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  • 04. Solid Earth::04.08. Volcanology::04.08.99. General or miscellaneous  (26)
  • 04. Solid Earth::04.08. Volcanology::04.08.07. Instruments and techniques  (21)
  • Arctic Ocean  (20)
  • Carbon cycle  (20)
  • American Geophysical Union  (80)
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  • 1
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    Radium inputs into the Arctic Ocean from rivers a basin‐wide estimate (2023)
    American Geophysical Union
    Details
    Publication Date: 2023-03-11
    Description: © The Author(s), 2022. This article is distributed under the terms of the Creative Commons Attribution License. The definitive version was published in Bullock, E., Kipp, L., Moore, W., Brown, K., Mann, P., Vonk, J., Zimov, N., & Charette, M. Radium inputs into the Arctic Ocean from rivers a basin‐wide estimate. Journal of Geophysical Research: Oceans, 127(9), (2022): e2022JC018964, https://doi.org/10.1029/2022jc018964.
    Description: Radium isotopes have been used to trace nutrient, carbon, and trace metal fluxes inputs from ocean margins. However, these approaches require a full accounting of radium sources to the coastal ocean including rivers. Here, we aim to quantify river radium inputs into the Arctic Ocean for the first time for 226Ra and to refine the estimates for 228Ra. Using new and existing data, we find that the estimated combined (dissolved plus desorbed) annual 226Ra and 228Ra fluxes to the Arctic Ocean are [7.0–9.4] × 1014 dpm y−1 and [15–18] × 1014 dpm y−1, respectively. Of these totals, 44% and 60% of the river 226Ra and 228Ra, respectively are from suspended sediment desorption, which were estimated from laboratory incubation experiments. Using Ra isotope data from 20 major rivers around the world, we derived global annual 226Ra and 228Ra fluxes of [7.4–17] × 1015 and [15–27] × 1015 dpm y−1, respectively. As climate change spurs rapid Arctic warming, hydrological cycles are intensifying and coastal ice cover and permafrost are diminishing. These river radium inputs to the Arctic Ocean will serve as a valuable baseline as we attempt to understand the changes that warming temperatures are having on fluxes of biogeochemically important elements to the Arctic coastal zone.
    Description: This study was a broad, collaborative effort that would not have been possible without contributions from numerous funding sources, including the National Science Foundation (NSF-0751525, NSF-1736277, NSF-1458305, NSF-1938873, NSF-2048067, NSF-2134865), the NERC-BMBF project CACOON [NE/R012806/1] (UKRI NERC) and BMBF-03F0806A, and an EU Starting Grant (THAWSOME-676982).
    Keywords: Radium isotopes ; Arctic Ocean ; River fluxes
    Repository Name: Woods Hole Open Access Server
    Type: Article
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  • 2
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    Sediments in sea ice drive the Canada Basin surface Mn maximum: insights from an Arctic Mn Ocean model (2023)
    American Geophysical Union
    Details
    Publication Date: 2023-02-28
    Description: Author Posting. © American Geophysical Union, 2022. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Global Biogeochemical Cycles 36(8), (2022): e2022GB007320, https://doi.org/10.1029/2022GB007320.
    Description: Biogeochemical cycles in the Arctic Ocean are sensitive to the transport of materials from continental shelves into central basins by sea ice. However, it is difficult to assess the net effect of this supply mechanism due to the spatial heterogeneity of sea ice content. Manganese (Mn) is a micronutrient and tracer which integrates source fluctuations in space and time while retaining seasonal variability. The Arctic Ocean surface Mn maximum is attributed to freshwater, but studies struggle to distinguish sea ice and river contributions. Informed by observations from 2009 IPY and 2015 Canadian GEOTRACES cruises, we developed a three-dimensional dissolved Mn model within a 1/12° coupled ocean-ice model centered on the Canada Basin and the Canadian Arctic Archipelago (CAA). Simulations from 2002 to 2019 indicate that annually, 87%–93% of Mn contributed to the Canada Basin upper ocean is released by sea ice, while rivers, although locally significant, contribute only 2.2%–8.5%. Downstream, sea ice provides 34% of Mn transported from Parry Channel into Baffin Bay. While rivers are often considered the main source of Mn, our findings suggest that in the Canada Basin they are less important than sea ice. However, within the shelf-dominated CAA, both rivers and sediment resuspension are important. Climate-induced disruption of the transpolar drift may reduce the Canada Basin Mn maximum and supply downstream. Other micronutrients found in sediments, such as Fe, may be similarly affected. These results highlight the vulnerability of the biogeochemical supply mechanisms in the Arctic Ocean and the subpolar seas to climatic changes.
    Description: This work was funded by the Natural Sciences and Engineering Research Council of Canada (NSERC) Climate Change and Atmospheric Research Grant: GEOTRACES (RGPCC 433848-12) and VITALS (RGPCC 433898), an NSERC Discovery Grant (RGPIN-2016-03865) to SEA, and by the University of British Columbia through a four year fellowship to BR. Computing resources were provided by Compute Canada (RRG 2648 RAC 2019, RRG 2969 RAC 2020, and RRG 1541 RAC 2021).
    Keywords: GEOTRACES ; Arctic Ocean ; Trace elements ; Canadian Arctic Archipelago ; Ocean modeling ; Micronutrients
    Repository Name: Woods Hole Open Access Server
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  • 3
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    The influence of ocean topography on the upwelling of carbon in the Southern Ocean (2023)
    American Geophysical Union
    Details
    Publication Date: 2023-02-17
    Description: Author Posting. © American Geophysical Union, 2021. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Geophysical Research Letters 48(19), (2021): e2021GL095088, https://doi.org/10.1029/2021GL095088.
    Description: The physical circulation of the Southern Ocean sets the surface concentration and thus air-sea exchange of CO2. However, we have a limited understanding of the three-dimensional circulation that brings deep carbon-rich waters to the surface. Here, we introduce and analyze a novel high-resolution ocean model simulation with active biogeochemistry and online Lagrangian particle tracking. We focus our attention on a subset of particles with high dissolved inorganic carbon (DIC) that originate below 1,000 m and eventually upwell into the near-surface layer (upper 200 m). We find that 71% of the DIC-enriched water upwelling across 1,000 m is concentrated near topographic features, which occupy just 33% of the Antarctic Circumpolar Current. Once particles upwell to the near-surface layer, they exhibit relatively uniform pCO2 levels and DIC decorrelation timescales, regardless of their origin. Our results show that Southern Ocean bathymetry plays a key role in delivering carbon-rich waters to the surface.
    Description: Riley X. Brady was supported by the Department of Energy's Computational Science Graduate Fellowship (DE-FG02-97ER25308), and particularly benefited from the fellowship's summer practicum at Los Alamos National Lab. Nicole S. Lovenduski and Riley X. Brady were further supported by the U.S. Department of Energy Biological and Environmental Research program (DE-SC0022243) and by the National Science Foundation (NSF-PLR 1543457; NSF-OCE 1924636; NSF-OCE 1752724; NSF-OCE 1558225). Mathew E. Maltrud and Phillip J. Wolfram were supported as part of the Energy Exascale Earth System Model (E3SM) project, funded by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research. This research used resources provided by the Los Alamos National Laboratory Institutional Computing Program, which is supported by the U.S. Department of Energy National Nuclear Security Administration under Contract No. 89233218CNA000001.
    Keywords: Southern Ocean ; Carbon cycle ; Upwelling ; Lagrangian modeling ; Ocean biogeochemistry ; Climate modeling
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  • 4
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    Tephra sedimentation during the 2010 Eyjafjallajökull eruption (Iceland) from deposit, radar, and satellite observations (2012)
    American Geophysical Union
    Details
    Publication Date: 2023-01-16
    Description: The April–May 2010 eruption of the Eyjafjallajökull volcano (Iceland) was characterized by a nearly continuous injection of tephra into the atmosphere that affected various economic sectors in Iceland and caused a global interruption of air traffic. Eruptive activity during 4–8 May 2010 was characterized based on short-duration physical parameters in order to capture transient eruptive behavior of a long-lasting eruption (i.e., total grain-size distribution, erupted mass, and mass eruption rate averaged over 30 min activity). The resulting 30 min total grain-size distribution based on both ground and Meteosat Second Generation-Spinning Enhanced Visible and Infrared Imager (MSG-SEVIRI) satellite measurements is characterized by Mdphi of about 2 and a fine-ash content of about 30 wt %. The accumulation rate varied by 2 orders of magnitude with an exponential decay away from the vent, whereas Mdphi shows a linear increase until about 18 km from the vent, reaching a plateau of about 4.5 between 20 and 56 km. The associated mass eruption rate is between 0.6 and 1.2 × 105 kg s−1. In situ sampling showed how fine ash mainly fell as aggregates of various typologies. About 5 to 9 wt % of the erupted mass remained in the cloud up to 1000 km from the vent, suggesting that nearly half of the ash 〉7 settled as aggregates within the first 60 km. Particle sphericity and shape factor varied between 0.4 and 1 with no clear correlation to the size and distance from vent. Our experiments also demonstrate how satellite retrievals and Doppler radar grain-size detection can provide a real-time description of the source term but for a limited particle-size range.
    Description: Published
    Description: B12202
    Description: 1.5. TTC - Sorveglianza dell'attività eruttiva dei vulcani
    Description: JCR Journal
    Description: reserved
    Keywords: MSG-SEVIRI, PLUDIX ; particle aggregation ; settling velocity ; tephra deposits ; weak plumes ; 04. Solid Earth::04.04. Geology::04.04.06. Rheology, friction, and structure of fault zones ; 04. Solid Earth::04.08. Volcanology::04.08.07. Instruments and techniques
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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  • 5
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    Shallow calcium carbonate cycling in the North Pacific Ocean (2022)
    American Geophysical Union
    Details
    Publication Date: 2022-11-06
    Description: Author Posting. © American Geophysical Union, 2022. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Global Biogeochemical Cycles 36(5), (2022): e2022GB007388, https://doi.org/10.1029/2022gb007388.
    Description: The cycling of biologically produced calcium carbonate (CaCO3) in the ocean is a fundamental component of the global carbon cycle. Here, we present experimental determinations of in situ coccolith and foraminiferal calcite dissolution rates. We combine these rates with solid phase fluxes, dissolved tracers, and historical data to constrain the alkalinity cycle in the shallow North Pacific Ocean. The in situ dissolution rates of coccolithophores demonstrate a nonlinear dependence on saturation state. Dissolution rates of all three major calcifying groups (coccoliths, foraminifera, and aragonitic pteropods) are too slow to explain the patterns of both CaCO3 sinking flux and alkalinity regeneration in the North Pacific. Using a combination of dissolved and solid-phase tracers, we document a significant dissolution signal in seawater supersaturated for calcite. Driving CaCO3 dissolution with a combination of ambient saturation state and oxygen consumption simultaneously explains solid-phase CaCO3 flux profiles and patterns of alkalinity regeneration across the entire N. Pacific basin. We do not need to invoke the presence of carbonate phases with higher solubilities. Instead, biomineralization and metabolic processes intimately associate the acid (CO2) and the base (CaCO3) in the same particles, driving the coupled shallow remineralization of organic carbon and CaCO3. The linkage of these processes likely occurs through a combination of dissolution due to zooplankton grazing and microbial aerobic respiration within degrading particle aggregates. The coupling of these cycles acts as a major filter on the export of both organic and inorganic carbon to the deep ocean.
    Description: This work was funded by NSF OCE-1220301 to W.B., NSF OCE-1220600 to J.F.A., and startup funding for A.V.S.
    Description: 2022-11-06
    Keywords: Calcium carbonate ; Dissolution ; Carbon cycle
    Repository Name: Woods Hole Open Access Server
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  • 6
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    Hurricanes enhance labile carbon export to the deep ocean (2019)
    American Geophysical Union
    Details
    Publication Date: 2022-10-27
    Description: Author Posting. © American Geophysical Union, 2019. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Geophysical Research Letters 46 (2019): 10484–10494, doi:10.1029/2019GL083719.
    Description: Tropical cyclones (hurricanes) generate intense surface ocean cooling and vertical mixing resulting in nutrient upwelling into the photic zone and episodic phytoplankton blooms. However, their influence on the deep ocean remains unknown. Here we present evidence that hurricanes also impact the ocean's biological pump by enhancing export of labile organic material to the deep ocean. In October 2016, Category 3 Hurricane Nicole passed over the Bermuda Time Series site in the oligotrophic NW Atlantic Ocean. Following Nicole's passage, particulate fluxes of lipids diagnostic of fresh phytodetritus, zooplankton, and microbial biomass increased by 30–300% at 1,500 m depth and 30–800% at 3,200 m depth. Mesopelagic suspended particles following Nicole were also enriched in phytodetrital material and in zooplankton and bacteria lipids, indicating particle disaggregation and a deepwater ecosystem response. Predicted climate‐induced increases in hurricane frequency and/or intensity may significantly alter ocean biogeochemical cycles by increasing the strength of the biological pump.
    Description: This work and the Oceanic Flux Program time series were supported by the National Science Foundation Chemical Oceanography Program Grant OCE 1536644. The Bermuda Atlantic Time Series and Hydrostation S time series were supported by NSF Grants OCE 1756105 and OCE 1633125, respectively. We acknowledge the contributions of BATS technicians with CTD and pigment analyses. We sincerely thank the officers and crew of R/V Atlantic Explorer (Bermuda Institute of Ocean Sciences) for their expert assistance on the cruises. The data used in this study are listed in the figures, tables, and references, and are also available in the NSF's Biological and Chemical Oceanography Data Management Office (BCO‐DMO, https://doi.org/10.1575/1912/bco‐dmo.775902.1).
    Description: 2020-02-16
    Keywords: Hurricanes ; Carbon cycle ; North Atlantic Ocean ; Deep ocean ; Particle fluxes ; Lipid biomarkers
    Repository Name: Woods Hole Open Access Server
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  • 7
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    Deepening of the winter mixed layer in the Canada Basin, Arctic Ocean over 2006-2017 (2019)
    American Geophysical Union
    Details
    Publication Date: 2022-10-26
    Description: Author Posting. © American Geophysical Union, 2019. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Journal of Geophysical Research-Oceans 124(7), (2019): 4618-4630, doi: 10.1029/2019JC014940.
    Description: The Arctic Ocean mixed layer interacts with the ice cover above and warmer, nutrient‐rich waters below. Ice‐Tethered Profiler observations in the Canada Basin of the Arctic Ocean over 2006–2017 are used to investigate changes in mixed layer properties. In contrast to decades of shoaling since at least the 1980s, the mixed layer deepened by 9 m from 2006–2012 to 2013–2017. Deepening resulted from an increase in mixed layer salinity that also weakened stratification at the base of the mixed layer. Vertical mixing alone can explain less than half of the observed change in mixed layer salinity, and so the observed increase in salinity is inferred to result from changes in freshwater accumulation via changes to ice‐ocean circulation or ice melt/growth and river runoff. Even though salinity increased, the shallowest density surfaces deepened by 5 m on average suggesting that Ekman pumping over this time period remained downward. A deeper mixed layer with weaker stratification has implications for the accessibility of heat and nutrients stored in the upper halocline. The extent to which the mixed layer will continue to deepen appears to depend primarily on the complex set of processes influencing freshwater accumulation.
    Description: We gratefully acknowledge J. Toole for helpful conversations. S. Cole was supported by the National Science Foundation under grant PLR‐1602926 and J. Stadler by the Woods Hole Oceanographic Institution Summer Student Fellowship program. Profile data are available via the Ice‐Tethered Profiler program website: http://whoi.edu/itp. SSM/I ice concentration data were downloaded from the National Snow and Ice Data Center.
    Description: 2019-12-22
    Keywords: Arctic Ocean ; Mixed layer ; Freshwater
    Repository Name: Woods Hole Open Access Server
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  • 8
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    Changes in the arctic ocean carbon cycle with diminishing ice cover (2020)
    American Geophysical Union
    Details
    Publication Date: 2022-10-26
    Description: © The Author(s), 2020. This article is distributed under the terms of the Creative Commons Attribution License. The definitive version was published in DeGrandpre, M., Evans, W., Timmermans, M., Krishfield, R., Williams, B., & Steele, M. Changes in the arctic ocean carbon cycle with diminishing ice cover. Geophysical Research Letters, 47(12), (2020): e2020GL088051, doi:10.1029/2020GL088051.
    Description: Less than three decades ago only a small fraction of the Arctic Ocean (AO) was ice free and then only for short periods. The ice cover kept sea surface pCO2 at levels lower relative to other ocean basins that have been exposed year round to ever increasing atmospheric levels. In this study, we evaluate sea surface pCO2 measurements collected over a 6‐year period along a fixed cruise track in the Canada Basin. The measurements show that mean pCO2 levels are significantly higher during low ice years. The pCO2 increase is likely driven by ocean surface heating and uptake of atmospheric CO2 with large interannual variability in the contributions of these processes. These findings suggest that increased ice‐free periods will further increase sea surface pCO2, reducing the Canada Basin's current role as a net sink of atmospheric CO2.
    Description: This research was made possible by grants from the NSF Arctic Observing Network program (ARC‐1107346, PLR‐1302884, PLR‐1504410, and OPP‐1723308). In addition, M. S. was supported by ONR (Grant 00014‐17‐1‐2545), NASA (Grant NNX16AK43G), and NSF (Grants PLR‐1503298 and OPP‐1751363).
    Keywords: Arctic Ocean ; Ice concentration ; Seawater CO2 ; Interannual variability ; Canada Basin ; Shipboard CO2 measurements
    Repository Name: Woods Hole Open Access Server
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  • 9
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    Shelf-basin interactions and water mass residence times in the western Arctic Ocean: Insights provided by radium isotopes (2019)
    American Geophysical Union
    Details
    Publication Date: 2022-10-26
    Description: Author Posting. © American Geophysical Union, 2019. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Journal of Geophysical Research-Oceans 124(5), (2019): 3279-3297, doi: 10.1029/2019JC014988.
    Description: Radium isotopes are produced through the decay of thorium in sediments and are soluble in seawater; thus, they are useful for tracing ocean boundary‐derived inputs to the ocean. Here we apply radium isotopes to study continental inputs and water residence times in the Arctic Ocean, where land‐ocean interactions are currently changing in response to rising air and sea temperatures. We present the distributions of radium isotopes measured on the 2015 U.S. GEOTRACES transect in the Western Arctic Ocean and combine this data set with historical radium observations in the Chukchi Sea and Canada Basin. The highest activities of radium‐228 were observed in the Transpolar Drift and the Chukchi shelfbreak jet, signaling that these currents are heavily influenced by interactions with shelf sediments. The ventilation of the halocline with respect to inputs from the Chukchi shelf occurs on time scales of ≤19–23 years. Intermediate water ventilation time scales for the Makarov and Canada Basins were determined to be ~20 and 〉30 years, respectively, while deep water residence times in these basins were on the order of centuries. The radium distributions and residence times described in this study serve as a baseline for future studies investigating the impacts of climate change on the Arctic Ocean.
    Description: We thank the captain and crew of the USCGC Healy (HLY1502) and the chief scientists D. Kadko and W. Landing for coordinating a safe and successful expedition. We thank the members of the pump team, P. Lam, E. Black, S. Pike, X. Yang, and M. Heller for their assistance with sample collection and for their unfailingly positive attitudes during this 65‐day expedition. We also appreciate sampling assistance from P. Aguilar and M. Stephens, and MATLAB assistance from B. Corlett, A. Pacini, P. Lin, and M. Li. The radium data from the HLY1502 expedition are available through the Biological & Chemical Oceanography Data Management Office (https://www.bco‐dmo.org/dataset/718440) and the radium measurements from the SHEBA, AWS‐2000, and SBI expeditions can be found in the supporting information. This work was funded by NSF awards OCE‐1458305 to M.A.C., OCE‐1458424 to W.S.M., and PLR‐1504333 to R.S.P. This research was conducted with Government support under and awarded by a DoD, Air Force Office of Scientific Research, National Defense Science and Engineering Graduate (NDSEG) Fellowship awarded to L.E.K., 32 CFR 168a.
    Description: 2019-10-26
    Keywords: Radium ; Arctic Ocean ; GEOTRACES ; Chukchi shelf
    Repository Name: Woods Hole Open Access Server
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  • 10
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    On the origin of aged sedimentary organic matter along a river-shelf-deep ocean transect (2020)
    American Geophysical Union
    Details
    Publication Date: 2022-10-26
    Description: Author Posting. © American Geophysical Union, 2019. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Journal of Geophysical Research: Biogeosciences 124(8), (2019): 2582-2594, doi: 10.1029/2019JG005107.
    Description: To assess the influences of carbon sources and transport processes on the 14C age of organic matter (OM) in continental margin sediments, we examined a suite of samples collected along a river‐shelf‐deep ocean transect in the East China Sea (ECS). Ramped pyrolysis‐oxidiation was conducted on suspended particulate matter in the Yangtze River and on surface sediments from the ECS shelf and northern Okinawa Trough. 14C ages were determined on OM decomposition products within different temperature windows. These measurements suggest that extensive amounts of pre‐old (i.e., millennial age) organic carbon (OC) are subject to degradation within and beyond the Yangtze River Delta, and this process is accompanied by an exchange of terrestrial and marine OM. These results, combined with fatty acid concentration data, suggest that both the nature and extent of OM preservation/degradation as well as the modes of transport influence the 14C ages of sedimentary OM. Additionally, we find that the age of (thermally) refractory OC increases during across‐shelf transport and that the age offset between the lowest and highest temperature OC decomposition fractions also increases along the shelf‐to‐trough transect. Amplified interfraction spread or 14C heterogeneity is the greatest in the Okinawa Trough. Aged sedimentary OM across the transect may be a consequence of several reasons including fossil OC input, selective degradation of younger OC, hydrodynamic sorting processes, and aging during lateral transport. Consequently, each of them should be considered in assessing the 14C results of sedimentary OM and its implications for the carbon cycle and interpretation of sedimentary records.
    Description: This study was supported by Doc. Mobility Fellowship (P1EZP2_159064; R. B.) from the Swiss National Science Foundation (SNSF). This study was also supported by SNF “CAPS‐LOCK” project 200021_140850 (T. I. E.), by the National Natural Science Foundation of China (NSFC; grants 41520104009 and 41630966, M. Z.), and by the “111” project (B13030). We are grateful for support of the NOSAMS staff in the execution of this project. We also appreciate the assistance from Yushuang Zhang (Ocean University of China) at NOSAMS and members of the Laboratory for Ion Beam Physics at ETH Zurich for AMS measurements. We acknowledge Lei Xing, Haidong Zhang, Guodong Song, Meng Yu, Yonghao Jia, and Shanshan Duan (Ocean University of China) for sampling assistance on the cruises. Assistance at sea by the crews of R/V Dongfanghong II and R/V Hakuhu Maru is also acknowledged. Readers can access or find the data from figures and tables in the supporting information.
    Keywords: Radiocarbon ; Carbon cycle ; Sediments ; Organic carbon ; Hydrodynamic processes
    Repository Name: Woods Hole Open Access Server
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