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  • 1
    Publication Date: 2017-04-28
    Print ISSN: 0094-8276
    Electronic ISSN: 1944-8007
    Topics: Geosciences , Physics
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  • 2
    Publication Date: 2018-05-02
    Description: A number of climate modeling studies have shown that differences between typical choices for representing ozone can affect climate change projections. Here we investigate potential climate impacts of a specific ozone representation used in simulations of the Hadley Centre Global Environment Model for the Coupled Model Intercomparison Project Phase 5. The method considers ozone changes only in the troposphere and lower stratosphere and prescribes stratospheric ozone elsewhere. For a standard climate sensitivity simulation, we find that this method leads to significantly increased global warming and specific patterns of regional surface warming compared with a fully interactive atmospheric chemistry setup. We explain this mainly by the suppressed part of the stratospheric ozone changes and the associated alteration of the stratospheric water vapor feedback. This combined effect is modulated by simultaneous cirrus cloud changes. We underline the need to understand better how representations of ozone can affect climate modeling results and, in particular, global and regional climate sensitivity estimates. ©2018. American Geophysical Union. All Rights Reserved.
    Print ISSN: 2169-897X
    Electronic ISSN: 2169-8996
    Topics: Geosciences , Physics
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  • 3
    Publication Date: 2017-10-09
    Description: A range of solar radiation management (SRM) techniques has been proposed to counter anthropogenic climate change. Here, we examine the potential effects of stratospheric sulfate aerosols and solar insolation reduction on tropospheric ozone and ozone at Earth's surface. Ozone is a key air pollutant, which can produce respiratory diseases and crop damage. Using a version of the Community Earth System Model from the National Center for Atmospheric Research that includes comprehensive tropospheric and stratospheric chemistry, we model both stratospheric sulfur injection and solar irradiance reduction schemes, with the aim of achieving equal levels of surface cooling relative to the Representative Concentration Pathway 6.0 scenario. This allows us to compare the impacts of sulfate aerosols and solar dimming on atmospheric ozone concentrations. Despite nearly identical global mean surface temperatures for the two SRM approaches, solar insolation reduction increases global average surface ozone concentrations, while sulfate injection decreases it. A fundamental difference between the two geoengineering schemes is the importance of heterogeneous reactions in the photochemical ozone balance with larger stratospheric sulfate abundance, resulting in increased ozone depletion in mid- and high latitudes. This reduces the net transport of stratospheric ozone into the troposphere and thus is a key driver of the overall decrease in surface ozone. At the same time, the change in stratospheric ozone alters the tropospheric photochemical environment due to enhanced ultraviolet radiation. A shared factor among both SRM scenarios is decreased chemical ozone loss due to reduced tropospheric humidity. Under insolation reduction, this is the dominant factor giving rise to the global surface ozone increase. Regionally, both surface ozone increases and decreases are found for both scenarios; that is, SRM would affect regions of the world differently in terms of air pollution. In conclusion, surface ozone and tropospheric chemistry would likely be affected by SRM, but the overall effect is strongly dependent on the SRM scheme. Due to the health and economic impacts of surface ozone, all these impacts should be taken into account in evaluations of possible consequences of SRM.
    Print ISSN: 1680-7316
    Electronic ISSN: 1680-7324
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 4
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  • 6
    Publication Date: 2017-05-19
    Description: A range of solar radiation management (SRM) techniques has been proposed to counter anthropogenic climate change. Here, we examine the potential effects of stratospheric sulfate aerosol and solar insolation reduction on tropospheric ozone and ozone at Earth’s surface. Ozone is a key air pollutant, which can produce respiratory diseases and crop damage. Using a version of the Community Earth System Model from the National Center for Atmospheric Research that includes comprehensive tropospheric and stratospheric chemistry, we model both stratospheric sulfur injection and solar irradiance reduction schemes, with the aim of achieving equal levels of surface cooling relative to the Representative Concentration Pathway 6.0 scenario. This allows us to compare the impacts of sulfate aerosol and solar dimming on atmospheric ozone concentrations. Despite nearly identical global mean surface temperatures for the two SRM approaches, solar insolation reduction increases global average surface ozone concentrations while sulfate injection decreases it. A key difference between the two geoengineering schemes is the importance of heterogeneous reactions in the photochemical ozone balance with larger stratospheric sulfate abundance, resulting in increased ozone depletion in mid- and high latitudes. This reduces the net transport of stratospheric ozone into the troposphere and thus is a key driver of the overall decrease in surface ozone. At the same time, the change in stratospheric ozone alters the tropospheric photochemical environment due to enhanced ultraviolet radiation. A shared factor among both SRM scenarios is decreased chemical ozone loss due to reduced tropospheric humidity. Under insolation reduction, this is the dominant factor giving rise to the global surface ozone increase. Regionally, both surface ozone increases and decreases are found for both scenarios, that is, SRM would affect regions of the world differently in terms of air pollution. In conclusion, surface ozone and tropospheric chemistry would likely be affected by SRM, but the overall effect is strongly dependent on the SRM scheme. Due to the health and economic impacts of surface ozone, all these impacts should be taken into account in evaluations of possible consequences of SRM.
    Electronic ISSN: 1680-7375
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 7
    Publication Date: 2019-01-07
    Description: Many modelling studies suggest that the El Niño Southern Oscillation (ENSO), in interaction with the tropical Pacific background climate, will change under rising atmospheric greenhouse gas concentrations. Solar geoengineering (reducing the solar flux from outer space) has been proposed as a means to counteract anthropogenic greenhouse-induced changes in climate. Effectiveness of solar geoengineering is uncertain. Robust results are particularly difficult to obtain for ENSO because existing geoengineering simulations are too short (typically ~ 50 years) to detect statistically significant changes in the highly variable tropical Pacific background climate. We here present results from a 1000-year sunshade geoengineering simulation, G1, carried out with the coupled atmosphere-ocean general circulation model HadCM3L. In agreement with previous studies, reducing the shortwave solar flux more than compensates the warming in the tropical Pacific that develops in the 4×CO2 scenario: we observe an overcooling of 0.3 °C (5 %) and 0.23-mm day−1 (5 %) reduction in mean rainfall relative to preindustrial conditions in the G1 simulation. This is due to the different latitudinal distributions of the shortwave (solar) and longwave (CO2) forcings.The location of the Intertropical Convergence Zone (ITCZ) located north of equator in the tropical Pacific, which moved 7.5° southwards under 4×CO2, is also restored to its preindustrial location. However, other aspects of the tropical Pacific mean climate are not reset as effectively. Relative to preindustrial conditions, in G1 the zonal wind stress, zonal sea surface temperature (SST) gradient, and meridional SST gradient are reduced by 10 %, 11 %, and 9 %, respectively, and the Pacific Walker Circulation (PWC) is consistently weakened. The overall amplitude of ENSO strengthens by 5–8 %, but there is a 65 % reduction in the asymmetry between cold and warm events: cold events intensify more than warm events. Importantly, the frequency of extreme El Niño and La Niña events increases by 44 % and 32 %, respectively, while the total number of El Niño events increases by 12 %. Paradoxically, while the number of total and extreme events increase, the most extreme El Niño events also become weaker relative to preindustrial state while the La Niña events become stronger. That is, extreme El Niño events in G1 become less extreme than in preindustrial conditions, but extreme El Niño events become more frequent. In contrast, extreme La Niña events become stronger in G1. This is in agreement with the general overcooling of the tropical Pacific in G1 relative to preindustrial conditions, which depict a shift towards generally more La Niña-like conditions.
    Electronic ISSN: 1680-7375
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 8
    Publication Date: 2019-09-11
    Description: There are discrepancies between global climate models regarding the evolution of the tropical tropopause layer (TTL) and also whether changes in ozone impact the surface under climate change. We use a 1D clear-sky radiative–convective equilibrium model to determine how a variety of factors can affect the TTL and how they influence surface climate. We develop a new method of convective adjustment, which relaxes the temperature profile toward the moist adiabat and allows for cooling above the level of neutral buoyancy. The TTL temperatures in our model are sensitive to CO2 concentration, ozone profile, the method of convective adjustment, and the upwelling velocity, which is used to calculate a dynamical cooling rate in the stratosphere. Moreover, the temperature response of the TTL to changes in each of the above factors sometimes depends on the others. The surface temperature response to changes in ozone and upwelling at and above the TTL is also strongly amplified by both stratospheric and tropospheric water vapor changes. With all these influencing factors, it is not surprising that global models disagree with regard to TTL structure and evolution and the influence of ozone changes on surface temperatures. On the other hand, the effect of doubling CO2 on the surface, including just radiative, water vapor, and lapse-rate feedbacks, is relatively robust to changes in convection, upwelling, or the applied ozone profile.
    Print ISSN: 0894-8755
    Electronic ISSN: 1520-0442
    Topics: Geography , Geosciences , Physics
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  • 9
    Publication Date: 2020-12-11
    Description: Many modelling studies suggest that the El Niño–Southern Oscillation (ENSO), in interaction with the tropical Pacific background climate, will change with rising atmospheric greenhouse gas concentrations. Solar geoengineering (reducing the solar flux from outer space) has been proposed as a means to counteract anthropogenic climate change. However, the effectiveness of solar geoengineering concerning a variety of aspects of Earth's climate is uncertain. Robust results are particularly challenging to obtain for ENSO because existing geoengineering simulations are too short (typically ∼ 50 years) to detect statistically significant changes in the highly variable tropical Pacific background climate. We here present results from a 1000-year-long solar-geoengineering simulation, G1, carried out with the coupled atmosphere–ocean general circulation model HadCM3L. In agreement with previous studies, reducing the solar irradiance (4 %) to offset global mean surface warming in the model more than compensates the warming in the tropical Pacific that develops in the 4 × CO2 scenario. We see an overcooling of 0.3 ∘C and a 0.23 mm d−1 (5 %) reduction in mean rainfall over the tropical Pacific relative to preindustrial conditions in the G1 simulation, owing to the different latitudinal distributions of the shortwave (solar) and longwave (CO2) forcings. The location of the Intertropical Convergence Zone (ITCZ) in the tropical Pacific, which moved 7.5∘ southwards under 4 × CO2, is restored to its preindustrial position. However, other aspects of the tropical Pacific mean climate are not reset as effectively. Relative to preindustrial conditions, in G1 the time-averaged zonal wind stress, zonal sea surface temperature (SST) gradient, and meridional SST gradient are each statistically significantly reduced by around 10 %, and the Pacific Walker Circulation (PWC) is consistently weakened, resulting in conditions conducive to increased frequency of El Niño events. The overall amplitude of ENSO strengthens by 9 %–10 % in G1, but there is a 65 % reduction in the asymmetry between cold and warm events: cold events intensify more than warm events. Notably, the frequency of extreme El Niño and La Niña events increases by ca. 60 % and 30 %, respectively, while the total number of El Niño events increases by around 10 %. All of these changes are statistically significant at either 95 or 99 % confidence level. Somewhat paradoxically, while the number of total and extreme events increases, the extreme El Niño events become weaker relative to the preindustrial state, while the extreme La Niña events become even stronger. That is, such extreme El Niño events in G1 become less intense than under preindustrial conditions but also more frequent. In contrast, extreme La Niña events become stronger in G1, which is in agreement with the general overcooling of the tropical Pacific in G1 relative to preindustrial conditions.
    Print ISSN: 1680-7316
    Electronic ISSN: 1680-7324
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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