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Formation of anomalous odd-numbered carbon cluster ions in the gas-phase coalescence reactions of fullerenes (1994)

Zhu, Lei ; Wang, Shenyi ; Li, Yufen

College Park, Md. : American Institute of Physics (AIP)

The Journal of Chemical Physics 101 (1994), S. 8592-8595

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ISSN: 1089-7690

Source: AIP Digital Archive

Topics: Physics , Chemistry and Pharmacology

Notes: We report the observation of efficient coalescence reactions of fullerenes in the negative ion channel by laser desorption ionization of chemical adduct compounds of C60. Not only the even-numbered daughter fullerenes by successive C2 losses or captures appeared, but also odd-numbered carbon cluster anions C−N (51≤N≤65) were detected in the chemical-fusion processes. The results suggest that the anomaly is originated from the special reaction activity of nascent C60 produced by laser-induced dissociation of adduct compound molecules, and thereby provide a new way to open fullerene cages.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1063/1.468054

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