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Non-Enzymatic Activation of Molecular Nitrogen (1969)

Henrici-Olivé, G. ; Olivé, S.

Weinheim : Wiley-Blackwell

Angewandte Chemie International Edition in English 8 (1969), S. 650-659

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ISSN: 0570-0833

Keywords: Activation ; Nitrogen fixation ; Nitrogen fixation ; Chemistry ; General Chemistry

Source: Wiley InterScience Backfile Collection 1832-2000

Topics: Chemistry and Pharmacology

Notes: Several transition metal complexes that can absorb nitrogen from the gas phase are now known. Some of the N2-metal complexes are stable enough to be isolated and their structure elucidated, the N2 molecule remaining chemically inert. In other cases reduction to N3- is possible, but the structure of the reactive intermediate N2-metal complex can be approached only by mechanistic studies. In the stable complexes the nitrogen is bound via a lone pair of electrons in the direction of the molecular axis (“end-on”), in the reducible complexes possibly “edge-on”.

Additional Material: 12 Ill.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1002/anie.196906501

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