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  • 1
    Electronic Resource
    Electronic Resource
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 107 (1997), S. 8759-8780 
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: Two-pulse four-wave-mixing signals from molecular aggregates, including effects of two-exciton states, static disorder, and exciton-phonon interaction represented by arbitrary spectral densities are calculated. Three types of contributions to the signal are identified. The first, reflecting exciton self-correlation, is similar to the photon echo from disordered two-level systems and dominates the signal for long time-delays. The second is related to correlations of one-exciton states, whereas the third reflects correlations between one- and two-exciton states. The information gained by completely resolving the signal field (both amplitude and phase) is analyzed using Wigner spectrograms. © 1997 American Institute of Physics.
    Type of Medium: Electronic Resource
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  • 2
    Electronic Resource
    Electronic Resource
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 107 (1997), S. 3876-3893 
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: A real-space formulation of time-resolved fluorescence of molecular aggregates is developed using the one-exciton density matrix ρ(t) of the optically driven system. A direct relationship is established between the superradiance enhancement factor Ls and the exciton coherence size Lρ associated with the off-diagonal density matrix elements in the molecular representation. Various factors which affect the latter, including finite temperature, energetic disorder, coupling with phonons, and polaron formation are explored. The theory is applied for the interpretation of recent measurements in the B850 system of the LH2 photosynthetic complexes. © 1997 American Institute of Physics.
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  • 3
    Electronic Resource
    Electronic Resource
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 106 (1997), S. 3837-3853 
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: The optical response of CdSe semiconductor nanocrystals is investigated using the reduced single-electron density matrix in real space, calculated by means of the time-dependent Hartree–Fock technique. The spectroscopic signatures of exciton confinement are analyzed using the frequency-dependent electronic coherence matrix (off-diagonal density-matrix elements). The effects of Hartree and the Fock (exchange) type Coulomb interactions on the exciton binding energy are discussed. The latter result in almost dark excitons situated energetically below the main transition. Off-diagonal Coulomb matrix elements lead to larger exciton binding energies compared with previous calculations, and result in a better agreement of the size dependence of the lowest optical transition with experiment. © 1997 American Institute of Physics.
    Type of Medium: Electronic Resource
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  • 4
    Electronic Resource
    Electronic Resource
    Woodbury, NY : American Institute of Physics (AIP)
    Applied Physics Letters 73 (1998), S. 2612-2614 
    ISSN: 1077-3118
    Source: AIP Digital Archive
    Topics: Physics
    Notes: Absorption and differential electroabsorption spectra of a GaInAs/InP superlattice in the regime of Wannier–Stark localization are compared with spectra derived from the Semiconductors Bloch Equations. The absorption is strongly underestimated for higher energies by the effective mass approximation but good agreement is achieved by using an energy dependent in-plane effective mass. No fitting parameters are used except for a phenomenological broadening. The lineshape of the field-modulated spectra is dominated by the strong field dependence of Wannier–Stark transitions and depends on the amplitude of the modulating field which should be kept small for best results. © 1998 American Institute of Physics.
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  • 5
    Electronic Resource
    Electronic Resource
    Woodbury, NY : American Institute of Physics (AIP)
    Applied Physics Letters 67 (1995), S. 2978-2980 
    ISSN: 1077-3118
    Source: AIP Digital Archive
    Topics: Physics
    Notes: Quasiequilibrium nonlinear optical absorption spectra are computed for semiconductor superlattices. The theory generalizes the semiconductor Bloch equations to describe anisotropic structures. The equation for the interband polarization is solved numerically and the carrier-density dependent optical nonlinearities are computed. Starting from excitonic absorption, with increasing density exciton saturation and the development of gain is observed. The dependence of the gain spectra on structural parameters of the superlattice is discussed. © 1995 American Institute of Physics.
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  • 6
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    Publication Date: 2020-02-12
    Type: info:eu-repo/semantics/workingPaper
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  • 7
    Publication Date: 2020-02-12
    Type: info:eu-repo/semantics/workingPaper
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