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A simplified proof of the Kosloff–Rice theorem: Intramolecular quantum dynamics cannot be chaotic (1989)

Manz, J.

College Park, Md. : American Institute of Physics (AIP)

The Journal of Chemical Physics 91 (1989), S. 2190-2193

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ISSN: 1089-7690

Source: AIP Digital Archive

Topics: Physics , Chemistry and Pharmacology

Notes: The title theorem follows from formally equivalent time evolutions of the bounded systems' quantum wave function described by the Schrödinger equation, and regular classical trajectories described by corresponding Hamilton's equations. Instructive model applications include dynamics of molecules with time-dependent Hamiltonians, e.g., intramolecular vibrational energy redistributions, and state selective vibrational transitions induced by periodic sub-ps IR laser pulses.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1063/1.457027

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