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  • 1
    ISSN: 1573-0867
    Keywords: methane emission ; rice fields ; temporal scaling ; spatial scaling ; regional estimates ; inverse modeling
    Source: Springer Online Journal Archives 1860-2000
    Topics: Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract The uncertainty in the methane (CH4) source strength of rice fields is among the highest of all sources in the global CH4 budget. Methods to estimate the source strength of rice fields can be divided into two scaling categories: bottom-up (upscaling) and top-down (downscaling). A brief review of upscaling and downscaling methodologies is presented. The combination of upscaling and downscaling methodologies is proposed as a potential method to reduce the uncertainty in the regional CH4 source strength of rice fields. Some preliminary results based on upscaling and downscaling are presented and the limitations of the approaches are discussed. The first case study focuses on upscaling by using a field-scale model in combination with spatial databases to calculate CH4 emissions for the island of Java. The reliability of upscaling results is limited by the uncertainty in model input parameters such as soil properties and organic carbon management. Because controlling variables such as harvested rice area may change on relatively short time scales, a land use change model (CLUE) was used to quantify the potential land use changes on Java in the period 1994–2010. The predicted changes were evaluated using the CH4 emission model. Temporal scaling by coupling land use change models and emission models is necessary to answer policy-related questions on future greenhouse gas emissions. In a downscaling case study, we investigate if inverse modeling can constrain the emissions from rice fields by testing a standard CH4 from rice scenario and a low CH4 from rice scenario (80 and 30 Tg CH4 yr−1, respectively). The results of this study are not yet conclusive; to obtain fine-resolution CH4 emission estimates over the Southeast Asian continent, the monitoring network atmospheric mixturing ratios need to be extended and located closer to the continental sources.
    Type of Medium: Electronic Resource
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  • 2
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  • 4
    Publication Date: 2008-07-15
    Description: Satellite observations of methane (CH4) using the Atmospheric Infrared Sounder (AIRS) on the EOS/Aqua platform from 2003–2007 demonstrate a strong, plume-like enhancement of CH4 in the middle to upper troposphere over the South Asia during July, August and September, and its maximum occurs in early September. Simulations using the global tracer model version 3 (TM3) also show similar seasonal enhancement of CH4 in the same region. The model results also suggest that this enhancement is associated with transport process and local surface emissions, thus the observations to tropospheric CH4during the monsoon season may be used to constrain the models for a better estimation of Asian CH4 sources. Further comparisons between AIRS observations and the model simulations indicate a possible overestimate of CH4 emissions from rice paddies in Southeast Asia. Moreover, the observed tropospheric CH4 enhancement from AIRS provides evidence for the strong transport of atmospheric pollutants from the lower to the upper troposphere in Asia during the monsoon season, and the observed rapid disappearance of local CH4 maximum in September may provide valuable information for studying the dissipation of the Tibetan anticyclone and the withdrawal of monsoon.
    Electronic ISSN: 1680-7375
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 5
    Publication Date: 2009-03-20
    Description: Inverse modeling techniques used to quantify surface carbon fluxes commonly assume that the uncertainty of fossil fuel CO2 (FFCO2) emissions is negligible and that intra-annual variations can be neglected. To investigate these assumptions, we analyzed the differences between four fossil fuel emission maps with spatial and temporal differences over Europe and their impact on the model simulated CO2 concentration. Large temporal flux variations characterize the hourly fields (~40% and ~80% for the seasonal and diurnal cycles, peak-to-peak) and annual country totals differ by 10% on average and up to 40% for some countries (i.e., The Netherlands). These emissions have been prescribed to seven different transport models, resulting in 28 different FFCO2 concentrations fields. The modeled FFCO2 concentration time series at surface sites using time-varying emissions show larger seasonal cycles (+2 ppm at the Hungarian tall tower (HUN)) and smaller diurnal cycles in summer (−1 ppm at HUN) than when using constant emissions. The concentration range spanned by all simulations varies between stations, and is generally larger in winter (up to ~10 ppm peak-to-peak at HUN) than in summer (~5 ppm). The contribution of transport model differences to the simulated concentration std-dev is 2–3 times larger than the contribution of emission differences only, at typical European sites used in global inversions. These contributions to the hourly (monthly) std-dev's amount to ~1.2 (0.8) ppm and ~0.4 (0.3) ppm for transport and emissions, respectively. First comparisons of the modeled concentrations with 14C-based fossil fuel CO2 observations show that the large transport differences still hamper a quantitative evaluation/validation of the emission inventories. Changes in the estimated monthly biosphere flux (Fbio) over Europe, using two inverse modeling approaches, are relatively small (less that 5%) while changes in annual Fbio (up to ~0.15 Gt C/yr) are only slightly smaller than the differences in annual emission totals and around 30% of the mean European ecosystem carbon sink. These results point to an urgent need to improve not only the transport models but also the assumed spatial and temporal distribution of fossil fuel emission maps.
    Electronic ISSN: 1680-7375
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 6
    Publication Date: 2017-10-04
    Description: Understanding changes in the burden and growth rate of atmospheric methane (CH 4 ) has been the focus of several recent studies but still lacks scientific consensus. Here we investigate the role of decreasing anthropogenic carbon monoxide (CO) emissions since 2002 on hydroxyl radical (OH) sinks and tropospheric CH 4 loss. We quantify this impact by contrasting two model simulations for 2002–2013: (1) a Measurement of the Pollution in the Troposphere (MOPITT) CO reanalysis and (2) a Control-Run without CO assimilation. These simulations are performed with the Community Atmosphere Model with Chemistry of the Community Earth System Model fully coupled chemistry climate model with prescribed CH 4 surface concentrations. The assimilation of MOPITT observations constrains the global CO burden, which significantly decreased over this period by ~20%. We find that this decrease results to (a) increase in CO chemical production, (b) higher CH 4 oxidation by OH, and (c) ~8% shorter CH 4 lifetime. We elucidate this coupling by a surrogate mechanism for CO-OH-CH 4 that is quantified from the full chemistry simulations. ©2017. American Geophysical Union. All Rights Reserved.
    Print ISSN: 0094-8276
    Electronic ISSN: 1944-8007
    Topics: Geosciences , Physics
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  • 7
  • 8
    Publication Date: 2004-03-25
    Description: Currently two polar orbiting satellite instruments measure CO2 concentrations in the Earth's atmosphere, while other missions are planned for the coming years. In the future such instruments might become powerful tools for monitoring changes in the atmospheric CO2 abundance and to improve our quantitative understanding of the leading processes controlling this. At the moment, however, we are still in an exploratory phase where first experiences are collected and promising new space-based measurement concepts are investigated. This study assesses the potential of some of these concepts to improve CO2 source and sink estimates obtained from inverse modelling. For this purpose the performance of existing and planned satellite instruments is quantified by synthetic simulations of their ability to reduce the uncertainty of the current source and sink estimates in comparison with the existing ground-based network of sampling sites. Our high resolution inversion of sources and sinks (at 8°x10°) allows us to investigate the variation of instrument performance in space and time and at various temporal and spatial scales. The results of our synthetic tests clearly indicate that the satellite performance increases with increasing sensitivity of the instrument to CO2 near the Earth's surface, favoring the near infra-red technique. Thermal infrared instruments, on the contrary, reach a better global coverage, because the performance in the near infrared is reduced over the oceans owing to a low surface albedo. Near infra-red sounders can compensate for this by measuring in sun-glint, which will allow accurate measurements over the oceans, at the cost, however, of a lower measurement density. Overall, the sun-glint pointing near infrared instrument is the most promising concept of those tested. We show that the ability of satellite instruments to resolve fluxes at smaller temporal and spatial scales is also related to surface sensitivity. All the satellite instruments performed relatively well over the continents resulting mainly from the larger prior flux uncertainties over land than over the oceans. In addition, the surface networks are rather sparse over land increasing the additional benefit of satellite measurements there. Globally, challenging satellite instrument precisions are needed to compete with the current surface network (about 1ppm for weekly and 8°x10° averaged SCIAMACHY columns). Regionally, however, these requirements relax considerably, increasing to 5ppm for SCIAMACHY over tropical continents. This points not only to an interesting research area using SCIAMACHY data, but also to the fact that satellite requirements should not be quantified by only a single number. The applicability of our synthetic results to real satellite instruments is limited by rather crude representations of instrument and data retrieval related uncertainties. This should receive high priority in future work.
    Print ISSN: 1680-7316
    Electronic ISSN: 1680-7324
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 9
    Publication Date: 2003-11-05
    Description: Based on about 20 years of NOAA/CMDL's atmospheric CO2 concentration data and a global atmospheric tracer transport model, we estimate interannual variations and spatial patterns of surface CO2 fluxes in the period 01/1982-12/2000, by using a time-dependent Bayesian inversion technique. To increase the reliability of the estimated temporal features, particular care is exerted towards the selection of data records that are homogeneous in time. Fluxes are estimated on a grid-scale resolution (~8º latitude x 10º longitude), constrained by a-priori spatial correlations, and then integrated over different sets of regions. The transport model is driven by interannually varying re-analyzed meteorological fields. We make consistent use of unsmoothed measurements. In agreement with previous studies, land fluxes are estimated to be the main driver of interannual variations in the global CO2 fluxes, with the pace predominantly being set by the El Niño/La Niña contrast. An exception is a 2-3 year period of increased sink of atmospheric carbon after Mt.  Pinatubo's volcanic eruption in 1991. The largest differences in fluxes between El Niño and La Niña are found in the tropical land regions, the main share being due to the Amazon basin. The flux variations for the Post-Pinatubo period, the 1997/1998 El Niño, and the 1999 La Niña events are exploited to investigate relations between CO2 fluxes and climate forcing. A rough comparison points to anomalies in precipitation as a prominent climate factor for short-term variability of tropical land fluxes, both through their role on NPP and through promoting fire in case of droughts. Some large flux anomalies seem to be directly related to large biomass burning events recorded by satellite observation. Global ocean carbon uptake shows a trend similar to the one expected if ocean uptake scales proportional to the anthropogenic atmospheric CO2 perturbation. In contrast to temporal variations, the longterm spatial flux distribution can be inferred with lesser robustness only. The tentative pattern estimated by the present inversion exhibits a northern hemisphere land sink on the order of 0.4 PgC/yr (for 01/1996-12/1999, non-fossil fuel carbon only) that is mainly confined to North America. Southern hemisphere land regions are carbon neutral, while the tropical land regions are taking up carbon (e.g., at a rate of 0.8 PgC/yr during 01/1996-12/1999). Ocean fluxes show larger uptake in the Northern mid to high latitudes than in the Southern mid latitude regions, in contrast to the estimates by Takahashi et al. (1999) based on in-situ measurements. On a regional basis, results that differ the most from previous estimates are large carbon uptake of 1 to 1.5 PgC/yr by the Southern temperate Pacific ocean region, weak outgassing from the Southern ocean, and a carbon source from eastern Europe.
    Print ISSN: 1680-7316
    Electronic ISSN: 1680-7324
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 10
    Publication Date: 2011-07-12
    Description: Inverse modeling techniques used to quantify surface carbon fluxes commonly assume that the uncertainty of fossil fuel CO2 (FFCO2) emissions is negligible and that intra-annual variations can be neglected. To investigate these assumptions, we analyzed the differences between four fossil fuel emission inventories with spatial and temporal differences over Europe and their impact on the model simulated CO2 concentration. Large temporal flux variations characterize the hourly fields (~40 % and ~80 % for the seasonal and diurnal cycles, peak-to-peak) and annual country totals differ by 10 % on average and up to 40 % for some countries (i.e., the Netherlands). These emissions have been prescribed to seven different transport models, resulting in 28 different FFCO2 concentrations fields. The modeled FFCO2 concentration time series at surface sites using time-varying emissions show larger seasonal cycles (+2 ppm at the Hungarian tall tower (HUN)) and smaller diurnal cycles in summer (−1 ppm at HUN) than when using constant emissions. The concentration range spanned by all simulations varies between stations, and is generally larger in winter (up to ~10 ppm peak-to-peak at HUN) than in summer (~5 ppm). The contribution of transport model differences to the simulated concentration std-dev is 2–3 times larger than the contribution of emission differences only, at typical European sites used in global inversions. These contributions to the hourly (monthly) std-dev's amount to ~1.2 (0.8) ppm and ~0.4 (0.3) ppm for transport and emissions, respectively. First comparisons of the modeled concentrations with 14C-based fossil fuel CO2 observations show that the large transport differences still hamper a quantitative evaluation/validation of the emission inventories. Changes in the estimated monthly biosphere flux (Fbio) over Europe, using two inverse modeling approaches, are relatively small (less that 5 %) while changes in annual Fbio (up to ~0.15 % GtC yr−1) are only slightly smaller than the differences in annual emission totals and around 30 % of the mean European ecosystem carbon sink. These results point to an urgent need to improve not only the transport models but also the assumed spatial and temporal distribution of fossil fuel emission inventories.
    Print ISSN: 1680-7316
    Electronic ISSN: 1680-7324
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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