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  • Articles  (190)
  • nitrogen  (78)
  • mercury  (63)
  • acid deposition  (49)
  • Energy, Environment Protection, Nuclear Power Engineering  (190)
  • 1
    Electronic Resource
    Electronic Resource
    Application of an ion mobility detector in radiation stimulated plasma chemistry
    Amsterdam : Elsevier
    Radiation Physics and Chemistry 42 (1993), S. 993-996 
    Details
    ISSN: 0969-806X
    Keywords: acceleration ; argon ; beta particles ; drift ; electric field ; electrons ; excited states ; ion mobility ; ions mobility ; nitrogen ; reactive species
    Source: Elsevier Journal Backfiles on ScienceDirect 1907 - 2002
    Topics: Chemistry and Pharmacology , Energy, Environment Protection, Nuclear Power Engineering , Physics
    Type of Medium: Electronic Resource
    URL: http://linkinghub.elsevier.com/retrieve/pii/0969-806X(93)90419-U
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  • 2
    Electronic Resource
    Electronic Resource
    Mercury and selenium in arctic and coastal seals off the coast of Norway
    Amsterdam : Elsevier
    Environmental Pollution 85 (1994), S. 153-160 
    Details
    ISSN: 0269-7491
    Keywords: grey seal ; harbour seal ; harp seal ; mercury ; ringed seal ; selenium
    Source: Elsevier Journal Backfiles on ScienceDirect 1907 - 2002
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1016/0269-7491(94)90081-7
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  • 3
    Electronic Resource
    Electronic Resource
    Influence of Prenatal Mercury Exposure Upon Scholastic and Psychological Test Performance: Benchmark Analysis of a New Zealand Cohort (1998)
    Springer
    Risk analysis 18 (1998), S. 701-713 
    Details
    ISSN: 1539-6924
    Keywords: Benchmark ; mercury ; risk assessment ; epidemiology
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract This paper presents benchmark (BMD) calculations and additional regression analyses of data from a study in which scores from 26 scholastic and psychological tests administered to 237 6- and 7-year-old New Zealand children were correlated with the mercury concentration in their mothers' hair during pregnancy. The original analyses of five test scores found an association between high prenatal mercury exposure and decreased test performance, using category variables for mercury exposure. Our regression analyses, which utilized the actual hair mercury level, did not find significant associations between mercury and children's test scores. However, this finding was highly influenced by a single child whose mother's mercury hair level (86 mg/kg) was more than four times that of any other mother. When that child was omitted, results were more indicative of a mercury effect and scores on six tests were significantly associated with the mothers' hair mercury level. BMDs calculated from five tests ranged from 32 to 73 mg/kg hair mercury, and corresponding BMDLs (95% lower limits on BMDs) ranged from 17 to 24 mg/kg. When the child with the highest mercury level was omitted, BMDs ranged from 13 to 21 mg/kg, and corresponding BMDLs ranged from 7.4 to 10 mg/kg.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/B:RIAN.0000005917.52151.e6
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  • 4
    Electronic Resource
    Electronic Resource
    Nitrogen mineralization in high elevation forests of the Appalachians. I. Regional patterns in southern spruce-fir forests (1989)
    Springer
    Biodegradation 7 (1989), S. 131-145 
    Details
    ISSN: 1572-9729
    Keywords: Picea rubens ; Abies fraseri ; acid deposition ; forest decline
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract Annual and seasonal rates of net nitrogen mineralization were determined for 19 sites in the spruce-fir forests of the Southern Appalachian Mountains. These sites included high and low elevation stands of red spruce (Picea rubens Sarg.) and Fraser fir (Abies fraseri (Pursh.) Poir.) on east and west exposures on Whitetop Mountain, Virginia; Mt. Mitchell, North Carolina; and Clingman's Dome in the Great Smoky Mountains National Park. Mineralization rates were determined using in situ soil incubations in PVC tubes with ion exchange resin bags placed in the bottom of the tubes to collect leachate. Throughfall was collected in resin bags placed in the top of the tubes. Average initial NH4-N + NO3-N ranged from 0.6 to 4.8 kg N/ha across all plots, and average mineralization rates ranged from 26 to 180 kg-N ha−1 yr−1. Throughfall ranged from 18 to 32 kg-N ha−1 yr−1 with NH4-N accounting for about two-thirds of the throughfall N across all sites. Throughfall and mineralization rates were not related to elevation or exposure. The high rates of N mineralization and relatively high nitrate concentrations indicate that leaching losses of nitrogen and associated cations could be substantial.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00004125
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  • 5
    Electronic Resource
    Electronic Resource
    Aboveground nitrogen and phosphorus use by five plantation-grown trees with different leaf longevities (1991)
    Springer
    Biodegradation 14 (1991), S. 167-191 
    Details
    ISSN: 1572-9729
    Keywords: leaf longevity ; nitrogen ; nutrient use efficiency ; phosphorus ; requirement ; retranslocation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract Aboveground nitrogen (N) and phosphorus (P) requirement, retranslocation and use efficiency were determined for 28-year-old red oak (Quercus rubra L.), European larch (Larix decidua Miller), white pine (Pinus strobes L.), red pine (Pinus resinosa Ait.) and Norway spruce (Picea abies (L) Karst.) plantations on a similar soil in southwestern Wisconsin. Annual aboveground N and P requirements (kg/ha/yr) totaled 126 and 13 for red oak, 86 and 9 for European larch, 80 and 9 for white pine, 38 and 6 for red pine, and 81 and 13 for Norway spruce, respectively. Nitrogen and P retranslocation from current foliage ranged from 81 and 72%, respectively, for European larch, whereas red pine retranslocated the smallest amount of N (13%) and Norway spruce retranslocated the smallest amount of P (18%). In three evergreen species, uptake accounted for 72 to 74% of annual N requirement whereas for two deciduous species retranslocation accounted for 76 to 77% of the annual N requirement. Nitrogen and P use (ANPP/uptake) was more efficient in deciduous species than evergreen species. The results from this common garden experiment demonstrate that differences in N and P cycling among species may result from intrinsic characteristics (e.g. leaf longevity) rather than environmental conditions.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00000806
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  • 6
    Electronic Resource
    Electronic Resource
    A ground water nitrogen budget for a headwater swamp in an area of permanent ground water discharge (1991)
    Springer
    Biodegradation 14 (1991), S. 209-224 
    Details
    ISSN: 1572-9729
    Keywords: ground water ; hydrology ; nitrogen ; mass balance ; nutrient retention ; swamp
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract Ground water inputs and outputs of N were studied for a small ground water discharge swamp situated in a headwater drainage basin in southern Ontario, Canada. Darcy's equation with data for piezometers was used to measure inputs of shallow local ground water at the swamp margin and deep regional ground water beneath the swamp. Ground water flux was also quantified by measuring ground water discharge to the outlet stream draining the swamp in combination with a chemical mixing model to separate shallow and deep ground water components based on chloride differences. Estimates of shallow ground water flux determined by these two approaches agreed closely however, the piezometer data seriously underestimated the deep ground water input to the swamp. An average ground water input-output budget of total N (TN) total organic nitrogen (TON) ammonium (NH4 +-N) and nitrate (NO3 --N) was estimated for stream base flow periods which occurred on an average of 328 days each year during 1986–1990. Approximately 90% of the annual NO3 --N input was contributed by shallow ground water at the swamp margin. Deep ground water represented about 65% of the total ground water input and a similar proportion of TON and NH4 +-N inputs. Annual ground water NO3 --N inputs and outputs were similar whereas NH4 +-N retention was 4 kg ha-1 representing about 68% of annual ground water input. Annual TON inputs in ground water exceeded outputs by 7.7 kg ha (27%). The capacity of the swamp to regulate ground water N fluxes was influenced by the N chemistry of ground water inputs and the hydrologic pathways of transport within the swamp.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00000808
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  • 7
    Electronic Resource
    Electronic Resource
    Soil chemistry change in a lowland english deciduous Woodland 1974–1991 (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 677-682 
    Details
    ISSN: 1573-2932
    Keywords: soils ; acidification ; ancient woodland ; nitrogen ; environmental change
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract This study outlines the results of analysis of soil samples collected from fixed quadrats located in a regular pattern across Wytham Wood. Oxfordshire, England. The site contains plots of mixed deciduous ancient woodland and more recent plantations. A previous soil study was undertaken in 1974 and samples archived. Soils were resampled in 1991 and some re-analysis of the 1974 samples was undertaken. Soils were of a wide range in types from sands to gravels with a pH range of 3.0–7.0. Results showed some decline in pH in lower horizons, but most striking was a large increase in soil nitrogen for all horizons and soil types.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00476907
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  • 8
    Electronic Resource
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    Nine years of measurements of atmospheric nitrogen and sulphur deposition to Danish forest (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2205-2210 
    Details
    ISSN: 1573-2932
    Keywords: Trend ; gas ; aerosol ; bulk precipitation ; throughfall ; acid deposition
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Since 1985 measurements of gasses, aerosols, precipitation and throughfall have been carried out at three forest sites in Denmark with equal aged Norway Spruce plantations. The times series show a downward trend in the concentration of sulphur dioxide. Particulate sulphate, ammonia and particulate ammonium and the total nitrate seem to have a more constant concentration level. The wet deposition measurements show a decreasing trend in the content of acid (protons), sulphate, ammonium and nitrate, though for the nitrogen compounds it is only a slight fall. A decrease in concentrations of protons and sulphate is also seen in the throughfall measurements, in throughfall the nitrogen compounds hardly seem to decrease.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01186161
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  • 9
    Electronic Resource
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    Deposition gradients and foliar and soil leachate concentrations of air pollutants in Scots pine stands of S.-E. Finland and the Karelian Isthmus, N.-W. Russia (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1263-1268 
    Details
    ISSN: 1573-2932
    Keywords: air pollution ; sulphur ; nitrogen ; base cations ; throughfall ; Scots pine ; needle elements ; soil leachate ; N.-W. Russia
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Bulk precipitation and throughfall analyses in 50–100-year-old Scots pine stands revealed decreasing sulphur, nitrogen, calcium and magnesium deposition gradients, which extend from the St. Petersburg-Leningrad region and N.-E. Estonia to S.-E. Finland. The Ca and Mg deposition alleviate the acidifying effect of sulphur and nitrogen. The Scots pine canopies acted as a sink for ammonium and nitrate, while the canopy interactions increased sulphur, calcium and magnesium content in throughfall. Foliar S, N and Ca concentrations correlated positively with the corresponding deposition loads. In contrast, low foliar magnesium concentrations were detected in the vicinity of St. Petersburg. The results indicate that the sulphur and calcium deposition may have increased soil leachate S and Ca concentrations in the most polluted Scots pine stands.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00477155
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  • 10
    Electronic Resource
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    Cost-Effective Nutrient Reductions to the Baltic Sea (1997)
    Springer
    Environmental and resource economics 10 (1997), S. 341-362 
    Details
    ISSN: 1573-1502
    Keywords: Baltic Sea ; eutrophication ; nitrogen ; phosphorus ; cost effective
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering , Economics
    Notes: Abstract Due to eutrophication caused by heavy loads of nitrogen and phosphorus, the biological conditions of the Baltic Sea have been disturbed: large sea bottom areas without any biological life, low stocks of cods, and toxic blue green algaes. It is recognized that the nitrogen and phosphorus loads to the Baltic Sea must be reduced by 50% in order to restore the sea. The main purpose of this paper is to calculate cost effective nitrogen and phosphorus reductions to the Baltic Sea from the nine countries surrounding the Baltic Sea. The results show a significant difference in minimum costs of decreasing nitrogen and phosphorus loads to the Sea: approximately 12 000 millions of SEK per year and 3 000 millions of SEK respectively for reductions by 50%. It is also shown that a change from a policy of cost-effective nutrient reductions to a policy where each country reduces the nutrient loads by 50% increase total costs for both nitrogen and phosphorus reductions by about 300%. The results are, however, sensitive to several of the underlying assumptions and should therefore be interpreted with much caution.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1026497515871
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  • 11
    Electronic Resource
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    Sulphur and nitrogen deposition in Norway, status and trends (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 623-628 
    Details
    ISSN: 1573-2932
    Keywords: monitoring ; deposition ; sulphur ; nitrogen
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The total deposition of sulphur (S) and nitrogen (N) components in Norway during the period 1988–1992 has been estimated on the basis of measurement data of air- and precipitation chemistry from the national monitoring network. There are large regional variations in depositions with highest values in the southwestern part of Norway. Time series analysis of annual mean concentrations of sulphur dioxide (SO2) and sulphate (SO4 −−) in air, non marine SO4 −−, nitrate (NO3 −) and ammonium (NH4 +) in precipitation, shows a significant reduction in the S concentrations both in air and precipitation. In precipitation the concentrations are reduced by 30–45 percent in Southern Norway and 45–55 percent in Central and Northern Norway. Even larger reductions are observed in air concentrations with 50–65 percent reduction in Southern Norway and 65–88 percent reduction further north. For N components there are generally no significant trends in concentration levels nor in precipitation or air. The observed trends are comparable with reported trends in emission.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00476898
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  • 12
    Electronic Resource
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    Soil sensitivity due to acid and heavy metal deposition in East Central Europe (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 737-742 
    Details
    ISSN: 1573-2932
    Keywords: acid deposition ; heavy metals ; cadmium ; soil contamination
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Simultaneous soil acidification and deposition of heavy metals is a major concern for forest and agricultural soils of the Black Triangle region of East Central Europe including southern former East Germany, northern Bohemia of the Czech Republic, and southern Poland. The objective of this project was to develop historical and future projections of acid and heavy metal deposition to soils (As, Cd, Pb, Zn) and to produce a preliminary map of soil sensitivity to cadmium pollution and uptake by crops. Ultimately, we wish to assess the relative hazard and recovery times of soils to metals deposition in the region. Emission and deposition data bases obtained from several models developed at IIASA were linked using the Geographical Information System ARC/INFO to produce soil maps of sensitivity to cadmium mobility based on metals deposition, soil type, soil texture, organic matter content, and acid deposition. RAINS 6.1 (Alcamo et al., 1990) was utilized to produce maps of acid deposition for EMEP grids (150 km x 150 km). The largest amount of acid load is deposited in southern East Germany. Sulfur deposition in that area was 10–12 gS/m2/yr in 1990, and S+N deposition exceeded 8000 eq/ha/yr. But the “hot spot” for metals deposition is further to the east, in the Silesia area of southern Poland. The TRACE2 trajectory model of Alcamo, Bartnicki, and Olendrzynski (1992) was used to estimate cumulative metals deposition since 1955 with scenarios to 2010. Pb has improved over Europe since 1970 when depositions in the Ruhr River Valley of West Germany exceeded 60 mg/m2/yr. But cadmium deposition in southern Poland (Katowice and Krakow) has now accumulated to 60–70 mg/m2 by atmospheric deposition alone. During base case simulations from 1955–87, approximately 1.8 mg/kg Pb and 0.12 mg/kg Cd have been added to the mixed plow-layer of ∼30 cm. If these emissions continue indefinitely, the accumulation of metals will become problematic for agriculture and the food chain.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00476917
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  • 13
    Electronic Resource
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    Implications of natural acidification for mitigation strategies in northern Sweden (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 499-504 
    Details
    ISSN: 1573-2932
    Keywords: Surface water ; water chemistry ; DOC ; liming ; acid deposition
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Northern Sweden has been regarded as unaffected by acid deposition, but many surface waters in the region fall within the definition of acid surface water (pH 〈 6.0, alkalinity 〈 50 mmolc m−3) permanently or during episodes. Approximatly 100 MSEK in spent annually on liming in northern Sweden. This paper summarizes our conclusions from a workshop on natural versus anthopogenic acidification held in February 1995. It was shown that organic substances have a key role in determining the acidity of surface waters in the region, although anthropogenic effects are documented in some coastal systems and in the southern mountain range. Sulfide oxidation occurs by the coast. It appears clear that many surface waters that were naturally acidic have been limed to unnatural pH levels. New criteria to screen liming candidates should be developed, and one such model based on water chemistry data is proposed.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00476878
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  • 14
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    Concentrations and depositions of SO2, SO4 2− etc. in a Chongqing suburban forested area (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1299-1304 
    Details
    ISSN: 1573-2932
    Keywords: forest decline ; SO2 ; sulfate ; tandem filter ; throughfall ; acid deposition
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract During the period from 25 May 1991 to 30 May 1992 the atmospheric concentrations and depositions of oxides of sulfur were continuously measured in a suburban masson pine forest which is currently experiencing severe dieback, in Chongqing, China. The annual mean concentrations of SO2 and particulate SO4 2− were 220 μ g/m3 (77 ppbv) and 32 μ g/m3 respectively. The atmospheric concentrations of these sulfur compounds were high in late autumn and winter. The annual wet and dry depositions of sulfur to the forest as measured by throughfall and stemflow were 93.1 and 46.6 kgSha−1a−1 respectively. These depositions are among the highest level ever reported in the world. Althogh the cause of the dieback of the masson pine trees has not been unequivocally determined, it is probable that the direct impact of SO2 is more likely the cause than acid deposition.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00477161
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  • 15
    Electronic Resource
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    Perch mercury content is related to acidity and color of 26 Russian lakes (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 823-828 
    Details
    ISSN: 1573-2932
    Keywords: fish ; mercury ; lake chemistry ; biomagnification
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract We determined mercury in fish (perch Perca fluviatilis) from 26 Russian lakes in three regions over four years. The lakes ranged in size from 2 to 395,000 ha, in pH from 4.5 to 10.0, and in color from 3 to 190 hazen. Sixteen lakes were drainage lakes, with permanent outlets, and 10 were seepage lakes, with no permanent inlets or outlets. The lakes were generally located in forested regions with little or no human habitation in the watershed. The three regions were geologically distinct: Precambrian Shield granitic bedrock covered with thin soil; Triassic bedrock covered with thick glacial tills; and Triassic bedrock covered with thin sediments. At each lake water samples were collected and analyzed for pH, add neutralizing capacity (ANC), major cations, and anions. Dissolved mercury species were estimated with a thermodynamic equilibrium model (MINTEQA2). Mercury content of dorsal muscle varied from 0.04 to 1.0 μg/g wet weight, and was linearly related to calculated HgCH3Cl (r20.68, p〈0.001). Lake HgCH3Cl, in turn, was related to lake pH (r2=0.86, p〈0.001). Stepwise multiple regression selected lake HgCH3Cl and color as the factors most highly related to fish mercury content, with the model accounting for 75% of the variation.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00476931
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  • 16
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    Indirect effects of N and S deposition on a Norway spruce ecosystem. An update of findings within the Skogaby project (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1613-1622 
    Details
    ISSN: 1573-2932
    Keywords: Deposition ; ecosystem ; nitrogen ; Norway spruce ; nutrient cycling ; production ; root function ; sulphur
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In this paper we try to interpret results from different investigations where an ecosystem with Norway spruce was manipulated with increased N and S deposition via the soil system. The site, in Skogaby in Southwest Sweden, had 1989–93 an annual deposition of 9 kg NH4-N; 7 kg NO3-N and 20 kg SO4-S ha−1. The stand was treated during 6 years with 100 kg N and 114 kg S ha− y−1 in the form of ammonium sulphate (NS treatment). The stand reacted with increased above ground production of 31% after 3 years of treatment. The uptake above ground of N was 155 kg ha−1 higher than in the control. Those trends were even stronger after 6 years of treatment. There were no decreases in the uptake of P, K, Ca or Mg (but for B) after 3 or 6 years of NS-treatment. Needle macro nutrient concentrations in relation to N decreased for several nutrients due to dilution effects. As result of the NS treatment pH increased markedly in the litter layer, and less, but significantly, in the humus layer. A decrease in pH value by about 0.3 units was found in the rest of the soil profile down to 50 cm. Dry mass of needle litter fall and litter layer both increased as a result of 6 years of NS-treatment. After three years of treatment 77–80% of all living fine roots in both control and NS treatment were found in the humus layer and the upper 10 cm of the mineral soil. The amount of living fine roots in the humus layer of NS-treated trees decreased to about one third of the control, and the amount of dead fine roots increased by 150% compared with untreated trees after 6 years of treatment. It is argued that the decreased amount of living and increased amount of dead fine roots not necessarily are indications of decreased root vitality. It can also be explained by increased root turnover rate and decreased decomposition rates of N rich new and old fine root litter. No inorganic N was leached from the control plots whereas the NS treated plots started to leach NO3 the second year of treatment. During 1989–1993 a total of 44 kg NO3-N and 30 kg NH4-N per ha was lost from the system which means that 88% of the N supplied was retained by the ecosystem. At first SO4 was adsorbed in the soil, but after five years of treatment the output was almost equal to the input.
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    URL: http://dx.doi.org/10.1007/BF00477211
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  • 17
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    Development and application of a reactive plume model for mercury emissions (1995)
    Springer
    Water, air & soil pollution 80 (1995), S. 325-335 
    Details
    ISSN: 1573-2932
    Keywords: Atmospheric chemistry ; mercury ; plume model
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A reactive plume model that includes atmospheric chemical reactions of mercury was developed. The model simulates advective transport with the mean wind flow; horizontal and vertical turbulent diffusion; gas phase; aqueous-phase and particulate chemistry; cloud microphysics; wet deposition and dry deposition. The model was applied to the simulation of clear sky, non-precipitating cloud and precipitating cloud scenarios. No significant mercury chemistry occurs in the absence of droplets. In clouds, Hg(II) is reduced to Hg(0) with more reduction taking place in precipitating clouds than in non-precipitating clouds.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01189682
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  • 18
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    Denuder-based techniques for sampling, separation and analysis of gaseous and participate mercury in air (1995)
    Springer
    Water, air & soil pollution 80 (1995), S. 1209-1216 
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    ISSN: 1573-2932
    Keywords: gaseous ; particulate ; mercury ; sampling ; silver ; gold ; denuder
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A denuder-based method for sampling and separating gaseous and participate mercury in the air is described. Two different denuder configurations developed in Vilnius, Lithuania (silver) and in Gothenburg, Sweden (gold) are compared. Data were acquired at different sampling locations around the cities of Vilnius and Gothenburg. The concentration of particulate Hg was found to be 0.04 to 0.40 ng m−3 in the Vilnius region, and 0.11 to 0.57 ng m−3 in the Gothenburg region. Intel-calibration results for the silver and gold denuders are presented. The results obtained by the two different denuder configurations and sampling set-ups display satisfactory agreement.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01189784
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  • 19
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    Acid deposition: Perspectives in time and space (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 15-24 
    Details
    ISSN: 1573-2932
    Keywords: Acid deposition ; global change ; Asia ; fertilizer ; nitrogen ; sulfur
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Most acid-deposition investigations have been concerned with the impact of nitrogen oxides (NOx) and sulfur dioxide (SO2) emissions on Europe and North America. This paper examines three issues beyond this central focus. Major conclusions are 1) ammonia (NH3) emissions and subsequent nitrogen (N) accumulation in terrestrial ecosystems have the potential to generate significant acidification in terrestrial and aquatic ecosystems; 2) sulfur (S) and N accumulation in environmental reservoirs will not only result in significant and extensive acidification but will also impact the earth's radiation balance, tropospheric oxidizing capacity, ecosystem nutrient balance and groundwater quality; and 3) future emissions will substantially increase in the developing world, especially in Asia. By 2020, Asian emissions of SO2, NOx and NH3 will be equal to or greater than the combined emissions from Europe and North America.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00483685
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  • 20
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    Soil changes induced by air pollutant deposition and their implication for forests in central Europe (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 63-76 
    Details
    ISSN: 1573-2932
    Keywords: Forest damage ; soil acidity ; N-saturation ; acid deposition ; root growth ; drought
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A survey of leaf and needle losses of European forests in 1993 revealed that 23% of the total forested area had defoliation of more than 25%. The focus of this defoliation is in Central Europe, namely in Poland, Slowakia, Czech Republic, and Germany. The annual surveys of leaf losses and discoloration indicated only small changes during the last years for the coniferous forests in Germany. However, the increasing leaf losses of oak and beech during the last years were alarming. Evaluating the potential relation between air pollutant deposition, soil changes and forest damage, we focus here on the recent changes in deposition and soil conditions, and their implication on tree root development and drought susceptability of trees. While deposition of SO4 2−, H+ and Ca2+ in many Central European forests decreased in the last decade, input of NH4 + and NO3 − remained high or even increased. The H+ load of many forest soils today is thus still high compared to weathering rates, but the proportion of the H+ load resulting from turnover of deposited N has increased. Recent effects of changing depositions on acid forest soils were: depletion of soil Al-pools, release of formerly stored soil SO4 2−, accumulation of N in soil organic matter, increasing N availability to trees and decreasing concentration of Ca2+ in the soil solution. We hypothesise that soil acidification and increased N availability will decrease the fine root biomass of trees and shift the rooting zone to upper soil layers. Increased above ground growth, observed in many areas of Europe, will furthermore decrease the root/shoot ratio. This development will finally cause increased drought susceptability of trees and is thus of destabilizing nature. The proposed chain of events might be overlapped by other effects of air pollutants on forest ecosystems, namely direct effects of gases on leaves, nutritional inbalances, and interactions with pests.
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    URL: http://dx.doi.org/10.1007/BF00483689
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    Global forest systems: An uncertain response to atmospheric pollutants and global climate change? (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 101-110 
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    ISSN: 1573-2932
    Keywords: carbon ; nitrogen ; sulfur ; biogeochemistry ; mitigation ; global change
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Forest systems cover more than 4.1×109 ha of the Earth's land area. The future response and feedbacks of forest systems to atmospheric pollutants and projected climate change may be significant. Boreal, temperate and tropical forest systems play a prominent role in carbon (C), nitrogen (N) and sulfur (S) biogeochemical cycles at regional and global scales. The timing and magnitude of future changes in forest systems will depend on environmental factors such as a changing global climate, an accumulation of CO2 in the atmosphere, and increase global mineralization of nutrients such as N and S. The interactive effects of all these factors on the world's forest regions are complex and not intuitively obvious and are likely to differ among geographic regions. Although the potential effects of some atmospheric pollutants on forest systems have been observed or simulated, large uncertainty exists in our ability to project future forest distribution, composition and productivity under transient or nontransient global climate change scenarios. The potential to manage and adapt forests to future global environmental conditions varies widely among nations. Mitigation practices, such as liming or fertilization to ameliorate excess NOx or SOx or forest management to sequester CO2 are now being applied in selected nations worldwide.
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    URL: http://dx.doi.org/10.1007/BF00483692
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    Establishing an acid deposition monitoring network in East Asia (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 273-278 
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    ISSN: 1573-2932
    Keywords: acid deposition ; expert meetings ; monitoring guidelines ; monitoring network ; East Asia ; Environment Agency of Japan
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Acid deposition is widely recognized as one of the most serious international atmospheric pollution problems. East Asian countries are currently experiencing acid deposition and have only recently begun expanding domestic research and monitoring activities. However, acid deposition is not only a domestic but also a transboundary problem. In addressing the transboundary aspect, cooperative and collaborative action will be essential. The Environment Agency of Japan is advocating the need to establish an acid deposition monitoring network in East Asia. Therefore, it is sponsoring three “Expert Meetings on Acid Precipitation Monitoring Network in East Asia” between 1993 and 1995. The meetings are attended by both scientific researchers and government officials from numerous East Asian countries. At the administrative and scientific discussions of the first two meetings a consensus on the desirability of establishing a monitoring network in East Asia was obtained and a preliminary technical guideline manual for monitoring acid deposition was adopted. By the end of the third meeting it is hoped that a basic consensus can be reached on a framework for an East Asian acid deposition monitoring network. It is essential to establish such a network in order to evaluate the present state of acid deposition in the region and to reach a common scientific understanding on the acid deposition problem. This is a vital step toward promoting international cooperation on the issue.
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    URL: http://dx.doi.org/10.1007/BF00483707
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    Integrated assessment models as a basis for air pollution negotiations (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 249-260 
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    ISSN: 1573-2932
    Keywords: acid deposition ; integrated assessment ; modeling ; protocols
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract During the last decade the issue of integrated assessment has received attention both in the scientific literature and in the negotiation of international air pollution agreements. More than often this literature does not differentiate between the integrated assessment as a process and the development and use of models as a tool for calculating the potentials of various scenarios. This paper describes the difference between the process and the tool, and illustrates this using the negotiations leading to the Second Sulfur Protocol (June 1994, Oslo). The situation in Europe (with a highly visible interaction between science and policy) will be compared with the United States (where new legislation was passed before the integrated assessment was finished). Further, the role of integrated assessment models in these negotiations will be discussed with special attention for the interaction between model builders and model users. Lessons from the recent European experience will be drawn. These include lessons for future protocols on acidification, and combined ozone/acidification/eutrophicationprotocols. These lessons will deal with the scale of the problem, the scope of the integrated assessment models, the development of models in parallel with scientific development and the various modes of interaction with the policy community.
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    URL: http://dx.doi.org/10.1007/BF00483705
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    Nutrient balance in Scots pine (Pinus sylvestris L.) forest. 2. Effects of plant growth and N-deposition on soil solution and leachate chemistry in a lysimeter experiment (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1149-1154 
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    ISSN: 1573-2932
    Keywords: forest soil ; leaching ; lysimeter ; nitrogen
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Three years of N application to a Cambic arenosol (Typic Udorthent) in two lysimeter series, one with and one without young saplings of Pinus sylvestris L. have produced significant changes in soil solution and leachate chemistry. An application of 30 kg N/ha*yr−1 significantly increased NO3 − leaching from the soil. This N load was also sufficient to significantly increase the mobility of the phyto-toxic elements Al3+ and Mn2+, likewise to increase leaching of the important plant nutrients Ca2+, Mg2+ and K+. At a N load of 90 kg N/ha*yr−1 significant increase in NH4 + leaching was observed, but total leaching of NH4 + was still very low compared to NO3 − leaching. No significant treatment effects were found for SO4 2−, Fe2+ and Cl− in the leachate. Trees grown in the lysimeters buffered the acidifying effect of N application and increased the leachate pH by 0.2 pH units compared to lysimeters without trees.
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    URL: http://dx.doi.org/10.1007/BF00477136
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    Effects of nitrogen load to the forest floor in sitka spruce stands (Picea sitchensis) as affected by difference in deposition and spruce aphid infestations (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1173-1178 
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    ISSN: 1573-2932
    Keywords: sitka spruce ; nitrogen ; deposition ; leaching ; proton production ; green spruce aphid
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Studies of biogeochemical cycling and soil acidification have been carried out in even aged stands of Norway spruce, sitka spruce, Douglas fir, beech and oak under the frame of “The Element Cycling Project”. Deposition of excess nitrogen to forests is important as a potential acidifying input. In Denmark, reduced vitality in Norway spruce has promoted extensive planting of sitka spruce. However, several spruce aphid infestations have caused defoliation in many sitka spruce stands. The objectives of this study were to evaluate the effects of deposition and increased litterfall due to spruce aphid infestations on nitrogen transformations in the forest floor in sitka spruce stands on different soil types. The deposition of throughfall nitrogen range from 19 to 35 kg/ha/year. Fluxes of nitrogen in litterfall ranged from 21 to 77 kg/ha/year, whereas nitrogen leaching range from 1 to 57 kg/ha/year. Leaching was lowest at the infertile sites, but increased with magnitude of deposition and aphid infestations. Proton production according to the nitrogen transformations was largest at the fertile site most often affected by infestations. Huge amounts of bird droppings, honey dew and input of easily available nutrients by canopy leaching probably induced litter decomposition and formation of NO 3 − in the soil water.
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    URL: http://dx.doi.org/10.1007/BF00477140
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    Elevational trends in the fluxes of sulphur and nitrogen in throughfall in the Southern Appalachian Mountains: Some surprising results (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2265-2270 
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    ISSN: 1573-2932
    Keywords: atmospheric deposition ; high elevation forests ; foliar uptake ; cloudwater ; nitrogen ; sulphur
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract From 1986–1989, a team of scientists measured atmospheric concentrations and fluxes in precipitation and throughfall, and modeled dry and cloudwater deposition in a spruce-fir forest of the Great Smoky Mountains National Park which is located in the Southern Appalachian Region of the United States. The work was part of the Integrated Forest Study (IFS) conducted at 12 forests in N. America and Europe. The spruce-fir forest at 1740 m consistently received the highest total deposition rates (∼2200, 1200, and 700 eq ha−1 yr−1 for SO4 2−, NO3 −, and NH4 +). During the summers of 1989 and 1990 we used multiple samplers to measure hydrologie, SO4 2−, and NO3 − fluxes in rain and throughfall events beneath spruce forests above (1940 m) and below (1720 m) cloud base. Throughfall was used to estimate total deposition using relationships determined during the IFS. Although the SO4 2− fluxes increased with elevation by a factor of ∼2 due to higher cloudwater interception at 1940 m, the NO3 − fluxes decreased with elevation by ∼30%. To investigate further, we began year round measurements of fluxes of all major ions in throughfall below spruce-fir forests at 1740 m and at 1920 m in 1993–1994. The fluxes of most ions showed a 10–50% increase with elevation due to the ∼70 cm yr−1 cloudwater input at 1920 m. However, total inorganic nitrogen exhibited a 40% lower flux in throughfall at 1920 m than at 1740 m suggesting either higher dry deposition to trees at 1740 m or much higher canopy uptake of nitrogen by trees at 1920 m. Differential canopy absorption of N by trees at different elevations would have significant consequences for the use of throughfall N fluxes to estimate deposition. We used artificial trees to understand the foliar interactions of N.
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    URL: http://dx.doi.org/10.1007/BF01186171
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    Sulphur and nitrogen input to the Ratanica forested catchment (Carpathian Foothills, southern Poland) (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1765-1770 
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    ISSN: 1573-2932
    Keywords: nitrogen ; sulphur ; input ; forested catchment
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The study covers 1991–1994 concentrations of SO2 and NO2 in the air, concentrations of sulphur and nitrogen in bulk precipitation, throughfall and stemflow as well as input of S and N to the Ratanica forested catchment (S. Poland), which is exposed to moderate anthropogenic pollution are presented. There was high input of sulphur (26 kg ha−1) and nitrogen (24 kg ha−1) to the catchment, mainly in NH4+ (18 kg ha−1). The significant contribution of NH4 + connected with intensive agriculture in surrounding fields has led to eutrophication of the ecosystem.
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    URL: http://dx.doi.org/10.1007/BF00477235
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    Can forest-soil liming mitigate acidification of surface waters in Sweden? (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1855-1860 
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    ISSN: 1573-2932
    Keywords: Acidification ; acid deposition ; liming ; forest soil ; surface waters ; aluminum ; alkalinity ; Sweden
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Acidification of surface waters and forest soils is severe in large parts of southern Sweden. The shallow groundwaters are also affected. Large scale liming of surface waters and streams is in operation, often combined with wetland liming to limit the effects of acid episodes, e.g. at snow melt. Acid episodes are perhaps the most severe problem in limed surface waters and in many as yet well buffered waters, because of temperature-layered acid inflow, often superficial. As a result of some investigations, a large scale forest liming programme covering 6.500–10.000 km2 was recently suggested. The main objectives of this forest liming programme are to retard cation depletion and to prevent nutrient imbalance and forest decline in acidified areas. This paper deals with the effects of forest soil liming on streams and surface waters. The response of water chemistry is very dependent on hydrological and soil properties. Although pH itself may be little affected by liming, the acidity (or negative ANC) decreases, inorganic Al-species decrease and the Al/BC-ratio increases in the runoff water. Especially interesting is that this is also true during acid episodes. This means that toxicity for acid sensitive biota decreases. These results indicate that large scale liming may have beneficial effects on surface water chemistry. Furthermore, as surface waters are expected to respond to smaller decreases in acid deposition than do forests soils, forest soil liming may allow less frequent liming of lakes. Consequently, forest soil liming in combination with the anticipated emission reductions may have very beneficial results on surface waters in certain areas of Sweden.
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    URL: http://dx.doi.org/10.1007/BF00477250
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    Biogeochemistry of a forested watershed in the central Adirondack Mountains: Temporal changes and mass balances (1996)
    Springer
    Water, air & soil pollution 88 (1996), S. 355-369 
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    ISSN: 1573-2932
    Keywords: atmospheric deposition ; ecosystem ; hydrology ; nitrogen ; sulfur
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Information on atmospheric inputs, water chemistry and hydrology were combined to evaluate elemental mass balances and assess temporal changes in elemental transport from 1983 through 1992 for the Arbutus Lake watershed. This watershed is located within a northern hardwood ecosystem at the Huntington Forest within the central Adirondack Mountains of New York (USA). Changes in water chemistry, including increasing NO3 − concentrations (1.1 μmol c , L−1 yr-1), have been detected during this study period. Starting in 1991 hydrological flow has been measured from Arbutus Lake and these measurements were compared with predicted flow using the BROOK2 hydrological simulation model. The model adequately (r2=0.79) simulated flow from this catchment and was used to estimate drainage for earlier periods when direct hydrological measurements were not available. Modeled drainage water losses coupled with estimates of wet and dry atmospheric deposition were used to calculate solute budgets. Export of SO4 2− (831 mol c ha−1 yr−1) from the greater Arbutus Lake watershed exceeded estimates of atmospheric deposition in an adjacent hardwood stand suggesting an additional source of S. These large drainage losses of SO4 2− also contributed to the drainage fluxes of basic cations (Ca2+, Mg2+, K+ and Na+). Most of the atmospheric inputs of inorganic N were retained (average of 74% of wet precipitation and 85% total deposition) in the watershed. There were differences among years (56 to 228 mol ha−1 yr−1) in drainage water losses of N with greatest losses occurring during a warm, wet period (1989–1991).
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    URL: http://dx.doi.org/10.1007/BF00294111
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    The acid buffer capacity of some finnish forest soils: Results of acid addition laboratory experiments (1996)
    Springer
    Water, air & soil pollution 89 (1996), S. 147-157 
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    ISSN: 1573-2932
    Keywords: Neutralization ; acid deposition ; organic matter ; cation exchange
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Batch acid addition experiments were carried out to determine the acid buffer capacities (amount of acid required to lower soil pH by one unit) of forest soils. Samples of O, E, B (or BC), and C horizons taken from 29 podzolic profiles in southern Finland were used in the experiments. Subsamples of soil were equilibrated for 24 h with NaCl solution containing additions of HCl acid. Cation exchange, mineral dissolution (weathering), and the protonation of organic matter all appeared to have been involved in the buffering of the acid additions. For the O horizon samples, most of the cations released in response to the acid additions were base cations. For the mineral soil samples, most of the cations released were Al3+ ions. With the exception of a few samples, the added acid was not fully neutralised and pH was lowered even with the lowest addition treatment. However, the acid addition treatments corresponded to many times the regional annual acid deposition load (1.6–2.0 cmol(c) m−2). Calculated acid buffer capacities (cmol(c) kg−1 pH−1) ranged from 9.8 to 40.8 for O horizon soil samples and from 0.1 (C horizon) to 5.2 (E horizon) for the mineral soil samples. Total acid buffer capacities for a profile (to a depth of 50 cm) ranged from 500 to 2349, with a mean value of 1091 cmol(c) m−2 pH−1. It is concluded that, in addition to CEC and base saturation, acid buffer capacity is a useful measure to describe the ecological effects of acid deposition on soil.
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    URL: http://dx.doi.org/10.1007/BF00300427
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    Chemical characteristics of leachate from pulp and paper mill residuals used to reclaim a sandy soil (1996)
    Springer
    Water, air & soil pollution 89 (1996), S. 167-187 
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    ISSN: 1573-2932
    Keywords: Pulp and paper mill sludge ; nitrogen ; DOC ; heavy metals ; water quality
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Primary sludge, secondary sludge, and wood ash from a pulp and paper mill were combined with sand to create a synthetic topsoil (C:N ratio of 18:1) to restore an abandoned gravel pit. Synthetic topsoil was applied to field microcosms at rates equivalent to 0, 2170, 4341, or 6511 kg N/ha; each was seeded with grass. Fifteen chemical constituents in leachate were measured during two field seasons. Cadmium, Ni and Zn were mobilized rapidly by soil disturbance. Chloride and SO4-S eluted rapidly from the sludge along with Na. Nitrate leached with Ca late in each field season when sludge N-mineralization and nitrification exceeded plant uptake and microbial immobilization. Ammonium elution was negligible. Dissolved organic carbon (DOC) was mobilized by decomposition of organic matter in the sludge, as were Mg and K. Copper eluted with DOC, probably as an organic ligand. Lead and ortho-P were below our detection limits. We concluded that a synthetic topsoil with a 30:1 C:N ratio applied at a rate of 2100-4300 kg N/ha should provide adequate plant nutrition while minimizing water quality hazards.
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    Mercury concentrations in forest trees from Slovakia (1996)
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    Water, air & soil pollution 89 (1996), S. 267-275 
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    ISSN: 1573-2932
    Keywords: mercury ; forest trees ; biomonitors ; contaminants
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The concentration of mercury has been determined in assimilation organs of forest trees from 10 main industrial regions of Slovakia, four mountain forests and one military area and compared with concentration of mercury from 1356 permanent monitoring plots of Slovakia. The mercury concentration ranges for 2 yr old needles of Picea abies Karst. were (in mg kg−1): 1.249–4.402 (Rudnany iron ore mines), 0.013–0.749 (nine other industrial regions), 0.021–0.737 (four mountain forests) and 0.053–0.538 (military area). The mercury content in the soil (0–5 cm) from a mercury smelting plant ranged from 9.9 to 130 mg kg−1, and the moss Pleurozium schreberi contained 3.8–9.1 mg kg−1. The values obtained were compared with the available literature data.
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    MODELLING LEACHING OF INORGANIC Hg(II) IN A SCANDINAVIAN IRON-HUMUS PODZOL - VALIDATION AND LONG-TERM LEACHING UNDER VARIOUS DEPOSITION RATES (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 301-320 
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    ISSN: 1573-2932
    Keywords: acid rain ; batch experiment ; Freundlich isotherm ; lysimeter experiment ; mercury ; simulation model
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Increasing mercury contents are reported from freshwater systems and fish in northern Europe and North America. Mercury input from soils is a major source with the leaching being affected by increased atmospheric mercury deposition compared to pre-industrial times and by other environmental conditions such as acid rain. The results of a mathematical model-calculation of vertical inorganic Hg(II) leaching in a Scandinavian iron-humus podzol under different atmospheric input rates of mercury are presented. Leaching under background rain conditions was calculated to be considerably stronger than under acid rain conditions. Increasing fractions of deposited soluble or solute atmospheric mercury were leached from the O f(h)-horizon with decreasing soil content of soluble mercury under acid rain conditions; this effect was less pronounced under background rain conditions. The steady state concentrations of soluble mercury of the upper soil horizons were calculated and compared with the actual concentrations of total (= soluble + insoluble mercury) and extractable (= estimate of soluble) mercury measured in these horizons. The results indicate that even if the deposition of airborne mercury to soil is strongly reduced, the total mercury content of the soil decreases only slowly. It may take decades or even centuries before a new steady state concentration of total mercury is established in the soil. The decrease of the mercury concentration in the O f(h)-horizon is probably largely dependent on the turnover of organic matter, binding most of the deposited airborne mercury in an insoluble form. Hence, present day mercury leaching is likely to be dominated by mercury deposited during former times and temporarily retained in an insoluble form in the organic matter.
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    URL: http://dx.doi.org/10.1023/A:1026476921969
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    The role of humic substances in the aqueous mobilization of mercury from contaminated floodplain soils (1996)
    Springer
    Water, air & soil pollution 90 (1996), S. 507-520 
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    ISSN: 1573-2932
    Keywords: mercury ; foodplains ; humic substances ; complexation ; speciation ; mobilization ; risk assessment ; water solubility
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The water-mobilizability of mercury from contaminated floodplain soils of the river Elbe in Northern Germany was evaluated by batch extraction experiments. It was shown that only a small amount of the total mercury present (about 1% per extraction) can be mobilized by water. This mercury is transported entirely in the form of a complex bound to humic acids (HA); particulates and fulvic acids (FA) did not seem to contribute to the process. It could not be removed from the HA even at pH 1, indicating an extremely strong complexation e.g. by sulfur-containing ligands. Furthermore, the influence of pH on the mobilization was investigated. It was found that in the range of natural pH-values, there was no observable effect of pH on the mobilization of either mercury or dissolved organic carbon (DOC). This surprising finding is explained by an unexpectedly high buffering capacity of the humics, both in the acidic and in the alkaline region. Only at extreme pH-values there was deviation from this behaviour. In contrast to other heavy metals, the amount of mobilized mercury decreases at pH 〈 3; and at pH 〉 12, an increased mobilization of mercury was observed because the humics are mobilized completely, accompanied by the total amount of mercury bound to them.
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    Global mercury pollution and the role of gold mining: An overview (1997)
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    Water, air & soil pollution 97 (1997), S. 205-207 
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    ISSN: 1573-2932
    Keywords: mercury ; gold mining ; ecosystems ; methyl-Hg ; cycling ; global sources
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract As described by Jemelov and Ramel (1995), the Scientific Committee on Problems of the Environment (SCOPE) sponsored an investigation of Hg in ecosystems with special emphasis on tropical regions. In these regions small-scale gold mining activities have occupied about 10 million people worldwide who use Hg for extracting gold.
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    Determination of atmospheric mercury during the North sea experiment (1997)
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    Water, air & soil pollution 97 (1997), S. 257-263 
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    ISSN: 1573-2932
    Keywords: mercury ; atmosphere ; rainwater ; marine
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Total gaseous mercury (TGM) and rainwater were collected on board of two research vessels (F. S. ALKOR and R.V. BELGICA) positioned 200 km apart in the center of the North Sea during the North Sea Experiment, September 1991. On the F. S. ALKOR (up-wind ship) TGM concentrations ranged from 0.7 to 2.6 ng·m−3 with an average of 1.5 ng m−3 and on the R. V. BELGICA (down-wind ship) TGM ranged from 0.7 to 1.9 ng·m−3 with an average of 1.2 ng·m−3. An average 20% decrease is observed from the up-wind to the down wind ship. which may largely be affected by entrainment into the free troposphere. An overall removal (entrainment) velocity of 0.95 cm·s−1 was calculated for the whole experiment. The average removal velocity was 0.5 cm·s−1 for dry periods and varied between 1 to 5 cm·s−1 during rain events. Rainwater concentrations varied between 5 and 25 ng·1−1. Based on these data an annual wet deposition flux of 1.08 ng Hg cm−2 yr1− was estimated for the North Sea.
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    Sediment Accumulation of Nutrients (N, P) in the Eastern Gulf of Finland (Baltic Sea) (1997)
    Springer
    Water, air & soil pollution 99 (1997), S. 477-486 
    Details
    ISSN: 1573-2932
    Keywords: sediment ; nitrogen ; phosphorus ; organic matter ; cluster analysis ; Gulf of Finland ; estuaries
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Dry weight (DW), ignition loss (IL) and concentrations of total nitrogen (TN) and total phosphorus (TP) of the sediment surface layer (0 to 10 cm, 1 cm slices) were analyzed from 20 sites in the eastern Gulf of Finland. The distance of the sampling sites from the mouth of the River Neva explained the nutrient concentrations of the sediments well, while the effect of water depth was negligible. The increase of TN and the decrease of TP along the transect from the river mouth towards the open Gulf were caused by the diminishing share of allochthonous material supplied from the River Neva. The mean TN concentration of the different accumulation areas was about 40 % higher in the sediment surface than in the deeper layer (9 to 10 cm). The corresponding difference for TP varied from 53 to 56 %. The results suggest considerable netflux of nutrients from sediment to water. The net sediment accumulation of nutrients were estimated as 6.0 g m-2 a-1 of N and 1.7 g m-2 a-1 of P corresponding 22 000 t a-1 of N and 6 100 t a-1 of P for the whole eastern Gulf.
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    TOTAL MERCURY AND METHYLMERCURY IN SEDIMENTS AND IN THE POLYCHAETE NEREIS DIVERSICOLOR AT GROOT BUITENSCHOOR (SCHELDT ESTUARY, BELGIUM) (1997)
    Springer
    Water, air & soil pollution 94 (1997), S. 109-123 
    Details
    ISSN: 1573-2932
    Keywords: mercury ; methylmercury ; sediment ; polychaete ; Nereis diversicolor ; methylation ; bioaccumulation ; Scheldt estuary
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Total mercury (Hg) and methylmercury (MeHg) concentrations were determined in sediments and in the polychaete worm Nereis diversicolor at 13 stations of a brackish water intertidal mudflat of the Scheldt estuary. Hg and MeHg concentrations in sediments ranged from 144 to 1192 ng g−1 dw and from 0.8 to 6 ng g−1 dw, respectively. Both Hg and MeHg concentrations increased with an increase of organic matter (OM) content and fine grain fraction. In contrast, Hg accumulation by N. diversicolor was significantly (p 〈 0.05) higher at stations with sandy sediments (mean value: 125 ng g−1 dw) than at stations with muddy sediments (mean value, 80 ng g−1), probably because Hg availability for bioaccumulation at muddy stations was reduced by high OM content of the muddy sediments. MeHg accounted for an average of 0.7% of the total Hg in sediments and 18% of the total Hg in N. diversicolor. Seasonal variations significantly affected Hg concentrations in sediments and MeHg in N. diversicolor. Total Hg concentrations in sediments were significantly (p 〈 0.05) higher in autumn and winter than in spring and summer whereas MeHg concentrations were lowest in winter compared to the other seasons. On the other hand, total Hg concentrations in the worms were lowest in spring whereas MeHg concentrations were significantly (p 〈 0.01) higher in spring and summer than in autumn and winter.
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    URL: http://dx.doi.org/10.1023/A:1026434629599
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    WHOLE-CATCHMENT LIMING AT TJØNNSTROND, NORWAY: AN 11-YEAR RECORD (1997)
    Springer
    Water, air & soil pollution 94 (1997), S. 163-180 
    Details
    ISSN: 1573-2932
    Keywords: acid deposition ; liming ; catchment ; lake ; water chemistry ; fish ; soil ; model
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In June 1983 a whole-catchment liming experiment was conducted at Tjønnstrond, southernmost Norway, to test the utility of terrestrial liming as a technique to restore fish populations in remote lakes with short water-retention times. Tjønnstrond consists of 2 small ponds of 3.0 and 1.5 ha in area which drain a 25-ha catchment. The area is located at about 650–700 meters above sea-level in sparse and unproductive forests of spruce, pine and birch with abundant peatlands. A dose of 3 ton/ha of powdered limestone were spread by helicopter to the terrestrial area. No limestone was added to the ponds themselves. The ponds were subsequently stocked with brown and brook trout. Liming caused large and immediate changes in surface water chemistry; pH increased from 4.5 to 7.0, Ca increased from 40 to 200 μeq/L, ANC increased from –30 to +70 μeq/L, and reactive-Al decreased from about 10 to 3 μmol/L. During the subsequent 11 years the chemical composition of runoff has decreased gradually back towards the acidic pre-treatment situation. The major trends in concentrations of runoff Ca, ANC, pH, Al and NO3 in runoff are all well simulated by the acidification model MAGIC. Neither the measured data nor the MAGIC simulations indicate significant changes in any other major ion as a result of liming. The soils at Tjønnstrond in 1992 contained significantly higher amounts of exchangeable Ca relative to those at the untreated reference catchment Storgama. In 1992 about 75% of the added Ca remains in the soil as exchangeable Ca, 15% has been lost in runoff, and 10% is unaccounted for. The whole-catchment liming experiment at Tjønnstrond clearly demonstrates that this liming technique produces a long-term stable and favourable water quality for fish. Brown trout in both ponds in 1994 have good condition factors, which indicate that the fish are not stressed by marginal water quality due to re-acidification. The water quality is still adequate after 11 years and 〉20 water renewals. Concentrations of H+ and inorganic Al have gradually increased and approach levels toxic to trout, but the toxicity of these are offset by the continued elevated Ca concentrations. Reduced sulphate deposition during the last 4 years (1990–94) has also helped to slow and even reverse the rate of reacidification. The experiment at Tjønnstrond demonstrates that for this type of upland, remote terrain typical of large areas of southern Norway, terrestrial liming offers a suitable mitigation technique for treating acidified surface waters with short retention times.
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    Comparison of two reagents, sodium pyrophosphate and sodium hydroxide, in the extraction of labile metal organic complexes (1997)
    Springer
    Water, air & soil pollution 99 (1997), S. 217-223 
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    ISSN: 1573-2932
    Keywords: selective leach ; organic ; humic ; fulvic ; analysis ; mercury ; zinc
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The international reference lake sediment, LKSD-4, was used to compare Hg, organic C and Zn extracted from its ‘soluble organic’ phase by two commonly used reagents: 0.1 M Na4P2O7 solution at pH 10 and 0.5 M NaOH solution at pH 12. While recoveries of Hg and Zn by 0.1 M Na4P2O7 are not affected by changes in sample weight to reagent volume ratio (W/V) or contact time, those by NaOH show a marked dependency. In general, the NaOH leach extracts more organic C and Hg from LKSD-4 but less Zn. Over the range of conditions studied, the NaOH-based method extracted 4.7–9.8% C, 27–103 ng g−1 Hg and 19–69 μg g−1 Zn from LKSD-4, compared to 2.3–2.8% C, 17–24 ng g−1 Hg and 64–72 μg g−1 Zn by the Na4P2O7 leach. Clearly, different groups of organic substances are being dissolved by these two reagents and therefore a comparison of data from different laboratories becomes meaningless. This paper suggests that more research is needed into the exactNature of metal-organic associations extracted by selective leaches and into associated artifacts of extraction such as readsorption phenomena.
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    Benthic fluxes of dissolved inorganic carbon, nutrients and oxygen in the Gulf of Trieste (Northern Adriatic) (1997)
    Springer
    Water, air & soil pollution 99 (1997), S. 305-314 
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    ISSN: 1573-2932
    Keywords: Adriatic Sea ; nutrients ; benthic fluxes ; carbon ; nitrogen ; silicon ; phosphorus ; budgets
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Benthic fluxes of dissolved inorganic N, Si and P nutrients, alkalinity, dissolved inorganic C (DIC), and O2 from sediments in the Gulf of Trieste (northern Adriatic, Italy) were measured monthly in the period September 1995 – August 1996 using in situ incubated light benthic chambers. The highest efluxes of DIC, NH4 +, PO4 3−, Si(OH)4, and NO3 − influxes encountered in late summer — early autumn were the consequence of degradation of benthic microalgae, and in autumn mostly of sedimented phytoplankton. High NO3 − efflux was observed in spring. Only NH4 + and Si(OH)4 fluxes were significantly correlated with temperature. This correlation suggests that the rate of downward input and the quality and quantity of sedimentary organic matter (autochthonous and allochthonous) were superimposed on the temperature fluctuations. High DIC, NH4 + and Si(OH)4 effluxes observed in July 1996 were due to the late spring — early summer degradation of sedimentary organic matter produced by benthic microalgae, while the autumn phytoplankton bloom was quickly reflected in enhanced benthic fluxes due to higher temperature. Significant correlations between NH4 +, PO4 3− and Si(OH)4 fluxes suggested their parallel regeneration and utilization at the sediment-water interface. The nutrient fluxes were linked to O2 consumption, suggesting that aerobic oxidation processes were important at the sediment-water interface in the Gulf. The N, P and Si nutrients released from sediment pore waters are probably utilized in benthic microalgal and bottom-water primary production. This indicates that pelagic and benthic communities in the central part of the Gulf of Trieste function relatively independently of each other.
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    Monitoring nitrogen pollution from sugarcane runoff using15N analysis (1997)
    Springer
    Water, air & soil pollution 98 (1997), S. 389-399 
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    ISSN: 1573-2932
    Keywords: fertilizer ; nitrogen ; pollution ; runoff ; stable isotopes ; sugarcane
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In many forested wetlands of Louisiana, surface water quality is being deteriorated by nutrient input from adjacent agricultural production area. This field study assesses the input of fertilizer N, applied to sugarcane fields, to forested wetlands. The potential use of natural abundance variations in15N/14N ratios for identification and tracing surface water N sources (NH 4 + - and NO 3 − -N) was evaluated. Runoff and surface water samples were collected from sugarcane fields and bordering forested wetlands (6 stations) over a 16 month period and analyzed for NH 4 + -N, NO 3 − -N, and associated NH 4 + -δ 15N and NO 3 − -δ 15N ratios. FertilizerN draining into adjacent forested wetland was estimated to be only a small fraction of the amount applied. Concentrations of NH 4 + - and NO 3 − -N in the collected water samples were low and ranged from 0.02 to 1.79 mg L−1. Isotopic analysis revealed NH 4 + -δ 15N and NO 3 − -δ 15N means were distinctive and may have the potential to be used as tracers of N contamination. The mean NH 4 + -δ 15N value was +18.6±7.1‰ and the NO 3 − -δ 15N mean was +8.3±3.1‰. Anomalously high NO 3 − -δ 15N values (〉30‰) were attributed to denitrification.
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    Mercury dynamics in young Common Tern (Sterna hirundo) chicks from a polluted environment (1993)
    Springer
    Ecotoxicology 2 (1993), S. 33-40 
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    ISSN: 1573-3017
    Keywords: mercury ; body distribution ; feather concentrations ; body burden ; tern chicks
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: We studied mercury concentrations and amounts in tissues of 19 starved young Common Tern chicks (median age 4 days) and in eggs from the same colony. Concentrations and burden were similar between eggs and newly hatched chicks. Mercury concentrations were highest in down, which contained at least 38% of the body mercury. The mercury burden of the whole body and of the tissues as well as the concentration in down increased with age and body mass, indicating the importance of down as an elimination pathway. Conversion ratios between mercury concentrations in tissues and the whole chick body varied according to the contamination level.
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    Allozymes Reflect the Population-Level Effect of Mercury: Simulations of the Mosquitofish (Gambusia holbrooki Girard) GPI-2 Response (1998)
    Springer
    Ecotoxicology 7 (1998), S. 141-150 
    Details
    ISSN: 1573-3017
    Keywords: fish ; mercury ; natural selection ; allozyme ; population
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Measurements of the differential tolerance between enzyme genotypes and shifts in allozyme frequencies in populations from contaminated habitats have prompted the use of allozymes as markers of population-level toxicant effects. However, such studies often do not consider other factors that influence allele frequencies, including natural clines, migration, the intensity and specificity of selection and toxicant-induced genetic bottlenecks. In addition, selection components other than survival are not included. Consequently, the associated conclusions remain speculative. To assess this approach rigorously, a simulation study was conducted with the mosquitofish (Gambusia holbrooki) GPI-2 locus. Laboratory studies have shown the GPI-238/38 homozygote at this locus to be less tolerant than other genotypes during acute exposure to mercury. The GPI-2100/100 genotype has also been shown to have a reproductive disadvantage at lower mercury concentrations. Simple and then more complex models were used to quantify the relative effects of viability selection, random genetic drift and migration on the GPI-238 allele frequency. Simulations were also performed to assess the contribution of sexual and fecundity selection. A simple population model suggested that viability selection plays a greater role than does mortality-driven, genetic drift in the decrease of the sensitive allele under the conditions of this study. A more complex, stochastic model indicated that no significant mortality-driven drift was taking place in this system. In both models, migration mitigated the effect of selection. Sexual and fecundity selection had little effect on the allele frequencies in these simulations. We conclude that, provided the system under study is clearly understood, shifts in allele frequency can indicate the population-level effects of pollutants.
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    Sources, sinks, and fluxes of nutrients (N + P) in a small highly modified urban estuary in southern California (2000)
    Springer
    Urban ecosystems 4 (2000), S. 125-144 
    Details
    ISSN: 1573-1642
    Keywords: nitrogen ; phosphorus ; macroalgae ; estuary ; anthropogenic
    Source: Springer Online Journal Archives 1860-2000
    Topics: Architecture, Civil Engineering, Surveying , Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Our objective was to begin to investigate sources, sinks, and flux rates of nitrogen (N) and phosphorus (P) in Famosa Slough, a small (12 ha) highly modified urban estuary in San Diego, California, U.S.A. The hydrology of Famosa Slough has been modified by culverts that dampen tidal influence and seasonal runoff from two urban watersheds, each of which has been implicated as a nutrient source that generates nuisance algal blooms. In 1995 and 1996, the ranges of nutrients measured in the water column were extremely wide; upper values exceeded those in other estuaries identified as eutrophic. Average dissolved inorganic nitrogen ranged from 2 to 250 μM, while dissolved inorganic phosphorus ranged from 〈1 to 15 μM. Nutrient content of the water changed rapidly both spatially and temporally depending on the tides and rainfall. While tidal water dominated this system, especially in the dry season, our results indicate that Famosa Slough's small watershed, not the larger watershed of the San Diego River, was the major source of nutrients during rainfall. Sediment nutrients were also high (∼3 mg N g dry wt−1 and 0.600 mg P g dry wt−1). Short-term flux studies suggest that the large accumulations of opportunistic green macroalgae commonly found in this estuary, and possibly the sediments, may act as a large and rapid sink for nutrients during times of high nutrient supply. We suggest that small, shallow estuaries in urban settings may have more complex and rapid nutrient dynamics than those found in larger systems.
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    Seasonal and spatial patterns of S, Ca, and N dynamics of a Northern Hardwood forest ecosystem (1992)
    Springer
    Biodegradation 17 (1992), S. 165-189 
    Details
    ISSN: 1572-9729
    Keywords: calcium ; fine roots ; nitrogen ; northern hardwood ; nutrient dynamics ; seasonality ; soils ; sulfur ; vegetation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract Seasonal dynamics of S, Ca and N were examined at the Huntington Forest, a northern hardwood ecosystem in the central Adirondacks of New York for a period of 34 months (1985–1988). Solute concentrations and fluxes in bulk precipitation, throughfall (TF) and leachates from the forest floor, E horizon and B horizon were quantified. Both above and below-ground elemental fluxes mediated by vegetation (e.g. uptake, litter inputs, and fine roots production) were also determined. The roles of abiotic and biotic processes were ascertained based on both changes in solute concentrations through the strata of the ecosystem as well as differences between dormant and growing seasons. Concentrations of SO4 2−, NO3 −, NH4 + and Ca2+ were greater in TF than precipitation. Forest floor leachates had greater concentrations of SO4 2−, NO3 − + NH4 + and Ca2+ (9, 6 and 77 µeq L−1, respectively) than TF. There were differences in concentrations of ions in leachates from the forest floor between the dormant and growing seasons presumably due to vegetation uptake and microbial immobilization. Concentrations and fluxes of NO3 − and NH; were greatest in early spring followed by a rapid decline which coincided with a demand for N by vegetation in late spring. Vegetation uptake (44.7 kg N ha−1 yr−1 ) could account for the low leaching rates of N03 −. Within the mineral soil, changes with soil depth and the absence of seasonal patterns suggest that cation exchange (Ca+) or anion sorption (SO4 2−) are primarily responsible for regulating solute concentrations. The increase in SO4 2− concentration after leachates passed through the mineral soil may be attributed to desorption of sulfate that was adsorbed during an earlier period when SO4 2− concentrations would have been greater due to elevated S inputs.
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    Nitrogen mass balances and denitrification rates in central Ontario Lakes (1993)
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    Biodegradation 20 (1993), S. 195-212 
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    ISSN: 1572-9729
    Keywords: denitrification ; lake ; mass balance ; nitrogen
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract Nitrogen mass balances for seven unproductive lakes and 20 forested catchments in central Ontario were measured between 1977 and 1989. Average annual lake denitrification rates calculated with the N/P ratio method were strongly correlated with summer anoxic factor (extent of surficial sediment anoxia) whereas denitrification rates calculated with a210Pb sediment N accumulation method were poorly correlated with the anoxic factor suggesting that the N/P method is superior. Substantial denitrification occurred in all lakes — an average of 36% of TN inputs or 75% of the net gain. On a regional area-weighted basis, 67% of bulk atmospheric TN deposition was stored or denitrified terrestrially, 12% was denitrified in lakes, 4% was stored in lake sediments, and 17% was exported from lakes. N/P ratios were generally less in streams than in precipitation suggesting preferential N retention in catchments, whereas the N/P ratios in lake outputs were slightly higher than lake input ratios, suggesting preferential P retention in lakes. This is consistent with the notion that P-limited lakes can exist adjacent to N-limited forests.
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    Effect of nitrogen and phosphorus addition on phenanthrene biodegradation in four soils (1999)
    Springer
    Biodegradation 10 (1999), S. 43-50 
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    ISSN: 1572-9729
    Keywords: biodegradation ; nitrogen ; nutrients ; phenanthrene ; phosphorus
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract Phenanthrene mineralization rates were found to vary widely among four soils; differences in soil nutrient levels was one hypothesis to explain this variation. To test this hypothesis, phenanthrene mineralization rates were measured in these soils with, and without, added nitrogen and phosphorus. Mineralization rates either remained unchanged or were depressed by the addition of nitrogen and phosphorus. Phenanthrene degradation rates remained unchanged in the soil which had the highest indigenous levels of nitrogen and phosphorus and which showed the largest increase in phosphorus levels after nutrients were added. The soils in which degradation rates were depressed had lower initial phosphorus concentrations and showed much smaller or no measurable increase in phosphorus levels after nutrients were added to the soils. To understand the response of phenanthrene degradation rates to added nitrogen and phosphorus, it may be necessary to consider the bioavailability of added nutrients and nutrient induced changes in microbial metabolism and ecology.
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    Nitrogen inputs to a marine embayment: the importance of groundwater (1990)
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    Biodegradation 10 (1990), S. 309-328 
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    ISSN: 1572-9729
    Keywords: estuaries ; groundwater ; nitrogen ; nitrogen cycle ; nitrogen loading
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
    Notes: Abstract We examined the importance of nitrogen inputs from groundwater and runoff in a small coastal marine cove on Cape Cod, MA, USA. We evaluated groundwater inputs by three different methods: a water budget, assuming discharge equals recharge; direct measurements of discharge using bell jars; and a budget of water and salt at the mouth of the Cove over several tidal cycles. The lowest estimates were obtained by using a water budget and the highest estimates were obtained using a budget of water and salt at the Cove mouth. Overall there was more than a five fold difference in the freshwater inputs calculated by using these methods. Nitrogen in groundwater appears to be largely derived from on site septic systems. Average nitrate concentrations were highest in the region where building density was greatest. Nitrate in groundwater appeared to behave conservatively in sandy sediments where groundwater flow rates were high (〉 11/m2/h), indicating that denitrification was not substantially reducing external nitrogen loading to the Cove. Nitrogen inputs from groundwater were approximately 300 mmol-N/m3/y of Cove water. Road runoff contributed an additional 60 mmol/m3/y. Total nitrogen inputs from groundwater and road runoff to this cove were similar in magnitude to river dominated estuaries in urbanized areas in the United States.
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    The anthropic catchment-ecosystem concept: An Irish example (1985)
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    Human ecology 13 (1985), S. 209-240 
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    ISSN: 1572-9915
    Keywords: catchment-ecosystem ; nutrient-budget ; anthropogenic inputs ; nitrogen ; phosphorus ; eutrophication ; agricultural policies
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology , Energy, Environment Protection, Nuclear Power Engineering , Ethnic Sciences
    Notes: Abstract The catchment-ecosystem concept is adapted to investigate the nutrient-budget of the highly-modified Colebrooke drainage basin in Northern Ireland. Anthropogenic inputs, mainly manures and fertilizers, account for 86% of the nitrogen and 96% of the phosphorus added to the catchment. These inputs greatly exceed the streamflow outputs, thereby indicating that the flow of nutrients is dominated by agriculture. This is explained by the transformation of traditional mixed farming into more intensive livestock production and is linked to policies encouraging increased agricultural production, amalgamation of farms, afforestation, rural depopulation, and urbanization. Substantial increases in the Nand Poutput of the catchment and further eutrophication of the recipient lake, Lough Erne, are predicted without the implementation of policies to reduce agricultural nutrient losses.
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    Long term effects of enhanced nitrogen deposition on a lowland dry heath in southern Britain (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1701-1706 
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    ISSN: 1573-2932
    Keywords: nitrogen ; heathland ; Calluna vulgaris ; critical load ; growth ; litter production
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Experimental additions of ammonium sulphate to a nitrogen-poor dry heathland have been carried out since 1989. There are four nitrogen treatments: a control (receiving artificial rain only), a low treatment which receives an additional 7.7 kg N ha−1 yr−1, a high treatment receiving 15.4 kg N ha−1 yr−1 and an alternating treatment which receives either the control or the high nitrogen additions, in alternate years. The estimated background deposition at the study site is 13–18 kg N ha−1 yr−1, a value similar to the critical load that has been suggested for the conversion of lowland heath to grassland. Over the past 5 years there have been significant stimulations in shoot growth, flowering, canopy density and litter production. Flowering, in particular, strongly reflects nitrogen additions in the alternating treatment. Current models of the response of dry Calluna heathlaud to enhanced nitrogen deposition suggest that higher tissue nitrogen levels will occur and will be accompanied by heightened sensitivity to secondary stresses. This may in turn lead to canopy breakdown and replacement by grassland. The application of nitrogen at deposition rates only slightly in excess of the critical load over five years has produced small, non-significant increases in shoot nitrogen content. However, there is clear evidence of a large positive effect on shoot growth, flowering, litter production and canopy density of Calluna. The observation of these responses at the application rates used in this study supports the current proposals for critical loads of nitrogen for lowland heaths.
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    Reducing the contribution of ammonia to nitrogen deposition across Europe (1995)
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    Water, air & soil pollution 85 (1995), S. 1891-1896 
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    ISSN: 1573-2932
    Keywords: emissions ; nitrogen ; ammonia ; agriculture ; integrated assessment modelling ; abatement strategies
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract European emissions of reduced nitrogen, arising principally from agriculture, are comparable with those of oxidised nitrogen from mobile and stationary combustion sources. It is therefore important to include ammonia emissions in working towards a new protocol on nitrogen under the programme of the UN Economic Commission for Europe on the control of transboundary air pollution. However the nature of the sources and the subsequent atmospheric transport and chemistry are very different from other acidifying pollutants. This paper describes work in hand under the MARACCAS project to compare agricultural activities in different European countries and to assess the applicability and efficacy of potential abatement measures. The aim is to derive abatement costs for each country relating successive emission reductions to the costs of achieving them, to be used by the UN ECE Task Force on Integrated Assessment Modelling (TFIAM) — in particular with our Abatement Strategies Assessment Model, ASAM. The paper will also address the large uncertainties involved in integrated assessment modelling with respect to ammonia, and suggest how these may be allowed for in deriving cost-effective abatement strategies.
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    Critical loads of acidity and nitrogen, based on multiple criteria for different swedish ecosystems (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2375-2380 
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    ISSN: 1573-2932
    Keywords: Critical load ; acidity ; nitrogen ; Norway spruce ; Scots pine ; ground vegetation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The critical loads of acidity and nitrogen has been mapped for Swedish forest soils, using data from the Swedish Forest Inventory. The Swedish critical load map used in negotiations has been based on a number of ecological receptors. For terrestrial ecosystems criteria based on no adverse effect on growth, soil stability and groundwater quality was used. For surface waters, stream and lake biology was used as indicators for setting limits to acidification. A reduction of 75% of the acidity deposition in relation to 1988 is required in order to protect 95% of the forest resource in Sweden from effects of soil acidification. A reduction of 50% of the nitrogen deposition is required to avoid exceedance in more than 5% of the area. The mapping work was carried out by using the PROFILE model.
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    The use of critical loads in emission reduction agreements in Europe (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2381-2388 
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    ISSN: 1573-2932
    Keywords: critical loads ; acid deposition ; emission reductions ; air pollution impacts ; ecosystem sensitivity
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Critical loads have been used in the revision of the Sulphur Protocol of the Convention on Long Range Transboundary Air Pollution (LRTAP) of the United Nations Economic Commission for Europe (UN/ECE). Critical loads, i.e. maximum allowable depositions which do not increase the probability of damage to forest soils and surface waters, have been computed and mapped for Europe by means of the Steady-state Mass Balance Method, using national data and, if national data were unavailable, using a European database. Results show that areas with low critical loads are located mostly in northern and central Europe. The reduction of the excess of sulfur (S) deposition over critical loads was a starting point for negotiations leading to the Oslo Protocol on Further Reduction of Sulphur Emissions (the “Second Sulphur Protocol”). The new protocol protects about 81%, 86% and 90% of the ecosystems' area in 2000, 2005 and 2010, respectively. In addition, the total European area in which sulphur deposition exceeds critical loads by more than 500 eq ha−1 yr−1 will be reduced from about 19% in 1980 to practically zero in 2010. Besides these results, a methodology is presented which allows the combined assessment of the acidifying effects of S and N as well as the eutrophying effects of N deposition on ecosystems (so-called critical load functions and the protection isolines derived from them). This methodology is well suited to integrate ecosystem sensitivities into future negotiations on the reductions of nitrogen (N) compounds, taking into account present or anticipated S emissions.
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    URL: http://dx.doi.org/10.1007/BF01186190
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    Calculation and mapping of critical loads of s, n and acidity on ecosystems of the Northern Asia (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2395-2400 
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    ISSN: 1573-2932
    Keywords: critical loads ; nitrogen ; sulphur ; northern Asia
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract On the basis of modified simple steady state mass-balance equations, the critical loads for nutrient and acidifying nitrogen as well as for sulphur and acidity have been calculated for various ecosystems of northern Asia using simplified expert-modelling GIS and grid cells 150×150 km. The minimal values of critical loads of nitrogen, CL(N), (〈50eq/ha/yr) were shown for arctic and subarctic ecosystems and the maximal ones (〉300eq/ha/yr) for ecosystems of chernozemic and chernozem-like soils in southern Siberia and the Far East. The minimal values of critical loads of sulphur, CL(S), as well as acidity were shown predominantly in the northern part of east Siberia and in the Kamchatka peninsula and the maximal ones for ecosystems having neutral and alcaline soils. The corresponding exceedances were indicated for many regions of the northern part of Asia with maximal values for regions of Ural mountains, frontery of Kazakhstan, Altai, lower Yenisei river flow, Far East, Sakhalin and South-Kurilean islands.
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    URL: http://dx.doi.org/10.1007/BF01186192
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    Assessment of critical loads in liuzhou, China using static and dynamic models (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2401-2406 
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    ISSN: 1573-2932
    Keywords: critical load ; acid deposition ; acidification model ; sulfur deposition
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The project Comprehensive Control and Demonstration for Acid Deposition in Liuzbou area is a national key project in the 8th Five-year-plan, and the study on critical loads will provide scientific and quantitative accordance for formulating control strategy. In this paper, critical loads of acid deposition to soil in Lirzhou area, China, were calculated using the Steady State Mass Balance method (SMB and PROFILE) and dynamic modeling methods(MAGIC), based on data obtained from field investigations and physiochemical properties measured through experiments such as the organic content, cation exchange capacity, base saturation, sulfate adsorption capacity, gibbsite coefficient, biomass base cation uptake and selectivity coefficient for cations. Weathering rates necessary to calculate soil chemistry in applying SMB and MAGIC model were determined by computation with PROFILE using independent geophysical properties such as soil texture and mineralogy as the input data, or by the total soil base cation content correlation. The results have shown that the critical loads of acidity in this area are in the range of 0.7–6.0 keq ha−1 yr−1, indicating sulfur deposition should be cut down by 50–90 percent of the present level. The upper soil layer is the most sensitive. The maximum allowable deposition loading of this area is also presented in the paper.
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    URL: http://dx.doi.org/10.1007/BF01186193
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    Critical loads mapping in Poland: Lessons learned (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2547-2552 
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    ISSN: 1573-2932
    Keywords: critical loads ; acid deposition ; forest soils ; mapping ; mathematical modelling
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Since 1990 the Institute for Ecology of Industrial Areas, acting as National Focal Center, is actively involved in an international research programme aimed at the calculation and mapping of critical loads of acidifying compounds. Following the methodological guidelines elaborated under the leadership of UN/ECE Task Force on Mapping and Coordination Center for Effects, national maps of critical loads and their exceedances for acidity, sulphur and nitrogen have been produced. These maps have already been utilized in derivation of European maps of critical loads of acidity and sulphur submitted to the UN/ECE LRTAP Convention as scientific input to the negotiations on the Second Sulphur Protocol. The lessons learned from the critical loads mapping exercise can be summarized as follow: the majority of Polish territory is covered with forest soils sensitive to acidification at an average Central European level; the exceedances of critical loads, estimated on the basis of national deposition data reveal the tune changes of ecological risks on the territory of Poland as a reflection of economic transition. The significant difference in the scale of those risks (measured by the percentage of the country territory with the maximum exceedances of critical loads) that appear in the period between 1987, representing the period of central planned economy and 1990, representing the early transition phase to a market economy, is particularly notable.
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    URL: http://dx.doi.org/10.1007/BF01186217
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    Uncertainty analysis of critical loads for terrestrial ecosystems in Russia (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2559-2564 
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    ISSN: 1573-2932
    Keywords: uncertainty analysis ; computed critical loads ; nitrogen ; sulpher ; acidity
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The goal of this study is to give a comprehensive and quantitative estimation of the uncertainty of computed in different scale nitrogen (N) and sulphur (S) critical loads (CL) values for terrestrial ecosystems of the Northern Asia, European part and the North-Western regions of Russia. The CL values are used to set goals for future deposition rates of acidifying compounds so that the environment is protected. In this research CL values for terrestrial ecosystems are determined using the expert-modelling geoinformation system (EM GIS) approach. UNCSAM software package is used as the tool for uncertainty analysis. The analysis presented here focuses on the estimation and effect of the input source uncertainties and sensitivities on the CL values in various regions under study. In spite of the region, nitrogen uptake by vegetation, nitrogen leaching from terrestrial ecosystems and the difference between deposition and uptake by plants of base cations (BC) are the most influential factors for all terrestrial ecosystems of Russia.
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    URL: http://dx.doi.org/10.1007/BF01186219
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    Deriving critical loads for Asia (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2565-2570 
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    ISSN: 1573-2932
    Keywords: acid deposition ; air pollution impacts ; critical loads ; integrated modeling ; ecosystem sensitivity
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Critical loads have been computed and mapped in Southeast Asia, comprising China, Korea, Japan, The Philippines, Indo-China, Indonesia and the Indian subcontinent. The methodology involved the Steady-State Mass Balance (SSMB) method, originally developed for Europe. In contrast to Europe, where critical loads were computed for forest soils and surface waters, in Asia critical loads for 31 different vegetation types have been computed. Critical chemical limits as well as soil stability criteria were derived for each of these vegetation types, which include both natural and managed ecosystems. Results show that low critical loads in Asia occur in Bangla-Desh, Indo-China, Indonesia and the southern part of China. Uncertainties of the results are mainly due to uncertainties in base cation deposition. The critical loads are part of the impact module of the Asian version of the Regional Air pollution INformation and Simulation model (RAINS-Asia), a model used to assess abatement strategies for sulfur emissions which are rapidly increasing in this part of the world. The difference in the level of detail between European and Asian critical load maps enables different applications. In Europe, critical loads for sulphur were used in comparison to actual sulphur deposition with the aim of decreasing the excess of sulphur deposition over critical loads through optimal emission abatement. In Asia in general and China in particular the geographical distribution of critical loads of sensitive ecosystems, with some emphasis on crops, is likely to be used as a basis for future emission (re-)allocation.
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    URL: http://dx.doi.org/10.1007/BF01186220
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    Testing, improvement, and confirmation of a watershed model of acid-base chemistry (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2607-2612 
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    ISSN: 1573-2932
    Keywords: acidification ; model testing ; modeling ; acid deposition
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Strategies to control the emission of atmospheric pollutants such as sulfur and nitrogen, are generally based in large part on projections using models that simulate the influence of sulfur and/or nitrogen deposition on the acid-base chemistry of surface waters. One of the principal models used throughout Europe and North America for such assessment is the Model of Acidification of Groundwater in Catchments (MAGIC). All watershed models are simplified representations of reality, and as such require careful testing to establish their veracity prior to use for making policy projections. This is particularly true where the use of these model projections has the potential for serious environmental or economic consequences. During the past five years, we have tested the MAGIC model in a large variety of settings and under quite varying environmental conditions. This work has included comparing model hindcast simulations with diatom-inferences of historical acidification, sensitivity analyses to examine the response of the model to alternative assumptions and formulations, and detailed testing of model forecasts by comparing simulated chemistry with the results of catchment-scale and plot-scale experimental acidification and deacidification. Our analyses have elucidated a number of potentially-important deficiencies in model structure and method of application. These have resulted in changes to the model and its calibration procedures. Our work has included in-depth evaluation of issues related to regional aggregation of soils data, background sulfur deposition, natural organic acidity, and aluminum mobilization. The result has been an improved and more thoroughly-tested version of MAGIC. The process we have followed to improve and confirm the MAGIC model has been iterative and time consuming. It required the availability of large volumes of data from experimental manipulation and paleolimnological studies. We believe that such model testing and confirmation efforts should be a critical prerequisite for regional or national assessment activities that are based largely on the results of environmental models.
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    URL: http://dx.doi.org/10.1007/BF01186227
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    Changing public interest in, and awareness of, acid deposition: Some evidence from the UK (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2631-2636 
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    ISSN: 1573-2932
    Keywords: Public awareness ; public information ; acid deposition
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract It is fundamental that the general public have access to usable environmental information on which they can base their decisions. Since 1984 the Atmospheric Research and Information Centre (ARIC) has operated a public information programme for the UK on the subject of acid deposition. The objective of the programme is to disseminate information on acid deposition without advocacy. ARIC provides enquirers with a broad range of authoritative and accurate facts and opinions from a wide range of parties from all sides of the debate. These sources include pressure groups, governmental bodies and industrialists from the UK and overseas. By deconstructing complex technical material and reassembling it for dissemination in a user friendly form, ARIC assists those receiving information to obtain a balanced perspective. This enables personal decision making within the context of the fullest information resource ARIC is able to provide.
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    URL: http://dx.doi.org/10.1007/BF01186231
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    Spatial variability in emissions reduction strategies for sulphur and nitrogen in the UK (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2619-2624 
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    ISSN: 1573-2932
    Keywords: sulphur ; nitrogen ; critical loads function ; emissions reductions
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The roles of sulphur (S) and nitrogen (N) in causing critical loads exceedance across the UK show considerable spatial variability at the present time. Over much of lowland Britain it appears that the environment can only be protected by reducing N deposition, whilst in upland areas (e.g. most of Scotland and Wales) reductions in S deposition are the primary requirement. Using the Hull Acid Rain Model (HARM) the effects of current and possible future emissions control legislation on critical loads exceedance can be explored. Based on HARM output, the implementation of the UNECE Sulphur Protocol (1994) will bring about a substantial reduction in the amount of S being deposited in the UK, especially in central and southern parts of the country. Some areas will remain where additional reductions in S are required. Over most of the country, however, the need to reduce N deposition will become paramount. The changing contributions and significance of non-UK sources can be estimated.
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    The United Kingdom national materials exposure programme (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2655-2660 
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    ISSN: 1573-2932
    Keywords: materials ; buildings ; stone ; metal ; pollution ; decay ; acid deposition
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In 1986, the National Materials Exposure Programme was set up within the United Kingdom to investigate the effects of acid deposition on buildings and building materials. Thirty sites were chosen, which represented a range of geographical and pollution climates. Each site met a minimum meteorological and pollution monitoring regime (including SO2, NO2). After four years, other sites were included (with less frequent data collection) and some sites removed. At each site, samples of 3 types of stone, mild steel, painted steel, Cu, Al and galvanised steel were exposed, with some of the stone sheltered from direct precipitation. Samples were removed periodically for analysis and dose-response relations derived for different materials. The empirical relationships derived are in the form of: decay rate=a [SO+] + b [H2] + c [rainfall] + d These dose response relations have been used to develop critical load maps for materials for the United Kingdom. Eight years of data have been collected, some for the UNECE task force programme. Laboratory tests using an Atmospheric Flow Chamber were also undertaken. Since the beginning of the programme addition materials have been exposed on some sites including mortars. A further set of eight sites has been used to assess the effects of ozone on a range of organic materials (for example polyvinyl chloride, polycarbonate, sealants). The paper presents up-to-date findings for the programme and confirms the dominance of dry deposition of sulphur dioxide as the main decay process for sensitive materials in areas of significant pollution.
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    URL: http://dx.doi.org/10.1007/BF01186235
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    Mapping of critical loads and levels for pollution damage to building materials in the United Kingdom (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2693-2699 
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    ISSN: 1573-2932
    Keywords: Critical loads ; Sulphur ; dose-response functions ; Damage functions ; acid deposition
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The United Kingdom National Materials Exposure Programme was initiated in 1986 to study the effects of acid deposition on building materials. The output data in the form of empirical dose-response equations (described elsewhere) have been incorporated into a geographical information system (GIS). In addition, data for the stock at risk of building materials has also been used. The dose-response relations indicate a dominance of dry deposition of sulphur dioxide in the decay process. Critical level/load maps have been determined for a number of materials. General pollution and meteorological data sets are also included in the mapping process. Maps give ‘exceedence squares’ on a 20 km square grid basis, indicating the unprotected areas or those still at risk for a given scenario for SO2 reduction in the context of the UNECE protocol for sulphur. In order to derive maps of areas sensitive to pollutants in the future a model, HARM 7.2, is used for the prediction of distribution of emissions of pollutants in the UK. A series of maps has now been produced for different materials at 70% and 80% scenarios for the reduction of SO2. Studies of the sensitivity of the exceedence maps to the accuracy or variation of the components in the dose-response equations have been undertaken. Results from the mapping programme and the sensitivity analysis are presented together with discussion of the concept of critical loads of materials.
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    URL: http://dx.doi.org/10.1007/BF01186241
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    Response of porous building stones to acid deposition (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2713-2718 
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    ISSN: 1573-2932
    Keywords: building stones ; porous carbonate stones ; acid deposition ; urban environment ; stone reactivity ; porosity ; petrophysics ; physical properties
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract This work investigates the response of porous carbonate building stones to acid deposition during a short-terra exposure period and the characteristics that influence their reactivity and/or durability. Several carbonate porous stones used in Spanish and English monuments were exposed to English urban and suburban environments. In each location they were both exposed to and sheltered from rainfall. Monthly analyses were carried out in order to investigate any possible sign of reaction. In addition, some physical properties of the stones relating to transfer of moisture were determined. Results indicate that the reactivity of these stones is relatively high, significant signs of reaction were detected within only a few months of exposure. Under the same environmental conditions, the response and reactivity of porous carbonate stones are determined by their petrophysical characteristics.
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    URL: http://dx.doi.org/10.1007/BF01186244
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    Effect of acid rain on sandstone: The Royal Palace and the Riddarholm church, Stockholm (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2719-2724 
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    ISSN: 1573-2932
    Keywords: Air pollution ; acid deposition ; sandstone deterioration ; gypsum formation ; sulphur isotopes
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The deterioration of two kinds of sandstone is discussed for two 18:th century buildings in central Stockholm: the Royal Palace, and the Royal Carolean Burial Chapel (Karolinska gravkoret) annexed to the mediaeval Riddarholm church. The facades of calcitic Gotland sandstone show many signs of serious decay, such as gypsum formation, pulverized surface, exfoliation, discolouration, and salt efflorescence. The socles are built of the more resistant quartzitic Roslagen sandstone, displaying some discolouration, cracks, and slight exfoliation. In total about 300 samples have been analysed. The surface concentration of sulphur is highest at ground level and at rain-sheltered positions. Chemical and sulphur isotope data indicate that the stone decay to a large part may be attributed to anthropogenic sources like acid deposition and car traffic.
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    Biogeochemistry of aluminum in a forest catchment in the Czech Republic impacted by atmospheric inputs of strong acids (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1831-1836 
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    ISSN: 1573-2932
    Keywords: acid deposition ; Al cycling ; forest soil ; jurbanite ; leucogranite ; soil solution ; stream water
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The Lysina catchment in the Czech Republic was studied to investigate the biogeochemical response of Al to high loadings of acidic deposition. The catchment supports Norway spruce plantations and is underlain by granite and podzolic soil. Atmospheric deposition to the site was characterized by high H+ and SO4 2− fluxes in throughfall. The volume-weighted average concentration of total Al (Alt) was 28 μmol L−1 in the O horizon soil solution. About 50% of Alt in the O horizon was in the form of potentially-toxic inorganic monomeric Al (Ali). In the E horizon, Alt increased to 71 μmol L−1, and Ali comprised 80% of Alt. The concentration of Alt (120 μmol L−1) and the fraction of Ali (85%) increased in the lower mineral soil due to increases in Ali and decreases in organic monomeric Al (Alo). Shallow ground water was less acidic and had lower Alt concentration (29 μmol L−1). The volume-weighted average concentration of Alt was extremely high in stream water (60 μmol L−1) with Ali accounting for about 60% of Alt. The major species of Ali in stream water were fluorocomplexes (Al-F) and aquo Al3+. Soil solutions in the root zone were undersaturated with respect to all Al-bearing mineral phases. However, stream water exhibited Ali concentrations close to solubility with jurbanite. Acidic waters and elevated Al concentrations reflected the limited supply of basic cations on the soil exchange complex and slow weathering, which was unable to neutralize atmospheric inputs of strong acids.
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    Increasing role of nitrogen in the acidification of surface waters in the Adirondack Mountains, New York (1997)
    Springer
    Water, air & soil pollution 95 (1997), S. 313-336 
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    ISSN: 1573-2932
    Keywords: nitrogen ; acidification ; Adirondack Mountains ; atmospheric deposition
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Assessments of the aquatic effects of acidic deposition have focused on sulfur, as have recent efforts to control the emissions of acidifying compounds. Nitrogen dynamics were excluded from most acidic deposition modeling studies because it was believed that terrestrial ecosystems strongly retain N and because modeling N is a more formidable task than modeling S due to the influence of complex biological processes on N cycling. Re-examination of available data for the Adirondack Mountains of New York suggests that N deposition may be contributing to both chronic and episodic acidification of freshwaters to a greater extent than is generally believed. Previous research concluded that N has played a limited role in acidification processes in these lakes, based on regional averages of chronic chemistry. However, it is now known that historic acidification responses have been spatially variable within the Adirondack Mountains and that the declines in lakewater pH have been less than previously believed. Lakewater NO3 − concentrations are commonly in the range of 5 to 25 μeq L−1 on a chronic basis in portions of the Adirondack region that have experienced significant chronic acidification. These NO3 − concentrations correspond in magnitude to inferred historical acidification. Furthermore, the relative importance of NO3 − as an agent of acidification increases dramatically during snowmelt when conditions are most toxic to fish. The consequence of not addressing N in formulating acidification recovery strategies for the Adirondacks includes the likelihood that we will overestimate the response of surface water to the mandated sulfur emissions reductions.
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    Effects of enhanced supplies of nitrogen and sulphur on rhizosphere and soil chemistry in a Norway spruce stand in SW Sweden (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 1777-1782 
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    ISSN: 1573-2932
    Keywords: aluminium ; base cations ; bulk soil ; nitrogen ; rhizosphere soil ; sulphur
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Rhizophere and bulk soil chemistry were investigated in a Norway spruce stand in SW Sweden. The rhizosphere and bulk soil chemistry in water extracts in control plots (C) and plots repeatedly treated with ammonium sulphate (NS) were compared. Treatment regime was started in 1988. Cylindrical core samples of the LFH-layer and mineral soil layers were collected in 1992 and used for water extract analyses. Samples of soil from LFH-layer and mineral soil layers were taken in 1991 and 1993 for determination of CEC and base saturation. Soil pH and NH4-N, NO3-N and SO4-S, Al, Ca, K and Mg concentrations in water extracts were measured for rhizosphere and bulk soils. The pH-values of bulk and rhizosphere soils in NS plots decreased compared with those in control plots, whereas concentrations of NH4-N, NO3-N, SO4-S, base cations and Al in water extract increased. In both bulk and rhizosphere soils the concentration of NH4-N was much higher than that of NO3-N. A significant difference in the pH and Mg concentration of bulk and rhizosphere soil between the treated and control plots was found only in the 0–10 cm layer. For all layers, there was a significant difference in NH4-N concentrations in the bulk and rhizosphere soil between the NS treatment and control plots. Concentrations of exchangeable base cations and the base saturation level in the LFH-layer decreased in the NS plots. The concentration of extractable SO4-S increased in the NS plots. The NS treatment enhanced the amount of litter in L-layer, owing to increases in needle biomass and litterfall but led to losses of base cations, mainly K and Mg, from LFH-layer. It was concluded that the NS treatment displaced cations from exchangeable sites in the LFH-layer leading to higher concentrations of these elements in both rhizosphere and bulk soil.
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    Behaviour of sulphur and nitrogen compounds measured at marine stations Lista and Säby in Scandinavia (1995)
    Springer
    Water, air & soil pollution 85 (1995), S. 2039-2044 
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    ISSN: 1573-2932
    Keywords: sulphur ; nitrogen ; Scandinavia ; long distance transport ; elemental tracers
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Long distance transport of various air pollutants has been studied at two Scandinavian coastal sites. The measuring period has covered one year divided into 4 campaigns. Seasonal variations for sulphur and nitrogen compounds as well as anthropogenically emitted metals are reported. Concentrations of Pb and Zn as well as the ratio of V/Ni concentrations have been used to trace sulphuric episodes. Covariation of anthropogenic pollutants for the two sites is demonstrated.
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    Modelling leaching of inorganic Hg(II) in a Scandinavian iron-humus podzol — validation and long-term leaching under various deposition rates (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 301-320 
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    ISSN: 1573-2932
    Keywords: acid rain ; batch experiment ; Freundlich isotherm ; lysimeter experiment ; mercury ; simulation model
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Increasing mercury contents are reported from freshwater systems and fish in northern Europe and North America. Mercury input from soils is a major source with the leaching being affected by increased atmospheric mercury deposition compared to pre-industrial times and by other environmental conditions such as acid rain. The results of a mathematical model-calculation of vertical inorganic Hg(II) leaching in a Scandinavian iron-humus podzol under different atmospheric input rates of mercury are presented. Leaching under background rain conditions was calculated to be considerably stronger than under acid rain conditions. Increasing fractions of deposited soluble or solute atmospheric mercury were leached from the O f(h)-horizon with decreasing soil content of soluble mercury under acid rain conditions; this effect was less pronounced under background rain conditions. The steady state concentrations of soluble mercury of the upper soil horizons were calculated and compared with the actual concentrations of total (= soluble + insoluble mercury) and extractable (= estimate of soluble) mercury measured in these horizons. The results indicate that even if the deposition of airborne mercury to soil is strongly reduced, the total mercury content of the soil decreases only slowly. It may take decades or even centuries before a new steady state concentration of total mercury is established in the soil. The decrease of the mercury concentration in the O f(h)-horizon is probably largely dependent on the turnover of organic matter, binding most of the deposited airborne mercury in an insoluble form. Hence, present day mercury leaching is likely to be dominated by mercury deposited during former times and temporarily retained in an insoluble form in the organic matter.
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    Variations in sulphur and nitrogen foliar concentration of deciduous and conifers vegetation in Slovakia (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 329-345 
    Details
    ISSN: 1573-2932
    Keywords: beech ; biomonitoring ; nitrogen ; solid particles ; spruce ; sulphur
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The foliage contents of Stotal and Ntotal were determined in 405 Permanent monitoring plots in four National Parks and sixteen Landscape Protection Areas and were compared with 1483 Permanent monitoring plots on Slovakia. The foliage content of S ranged from 0.72 to 6.77 g kg−1 in hardwoods and from 0.98 to 4.3 g kg−1 in softwoods. A critical increase was determined in one National Park and in four Landscape Protection Areas. The foliage content of N ranged from 9.7 to 48.7 g kg−1 in softwoods, and from 7.8 to 51.4 g kg−1 in hardwoods. An insufficient level of N was determined in one Landscape Protection Area and a critical increase in four Landscape Protection Areas. The sulphur to nitrogen ratio ranged from 0.08 to 0.176 in softwoods, and from 0.078 to 0.253 in hardwoods. The foliage surface on hitherto explored four National Parks and sixteen Landscape Protection Areas in network 4×4 km was covered by all categories of rigid fallout particles. Fly-ash from coal combustion were observed each of National Parks and Landscape Protection Areas by scanning electron microscopy. Mycelia and spore, mineral matters, sand and soil particles were present on all National Parks and Landscape Protection Areas. Particles derived from aluminium production were observed at three Landscape Protection Areas. Particles derived from cement production and from lime works were observed at two National Parks and six Landscape Protection Areas. Particles derived from ferrous metals industry were observed at each of National Parks and Landscape Protection Areas and particles typical for other technologies were present in three of National Parks and twelve Landscape Protection Areas.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF02407213
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  • 73
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    VARIATIONS IN SULPHUR AND NITROGEN FOLIAR CONCENTRATION OF DECIDUOUS AND CONIFERS VEGETATION IN SLOVAKIA (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 329-345 
    Details
    ISSN: 1573-2932
    Keywords: beech ; biomonitoring ; nitrogen ; solid particles ; spruce ; sulphur
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The foliage contents of Stotal and Ntotal were determined in 405 Permanent monitoring plots in four National Parks and sixteen Landscape Protection Areas and were compared with 1483 Permanent monitoring plots on Slovakia. The foliage content of S ranged from 0.72 to 6.77 g kg-1 in hardwoods and from 0.98 to 4.3 g kg-1 in softwoods. A critical increase was determined in one National Park and in four Landscape Protection Areas. The foliage content of N ranged from 9.7 to 48.7 g kg-1 in softwoods, and from 7.8 to 51.4 g kg -1 in hardwoods. An insufficient level of N was determined in one Landscape Protection Area and a critical increase in four Landscape Protection Areas. The sulphur to nitrogen ratio ranged from 0.08 to 0.176 in softwoods, and from 0.078 to 0.253 in hardwoods. The foliage surface on hitherto explored four National Parks and sixteen Landscape Protection Areas in network 4 × 4 km was covered by all categories of rigid fall-out particles. Fly-ash from coal combustion were observed each of National Parks and Landscape Protection Areas by scanning electron microscopy. Mycelia and spore, mineral matters, sand and soil particles were present on all National Parks and Landscape Protection Areas. Particles derived from aluminium production were observed at three Landscape Protection Areas. Particles derived from cement production and from lime works were observed at two National Parks and six Landscape Protection Areas. Particles derived from ferrous metals industry were observed at each of National Parks and Landscape Protection Areas and particles typical for other technologies were present in three of National Parks and twelve Landscape Protection Areas.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1026422606600
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  • 74
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    Mercury from Combustion Sources: A Review of the Chemical Species Emitted and Their Transport in the Atmosphere (1997)
    Springer
    Water, air & soil pollution 98 (1997), S. 241-254 
    Details
    ISSN: 1573-2932
    Keywords: coal ; deposition ; emission ; mercury ; municipal solidwaste
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Different species of mercury have different physical/chemical properties and thus behave quite differently in air pollution control equipment and in the atmosphere. In general, emissions of mercury from coal combustion sources are approximately 20–50% elemental mercury (Hg°) and 50–80% divalent mercury (Hg(II)), which may be predominantly HgCl2. Emissions of mercury from waste incinerators are approximately 10–20% Hg° and 75–85% Hg(II). The partitioning of mercury in flue gas between the elemental and divalent forms may be dependent on the concentration of particulate carbon, HCl and other pollutants in the stack emissions. The emission of mercury from combustion facilities depends on the species in the exhaust stream and the type of air pollution control equipment used at the source. Air pollution control equipment for mercury removal at combustion facilities includes activated carbon injection, sodium sulfide injection and wet lime/limestone flue gas desulfurization. While Hg(II) is water-soluble and may be removed from the atmosphere by wet and dry deposition close to combustion sources, the combination of a high vapor pressure and low water-solubility facilitate the long-range transport of Hg° in the atmosphere. Background mercury in the atmosphere is predominantly Hg°. Elemental mercury is eventually removed from the atmosphere by dry deposition onto surfaces and by wet deposition after oxidation to water- soluble, divalent mercury.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1026429911010
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  • 75
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    MONITORING NITROGEN POLLUTION FROM SUGARCANE RUNOFF USING 15N ANALYSIS (1997)
    Springer
    Water, air & soil pollution 98 (1997), S. 389-399 
    Details
    ISSN: 1573-2932
    Keywords: fertilizer ; nitrogen ; pollution ; runoff ; stable isotopes ; sugarcane
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract In many forested wetlands of Louisiana, surface water quality is being deteriorated by nutrient input from adjacent agricultural production areas. This field study assesses the input of fertilizer N, applied to sugarcane fields, to forested wetlands. The potential use of natural abundance variations in 15N14N ratios for identification and tracing surface water N sources (NH 4 + - and NO3 --N) was evaluated. Runoff and surface water samples were collected from sugarcane fields and bordering forested wetlands (6 stations) over a 16 month period and analyzed for NH 4 + -N, NO 3 - -N, and associated NH 4 + -δ15N and NO 3 - -δ15N ratios. Fertilizer N draining into adjacent forested wetland was estimated to be only a small fraction of the amount applied. Concentrations of NH 4 + - and NO 3 - -N in the collected water samples were low and ranged from 0.02 to 1.79 mg L-1. Isotopic analysis revealed NH 4 + -δ15N and NO 3 - -δ15N means were distinctive and may have the potential to be used as tracers of N contamination. The mean NH 4 + -δ15N value was +18.6 ± 7.1‰ and the NO 3 - -δ15N mean was +8.3 ± 3.1‰. Anomalously high NO 3 - -δ15N values (〉30‰) were attributed to denitrification.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1026483228623
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  • 76
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    UNCERTAINTY IN THE ESTIMATION OF CRITICAL LOADS: A PRACTICAL METHODOLOGY (1997)
    Springer
    Water, air & soil pollution 98 (1997), S. 297-316 
    Details
    ISSN: 1573-2932
    Keywords: acid deposition ; ecosystem ; GLUE ; PROFILE
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Critical loads of acid deposition for forest soils, ground and surface water resources are calculated utilising a variety of mathematical models. The estimation of the predictive uncertainty inherent in these models is important since the model predictions constitute the cornerstone of the development of emissions abatement policy decisions in Europe and the United Kingdom. The Generalised Likelihood Uncertainty Estimation (GLUE) approach is presented here as a tool for estimating the predictive uncertainty of PROFILE, a steady-state geochemical model that is widely applied within the critical loads community. GLUE is based on Monte Carlo simulation and explicitly recognises the possible equifinality of parameter sets. With this methodology it is possible to make an assessment of the likelihood of a parameter set being an acceptable simulator of a system when model predictions are compared to observed field data. The methodology is applied to a small catchment at Plynlimon, Mid-Wales. The results highlight that there is a large amount of predictive uncertainty associated with the model at the site: three of the six chosen field characteristics lie within the predicted distribution. The study also demonstrates that a wide range of parameter sets exist that give acceptable simulations of site characteristics as well as a broad distribution of critical load values that are consistent with the site data. Additionally, a sensitivity analysis of model parameters is presented.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1026496930386
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  • 77
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    Electronic Resource
    Mercury from combustion sources: A review of the chemical species emitted and their transport in the atmosphere (1997)
    Springer
    Water, air & soil pollution 98 (1997), S. 241-254 
    Details
    ISSN: 1573-2932
    Keywords: coal ; deposition ; emission ; mercury ; municipal solid waste
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Different species of mercury have different physical/chemical properties and thus behave quite differently in air pollution control equipment and in the atmosphere. In general, emissions of mercury from coal combustion sources are approximately 20–50% elemental mercury (Hg°) and 50–80% divalent mercury (Hg(II)), which may be predominantly HgCl2. Emissions of mercury from waste incinerators are approximately 10–20% Hg° and 75–85% Hg(II). The partitioning of mercury in flue gas between the elemental and divalent forms may be dependent on the concentration of particulate carbon, HCl and other pollutants in the stack emissions. The emission of mercury from combustion facilities depends on the species in the exhaust stream and the type of air pollution control equipment used at the source. Air pollution control equipment for mercury removal at combustion facilities includes activated carbon injection, sodium sulfide infection and wet lime/limestone flue gas desulfurization. While Hg(II) is water-soluble and may be removed from the atmosphere by wet and dry deposition close to combustion sources, the combination of a high vapor pressure and low water-solubility facilitate the long-range transport of Hg° in the atmosphere. Background mercury in the atmosphere is predominantly Hg°. Elemental mercury is eventually removed from the atmosphere by dry deposition onto surfaces and by wet deposition after oxidation to water-soluble, divalent mercury.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF02047037
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  • 78
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    Electronic Resource
    Uncertainty in the estimation of critical loads: A practical methodology (1997)
    Springer
    Water, air & soil pollution 98 (1997), S. 297-316 
    Details
    ISSN: 1573-2932
    Keywords: acid deposition ; ecosystem ; GLUE ; PROFILE
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Critical loads of acid deposition for forest soils, ground and surface water resources are calculated utilising a variety of mathematical models. The estimation of the predictive uncertainty inherent in these models is important since the model predictions constitute the cornerstone of the development of emissions abatement policy decisions in Europe and the United Kingdom. The Generalised Likelihood Uncertainty Estimation (GLUE) approach is presented here as a tool for estimating the predictive uncertainty of PROFILE, a steady-state geochemical model that is widely applied within the critical loads community. GLUE is based on Monte Carlo simulation and explicitly recognises the possible equifinality of parameter sets. With this methodology it is possible to make an assessment of the likelihood of a parameter set being an acceptable simulator of a system when model predictions are compared to observed field data. The methodology is applied to a small catchment at Plynlimon, Mid-Wales. The results highlight that there is a large amount of predictive uncertainty associated with the model at the site: three of the six chosen field characteristics lie within the predicted distribution. The study also demonstrates that a wide range of parameter sets exist that give acceptable simulations of the site characteristics as well as a broad distribution of critical load values that are consistent with the site data. Additionally, a sensitivity analysis of model parameters is presented.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF02047040
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  • 79
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    Sediment accumulation of nutrients (N, P) in the eastern Gulf of Finland (Baltic Sea) (1997)
    Springer
    Water, air & soil pollution 99 (1997), S. 477-486 
    Details
    ISSN: 1573-2932
    Keywords: sediment ; nitrogen ; phosphorus ; organic matter ; cluster analysis ; Gulf of Finland ; estuaries
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Dry weight (DW), ignition loss (IL) and concentrations of total nitrogen (TN) and total phosphorus (TP) of the sediment surface layer (0 to 10 cm, 1 cm slices) were analyzed from 20 sites in the eastern Gulf of Finland. The distance of the sampling sites from the mouth of the River Neva explained the nutrient concentrations of the sediments well, while the effect of water depth was negligible. The increase of TN and the decrease of TP along the transect from the river mouth towards the open Gulf were caused by the diminishing share of allochthonous material supplied from the River Neva. The mean TN concentration of the different accumulation areas was about 40 % higher in the sediment surface than in the deeper layer (9 to 10 cm). The corresponding difference for TP varied from 53 to 56 %. The results suggest considerable netflux of nutrients from sediment to water. The net sediment accumulation of nutrients were estimated as 6.0 g m−2 a−1 of N and 1.7 g m−2 a−1 of P corresponding 22 000 t a− of N and 6 100 t a−1 of P for the whole eastern Gulf.
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    URL: http://dx.doi.org/10.1007/BF02406887
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  • 80
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    INCREASING ROLE OF NITROGEN IN THE ACIDIFICATION OF SURFACE WATERS IN THE ADIRONDACK MOUNTAINS, NEW YORK (1997)
    Springer
    Water, air & soil pollution 95 (1997), S. 313-336 
    Details
    ISSN: 1573-2932
    Keywords: nitrogen ; acidification ; Adirondack Mountains ; atmospheric deposition
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Assessments of the aquatic effects of acidic deposition have focused on sulfur, as have recent efforts to control the emissions of acidifying compounds. Nitrogen dynamics were excluded from most acidic deposition modeling studies because it was believed that terrestrial ecosystems strongly retain N and because modeling N is a more formidable task than modeling S due to the influence of complex biological processes on N cycling. Re-examination of available data for the Adirondack Mountains of New York suggests that N deposition may be contributing to both chronic and episodic acidification of freshwaters to a greater extent than is generally believed. Previous research concluded that N has played a limited role in acidification processes in these lakes, based on regional averages of chronic chemistry. However, it is now known that historic acidification responses have been spatially variable within the Adirondack Mountains and that the declines in lakewater pH have been less than previously believed. Lakewater NO3 - concentrations are commonly in the range of 5 to 25 μeq L-1 on a chronic basis in portions of the Adirondack region that have experienced significant chronic acidification. These NO3 - concentrations correspond in magnitude to inferred historical acidification. Furthermore, the relative importance of NO3 - as an agent of acidification increases dramatically during snowmelt when conditions are most toxic to fish. The consequence of not addressing N in formulating acidification recovery strategies for the Adirondacks includes the likelihood that we will overestimate the response of surface water to the mandated sulfur emissions reductions.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1026422031266
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  • 81
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    REAL-TIME MEASUREMENT AND INTERPRETATION OF THE CONDUCTIVITY AND pH OF PRECIPITATION SAMPLES (1997)
    Springer
    Water, air & soil pollution 98 (1997), S. 325-344 
    Details
    ISSN: 1573-2932
    Keywords: acid rain ; acid deposition ; acid fraction ; precipitation pH and conductivity
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A microprocessor-based acid rain monitor was used to make real-time measurements of conductivity and pH of rainwater within individual storms. The automated measurements were compared with laboratory analyses of a subset of the samples taken. The laboratory measurements tended to overestimate the pH because of temperature induced changes in dissociation and Henry's Law constants affecting ionic compounds in the rainwater. The measurement artefact due to these effects may result in average hydrogen ion concentrations being underestimated by approximately 10 to 15% at UK sites. The greatest systematic discrepancies would be anticipated at highly polluted sites and during low temperature acidic episodes. The concept of a rainwater acid fraction was investigated and found to be useful for quality control and interpretative purposes. The field measurement of conductivity of low ionic strength samples was slightly lower than the corresponding laboratory measurement, possibly caused by limited resolution of the conductivity probe or dissolution of fine particulate material.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1026407027848
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  • 82
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    MERCURY ACCUMULATION IN DEVILS LAKE, NORTH DAKOTA – EFFECTS OF ENVIRONMENTAL VARIATION IN CLOSED-BASIN LAKES ON MERCURY CHRONOLOGIES (1997)
    Springer
    Water, air & soil pollution 98 (1997), S. 275-296 
    Details
    ISSN: 1573-2932
    Keywords: mercury ; mercury accumulation ; mercury deposition ; North Dakota ; saline lakes ; sediment cores
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Sediment cores were collected from lakes in the Devils Lake Basin in North Dakota to determine if mercury (Hg) accumulation chronologies from sediment-core data are good indicators of variations in Hg accumulation rates in saline lakes. Sediment cores from Creel Bay and Main Bay, Devils Lake were selected for detailed analysis and interpretation. The maximum Hg concentration in the Creel Bay core was 0.15 micrograms per gram at 8 to 9 centimeters. The maximum Hg concentration in the Main Bay core was 0.07 micrograms per gram at 5 to 7 centimeters. The general decreases in Hg concentrations with depth are attributed to historic variations in atmospheric Hg deposition rate. Hg stratigraphies combined with210 Pb and 137Cs dating analyses yield Hg chronologies that indicate a general increase in Hg accumulation rates in Devils Lake since the middle of the 19th century. Mean modern Hg accumulation rates in Creel Bay were 4.9 nanograms per square centimeter per year, and rates in Main Bay were 1.8 nanograms per square centimeter per year. Mean preindustrial Hg accumulation rates in Creel Bay were 1.2 nanograms per square centimeter per year, and rates in Main Bay were 1.6 nanograms per square centimeter per year. Relatively low Hg concentrations in recent sediments in the Devils Lake Basin, along with similarities in Hg accumulation rates between lakes in the Devils Lake Basin and other lakes in the northern interior of North America, indicate that local sources of Hg are not important sources of Hg. Results of the study indicate that accurate Hg chronologies are discernible in sediment cores collected from saline lakes. However, spatial and temporal variations in lake level and water chemistry common to saline lakes make interpretation of radioisotopic and geochemical chronologies difficult. Hg geochemistry in Devils Lake, and presumably in other saline lakes, is dynamic. The results of this study indicate that the absolute amount of sediment transported to Devils Lake, along with the associated Hg and total organic carbon, and the distribution of sedimentation patterns in Devils Lake may be affected by changing lake levels.
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    URL: http://dx.doi.org/10.1023/A:1026415001754
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  • 83
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    An Overview of Contaminant-Related Issues Identified by Monitoring in San Francisco Bay (2000)
    Springer
    Environmental monitoring and assessment 64 (2000), S. 409-419 
    Details
    ISSN: 1573-2959
    Keywords: monitoring ; assessment ; water ; sediment ; bioaccumulation ; toxicity ; pesticides ; mercury ; PCB
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The San Francisco Estuary Regional Monitoring Program for Trace Substances (RMP) began in 1993 and is sponsored by 74 local, state, and federal agencies and companies through their discharge or Bay use permits. The RMP monitors water, sediment, toxicity, and bivalve bioaccumulation at 25 sites in the Bay that are considered to represent "background" conditions. Several major environmental issues have been identified by the RMP. Polychlorinated biphenyls and mercury were often above water quality guidelines, and often occurred in fish tissues above U.S. Environmental Protection Agency (U.S. EPA) screening values. Concentrations do not appear to be decreasing, suggesting continuing inputs. Episodes of aquatic toxicity often occurred following runoff events that transport contaminants into the Bay from urbanized and agricultural portions of the watershed. Sediment toxicity occurred throughout the Bay, and has been correlated with concentrations of specific contaminants (chlordanes, polynuclear aromatic hydrocarbons) at some locations; mixtures of contaminants were probably also important. Since the RMP does not monitor all ecosystem components, assessments of the overall condition of the Bay cannot be made. However, in terms of contamination, the RMP samples suggest that the South Bay, and North Bay sites are moderately contaminated.
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    URL: http://dx.doi.org/10.1023/A:1006459605924
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  • 84
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    Contamination Near Chernobyl: radiocaesium, Lead and Mercury in Fish and Sediment Radiocaesium from Waters Within the 10 km Zone (1998)
    Springer
    Ecotoxicology 7 (1998), S. 201-209 
    Details
    ISSN: 1573-3017
    Keywords: radiocaesium ; mercury ; lead ; fish ; Chernobyl
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Samples of fish and sediments collected from waters within 10 km of the Chernobyl Nuclear Power Plant were analysed for radiocaesium and other atmospherically transported pollutants (lead (Pb) and mercury (Hg)) were measured in fish tissues. For comparison, fish muscle was also sampled from a less-contaminated area of the Kiev Reservoir and from a hatchery in Kiev. In sediments, 137Cs was the major gamma-emitting isotope, with concentrations of over 100 Bq g−1 in canals adjacent to the reactor and in ponds that were downwind during the accident. The radiocaesium distributions appeared non-normal, were very patchy and could vary by over 100% in samples collected metres to tens of metres apart. Fish muscle radiocaesium from ponds within 10 km of the power plant was in the range of 6–192 Bq g−1. The fish muscle radiocaesium concentrations were highest in ponds from the downwind sites and were correlated with the sediment radiocaesium concentrations. The lead and mercury concentrations in fish were relatively low (medians 〈0.8 μg Hg per g dry mass and 〈150 ng Pb per g dry mass), suggesting little contamination from lead applied to the burning reactor after the accident. The radiocaesium levels in fish in areas close to the reactor continue to be high enough to cause health concerns to humans that might utilize these resources.
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    URL: http://dx.doi.org/10.1023/A:1008934710904
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    The Bioaccumulation of Mercury in Aquatic Organisms from Two Similar Lakes with Differing pH (1999)
    Springer
    Ecotoxicology 8 (1999), S. 49-56 
    Details
    ISSN: 1573-3017
    Keywords: mercury ; methylmercury ; fish ; acidification ; biomagnification
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Two small drainage lakes of similar surface area (0.4–0.6 km 2 ) and depth, and situated in close proximity to one another (about 9 km apart) in the Muskoka-Haliburton district of rural Ontario, Canada were chosen to investigate the effects of differing pH on Hg accumulation in fish and other biota. Blue Chalk Lake is circumneutral (pH = 6.3–6.9) with an average dissolved organic carbon (DOC) concentration of 2.69 mg/L; Plastic Lake is acidic (pH = 5.2–5.6) with a similar DOC level (2.72 mg/L). Neither lake is an impoundment, and neither receives inputs from point-source urban or industrial waste emissions. Surficial (top 4 cm) sediments and various aquatic biota, including crayfish (Orconectes virilis)], and 5 species of fish [brown bullhead (Ictalurus nebulosus), creek chub (Semotilus atromaculatus), pumpkinseed sunfish (Lepomis gibbosus), yellow perch (Perca flavenscens) and rock bass (Ambloplites rupestris)] were sampled for Hg analysis. Only creek chub and pumpkinseed occurred in both lakes. Significant size (length) vs. Hg-concentration relationships were observed for brown bullhead, pumpkinseed, yellow perch and rock bass, but not for crayfish nor for creek chub in either lake. Rock bass had the highest mean Hg concentration (1.02 ± 0.98 μg/g dry wt.). Pumpkinseed from Plastic Lake had the highest overall rate of accumulation with increasing size. Several individual pumpkinseed and rock bass sampled from the acidic Plastic Lake had Hg concentrations equal to or greater than levels reported to be hazardous to breeding piscivorous birds, such as common loons (Gavia immer), whereas no fish from Blue Chalk approached this threshold (0.3 μg/g wet wt). This study illustrates the importance of within-lake parameters, particularly pH, and species trophic level, in determining Hg accumulation in fish in lakes of similar size that receive similar atmospheric Hg inputs.
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    URL: http://dx.doi.org/10.1023/A:1008936910823
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    Effects of humic acid on transport and transformation of mercury in soil-plant systems (1997)
    Springer
    Water, air & soil pollution 95 (1997), S. 35-43 
    Details
    ISSN: 1573-2932
    Keywords: humic acid ; mercury ; transport ; transformation ; soil-plant system
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The influence of humic acid (HA) on the transport and transformation of mercury (Hg) in soil was studied. No available Hg could be detected (〈2.5 μg kg−1) in alluvial soil when the content of HA-carbon (HA-C) was higher than 0.2 g kg−1 although a large amount of Hg (8 μg kg−1) was applied to the soil. The available Hg decreased with the increase of HA in purple soil (r=0.735). There are significant correlations between HA concentration and organic Hg in the tested soils (r=0.974 for the purple soil and r=0.979 for the alluvial soil). The increase of HA results in decrease of Hg absorbed by plant from the soil. A loss of Hg from soil caused by microbes was observed.
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    URL: http://dx.doi.org/10.1007/BF02406154
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    EFFECTS OF HUMIC ACID ON TRANSPORT AND TRANSFORMATION OF MERCURY IN SOIL-PLANT SYSTEMS (1997)
    Springer
    Water, air & soil pollution 95 (1997), S. 35-43 
    Details
    ISSN: 1573-2932
    Keywords: humic acid ; mercury ; transport ; transformation ; soil-plant system
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The influence of humic acid (HA) on the transport and transformation of mercury (Hg) in soil was studied. No available Hg could be detected (〈2.5 μg kg-1) in alluvial soil when the content of HA-carbon (HA-C) was higher than 0.2 g kg-1 although a large amount of Hg (8 μg kg-1) was applied to the soil. The available Hg decreased with the increase of HA in purple soil (r=0.735). There are significant correlations between HA concentration and organic Hg in the tested soils (r=0.974 for the purple soil and r=0.979 for the alluvial soil). The increase of HA results in decrease of Hg absorbed by plant from the soil. A loss of Hg from soil caused by microbes was observed.
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    URL: http://dx.doi.org/10.1023/A:1026468724284
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  • 88
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    Acid deposition during two contrasting frontal rainfall events (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 93-106 
    Details
    ISSN: 1573-2932
    Keywords: acid deposition ; acid rain ; back trajectory analysis ; precipitation events ; precipitation scavenging ; sub-event chemistry ; sub-event sampling
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Analysis of the chemical composition of rain at high temporal resolution provides additional information on wet deposition processes. High resolution data was obtained using a microprocessor-based acid rain monitor at two sites in SW Scotland and SE England. Meteorological details of the transport and wet deposition processes during two frontal rain events were examined and related to rainfall composition. Rapid depletions of ion concentrations during heavy rainfall in the first event were interpreted using a rainfall scavenging model. The sub-event data for the second event showed the influence of frontal discontinuities. Increasing ionic concentrations during this second event were attributed both to the change in air mass, and to diminished upwind precipitation scavenging.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF02407198
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  • 89
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    ACID DEPOSITION DURING TWO CONTRASTING FRONTAL RAINFALL EVENTS (1997)
    Springer
    Water, air & soil pollution 96 (1997), S. 93-106 
    Details
    ISSN: 1573-2932
    Keywords: acid deposition ; acid rain ; back trajectory analysis ; precipitation events ; precipitation scavenging ; sub-event chemistry ; sub-event sampling
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Analysis of the chemical composition of rain at high temporal resolution provides additional information on wet deposition processes. High resolution data was obtained using a microprocessor-based acid rain monitor at two sites in SW Scotland and SE England. Meteorological details of the transport and wet deposition processes during two frontal rain events were examined and related to rainfall composition. Rapid depletions of ion concentrations during heavy rainfall in the first event were interpreted using a rainfall scavenging model. The sub-event data for the second event showed the influence of frontal discontinuities. Increasing ionic concentrations during this second event were attributed both to the change in air mass, and to diminished upwind precipitation scavenging.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1026430913153
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  • 90
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    Global Mercury Pollution and the Role of Gold Mining: An Overview (1997)
    Springer
    Water, air & soil pollution 97 (1997), S. 205-207 
    Details
    ISSN: 1573-2932
    Keywords: mercury ; gold mining ; ecosystems ; methyl-Hg ; cycling ; global sources
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract As described by Jernelov and Ramel (1995), the Scientific Committee on Problems of the Environment (SCOPE) sponsored an investigation of Hg in ecosystems with special emphasis on tropical regions. In these regions small-scale gold mining activities have occupied about 10 million people worldwide who use Hg for extracting gold.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1018304920365
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  • 91
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    Determination of Atmospheric Mercury During the North Sea Experiment (1997)
    Springer
    Water, air & soil pollution 97 (1997), S. 257-263 
    Details
    ISSN: 1573-2932
    Keywords: mercury ; atmosphere ; rainwater ; marine
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Total gaseous mercury (TGM) and rainwater were collected on board of two research vessels (F. S. ALKOR and R.V. BELGICA) positioned 200 km apart in the center of the North Sea Experiment, September 1991. On the F.S. ALKOR (up-wind ship) TGM concentrations ranged from 0.7 to 2.6 ng·m-3 with an average of 1.5 ng·m-3 and on the R. V. BELGICA (down-wind ship) TGM ranged from 0.7 to 1.9 ng·m-3 with an average of 1.2 ng·m-3. An average 20% decrease is observed from the up-wind to the downwind ship, which may largely be affected by entrainment into the free troposphere. An overall removal was 0.5 cm·s-1 for dry periods and varied between 1 to 5 cm·s-1 during rain events. Rainwater concentrations varied between 5 and 25 ng·l-1. Based on these data an annual wet deposition flux of 1.08 ng Hg cm-2 yr1- was estimated for the North Sea.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1018311107587
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  • 92
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    Nutrient distribution in a Norway spruce stand after long-term application of ammonium nitrate and superphosphate (1996)
    Springer
    Water, air & soil pollution 92 (1996), S. 451-467 
    Details
    ISSN: 1573-2932
    Keywords: Biomass ; calcium ; fertilization ; loss ; magnesium ; nitrogen ; nutrient ; potassium ; recovery ; soil
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The distribution of nutrients between soil layers and above-ground tree components was examined in a Norway spruce stand that had received ammonium nitrate (annually) and superphosphate (about every third year) for 22 years. Four treatments were included in the study; control (n = 4), N1P1, N2P2 and N3P2 (n = 2), which had received a total of 0, 730, 1700 and 2550 kg nitrogen (N) ha-1, 0, 130, 300 and 300 kg phosphorus (P) ha-1 and 0, 340, 784 and 784 kg calcium (Ca) ha-1, respectively. Compared with the control, stem-wood growth had been three times higher in N1P1 and three and a half times higher in N2P2 and N3P2. Amounts of N, P, Ca, potassium (K) and magnesium (Mg) in the above-ground tree biomass increased (p〈0.05) with the fertilizer dose, whereas manganese (Mn) did not. The recovery of fertilizer N and Ca in soil and above-ground tree biomass was negatively related to the fertilizer dose, although there had been a buildup of the N and Ca pools in the mor layer. This strongly indicates that at least the higher doses of N addition caused substantial nitrate leaching. Soil pools of K, Mg and Mn decreased as the fertilizer dose increased. However, the system total amounts (above-ground tree biomass plus soil) of K and Mg did not differ between treatments suggesting that no extra losses of these ions induced by nitrate leaching have occurred. Thus, in an aggrading forest ecosystem, N additions are likely to be followed by increased uptake of K, Mg and Ca. This may to some extent prevent extra leaching of these ions, which otherwise would be expected when there is an increase in nitrate leaching.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00283572
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  • 93
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    Carbon and Nitrogen Stable Isotope Fractionation in the Sediment of Lake Bled (Slovenia) (1997)
    Springer
    Water, air & soil pollution 99 (1997), S. 315-323 
    Details
    ISSN: 1573-2932
    Keywords: lake ; sediment ; carbon ; nitrogen ; stable isotope ; fractionation
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Stable isotope composition of carbon and nitrogen in the sediment and pore water of a eutrophic freshwater lake was studied. Based on changes in the δ13C and δ15N values of dissolved components and sediment fraction, possible processes involved in the decomposition of sedimentary organic matter are outlined. The relative importance of acetate fermentation and CO2 reduction was estimated using known mathematical models, and ammonia assimilation by methanogenic bacteria is hypothesised to be the main process governing the isotope fractionation of dissolved nitrogen in pore water.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1018354415109
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  • 94
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    Benthic Fluxes of Dissolved Inorganic Carbon, Nutrients and Oxygen in the Gulf of Trieste (Northern Adriatic) (1997)
    Springer
    Water, air & soil pollution 99 (1997), S. 305-314 
    Details
    ISSN: 1573-2932
    Keywords: Adriatic Sea ; nutrients ; benthic fluxes ; carbon ; nitrogen ; silicon ; phosphorus ; budgets
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Benthic fluxes of dissolved inorganic N, Si and P nutrients, alkalinity, dissolved inorganic C (DIC), and O2 from sediments in the Gulf of Trieste (northern Adriatic, Italy) were measured monthly in the period September 1995 - August 1996 using in situ incubated light benthic chambers. The highest efluxes of DIC, NH4+, PO43-, Si(OH)4, and NO3- influxes encountered in late summer - early autumn were the consequence of degradation of benthic microalgae, and in autumn mostly of sedimented phytoplankton. High NO3- efflux was observed in spring. Only NH4+ and Si(OH)4 fluxes were significantly correlated with temperature. This correlation suggests that the rate of downward input and the quality and quantity of sedimentary organic matter (autochthonous and allochthonous) were superimposed on the temperature fluctuations. High DIC, NH4+ and Si(OH)4 effluxes observed in July 1996 were due to the late spring - early summer degradation of sedimentary organic matter produced by benthic microalgae, while the autumn phytoplankton bloom was quickly reflected in enhanced benthic fluxes due to higher temperature. Significant correlations between NH4+, PO43- and Si(OH)4 fluxes suggested their parallel regeneration and utilization at the sediment-water interface. The nutrient fluxes were linked to O2 consumption, suggesting that aerobic oxidation processes were important at the sediment-water interface in the Gulf. The N, P and Si nutrients released from sediment pore waters are probably utilized in benthic microalgal and bottom-water primary production. This indicates that pelagic and benthic communities in the central part of the Gulf of Trieste function relatively independently of each other.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1018398231038
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  • 95
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    Seasonal Changes in Cystoseira Myrica and Phosphorus Input at Two Sites of the Red Sea Egyptian Coast (1997)
    Springer
    Water, air & soil pollution 93 (1997), S. 199-211 
    Details
    ISSN: 1573-2932
    Keywords: Cystoseira myrica ; Red Sea ; coral reefs ; nitrogen ; phosphorus ; pollution ; eutrophication
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Elevated phosphate concentrations at Safaga and Quseir, Red Sea, Egyptian coast, wererelated to some ecological and nutritional aspects of the macro-alga Cystoseira myrica during1985. The results obtained were compared with those recorded for a non-polluted control site atGhardaqa. Chemical analysis of surface seawater samples revealed that the concentrations of dissolvedphosphate at Safaga and Quseir were 3 and 20 times as much as that at Ghardaqa, respectively.The standing crop of C. myrica showed two peaks in spring and autumn. Maximum biomass yield(491 g m-2) and number of individuals (127 m-2) of C. myrica were recorded in the spring at theGhardaqa site. Quseir C. myrica samples contained significantly higher protein-N, total-N andtotal-P values but lower carbohydrate values than the Safaga and Ghardaqa samples (LSD at 1%level). Tissue N:P molar ratios for C. myrica, Laurencia papillosa and Ulva lactuca collected fromGhardaqa ranged from 68-98, compared to 30-59 for the same species collected at thephosphorus polluted sites at Safaga and Quseir. The carbon levels and the C:N ratios of C. myricaexhibited no significant variations in the three studied sites. However, the C:P ratios of Ghardaqaplants were significantly higher than those of Safaga and Quseir.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1022196227853
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  • 96
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    Mercury accumulation in Devils Lake, North Dakota — Effects of environmental variation in closed-basin lakes on mercury chrologies (1997)
    Springer
    Water, air & soil pollution 98 (1997), S. 275-296 
    Details
    ISSN: 1573-2932
    Keywords: mercury ; mercury accumulation ; mercury deposition ; North Dakota ; saline lakes ; sediment cores
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Sediment cores were collected from lakes in the Devils Lake Basin in North Dakota to determine if mercury (Hg) accumulation chronologies from sediment-core data are good indicators of variations in Hg accumulation rates in saline lakes. Sediment cores from Creel Bay and Main Bay, Devils Lake were selected for detailed analysis and interpretation. The maximum Hg concentration in the Creel Bay core was 0.15 micrograms per gram at 8 to 9 centimeters. The maximum Hg concentration in the Main Bay core was 0.07 micrograms per gram at 5 to 7 centimeters. The general decreases in Hg concentrations with depth are attributed to historic variations in atmospheric Hg deposition rate. Hg stratigraphies combined with210Pb and137Cs dating analyses yield Hg chronologies that indicate a general increase in Hg accumulation rates in Devils Lake since the middle of the 19th century. Mean modern Hg accumulation rates in Creel Bay were 4.9 nanograms per square centimeter per year, and rates in Main Bay were 1.8 nanograms per square centimeter per year. Mean preindustrial Hg accumulation rates in Creel Bay were 1.2 nanograms per square centimeter per year, and rates in Main Bay were 1.6 nanograms per square centimeter per year. Relatively low Hg concentrations in recent sediments in the Devils Lake Basin, along with similarities in Hg accumulation rates between lakes in the Devils Lake Basin and other lakes in the northern interior of North America, indicate that local sources of Hg are not important sources of Hg. Results of the study indicate that accurate Hg chronologies are discernible in sediment cores collected from saline lakes. However, spatial and temporal variations in lake level and water chemistry common to saline lakes make interpretation of radioisotopic and geochemical chronologies difficult. Hg geochemistry in Devils Lake, and presumably in other saline lakes, is dynamic. The results of this study indicate that the absolute amount of sediment transported to Devils Lake, along with the associated Hg and total organic carbon, and the distribution of sedimentation patterns in Devils Lake may be affected by changing lake levels.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF02047039
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  • 97
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    Real-time measurement and interpretation of the conductivity and pH of precipitation samples (1997)
    Springer
    Water, air & soil pollution 98 (1997), S. 325-344 
    Details
    ISSN: 1573-2932
    Keywords: acid rain ; acid deposition ; acid fraction ; precipitation pH and conductivity
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract A microprocessor-based acid rain monitor was used to make real-time measurements of conductivity and pH of rainwater within individual storms. The automated measurements were compared with laboratory analyses of a subset of the samples taken. The laboratory measurements tended to overestimate the pH because of temperature induced changes in dissociation and Henry's Law constants affecting ionic compounds in the rainwater. The measurement artefact due to these effects may result in average hydrogen ion concentrations being underestimated by approximately 10 to 15% at UK sites. The greatest systematic discrepancies would be anticipated at highly polluted sites and during low temperature acidic episodes. The concept of a rainwater acid fraction was investigated and found to be useful fro quality control and interpretative purposes. The field measurement of conductivity of low ionic strength samples was slightly lower than the corresponding laboratory measurement, possibly caused by limited resolutio nof the conductivity probe or dissolution of fine particulate material.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF02047042
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  • 98
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    Holling's Figure-Eight Model: A Technical Reevaluation in Relation to Climate Change and Biodiversity (1998)
    Springer
    Environmental monitoring and assessment 49 (1998), S. 157-168 
    Details
    ISSN: 1573-2959
    Keywords: biodiversity ; carbon storage ; climate change ; conservation ; creative destruction ; ecological succession ; ecosystem stability ; Holling figure-eight ; nitrogen ; resilience
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract Holling proposed a four-phase conceptual model of ecosystem dynamics that includes exploitation, conservation, and destructive and renewal components to explain the failure of many natural resource management schemes. The model is drawn as a sideways figure-eight i.e. ∞. There are two dimensions in this model, connectivity (abscissa) and the amount of capital stored in the system (ordinate). This conceptual model has been suggested as a guide to thinking about the impact of climate change on biodiversity, but the two dimensions are insufficient and the alignment of the figure-eight model is problematic when compared with actual data. Kay has adjusted the dimensions of the figure-eight model and renamed the abscissa as exergy stored and the ordinate as exergy consumed. We realign the original figure-eight model, labeling the abscissa as carbon stored and the ordinate as nutrients, such that the relative values of both axes are in qualitative agreement with data from four different studies. This new alignment is then shown to fit relatively well with Holling's original labels. This revision of the figure-eight model brings Holling's model into agreement with observations and provides insight into the linkages between biodiversity and climate change.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1005813702080
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  • 99
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    Restoration of the Kissimmee River, Florida: Water Quality Impacts from Canal Backfilling (1999)
    Springer
    Environmental monitoring and assessment 57 (1999), S. 85-107 
    Details
    ISSN: 1573-2959
    Keywords: Kissimmee River ; mercury ; nutrients ; restoration ; water quality
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract The planned restoration of the Kissimmee River ecocystem will backfill approximately 35 km of flood control canal (C-38) that cuts through the meandering river channel, re-establish natural flow patterns, and restore the river/floodplain ecosystem. Water quality monitoring, including nutrients, total suspended solids (TSS), turbidity, dissolved oxygen (DO), and mercury, was conducted during a pilot `test fill' project to determine if soil disturbance during canal backfilling would negatively impact these water quality constituents. Surface water nutrient concentrations varied little between sites. Generally, highest concentrations occurred prior to construction, with lowest concentrations occurring during and after construction. During construction, TSS concentrations increased at sites immediately upstream, downstream, and adjacent to the construction area. Increased turbidity was generally restricted to areas immediately upstream and downstream of the test plug, with maximum levels occurring during the initial construction phase. Some downstream increases in turbidity were observed; however, impacts were short-term, lasting less than 24 h. Depresssed DO levels (〈2 mg/l) were observed upstream of the test plug following completion of the initial plug across C-38. Dissolved oxygen levels remained low for approximately 6 weeks, with no apparent ecological impacts. Total mercury (HgT) within canal sediment ranged from 9.2–180 ng/g and methylmercury concentrations ranged from 0.037–0.708 ng/g. Concentration of total mercury and total methylmercury (MeHgT) in the backfill material were much lower than concentrations in the canal sediment. No significant change in aqueous HgT concentrations occurred over the sampling period, although construction-induced turbidity could have temporarily caused a slightly elevated concentration immediately downstream of the construction site. Methylmercury concentrations in the water column ranged from 0.033–0.518 ng/l. No significant differences in mean MeHgT concentrations occured between sites or between sampling dates, except at one downstream site where MeHgT declined significantly over the sampling period.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1005962006268
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  • 100
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    Estimation of riverine loads of nitrogen and phosphorus to the Baltic Sea, 1970–1993 (1999)
    Springer
    Environmental monitoring and assessment 58 (1999), S. 173-200 
    Details
    ISSN: 1573-2959
    Keywords: Baltic Sea ; nitrogen ; phosphorous ; riverine load ; timeseries
    Source: Springer Online Journal Archives 1860-2000
    Topics: Energy, Environment Protection, Nuclear Power Engineering
    Notes: Abstract This article presents the results of the first critical examination of time series of riverine nutrient-load data for the entire Baltic Sea drainage area. Water quality data collected by or for the different national environmental agencies were compiled and analysed statistically to identify and remove inconsistent or obviously incorrect observations. Moreover, sampling tours were undertaken to acquire additional information about the present nutrient concentrations in the largest rivers in the study area. Gaps in the time series of approved data were then filled in by employing statistical interpolation and extrapolation methods. Thereafter, the concentration and runoff data were combined to obtain estimates of monthly nutrient loads for the time period 1970–93. The results of the calculations showed that although there had been substantial changes in land use, atmospheric deposition and wastewater treatment in many parts of the study area, the total riverine loads of nitrogen (N) and phosphorus (P) to the Baltic Sea have been fairly constant since 1980, and most likely also since 1970. Moreover, the interannual variation was clearly correlated to the runoff. The mean annual loads for the time period 1980–93 were found to be about 825 000 tonnes N and 41 000 tonnes P, respectively. This implies that (i) several other investigators have strongly underestimated the riverine loads of nutrients, especially the nitrogen, and that (ii) the riverine loads by far exceed the input to the Baltic Sea from other sources, {i.e.} atmospheric deposition, direct emissions from cities and industries along the Baltic Sea coast and nitrogen fixation by marine algae.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1023/A:1006073015871
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