ALBERT

Description: This paper describes the retrievals algorithm used to determine temperature and height from radiance measurements by the Microwave Limb Sounder on EOS Aura. MLS is a "limbscanning" instrument, meaning that it views the atmosphere along paths that do not intersect the surface - it actually looks forwards from the Aura satellite. This means that the temperature retrievals are for a "profile" of the atmosphere somewhat ahead of the satellite. Because of the need to view a finite sample of the atmosphere, the sample spans a box about 1.5km deep and several tens of kilometers in width; the optical characteristics of the atmosphere mean that the sample is representative of a tube about 200-300km long in the direction of view. The retrievals use temperature analyses from NASA's Goddard Earth Observing System, Version 5 (GEOS-5) data assimilation system as a priori states. The temperature retrievals are somewhat deperrde~zt on these a priori states, especially in the lower stratosphere. An important part of the validation of any new dataset involves comparison with other, independent datasets. A large part of this study is concerned with such comparisons, using a number of independent space-based measurements obtained using different techniques, and with meteorological analyses. The MLS temperature data are shown to have biases that vary with height, but also depend on the validation dataset. MLS data are apparently biased slightly cold relative to correlative data in the upper troposphere and slightly warm in the middle stratosphere. A warm MLS bias in the upper stratosphere may be due to a cold bias in GEOS-5 temperatures.

Description: The 2003-2004 Arctic winter was remarkable in the 40-year record of meteorological analyses. A major warming beginning in early January 2004 led to nearly two months of vortex disruption with high-latitude easterlies in the middle to lower stratosphere. The upper stratospheric vortex broke up in late December, but began to recover by early January, and in February and March was the strongest since regular observations began in 1979. The lower stratospheric vortex broke up in late January. Comparison with two previous years, 1984-1985 and 1986-1987, with prolonged mid-winter warming periods shows unique characteristics of the 2003-2004 warming period: The length of the vortex disruption, the strong and rapid recovery in the upper stratosphere, and the slow progression of the warming from upper to lower stratosphere. January 2004 zonal mean winds in the middle and lower stratosphere were over two standard deviations below average. Examination of past variability shows that the recent frequency of major stratospheric warmings (seven in the past six years) is unprecedented. Lower stratospheric temperatures were unusually high during six of the past seven years, with five having much lower than usual potential for PSC formation and ozone loss (nearly none in 1998-1999, 2001-2002 and 2003-2004, and very little in 1997-1998 and 2000-2001). Middle and upper stratospheric temperatures, however, were unusually low during and after February. The pattern of five of the last seven years with very low PSC potential would be expected to occur randomly once every approximately 850 years. This cluster of warm winters, immediately following a period of unusually cold winters, may have important implications for possible changes in interannual variability and for determination and attribution of trends in stratospheric temperatures and ozone.

Description: A major stratospheric sudden warming (SSW) in January 2009 was the strongest and most prolonged on record. Aura Microwave Limb Sounder (MLS) observations are used to provide an overview of dynamics and transport during the 2009 SSW, and to compare with the intense, long-lasting SSW in January 2006. The Arctic polar vortex split during the 2009 SSW, whereas the 2006 SSW was a vortex displacement event. Winds reversed to easterly more rapidly and reverted to westerly more slowly in 2009 than in 2006. More mixing of trace gases out of the vortex during the decay of the vortex fragments, and less before the fulfillment of major SSW criteria, was seen in 2009 than in 2006; persistent well-defined fragments of vortex and anticyclone air were more prevalent in 2009. The 2009 SSW had a more profound impact on the lower stratosphere than any previously observed SSW, with no significant recovery of the vortex in that region. The stratopause breakdown and subsequent reformation at very high altitude, accompanied by enhanced descent into a rapidly strengthening upper stratospheric vortex, were similar in 2009 and 2006. Many differences between 2006 and 2009 appear to be related to the different character of the SSWs in the two years.

Description: Localized rapid reductions in total ozone (miniholes), which were observed during the Airborne Antarctic Ozone Experiment, are studied with particular attention given to meteorological aspects. It is suggested that miniholes are forced by tropospheric weather features and that they are largely reversible distortions to the airflow around the vortex. The relationship between the miniholes and upper tropospheric and lower stratospheric synoptic-scale disturbances is studied. Trajectory calculations are presented which demonstrate the exchange of air from low latitudes with air from within the vortex, with the vortex air subsequently moving to lower latitudes.

Description: A program designed to study the Antarctic ozone hole using ER-2 high-altitude and DC-8 aircraft was conducted out of Punta Arenas, Chile during August 17-September 22, 1987. Graphs are presented of ozone and chlorine monoxide when crossing the boundary of the chemically perturbed region on August 23 and on September 21. Interpretations of ClO, H2O, and N2O measurements are presented, indicating ongoing diabetic cooling and advective poleward transport across the boundary.

Description: Results are presented on ozone measurements in the upper troposphere/lower stratosphere over Antarctica, obtained by NASA DC-8 aircraft during the August/September 1987 Airborne Antarctic Ozone Experiment. The ozone mixing ratios as high as several hundred ppbv were measured, but in all cases these ratios were observed in pockets of upper atmospheric air, both in the vicinity of and away from the location of the ozone hole. The background ozone values in the surrounding troposphere were typically in the range of 20-50 ppbv. Correlation of tropospheric ozone observations with the boundaries of the ozone hole differed in the course of the experiment. During the August 28 - September 2 flights, encounters with ozone-rich air were limited, and the background tropospheric ozone appeared to decrease beneath the hole. For the later flights, and as the ozone hole deepened, the ozone-rich air was frequently observed in the vicinity of the hole, and the average ozone values at the flight altitude were frequently higher than the background values.

Description: Measurements of the abundances of ozone over Antarctica in August and September 1987 obtained during the Airborne Antarctic Ozone Experiment are intercompared. These measurements of ozone concentrations and total column abundance were obtained by three satellite instruments, two IR and one UV column-measuring instruments aboard the DC-8, one in situ DC-8, and two in situ ER-2 instruments, an upward looking lidar aboard the DC-8, and ozone sondes from four sites in Antarctica. This paper presents a summary of the ozone data, using the data and accuracies given by the individual investigators in the individual papers in this issue, without any attempt to critically review or evaluate the data. In general, very good agreement (within about 10-20 percent, limited by natural variability) among the various techniques was found, with no systematic biases detected. These observations confirm the low ozone amounts reported in the Antarctic stratosphere.

Description: The ultraviolet earth radiance data from the backscatter ultraviolet experiment on Nimbus 4 have been inverted to infer ozone profiles using a single Rayleigh scattering model. Two methods of solution give essentially the same results. Comparison of these profiles with simultaneous rocket sounding data shows satisfactory agreement at low and middle latitudes. Vertical cross-sections of ozone mixing ratio along the orbital tracks indicate that while the gross characteristics of the ozone field above 10 mb are under photochemical control, the influence of atmospheric motions can be found up to the 4 mb level.

Description: Review of some of the procedures and results of the double monochromator and colinear photometer Nimbus-4 satellite experiment that measures ultraviolet terrestrial radiance, Lambert reflectivity of the lower boundary of the scattering atmosphere, and extraterrestrial solar irradiance. The experiment has produced nearly three years of almost continuous data which are being used to infer the high-level ozone distribution and total ozone on a global basis. The high-level ozone data have been verified by independent coincident rocket ozone soundings, and the total ozone values show good agreement with Dobson spectrophotometer determinations. An increase has been observed in equatorial radiance at 2550 A relative to 2900 A, which seems to indicate that the amount of ozone in the upper stratosphere is related to the eleven-year solar cycle.

Description: A new TOMS instrument (Total Ozone Mapping Spectrometer) was launched from the Plesetsk Cosomodrome, Russia on August 15, 1991. The purpose of the joint project between the U.S. and Russia was to continue the long-term record of ozone measurements from Nimbus-7/TOMS (launched in October 1978). Ozone data from the two satellites compare very closely. When the orbital positions were nearly the same, the comparison over the entire globe showed an offset of 2 percent with a standard deviation of 5 percent. Comparisons were made with several ground based M124 and Dobson stations showing good agreement in absolute value and with the day-to-day variations seen by the ground stations.

Description: Model simulations were used to investigate the seasonal and interannual behavior of ozone for different choices of initial odd nitrogen concentration in July and different assumptions on the heterogeneous reactions, with particular consideration given to the possible contribution of chlorine chemistry to the ozone hole phenomenon. The numerical experiments were selected based on the simulations of the observed trace gas concentrations during the Airborne Antarctic Ozone Experiment in 1987. In all cases considered, the catalytic cycle associated with the formation and photolysis of Cl2O2 could account for more than half of the photochemical removal of O3 within the Antarctic vortex through mid-September. The reaction of BrO with ClO, which accounts for 15-20 percent of O3 removal in the same period, tends to play a more important role toward the end of September, when the concentration of ClO is expected to decrease. No simple relationship was found between the increase in chlorine lavel and the interannual decrease in Antarctic O3.

Description: Data obtained with the total ozone mapping spectrometer (TOMS) onboard the Nimbus-7 satellite are presented. An attempt is made to relate and synthesize TOMS data with conventional radiosonde analyses and with midtropospheric moisture data available from the VISSR onboard the GOES. Case studies are described which relate the potential vorticity structure of the upper troposphere to the total ozone distribution as measured by TOMS. Cyclogenesis, frontogenesis, and the formation of severe weather outbreaks are then related to jet streaks and their characteristic ozone signature. It is shown that the primary maxima of ozone and potential vorticity are associated with cold advection and subsidence in the main upper-air trough as suggested earlier. The secondary maxima of the three quantities diagnosed in the present work appear in the left front quadrant of a jet streak, revealing the importance of transverse, secondary motions induced by a jet streak above the level of maximum winds in further modifying the potential vorticity and ozone structures.

Description: Microwave Limb Sounder and Sounding of the Atmosphere with Broadband Emission Radiometry data show the polar stratopause, usually higher than and separated from that at midlatitudes, dropping from 〈55-60 to near 30 km, and cooling dramatically in January 2006 during a major stratospheric sudden warming (SSW). After a nearly isothermal period, a cool stratopause reforms near 75 km in early February, then drops to 〈55 km and warms. The stratopause is separated in longitude as well as latitude, with lowest temperatures in the transition regions between higher and lower stratopauses. Operational assimilated meteorological analyses, which are not constrained by data at stratopause altitude, do not capture a secondary temperature maximum that overlies the stratopause or the very high stratopause that reforms after the SSW; they underestimate the stratopause altitude variation during the SSW. High-quality daily satellite temperature measurements are invaluable in improving our understanding of stratopause evolution and its representation in models and assimilation systems.

Description: High-energy proton data obtained by polar-orbiting satellite and several balloon flights are used to derive the spatial extent and ionization profiles of regions irradiated by the intense solar particle events (SPE) of August 1972. Backscattered ultraviolet ozone sensors on the Nimbus 4 satellite identified and tracked the polar ozone cavity created by particle ionization during the intense, ten-hour period of August 4, which persisted and rotated as a semirigid mass in an east-to-west direction during 53 days of continuous tracking. Time-dependent chemistry calculations have been performed to show the cause, magnitude, and temporal features of the ozone reduction. Attempts to verify the predicted temperature changes have been unsuccessful due to limitations in the temperature measurement techniques used.

Description: The ultraviolet earth radiance data from the Backscatter Ultraviolet Experiment on Nimbus 4 have been inverted to infer ozone profiles using a single Rayleigh scattering model. Two methods of solution give essentially the same results. Comparisons of these profiles with simultaneous rocket sounding data shows satisfactory agreement at low and middle latitudes. Vertical cross sections of ozone mixing ratio along the orbital tracks indicate that while the gross characteristics of the ozone field above 10 mb are under photochemical control, the influence of atmospheric motions can be found up to the 4 mb level.

Description: Simulations of deep tropical clouds by both cloud-resolving models (CRMs) and single-column models (SCMs) in the GEWEX Cloud System Study (GCSS) Working Group 4 (WG4; Precipitating Convective Cloud Systems), Case 2 (19-27 December 1992, TOGA-COARE IFA) have produced large differences in the mean heating and moistening rates (-1 to -5 K and -2 to 2 grams per kilogram respectively). Since the large-scale advective temperature and moisture "forcing" are prescribed for this case, a closer examination of two of the remaining external types of "forcing", namely radiative heating and air/sea hear and moisture transfer, are warranted. This paper examines the current radiation and surface flux of parameterizations used in the cloud models participating in the GCSS WG4, be executing the models "offline" for one time step (12 s) for a prescribed atmospheric state, then examining the surface and radiation fluxes from each model. The dynamic, thermodynamic, and microphysical fluids are provided by the GCE-derived model output for Case 2 during a period of very active deep convection (westerly wind burst). The surface and radiation fluxes produced from the models are then divided into prescribed convective, stratiform, and clear regions in order to examine the role that clouds play in the flux parameterizations. The results suggest that the differences between the models are attributed more to the surface flux parameterizations than the radiation schemes.

Description: The Backscatter Ultraviolet (BUV) experiment aboard the Nimbus-4 satellite is discussed. This double monochromator experiment measures ultraviolet terrestrial radiance at 12 discrete wavelengths between 2550 A and 3400 A. Approximately 100 scans covering a 230 kilometer square are made between terminator crossings on the daylight side of the earth. A colinear photometer channel with the same field of view is used to derive the Lambert reflectivity of the lower boundary of the scattering atmosphere. The extraterrestrial solar irradiance is measured at the northern terminator. The instrument has currently produced almost three years of nearly continuous data which are being used to infer the high-level ozone distribution and total ozone on a global basis. The high-level ozone data have been verified by independent coincident rocket ozone soundings, and the total ozone values show good agreement with Dobson spectrophotometer determinations as well as those made with the Infrared Interferometer Spectrometer also on Nimbus-4.

Description: Estimation of total ozone from Nimbus 4 satellite measurements of backscattered ultraviolet earth radiance

Description: Microwave Limb Sounder and Sounding of the Atmosphere with Broadband Emission Radiometry data provide the first opportunity to characterize the four-dimensional stratopause evolution throughout the life-cycle of a major stratospheric sudden warming (SSW). The polar stratopause, usually higher than that at midlatitudes, dropped by 30 km and warmed during development of a major "wave 1" SSW in January 2006, with accompanying mesospheric cooling. When the polar vortex broke down, the stratopause cooled and became ill-defined, with a nearly isothermal stratosphere. After the polar vortex started to recover in the upper stratosphere/lower mesosphere (USLM), a cool stratopause reformed above 75 km, then dropped and warmed; both the mesosphere above and the stratosphere below cooled at this time. The polar stratopause remained separated from that at midlatitudes across the core of the polar night jet. In the early stages of the SSW, the strongly tilted (westward with increasing altitude) polar vortex extended into the mesosphere, and enclosed a secondary temperature maximum extending westward and slightly equatorward from the highest altitude part of the polar stratopause over the cool stratopause near the vortex edge. The temperature evolution in the USLM resulted in strongly enhanced radiative cooling in the mesosphere during the recovery from the SSW, but significantly reduced radiative cooling in the upper stratosphere. Assimilated meteorological analyses from the European Centre for Medium-Range weather Forecasts (ECMWF) and Goddard Earth Observing System Version 5.0.1 (GEOS-5), which are not constrained by data at polar stratopause altitudes and have model tops near 80 km, could not capture the secondary temperature maximum or the high stratopause after the SSW; they also misrepresent polar temperature structure during and after the stratopause breakdown, leading to large biases in their radiative heating rates. ECMWF analyses represent the stratospheric temperature structure more accurately, suggesting a better representation of vertical motion; GEOS-5 analyses more faithfully describe stratopause level wind and wave amplitudes. The high-quality satellite temperature data used here provide the first daily, global, multiannual data sets suitable for assessing and, eventually, improving representation of the USLM in models and assimilation systems.

Description: The results of the ozone measurements taken during rocket-busted flights of the rocket ozonesonde Rocoz-A at the NASA Wallops Flight Facility from August 1983 to September 1985 are presented. Nineteen profiles were obtained using Rocoz-A and electrochemical concentration cell ozonesondes, standard U.S. meteorological radiosondes, and Super-Loki datasondes. The results were found to agree with the Krueger and Minzner (1976) midlatitude ozone model for the 1976 U.S. Standard Atmosphere.