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  • Carbon isotopes  (5)
  • American Geophysical Union  (4)
  • Springer  (1)
  • American Institute of Physics (AIP)
  • Periodicals Archive Online (PAO)
  • University of Chicago Press
  • 2020-2023  (5)
  • 1935-1939
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  • 1
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    Little change in ice age water mass structure from Cape Basin benthic neodymium and carbon isotopes (2022)
    American Geophysical Union
    Details
    Publication Date: 2022-05-27
    Description: © The Author(s), 2021. This article is distributed under the terms of the Creative Commons Attribution License. The definitive version was published in Hines, S. K. V., Bolge, L., Goldstein, S. L., Charles, C. D., Hall, I. R., & Hemming, S. R. Little change in ice age water mass structure from Cape Basin benthic neodymium and carbon isotopes. Paleoceanography and Paleoclimatology, 36(11), (2021): e2021PA004281, https://doi.org/10.1029/2021PA004281.
    Description: A common conception of the deep ocean during ice age episodes is that the upper circulation cell in the Atlantic was shoaled at the Last Glacial Maximum compared to today, and that this configuration facilitated enhanced carbon storage in the deep ocean, contributing to glacial CO2 draw-down. Here, we test this notion in the far South Atlantic, investigating changes in glacial circulation structure using paired neodymium and benthic carbon isotope measurements from International Ocean Discovery Program Site U1479, at 2,615 m water depth in the Cape Basin. We infer changes in circulation structure across the last glacial cycle by aligning our site with other existing carbon and neodymium isotope records from the Cape Basin, examining vertical isotope gradients, while determining the relative timing of inferred circulation changes at different depths. We find that Site U1479 had the most negative neodymium isotopic composition across the last glacial cycle among the analyzed sites, indicating that this depth was most strongly influenced by North Atlantic Deep Water (NADW) in both interglacial and glacial intervals. This observation precludes a hypothesized dramatic shoaling of NADW above ∼2,000 m. Our evidence, however, indicates greater stratification between mid-depth and abyssal sites throughout the last glacial cycle, conditions that developed in Marine Isotope Stage 5. These conditions still may have contributed to glacial carbon storage in the deep ocean, despite little change in the mid-depth ocean structure.
    Description: This work was supported by NSF grant OCE-1831415 (S. K. V. Hines, S. L. Goldstein., S. R. Hemming.).
    Description: 2022-04-25
    Keywords: Ocean circulation ; Neodymium isotopes ; Carbon isotopes
    Repository Name: Woods Hole Open Access Server
    Type: Article
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  • 2
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    Isotopic evidence for sources of dissolved carbon and the role of organic matter respiration in the Fraser River basin, Canada (2022)
    Springer
    Details
    Publication Date: 2022-11-04
    Description: © The Author(s), 2022. This article is distributed under the terms of the Creative Commons Attribution License. The definitive version was published in Voss, B., Eglinton, T., Peucker-Ehrenbrink, B., Galy, V., Lang, S., McIntyre, C., Spencer, R., Bulygina, E., Wang, Z., & Guay, K. Isotopic evidence for sources of dissolved carbon and the role of organic matter respiration in the Fraser River basin, Canada. Biogeochemistry. (2022), https://doi.org/10.1007/s10533-022-00945-5.
    Description: Sources of dissolved and particulate carbon to the Fraser River system vary significantly in space and time. Tributaries in the northern interior of the basin consistently deliver higher concentrations of dissolved organic carbon (DOC) to the main stem than other tributaries. Based on samples collected near the Fraser River mouth throughout 2013, the radiocarbon age of DOC exported from the Fraser River does not change significantly across seasons despite a spike in DOC concentration during the freshet, suggesting modulation of heterogeneous upstream chemical and isotopic signals during transit through the river basin. Dissolved inorganic carbon (DIC) concentrations are highest in the Rocky Mountain headwater region where carbonate weathering is evident, but also in tributaries with high DOC concentrations, suggesting that DOC respiration may be responsible for a significant portion of DIC in this basin. Using an isotope and major ion mass balance approach to constrain the contributions of carbonate and silicate weathering and DOC respiration, we estimate that up to 33 ± 11% of DIC is derived from DOC respiration in some parts of the Fraser River basin. Overall, these results indicate close coupling between the cycling of DOC and DIC, and that carbon is actively processed and transformed during transport through the river network.
    Description: Open Access funding provided by the MIT Libraries. This work was supported by the WHOI Academic Programs Office, the MIT EAPS Department Student Assistance Fund, and the PAOC Houghton Fund to BMV; NSF-ETBC grants OCE-0851015 to BPE, VG, and TIE and OCE-0851101 to RGMS; NSF grant EAR-1226818 to BPE; NSF grant OCE-0928582 to TIE and VG; and a WHOI Arctic Research Initiative grant to ZAW.
    Keywords: River ; Carbon isotopes ; Radiocarbon ; Weathering ; Carbon cycle
    Repository Name: Woods Hole Open Access Server
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  • 3
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    Soil organic carbon development and turnover in natural and disturbed salt marsh environments (2021)
    American Geophysical Union
    Details
    Publication Date: 2022-10-26
    Description: Author Posting. © American Geophysical Union, 2021. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Geophysical Research Letters 48(2), (2021): e2020GL090287, https://doi.org/10.1029/2020GL090287.
    Description: Salt marsh survival with sea‐level rise (SLR) increasingly relies on soil organic carbon (SOC) accumulation and preservation. Using a novel combination of geochemical approaches, we characterized fine SOC (≤1 mm) supporting marsh elevation maintenance. Overlaying thermal reactivity, source (δ13C), and age (F14C) information demonstrates several processes contributing to soil development: marsh grass production, redeposition of eroded material, and microbial reworking. Redeposition of old carbon, likely from creekbanks, represented ∼9%–17% of shallow SOC (≤26 cm). Soils stored marsh grass‐derived compounds with a range of reactivities that were reworked over centuries‐to‐millennia. Decomposition decreases SOC thermal reactivity throughout the soil column while the decades‐long disturbance of ponding accelerated this shift in surface horizons. Empirically derived estimates of SOC turnover based on geochemical composition spanned a wide range (640–9,951 years) and have the potential to inform predictions of marsh ecosystem evolution.
    Description: This work was supported by NSF (OCE1233678) and NOAA (NA14OAR4170104 and NA14NOS4190145) grants to ACS, USGS Coastal & Marine Geology Program, and PIE‐LTER (NSF OCE1238212 and OCE1637630).
    Description: 2021-06-11
    Keywords: Carbon isotopes ; Decomposition ; Organic matter composition ; Salt marsh ; Soil organic carbon
    Repository Name: Woods Hole Open Access Server
    Type: Article
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  • 4
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    Evidence for decreased precipitation variability in the Yucatán Peninsula during the mid-Holocene (2021)
    American Geophysical Union
    Details
    Publication Date: 2022-10-26
    Description: Author Posting. © American Geophysical Union, 2021. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Paleoceanography and Paleoclimatology 36(5), (2021): e2021PA004219, https://doi.org/10.1029/2021PA004219.
    Description: The Yucatán Peninsula (YP) has a complex hydroclimate with many proposed drivers of interannual and longer-term variability, ranging from coupled ocean–atmosphere processes to frequency of tropical cyclones. The mid-Holocene, a time of higher Northern Hemisphere summer insolation, provides an opportunity to test the relationship between YP precipitation and ocean temperature. Here, we present a new, ∼annually resolved speleothem record of stable isotope (δ18O and δ13C) and trace element (Mg/Ca and Sr/Ca) ratios for a section of the mid-Holocene (5.2–5.7 kyr BP), before extensive agriculture began in the region. A meter-long stalagmite from Río Secreto, a cave system in Playa del Carmen, Mexico, was dated using U–Th geochronology and layer counting, yielding multidecadal age uncertainty (median 2SD of ±70 years). New proxy data were compared to an existing late Holocene stalagmite record from the same cave system, allowing us to examine changes in hydrology over time and to paleoclimate records from the southern YP. The δ18O, δ13C, and Mg/Ca data consistently indicate higher mean precipitation and lower precipitation variability during the mid-Holocene compared to the late Holocene. Despite this reduced variability, multidecadal precipitation variations were persistent in regional hydroclimate during the mid-Holocene. We therefore conclude that higher summer insolation led to increased mean precipitation and decreased precipitation variability in the northern YP but that the region is susceptible to dry periods across climate mean states. Given projected decreases in wet season precipitation in the YP’s near future, we suggest that climate mitigation strategies emphasize drought preparation.
    Description: This work was funded by US National Science Foundation grants AGS-1702848 (M. Medina-Elizalde) and AGS-1502877 (S. Burns). This material is based on work supported by the National Science Foundation Graduate Research Fellowship under grant 1122374 (G. Serrato Marks). Additional support was provided by the MIT EAPS Student Research Fund and the WHOI Ocean Ventures Fund.
    Description: 2021-11-06
    Keywords: Carbon isotopes ; Drought ; Hydroclimate ; Oxygen isotopes ; Speleothems ; Trace elements ; Yucatán Peninsula
    Repository Name: Woods Hole Open Access Server
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  • 5
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    Influence of hydraulic connectivity on carbon burial efficiency in Mackenzie Delta lake sediments (2021)
    American Geophysical Union
    Details
    Publication Date: 2022-10-26
    Description: © The Author(s), 2021. This article is distributed under the terms of the Creative Commons Attribution License. The definitive version was published in Lattaud, J., Broder, L., Haghipour, N., Rickli, J., Giosan, L., & Eglinton, T., I. Influence of hydraulic connectivity on carbon burial efficiency in Mackenzie Delta lake sediments. Journal of Geophysical Research: Biogeosciences, 126(3), (2021): e2020JG006054, https://doi.org/10.1029/2020JG006054.
    Description: The Arctic is undergoing accelerated changes in response to ongoing modifications to the climate system, and there is a need for local to regional scale records of past climate variability in order to put these changes into context. The Mackenzie Delta region in northern Canada is populated by numerous small shallow lakes. They are classified as no-, low-, and high-closure (NC, LC, and HC, respectively) lakes, reflecting varying degrees of connection to the river main stem, and have different sedimentation characteristics. This study examines sedimentological (mineral surface area, grain size), carbon isotopic (bulk and molecular-level) and inorganic isotopic (neodymium) characteristics of sediment cores from three lakes representing each class. We find that HC lake sediments exhibit strikingly different properties from the other lake sediments. Specifically, they are characterized by higher organic carbon loadings per unit mineral surface area and with relatively minor influence from allochthonous, petrogenic (rock-derived) organic carbon. In contrast, LC and NC lakes have the potential to record basin-scale climatic changes at a high resolution by virtue of enhanced detrital sedimentation. Overall the delta lakes have the capacity to bury about 2 MtC year−1, with little changes in the last 200 years. However, in the (near) future, an increased number of high closure lakes might change the carbon burial efficiency of the Mackenzie Delta as they seem to retain less carbon than NC and LC lakes.
    Description: J. Lattaud was funded by a Rubicon grant (019.183EN.002) from NWO, Netherlands Organization for scientific research.
    Keywords: Bulk radiocarbon ; Carbon isotopes ; Mackenzie Delta ; Mineral loading ; N-alkanes
    Repository Name: Woods Hole Open Access Server
    Type: Article
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