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  • 1
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Review of Scientific Instruments 60 (1989), S. 730-734 
    ISSN: 1089-7623
    Source: AIP Digital Archive
    Topics: Physics , Electrical Engineering, Measurement and Control Technology
    Notes: We present the design and performance of an alkali ion source which is the injection stage of an ion beam system for surface scattering experiments in the range of 10 eV to 10 keV. In order to maximize emitter lifetimes, emphasis was placed on obtaining low phase space beams which minimize current losses in later stages of the optics. The source is based on a commercially available solid state β-eucryptite emitter, uses two stages of extraction for independent control of extracted current and final beam energy, and has a modified Pierce confinement electrode to control space charge spreading inside the source. Results of computer ray tracing are included to illustrate the operation of this source. Tests with K+ ions at 500 eV have produced beams which, in the range of 600–700 nA, were space-charge limited in transport through the remainder of the system. Beam currents measured more than 1 m downstream of the source are nearly independent of the emitter surface temperature over a range of 1023 to 1142 °C. Emitter lifetimes in excess of 200 h have been obtained. Using this source and our beamline optics, we have produced at the sample position low phase space beams ranging in energy from 10 eV to several kiloelectron volts.
    Type of Medium: Electronic Resource
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  • 2
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Review of Scientific Instruments 59 (1988), S. 2560-2567 
    ISSN: 1089-7623
    Source: AIP Digital Archive
    Topics: Physics , Electrical Engineering, Measurement and Control Technology
    Notes: We have designed and constructed an apparatus that combines hyperthermal energy ion scattering (〈100 eV) with low-energy ion scattering (a few hundred eV to several keV). The UHV scattering chamber possesses a full range of sample preparation and characterization capabilities, including LEED, Auger spectroscopy, a Kelvin probe for work function measurements, and facilities for gas or alkali-metal deposition. The differentially pumped beamline provides well-collimated, monoenergetic beams of gas or alkali-metal ions ranging in energy from 〈10 eV to 10 keV. To illustrate the qualitative changes in the scattering behavior observed over this range, we present experimental results for Na+ scattered off the Cu(110) surface with the incident ion energy ranging from 56 eV to 4 keV. We also show a comparison between 1 keV K+ and 1 keV Ar+ scattered from the same surface.
    Type of Medium: Electronic Resource
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  • 3
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Review of Scientific Instruments 59 (1988), S. 137-145 
    ISSN: 1089-7623
    Source: AIP Digital Archive
    Topics: Physics , Electrical Engineering, Measurement and Control Technology
    Notes: We have constructed and tested an UHV beamline to produce beams of alkali metal and noble gas ions over the energy range 〈20 eV to 10 keV with energy resolution ΔE/E of 1% or better. At the sample position, we have attained tens of nanoamps of current for keV energy beams in a 1–2-mm beam spot with about ±1° angular divergence, and nanoamps of current at 25 eV in a 4-mm beam spot with ±2° angular divergence. By applying Liouville's theorem to the beam's emittance and using waist-to-waist transport through the beam optics, the current on the sample is maximized while limiting the spot size and angular divergence. To achieve useful current at the lowest energies, special attention was paid to minimizing space-charge effects. Beam emittances measured at the sample position are consistent with Liouville's theorem. Equations for waist-to-waist transport are derived in the Appendix.
    Type of Medium: Electronic Resource
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  • 4
    Electronic Resource
    Electronic Resource
    Palo Alto, Calif. : Annual Reviews
    Annual Review of Nutrition 7 (1987), S. 291-320 
    ISSN: 0199-9885
    Source: Annual Reviews Electronic Back Volume Collection 1932-2001ff
    Topics: Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Type of Medium: Electronic Resource
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  • 5
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 64 (1988), S. 5587-5591 
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: Over the past decade, we have: (1) developed phenomenological theory for the behavior of "well-ordered'' magnetic states of moderately delocalized light rare-earth and actinide systems (characteristically obtaining unusual anisotropic magnetism in agreement with experiment); (2) developed theory and computational technique to synthesize first principles electronic structure information into that phenomenological theory to make it materially predictive. As discussed in this paper, the resulting theory allows us to predict the triggering of an instability from unusual anisotropic, but well-ordered, magnetism to an unstable state. The unstable state can be either of a valence fluctuation type or of what probably is a heavy fermion type, and the detailed way in which these two types of instability is triggered differs.
    Type of Medium: Electronic Resource
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  • 6
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 63 (1988), S. 3683-3685 
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: A sharp change in the nature of the magnetic ordering has been observed on going from CeSb to CeTe, both of which have NaC1 structures with a small decrease in lattice parameter. This is an interesting example of the way in which hybridization of partially delocalized f electrons with band electrons gives rise to highly unusual magnetic properties which show great chemical sensitivity. In the present paper we apply our previous ab initio treatment of hybridization-induced effects to investigate this striking change in magnetic behavior. We have performed self-consistent warped muffin-tin LMTO band calculations treating the Ce 4f states as resonance states that are constrained to be localized. Compared to CeSb, the anion-derived p bands in CeTe sink well below the Fermi energy, thus strongly changing the band-f hybridization. We have calculated the hybridization dressing of the crystal-field levels and the anisotropic two-ion exchange interaction and compared them with those calculated for CeSb and with experiment. A strong decrease in the two-ion interaction explains the drastic change in observed magnetic behavior between CeSb and CeTe.
    Type of Medium: Electronic Resource
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  • 7
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 61 (1987), S. 3385-3387 
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: To understand the magnetic properties of moderately delocalized light actinide (uranium, neptunium, plutonium) systems, it is necessary to treat correctly the way in which the highly correlated behavior of the f electrons within the actinide ion is linked to the non-f band behavior via the hybridization process. We do this by transforming the hybridization into band-f resonant scattering. We have successfully applied the theory to PuSb by considering both dominant and next-to-dominant scattering channels.
    Type of Medium: Electronic Resource
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  • 8
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 61 (1987), S. 3388-3390 
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: Hybridization of moderately delocalized f electrons with band electrons gives rise to a highly anisotropic two-ion interaction, which, as Siemann and Cooper first showed, accounts well for the unusual magnetic behavior of CeBi. In the present paper it is shown that the even more unusual magnetic behavior of CeSb with a succession of magnetic structures in which the higher-temperature structures (AFP) involve a periodic stacking of nonmagnetic {001} planes alternating with magnetically ordered {001} planes of [001] moment alignment can be understood on the basis of the same hybridization-mediated interionic interaction in the presence of a cubic crystal field (CF) of comparable strength. The tendency to form nonmagnetic planes, which are indeed paramagnetic in nature (Kramers doublets), is found to increase with increasing CF strength, and the stability of the AFP phases at high temperatures is shown to arise from the reconciliation of the magnetic ordering with the CF interactions. The calculations yield first-order phase transitions from a low-temperature type I antiferromagnetic phase to two high-temperature AFP phases. The possibility of a fully nonmagnetic singlet ground state, which, however, is not Kondo-like, also occurs and will be discussed.
    Type of Medium: Electronic Resource
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  • 9
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 57 (1985), S. 3185-3187 
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: The unusual magnetic ordering, magnetic excitation behavior, and anomalous crystal-field splitting in CeBi and CeSb can be explained using a model Hamiltonian obtained by applying the Schrieffer–Wolff transformation to the Anderson Hamiltonian. It is highly desirable to obtain a first principles prediction of the parameters of the theory in order to extend this understanding quantitatively to other cerium and light actinide materials. To this end, we have calculated the electronic structure of CeBi and CeSb with the linear muffin-tin orbital (LMTO) method, using a self-consistent fully warped potential, and have obtained the coupling between non-f band states and f states localized in the sense of the Anderson Hamiltonian. This is applied to a calculation of the anomalous crystal-field splitting in CeBi and CeSb, and application to calculating the anisotropic two-ion interaction is discussed. We find that the dominant contribution to the anomalous crystal-field effect (about two thirds) comes from hybridization with d bands.
    Type of Medium: Electronic Resource
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  • 10
    Electronic Resource
    Electronic Resource
    Oxford, UK : Blackwell Publishing Ltd
    Annals of the New York Academy of Sciences 475 (1986), S. 0 
    ISSN: 1749-6632
    Source: Blackwell Publishing Journal Backfiles 1879-2005
    Topics: Natural Sciences in General
    Type of Medium: Electronic Resource
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