Electronic Resource
College Park, Md.
:
American Institute of Physics (AIP)
The Journal of Chemical Physics
107 (1997), S. 8759-8780
ISSN:
1089-7690
Source:
AIP Digital Archive
Topics:
Physics
,
Chemistry and Pharmacology
Notes:
Two-pulse four-wave-mixing signals from molecular aggregates, including effects of two-exciton states, static disorder, and exciton-phonon interaction represented by arbitrary spectral densities are calculated. Three types of contributions to the signal are identified. The first, reflecting exciton self-correlation, is similar to the photon echo from disordered two-level systems and dominates the signal for long time-delays. The second is related to correlations of one-exciton states, whereas the third reflects correlations between one- and two-exciton states. The information gained by completely resolving the signal field (both amplitude and phase) is analyzed using Wigner spectrograms. © 1997 American Institute of Physics.
Type of Medium:
Electronic Resource
URL:
http://dx.doi.org/10.1063/1.475169
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