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  • American Chemical Society  (44,296)
  • American Geophysical Union
  • 2025-2025
  • 2020-2022
  • 2015-2019  (51,325)
  • 2016  (51,325)
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  • 2025-2025
  • 2020-2022
  • 2015-2019  (51,325)
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  • 1
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    Intense magmatic degassing through the lake of Copahue volcano, 2013-2014 (2016)
    American Geophysical Union
    Details
    Publication Date: 2024-05-09
    Description: Here we report on the first assessment of volatile fluxes from the hyperacid crater lake hosted within the summit crater of Copahue, a very active volcano on the Argentina-Chile border. Our observations were performed using a variety of in situ and remote sensing techniques during field campaigns in March 2013, when the crater hosted an active fumarole field, and in March 2014, when an acidic volcanic lake covered the fumarole field. In the latter campaign, we found that 566 to 1373 t d−1 of SO2 were being emitted from the lake in a plume that appeared largely invisible. This, combined with our derived bulk plume composition, was converted into flux of other volcanic species (H2O ~ 10989 t d−1, CO2 ~ 638 t d−1, HCl ~ 66 t d−1, H2 ~ 3.3 t d−1, and HBr ~ 0.05 t d−1). These levels of degassing, comparable to those seen at many open-vent degassing arc volcanoes, were surprisingly high for a volcano hosting a crater lake. Copahue's unusual degassing regime was also confirmed by the chemical composition of the plume that, although issuing from a hot (65°C) lake, preserves a close-to-magmatic signature. EQ3/6 models of gas-water-rock interaction in the lake were able to match observed compositions and demonstrated that magmatic gases emitted to the atmosphere were virtually unaffected by scrubbing of soluble (S and Cl) species. Finally, the derived large H2O flux (10,988 t d−1) suggested a mechanism in which magmatic gas stripping drove enhanced lake water evaporation, a process likely common to many degassing volcanic lakes worldwide.
    Description: Published
    Description: 6071–6084
    Description: 3V. Dinamiche e scenari eruttivi
    Description: JCR Journal
    Description: restricted
    Keywords: water/rock interaction ; volcanic lakes ; volcanic/hydrothermal gases ; 04. Solid Earth::04.02. Exploration geophysics::04.02.01. Geochemical exploration ; 04. Solid Earth::04.02. Exploration geophysics::04.02.07. Instruments and techniques ; 04. Solid Earth::04.04. Geology::04.04.12. Fluid Geochemistry
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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  • 2
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    Nearshore Hydroacoustic Seafloor Mapping In The German Bight (North Sea): Hydroacoustic Interpretation With And Without Classification (2016)
    American Geophysical Union
    In:  EPIC3AGU Fall Meeting, 2016-12-2016-12American Geophysical Union
    Details
    Publication Date: 2022-09-29
    Description: Nearshore habitats are in constant dynamic change. They need regular assessment and appropriate monitoring of areas of special interest. To accomplish this, hydroacoustic seabed characterization tools are applied to allow for cost-effective and efficient mapping of the seafloor. In this context single beam echosounders (SBES) systems provide a comprehensive view by analyzing the hardness and roughness characteristics of the seafloor. Interpolation between transect lines becomes necessary when gapless maps are needed. This study presents a simple method to process and visualize data recorded with RoxAnn (Sonavision, Edinburgh, UK) and similar SBES. Both, hardness and roughness data are merged to one combined parameter that receives a color code (RGB) according to the acoustic properties of the seafloor. This color information is then interpolated to obtain an area-wide map that provides unclassified and thus unbiased seabed information. The RGB color data can subsequently be used for classification and modeling purposes. Four surveys are shown from a morphologically complex nearshore area west of the island of Helgoland (SE North Sea). The area has complex textural and dynamic characteristics reaching from outcropping bedrock via sandy to muddy areas with mostly gradual transitions. RoxAnn data allow to discriminate all seafloor types that were suggested by ground-truth information (seafloor samples, video). The area appears to be fluctuating within certain limits. Sediment import (sand and fluid mud) paths can be reconstructed. Manually, six RoxAnn zones (RZ) were identified and left without hard boundaries to better match the seafloor types of the study site. The k-means fuzzy cluster analysis employed yields best results with 3 classes. We show that interpretations on the basis of largely non-classified, color-coded and interpolated data provide the best gain of information in the highest possible resolution. Classification with hard boundaries is necessary for stakeholders but may cause reduction of information important to science. It becomes apparent that the type of classification addressing stakeholder issues is not always compatible with scientific objectives.
    Repository Name: EPIC Alfred Wegener Institut
    Type: Conference , notRev
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  • 3
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    LOBSTAHS : an adduct-based lipidomics strategy for discovery and identification of oxidative stress biomarkers (2016)
    American Chemical Society
    Details
    Publication Date: 2022-05-26
    Description: © The American Chemical Society, 2016. This is an open access article published under an ACS AuthorChoice License. The definitive version was published in Analytical Chemistry 88 (2016): 7154–7162, doi:10.1021/acs.analchem.6b01260.
    Description: Discovery and identification of molecular biomarkers in large LC/MS data sets requires significant automation without loss of accuracy in the compound screening and annotation process. Here, we describe a lipidomics workflow and open-source software package for high-throughput annotation and putative identification of lipid, oxidized lipid, and oxylipin biomarkers in high-mass-accuracy HPLC-MS data. Lipid and oxylipin biomarker screening through adduct hierarchy sequences, or LOBSTAHS, uses orthogonal screening criteria based on adduct ion formation patterns and other properties to identify thousands of compounds while providing the user with a confidence score for each assignment. Assignments are made from one of two customizable databases; the default databases contain 14 068 unique entries. To demonstrate the software’s functionality, we screened more than 340 000 mass spectral features from an experiment in which hydrogen peroxide was used to induce oxidative stress in the marine diatom Phaeodactylum tricornutum. LOBSTAHS putatively identified 1969 unique parent compounds in 21 869 features that survived the multistage screening process. While P. tricornutum maintained more than 92% of its core lipidome under oxidative stress, patterns in biomarker distribution and abundance indicated remodeling was both subtle and pervasive. Treatment with 150 μM H2O2 promoted statistically significant carbon-chain elongation across lipid classes, with the strongest elongation accompanying oxidation in moieties of monogalactosyldiacylglycerol, a lipid typically localized to the chloroplast. Oxidative stress also induced a pronounced reallocation of lipidome peak area to triacylglycerols. LOBSTAHS can be used with environmental or experimental data from a variety of systems and is freely available at https://github.com/vanmooylipidomics/LOBSTAHS.
    Description: This research was supported by the Gordon and Betty Moore Foundation through Grant GBMF3301 to B.A.S.V.M. This research was also funded in part by a grant to B.A.S.V.M. from the Simons Foundation and is a contribution of the Simons Collaboration on Ocean Processes and Ecology (SCOPE). J.R.C. acknowledges support from a U.S. Environmental Protection Agency (EPA) STAR Graduate Fellowship (Fellowship Assistance Agreement No. FP-91744301-0).
    Repository Name: Woods Hole Open Access Server
    Type: Article
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  • 4
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    Simulating gas–liquid−water partitioning and fluid properties of petroleum under pressure : implications for deep-sea blowouts (2016)
    American Chemical Society
    Details
    Publication Date: 2022-05-26
    Description: © American Chemical Society, 2016. This article is distributed under the terms of the AuthorsChoice License. The definitive version was published in Environmental Science & Technology 50 (2016): 7397–7408, doi:10.1021/acs.est.5b04617.
    Description: With the expansion of offshore petroleum extraction, validated models are needed to simulate the behaviors of petroleum compounds released in deep (〉100 m) waters. We present a thermodynamic model of the densities, viscosities, and gas–liquid−water partitioning of petroleum mixtures with varying pressure, temperature, and composition based on the Peng–Robinson equation-of-state and the modified Henry’s law (Krychevsky−Kasarnovsky equation). The model is applied to Macondo reservoir fluid released during the Deepwater Horizon disaster, represented with 279–280 pseudocomponents, including 131–132 individual compounds. We define 〉n-C8 pseudocomponents based on comprehensive two-dimensional gas chromatography (GC × GC) measurements, which enable the modeling of aqueous partitioning for n-C8 to n-C26 fractions not quantified individually. Thermodynamic model predictions are tested against available laboratory data on petroleum liquid densities, gas/liquid volume fractions, and liquid viscosities. We find that the emitted petroleum mixture was ∼29–44% gas and ∼56–71% liquid, after cooling to local conditions near the broken Macondo riser stub (∼153 atm and 4.3 °C). High pressure conditions dramatically favor the aqueous dissolution of C1−C4 hydrocarbons and also influence the buoyancies of bubbles and droplets. Additionally, the simulated densities of emitted petroleum fluids affect previous estimates of the volumetric flow rate of dead oil from the emission source.
    Description: This research was made possible by grants from the NSF (OCE- 0960841, OCE-1043976, and EAR-0950600) and the Gulf of Mexico Research Initiative (GoMRI) to the C-IMAGE and DEEP-C consortia.
    Repository Name: Woods Hole Open Access Server
    Type: Article
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  • 5
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    Tools for the microbiome : nano and beyond (2016)
    American Chemical Society
    Details
    Publication Date: 2022-05-25
    Description: © American Chemical Society, 2015. This article is posted here by permission of American Chemical Society; copying and redistribution for non-commercial research and education purposes only. The definitive version was published in ACS Nano 10 (2016): 6-37, doi:10.1021/acsnano.5b07826.
    Description: The microbiome presents great opportunities for understanding and improving the world around us and elucidating the interactions that compose it. The microbiome also poses tremendous challenges for mapping and manipulating the entangled networks of interactions among myriad diverse organisms. Here, we describe the opportunities, technical needs, and potential approaches to address these challenges, based on recent and upcoming advances in measurement and control at the nanoscale and beyond. These technical needs will provide the basis for advancing the largely descriptive studies of the microbiome to the theoretical and mechanistic understandings that will underpin the discipline of microbiome engineering. We anticipate that the new tools and methods developed will also be more broadly useful in environmental monitoring, medicine, forensics, and other areas.
    Description: This research was supported by the Office of Naval Research Grant #N000141410051 (P.S.W., G.C.L.W., and T.Y.), the Genomic Science Program of the U.S. DOE-OBER,
    Repository Name: Woods Hole Open Access Server
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  • 6
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    Emission of gas and atmospheric dispersion of SO2 during the December 2013 eruption at San Miguel volcano (El Salvador, Central America). (2016)
    American Geophysical Union
    Details
    Publication Date: 2022-05-04
    Description: Abstract San Miguel volcano, El Salvador, erupted on 29 December 2013, after a 46 year period characterized by weak activity. Prior to the eruption a trend of increasing SO2 emission rate was observed, with all values measured after mid-November greater than the average value of the previous year (~310 t d 1). During the eruption, SO2 emissions increased from the level of ~330 t d 1 to 2200 t d 1, dropping after the eruption to an average level of 680 t d 1. Wind measurements and SO2 emission rates during the preeruptive, syneruptive, and posteruptive stages were used to model SO2 dispersion around the volcano. Atmospheric SO2 concentration exceeded the dangerous threshold of 5 ppm in the crater region and in some sectors with medium elevation of the highly visited volcanic cone. Combining the SO2 emission rate with measured CO2/SO2, HCl/SO2, and HF/SO2 plume gas ratios, we estimate the CO2, HCl, and HF outputs for the first time on this volcano.
    Description: Published
    Description: 5847–5854
    Description: 3V. Dinamiche e scenari eruttivi
    Description: JCR Journal
    Description: restricted
    Keywords: SO2 flux, Clorine and CO2 at San miguel, cloud dispersion and hazard ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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  • 7
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    Gas emission strength and evolution of the molar ratio of BrO/SO2 in the plume of Nyiragongo in comparison to Etna (2016)
    American Geophysical Union
    Details
    Publication Date: 2021-06-25
    Description: Airborne and ground-based differential optical absorption spectroscopy observations have been carried out at the volcano Nyiragongo (Democratic Republic of Congo) tomeasure SO2 and bromine monoxide (BrO) in the plume inMarch 2004 and June 2007, respectively. Additionally filter pack andmulticomponent gas analyzer system (Multi-GAS)measurements were carried out in June 2007. Ourmeasurements provide valuable information on the chemical composition of the volcanic plume emitted fromthe lava lake of Nyiragongo. The main interest of this study has been to investigate for the first time the bromine emission flux of Nyiragongo (a rift volcano) and the BrO formation in its volcanic plume. Measurement data and results from a numerical model of the evolution of BrO in Nyiragongo volcanic plume are compared with earlier studies of the volcanic plume of Etna (Italy). Even though the bromine flux from Nyiragongo (2.6 t/d) is slightly greater than that from Etna (1.9 t/d), the BrO/SO2 ratio (maximum 7 × 10 5) is smaller than in the plume of Etna (maximum 2.1 × 10 4). A one-dimensional photochemical model to investigate halogen chemistry in the volcanic plumes of Etna and Nyiragongo was initialized using data from Multi-GAS and filter pack measurements. Model runs showed that the differences in the composition of volcanic volatiles led to a smaller fraction of total bromine being present as BrO in the Nyiragongo plume and to a smaller BrO/SO2 ratio.
    Description: Published
    Description: 277-291
    Description: 4V. Vulcani e ambiente
    Description: JCR Journal
    Description: restricted
    Keywords: Intraplate volcano Nyiragongo is bromine rich although chlorine poor ; BrO/Br in volcanic plumes depends on initial plume composition ; Determination of Nyiragongo chlorine, bromine, sulfur emission strength ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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  • 8
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    Are there new findings in the search for ULF magnetic precursors to earthquakes? (2016)
    American Geophysical Union
    Details
    Publication Date: 2021-02-10
    Description: Moore (1964) in a letter published in Nature reported disturbances in geomagnetic field data prior to the 27 March 1964 Alaska earthquake. After the publication of this report, many papers have shown magnetic changes preceding earthquakes. However, a causal relationship between preearthquake magnetic changes and impending earthquakes has never been demonstrated. As a consequence, after 50 years, magnetic disturbances in the geomagnetic field are still candidate precursory phenomena. Some researchers consider the investigation of ultra low frequency (ULF: 0.001–10 Hz) magnetic data the correct approach for identifying precursory signatures of earthquakes. Other researchers, instead, have recently reviewed many published ULF magnetic changes that preceded earthquakes and have shown that these are not actual precursors. The recent studies by Currie and Waters (2014) and Han et al. (2014) aim to provide relevant new findings in the search for ULF magnetic precursory signals. However, in order to contribute to science, alleged precursors must be shown to be valid and reproducible by objective testing. Here we will briefly discuss the state of the art in the search for ULF magnetic precursors, paying special attention to the recent findings of Currie and Waters (2014) and Han et al. (2014). We do not see in these two reports significant evidence that may support the observation of precursory signatures of earthquakes in ULF magnetic records.
    Description: Published
    Description: 10289–10304
    Description: 1A. Geomagnetismo e Paleomagnetismo
    Description: JCR Journal
    Description: restricted
    Keywords: Geomagnetic field ; Magnetic anomalies ; Earthquake precursors ; 01. Atmosphere::01.03. Magnetosphere::01.03.03. Magnetospheric physics ; 04. Solid Earth::04.05. Geomagnetism::04.05.04. Magnetic anomalies
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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  • 9
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    Seismic hydraulic fracture migration originated by successive deep magma pulses: The 2011–2013 seismic series associated to the volcanic activity of El Hierro Island (2016)
    American Geophysical Union
    Details
    Publication Date: 2020-12-15
    Description: In thismanuscript we present a new interpretation of the seismic series that accompanied eruptive activity off the coast of El Hierro, Canary Islands, during 2011–2013. We estimated temporal variations of the Gutenberg-Richter b value throughout the period of analysis, and performed high-precision relocations of the preeruptive and syneruptive seismicity using a realistic 3-D velocity model. Our results suggest that eruptive activity and the accompanying seismicity were caused by repeated injections of magma from the mantle into the lower crust. These magma pulses occurred within a small and well-defined volume resulting in the emplacement of fresh magma along the crust-mantle boundary underneath El Hierro. We analyzed the distribution of earthquake hypocenters in time and space in order to assess seismic diffusivity in the lower crust. Our results suggest that very high earthquake rates underneath El Hierro represent the response of a stable lower crust to stress perturbations with pulsatory character, linked to the injection of magma from the mantle. Magma input from depth caused large stress perturbations to propagate into the lower crust generating energetic seismic swarms. The absence of any preferential alignment in the spatial pattern of seismicity reinforces our hypothesis that stress perturbation and related seismicity, had diffusive character. We conclude that the temporal and spatial evolution of seismicity was neither tracking the path of magma migration nor it defines the boundaries of magma storage volumes such as a midcrustal sill. Our conceptual model considers pulsatorymagma injection fromthe uppermantle and its propagation along the Moho.We suggest, within this framework, that the spatial and temporal distributions of earthquake hypocenters reflect hydraulic fracturing processes associated with stress propagation due to magma movement.
    Description: Published
    Description: 7749–7770
    Description: 1T. Geodinamica e interno della Terra
    Description: JCR Journal
    Description: restricted
    Keywords: b value, relocation, Hydraulic fracturing, Magma influx ; 05. General::05.02. Data dissemination::05.02.99. General or miscellaneous
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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  • 10
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    Bioavailability and Chronic Toxicity of Metal Sulfide Minerals to Benthic Marine Invertebrates: Implications for Deep Sea Exploration, Mining and Tailings Disposal (2016)
    American Chemical Society
    In:  Environmental Science & Technology, 50 (7). pp. 4061-4070.
    Details
    Publication Date: 2020-12-02
    Description: The exploration and proposed mining of sulfide massive deposits in deep-sea environments and increased use deep-sea tailings placement (DSTP) in coastal zones has highlighted the need to better understand the fate and effects of mine-derived materials in marine environments. Metal sulfide ores contain high concentrations of metal(loid)s, of which a large portion exist in highly mineralized or sulfidised forms and are predicted to exhibit low bioavailability. In this study, sediments were spiked with a range of natural sulfide minerals (including chalcopyrite, chalcocite, galena, sphalerite) to assess the bioavailability and toxicity to benthic invertebrates (bivalve survival and amphipod survival and reproduction). The metal sulfide phases were considerably less bioavailable than metal contaminants introduced to sediment in dissolved forms, or in urban estuarine sediments contaminated with mixtures of metal(loid)s. Compared to total concentrations, the dilute-acid extractable metal(loid) (AEM) concentrations, which are intended to represent the more oxidized and labile forms, were more effective for predicting the toxicity of the sulfide mineral contaminated sediments. The study indicates that sediment quality guidelines based on AEM concentrations provide a useful tool for assessing and monitoring the risk posed by sediments impacted by mine-derived materials in marine environments.
    Type: Article , PeerReviewed
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