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Modeling of sintering and redispersion of supported metal catalysts (1983)

Handa, P. K. ; Matthews, J. C.

Hoboken, NJ : Wiley-Blackwell

AIChE Journal 29 (1983), S. 717-725

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ISSN: 0001-1541

Keywords: Chemistry ; Chemical Engineering

Source: Wiley InterScience Backfile Collection 1832-2000

Topics: Chemistry and Pharmacology , Process Engineering, Biotechnology, Nutrition Technology

Notes: A model, which utilizes a Monte Carlo simulation, of the sintering and the redispersion of supported metal catalysts is presented and compared with experimental data from a Pt/Al2O3 system. The model is based on an atomic migration mechanism, but includes instantaneous diffusion and coalescence of crystallites of size 〈1 nm in reducing and inert atmospheres. It was found that behavior in reducing, oxidizing and inert atmospheres could be predicted.

Additional Material: 9 Ill.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1002/aic.690290504

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