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Nanocrystal size dependence of the third-order nonlinear optical response of Cu:Al2O3 thin films (1999)

Ballesteros, J. M. ; Solis, J. ; Serna, R. ; [et al.]

Woodbury, NY : American Institute of Physics (AIP)

Applied Physics Letters 74 (1999), S. 2791-2793

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ISSN: 1077-3118

Source: AIP Digital Archive

Topics: Physics

Notes: Metal nanocomposite thin films formed by Cu nanocrystals embedded in an amorphous Al2O3 host have been synthesized by pulsed laser deposition. The mean nanocrystal diameter d was varied in the range 3.0±0.6 to 6±1 nm. The linear and nonlinear optical properties of the films were studied in the vicinity of the surface plasmon resonance and the size dependence of the third-order nonlinear optical susceptibility of the metal nanocrystals has been determined. The observed dependence (1/d3) indicates that in the studied diameter interval, the nonlinear response is due to quantum confinement effects in which the major contribution is associated with electronic intraband transitions. © 1999 American Institute of Physics.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1063/1.124015

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