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  • 1
    Publication Date: 2023-06-08
    Description: Previous paleolimnological studies demonstrated that the sediments of Garba Guracha, situated at 3950 m asl in the afro-alpine zone of the Bale Mountains of Ethiopia, provide a complete Late Glacial and Holocene paleoclimate and environmental archive. We revisited Garba Guracha in order to retrieve new sediment cores and to apply new environmental proxies, e.g. charcoal, diatoms, biomarkers, and stable isotopes. Our chronology is established using 210Pb dating and radiocarbon dating of bulk sedimentary organic matter, bulk n-alkanes, and charcoal. Although bedrock was not reached during coring, basal ages confirm that sedimentation started at the earliest ~ 16 cal kyr BP. The absence of a systematic age offset for the n-alkanes suggests that “pre-aging” is not a prominent issue in this lake, which is characterised by a very small afro-alpine catchment. X-ray fluorescence scans and total organic carbon contents show a prominent transition from minerogenic to organic-rich sediments around 11 cal kyr BP coinciding with the Holocene onset. While an unambiguous terrestrial versus aquatic source identification seems challenging, the n-alkane-based Paq proxy, TOC/N ratios, δ13C values, and the sugar biomarker patterns suggest a predominantly autochthonous organic matter source. Supraregional climate events, such as the African Humid Period, the Younger Dryas (YD), a 6.5 cal kyr BP short drying event, and the 4.2 cal kyr BP transition to overall drier climate are recorded in our archive. The Garba Guracha record suggests that northern hemisphere forcings played a role in the Eastern African highland paleoclimate.
    Description: Deutsche Forschungsgemeinschaft http://dx.doi.org/10.13039/501100001659
    Keywords: ddc:551 ; Paleolimnology ; Afro-alpine ; Radiocarbon dating ; XRF scanning ; Sedimentation rate ; Biomarkers
    Language: English
    Type: doc-type:article
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  • 2
    Publication Date: 2024-02-22
    Description: Formalised knowledge systems, including universities and research institutes, are important for contemporary societies. They are, however, also arguably failing humanity when their impact is measured against the level of progress being made in stimulating the societal changes needed to address challenges like climate change. In this research we used a novel futures-oriented and participatory approach that asked what future envisioned knowledge systems might need to look like and how we might get there. Findings suggest that envisioned future systems will need to be much more collaborative, open, diverse, egalitarian, and able to work with values and systemic issues. They will also need to go beyond producing knowledge about our world to generating wisdom about how to act within it. To get to envisioned systems we will need to rapidly scale methodological innovations, connect innovators, and creatively accelerate learning about working with intractable challenges. We will also need to create new funding schemes, a global knowledge commons, and challenge deeply held assumptions. To genuinely be a creative force in supporting longevity of human and non-human life on our planet, the shift in knowledge systems will probably need to be at the scale of the enlightenment and speed of the scientific and technological revolution accompanying the second World War. This will require bold and strategic action from governments, scientists, civic society and sustained transformational intent.
    Language: English
    Type: info:eu-repo/semantics/article
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  • 3
    Publication Date: 2023-12-16
    Description: 〈title xmlns:mml="http://www.w3.org/1998/Math/MathML"〉Abstract〈/title〉〈p xmlns:mml="http://www.w3.org/1998/Math/MathML" xml:lang="en"〉Three volcanic arcs have been the source of New Zealand's volcanic activity since the Neogene: Northland arc, Coromandel Volcanic Zone (CVZ) and Taupō Volcanic Zone (TVZ). The eruption chronology for the Quaternary, sourced by the TVZ, is well studied and established, whereas the volcanic evolution of the precursor arc systems, like the CVZ (central activity c. 18 to 2 Ma), is poorly known due to limited accessibility to, or identification of, onshore volcanic deposits and their sources. Here, we investigate the marine tephra record of the Neogene, mostly sourced by the CVZ, of cores from IODP Exp. 375 (Sites U1520 and U1526), ODP Leg 181 (Sites 1123, 1124 and 1125), IODP Leg 329 (Site U1371) and DSDP Leg 90 (Site 594) offshore of New Zealand. In total, we identify 306 primary tephra layers in the marine sediments. Multi‐approach age models (e.g. biostratigraphy, zircon ages) are used in combination with geochemical fingerprinting (major and trace element compositions) and the stratigraphic context of each marine tephra layer to establish 168 tie‐lines between marine tephra layers from different holes and sites. Following this approach, we identify 208 explosive volcanic events in the Neogene between c. 17.5 and 2.6 Ma. This is the first comprehensive study of New Zealand's Neogene explosive volcanism established from tephrochronostratigraphic studies, which reveals continuous volcanic activity between c. 12 and 2.6 Ma with an abrupt compositional change at c. 4.5 Ma, potentially associated with the transition from CVZ to TVZ.〈/p〉
    Description: Plain Language Summary: Since 18 Ma, volcanic activity in New Zealand is dominantly sourced by the Coromandel Volcanic Zone (CVZ). Most caldera systems of the CVZ identified so far are located on Coromandel Peninsula in the NW of North Island, New Zealand, but studies of the CVZ are rare mainly due to the limited accessibility of its volcanic deposits, as well as missing stratigraphic continuity between different outcrops and the volcanic source. Here, our ocean drilling tephra record—mainly volcanic ash from explosive eruptions, distributed and falling out over the ocean—has a great potential to reveal the eruption history of the CVZ because it is preserved in marine sediments in a nearly undisturbed stratigraphic context. We analyzed ∼400 marine tephra layers from multiple ocean sediment cores off the coast of New Zealand for their geochemical glass compositions and identified 306 as largely undisturbed ash deposits. These primary ash deposits correspond to a total number of 208 Neogene volcanic events. Different dating methods result in a continuous marine tephra record for the last 12 Ma, equivalent to a unique and most complete eruptive history for the CVZ. This enables us to further unravel changes in the composition of the associated magmas with time.〈/p〉
    Description: Key Points: 〈list list-type="bullet"〉 〈list-item〉 〈p xml:lang="en"〉New Zealand's Neogene explosive volcanism based on the marine tephra record〈/p〉〈/list-item〉 〈list-item〉 〈p xml:lang="en"〉Geochemical fingerprinting of marine tephra layers across the study area to establish volcanic events〈/p〉〈/list-item〉 〈list-item〉 〈p xml:lang="en"〉Insights into geochemical variations with time, repose times and spatiotemporal distribution〈/p〉〈/list-item〉 〈/list〉 〈/p〉
    Description: DFG
    Description: Marsden project
    Description: https://doi.org/10.14379/iodp.proc.372B375.210.2023
    Keywords: ddc:551 ; marine tephrochronostratigraphy ; geochemical fingerprinting ; correlations of marine tephras between individual drill sites ; IODP ; ODP and DSDP drill sites ; neogene eruption record of New Zealand
    Language: English
    Type: doc-type:article
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  • 4
    Publication Date: 2023-06-16
    Description: Secondary organic aerosol (SOA) forms a major part of the tropospheric submicron particle mass. Still, the exact formation mechanisms of SOA have remained elusive. It is now admitted that highly oxygenated organic molecules (HOMs) can contribute to a large fraction of SOA formation. In this study, we performed a set of chamber experiments to investigate the SOA formation, and the HOMs uptake and processing directly formed by OH‐radical initiated oxidation of α‐pinene under two different aerosol seed conditions. Numerous HOM compounds were identified using advanced online and offline analytical techniques, and grouped into four classes according to their different uptake behaviors. For the first time, individual HOMs uptake coefficients ranging from 1.1 × 10−2 to 1.5 × 10−1 were experimentally determined and analyzed using a resistance model which considers uptake limitations by individual gas‐ and/or particle‐phase processes. This study demonstrates that the uptake coefficients of HOMs strongly depend on their molar mass and their respective O/C ratio. Results show that aerosol seed composition and phase state affect the initial uptake of HOMs. Furthermore, the study demonstrates that the acidity and/or different seed phase‐state can significantly enhance the subsequent uptake through occurring acidity‐driven reactions reflected in a reactive behavior, particularly under (NH4)HSO4 seed conditions, promoting up to 3 times a higher SOA mass formation including the formation of highly oxidized organosulfates (HOOS). Overall, the present study implies that HOMs and their subsequent chemical processing can play an important role in both the early growth of newly formed particles and SOA formation when particle acidity is high.
    Description: Plain Language Summary: Tropospheric organic aerosol (OA) compounds represent a large part of submicron particulate matter. A big fraction of OA is formed from oxidation of emitted gaseous volatile organic compounds such as α‐pinene. Oxidation products are less‐volatile compounds that tend to condense on aerosol particles. Recently identified “highly oxygenated organic molecules” (HOMs) are formed by gas‐phase autoxidation processes and exhibit very low vapor pressures. Therefore, HOMs are expected to efficiently contribute to secondary organic aerosol (SOA). However, up to now, SOA formation potential of HOMs is still not well described because of lacking experimental investigations and analysis. Consequently, this study aims to investigate the mentioned HOMs partitioning and subsequent SOA formation from the OH‐radical initiated oxidation of α‐pinene under both Na2SO4 and (NH4)HSO4 aerosol seed conditions through complex chamber experiments. For the first time, individual HOMs uptake coefficients were determined experimentally. Further investigations demonstrated that the uptake coefficients of HOMs strongly depend on their molar mass, as well as on their respective O/C ratio. Finally, the results show that aerosol acidity and/or phase state significantly enhances the HOMs uptake and promotes up to three times higher SOA mass formation under (NH4)HSO4 seed conditions compared to that under neutral seed conditions.
    Description: Key Points: Uptake coefficients of numerous highly oxygenated organic molecules (HOMs) were experimentally determined for the first time. HOMs uptake and secondary organic aerosol formation were significantly enhanced by acidic (NH4)HSO4 seed. Highly oxidized organosulfates formation were observed under acidic (NH4)HSO4 seed conditions.
    Description: European Commission http://dx.doi.org/10.13039/501100000780
    Description: National Natural Science Foundation of China http://dx.doi.org/10.13039/501100001809
    Description: https://doi.org/10.25326/FJNF-7224
    Description: https://doi.org/10.25326/KC8N-DY53
    Keywords: ddc:551 ; aerosol study ; highly oxygenated organic molecules
    Language: English
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  • 5
    Publication Date: 2024-01-26
    Description: 〈title xmlns:mml="http://www.w3.org/1998/Math/MathML"〉Abstract〈/title〉〈p xmlns:mml="http://www.w3.org/1998/Math/MathML" xml:lang="en"〉Version 5 (v05) of the thermospheric wind data from the Michelson Interferometer for Global High‐resolution Thermospheric Imaging (MIGHTI) instrument on the Ionospheric Connection Explorer (ICON) mission has been recently released, which largely avoids local‐time dependent artificial baseline drifts that are found in previous versions of the ICON/MIGHTI wind data. This paper describes monthly climatologies of zonal‐mean winds and tides based on the v05 ICON/MIGHTI data under geomagnetically quiet conditions (Hp30 〈 3o) during April 2020–March 2022. Green‐line winds in the lower thermosphere (90–110 km) and red‐line winds in the middle thermosphere (200–300 km) are analyzed, as these data cover both daytime and nighttime. The latitude and height structures of zonal‐mean winds and tides are presented for each month, and the results are compared with the widely used empirical model, Horizontal Wind Model 2014 (HWM14). The ICON/MIGHTI and HWM14 results are in general agreement, providing a validation of the v05 ICON/MIGHTI data. The agreement is especially good for the zonal‐mean winds. Amplitudes of lower thermospheric tides from ICON/MIGHTI tend to be larger than those from HWM14 as well as from an empirical model, Climatological Tidal Model of the Thermosphere (CTMT). This could be due to the influence of interannual variability of the tides. The amplitude structure of lower thermospheric tides in HWM14 does not match those from ICON/MIGHTI and CTMT in some months. Also, HWM14 underestimates the meridional‐wind amplitude of the migrating diurnal tide in the middle thermosphere. These results highlight the need for improved tidal representation in HWM14.〈/p〉
    Description: Key Points: 〈list list-type="bullet"〉 〈list-item〉 〈p xml:lang="en"〉Monthly climatologies of zonal‐mean winds and tides at 90–110 km and 200–300 km are determined using v05 Ionospheric Connection Explorer/Michelson Interferometer for Global High‐resolution Thermospheric Imaging (ICON/MIGHTI) observations〈/p〉〈/list-item〉 〈list-item〉 〈p xml:lang="en"〉ICON/MIGHTI and Horizontal Wind Model 2014 results are in general agreement, providing a validation of the Version 5 ICON/MIGHTI data〈/p〉〈/list-item〉 〈list-item〉 〈p xml:lang="en"〉The agreement is especially good for the zonal‐mean winds, while some discrepancies are found in tidal amplitudes〈/p〉〈/list-item〉 〈/list〉 〈/p〉
    Description: Deutsche Forschungsgemeinschaft http://dx.doi.org/10.13039/501100001659
    Description: NASA
    Description: https://icon.ssl.berkeley.edu/Data
    Description: https://kp.gfz-potsdam.de/en/hp30-hp60/data
    Description: https://doi.org/10.5880/Hpo.0002
    Description: https://spaceweather.gc.ca/forecast-prevision/solar-solaire/solarflux/sx-5-mavg-en.php
    Description: https://globaldynamics.sites.clemson.edu/articles/ctmt.html
    Description: https://doi.org/10.5281/zenodo.5541913
    Keywords: ddc:551.5 ; thermosphere ; zonal‐mean winds ; tides ; ionospheric connection explorer (ICON) ; MIGHTI ; HWM14
    Language: English
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  • 6
    Publication Date: 2024-04-03
    Description: 〈title xmlns:mml="http://www.w3.org/1998/Math/MathML"〉Abstract〈/title〉〈p xmlns:mml="http://www.w3.org/1998/Math/MathML" xml:lang="en"〉On 15 January 2022, the Hunga volcano produced a massive explosion that generated perturbations in the entire atmosphere. Nonetheless, signatures in the mesosphere and lower thermosphere (MLT) have been challenging to identify. We report MLT horizontal wind perturbations using three multistatic specular meteor radars on the west side of South America (spanning more than 3,000 km). The most notorious signal is an exceptional solitary wave with a large vertical wavelength observed around 18 UT at all three sites, with an amplitude of ∼50 m/s mainly in the westward direction. Using a customized analysis, the wave is characterized as traveling at ∼200 m/s, with a period of ∼2 hr and a horizontal wavelength of ∼1,440 km in the longitudinal direction, away from the source. The perturbation is consistent with an 〈italic〉L〈/italic〉〈sub〉1〈/sub〉 Lamb wave mode. The signal's timing coincides with the arrival time of the tsunami triggered by the eruption.〈/p〉
    Description: Plain Language Summary: The eruption of the Hunga volcano in January 2022 had a widespread impact on the atmosphere, affecting various layers. We describe a perturbation in horizontal winds caused by the event, which was observed over the west coast of South America by three different meteor radar systems separated by more than 3,000 km between them. The perturbation behaved similarly in the altitude range of 80–100 km, and the wave parameters observed were consistent with high‐order Lamb wave solutions from simulations carried out using the Whole Atmosphere Community Climate Model with thermosphere/ionosphere extension. This finding complements other studies that have explored the impacts of the eruption on different atmospheric levels. Overall, this study provides valuable insights into the complex and far‐reaching effects of volcanic eruptions on the atmosphere.〈/p〉
    Description: Key Points: 〈list list-type="bullet"〉 〈list-item〉 〈p xml:lang="en"〉Hunga eruption generated extreme horizontal wind perturbations at 80–100 km of altitude over South America〈/p〉〈/list-item〉 〈list-item〉 〈p xml:lang="en"〉The signal was detected almost simultaneously by three multistatic meteor radar systems spanning more than 3,000 km〈/p〉〈/list-item〉 〈list-item〉 〈p xml:lang="en"〉The perturbation had a period of ∼2 hr, a horizontal phase velocity of ∼200 m/s, and a horizontal wavelength of ∼1,440 km〈/p〉〈/list-item〉 〈/list〉 〈/p〉
    Description: Leibniz SAW project FORMOSA
    Description: https://doi.org/10.22000/956
    Keywords: ddc:551.5 ; South America ; 2022 Hunga Eruption ; mesosphere ; lower thermosphere ; horizontal wind perturbations
    Language: English
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  • 7
    Publication Date: 2023-07-26
    Description: Assessing global progress on human adaptation to climate change is an urgent priority. Although the literature on adaptation to climate change is rapidly expanding, little is known about the actual extent of implementation. We systematically screened 〉48,000 articles using machine learning methods and a global network of 126 researchers. Our synthesis of the resulting 1,682 articles presents a systematic and comprehensive global stocktake of implemented human adaptation to climate change. Documented adaptations were largely fragmented, local and incremental, with limited evidence of transformational adaptation and negligible evidence of risk reduction outcomes. We identify eight priorities for global adaptation research: assess the effectiveness of adaptation responses, enhance the understanding of limits to adaptation, enable individuals and civil society to adapt, include missing places, scholars and scholarship, understand private sector responses, improve methods for synthesizing different forms of evidence, assess the adaptation at different temperature thresholds, and improve the inclusion of timescale and the dynamics of responses.
    Type: info:eu-repo/semantics/article
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  • 8
    Publication Date: 2023-07-27
    Description: We summarise the discussions at a virtual Community Workshop on Cold Atoms in Space concerning the status of cold atom technologies, the prospective scientific and societal opportunities offered by their deployment in space, and the developments needed before cold atoms could be operated in space. The cold atom technologies discussed include atomic clocks, quantum gravimeters and accelerometers, and atom interferometers. Prospective applications include metrology, geodesy and measurement of terrestrial mass change due to, e.g., climate change, and fundamental science experiments such as tests of the equivalence principle, searches for dark matter, measurements of gravitational waves and tests of quantum mechanics. We review the current status of cold atom technologies and outline the requirements for their space qualification, including the development paths and the corresponding technical milestones, and identifying possible pathfinder missions to pave the way for missions to exploit the full potential of cold atoms in space. Finally, we present a first draft of a possible road-map for achieving these goals, that we propose for discussion by the interested cold atom, Earth Observation, fundamental physics and other prospective scientific user communities, together with the European Space Agency (ESA) and national space and research funding agencies.
    Language: English
    Type: info:eu-repo/semantics/article
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  • 9
    Publication Date: 2023-12-07
    Description: Accurate assessment of anthropogenic carbon dioxide (CO2) emissions and their redistribution among the atmosphere, ocean, and terrestrial biosphere in a changing climate is critical to better understand the global carbon cycle, support the development of climate policies, and project future climate change. Here we describe and synthesize data sets and methodology to quantify the five major components of the global carbon budget and their uncertainties. Fossil CO2 emissions (EFOS) are based on energy statistics and cement production data, while emissions from land-use change (ELUC), mainly deforestation, are based on land-use and land-use change data and bookkeeping models. Atmospheric CO2 concentration is measured directly, and its growth rate (GATM) is computed from the annual changes in concentration. The ocean CO2 sink (SOCEAN) is estimated with global ocean biogeochemistry models and observation-based fCO2 products. The terrestrial CO2 sink (SLAND) is estimated with dynamic global vegetation models. Additional lines of evidence on land and ocean sinks are provided by atmospheric inversions, atmospheric oxygen measurements, and Earth system models. The resulting carbon budget imbalance (BIM), the difference between the estimated total emissions and the estimated changes in the atmosphere, ocean, and terrestrial biosphere, is a measure of imperfect data and incomplete understanding of the contemporary carbon cycle. All uncertainties are reported as ±1σ. For the year 2022, EFOS increased by 0.9 % relative to 2021, with fossil emissions at 9.9±0.5 Gt C yr−1 (10.2±0.5 Gt C yr−1 when the cement carbonation sink is not included), and ELUC was 1.2±0.7 Gt C yr−1, for a total anthropogenic CO2 emission (including the cement carbonation sink) of 11.1±0.8 Gt C yr−1 (40.7±3.2 Gt CO2 yr−1). Also, for 2022, GATM was 4.6±0.2 Gt C yr−1 (2.18±0.1 ppm yr−1; ppm denotes parts per million), SOCEAN was 2.8±0.4 Gt C yr−1, and SLAND was 3.8±0.8 Gt C yr−1, with a BIM of −0.1 Gt C yr−1 (i.e. total estimated sources marginally too low or sinks marginally too high). The global atmospheric CO2 concentration averaged over 2022 reached 417.1±0.1 ppm. Preliminary data for 2023 suggest an increase in EFOS relative to 2022 of +1.1 % (0.0 % to 2.1 %) globally and atmospheric CO2 concentration reaching 419.3 ppm, 51 % above the pre-industrial level (around 278 ppm in 1750). Overall, the mean of and trend in the components of the global carbon budget are consistently estimated over the period 1959–2022, with a near-zero overall budget imbalance, although discrepancies of up to around 1 Gt C yr−1 persist for the representation of annual to semi-decadal variability in CO2 fluxes. Comparison of estimates from multiple approaches and observations shows the following: (1) a persistent large uncertainty in the estimate of land-use changes emissions, (2) a low agreement between the different methods on the magnitude of the land CO2 flux in the northern extra-tropics, and (3) a discrepancy between the different methods on the strength of the ocean sink over the last decade.
    Language: English
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  • 10
    Publication Date: 2023-07-18
    Description: Assessing global progress on human adaptation to climate change is an urgent priority. Although the literature on adaptation to climate change is rapidly expanding, little is known about the actual extent of implementation. We systematically screened 〉48,000 articles using machine learning methods and a global network of 126 researchers. Our synthesis of the resulting 1,682 articles presents a systematic and comprehensive global stocktake of implemented human adaptation to climate change. Documented adaptations were largely fragmented, local and incremental, with limited evidence of transformational adaptation and negligible evidence of risk reduction outcomes. We identify eight priorities for global adaptation research: assess the effectiveness of adaptation responses, enhance the understanding of limits to adaptation, enable individuals and civil society to adapt, include missing places, scholars and scholarship, understand private sector responses, improve methods for synthesizing different forms of evidence, assess the adaptation at different temperature thresholds, and improve the inclusion of timescale and the dynamics of responses.
    Language: English
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