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Kinetics of the reaction of nitric oxide with hydrogen (1974)

Kruger, C. H. ; Flower, W. L. ; Hanson, R. K.

In: CASI

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Publication Date: 2019-06-27

Description: Mixtures of NO and H2 diluted in argon or krypton were heated by incident shock waves, and the infrared emission from the fundamental vibration-rotation band of NO at 5.3 microns was used to monitor the time-varying NO concentration. The reaction kinetics were studied in the temperature range 2400-4500 K using a shock-tube technique. The decomposition of nitric oxide behind the shock was found to be modeled well by a fifteen-reaction system. A principle result of the study was the determination of the rate constant for the reaction H + NO yields N + OH, which may be the rate-limiting step for NO removal in some combustion systems. Experimental values of k sub 1 were obtained for each test through comparisons of measured and numerically predicted NO profiles.

Keywords: INORGANIC AND PHYSICAL CHEMISTRY

Type: NASA-CR-141273

Format: application/pdf

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