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Semiclassical study of reactive scattering in a laser field - F + H2 + barred-h times omega times /1.06 microns/ system (1979)

George, T. F. ; Yuan, J.-M.

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Publication Date: 2019-06-27

Description: Semiclassical calculations of collinear F+H2(nu = 0) reactive and inelastic scattering in an Nd-glass laser field of various intensities are described. The decoupling approximation developed for the Miller-George theory is used for nonadiabatic transitions between the electronic-field surfaces, and special attention is paid to the choice of a proper coordinate system for applying the decoupling approximation. An increase in the total reaction probability and population ratio of the nu = 3 over nu = 2 vibrational state of HF occurs suddenly as the field intensity increases beyond 10 TW/sq cm. It is found that in a laser field the H2 molecule can be vibrationally excited while the F atom is electronically excited.

Keywords: LASERS AND MASERS

Type: Journal of Chemical Physics; 70; Jan. 15

Format: text

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