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State-resolved differential cross sections for the reaction D+H2→HD+H (1987)

Buntin, Steven A. ; Giese, Clayton F. ; Gentry, W. Ronald

College Park, Md. : American Institute of Physics (AIP)

The Journal of Chemical Physics 87 (1987), S. 1443-1445

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ISSN: 1089-7690

Source: AIP Digital Archive

Topics: Physics , Chemistry and Pharmacology

Notes: Differential cross sections for the reaction D+H2→HD+H were measured with a novel crossed molecular beam technique, in which a pulse of energetic D atoms is formed by 193 nm photolysis of D2S and crossed with a pulse of H2 at a variable intersection angle. Speed distributions of the product HD, measured by time-of-flight to a mass spectrometer detector, show clearly resolved peaks for v=0 and v=1 at center-of-mass scattering angles near 180°, for an initial relative kinetic energy of 0.95 eV. Analysis of the data by computer simulation of the experiment yields a v=0/v=1 population ratio of 5.1, and average rotational energies of 0.26 eV in V=0 and 0.11 eV in v=1.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1063/1.453275

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