6.3 Measurement of Aerosol Scattering. - 6.6.4 Measurement of Aerosol Absorption. - 6.7 Conclusions. - References. - Further Reading (Textbooks and Articles). - 7 Aerosol Data Assimilation. - 7.1 Introduction. - 7.2 Basic Principles of Data Assimilation. - 7.3 Applications of Data Assimilation for Aerosols. - References. - Further Reading (Textbooks and Articles). - 8 Aerosol-Radiation Interactions. - 8.1 Introduction. - 8.2 Atmospheric Radiative Effects Due to Aerosols. - 8.2.1 Simplified Equation for Scattering Aerosols. - 8.2.2 Simplified Equation for Absorbing Aerosols. - 8.2.3 Radiative Transfer Calculations. - 8.2.4 Global Estimates and Sources of Uncertainty. - 8.3 Rapid Adjustments to Aerosol-Radiation Interactions. - 8.4 Radiative Impact of Aerosols on Surface Snow and Ice. - References. - Further Reading (Textbooks and Articles). - 9 Aerosol-Cloud lnteractions. - 39.1 Introduction. - 9 .1.1 Cloud Formation. - 9 .1.2 Cloud Distribution. - 9 .1.3 Aerosol-Cloud Interactions. - 9.2 Aerosol Effects on Liquid Clouds. - 9 .2.1 Saturation Pressure of Water Vapour. - 9.2.2 Kelvin Effect. - 9.2.3 Raoult's Law. - . - 9.2.4 Köhler Theory. - 9.2.5 Extensions to the Köhler Theory. - 9.2.6 CCN and Supersaturation in the Cloud. - 9.2.7 Dynamical and Radiative Effects in Clouds. - 9.2.8 Principle of the Cloud Albedo Effect. - 9.2.9 Observations of the Cloud Albedo Effect. - 9.2.10 Adjustments in Liquid Water Clouds. - 9.2.11 Rapid Adjustments Occurring in Liquid Clouds. - 9.3 Aerosols Effects on Mixed-Phased and Ice Clouds. - 9.3.1 Elements of Microphysics of Ice Clouds. - 9.3.2 Impact of Anthropogenic Aerosols on Ice Clouds. - 9.4 Forcing Due to Aerosol-Cloud lnteractions. - 9.5 Aerosols, Contrails and Aviation-Induced Cloudiness. - 9.5.1 Formation of Condensation Trails. - 9.5.2 Estimate of the Climate Impact of Contrails. - References. - Further Reading (Textbooks and Articles). - 10 Climate Response to Aerosol Forcings. - 10.1 Introduction. - 10.2 Radiative Forcing, Feedbacks and Climate Response. - 10.2.1 Radiative Forcing. - 10.2.2 Climate Feedbacks. - 10.2.3 Rapid Adjustments and Effective Radiative Forcing. - 10.2.4 Climate Response and Climate Efficacy. - 10.3 Climate Response to Aerosol Forcings. - 10.3.1 Equilibrium Response. - 10.3.2 Past Emissions. - 10.3.3 Detection and Attribution of Aerosol Impacts. - 10.3.4 Future Emissions Scenarios. - 10.4 Nuclear Winter. - References. - Further Reading (Textbooks and Articles). - 11 Biogeochemical Effects and Climate Feedbacks of Aerosols. - 11 .1 Introduction. - 11.2 Impact of Aerosols on Terrestrial Ecosystems. - 11.2.1 Diffuse Radiation and Primary Productivity. - 11.2.2 Aerosols as a Source of Nutrients. - 11.2.3 Acidification of Precipitation. - 11.3 Impact of Aerosols on Marine Ecosystems. - 11.4 Aerosols-Atmospheric Chemistry Interactions. - 11.4.1 Interactions with Tropospheric Chemistry. - 11.4.2 Impact of Stratospheric Aerosols on the Ozone Layer and Ultravialet Radiation. - 11.5 Climate Feedbacks Involving Marine Aerosols. - 11.5.1 Sulphate Aerosols from DMS Emissions. - 11.5.2 Marine Aerosols. - 11.5.3 Other Aerosols of Maritime Origin. - 11.6 Climate Feedbacks Involving Continental Aerosols. - 11.6.1 Secondary Organic Aerosols. - 11.6.2 Primary Aerosols of Biogenic Origin. - 11.6.3 Aerosols from Vegetation Fires. - 11.6.4 Desert Dust. - 11.7 Climate Feedbacks Involving Stratospheric Aerosols. - References. - Further Reading (Textbooks and Articles). - 12 Strato