ALBERT

Description: The global variability of clouds and their interactions with aerosol and radiation make them one of our largest sources of uncertainty related to global radiative forcing. The droplet size distribution (DSD) of clouds is an excellent proxy that connects cloud microphysical properties with radiative impacts on our climate. However, traditional radiometric instruments are information-limited in their DSD retrievals. Radiometric sensors can infer droplet effective radius directly but not the distribution width, which is an important parameter tied to the growth of a cloud field and to the onset of precipitation. DSD heterogeneity hidden inside large pixels, a lack of angular information, and the absence of polarization limit the amount of information these retrievals can provide. Next-generation instruments that can measure at narrow resolutions with multiple view angles on the same pixel, a broad swath, and sensitivity to the intensity and polarization of light are best situated to retrieve DSDs at the pixel level and over a wide spatial field. The Airborne Hyper-Angular Rainbow Polarimeter (HARP) is a wide-field-of-view imaging polarimeter instrument designed by the University of Maryland, Baltimore County (UMBC), for retrievals of cloud droplet size distribution properties over a wide swath, at narrow resolution, and at up to 60 unique, co-located view zenith angles in the 670 nm channel. The cloud droplet effective radius (CDR) and variance (CDV) of a unimodal gamma size distribution are inferred simultaneously by matching measurement to Mie polarized phase functions. For all targets with appropriate geometry, a retrieval is possible, and unprecedented spatial maps of CDR and CDV are made for cloud fields that stretch both across the swath and along the entirety of a flight observation. During the NASA Lake Michigan Ozone Study (LMOS) aircraft campaign in May–June 2017, the Airborne HARP (AirHARP) instrument observed a heterogeneous stratocumulus cloud field along the solar principal plane. Our retrievals from this dataset show that cloud DSD heterogeneity can occur at the 200 m scale, much smaller than the 1–2 km resolution of most spaceborne sensors. This heterogeneity at the sub-pixel level can create artificial broadening of the DSD in retrievals made at resolutions on the order of 0.5 to 1 km. This study, which uses the AirHARP instrument and its data as a proxy for upcoming HARP CubeSat and HARP2 spaceborne instruments, demonstrates the viability of the HARP concept to make cloud measurements at scales of individual clouds, with global coverage, and in a low-cost, compact CubeSat-sized payload.

Description: The Dark Target aerosol algorithm was developed to exploit the information content available from the observations of Moderate-Resolution Imaging Spectroradiometers (MODIS), to better characterize the global aerosol system. The algorithm is based on measurements of the light scattered by aerosols toward a space-borne sensor against the backdrop of relatively dark Earth scenes, thus giving rise to the name “Dark Target”. Development required nearly a decade of research that included application of MODIS airborne simulators to provide test beds for proto-algorithms and analysis of existing data to form realistic assumptions to constrain surface reflectance and aerosol optical properties. This research in itself played a significant role in expanding our understanding of aerosol properties, even before Terra MODIS launch. Contributing to that understanding were the observations and retrievals of the growing Aerosol Robotic Network (AERONET) of sun-sky radiometers, which has walked hand-in-hand with MODIS and the development of other aerosol algorithms, providing validation of the satellite-retrieved products after launch. The MODIS Dark Target products prompted advances in Earth science and applications across subdisciplines such as climate, transport of aerosols, air quality, and data assimilation systems. Then, as the Terra and Aqua MODIS sensors aged, the challenge was to monitor the effects of calibration drifts on the aerosol products and to differentiate physical trends in the aerosol system from artefacts introduced by instrument characterization. Our intention is to continue to adapt and apply the well-vetted Dark Target algorithms to new instruments, including both polar-orbiting and geosynchronous sensors. The goal is to produce an uninterrupted time series of an aerosol climate data record that begins at the dawn of the 21st century and continues indefinitely into the future.

Description: The state-of-art satellite observations of atmospheric aerosols over the last two decades from NASA’s Moderate Resolution Imaging Spectroradiometer (MODIS) instruments have been extensively utilized in climate change and air quality research and applications. The operational algorithms now produce Level 2 aerosol data at varying spatial resolutions (1, 3, and 10 km) and Level 3 data at 1 degree. The local and global applications have benefited from the coarse resolution gridded data sets (i.e., Level 3, 1 degree), as it is easier to use since data volume is low, and several online and offline tools are readily available to access and analyze the data with minimal computing resources. At the same time, researchers who require data at much finer spatial scales have to go through a challenging process of obtaining, processing, and analyzing larger volumes of data sets that require high-end computing resources and coding skills. Therefore, we created a high spatial resolution (high-resolution gridded (HRG), 0.1 × 0.1 degree) daily and monthly aerosol optical depth (AOD) product by combining two MODIS operational algorithms, namely Deep Blue (DB) and Dark Target (DT). The new HRG AODs meet the accuracy requirements of Level 2 AOD data and provide either the same or more spatial coverage on daily and monthly scales. The data sets are provided in daily and monthly files through open an Ftp server with python scripts to read and map the data. The reduced data volume with an easy to use format and tools to access the data will encourage more users to utilize the data for research and applications.

Description: For reflected sunlight observed from space at visible and near-infrared wavelengths, particles suspended in Earth’s atmosphere provide contrast with vegetation or dark water at the surface. This is the physical motivation for the Dark Target (DT) aerosol retrieval algorithm developed for the Moderate Resolution Imaging Spectrometer (MODIS). To extend the data record of aerosol optical depth (AOD) beyond the expected 20-year lifespan of the MODIS sensors, DT must be adapted for other sensors. A version of the DT AOD retrieval for the Visible Infrared Imaging Radiometer Suite (VIIRS) on the Suomi-National Polar-Orbiting Partnership (SNPP) is now mature enough to be released as a standard data product, and includes some upgraded features from the MODIS version. Differences between MODIS Aqua and VIIRS SNPP lead to some inevitable disagreement between their respective AOD measurements, but the offset between the VIIRS SNPP and MODIS Aqua records is smaller than the offset between those of MODIS Aqua and MODIS Terra. The VIIRS SNPP retrieval shows good agreement with ground-based measurements. For most purposes, DT for VIIRS SNPP is consistent enough and in close enough agreement with MODIS to continue the record of satellite AOD. The reasons for the offset from MODIS Aqua, and its spatial and temporal variability, are investigated in this study.

Description: Multi-angle polarimetric (MAP) imaging of Earth scenes can be used for the retrieval of microphysical and optical parameters of aerosols and clouds. The Airborne Hyper-Angular Rainbow Polarimeter (AirHARP) is an aircraft MAP instrument with a hyper-angular imaging capability of 60 along-track viewing angles at 670 nm and 20 along-track viewing angles at other wavelengths – 440, 550, and 870 nm – across the full 114∘ (94∘) along-track (cross-track) field of view. Here we report the retrieval of aerosol properties using the Generalized Retrieval of Aerosols and Surface Properties (GRASP) algorithm applied to AirHARP observations collected during the NASA Aerosol Characterization from Polarimeter and Lidar (ACEPOL) campaign in October–November 2017. The retrieved aerosol properties include spherical fraction (SF), aerosol column concentration in multiple size distribution modes, and, with sufficient aerosol loading, complex aerosol refractive index. From these primary retrievals, we derive aerosol optical depth (AOD), Angstrom exponent (AE), and single scattering albedo (SSA). AODs retrieved from AirHARP measurements are compared with the High Spectral Resolution LiDAR-2 (HSRL2) AOD measurements at 532 nm and validated with measurements from collocated Aerosol Robotic NETwork (AERONET) stations. A good agreement with HSRL2 (ρ=0.940, |BIAS|=0.062, mean absolute error (MAE) = 0.122) and AERONET AOD (0.010≤MAE≤0.015, 0.002≤|BIAS|≤0.009) measurements is observed for the collocated points. There was a mismatch between the HSRL2- and AirHARP-retrieved AOD for the pixels close to the forest fire smoke source and to the edges of the plume due to spatial mismatch in the sampling. This resulted in a higher BIAS and MAE for the HSRL2 AOD comparison. For the case of AERONET AOD comparison, two different approaches are used in the GRASP retrievals, and the simplified aerosol component-based GRASP/Models kernel which retrieves fewer number of aerosol parameter performed well compared to a more generous GRASP/Five mode approach in the low aerosol loading cases. Forest fire smoke intercepted during ACEPOL provided a situation with homogenous plume and sufficient aerosol loading to retrieve the real part of the refractive index (RRI) of 1.55 and the imaginary part of the refractive index (IRI) of 0.024. The derived SSAs for this case are 0.87, 0.86, 0.84, and 0.81 at wavelengths of 440, 550, 670, and 870 nm, respectively. Finer particles with an average AE of 1.53, a volume median radius of 0.157 µm, and a standard deviation (SD) of 0.55 for fine mode is observed for the same smoke plume. These results serve as a proxy for the scale and detail of aerosol retrievals that are anticipated from future space mission data, as HARP CubeSat (mission begins 2020) and HARP2 (aboard the NASA PACE mission with launch in 2023) are near duplicates of AirHARP and are expected to provide the same level of aerosol characterization.

Description: Emissions and long-range transport of mineral dust and combustion-related aerosol from burning fossil fuels and biomass vary from year to year, driven by the evolution of the economy and changes in meteorological conditions and environmental regulations. This study offers both satellite and model perspectives on the interannual variability and possible trends of combustion aerosol and dust in major continental outflow regions over the past 15 years (2003–2017). The decade-long record of aerosol optical depth (AOD, denoted as τ), separately for combustion aerosol (τc) and dust (τd), over global oceans is derived from the Collection 6 aerosol products of the Moderate Resolution Imaging Spectroradiometer (MODIS) onboard both Terra and Aqua. These MODIS Aqua datasets, complemented by aerosol source-tagged simulations using the Community Atmospheric Model version 5 (CAM5), are then analyzed to understand the interannual variability and potential trends of τc and τd in the major continental outflows. Both MODIS and CAM5 consistently yield a similar decreasing trend of −0.017 to −0.020 per decade for τc over the North Atlantic Ocean and the Mediterranean Sea that is attributable to reduced emissions from North America and Europe, respectively. On the contrary, both MODIS and CAM5 display an increasing trend of +0.017 to +0.036 per decade for τc over the tropical Indian Ocean, the Bay of Bengal, and the Arabian Sea, which reflects the influence of increased anthropogenic emissions from South Asia and the Middle East in the last 2 decades. Over the northwestern Pacific Ocean, which is often affected by East Asian emissions of pollution and dust, the MODIS retrievals show a decreasing trend of −0.021 per decade for τc and −0.012 per decade for τd, which is, however, not reproduced by the CAM5 model. In other outflow regions strongly influenced by biomass burning smoke or dust, both MODIS retrievals and CAM5 simulations show no statistically significant trends; the MODIS-observed interannual variability is usually larger than that of the CAM5 simulation.

Description: Proven by multiple theoretical and practical studies, multi-angular spectral polarimetry is ideal for comprehensive retrieval of properties of aerosols. Furthermore, a large number of advanced space polarimeters have been launched recently or planned to be deployed in the coming few years (Dubovik et al., 2019). Nevertheless, at present, practical utilization of aerosol products from polarimetry is rather limited, due to the relatively small number of polarimetric compared to photometric observations, as well as challenges in making full use of the extensive information content available in these complex observations. Indeed, while in recent years several new algorithms have been developed to provide enhanced aerosol retrievals from satellite polarimetry, the practical value of available aerosol products from polarimeters yet remains to be proven. In this regard, this paper presents the analysis of aerosol products obtained by the Generalized Retrieval of Atmosphere and Surface Properties (GRASP) algorithm from POLDER/PARASOL observations. After about a decade of development, GRASP has been adapted for operational processing of polarimetric satellite observations and several aerosol products from POLDER/PARASOL observations have been released. These updated PARASOL/GRASP products are publicly available (e.g., http://www.icare.univ-lille.fr, last access: 16 October 2018, http://www.grasp-open.com/products/, last access: 28 March 2020); the dataset used in the current study is registered under https://doi.org/10.5281/zenodo.3887265 (Chen et al., 2020). The objective of this study is to comprehensively evaluate the GRASP aerosol products obtained from POLDER/PARASOL observations. First, the validation of the entire 2005–2013 archive was conducted by comparing to ground-based Aerosol Robotic Network (AERONET) data. The subjects of the validation are spectral aerosol optical depth (AOD), aerosol absorption optical depth (AAOD) and single-scattering albedo (SSA) at six wavelengths, as well as Ångström exponent (AE), fine-mode AOD (AODF) and coarse-mode AOD (AODC) interpolated to the reference wavelength 550 nm. Second, an inter-comparison of PARASOL/GRASP products with the PARASOL/Operational, MODIS Dark Target (DT), Deep Blue (DB) and Multi-Angle Implementation of Atmospheric Correction (MAIAC) aerosol products for the year 2008 was performed. Over land both satellite data validations and inter-comparisons were conducted separately for different surface types, discriminated by bins of normalized difference vegetation index (NDVI):