ALBERT

Description: The contribution of turbulent mixing to heat and tracer transport in the tropical tropopause layer (TTL) is poorly constrained, partly owing to a lack of direct observations. Here, the authors use high-resolution (20 Hz) airborne measurements to study the occurrence and properties of small-scale (

Description: Due to their increasing spatial resolution, numerical weather prediction (NWP) models and the associated analyses resolve a growing fraction of the gravity wave (GW) spectrum. However, it is unclear how well this “resolved” part of the spectrum truly compares to the actual atmospheric variability. In particular, the Lagrangian variability, relevant, for example, to atmospheric dispersion and to microphysical modeling in the upper troposphere–lower stratosphere (UTLS), has not yet been documented in recent products. To address this shortcoming, this paper presents an assessment of the GW spectrum as a function of the intrinsic (air parcel following) frequency in recent (re)analyses (ERA-Interim, ERA5, the ECMWF operational analysis and MERRA-2). Long-duration, quasi-Lagrangian balloon observations in the equatorial and Antarctic lower stratosphere are used as a reference for the atmospheric spectrum and are compared to synthetic balloon observations along trajectories calculated using the wind and temperature fields of the reanalyses. Overall, the reanalyses represent realistic features of the spectrum, notably the spectral gap between planetary and gravity waves and a peak in horizontal kinetic energy associated with inertial waves near the Coriolis frequency f in the polar region. In the tropics, they represent the slope of the spectrum at low frequency. However, the variability is generally underestimated even in the low-frequency portion of the spectrum. In particular, the near-inertial peak, although present in the reanalyses, has a reduced magnitude compared to balloon observations. We compare the observed and modeled variabilities of temperature, zonal momentum flux and vertical wind speed, which are related to low-, mid- and high-frequency waves, respectively. The probability density function (PDF) distributions have similar shapes but show increasing disagreement with increasing intrinsic frequency. Since at those altitudes they are mainly caused by gravity waves, we also compare the geographic distribution of vertical wind fluctuations in the different products, which emphasizes the increase of both GW variance and intermittency with horizontal resolution. Finally, we quantify the fraction of resolved variability and its dependency on model resolution for the different variables. In all (re)analysis products, a significant part of the variability is still missing, especially at high frequencies, and should hence be parameterized. Among the two polar balloon datasets used, one was broadcast on the Global Telecommunication System for assimilation in NWP models, while the other consists of independent observations (unassimilated in the reanalyses). Comparing the Lagrangian spectra between the two campaigns shows that the (re)analyses are largely influenced by balloon data assimilation, which especially enhances the variance at low GW frequency.

Description: Transport of pollutants into the stratosphere via the Asian summer monsoon (ASM) or North American summer monsoon (NASM) may affect the atmospheric composition and climate both locally and globally. We identify and study the robust characteristics of transport from the ASM and NASM regions to the stratosphere using the Lagrangian chemistry transport model CLaMS driven by both the ERA-Interim and MERRA-2 reanalyses. In particular, we quantify the relative influences of the ASM and NASM on stratospheric composition and investigate the transport pathways and efficiencies of transport of air masses originating at different altitudes in these two monsoon regions to the stratosphere. We release artificial tracers in several vertical layers from the middle troposphere to the lower stratosphere in both ASM and NASM source regions during July and August 2010–2013 and track their evolution until the following summer. We find that more air mass is transported from the ASM and NASM regions to the tropical stratosphere, and even to the southern hemispheric stratosphere, when the tracers are released clearly below the tropopause (350–360 K) than when they are released close to the tropopause (370–380 K). For tracers released close to the tropopause (370–380 K), transport is primarily into the northern hemispheric lower stratosphere. Results for different vertical layers of air origin reveal two transport pathways from the upper troposphere over the ASM and NASM regions to the tropical pipe: (i) quasi-horizontal transport to the tropics below the tropopause followed by ascent to the stratosphere via tropical upwelling, and (ii) ascent into the stratosphere inside the ASM/NASM followed by quasi-horizontal transport to the tropical lower stratosphere and further to the tropical pipe. Overall, the tropical pathway (i) is faster than the monsoon pathway (ii), particularly in the ascending branch. The abundance of air in the tropical pipe that originates in the ASM upper troposphere (350–360 K) is comparable to the abundance of air ascending directly from the tropics to the tropical pipe 10 months after (the following early summer) the release of the source tracers. The air mass contributions from the ASM to the tropical pipe are about 3 times larger than the corresponding contributions from the NASM. The transport efficiency into the tropical pipe, the air mass fraction inside this destination region normalized by the mass of the domain of origin, is greatest from the ASM region at 370–380 K. Although the contribution from the NASM to the stratosphere is less than that from either the ASM or the tropics, the transport efficiency from the NASM is comparable to that from the tropics.

Description: Water vapour (H2O) in the upper troposphere and lower stratosphere (UTLS) has a significant role for global radiation. A realistic representation of H2O is therefore critical for accurate climate model predictions of future climate change. In this paper we investigate the effects of current uncertainties in tropopause temperature, horizontal transport and small-scale mixing on simulated H2O in the lower stratosphere (LS). To assess the sensitivities of simulated H2O, we use the Chemical Lagrangian Model of the Stratosphere (CLaMS). First, we examine CLaMS, which is driven by two reanalyses, from the European Centre of Medium-Range Weather Forecasts (ECMWF) ERA-Interim and the Japanese 55-year Reanalysis (JRA-55), to investigate the robustness with respect to the meteorological dataset. Second, we carry out CLaMS simulations with transport barriers along latitude circles (at the Equator, 15 and 35∘ N/S) to assess the effects of horizontal transport. Third, we vary the strength of parametrized small-scale mixing in CLaMS. Our results show significant differences (about 0.5 ppmv) in simulated stratospheric H2O due to uncertainties in the tropical tropopause temperatures between the two reanalysis datasets, JRA-55 and ERA-Interim. The JRA-55 based simulation is significantly moister when compared to ERA-Interim, due to a warmer tropical tropopause (approximately 2 K). The transport barrier experiments demonstrate that the Northern Hemisphere (NH) subtropics have a strong moistening effect on global stratospheric H2O. The comparison of tropical entry H2O from the sensitivity 15∘ N/S barrier simulation and the reference case shows differences of up to around 1 ppmv. Interhemispheric exchange shows only a very weak effect on stratospheric H2O. Small-scale mixing mainly increases troposphere–stratosphere exchange, causing an enhancement of stratospheric H2O, particularly along the subtropical jets in the summer hemisphere and in the NH monsoon regions. In particular, the Asian and American monsoon systems during a boreal summer appear to be regions especially sensitive to changes in small-scale mixing, which appears crucial for controlling the moisture anomalies in the monsoon UTLS. For the sensitivity simulation with varied mixing strength, differences in tropical entry H2O between the weak and strong mixing cases amount to about 1 ppmv, with small-scale mixing enhancing H2O in the LS. The sensitivity studies presented here provide new insights into the leading processes that control stratospheric H2O, which are important for assessing and improving climate model projections.

Description: Surface-emitted tracers with different dependencies on transit time (e.g., due to chemical loss or time-dependent boundary conditions) carry independent pieces of information on the age of air spectrum (the distribution of transit times from the surface). This paper investigates how and to what extent knowledge of tracer concentrations can be used to retrieve the age spectrum. Since the mixing ratios of the tracers considered depend linearly on the transit time distribution, the question posed can be formulated as a linear inverse problem of small dimension. An inversion methodology is introduced, which does not assume a prescribed shape for the spectrum. The performance of the approach is first evaluated on a constructed set of artificial radioactive tracers derived from idealized spectra. Hereafter, the inversion method is applied to outputs of a chemistry–transport model. The latter experiment highlights the limits of inversions using only parent radioactive tracers: they are unable to retrieve fine-scale structures such as the annual cycle. Improvements can be achieved by including daughter decaying tracers and tracers with an annual cycle at the surface. This study demonstrates the feasibility of retrieving the age spectrum from tracers and has implications for transport diagnosis in models and observations.

Description: Gravity waves are an ubiquitous feature of the atmosphere and influence clouds in multiple ways. Regarding cirrus clouds, many studies have emphasized the impact of wave-induced temperature fluctuations on the nucleation of ice crystals. This paper investigates the impact of the waves on the motion and distribution of ice particles, using the idealized 2-D framework of a monochromatic gravity wave. Contrary to previous studies, special attention is given to the impact of the wind field induced by the wave. Assuming no feedback of the ice on the water vapor content, theoretical and numerical analyses both show the existence of a wave-driven localization of ice crystals, where some ice particles remain confined in a specific phase of the wave. The precise location where the confinement occurs depends on the background relative humidity, but it is always characterized by a relative humidity near saturation and a positive vertical wind anomaly. Hence, the wave has an impact on the mean motion of the crystals and may reduce dehydration in cirrus by slowing down the sedimentation of the ice particles. The results also provide a new insight into the relation between relative humidity and ice crystals' presence. The wave-driven localization is consistent with temperature–cirrus relationships recently observed in the tropical tropopause layer (TTL) over the Pacific during the Airborne Tropical Tropopause EXperiment (ATTREX). It is argued that this effect may explain such observations. Finally, the impact of the described interaction on TTL cirrus dehydration efficiency is quantified using ATTREX observations of clouds and temperature lapse rate.

Description: We use the Weather Research and Forecast (WRF) model to simulate a large-scale tropical tropopause layer (TTL) cirrus in order to understand the formation and life cycle of the cloud. This cirrus event has been previously described through satellite observations by Taylor et al. (2011). Comparisons of the simulated and observed cirrus show a fair agreement and validate the reference simulation regarding cloud extension, location and life time. The validated simulation is used to understand the causes of cloud formation. It is shown that several cirrus clouds successively form in the region due to adiabatic cooling and large-scale uplift rather than from convective anvils. The structure of the uplift is tied to the equatorial response (equatorial wave excitation) to a potential vorticity intrusion from the midlatitudes. Sensitivity tests are then performed to assess the relative importance of the choice of the microphysics parameterization and of the initial and boundary conditions. The initial dynamical conditions (wind and temperature) essentially control the horizontal location and area of the cloud. However, the choice of the microphysics scheme influences the ice water content and the cloud vertical position. Last, the fair agreement with the observations allows to estimate the cloud impact in the TTL in the simulations. The cirrus clouds have a small but not negligible impact on the radiative budget of the local TTL. However, for this particular case, the cloud radiative heating does not significantly influence the simulated dynamics. This result is due to (1) the lifetime of air parcels in the cloud system, which is too short to significantly influence the dynamics, and (2) the fact that induced vertical motions would be comparable to or smaller than the typical mesoscale motions present. Finally, the simulation also provides an estimate of the vertical redistribution of water by the cloud and the results emphasize the importance in our case of both rehydration and dehydration in the vicinity of the cirrus.

Description: This paper investigates the accuracy of simulated long-duration super-pressure balloon trajectories in the lower stratosphere. The observed trajectories were made during the (tropical) Pre-Concordiasi and (polar) Concordiasi campaigns in 2010, while the simulated trajectories are computed using analyses and forecasts from the European Centre for Medium-Range Weather Forecasts (ECMWF) Integrated Forecast System model. In contrast with the polar stratosphere situation, modelling accurate winds in the tropical lower stratosphere remains challenging for numerical weather prediction systems. The accuracy of the simulated tropical trajectories are quantified with the operational products of 2010 and 2016 in order to understand the impact of model physics and vertical resolution improvements. The median errors in these trajectories are large (typically ≳ 250 km after 24 h), with a significant negative bias in longitude, for both model versions. In contrast, using analyses in which the balloon-borne winds have been assimilated reduces the median error in the balloon position after 24 h to ∼60 km. For future campaigns, we describe operational strategies that take advantage of the geographic distribution and the episodic nature of large error events to anticipate the amplitude of error in trajectory forecasts. We finally stress the importance of a high vertical resolution in the model, given the intense shears encountered in the tropical lower stratosphere.