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  • 1
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    AGU (American Geophysical Union)
    In:  Journal of Geophysical Research: Oceans, 111 . C06024.
    Publication Date: 2018-04-19
    Description: Surface seawater pCO2 and related parameters were measured at high frequency onboard the volunteer observing ship M/V Falstaff in the North Atlantic Ocean between 36° and 52°N. Over 90,000 data points were used to produce monthly CO2 fluxes for 2002/2003. The air-sea CO2 fluxes calculated by two different averaging schemes were compared. The first approach used gas transfer velocity determined from wind speed retrieved at the location of the ship and called colocated winds, while for the second approach a monthly averaged gas transfer velocity was calculated from the wind for each grid pixel including the variability in wind. The colocated wind speeds determined during the time of passage do not capture the monthly wind speed variability of the grid resulting in fluxes that were 47% lower than fluxes using the monthly averaged wind products. The Falstaff CO2 fluxes were in good agreement with a climatology using averaged winds. Over the entire region they differed by 2–5%, depending on the time-dependent correction scheme to account for the atmospheric in increase in pCO2. However, locally the flux differences between the ship measurements and the climatology were greater, especially in regions north of 45°N, like the eastern sector. A comparison of two wind speed products showed that the annual CO2 sink is 4% less when using 6 hourly NCEP/NCAR wind speeds compared to the QuikSCAT wind speed data.
    Type: Article , PeerReviewed
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  • 2
    Publication Date: 2024-02-07
    Description: This contribution to the RECCAP2 (REgional Carbon Cycle Assessment and Processes) assessment analyzes the processes that determine the global ocean carbon sink, and its trends and variability over the period 1985-2018, using a combination of models and observation-based products. The mean sea-air CO2 flux from 1985 to 2018 is -1.6 +/- 0.2 PgC yr(-1) based on an ensemble of reconstructions of the history of sea surface pCO(2) (pCO(2) products). Models indicate that the dominant component of this flux is the net oceanic uptake of anthropogenic CO2, which is estimated at -2.1 +/- 0.3 PgC yr(-1) by an ensemble of ocean biogeochemical models, and -2.4 +/- 0.1 PgC yr(-1) by two ocean circulation inverse models. The ocean also degasses about 0.65 +/- 0.3 PgC yr(-1) of terrestrially derived CO2, but this process is not fully resolved by any of the models used here. From 2001 to 2018, the pCO2 products reconstruct a trend in the ocean carbon sink of -0.61 +/- 0.12 PgC yr(-1) decade(-1), while biogeochemical models and inverse models diagnose an anthropogenic CO2-driven trend of -0.34 +/- 0.06 and -0.41 +/- 0.03 PgC yr(-1) decade(-1), respectively. This implies a climate-forced acceleration of the ocean carbon sink in recent decades, but there are still large uncertainties on the magnitude and cause of this trend. The interannual to decadal variability of the global carbon sink is mainly driven by climate variability, with the climate-driven variability exceeding the CO2-forced variability by 2-3 times. These results suggest that anthropogenic CO2 dominates the ocean CO2 sink, while climate-driven variability is potentially large but highly uncertain and not consistently captured across different methods.
    Type: Article , PeerReviewed
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  • 3
    Publication Date: 2024-02-07
    Description: Accurately predicting future ocean acidification (OA) conditions is crucial for advancing OA research at regional and global scales, and guiding society's mitigation and adaptation efforts. This study presents a new model-data fusion product covering 10 global surface OA indicators based on 14 Earth System Models (ESMs) from the Coupled Model Intercomparison Project Phase 6 (CMIP6), along with three recent observational ocean carbon data products. The indicators include fugacity of carbon dioxide, pH on total scale, total hydrogen ion content, free hydrogen ion content, carbonate ion content, aragonite saturation state, calcite saturation state, Revelle Factor, total dissolved inorganic carbon content, and total alkalinity content. The evolution of these OA indicators is presented on a global surface ocean 1° × 1° grid as decadal averages every 10 years from preindustrial conditions (1750), through historical conditions (1850–2010), and to five future Shared Socioeconomic Pathways (2020–2100): SSP1-1.9, SSP1-2.6, SSP2-4.5, SSP3-7.0, and SSP5-8.5. These OA trajectories represent an improvement over previous OA data products with respect to data quantity, spatial and temporal coverage, diversity of the underlying data and model simulations, and the provided SSPs. The generated data product offers a state-of-the-art research and management tool for the 21st century under the combined stressors of global climate change and ocean acidification. The gridded data product is available in NetCDF at the National Oceanic and Atmospheric Administration (NOAA) National Centers for Environmental Information: https://www.ncei.noaa.gov/data/oceans/ncei/ocads/metadata/0259391.html, and global maps of these indicators are available in jpeg at: https://www.ncei.noaa.gov/access/ocean-carbon-acidification-data-system/synthesis/surface-oa-indicators.html. Key Points: - This study presents the evolution of 10 ocean acidification (OA) indicators in the global surface ocean from 1750 to 2100 - By leveraging 14 Earth System Models (ESMs) and the latest observational data, it represents a significant advancement in OA projections - This inter-model comparison effort showcases the overall agreements among different ESMs in projecting surface ocean carbon variables
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  • 4
    Publication Date: 2016-09-19
    Repository Name: EPIC Alfred Wegener Institut
    Type: Article , isiRev
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  • 5
    Publication Date: 2021-01-26
    Repository Name: EPIC Alfred Wegener Institut
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  • 6
    Publication Date: 2023-12-19
    Description: 〈jats:p〉Abstract. Accurate assessment of anthropogenic carbon dioxide (CO2) emissions and their redistribution among the atmosphere, ocean, and terrestrial biosphere in a changing climate is critical to better understand the global carbon cycle, support the development of climate policies, and project future climate change. Here we describe and synthesize data sets and methodology to quantify the five major components of the global carbon budget and their uncertainties. Fossil CO2 emissions (EFOS) are based on energy statistics and cement production data, while emissions from land-use change (ELUC), mainly deforestation, are based on land-use and land-use change data and bookkeeping models. Atmospheric CO2 concentration is measured directly, and its growth rate (GATM) is computed from the annual changes in concentration. The ocean CO2 sink (SOCEAN) is estimated with global ocean biogeochemistry models and observation-based fCO2 products. The terrestrial CO2 sink (SLAND) is estimated with dynamic global vegetation models. Additional lines of evidence on land and ocean sinks are provided by atmospheric inversions, atmospheric oxygen measurements, and Earth system models. The resulting carbon budget imbalance (BIM), the difference between the estimated total emissions and the estimated changes in the atmosphere, ocean, and terrestrial biosphere, is a measure of imperfect data and incomplete understanding of the contemporary carbon cycle. All uncertainties are reported as ±1σ. For the year 2022, EFOS increased by 0.9 % relative to 2021, with fossil emissions at 9.9±0.5 Gt C yr−1 (10.2±0.5 Gt C yr−1 when the cement carbonation sink is not included), and ELUC was 1.2±0.7 Gt C yr−1, for a total anthropogenic CO2 emission (including the cement carbonation sink) of 11.1±0.8 Gt C yr−1 (40.7±3.2 Gt CO2 yr−1). Also, for 2022, GATM was 4.6±0.2 Gt C yr−1 (2.18±0.1 ppm yr−1; ppm denotes parts per million), SOCEAN was 2.8±0.4 Gt C yr−1, and SLAND was 3.8±0.8 Gt C yr−1, with a BIM of −0.1 Gt C yr−1 (i.e. total estimated sources marginally too low or sinks marginally too high). The global atmospheric CO2 concentration averaged over 2022 reached 417.1±0.1 ppm. Preliminary data for 2023 suggest an increase in EFOS relative to 2022 of +1.1 % (0.0 % to 2.1 %) globally and atmospheric CO2 concentration reaching 419.3 ppm, 51 % above the pre-industrial level (around 278 ppm in 1750). Overall, the mean of and trend in the components of the global carbon budget are consistently estimated over the period 1959–2022, with a near-zero overall budget imbalance, although discrepancies of up to around 1 Gt C yr−1 persist for the representation of annual to semi-decadal variability in CO2 fluxes. Comparison of estimates from multiple approaches and observations shows the following: (1) a persistent large uncertainty in the estimate of land-use changes emissions, (2) a low agreement between the different methods on the magnitude of the land CO2 flux in the northern extra-tropics, and (3) a discrepancy between the different methods on the strength of the ocean sink over the last decade. This living-data update documents changes in methods and data sets applied to this most recent global carbon budget as well as evolving community understanding of the global carbon cycle. The data presented in this work are available at https://doi.org/10.18160/GCP-2023 (Friedlingstein et al., 2023). 〈/jats:p〉
    Repository Name: EPIC Alfred Wegener Institut
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  • 7
    Publication Date: 2022-05-26
    Description: © The Author(s), 2015. This article is distributed under the terms of the Creative Commons Attribution License. The definitive version was published in Earth System Science Data 7 (2015): 47-85, doi:10.5194/essd-7-47-2015.
    Description: Accurate assessment of anthropogenic carbon dioxide (CO2) emissions and their redistribution among the atmosphere, ocean, and terrestrial biosphere is important to better understand the global carbon cycle, support the development of climate policies, and project future climate change. Here we describe data sets and a methodology to quantify all major components of the global carbon budget, including their uncertainties, based on the combination of a range of data, algorithms, statistics, and model estimates and their interpretation by a broad scientific community. We discuss changes compared to previous estimates, consistency within and among components, alongside methodology and data limitations. CO2 emissions from fossil fuel combustion and cement production (EFF) are based on energy statistics and cement production data, respectively, while emissions from land-use change (ELUC), mainly deforestation, are based on combined evidence from land-cover-change data, fire activity associated with deforestation, and models. The global atmospheric CO2 concentration is measured directly and its rate of growth (GATM) is computed from the annual changes in concentration. The mean ocean CO2 sink (SOCEAN) is based on observations from the 1990s, while the annual anomalies and trends are estimated with ocean models. The variability in SOCEAN is evaluated with data products based on surveys of ocean CO2 measurements. The global residual terrestrial CO2 sink (SLAND) is estimated by the difference of the other terms of the global carbon budget and compared to results of independent dynamic global vegetation models forced by observed climate, CO2, and land-cover-change (some including nitrogen–carbon interactions). We compare the mean land and ocean fluxes and their variability to estimates from three atmospheric inverse methods for three broad latitude bands. All uncertainties are reported as ±1σ, reflecting the current capacity to characterise the annual estimates of each component of the global carbon budget. For the last decade available (2004–2013), EFF was 8.9 ± 0.4 GtC yr−1, ELUC 0.9 ± 0.5 GtC yr−1, GATM 4.3 ± 0.1 GtC yr−1, SOCEAN 2.6 ± 0.5 GtC yr−1, and SLAND 2.9 ± 0.8 GtC yr−1. For year 2013 alone, EFF grew to 9.9 ± 0.5 GtC yr−1, 2.3% above 2012, continuing the growth trend in these emissions, ELUC was 0.9 ± 0.5 GtC yr−1, GATM was 5.4 ± 0.2 GtC yr−1, SOCEAN was 2.9 ± 0.5 GtC yr−1, and SLAND was 2.5 ± 0.9 GtC yr−1. GATM was high in 2013, reflecting a steady increase in EFF and smaller and opposite changes between SOCEAN and SLAND compared to the past decade (2004–2013). The global atmospheric CO2 concentration reached 395.31 ± 0.10 ppm averaged over 2013. We estimate that EFF will increase by 2.5% (1.3–3.5%) to 10.1 ± 0.6 GtC in 2014 (37.0 ± 2.2 GtCO2 yr−1), 65% above emissions in 1990, based on projections of world gross domestic product and recent changes in the carbon intensity of the global economy. From this projection of EFF and assumed constant ELUC for 2014, cumulative emissions of CO2 will reach about 545 ± 55 GtC (2000 ± 200 GtCO2) for 1870–2014, about 75% from EFF and 25% from ELUC. This paper documents changes in the methods and data sets used in this new carbon budget compared with previous publications of this living data set (Le Quéré et al., 2013, 2014). All observations presented here can be downloaded from the Carbon Dioxide Information Analysis Center (doi:10.3334/CDIAC/GCP_2014).
    Description: NERC provided funding to C. Le Quéré, R. Moriarty, and the GCP though their International Opportunities Fund specifically to support this publication (NE/103002X/1), and to U. Schuster through UKOARP (NE/H017046/1). G. P. Peters and R. M. Andrews were supported by the Norwegian Research Council (236296). T. A. Boden was supported by US Department of Energy, Office of Science, Biological and Environmental Research (BER) programmes under US Department of Energy contract DEAC05- 00OR22725. Y. Bozec was supported by Region Bretagne, CG29, and INSU (LEFE/MERMEX) for CARBORHONE cruises. J. G. Canadell and M. R. Raupach were supported by the Australian Climate Change Science Programme. M. Hoppema received ICOSD funding through the German Federal Ministry of Education and Research (BMBF) to the AWI (01 LK 1224I). J. I. House was supported by a Leverhulme Early Career Fellowship. A. K. Jain was supported by the US National Science Foundation (NSF AGS 12-43071) the US Department of Energy, Office of Science, and BER programmes (DOE DE-SC0006706) and the NASA LCLUC programme (NASA NNX14AD94G). E. Kato was supported by the Environment Research and Technology Development Fund (S-10) of the Ministry of Environment of Japan. C. Koven was supported by the Director, Office of Science, Office of Biological and Environmental Research, of the US Department of Energy under contract no. DE-AC02-05CH11231 as part of their Regional and Global Climate Modeling Program. I. D. Lima was supported by the U.S. National Science Foundation (NSF AGS-1048827). N. Metzl was supported by Institut National des Sciences de l’Univers (INSU) and Institut Paul Emile Victor (IPEV) for OISO cruises. A. Olsen was supported by the Centre for Climate Dynamics at the Bjerknes Centre for Climate Research. J. E. Salisbury was supported by grants from NOAA/NASA. T. Steinhoff was supported by ICOS-D (BMBF FK 01LK1101C). B. D. Stocker was supported by the Swiss National Science Foundation and FP7 funding through project EMBRACE (282672). A. J. Sutton was supported by NOAA. T. Takahashi was supported by grants from NOAA and the Comer Education and Science Foundation. B. Tilbrook was supported by the Australian Department of the Environment and the Integrated Marine Observing System. A.Wiltshire was supported by the Joint UK DECC/Defra Met Office Hadley Centre Climate Programme (GA01101). P. Ciais,W. Peters, C. Le Quére, P. Regnier, and U. Schuster were supported by the EU FP7 through project GEOCarbon (283080). A. Arneth, P. Ciais, S. Sitch, and A. Wiltshire were supported by COMBINE (226520). V. Kitidis, M. Hoppema, N. Metzl, C. Le Quéré, U. Schuster, J. Schwiger, J. Segschneider, and T. Steinhoff were supported by the EU FP7 through project CARBOCHANGE (264879). A. Arnet, P. Friedlingstein, B. Poulter, and S. Sitch were supported by the EU FP7 through projects LUC4C (GA603542). P. Friedlingstein was also supported by EMBRACE (GA282672). F. Chevallier and G. R. van der Werf were supported by the EU FP7 through project MACC-II (283576).
    Repository Name: Woods Hole Open Access Server
    Type: Article
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