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  • 1
    Call number: AWI A12-96-0373
    In: Publication / Commission of the European Communities
    Type of Medium: Monograph available for loan
    Pages: V, 471 S.
    ISBN: 9282682811
    Series Statement: Publication / Commission of the European Communities EUR 16209 EN
    Branch Library: AWI Library
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  • 2
    Publication Date: 2018-12-11
    Description: A regional modeling study on the impact of desert dust on cloud formation is presented for a major Saharan dust outbreak over Europe from 2 to 5 April 2014. The dust event coincided with an extensive and dense cirrus cloud layer, suggesting an influence of dust on atmospheric ice nucleation. Using interactive simulation with the regional dust model COSMO-MUSCAT, we investigate cloud and precipitation representation in the model and test the sensitivity of cloud parameters to dust–cloud and dust–radiation interactions of the simulated dust plume. We evaluate model results with ground-based and spaceborne remote sensing measurements of aerosol and cloud properties, as well as the in situ measurements obtained during the ML-CIRRUS aircraft campaign. A run of the model with single-moment bulk microphysics without online dust feedback considerably underestimated cirrus cloud cover over Germany in the comparison with infrared satellite imagery. This was also reflected in simulated upper-tropospheric ice water content (IWC), which accounted for only 20 % of the observed values. The interactive dust simulation with COSMO-MUSCAT, including a two-moment bulk microphysics scheme and dust–cloud as well as dust–radiation feedback, in contrast, led to significant improvements. The modeled cirrus cloud cover and IWC were by at least a factor of 2 higher in the relevant altitudes compared to the noninteractive model run. We attributed these improvements mainly to enhanced deposition freezing in response to the high mineral dust concentrations. This was corroborated further in a significant decrease in ice particle radii towards more realistic values, compared to in situ measurements from the ML-CIRRUS aircraft campaign. By testing different empirical ice nucleation parameterizations, we further demonstrate that remaining uncertainties in the ice-nucleating properties of mineral dust affect the model performance at least as significantly as including the online representation of the mineral dust distribution. Dust–radiation interactions played a secondary role for cirrus cloud formation, but contributed to a more realistic representation of precipitation by suppressing moist convection in southern Germany. In addition, a too-low specific humidity in the 7 to 10 km altitude range in the boundary conditions was identified as one of the main reasons for misrepresentation of cirrus clouds in this model study.
    Print ISSN: 1680-7316
    Electronic ISSN: 1680-7324
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 3
    Publication Date: 2018-07-12
    Description: Air traffic affects cloudiness, and thus climate, by emitting exhaust gases and particles. The study of the evolution of contrail properties is very challenging due to the complex interplay of vortex dynamics and the atmospheric environment (e.g. temperature, supersaturation). Despite substantial progress in recent years, the optical, microphysical, and macrophysical properties of contrails and ambient cirrus during contrail formation and subsequent ageing are still subject to large uncertainties due to instrumental and observational limitations and the large number of variables influencing the contrail life cycle. In this study, various contrail cases corresponding to different aircraft types and atmospheric conditions are investigated using a statistical method based on the in situ optical measurements performed during the Contrail and Cirrus Experiments (CONCERT) campaigns 2008 and 2011. The two aircraft campaigns encompass more than 17 aircraft contrail cases. A principal component analysis (PCA) of the angular scattering coefficients measured by the polar nephelometer is implemented. The goal is to classify the sampled ice cloud measurements in several clusters representative of different contrail development stages (primary wake, young contrail, aged contrail, and cirrus). Extinction and asymmetry coefficients, nitrogen oxide concentrations, and relative humidity with respect to ice and particle size distributions are analysed for each cluster to characterize the evolution of ice cloud properties during the contrail to cirrus evolution. The PCA demonstrates that contrail optical properties are well suited to identify and discriminate between the different contrail growth stages and to characterize the evolution of contrail properties.
    Print ISSN: 1680-7316
    Electronic ISSN: 1680-7324
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 4
    Publication Date: 2017-02-14
    Description: This study has two objectives: (1) it characterizes contrails at very low temperatures and (2) it discusses convective cirrus in which the contrails occurred. (1) Long-lived contrails and cirrus from overshooting convection are investigated above the tropical tropopause at low temperatures down to −88 °C from measurements with the Russian high-altitude research aircraft M-55 Geophysica, as well as related observations during the SCOUT-O3 field experiment near Darwin, Australia, in 2005. A contrail was observed to persist below ice saturation at low temperatures and low turbulence in the stratosphere for nearly 1 h. The contrail occurred downwind of the decaying convective system Hector of 16 November 2005. The upper part of the contrail formed at 19 km altitude in the tropical lower stratosphere at ∼ 60 % relative humidity over ice at −82 °C. The ∼ 1 h lifetime is explained by engine water emissions, slightly enhanced humidity from Hector, low temperature, low turbulence, and possibly nitric acid hydrate formation. The long persistence suggests large contrail coverage in case of a potential future increase of air traffic in the lower stratosphere. (2) Cirrus observed above the strongly convective Hector cloud on 30 November 2005 was previously interpreted as cirrus from overshooting convection. Here we show that parts of the cirrus were caused by contrails or are mixtures of convective and contrail cirrus. The in situ data together with data from an upward-looking lidar on the German research aircraft Falcon, the CPOL radar near Darwin, and NOAA-AVHRR satellites provide a sufficiently complete picture to distinguish between contrail and convective cirrus parts. Plume positions are estimated based on measured or analyzed wind and parameterized wake vortex descent. Most of the non-volatile aerosol measured over Hector is traceable to aircraft emissions. Exhaust emission indices are derived from a self-match experiment of the Geophysica in the polar stratosphere in 2010. The number of ice particles in the contrails is less than 1 % of the number of non-volatile aerosol particles, possibly because of sublimation losses and undetected very small ice particles. The radar data show that the ice water content in convective overshoots is far higher than measured along the flight path. These findings add insight into overshooting convection and are of relevance with respect to hydration of the lower stratosphere.
    Print ISSN: 1680-7316
    Electronic ISSN: 1680-7324
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 5
    Publication Date: 2018-11-27
    Description: Accurate measurement of water vapor in the climate-sensitive region near the tropopause is very challenging. Unexplained systematic discrepancies between measurements at low water vapor mixing ratios made by different instruments on airborne platforms have limited our ability to adequately address a number of relevant scientific questions on the humidity distribution, cloud formation and climate impact in that region. Therefore, during the past decade, the scientific community has undertaken substantial efforts to understand these discrepancies and improve the quality of water vapor measurements. This study presents a comprehensive intercomparison of airborne state-of-the-art in situ hygrometers deployed on board the DLR (German Aerospace Center) research aircraft HALO (High Altitude and LOng Range Research Aircraft) during the Midlatitude CIRRUS (ML-CIRRUS) campaign conducted in 2014 over central Europe. The instrument intercomparison shows that the hygrometer measurements agree within their combined accuracy (±10 % to 15 %, depending on the humidity regime); total mean values agree within 2.5 %. However, systematic differences on the order of 10 % and up to a maximum of 15 % are found for mixing ratios below 10 parts per million (ppm) H2O. A comparison of relative humidity within cirrus clouds does not indicate a systematic instrument bias in either water vapor or temperature measurements in the upper troposphere. Furthermore, in situ measurements are compared to model data from the European Centre for Medium-Range Weather Forecasts (ECMWF) which are interpolated along the ML-CIRRUS flight tracks. We find a mean agreement within ±10 % throughout the troposphere and a significant wet bias in the model on the order of 100 % to 150 % in the stratosphere close to the tropopause. Consistent with previous studies, this analysis indicates that the model deficit is mainly caused by too weak of a humidity gradient at the tropopause.
    Print ISSN: 1680-7316
    Electronic ISSN: 1680-7324
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 6
    Publication Date: 2017-11-21
    Description: Earth's surface temperature sensitivity to radiative forcing (RF) by contrail cirrus and the related RF efficacy relative to CO2 are investigated in a one-dimensional idealized model of the atmosphere. The model includes energy transport by shortwave (SW) and longwave (LW) radiation and by mixing in an otherwise fixed reference atmosphere (no other feedbacks). Mixing includes convective adjustment and turbulent diffusion, where the latter is related to the vertical component of mixing by large-scale eddies. The conceptual study shows that the surface temperature sensitivity to given contrail RF depends strongly on the timescales of energy transport by mixing and radiation. The timescales are derived for steady layered heating (ghost forcing) and for a transient contrail cirrus case. The radiative timescales are shortest at the surface and shorter in the troposphere than in the mid-stratosphere. Without mixing, a large part of the energy induced into the upper troposphere by radiation due to contrails or similar disturbances gets lost to space before it can contribute to surface warming. Because of the different radiative forcing at the surface and at top of atmosphere (TOA) and different radiative heating rate profiles in the troposphere, the local surface temperature sensitivity to stratosphere-adjusted RF is larger for SW than for LW contrail forcing. Without mixing, the surface energy budget is more important for surface warming than the TOA budget. Hence, surface warming by contrails is smaller than suggested by the net RF at TOA. For zero mixing, cooling by contrails cannot be excluded. This may in part explain low efficacy values for contrails found in previous global circulation model studies. Possible implications of this study are discussed. Since the results of this study are model dependent, they should be tested with a comprehensive climate model in the future.
    Print ISSN: 1680-7316
    Electronic ISSN: 1680-7324
    Topics: Geosciences
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  • 7
    Publication Date: 2017-01-10
    Description: Mean properties of individual contrails are characterized for a wide range of jet aircraft as a function of age during their life cycle from seconds to 11.5 h (7.4–18.7 km altitude, −88 to −31 °C ambient temperature), based on a compilation of about 230 previous in situ and remote sensing measurements. The airborne, satellite, and ground-based observations encompass exhaust contrails from jet aircraft from 1972 onwards, as well as a few older data for propeller aircraft. The contrails are characterized by mean ice particle sizes and concentrations, extinction, ice water content, optical depth, geometrical depth, and contrail width. Integral contrail properties include the cross-section area and total number of ice particles, total ice water content, and total extinction (area integral of extinction) per contrail length. When known, the contrail-causing aircraft and ambient conditions are characterized. The individual datasets are briefly described, including a few new analyses performed for this study, and compiled together to form a contrail library (COLI). The data are compared with results of the Contrail Cirrus Prediction (CoCiP) model. The observations confirm that the number of ice particles in contrails is controlled by the engine exhaust and the formation process in the jet phase, with some particle losses in the wake vortex phase, followed later by weak decreases with time. Contrail cross sections grow more quickly than expected from exhaust dilution. The cross-section-integrated extinction follows an algebraic approximation. The ratio of volume to effective mean radius decreases with time. The ice water content increases with increasing temperature, similar to non-contrail cirrus, while the equivalent relative humidity over ice saturation of the contrail ice mass increases at lower temperatures in the data. Several contrails were observed in warm air above the Schmidt–Appleman threshold temperature. The emission index of ice particles, i.e., the number of ice particles formed in the young contrail per burnt fuel mass, is estimated from the measured concentrations for estimated dilution; maximum values exceed 1015 kg−1. The dependence of the data on the observation methods is discussed. We find no obvious indication for significant contributions from spurious particles resulting from shattering of ice crystals on the microphysical probes.
    Print ISSN: 1680-7316
    Electronic ISSN: 1680-7324
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 8
    Publication Date: 2017-10-13
    Description: Air traffic affects the cloudiness, and thus the climate, by emitting exhaust gases and particles. The study of the evolution of contrail properties is very challenging due to the complex interplay of vortex dynamics and atmospheric environment (e.g. temperature, supersaturation). Despite substantial progress in recent years, the optical, microphysical, and macrophysical properties of contrails and ambient cirrus during contrail formation and subsequent ageing are still subject to large uncertainties due to instrumental and observational limitations and the large number of variables influencing the contrail life cycle. In this study, various contrail cases corresponding to different aircraft types and atmospheric conditions are investigated using a statistical method based on the in situ optical measurements performed during the CONCERT campaigns 2008 and 2011. These two aircraft campaigns encompass more than 17 aircraft contrail cases. A Principal Component Analysis (PCA) of the angular scattering coefficients measured by the Polar Nephelometer has been implemented in order to classify the sampled ice cloud measurements in 6 clusters representative of different development stages of the contrails (primary wake, young contrail, contrail-cirrus and natural cirrus). Based on the information derived from air traffic control, extinction coefficients, asymmetry coefficients, nitrogen oxide concentrations, relative humidity with respect to ice (RHI) and particle size distributions are analyzed for each cluster to provide a characterization of the evolution of ice-cloud properties during the contrail to cirrus evolution. The PCA demonstrates that contrail optical properties are well suited to identify and discriminate the different contrail growth stages and to provide an independent method for the characterization of the evolution of contrail properties.
    Electronic ISSN: 1680-7375
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 9
    Publication Date: 2017-05-29
    Description: Earth surface temperature changes induced by added thin cirrus or contrails are investigated with a radiative-convective-diffusive model, basically without climate system changes, with relaxation of the temperature profile by radiation and mixing. The conceptual study shows that the surface temperature sensitivity to cirrus depends strongly on the ratio of the time scales of energy transport by mixing and radiation, where mixing may include turbulent diffusion, convection and transports by the large-scale circulation. The time scales are derived for steady layered heating (ghost-forcing) and for a transient cirrus case. The time scales are shortest at the surface and shorter in the troposphere than in the mid-stratosphere. Heat induced by cirrus in the upper troposphere reaches the surface only for strong vertical mixing. The local surface-temperature sensitivity to adjusted radiative forcing (RF) is larger for the shortwave (SW) than the longwave (LW) cirrus forcing. For weak mixing, cirrus may cool the surface even if the cirrus causes a positive instantaneous or stratosphere-adjusted radiative forcing (RF) at the tropopause. The shorter time scales near the surface indicate a potential for dominant SW surface cooling regionally where cirrus or contrails form, while weak LW warming may dominate at larger distances.
    Electronic ISSN: 1680-7375
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 10
    Publication Date: 2016-09-15
    Description: Mean properties of individual contrails are characterized for a wide range of jet aircraft as a function of age during their lifecycle from seconds to 11.5 hours (7.4 to 18.7 km altitude, −88 °C to −31 °C ambient temperature), based on a compilation of about 230 previous in-situ and remote sensing measurements. The airborne, satellite, and ground-based observations encompass exhaust contrails from jet aircraft since 1972, and a few older data for propeller aircraft. The contrails are characterized by mean ice particle sizes and concentrations, extinction, ice water content, optical depth, geometrical depth, and contrail width. Integral contrail properties include the cross-section area and total number of ice particles, total ice water content, and total extinction (area-integral of extinction) per contrail length. When known, the contrail-causing aircraft and ambient conditions are characterized. The individual datasets are briefly described, including a few new analyses performed for this study, and compiled together to form a "contrail library" (COLI). The data are compared with results of the Contrail Cirrus Prediction model CoCiP. The observations confirm that the number of ice particles in contrails is controlled by the engine exhaust and the formation process in the jet phase, with some particle losses in the wake vortex phase, followed later by weak decreases with time. Contrail cross-sections grow more quickly than expected from exhaust dilution. The cross-section integrated extinction follows an algebraic approximation. The ratio of volume to effective mean radius decreases with time. The ice water content increases with increasing temperature, similar to non-contrail cirrus, while the equivalent relative humidity over ice saturation of the contrail ice mass increases at lower temperatures in the data. Several contrails were observed in warm air above the Schmidt–Appleman threshold temperature. The “emission index” of ice particles, i.e. the number of ice particles formed in the young contrail per burnt fuel mass, is estimated from the measured concentrations for estimated dilution; maximum values exceed 1015 kg−1. The dependence of the data on the observation methods is discussed. We find no obvious indication for significant contributions from spurious particles resulting from shattering of ice crystals on the microphysical probes.
    Electronic ISSN: 1680-7375
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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