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  • 1
    Publication Date: 2023-12-19
    Description: The formation of the Aralkum (Aral Desert), following the severe desiccation of the former Aral Sea since the 1960s, has created what may be regarded as one of the world's most significant anthropogenic dust sources. In this paper, focusing on dust emission and transport patterns from the Aralkum, the dust life‐cycle has been simulated over Central Asia using the aerosol transport model COSMO‐MUSCAT (COnsortium for Small‐scale MOdelling‐MUltiScale Chemistry Aerosol Transport Model), making use of the Global Surface Water data set to take into account the sensitivity to changes in surface water coverage over the region between the 1980s (the “past”) and the 2010s (the “present”). Over a case study 1‐year period, the simulated dust emissions from the Aralkum region increased from 14.3 to 27.1 Tg year〈sup〉−1〈/sup〉 between the past and present, an increase driven solely by the changes in the surface water environment. Of these simulated modern emissions, 14.5 Tg are driven by westerly winds, indicating that regions downwind to the east may be worst affected by Aralkum dust. However a high degree of interannual variability in the prevailing surface wind patterns ensures that these transport patterns of Aralkum dust do not occur every year. Frequent cloud cover poses substantial challenges for observations of Central Asian dust: in the Aralkum, over two‐thirds of the yearly emissions are emitted under overcast skies, dust which may be impossible to observe using traditional satellite or ground‐based passive remote sensing techniques. Furthermore, it is apparent that the pattern of dust transport from the Aralkum under clear‐sky conditions is not representative of the pattern under all‐sky conditions.
    Description: Plain Language Summary: Since the 1960s the Central Asian lake that used to be known as the Aral Sea has almost completely dried out, due to human activity. This environmental disaster has created a new desert known as the Aralkum (the “Aral Desert”), which now has a size of 245 km × 245 km across. Dried lakes such as the Aralkum can be very effective sources of wind‐driven atmospheric dust. The soils of the Aralkum are also contaminated with agricultural chemicals from nearby croplands, making the Aralkum a major regional threat to human health. Using an atmospheric computer model, we explore the consequences of the new Aralkum for the patterns of atmospheric dust and their potential impacts in Central Asia. We find that the new Aralkum has contributed an extra 7% per year to the total dust quantity over Central Asia, however due to thick cloud cover over two thirds of this dust from the Aralkum cannot be seen by Earth‐observing satellites. The wind patterns over the Aralkum vary from year to year, so while our simulations predict that most of the Aralkum's dust is transported to the east during the simulation year, during other years plenty more dust will be transported elsewhere.
    Description: Key Points: The impact of changes in surface water coverage over the Aralkum (the former Aral Sea) for dust emission and transport is investigated. There is a high degree of interannual variability in the directions of dust‐emitting winds over the Aralkum. Over two thirds of Aralkum dust activity occurs under thick cloud cover, limiting the possibility of it being observed by satellites.
    Description: Deutsche Forschungsgemeinschaft http://dx.doi.org/10.13039/501100001659
    Description: https://doi.org/10.5281/zenodo.6022747
    Description: https://global-surface-water.appspot.com/download
    Description: https://soilgrids.org/
    Description: https://search.earthdata.nasa.gov/search
    Description: https://cds.climate.copernicus.eu/cdsapp#!/dataset/reanalysis-era5-single-levels
    Description: https://ads.atmosphere.copernicus.eu/cdsapp#!/dataset/cams-global-reanalysis-eac4
    Description: https://ladsweb.modaps.eosdis.nasa.gov/search/
    Description: https://aeronet.gsfc.nasa.gov/
    Description: https://worldview.earthdata.nasa.gov/
    Keywords: ddc:551.5 ; dust aerosol ; Aralkum ; Central Asia ; modeling
    Language: English
    Type: doc-type:article
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  • 2
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    In:  Leibniz-Institut für Troposphärenforschung e.V., Leipzig | Supplement to: Schacht, Jacob; Heinold, Bernd; Quaas, Johannes; Backman, John; Cherian, Ribu; Ehrlich, André; Herber, Andreas; Huang, Wan Ting Katty; Kondo, Y; Massling, Andreas; Sinha, P R; Weinzierl, Bernadett; Zanatta, Marco; Tegen, Ina (2019): The importance of the representation of air pollution emissions for the modeled distribution and radiative effects of black carbon in the Arctic. Atmospheric Chemistry and Physics, 19(17), 11159-11183, https://doi.org/10.5194/acp-19-11159-2019
    Publication Date: 2023-10-28
    Description: All data as used in the Schacht et al. (2019) paper. This includes mothly means of: - BC sedimentation - BC drydeposition - BC wetdeposition - BC emission Monthly Arctic fieldsums of: - SO4 emission - SO2 emission 2005 to 2015 fieldmeans of: - BC burden - aerosol DRE (LW & SW, TOA & BOA) - aerosol DRE without bc (LW & SW, TOA & BOA) - DRE of BC-in-snow (SW, TOA & BOA) Timeseries of BC mass mixing ratios connected to measurements: - at Alert, Oulanka, Barrow, Ny-Alesund, Villum, Tiksi, Pallas, Summit, Zeppelin Station, Gates of the Arctic NP, Trapper Creek, Tuxedni, Simeonof and Denali NP - for the campaigns ACLOUD, Pamarcmip 2017, HIPPO, ACCESS and ARCTAS
    Keywords: AC3; Arctic; Arctic Amplification; File content; File format; File name; File size; modelled; pan-Arctic; Uniform resource locator/link to file
    Type: Dataset
    Format: text/tab-separated-values, 225 data points
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  • 3
    Publication Date: 2017-02-01
    Description: The Midlatitude Cirrus experiment (ML-CIRRUS) deployed the High Altitude and Long Range Research Aircraft (HALO) to obtain new insights into nucleation, life cycle, and climate impact of natural cirrus and aircraft-induced contrail cirrus. Direct observations of cirrus properties and their variability are still incomplete, currently limiting our understanding of the clouds’ impact on climate. Also, dynamical effects on clouds and feedbacks are not adequately represented in today’s weather prediction models. Here, we present the rationale, objectives, and selected scientific highlights of ML-CIRRUS using the G-550 aircraft of the German atmospheric science community. The first combined in situ–remote sensing cloud mission with HALO united state-of-the-art cloud probes, a lidar and novel ice residual, aerosol, trace gas, and radiation instrumentation. The aircraft observations were accompanied by remote sensing from satellite and ground and by numerical simulations. In spring 2014, HALO performed 16 flights above Europe with a focus on anthropogenic contrail cirrus and midlatitude cirrus induced by frontal systems including warm conveyor belts and other dynamical regimes (jet streams, mountain waves, and convection). Highlights from ML-CIRRUS include 1) new observations of microphysical and radiative cirrus properties and their variability in meteorological regimes typical for midlatitudes, 2) insights into occurrence of in situ–formed and lifted liquid-origin cirrus, 3) validation of cloud forecasts and satellite products, 4) assessment of contrail predictability, and 5) direct observations of contrail cirrus and their distinction from natural cirrus. Hence, ML-CIRRUS provides a comprehensive dataset on cirrus in the densely populated European midlatitudes with the scope to enhance our understanding of cirrus clouds and their role for climate and weather.
    Print ISSN: 0003-0007
    Electronic ISSN: 1520-0477
    Topics: Geography , Physics
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  • 4
    Publication Date: 2019-05-01
    Description: Clouds play an important role in Arctic amplification. This term represents the recently observed enhanced warming of the Arctic relative to the global increase of near-surface air temperature. However, there are still important knowledge gaps regarding the interplay between Arctic clouds and aerosol particles, and surface properties, as well as turbulent and radiative fluxes that inhibit accurate model simulations of clouds in the Arctic climate system. In an attempt to resolve this so-called Arctic cloud puzzle, two comprehensive and closely coordinated field studies were conducted: the Arctic Cloud Observations Using Airborne Measurements during Polar Day (ACLOUD) aircraft campaign and the Physical Feedbacks of Arctic Boundary Layer, Sea Ice, Cloud and Aerosol (PASCAL) ice breaker expedition. Both observational studies were performed in the framework of the German Arctic Amplification: Climate Relevant Atmospheric and Surface Processes, and Feedback Mechanisms (AC) project. They took place in the vicinity of Svalbard, Norway, in May and June 2017. ACLOUD and PASCAL explored four pieces of the Arctic cloud puzzle: cloud properties, aerosol impact on clouds, atmospheric radiation, and turbulent dynamical processes. The two instrumented Polar 5 and Polar 6 aircraft; the icebreaker Research Vessel (R/V) Polarstern; an ice floe camp including an instrumented tethered balloon; and the permanent ground-based measurement station at Ny-Ålesund, Svalbard, were employed to observe Arctic low- and mid-level mixed-phase clouds and to investigate related atmospheric and surface processes. The Polar 5 aircraft served as a remote sensing observatory examining the clouds from above by downward-looking sensors; the Polar 6 aircraft operated as a flying in situ measurement laboratory sampling inside and below the clouds. Most of the collocated Polar 5/6 flights were conducted either above the R/V Polarstern or over the Ny-Ålesund station, both of which monitored the clouds from below using similar but upward-looking remote sensing techniques as the Polar 5 aircraft. Several of the flights were carried out underneath collocated satellite tracks. The paper motivates the scientific objectives of the ACLOUD/PASCAL observations and describes the measured quantities, retrieved parameters, and the applied complementary instrumentation. Furthermore, it discusses selected measurement results and poses critical research questions to be answered in future papers analyzing the data from the two field campaigns.
    Print ISSN: 0003-0007
    Electronic ISSN: 1520-0477
    Topics: Geography , Physics
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  • 5
    Publication Date: 2020-04-21
    Description: The spatial distribution and properties of submicron organic aerosol (OA) are among the key sources of uncertainty in our understanding of aerosol effects on climate. Uncertainties are particularly large over remote regions of the free troposphere and Southern Ocean, where very few data have been available and where OA predictions from AeroCom Phase II global models span 2 to 3 orders of magnitude, greatly exceeding the model spread over source regions. The (nearly) pole-to-pole vertical distribution of non-refractory aerosols was measured with an aerosol mass spectrometer onboard the NASA DC-8 aircraft as part of the Atmospheric Tomography (ATom) mission during the Northern Hemisphere summer (August 2016) and winter (February 2017). This study presents the first extensive characterization of OA mass concentrations and their level of oxidation in the remote atmosphere. OA and sulfate are the major contributors by mass to submicron aerosols in the remote troposphere, together with sea salt in the marine boundary layer. Sulfate was dominant in the lower stratosphere. OA concentrations have a strong seasonal and zonal variability, with the highest levels measured in the lower troposphere in the summer and over the regions influenced by biomass burning from Africa (up to 10 µg sm−3). Lower concentrations (∼0.1–0.3 µg sm−3) are observed in the northern middle and high latitudes and very low concentrations (
    Print ISSN: 1680-7316
    Electronic ISSN: 1680-7324
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 6
    Publication Date: 2020-07-13
    Description: The magnitude of solar radiative effects (cooling or warming) of black carbon (BC) particles embedded in the Arctic atmosphere and surface snow layer was explored on the basis of case studies. For this purpose, combined atmospheric and snow radiative transfer simulations were performed for cloudless and cloudy conditions on the basis of BC mass concentrations measured in pristine early summer and more polluted early spring conditions. The area of interest is the remote sea-ice-covered Arctic Ocean in the vicinity of Spitsbergen, northern Greenland, and northern Alaska typically not affected by local pollution. To account for the radiative interactions between the black-carbon-containing snow surface layer and the atmosphere, an atmospheric and snow radiative transfer model were coupled iteratively. For pristine summer conditions (no atmospheric BC, minimum solar zenith angles of 55∘) and a representative BC particle mass concentration of 5 ng g−1 in the surface snow layer, a positive daily mean solar radiative forcing of +0.2 W m−2 was calculated for the surface radiative budget. A higher load of atmospheric BC representing early springtime conditions results in a slightly negative mean radiative forcing at the surface of about −0.05 W m−2, even when the low BC mass concentration measured in the pristine early summer conditions was embedded in the surface snow layer. The total net surface radiative forcing combining the effects of BC embedded in the atmosphere and in the snow layer strongly depends on the snow optical properties (snow specific surface area and snow density). For the conditions over the Arctic Ocean analyzed in the simulations, it was found that the atmospheric heating rate by water vapor or clouds is 1 to 2 orders of magnitude larger than that by atmospheric BC. Similarly, the daily mean total heating rate (6 K d−1) within a snowpack due to absorption by the ice was more than 1 order of magnitude larger than that of atmospheric BC (0.2 K d−1). Also, it was shown that the cooling by atmospheric BC of the near-surface air and the warming effect by BC embedded in snow are reduced in the presence of clouds.
    Print ISSN: 1680-7316
    Electronic ISSN: 1680-7324
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 7
    Publication Date: 2020-07-24
    Description: Atmospheric aerosol particles are the precondition for the formation of cloud droplets and therefore have large influence on the microphysical and radiative properties of clouds. In this work, four different methods to derive or measure number concentrations of cloud condensation nuclei (CCN) were analyzed and compared for present-day aerosol conditions: (i) a model parameterization based on simulated particle concentrations, (ii) the same parameterization based on gravimetrical particle measurements, (iii) direct CCN measurements with a CCN counter, and (iv) lidar-derived and in situ measured vertical CCN profiles. In order to allow for sensitivity studies of the anthropogenic impact, a scenario to estimate the maximum CCN concentration under peak aerosol conditions of the mid-1980s in Europe was developed as well. In general, the simulations are in good agreement with the observations. At ground level, average values between 0.7 and 1.5×109 CCN m−3 at a supersaturation of 0.2 % were found with the different methods under present-day conditions. The discrimination of the chemical species revealed an almost equal contribution of ammonium sulfate and ammonium nitrate to the total number of CCN for present-day conditions. This was not the case for the peak aerosol scenario, in which it was assumed that no ammonium nitrate was formed while large amounts of sulfate were present, consuming all available ammonia during ammonium sulfate formation. The CCN number concentration at five different supersaturation values has been compared to the measurements. The discrepancies between model and in situ observations were lowest for the lowest (0.1 %) and highest supersaturations (0.7 %). For supersaturations between 0.3 % and 0.5 %, the model overestimated the potentially activated particle fraction by around 30 %. By comparing the simulation with observed profiles, the vertical distribution of the CCN concentration was found to be overestimated by up to a factor of 2 in the boundary layer. The analysis of the modern (year 2013) and the peak aerosol scenario (expected to be representative of the mid-1980s over Europe) resulted in a scaling factor, which was defined as the quotient of the average vertical profile of the peak aerosol and present-day CCN concentration. This factor was found to be around 2 close to the ground, increasing to around 3.5 between 2 and 5 km and approaching 1 (i.e., no difference between present-day and peak aerosol conditions) with further increasing height.
    Print ISSN: 1680-7316
    Electronic ISSN: 1680-7324
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 8
    Publication Date: 2020-09-16
    Description: It was hypothesized that using mineral dust emission climatologies in global chemistry climate models (GCCMs), i.e. prescribed monthly-mean dust emissions representative of a specific year, may lead to misrepresentations of strong dust burst events. This could result in a negative bias of model dust concentrations compared to observations for these episodes. Here, we apply the aerosol microphysics submodel MADE3 (Modal Aerosol Dynamics model for Europe, adapted for global applications, third generation) as part of the ECHAM/MESSy Atmospheric Chemistry (EMAC) general circulation model. We employ two different representations of mineral dust emissions for our model simulations: (i) a prescribed monthly-mean climatology of dust emissions representative of the year 2000 and (ii) an online dust parametrization which calculates wind-driven mineral dust emissions at every model time step. We evaluate model results for these two dust representations by comparison with observations of aerosol optical depth from ground-based station data. The model results show a better agreement with the observations for strong dust burst events when using the online dust representation compared to the prescribed dust emissions setup. Furthermore, we analyse the effect of increasing the vertical and horizontal model resolution on the mineral dust properties in our model. We compare results from simulations with T42L31 and T63L31 model resolution (2.8∘×2.8∘ and 1.9∘×1.9∘ in latitude and longitude, respectively; 31 vertical levels) with the reference setup (T42L19). The different model versions are evaluated against airborne in situ measurements performed during the SALTRACE mineral dust campaign (Saharan Aerosol Long-range Transport and Aerosol-Cloud Interaction Experiment, June–July 2013), i.e. observations of dust transported from the Sahara to the Caribbean. Results show that an increased horizontal and vertical model resolution is able to better represent the spatial distribution of airborne mineral dust, especially in the upper troposphere (above 400 hPa). Additionally, we analyse the effect of varying assumptions for the size distribution of emitted dust but find only a weak sensitivity concerning these changes. The results of this study will help to identify the model setup best suited for future studies and to further improve the representation of mineral dust particles in EMAC-MADE3.
    Print ISSN: 1991-959X
    Electronic ISSN: 1991-9603
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 9
    Publication Date: 2015-12-01
    Print ISSN: 1352-2310
    Electronic ISSN: 1873-2844
    Topics: Energy, Environment Protection, Nuclear Power Engineering , Geosciences , Physics
    Published by Elsevier
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  • 10
    Publication Date: 2012-03-01
    Print ISSN: 1352-2310
    Electronic ISSN: 1873-2844
    Topics: Energy, Environment Protection, Nuclear Power Engineering , Geosciences , Physics
    Published by Elsevier
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