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  • 1
    Electronic Resource
    Electronic Resource
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 92 (1990), S. 358-363 
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: Ionization potentials (IPs) for carbon clusters containing 6–24 atoms have been determined from charge transfer reactions of carbon cluster ions with compounds of known ionization potential in a Fourier transform ion cyclotron resonance mass spectrometer. Cluster IPs generally decrease with increasing cluster size, but the IPs for clusters containing 4n+3 atoms (n=1–5) are found to be ∼0.5 eV lower than those of neighboring clusters. The relationship between cluster IP and structure is discussed.
    Type of Medium: Electronic Resource
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  • 2
    Electronic Resource
    Electronic Resource
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 94 (1991), S. 3556-3562 
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: The ionization potentials (IPs) of several large carbon clusters Cn (n≥48), including the enhanced abundance ("magic number'') clusters C50, C60, and C70, have been determined by Fourier transform ion cyclotron resonance (FTICR) mass spectrometric charge transfer bracketing experiments. The IPs of C50, C60, and C70 were bracketed by the same two charge transfer compounds, leading to a common value of 7.61±0.11 eV. The IPs of even numbered clusters adjacent to these magic number clusters were found to be lower by as much as 0.5 eV and all clusters between C50 and C200 were determined to have IPs greater than 6.20 eV. The reaction rates of C+60 and C+70 with metallocenes were anomalously slow in comparison to the other large carbon cluster ions. IP and reactivity results suggest that C50, C60, and C70 may indeed have different or more stable structures than neighboring clusters, which supports the hypothesis of closed-shell, spherical species. The implications of these results for the mechanism of C+n formation by direct laser vaporization are also discussed.
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  • 3
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 75 (1994), S. 6069-6071 
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: Triple-axis inelastic polarized neutron measurements have been performed as a function of temperature on a single crystal of the Invar alloy Fe65Ni35 to distinguish longitudinal from transverse magnetic excitations in the magnetically ordered phase. Well below the Curie temperature of 501 K the magnetic excitation spectrum is dominated by conventional transverse spin-wave excitations, which in fact follow the predictions of spin-wave theory very well. In particular, we find no evidence for propagating longitudinal excitations in this system, in sharp contrast to the behavior observed in the amorphous Invar Fe86B14 material as well as the non-Invar amorphous system Fe40Ni40P14B6.
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  • 4
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: We have performed inelastic neutron scattering measurements of the long-wavelength spin wave excitations of both ordered and disordered Fe72Pt28 single crystals below their critical temperatures, TC=510 and 375 K, respectively. The spin waves followed the expected E=Dq2 dependence, and the temperature-dependent spin stiffness D decreased as (T/TC)5/2, as expected for an isotropic ferromagnet. The extrapolated zero-temperature spin stiffness was D=98(4) meV A(ring)2 and 107(1) meV A(ring)2 for the disordered and ordered alloy, respectively. These values are significantly higher than the zero-temperature stiffness as determined by magnetization measurements.
    Type of Medium: Electronic Resource
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  • 5
    Electronic Resource
    Electronic Resource
    New York, NY : American Institute of Physics (AIP)
    Physics of Fluids 4 (1992), S. 3747-3752 
    ISSN: 1089-7666
    Source: AIP Digital Archive
    Topics: Physics
    Notes: A CO2 laser was used to irradiate hollow polystyrene cylinders along their axis. The laser-generated high-energy electrons appear to uniformly heat the cylinder throughout its volume and the cylinder explodes. The imploding and stagnation character of the exploding cylinder gives rise to a long x-ray pulse, much longer than the laser pulse, and to a peak emission that occurs after the laser pulse. The fast ions that are generated appear not to interact with the thermal plasma. Two-dimensional calculations that reproduce much of the experimental x-ray signature and observed hydrodynamic flow are presented.
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  • 6
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Physics of Fluids 6 (1994), S. 3200-3202 
    ISSN: 1089-7666
    Source: AIP Digital Archive
    Topics: Physics
    Notes: This note attempts to connect the skewness of the probability distribution function (PDF) of pressure, which is commonly observed in two-dimensional turbulence, to differences in the geometry of the strain and vorticity fields. This paper illustrates analytically the respective roles of strain and vorticity in shaping the PDF of pressure, in the particular case of a joint normal distribution of velocity gradients. The latter assumption is not valid in general in direct numerical simulations (DNS) of two-dimensional turbulence but may apply to geostrophic turbulence in presence of a differential rotation (β effect). In essence, minus the Laplacian of pressure is the difference of squared strain and vorticity, a quantity which is named the generalized centrifugal force divergence (GCFD). Square strain and vorticity distributions follow chi-square statistics with unequal numbers of degrees of freedom, when one assumes a joint normal distribution of their components. Squared strain has two degrees of freedom and squared vorticity only one, thereby causing a skewness of the PDF of GCFD and hence of pressure.
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  • 7
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 70 (1991), S. 6537-6539 
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: Elastic anomalies in an Fe75Pt25 single crystal have been investigated by ultrasonic pulse echo and inelastic neutron scattering measurements in the temperature range 200 to 800 K. The single crystal which was grown by the Bridgman–Stockbarger process undergoes a magnetic transition at Tc = 370 K and a martensitic transformation at Ms = 200 K corresponding to a degree of order of S=0.7. Both ultrasonics and neutron scattering reveal a softening of the transverse modes below Tc. The excess elastic constants obey an M2 law as expected from a local magnetoelastic interaction model. The longitudinal ultrasonic velocities already start to soften at 700 K whereas the neutron data for the same acoustic branch do not show any anomaly down to 200 K. The observed q dependences of the acoustic branches point towards a softening confined to the very center of the Brillouin zone.
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  • 8
    ISSN: 1077-3118
    Source: AIP Digital Archive
    Topics: Physics
    Notes: A detector stage comprising a photodiode, a field-effect transistor, and a load resistor, and a wavelength demultiplexer have been monolithically integrated in the GaInAsP/InP material system. Chips were mounted into complete modules and operated in a 1.3 μm/1.55 μm bidirectional transmission link. At 576 Mbit/s and 10−9 bit error rate the sensitivity of the module was −21 dBm, while the intrinsic sensitivity of the receiver was determined to be −28 dBm.
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