ALBERT

Description: Saharan dust was observed over the Caribbean basin during the summer 2007 NASA Tropical Composition, Cloud, and Climate Coupling (TC4) field experiment. Airborne Cloud Physics Lidar (CPL) and satellite observations from MODIS suggest a barrier to dust transport across Central America into the eastern Pacific. We use the NASA GEOS-5 atmospheric transport model with online aerosol tracers to perform simulations of the TC4 time period in order to understand the nature of this barrier. Our simulations are driven by the Modem Era Retrospective-Analysis for Research and Applications (MERRA) meteorological analyses. We evaluate our baseline simulated dust distributions using MODIS and CALIOP satellite and ground-based AERONET sun photometer observations. GEOS-5 reproduces the observed location, magnitude, and timing of major dust events, but our baseline simulation does not develop as strong a barrier to dust transport across Central America as observations suggest. Analysis of the dust transport dynamics and lost processes suggest that while both mechanisms play a role in defining the dust transport barrier, loss processes by wet removal of dust are about twice as important as transport. Sensitivity analyses with our model showed that the dust barrier would not exist without convective scavenging over the Caribbean. The best agreement between our model and the observations was obtained when dust wet removal was parameterized to be more aggressive, treating the dust as we do hydrophilic aerosols.

Description: In situ measurements of ice crystal concentrations and sizes made with aircraft instrumentation over the past two decades have often indicated the presence of numerous relatively small (〈 50 m diameter) crystals in cirrus clouds. Further, these measurements frequently indicate that small crystals account for a large fraction of the extinction in cirrus clouds. The fact that the instruments used to make these measurements, such as the Forward Scattering Spectrometer Probe (FSSP) and the Cloud Aerosol Spectrometer (CAS), ingest ice crystals into the sample volume through inlets has led to suspicion that the indications of numerous small ]crystals could be artifacts of large ]crystal shattering on the instrument inlets. We present new aircraft measurements in anvil cirrus sampled during the Tropical Composition, Cloud, and Climate Coupling (TC4) campaign with the 2 ] Dimensional Stereo (2D ]S) probe, which detects particles as small as 10 m. The 2D ]S has detector "arms" instead of an inlet tube. Since the 2D ]S probe surfaces are much further from the sample volume than is the case for the instruments with inlets, it is expected that 2D ]S will be less susceptible to shattering artifacts. In addition, particle inter ]arrival times are used to identify and remove shattering artifacts that occur even with the 2D ]S probe. The number of shattering artifacts identified by the 2D ]S interarrival time analysis ranges from a negligible contribution to an order of magnitude or more enhancement in apparent ice concentration over the natural ice concentration, depending on the abundance of large crystals and the natural small ]crystal concentration. The 2D ]S measurements in tropical anvil cirrus suggest that natural small ]crystal concentrations are typically one to two orders of magnitude lower than those inferred from CAS. The strong correlation between the CAS/2D ]S ratio of small ]crystal concentrations and large ]crystal concentration suggests that the discrepancy is likely caused by shattering of large crystals on the CAS inlet. We argue that past measurements with CAS in cirrus with large crystals present may contain errors due to crystal shattering, and past conclusions derived from these measurements may need to be revisited. Further, we present correlations between CAS spurious concentration and 2D ]S large ]crystal mass from spatially uniform anvil cirrus sampling periods as an approximate guide for estimating quantitative impact of large ]crystal shattering on CAS concentrations in previous datasets. We use radiative transfer calculations to demonstrate that in the maritime anvil cirrus sampled during TC4, small crystals indicated by 2D ]S contribute relatively little cloud extinction, radiative forcing, or radiative heating in the anvils, regardless of anvil age or vertical location in the clouds. While 2D ]S ice concentrations in fresh anvil cirrus may often exceed 1 cm.3, and are observed to exceed 10 cm.3 in turrets, they are typically ~0.1 cm.3 and rarely exceed 1 cm.3 (〈1.4% of the time) in aged anvil cirrus. We hypothesize that isolated occurrences of higher ice concentrations in aged anvil cirrus may be caused by ice nucleation driven by either small ]scale convection or gravity waves. It appears that the numerous small crystals detrained from convective updrafts do not persist in the anvil cirrus sampled during TC ]4.

Description: This paper presents a comparison of volume extinction coefficients in tropical ice clouds retrieved from two instruments : the 532-nm Cloud Physics Lidar (CPL), and the in-situ probe Cloud Integrating Nephelometer (CIN). Both instruments were mounted on airborne platforms during the CRYSTAL-FACE campaign and took measurements in ice clouds up to 17km. Coincident observations from three cloud cases are compared : one synoptically-generated cirrus cloud of low optical depth, and two ice clouds located on top of convective systems. Emphasis is put on the vertical variability of the extinction coefficient. Results show small differences on small spatial scales (approx. 100m) in retrievals from both instruments. Lidar retrievals also show higher extinction coefficients in the synoptic cirrus case, while the opposite tendency is observed in convective cloud systems. These differences are generally variations around the average profile given by the CPL though, and general trends on larger spatial scales are usually well reproduced. A good agreement exists between the two instruments, with an average difference of less than 16% on optical depth retrievals.

Description: An eruption of Italian volcano Mount Etna on 3 December 2015 produced fast-moving sulfur dioxide (SO2) and sulfate aerosol clouds that traveled across Asia and the Pacific Ocean, reaching North America in just 5days. The Ozone Profiler and Mapping Suite's Nadir Mapping UV spectrometer aboard the U.S. National Polar-orbiting Partnership satellite observed the horizontal transport of the SO2 cloud. Vertical profiles of the colocated volcanic sulfate aerosols were observed between 11.5 and 13.5 km by the new Cloud Aerosol Transport System (CATS) space-based lidar aboard the International Space Station. Backward trajectory analysis estimates the SO2 cloud altitude at 7-12 km. Eulerian model simulations of the SO2 cloud constrained by CATS measurements produced more accurate dispersion patterns compared to those initialized with the back trajectory height estimate. The near-real-time data processing capabilities of CATS are unique, and this work demonstrates the use of these observations to monitor and model volcanic clouds.

Description: A method of retrieving cloud microphysical properties using combined observations from both cloud radar and lidar is introduced. This retrieval makes use of an improvement to the traditional optimal estimation retrieval method, whereby a series of corrections are applied to the state vector during the search for an iterative solution. This allows faster convergence to a solution and is less processor intensive. The method is first applied to a synthetic cloud t o demonstrate its validity, and it is shown that the retrieval reliably reproduces vertical profiles of ice water content. The retrieval method is then applied to radar and lidar observations from the CRYSTAL-FACE experiment, and vertical profiles of ice crystal diameter, number concentration, and ice water content are retrieved for a cirrus cloud layers observed one day of that experiment. The validity of the relationship between visible extinction coefficient and radar reflectivity was examined. While synthetic tests showed such a functional relationship, the measured data only partially supported such a conclusion. This is due to errors in the forward model (as explained above) as well as errors in the data sets, including possible mismatch between lidar and radar profiles or errors in the optical depth. Empirical relationships between number concentrations and mean particle diameter were also examined. The results indicate that a distinct and robust relationship exists between these retrieved quantities and it is argued that such a relationship is more than an artifact of the retrieval process offering insight into the nature of the microphysical processes taking place in cirrus.

Description: During the NASA Cirrus Regional Study of Tropical Anvils and Cirrus Layers-Florida Area Cirrus Experiment (CRYSTAL-FACE) enhanced mixing ratios of nitric oxide were measured in the anvils of thunderstorms and in clear air downwind of storm systems on flights of a Wl3-57F high-altitude aircraft. Mixing ratios greater than l0 - 20 times background were readily observed over distances of 25-120 km due to lightning activity. In many of the Florida storms deposition of NO occurred up to near the tropopause but major deposition usually occurred 1 - 2 km below the tropopause, or mostly within the visible anvil volume formed prior to storm decay. Observations from two storms of very different anvil size and electrical activity allowed estimates of the total mass of NO, vented to the middle and upper troposphere. Using the cloud-to ground (CG) flash accumulations from the National Lightning Detection Network, climatological intra-cloud (IC) to CG ratios, and assuming that CG and IC flashes were of equivalent efficiency for NO production, the ranges of production per flash for a moderate-sized and a large storm were (0.51 - 1.0) x l0(exp 26) and (2.3 - 3.1) x 10(exp 26) molecules NO/flash, respectively. Using the recently determined average global flash rate of 44 8, a gross extrapolation of these two storms to represent possible global annual production rates yield 1.6 - 3.2 and 7.3 - 9.9 Tg(N)/yr, respectively. If the more usual assumption is made that IC efficiency is l/l0th that of CG activity, the ranges of production for the moderate-sized and large storm were (1.3 - 2.7) x l0(exp 26) and (6.0 - 8.1) x l0(exp 26) molecules NO/CG flash, respectively. The estimates from the large storm may be high because there is indirect evidence that the IC/CG ratio was larger than would be derived from climatology. These two storms and others studied did not have flash rates that scaled as approx. H(sup 5) where H is the cloud top altitude. The observed CG flash accumulations and NO(x) mass production estimate for the month of July over the Florida area were compared with a representative 3D global Chemistry-Transport Model (CTMJ that uses the Price et al. lightning parameterization. For two land grid points representing the Florida peninsula the model compared well with the observations: CG flash rates were low by only a factor of approx. 2. When the model grid points included the coastal regions of Florida the flash accumulations were lower than observed by a factor of 3.4 - 4.6. It is recommended that models using the Price et al. parameterization allow any global coastal grid point to maintain the land rather than the marine flash rate parameterization. The convection in this CTM underestimated the actual cloud top heights over Florida by 1 - 2 km and thus the total lightning flash rates and the altitude range of reactive nitrogen deposition. Broad scale (20 - 120 km) median mixing ratios of NO within anvils over Florida were significantly larger than in storms previously investigated over Colorado and New Mexico.

Description: A key focus of CRYSTAL-FACE (Cirrus Regional Study of Tropical Anvils and cirrus Layers - Florida Area Cirrus Experiment) was the generation and subsequent evolution of cirrus outflow from deep convective cloud systems. A preliminary integrated look at the observations of an extended cirrus anvil cloud system observed on 23 July 2002 will be presented, including lidar and millimeter radar observations from NASA's ER-2 and in- situ observations from NASA's WB-57 and University of North Dakota Citation. The observations will be compared to preliminary results of simulations using 1-D and 2-D high-resolution (100 meter) cloud resolving models. The CRMs explicitly account for cirrus microphysical development by resolving the evolving ice crystal size distribution (bin model) in time and space. Both homogeneous and heterogeneous nucleation are allowed in the model. The CRM simulations are driven using the output of regional simulations using MM5 that produces deep convection similar to what was observed. The MM5 model employs a 2 km inner grid (32 layers) over a 360 km domain, nested within a 6 km grid over a 600 km domain. Initial and boundary conditions for the 36- hour MM5 simulation are taken from NCEP Eta model analysis at 32 km resolution. Key issues to be explored are the settling of the observed anvil versus the model simulations, and comparisons of dynamical properties, such as vertical motions, occurring in the observations and models. The former provides an integrated measure of the validity of the model microphysics (fallspeed) while the latter is the key factor in forcing continued ice generation.

Description: Physical thickness of a cloud layer, and sometimes multiple cloud layers, can be estimated from the time delay of off-beam returns from a pulsed laser source illuminating one side of the cloud layer. In particular, the time delay of light returning from the outer diffuse halo of light surrounding the beam entry point, relative to the time delay at beam center, determines the cloud physical thickness. The delay combined with the pulse stretch gives the optical thickness. The halo method works best for thick cloud layers, typically optical thickness exceeding 2, and thus compliments conventional lidar which cannot penetrate thick clouds. Cloud layer top and base have been measured independently over the ARM/SGP site using conventional laser ranging (lidar) and the top minus base thickness are compared with a cloud top halo estimate obtained from the NASA/Goddard THOR System (THOR = THickness from Offbeam Returns). THOR flies on the NASA P3, and measures the halo timings from several km above cloud top, at the same time providing conventional lidar cloud top height. The ARM/SGP micropulse lidar provides cloud base height for validation.

Description: The February through March 2014 deployment of the NASA Airborne Tropical TRopopause EXperiment (ATTREX) provided unique in situ measurements in the western Pacific Tropical Tropopause Layer (TTL). Six flights were conducted from Guam with the long-range, high-altitude, unmanned Global Hawk aircraft. The ATTREX Global Hawk payload provided measurements of water vapor, meteorological conditions, cloud properties, tracer and chemical radical concentrations, and radiative fluxes. The campaign was partially coincident with the CONTRAST and CAST airborne campaigns based in Guam using lower-altitude aircraft The ATTREX dataset is being used for investigations of TTL cloud, transport, dynamical, and chemical processes as well as for evaluation and improvement of global-model representations of TTL processes.

Description: Physical thickness of a cloud layer, sometimes multiple cloud layers, is a crucial controller of solar heating of the Earth- atmosphere system, which drives the convective processes that produce storm systems. Yet clouds of average optical thickness are opaque to conventional lidar, so their thickness is well estimated only by combining a lidar above and another below cloud, or a radar and lidar on the same side, dual facilities not widely available. Here we report initial observations of a new airborne multiple field of view lidar, capable of determining physical thickness of cloud layers from time signatures of off-beam returns from a I kHz micropulse lidar at 540 rim. For a single layer, the time delay of light returning from the outer diffuse halo of light surrounding the beam entry point, relative to the time delay at beam center, determines the cloud physical thickness. The delay combined with the pulse stretch gives the optical thickness. This halo method requires cloud optical thickness exceeding 2, and improves with cloud thickness, thus complimenting conventional lidar, which cannot penetrate thick clouds. Results are presented from March 25, 2002, when THOR flew a butterfly pattern over the ARM site at 8.3 km, above a thin ice cloud at 5 km, and a thick boundary-layer stratus deck with top at 1.3 km, as shown by THOR channel 1, and a base at about 0.3 km as shown by the ground-based MPL. Additional information is included in the original extended abstract.