Electronic Resource
College Park, Md.
:
American Institute of Physics (AIP)
The Journal of Chemical Physics
105 (1996), S. 1023-1028
ISSN:
1089-7690
Source:
AIP Digital Archive
Topics:
Physics
,
Chemistry and Pharmacology
Notes:
We use a density matrix theory to describe the photoinduced electron transfer dynamics of betaine-30 in solution, including environmental effects which may lead to relaxation and dephasing. We restrict ourselves to only one reaction coordinate. The remaining degrees of freedom of the molecule and the solvent form the environment which is bilinearly coupled to the relevant system. We investigate the S1→S0 reverse electron transfer of betaine-30 in solution, which occurs in the Marcus inverted region. We compare the temperature dependence of our theoretical results with experimental data and other theoretical predictions. © 1996 American Institute of Physics.
Type of Medium:
Electronic Resource
URL:
http://dx.doi.org/10.1063/1.471946
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