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Synthesis of γ-Amino- and δ-Amino-Functionalised Ethers, Amines, or Silanes by Hydroaminomethylation of Heterofunctionalised Allylic Compounds (1999)

Rische, Thorsten ; Bärfacker, Lars ; Eilbracht, Peter

Weinheim : Wiley-Blackwell

Liebigs Annalen 1999 (1999), S. 653-660

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ISSN: 1434-193X

Keywords: Hydroaminomethylation ; Rhodium ; Catalysis ; Carbonylation ; Heterofunctionalised allylic compounds ; Chemistry ; General Chemistry

Source: Wiley InterScience Backfile Collection 1832-2000

Topics: Chemistry and Pharmacology

Notes: -Heterofunctionalised allylic ethers 1, silanes 5, and amines 9 are hydroformylated in the presence of primary or secondary amines 2 to form the corresponding γ-amino- and δ-amino-functionalised compounds. The rhodium(I)-catalysed reaction sequence proceeds by aldehyde formation and subsequent reductive amination to generate the corresponding functionalised secondary or tertiary amines. This selective one-pot hydroaminomethylation procedure establishes access to γ-amino- and δ-amino-functionalised ethers, amines or silanes with potential biological activity.

Additional Material: 4 Tab.

Type of Medium: Electronic Resource

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