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Influence of transport limitations on the kinetics of homopolymerization reactions (1995)

Oshanin, G. ; Moreau, M.

College Park, Md. : American Institute of Physics (AIP)

The Journal of Chemical Physics 102 (1995), S. 2977-2985

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ISSN: 1089-7690

Source: AIP Digital Archive

Topics: Physics , Chemistry and Pharmacology

Notes: We discuss the influence of transport limitations on the kinetics of homopolymerization reactions. We show that in the systems in which the polymer's diffusivity decreases faster than the first inverse power of its radius of gyration, the transport limitations represent the rate-controlling step and induce anomalous behavior of the characteristics of the process. For such systems we compute the evolution of the molecular weight distribution and its zeroth moment explicitly. © 1995 American Institute of Physics.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1063/1.468606

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