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  • Artikel  (948.124)
  • American Chemical Society  (545.496)
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  • 1
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    Comparison of Raman and Fourier Transform Infrared Spectroscopy for the Quantification of Microplastics in the Aquatic Environment (2018)
    American Chemical Society
    In:  EPIC3Environmental Science & Technology, American Chemical Society, 52(22), pp. 13279-13288
    Details
    Publikationsdatum: 2019-03-13
    Repository-Name: EPIC Alfred Wegener Institut
    Materialart: Article , isiRev
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  • 2
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    Glucose as a potential chemical marker for ice nucleating activity in Arctic seawater samples. (2019)
    American Chemical Society
    In:  EPIC3Environmental Science & Technology, American Chemical Society, 53, pp. 8747-8756, ISSN: 1520-5851
    Details
    Publikationsdatum: 2020-06-04
    Beschreibung: Recent studies pointed to a high ice nucleating activity (INA) in the Arctic sea surface microlayer (SML). However, related chemical information is still sparse. In the present study, INA and free glucose concentrations were quantified in Arctic SML and bulk water samples from the marginal ice zone, the ice-free ocean, melt ponds, and open waters within the ice pack. T50 (defining INA) ranged from −17.4 to −26.8 °C. Glucose concentrations varied from 0.6 to 51 μg/L with highest values in the SML from the marginal ice zone and melt ponds (median 16.3 and 13.5 μg/L) and lower values in the SML from the ice pack and the ice-free ocean (median 3.9 and 4.0 μg/L). Enrichment factors between the SML and the bulk ranged from 0.4 to 17. A positive correlation was observed between free glucose concentration and INA in Arctic water samples (T50(°C) = (−25.6 ± 0.6) + (0.15 ± 0.04)·Glucose(μg/L), RP = 0.66, n = 74). Clustering water samples based on phytoplankton pigment composition resulted in robust but different correlations within the four clusters (RP between 0.67 and 0.96), indicating a strong link to phytoplankton-related processes. Since glucose did not show significant INA itself, free glucose may serve as a potential tracer for INA in Arctic water samples.
    Repository-Name: EPIC Alfred Wegener Institut
    Materialart: Article , isiRev
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  • 3
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    A Method for Continuous 239Pu Determinations in Arctic and Antarctic Ice Cores (2016)
    American Chemical Society
    In:  EPIC3Environmental Science and Technology, American Chemical Society, 50(13), pp. 7066-7073, ISSN: 0013936X
    Details
    Publikationsdatum: 2016-10-12
    Beschreibung: Atmospheric nuclear weapons testing (NWT) resulted in the injection of plutonium (Pu) into the atmosphere and subsequent global deposition. We present a new method for continuous semiquantitative measurement of 239Pu in ice cores, which was used to develop annual records of fallout from NWT in ten ice cores from Greenland and Antarctica. The 239Pu was measured directly using an inductively coupled plasma-sector field mass spectrometer, thereby reducing analysis time and increasing depth-resolution with respect to previous methods. To validate this method, we compared our one year averaged results to published 239Pu records and other records of NWT. The 239Pu profiles from the Arctic ice cores reflected global trends in NWT and were in agreement with discrete Pu profiles from lower latitude ice cores. The 239Pu measurements in the Antarctic ice cores tracked low latitude NWT, consistent with previously published discrete records from Antarctica. Advantages of the continuous 239Pu measurement method are (1) reduced sample preparation and analysis time; (2) no requirement for additional ice samples for NWT fallout determinations; (3) measurements are exactly coregistered with all other chemical, elemental, isotopic, and gas measurements from the continuous analytical system; and (4) the long half-life means the 239Pu record is stable through time.
    Repository-Name: EPIC Alfred Wegener Institut
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  • 4
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    Contribution of Atmospheric Advection to the Amplified Winter Warming in the Arctic North Atlantic Region (2017)
    Hindawi
    In:  EPIC3Advances in Meteorology, Hindawi, (492862), ISSN: 1687-9317
    Details
    Publikationsdatum: 2020-03-05
    Beschreibung: Arctic Amplification of climate warming is caused by various feedback processes in the atmosphere-ocean-ice system and yields the strongest temperature increase during winter in the Arctic North Atlantic region. In our study, we attempt to quantify the advective contribution to the observed atmospheric warming in the Svalbard area. Based on radiosonde measurements from Ny-Ålesund, a strong dependence of the tropospheric temperature on the synoptic flow direction is revealed. Using FLEXTRA backward trajectories, an increase of advection from the lower latitude Atlantic region towards Ny-Ålesund is found that is attributed to a change in atmospheric circulation patterns. We find that about one-quarter (0.45 K per decade) of the observed atmospheric winter near surface warming trend in the North Atlantic region of the Arctic (2 K per decade) is due to increased advection of warm and moist air from the lower latitude Atlantic region, affecting the entire troposphere.
    Repository-Name: EPIC Alfred Wegener Institut
    Materialart: Article , isiRev
    Format: application/pdf
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  • 5
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    Growth of Ice Crystals in the Presence of Type III Antifreeze Protein (2018)
    American Chemical Society
    In:  EPIC3Crystal Growth & Design, American Chemical Society, 18, pp. 2563-2571
    Details
    Publikationsdatum: 2018-04-23
    Beschreibung: The morphology and growth kinetics of ice single crystals in aqueous solutions of type III antifreeze protein (AFP-III) have been studied in detail over a range of AFP-III concentrations and supercoolings. In pure water, the shape of ice crystals changes from the circular disklike to planar dendritic with increasing supercooling. In AFP-III solutions, ice crystals in the form of faceted plates, irregular dendrites with polygonized tips, and needles appear with increasing supercooling and AFP-III concentration. The growth rate of ice crystals in the crystallographic a direction is 2 orders of magnitude higher than that in the c direction. AFP-III molecules cause the stoppage of the growth of the prismatic and basal faces at low supercoolings. When supercooling exceeds the critical value, AFP-III favors the acceleration of the growth in both a and c directions. The observed behavior of AFP-III is explained in terms of the Cabrera-Vermilyea pinning model and the specificity of the dissipation of latent heat from the growing crystals with different shapes.
    Repository-Name: EPIC Alfred Wegener Institut
    Materialart: Article , isiRev
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  • 6
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    The Marsili Volcanic Seamount (Southern Tyrrhenian Sea): A Potential Offshore Geothermal Resource (2015)
    Molecular Diversity Preservation International
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    Publikationsdatum: 2017-04-04
    Beschreibung: Italy has a strong geothermal potential for power generation, although, at present, the only two geothermal fields being exploited are Larderello-Travale/Radicondoli and Mt. Amiata in the Tyrrhenian pre-Apennine volcanic district of Southern Tuscany. A new target for geothermal exploration and exploitation in Italy is represented by the Southern Tyrrhenian submarine volcanic district, a geologically young basin (Upper Pliocene-Pleistocene) characterised by tectonic extension where many seamounts have developed. Heat-flow data from that area show significant anomalies comparable to those of onshore geothermal fields. Fractured basaltic rocks facilitate seawater infiltration and circulation of hot water chemically altered by rock/water interactions, as shown by the widespread presence of hydrothermal deposits. The persistence of active hydrothermal activity is consistently shown by many different sources of evidence, including: heat-flow data, gravity and magnetic anomalies, widespread presence of hydrothermal-derived gases (CO2, CO, CH4), 3He/4He isotopic ratios, as well as broadband OBS/H seismological information, which demonstrates persistence of volcano-tectonic events and High Frequency Tremor (HFT). The Marsili and Tyrrhenian seamounts are thus an important—and likely long-lasting-renewable energy resource. This raises the possibility of future development of the world’s first offshore geothermal power plant.
    Beschreibung: Published
    Beschreibung: 4068-4086
    Beschreibung: 3A. Ambiente Marino
    Beschreibung: JCR Journal
    Beschreibung: open
    Schlagwort(e): Marsili seamount ; hydrothermal circulation ; geothermal resource ; 04. Solid Earth::04.04. Geology::04.04.04. Marine geology
    Repository-Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Materialart: article
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  • 7
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    Geochemical and Isotopic Characterisation of Actual Lacustrine Sediments from the Hydrothermal Lake Specchio di Venere, Pantelleria Island (Italy) (2016)
    Hindawi
    Details
    Publikationsdatum: 2017-04-04
    Beschreibung: Hydrothermal lakes are a very common feature in volcanic environments, and among these lake Specchio di Venere (Pantelleria island, Italy) has attracted the interest of several researchers due to its peculiar characteristics. With the aim of improving the knowledge of its mineralogy, our work pointed out the characterisation of the bottom lake sediments. We collected and analysed 5 sediments cores around the shoreline, determining the mineralogical phases, concentration of major, minor, and trace elements, and the isotopic composition of carbon and oxygen in the carbonate phases. Our findings remarked a general compositional homogeneity in both the vertical and horizontal distribution of mineral phases, with the exception of peculiar geological niches connoted by biological and hydrothermal activities.
    Beschreibung: Published
    Beschreibung: ID 8414581
    Beschreibung: 4V. Vulcani e ambiente
    Beschreibung: JCR Journal
    Beschreibung: open
    Schlagwort(e): Pantelleria ; Sediments ; Geochemistry ; 04. Solid Earth::04.04. Geology::04.04.08. Sediments: dating, processes, transport
    Repository-Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Materialart: article
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  • 8
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    Tools for the microbiome : nano and beyond (2016)
    American Chemical Society
    Details
    Publikationsdatum: 2022-05-25
    Beschreibung: © American Chemical Society, 2015. This article is posted here by permission of American Chemical Society; copying and redistribution for non-commercial research and education purposes only. The definitive version was published in ACS Nano 10 (2016): 6-37, doi:10.1021/acsnano.5b07826.
    Beschreibung: The microbiome presents great opportunities for understanding and improving the world around us and elucidating the interactions that compose it. The microbiome also poses tremendous challenges for mapping and manipulating the entangled networks of interactions among myriad diverse organisms. Here, we describe the opportunities, technical needs, and potential approaches to address these challenges, based on recent and upcoming advances in measurement and control at the nanoscale and beyond. These technical needs will provide the basis for advancing the largely descriptive studies of the microbiome to the theoretical and mechanistic understandings that will underpin the discipline of microbiome engineering. We anticipate that the new tools and methods developed will also be more broadly useful in environmental monitoring, medicine, forensics, and other areas.
    Beschreibung: This research was supported by the Office of Naval Research Grant #N000141410051 (P.S.W., G.C.L.W., and T.Y.), the Genomic Science Program of the U.S. DOE-OBER,
    Repository-Name: Woods Hole Open Access Server
    Materialart: Article
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  • 9
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    Photochemical oxidation of oil reduced the effectiveness of aerial dispersants applied in response to the Deepwater Horizon spill (2018)
    American Chemical Society
    Details
    Publikationsdatum: 2022-05-25
    Beschreibung: Author Posting. © American Chemical Society, 2018. This is an open access article published under an ACS AuthorChoice License. The definitive version was published in Environmental Science and Technology Letters 5 (2018): 226–231, doi:10.1021/acs.estlett.8b00084.
    Beschreibung: Chemical dispersants are one of many tools used to mitigate the overall environmental impact of oil spills. In principle, dispersants break up floating oil into small droplets that disperse into the water column where they are subject to multiple fate and transport processes. The effectiveness of dispersants typically decreases as oil weathers in the environment. This decrease in effectiveness is often attributed to evaporation and emulsification, with the contribution of photochemical weathering assumed to be negligible. Here, we aim to test this assumption using Macondo well oil released during the Deepwater Horizon spill as a case study. Our results indicate that the effects of photochemical weathering on Deepwater Horizon oil properties and dispersant effectiveness can greatly outweigh the effects of evaporative weathering. The decrease in dispersant effectiveness after light exposure was principally driven by the decreased solubility of photo-oxidized crude oil residues in the solvent system that comprises COREXIT EC9500A. Kinetic modeling combined with geospatial analysis demonstrated that a considerable fraction of aerial applications targeting Deepwater Horizon surface oil had low dispersant effectiveness. Collectively, the results of this study challenge the paradigm that photochemical weathering has a negligible impact on the effectiveness of oil spill response and provide critical insights into the “window of opportunity” to apply chemical dispersants in response to oil spills in sunlit waters.
    Beschreibung: This work was supported, in part, by National Science Foundation Grant OCE-1333148, Gulf of Mexico Research Initiative Grants 015, SA 16-30, the DEEP-C consortium, and the Clark Family Foundation, Inc. EPA funding was provided to R.N.C. from the Oil Spill Liability Trust Fund.
    Repository-Name: Woods Hole Open Access Server
    Materialart: Article
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  • 10
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    Land subsidence, Ground Fissures and Buried Faults: InSAR Monitoring of Ciudad Guzmán (Jalisco, Mexico) (2015)
    Molecular Diversity Preservation International
    Details
    Publikationsdatum: 2017-04-04
    Beschreibung: We study land subsidence processes and the associated ground fissuring, affecting an active graben filled by thick unconsolidated deposits by means of InSAR techniques and fieldwork. On 21 September 2012, Ciudad Guzmán (Jalisco, Mexico) was struck by ground fissures of about 1.5 km of length, causing the deformation of the roads and the propagation of fissures in adjacent buildings. The field survey showed that fissures alignment is coincident with the escarpments produced on 19 September 1985, when a strong earthquake with magnitude 8.1 struck central Mexico. In order to detect and map the spatio-temporal features of the processes that led to the 2012 ground fissures, we applied InSAR multitemporal techniques to process ENVISAT-ASAR and RADARSAT-2 satellite SAR images acquired between 2003 and 2012. We detect up to 20 mm/year of subsidence of the northwestern part of Ciudad Guzmán. These incremental movements are consistent with the ground fissures observed in 2012. Based on interferometric results, field data and 2D numerical model, we suggest that ground deformations and fissuring are due to the presence of areal subsidence correlated with variable sediment thickness and differential compaction, partly driven by the exploitation of the aquifers and controlled by the distribution and position of buried faults.
    Beschreibung: Published
    Beschreibung: 8610-8630
    Beschreibung: 6A. Monitoraggio ambientale, sicurezza e territorio
    Beschreibung: JCR Journal
    Beschreibung: open
    Schlagwort(e): InSAR ; ground subsidence ; buried faults ; ground fissuring ; 04. Solid Earth::04.01. Earth Interior::04.01.02. Geological and geophysical evidences of deep processes
    Repository-Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Materialart: article
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