ALBERT

Description: Desert dust and marine aerosols are receiving increased scientific attention because of their prevalence on intercontinental scales and their potentially large effects on Earth radiation and climate, as well as on other aerosols, clouds, and precipitation. The relatively large size of desert dust and marine aerosols produces scattering phase functions that are strongly forward- peaked. Hence, Sun photometry and pyrheliometry of these aerosols are more subject to diffuse-light errors than is the case for smaller aerosols. Here we quantify these diffuse-light effects for common Sun photometer and pyrheliometer fields of view (FOV), using a data base on dust and marine aerosols derived from (1) AERONET measurements of sky radiance and solar beam transmission and (2) in situ measurements of aerosol layer size distribution and chemical composition. Accounting for particle non-sphericity is important when deriving dust size distribution from both AERONET and in situ aerodynamic measurements. We express our results in terms of correction factors that can be applied to Sun photometer and pyrheliometer measurements of aerosol optical depth (AOD). We find that the corrections are negligible (less than approximately 1% of AOD) for Sun photometers with narrow FOV (half-angle eta less than degree), but that they can be as large as 10% of AOD at 354 nm wavelength for Sun photometers with eta = 1.85 degrees. For pyrheliometers (which can have eta up to approximately 2.8 degrees), corrections can be as large as 16% at 354 nm. We find that AOD correction factors are well correlated with AOD wavelength dependence (hence Angstrom exponent). We provide best-fit equations for determining correction factors from Angstrom exponents of uncorrected AOD spectra, and we demonstrate their application to vertical profiles of multiwavelength AOD.

Description: Global ozone trends derived from the Stratospheric Aerosol and Gas Experiment I and II (SAGE I/II) combined with the more recent Halogen Occultation Experiment (HALOE) observations provide evidence of a slowdown in stratospheric ozone losses since 1997. This evidence is quantified by the cumulative sum of residual differences from the predicted linear trend. The cumulative residuals indicate that the rate of ozone loss at 35- 45 km altitudes globally has diminished. These changes in loss rates are consistent with the slowdown of total stratospheric chlorine increases characterized by HALOE HCI measurements. These changes in the ozone loss rates in the upper stratosphere are significant and constitute the first stage of a recovery of the ozone layer.

Description: Using measurements of the spectral solar radiative flux and optical depth for 2 days (24 August and 6 September 2000) during the SAFARI 2000 intensive field experiment and a detailed radiative transfer model, we estimate the spectral single scattering albedo of the aerosol layer. The single scattering albedo is similar on the 2 days even though the optical depth for the aerosol layer was quite different. The aerosol single scattering albedo was between 0.85 and 0.90 at 350 nm, decreasing to 0.6 in the near infrared. The magnitude and decrease with wavelength of the single scattering albedo are consistent with the absorption properties of small black carbon particles. We estimate the uncertainty in the single scattering albedo due to the uncertainty in the measured fractional absorption and optical depths. The uncertainty in the single scattering albedo is significantly less on the high-optical-depth day (6 September) than on the low-optical-depth day (24 August). On the high-optical-depth day, the uncertainty in the single scattering albedo is 0.02 in the midvisible whereas on the low-optical-depth day the uncertainty is 0.08 in the midvisible. On both days, the uncertainty becomes larger in the near infrared. We compute the radiative effect of the aerosol by comparing calculations with and without the aerosol. The effect at the top of the atmosphere (TOA) is to cool the atmosphere by 13 W/sq m on 24 August and 17 W/sq m on 6 September. The effect on the downward flux at the surface is a reduction of 57 W/sq m on 24 August and 200 W/sq m on 6 September. The aerosol effect on the downward flux at the surface is in good agreement with the results reported from the Indian Ocean Experiment (INDOEX).

Description: This investigation has had four main thrusts: 1) The analysis of seasonal variations of the Earth's gravitational field using Lageos 1 and 2 SLR data and comparisons to geophysical models. We have estimated the annual variation of the gravity field via a spherical harmonic expansion complete to degree and order 4. We have also constructed a similar model using models of the annual variation in the gravity field due to atmospheric, hydrologic, and ocean mass redistribution. These three models, when combined together, are in excellent agreement with the variations observed by satellite laser ranging. An article on these results was published in the journal Geophysical Research Letters. 2) The second thrust of our investigation has been to analyze the output of a Global Climate Model (GCM) to determine if the GRACE gravity mission can be expected to detect climate change signals. Working with Gary Russell at the Goddard Institute for Space Studies (GISS), we have determined that there are several large secular signals that GRACE might be able to detect, including secular changes in snow cover, sea ice, polar ice, ocean mass, and other variables. It is possible that some of these signals could be detected with 5 years of GRACE measurements - its hard to judge this because the interannual variability in the GCM, which could mask the climate signals, is unreliable. Certainly a follow-on GRACE mission could detect these signals when compared to the data from the initial GRACE mission.). An article on these results will be published in the journal Journal of Geophysical Research. 3) In the last year of the investigation, we developed a new technique for analyzing temporal gravity variations using "geophysical fingerprints", which was successfully demonstrated on 20 years of satellite laser ranging data [Nerem et al., 20031. 4]. We also participated in a workshop on future satellite gravity measurements, which resulted in paper on measuring ocean mass variations using GRACE [Nerem et al., 20031 and on using laser interferometry for future gravity missions [Bender et al., 20031].