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  • Engineering  (96)
  • Physical Chemistry  (31)
  • Wiley-Blackwell  (127)
  • American Meteorological Society (AMS)
  • PANGAEA
  • 1990-1994  (73)
  • 1980-1984  (54)
  • 1993  (73)
  • 1984  (54)
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  • 1990-1994  (73)
  • 1980-1984  (54)
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  • 1
    Electronic Resource
    Electronic Resource
    A posteriori pointwise upper bound error estimates in the finite element method (1993)
    Chichester [u.a.] : Wiley-Blackwell
    International Journal for Numerical Methods in Engineering 36 (1993), S. 1279-1298 
    Details
    ISSN: 0029-5981
    Keywords: Engineering ; Engineering General
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Mathematics , Technology
    Notes: An error estimate for the finite element method is presented in this paper. The error is identified as the response to a set of residual forces, and a complementary analysis provides an upper bound estimate of the global energy of the error. The inequality proposed by Babuška and Miller1 is then employed to bound the error in stress and displacement at a point. The formula is derived for two-dimensional elasticity, but the procedure is general; and can be applied to three-dimensional and other problems. Numerical experiments using the procedure are carried out and the results are given for the four-node bilinear compatible element and plane stress.
    Additional Material: 19 Ill.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/nme.1620360803
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  • 2
    Electronic Resource
    Electronic Resource
    A model of binary alloy solidification (1984)
    Chichester [u.a.] : Wiley-Blackwell
    International Journal for Numerical Methods in Engineering 20 (1984), S. 1067-1084 
    Details
    ISSN: 0029-5981
    Keywords: Engineering ; Engineering General
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Mathematics , Technology
    Notes: A linear model for the solidification of a dilute binary alloy is presented. In this model the solidus and liquidus curves are linear. As a consequence internal energy depends linearly upon temperature and concentration. The formulation is a generalization of the well-known enthalpy method to treat a phase change problem involving coupled heat and mass transfer. Both analytic and numerical formulations are given. Results from the latter are presented and compared with an explicit solution of Rubinstein for a Stefan-like problem posed in a semi-infinite slab. Some remarks on the behaviour of the explicit solution are given.
    Additional Material: 5 Ill.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/nme.1620200609
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  • 3
    Electronic Resource
    Electronic Resource
    Letters to the editor (1984)
    Chichester [u.a.] : Wiley-Blackwell
    International Journal for Numerical Methods in Engineering 20 (1984), S. 1169-1174 
    Details
    ISSN: 0029-5981
    Keywords: Engineering ; Engineering General
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Mathematics , Technology
    Additional Material: 2 Tab.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/nme.1620200616
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  • 4
    Electronic Resource
    Electronic Resource
    Stereochemistry of aminolysis of N-pentafluorophenylcarbonimidoyl dichloride. Crystal and molecular structures of N2-pentafluorophenyl-N1,N1-dibenzylchloroformamidine (1993)
    Chichester : Wiley-Blackwell
    Journal of Physical Organic Chemistry 6 (1993), S. 319-325 
    Details
    ISSN: 0894-3230
    Keywords: Organic Chemistry ; Physical Chemistry
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology , Physics
    Notes: It has been established that the product of the reaction of N-pentafluorophenylcarbonimidoyl dichloride (1) with dibenzylamine, viz. N2-pentafluorophenyl-N1,N1-dibenzylchloroformamidine (4a) is a Z-isomer, whereas according to the concept of stereoelectronic control one might have expected a product with E-configuration. The heat of formation and the geometry of Z- and E isomer of N2-pentafluorophenyl-N1,N1-diethylchloroformamidine (4b) (the latter is a product of the reaction of 1 with diethylamine) were calculated with the semi-empirical MNDO method. The calculated geometry of (Z)-4b was found to be in a good agreement with the experimentally determined structure of 4a. The formation of (Z)-4b is more preferable energetically than that of (E)-4b; the calculated difference in the heats of formation is 2·8 kcal mol-1. Thermodynamic control of the reaction stereochemistry is proposed.
    Additional Material: 1 Ill.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/poc.610060602
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  • 5
    Electronic Resource
    Electronic Resource
    BEM analysis of reduced dynamic stress concentration by multiple holes (1993)
    Chichester : Wiley-Blackwell
    Communications in Numerical Methods in Engineering 9 (1993), S. 917-924 
    Details
    ISSN: 1069-8299
    Keywords: Engineering ; Engineering General
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Mathematics , Technology
    Notes: The reduction of stress concentration around a circular hole in a dynamically loaded plate by introducing auxiliary holes around the original hole is studied numerically. The solution of this plane stress problem is carried out in the Laplace transformed domain with the aid of the boundary-element method, and subsequently the time domain response is obtained by numerically inverting the transformed solution. Numerical examples are presented which demonstrate a stress reduction as high as 18 per pent by the introduction of two auxiliary holes in the loading direction for the uniaxial case.
    Additional Material: 4 Ill.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/cnm.1640091108
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  • 6
    Electronic Resource
    Electronic Resource
    Stratified flow under an ice keel - a numerical approach (1993)
    Chichester : Wiley-Blackwell
    International Journal for Numerical Methods in Fluids 16 (1993), S. 353-364 
    Details
    ISSN: 0271-2091
    Keywords: Ice keels ; Drag ; Stratified flow ; Marker and cell ; SOLA-VOF ; Engineering ; Engineering General
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Mechanical Engineering, Materials Science, Production Engineering, Mining and Metallurgy, Traffic Engineering, Precision Mechanics
    Notes: A numerical investigation of the flow of two immiscible stratified fluids under an isolated keel has been undertaken. The investigation utilized the two-dimensional Euler equations for incompressible flow, and the solution of these equations has been obtained by using the well-known finite volume marker and cell approach. Experimental drag-force measurements are also presented for a family of two-dimensional topographic models of fixed height with increasing surface slopes in a two-layer density system. The range of flow speeds explored covers the Froude number range from subcritical to fully supercritical. The drag force measurements are augmented by detailed observations of the interface distortion. The results clearly show large drag increases arising from the internal wave systems generated in the stratified flow. Very good agreement has been found between the experimental and numerical results for both the interface shape between the two fluids and the drag force on a variety of keels.
    Additional Material: 8 Ill.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/fld.1650160502
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  • 7
    Electronic Resource
    Electronic Resource
    Modelling large-bubble formation at submerged orifices (1993)
    Chichester : Wiley-Blackwell
    International Journal for Numerical Methods in Fluids 16 (1993), S. 813-825 
    Details
    ISSN: 0271-2091
    Keywords: Bubble formation ; Bubble growth ; Bubbling regimes ; Free boundaries ; Interface advection ; Engineering ; Engineering General
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Mechanical Engineering, Materials Science, Production Engineering, Mining and Metallurgy, Traffic Engineering, Precision Mechanics
    Notes: The formation of large gas bubbles at submerged orifices is investigated numerically with a two-dimensional, transient, finite difference model using a volume fraction specification to track the movement of the gas-liquid interface. Experimentally observed features of large-bubble formation such as the initial toroidal shape of the bubbles and the penetration of liquid down the pipe centreline are well predicted by the model. The expected oscillatory nature of growth is also observed. The bubble departure volume corresponds to experiments and to the model of Davidson and Schuler. At present the simulations do not extend far enough to investigate multiple-bubble ejection and important bubble-to-bubble interactions during growth and after departure.
    Additional Material: 9 Ill.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/fld.1650160905
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  • 8
    Electronic Resource
    Electronic Resource
    Basic hydrolysis of glyceryl nitrate esters. III. Trinitroglycerin (1984)
    New York, NY : Wiley-Blackwell
    International Journal of Chemical Kinetics 16 (1984), S. 1027-1051 
    Details
    ISSN: 0538-8066
    Keywords: Chemistry ; Physical Chemistry
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology
    Notes: Kinetics of the basic hydrolysis of glyceryl trinitrate (TNG) were investigated in CO2-free aqueous calcium hydroxide solutions. The hydrolysis reactions were carried out in a temperature controlled reactor vessel with provision for continuous N2 sparging of the reaction mixture. TNG hydrolyzed via second-order reaction at 25°C, 18°C, and 10°C. The activation energy of the hydrolysis reaction of TNG was calculated from the kinetic data and found to be equal to 27.53 kcal/mol. The major products of the hydrolysis of TNG in solution of calcium hydroxide were calcium nitrate and calcium nitrite, accounting for approximately 50% of the degradation products. The minor identified products such as calcium oxalate and nitrate esters amounted to approximatey 6% of the products. The remaining 30% of the isolated products was a mixture of calcium formate, a nitrate ester, and unidentified volatiles, polymerlike substances, and other organic residue.
    Additional Material: 11 Ill.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/kin.550160808
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  • 9
    Electronic Resource
    Electronic Resource
    Thermal decomposition of methyl nitrite in shock waves studied by laser probing (1984)
    New York, NY : Wiley-Blackwell
    International Journal of Chemical Kinetics 16 (1984), S. 1139-1150 
    Details
    ISSN: 0538-8066
    Keywords: Chemistry ; Physical Chemistry
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology
    Notes: The unimolecular decomposition of methyl nitrite in the temperature range 680-955 K and pressure range 0.64 to 2.0 atm has been studied in shock-tube experiments employing real-time absorption of CW CO laser radiation by the NO product. Computer kinetic modeling using a set of 23 reactions shows that NO product is relatively unreactive. Its initial rate of production can be used to yield directly the unimolecular rate constant, which in the fall-off region, can be represented by the second-order rate coefficient in the Arrhenius form: \documentclass{article}\pagestyle{empty}\begin{document}$$k_1 = 10^{17.90 \pm 0.21} \exp (- 17200 \pm 400/T){\rm cm}^{\rm 3} {\rm mol}^{ - 1} {\rm s}^{ - 1}$$\end{document} A RRKM model calculation, assuming a loose CH3ONO≠ complex with two degrees of free internal rotation, gives good agreement with the experimental rate constants.
    Additional Material: 5 Ill.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/kin.550160909
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  • 10
    Electronic Resource
    Electronic Resource
    Basic hydrolysis of glyceryl nitrate esters. II. 1,2-glyceryl and 1, 3-glyceryl dinitrate esters (1984)
    New York, NY : Wiley-Blackwell
    International Journal of Chemical Kinetics 16 (1984), S. 1009-1026 
    Details
    ISSN: 0538-8066
    Keywords: Chemistry ; Physical Chemistry
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology
    Notes: Kinetics of the basic hydrolysis of 1,2-glyceryl dinitrate (1,2-DNG) and 1,3-glyceryl dinitrate (1,3-DNG) esters were investigated in CO2-free aqueous calcium hydroxide solutions. The hydrolysis reactions were carried out in a temperature controlled reactor vessel with provision for continuous N2 sparging of the reaction mixture. Both glyceryl dinitrate esters hydrolyzed via second-order reaction at 25°C. 1,2-DNG in basic solutions isomerized to 1,3-DNG which subsequently hydrolyzed to yield products. The main hydrolysis product of 1,3-DNG was identified as glycidyl nitrate. Other products formed during the basic hydrolysis of DNGs were nitrites and nitrates.
    Additional Material: 11 Ill.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/kin.550160807
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