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  • Articles  (39)
  • Hindawi  (39)
  • American Chemical Society (ACS)
  • American Meteorological Society
  • American Physical Society
  • American Physical Society (APS)
  • Institute of Physics
  • Oxford University Press
  • Public Library of Science
  • 2020-2024
  • 2015-2019  (39)
  • 1985-1989
  • 1945-1949
  • 1940-1944
  • 2017  (39)
  • 1945
  • 1942
  • Journal of Combustion  (15)
  • International Journal of Electrochemistry  (7)
  • 149161
  • 165403
  • Energy, Environment Protection, Nuclear Power Engineering  (27)
  • Electrical Engineering, Measurement and Control Technology  (12)
  • Mathematics
  • Geosciences
  • Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
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  • Articles  (39)
Source
Publisher
  • Hindawi  (39)
  • American Chemical Society (ACS)
  • American Meteorological Society
  • American Physical Society
  • American Physical Society (APS)
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  • 2020-2024
  • 2015-2019  (39)
  • 1985-1989
  • 1945-1949
  • 1940-1944
Year
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  • Energy, Environment Protection, Nuclear Power Engineering  (27)
  • Electrical Engineering, Measurement and Control Technology  (12)
  • Mathematics
  • Geosciences
  • Agriculture, Forestry, Horticulture, Fishery, Domestic Science, Nutrition
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  • 1
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    Study of the Radical Chain Mechanism of Hydrocarbon Oxidation for In Situ Combustion Process (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: Despite the abundance of in situ combustion models of oil oxidation, many of the effects are still beyond consideration. For example, until now, initial stages of oxidation were not considered from a position of radical chain process. This is a serious difficulty for the simulation of oil recovery process that involves air injection. To investigate the initial stages of oxidation, the paper considers the sequence of chemical reactions, including intermediate short-living compounds and radicals. We have attempted to correlate the main stages of the reaction with areas of heat release observed in the experiments. The system of differential equations based on the equations of oxidation reactions was solved. Time dependence of peroxides formation and start of heat release is analytically derived for the initial stages. We have considered the inhibition of initial oxidation stages by aromatic oil compounds and have studied the induction time in dependence on temperature. Chain ignition criteria for paraffins and crude oil in presence of core samples were obtained. The calculation results are compared with the stages of oxidation that arise by high-pressure differential scanning calorimetry. According to experimental observations we have determined which reactions are important for the process and which can be omitted or combined into one as insignificant.
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  • 2
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    Decomposition Characteristics and Kinetics of Microalgae in N2 and CO2 Atmospheres by a Thermogravimetry (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: The thermal degradation characteristics of microalgae were investigated in highly purified N2 and CO2 atmospheres by a thermogravimetric analysis (TGA) under different heating rates (10, 20, and 40°C/min). The results indicated that the total residual mass in CO2 atmosphere (16.86%) was less than in N2 atmosphere (23.12%); in addition, the kinetics of microalgae in N2 and CO2 atmospheres could be described by the pseudo bicomponent separated state model (PBSM) and pseudo-multi-component overall model (PMOM), respectively. The kinetic parameters calculated by Coats-Redfern method showed that, in CO2 atmosphere, the apparent activation energy () of microalgae was between 9.863 and 309.381 kJ mol−1 and the reaction order () was varied from 1.1 to 7. The kinetic parameters of the second stage in CO2 atmosphere were quite similar to those in N2 atmosphere.
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  • 3
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    Effects of Injection Rate Profile on Combustion Process and Emissions in a Diesel Engine (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: When multi-injection is implemented in diesel engine via high pressure common rail injection system, changed interval between injection pulses can induce variation of injection rate profile for sequential injection pulse, though other control parameters are the same. Variations of injection rate shape which influence the air-fuel mixing and combustion process will be important for designing injection strategy. In this research, CFD numerical simulations using KIVA-3V were conducted for examining the effects of injection rate shape on diesel combustion and emissions. After the model was validated by experimental results, five different shapes (including rectangle, slope, triangle, trapezoid, and wedge) of injection rate profiles were investigated. Modeling results demonstrate that injection rate shape can have obvious influence on heat release process and heat release traces which cause different combustion process and emissions. It is observed that the baseline, rectangle (flat), shape of injection rate can have better balance between NOx and soot emissions than the other investigated shapes. As wedge shape brings about the lowest NOx emissions due to retarded heat release, it produces the highest soot emissions among the five shapes. Trapezoid shape has the lowest soot emissions, while its NOx is not the highest one. The highest NOx emissions were produced by triangle shape due to higher peak injection rate.
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  • 4
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    Online Monitoring of Copper Damascene Electroplating Bath by Voltammetry: Selection of Variables for Multiblock and Hierarchical Chemometric Analysis of Voltammetric Data (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: The Real Time Analyzer (RTA) utilizing DC- and AC-voltammetric techniques is an in situ, online monitoring system that provides a complete chemical analysis of different electrochemical deposition solutions. The RTA employs multivariate calibration when predicting concentration parameters from a multivariate data set. Although the hierarchical and multiblock Principal Component Regression- (PCR-) and Partial Least Squares- (PLS-) based methods can handle data sets even when the number of variables significantly exceeds the number of samples, it can be advantageous to reduce the number of variables to obtain improvement of the model predictions and better interpretation. This presentation focuses on the introduction of a multistep, rigorous method of data-selection-based Least Squares Regression, Simple Modeling of Class Analogy modeling power, and, as a novel application in electroanalysis, Uninformative Variable Elimination by PLS and by PCR, Variable Importance in the Projection coupled with PLS, Interval PLS, Interval PCR, and Moving Window PLS. Selection criteria of the optimum decomposition technique for the specific data are also demonstrated. The chief goal of this paper is to introduce to the community of electroanalytical chemists numerous variable selection methods which are well established in spectroscopy and can be successfully applied to voltammetric data analysis.
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  • 5
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    Removal of Pb, Cu, Cd, and Zn Present in Aqueous Solution Using Coupled Electrocoagulation-Phytoremediation Treatment (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: This study presents the results of a coupled electrocoagulation-phytoremediation treatment for the reduction of copper, cadmium, lead, and zinc, present in aqueous solution. The electrocoagulation was carried out in a batch reactor using aluminum electrodes in parallel arrangement; the optimal conditions were current density of 8 mA/cm2 and operating time of 180 minutes. For phytoremediation the macrophytes, Typha latifolia L., were used during seven days of treatment. The results indicated that the coupled treatment reduced metal concentrations by 99.2% Cu, 81.3% Cd, and 99.4% Pb, while Zn increased due to the natural concentrations of the plant used.
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  • 6
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    Reduction of the Electrode Overpotential of the Oxygen Evolution Reaction by Electrode Surface Modification (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: Metal–air batteries exhibit high potential for grid-scale energy storage because of their high theoretical energy density, their abundance in the earth’s crust, and their low cost. In these batteries, the oxygen evolution reaction (OER) occurs on the air electrode during charging. This study proposes a method for improving the OER electrode performance. The method involves sequentially depositing a Ni underlayer, Sn whiskers, and a Ni protection layer on the metal mesh. Small and uniform gas bubbles form on the Ni/Sn/Ni mesh, leading to low overpotential and a decrease in the overall resistance of the OER electrode. The results of a simulated life cycle test indicate that the Ni/Sn/Ni mesh has a life cycle longer than 1,300 cycles when it is used as the OER electrode in 6 M KOH.
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  • 7
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    Thermodynamics of Lithium Intercalation in Randomly Oriented High Graphene Carbon (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: This paper covers details of systematic investigation of the thermodynamics (entropy and enthalpy) of intercalation associated with lithium ion in a structurally novel carbon, called Randomly Oriented High Graphene (ROHG) carbon and graphite. Equilibrated OCV (Open Circuit Voltage) versus temperature relationship is investigated to determine the thermodynamic changes with the lithium intercalation. ROHG carbon shows entropy of 9.36 J·mol−1·K−1 and shows no dependency on the inserted lithium concentration. Graphite shows initial entropy of 84.27 J·mol−1·K−1 and shows a strong dependence on lithium concentration. ROHG carbon (from −90.85 kJ mol−1 to −2.88 kJ mol−1) shows gradual change in the slope of enthalpy versus lithium ion concentration plot compared to graphite (−48.98 kJ mol−1 to 1.84 kJ mol−1). The study clearly shows that a lower amount of energy is required for the lithium ion intercalation into the ROHG structure compared to graphite structure. Randomly oriented graphene platelet cluster structure of ROHG carbon makes it easier for the intercalation or deintercalation of lithium ion. The ease of intercalation and the small cluster structure of ROHG as opposed to the long linear platelet structure of graphite lead to higher rates of the charge-discharge process for ROHG, when used as an electrode material in electrochemical applications.
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  • 8
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    Status of Biomass Derived Carbon Materials for Supercapacitor Application (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: Environmental concerns and energy security uncertainties associated with fossil fuels have driven the world to shift to renewable energy sources. However, most renewable energy sources with exception of hydropower are intermittent in nature and thus need storage systems. Amongst various storage systems, supercapacitors are the promising candidates for energy storage not only in renewable energies but also in hybrid vehicles and portable devices due to their high power density. Supercapacitor electrodes are almost invariably made of carbon derived from biomass. Several reviews had been focused on general carbon materials for supercapacitor electrode. This review is focused on understanding the extent to which different types of biomasses have been used as porous carbon materials for supercapacitor electrodes. It also details hydrothermal microwave assisted, ionothermal, and molten salts carbonization as techniques of synthesizing activated carbon from biomasses as well as their characteristics and their impacts on electrochemical performance.
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  • 9
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    Adiabatic Fixed-Bed Gasification of Colombian Coffee Husk Using Air-Steam Blends for Partial Oxidation (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: The increasing energy consumption, mostly supplied by fossil fuels, has motivated the research and development of alternative fuel technologies to decrease the humanity’s dependence on fossil fuels, which leads to pollution of natural sources. Small-scale biomass gasification, using air-steam blends for partial oxidation, is a good alternative since biomass is a neutral carbon feedstock for sustainable energy generation. This research presents results obtained from an experimental study on coffee husk (CH) gasification, using air-steam blends for partial oxidation in a 10 kW fixed-bed gasifier. Parametric studies on equivalence ratio (ER) (1.53
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  • 10
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    The Role of Liquid Fuels Channel Configuration on the Combustion inside Cylindrical Mesoscale Combustor (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: This research intended to investigate combustion of liquid fuel in 3.5 mm inner diameter quartz glass tube mesocombustor, based on liquid film evaporation by using heat recirculation. The mesocombustor has a copper section for heating and evaporating the liquid fuel. In mesocombustor type A, the fuel was glided through the narrow canal in the copper wall while the air was glided through the axial of combustor. The flame could only be successfully stabilized in high-ratio equivalent ranging from to , due to the gap without combustion reaction caused by high air-fuel mixture over the limits of flame stability. Mesocombustor type B, which has annulus-shaped canal, could shift the flame stability from to ; however, it also narrowed the limits of flame stability due to the wall cooling. In mesocombustor type C, both liquid fuel and air were glided through the annulus-shaped canal in the copper wall to fix the fuel evaporation and air mixture. The flame of type C was successfully stabilized, from to wider than types A and B. The flame of type C mesocombustor is circle-shaped and fitted to cross section of mesocombustor, but it still has thin gap without any flames due to thermal quenching by the wall.
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  • 11
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    Small Engines as Bottoming Cycle Steam Expanders for Internal Combustion Engines (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: Heat recovery bottoming cycles for internal combustion engines have opened new avenues for research into small steam expanders (Stobart and Weerasinghe, 2006). Dependable data for small steam expanders will allow us to predict their suitability as bottoming cycle engines and the fuel economy achieved by using them as bottoming cycles. Present paper is based on results of experiments carried out on small scale Wankel and two-stroke reciprocating engines as air expanders and as steam expanders. A test facility developed at Sussex used for measurements is comprised of a torque, power and speed measurements, electronic actuation of valves, synchronized data acquisition of pressure, and temperatures of steam and inside of the engines for steam and internal combustion cycles. Results are presented for four engine modes, namely, reciprocating engine in uniflow steam expansion mode and air expansion mode and rotary Wankel engine in steam expansion mode and air expansion mode. The air tests will provide base data for friction and motoring effects whereas steam tests will tell how effective the engines will be in this mode. Results for power, torque, and diagrams are compared to determine the change in performance from air expansion mode to steam expansion mode.
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  • 12
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    Parametric Study to Improve Subpixel Accuracy of Nitric Oxide Tagging Velocimetry with Image Preprocessing (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: Biacetyl phosphorescence has been the commonly used molecular tagging velocimetry (MTV) technique to investigate in-cylinder flow evolution and cycle-to-cycle variations in an optical engine. As the phosphorescence of biacetyl tracer deteriorates in the presence of oxygen, nitrogen was adopted as the working medium in the past. Recently, nitrous oxide MTV technique was employed to measure the velocity profile of an air jet. The authors here plan to investigate the potential application of this technique for engine flow studies. A possible experimental setup for this task indicated different permutations of image signal-to-noise ratio (SNR) and laser line width. In the current work, a numerical analysis is performed to study the effect of these two factors on displacement error in MTV image processing. Also, several image filtering techniques were evaluated and the performance of selected filters was analyzed in terms of enhancing the image quality and minimizing displacement errors. The flow displacement error without image preprocessing was observed to be inversely proportional to SNR and directly proportional to laser line width. The mean filter resulted in the smallest errors for line widths smaller than 9 pixels. The effect of filter size on subpixel accuracy showed that error levels increased as the filter size increased.
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  • 13
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    An Experimental Insight into the Smoldering-Flaming Transition Phenomenon (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: Transitional phenomena of smoldering combustion over thin solid fuels are investigated. An experimental setup was upraised and implications of both smoldering and flaming external heat sources are estimated. Incense sticks were used as potential fuel and external smoldering heat source along with a fixed candle flame. The role of key controlling parameters, namely, separation distance and number of external heat sources in horizontal and vertical direction, was extensively examined. The surfacing issues of enclosure effect and the external heat sources orientation are addressed. The study primarily aims at understanding the feasibility and spontaneity of transition owing to external heat sources (both flaming and smoldering). Forward heat transfer significantly deviates qualitatively and quantitatively with varying separation distance in both directions. Number of external heat sources intensifies the transition phenomenon in smoldering combustion. With practical considerations, external heat sources arrangement and orientation have substantial effect on the combustion process.
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  • 14
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    Influence of Advanced Injection Timing and Fuel Additive on Combustion, Performance, and Emission Characteristics of a DI Diesel Engine Running on Plastic Pyrolysis Oil (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: This paper presents the investigation of engine optimisation when plastic pyrolysis oil (PPO) is used as the primary fuel of a direct injection diesel engine. Our previous investigation revealed that PPO is a promising fuel; however the results suggested that control parameters should be optimised in order to obtain a better engine performance. In the present work, the injection timing was advanced, and fuel additives were utilised to overcome the issues experienced in the previous work. In addition, spray characteristics of PPO were investigated in comparison with diesel to provide in-depth understanding of the engine behaviour. The experimental results on advanced injection timing (AIT) showed reduced brake thermal efficiency and increased carbon monoxide, unburned hydrocarbons, and nitrogen oxides emissions in comparison to standard injection timing. On the other hand, the addition of fuel additive resulted in higher engine efficiency and lower exhaust emissions. Finally, the spray tests revealed that the spray tip penetration for PPO is faster than diesel. The results suggested that AIT is not a preferable option while fuel additive is a promising solution for long-term use of PPO in diesel engines.
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  • 15
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    Experimental Study of the Combustion of Kerosene and Binary Surrogate in the Model Combustion Chamber (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: The purpose of this paper is to conduct experimental research of hazardous substance emissions at the simulated combustion chamber output. The experiment was carried in a simulated combustion chamber. The combustion chamber included a burner device; a liquid fuel feed system; and a flame tube with two rows of mixing holes and one row of cooling holes. The combustion chamber operation mode was = 0.435, = 423 K, and the atmospheric pressure. The liquid fuel burn rate was 0.77 g/s. The pressure ratio in the combustion chamber remained constant at = 3%. Two types of fuel were used: aviation kerosene of Russia’s TS-1 brand and the fuel surrogate was n-decane mixture (C10H22) with benzene additions (C6H6). The benzene additions were 5% through 30% (n-decane/benzene: 95/5, 90/10, 85/15, 80/20, 75/25, and 70/30).
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  • 16
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    Advanced Engine Flows and Combustion (2017)
    Hindawi
    Details
    Publication Date: 2017
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  • 17
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    Numerical Investigation of Critical Velocity in Reduced Scale Tunnel Fire with Constant Heat Release Rate (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: When a fire occurs in a tunnel in the absence of sufficient air supply, large quantities of smoke are generated, filling the vehicles and any space available around them. Hot gases and smoke produced by fire form layers flowing towards extremities of the tunnel which may interfere with person’s evacuation and firefighter’s intervention. This paper carries out a numerical simulation of an unexpected fire occurring in a one-way tunnel in order to investigate for the critical velocity of the ventilation airflow; this one is defined as the minimum velocity able to maintain the combustion products in the downstream side of tunnel. The computation is performed successively with two types of fuels representing a large and a small heat release rate, owing to an open source CFD code called ISIS, which is specific to fires in confined and nonconfined environments. It is indicated that, after several computations of full-scale fires of 43.103 and 19.103 kJ/kg as heat release rate, the velocities satisfying the criterion of healthy environment in the upstream side of the tunnel are 1.34 m/s and 1.12 m/s, respectively.
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  • 18
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    Removal of Pb, Cu, Cd, and Zn Present in Aqueous Solution Using Coupled Electrocoagulation-Phytoremediation Treatment (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: This study presents the results of a coupled electrocoagulation-phytoremediation treatment for the reduction of copper, cadmium, lead, and zinc, present in aqueous solution. The electrocoagulation was carried out in a batch reactor using aluminum electrodes in parallel arrangement; the optimal conditions were current density of 8 mA/cm2 and operating time of 180 minutes. For phytoremediation the macrophytes, Typha latifolia L., were used during seven days of treatment. The results indicated that the coupled treatment reduced metal concentrations by 99.2% Cu, 81.3% Cd, and 99.4% Pb, while Zn increased due to the natural concentrations of the plant used.
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  • 19
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    Online Monitoring of Copper Damascene Electroplating Bath by Voltammetry: Selection of Variables for Multiblock and Hierarchical Chemometric Analysis of Voltammetric Data (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: The Real Time Analyzer (RTA) utilizing DC- and AC-voltammetric techniques is an in situ, online monitoring system that provides a complete chemical analysis of different electrochemical deposition solutions. The RTA employs multivariate calibration when predicting concentration parameters from a multivariate data set. Although the hierarchical and multiblock Principal Component Regression- (PCR-) and Partial Least Squares- (PLS-) based methods can handle data sets even when the number of variables significantly exceeds the number of samples, it can be advantageous to reduce the number of variables to obtain improvement of the model predictions and better interpretation. This presentation focuses on the introduction of a multistep, rigorous method of data-selection-based Least Squares Regression, Simple Modeling of Class Analogy modeling power, and, as a novel application in electroanalysis, Uninformative Variable Elimination by PLS and by PCR, Variable Importance in the Projection coupled with PLS, Interval PLS, Interval PCR, and Moving Window PLS. Selection criteria of the optimum decomposition technique for the specific data are also demonstrated. The chief goal of this paper is to introduce to the community of electroanalytical chemists numerous variable selection methods which are well established in spectroscopy and can be successfully applied to voltammetric data analysis.
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  • 20
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    Adiabatic Fixed-Bed Gasification of Colombian Coffee Husk Using Air-Steam Blends for Partial Oxidation (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: The increasing energy consumption, mostly supplied by fossil fuels, has motivated the research and development of alternative fuel technologies to decrease the humanity’s dependence on fossil fuels, which leads to pollution of natural sources. Small-scale biomass gasification, using air-steam blends for partial oxidation, is a good alternative since biomass is a neutral carbon feedstock for sustainable energy generation. This research presents results obtained from an experimental study on coffee husk (CH) gasification, using air-steam blends for partial oxidation in a 10 kW fixed-bed gasifier. Parametric studies on equivalence ratio (ER) (1.53
    Print ISSN: 2090-1968
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    Topics: Energy, Environment Protection, Nuclear Power Engineering
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  • 21
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    The Role of Liquid Fuels Channel Configuration on the Combustion inside Cylindrical Mesoscale Combustor (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: This research intended to investigate combustion of liquid fuel in 3.5 mm inner diameter quartz glass tube mesocombustor, based on liquid film evaporation by using heat recirculation. The mesocombustor has a copper section for heating and evaporating the liquid fuel. In mesocombustor type A, the fuel was glided through the narrow canal in the copper wall while the air was glided through the axial of combustor. The flame could only be successfully stabilized in high-ratio equivalent ranging from to , due to the gap without combustion reaction caused by high air-fuel mixture over the limits of flame stability. Mesocombustor type B, which has annulus-shaped canal, could shift the flame stability from to ; however, it also narrowed the limits of flame stability due to the wall cooling. In mesocombustor type C, both liquid fuel and air were glided through the annulus-shaped canal in the copper wall to fix the fuel evaporation and air mixture. The flame of type C was successfully stabilized, from to wider than types A and B. The flame of type C mesocombustor is circle-shaped and fitted to cross section of mesocombustor, but it still has thin gap without any flames due to thermal quenching by the wall.
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  • 22
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    Experimental Study of the Combustion of Kerosene and Binary Surrogate in the Model Combustion Chamber (2017)
    Hindawi
    Details
    Publication Date: 2017
    Description: The purpose of this paper is to conduct experimental research of hazardous substance emissions at the simulated combustion chamber output. The experiment was carried in a simulated combustion chamber. The combustion chamber included a burner device; a liquid fuel feed system; and a flame tube with two rows of mixing holes and one row of cooling holes. The combustion chamber operation mode was = 0.435, = 423 K, and the atmospheric pressure. The liquid fuel burn rate was 0.77 g/s. The pressure ratio in the combustion chamber remained constant at = 3%. Two types of fuel were used: aviation kerosene of Russia’s TS-1 brand and the fuel surrogate was n-decane mixture (C10H22) with benzene additions (C6H6). The benzene additions were 5% through 30% (n-decane/benzene: 95/5, 90/10, 85/15, 80/20, 75/25, and 70/30).
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  • 23
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    Status of Biomass Derived Carbon Materials for Supercapacitor Application (2017)
    Hindawi
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    Publication Date: 2017-01-01
    Description: Environmental concerns and energy security uncertainties associated with fossil fuels have driven the world to shift to renewable energy sources. However, most renewable energy sources with exception of hydropower are intermittent in nature and thus need storage systems. Amongst various storage systems, supercapacitors are the promising candidates for energy storage not only in renewable energies but also in hybrid vehicles and portable devices due to their high power density. Supercapacitor electrodes are almost invariably made of carbon derived from biomass. Several reviews had been focused on general carbon materials for supercapacitor electrode. This review is focused on understanding the extent to which different types of biomasses have been used as porous carbon materials for supercapacitor electrodes. It also details hydrothermal microwave assisted, ionothermal, and molten salts carbonization as techniques of synthesizing activated carbon from biomasses as well as their characteristics and their impacts on electrochemical performance.
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    Online Monitoring of Copper Damascene Electroplating Bath by Voltammetry: Selection of Variables for Multiblock and Hierarchical Chemometric Analysis of Voltammetric Data (2017)
    Hindawi
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    Publication Date: 2017-01-01
    Description: The Real Time Analyzer (RTA) utilizing DC- and AC-voltammetric techniques is an in situ, online monitoring system that provides a complete chemical analysis of different electrochemical deposition solutions. The RTA employs multivariate calibration when predicting concentration parameters from a multivariate data set. Although the hierarchical and multiblock Principal Component Regression- (PCR-) and Partial Least Squares- (PLS-) based methods can handle data sets even when the number of variables significantly exceeds the number of samples, it can be advantageous to reduce the number of variables to obtain improvement of the model predictions and better interpretation. This presentation focuses on the introduction of a multistep, rigorous method of data-selection-based Least Squares Regression, Simple Modeling of Class Analogy modeling power, and, as a novel application in electroanalysis, Uninformative Variable Elimination by PLS and by PCR, Variable Importance in the Projection coupled with PLS, Interval PLS, Interval PCR, and Moving Window PLS. Selection criteria of the optimum decomposition technique for the specific data are also demonstrated. The chief goal of this paper is to introduce to the community of electroanalytical chemists numerous variable selection methods which are well established in spectroscopy and can be successfully applied to voltammetric data analysis.
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    Thermodynamics of Lithium Intercalation in Randomly Oriented High Graphene Carbon (2017)
    Hindawi
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    Publication Date: 2017-01-01
    Description: This paper covers details of systematic investigation of the thermodynamics (entropy and enthalpy) of intercalation associated with lithium ion in a structurally novel carbon, called Randomly Oriented High Graphene (ROHG) carbon and graphite. Equilibrated OCV (Open Circuit Voltage) versus temperature relationship is investigated to determine the thermodynamic changes with the lithium intercalation. ROHG carbon shows entropy of 9.36 J·mol−1·K−1 and shows no dependency on the inserted lithium concentration. Graphite shows initial entropy of 84.27 J·mol−1·K−1 and shows a strong dependence on lithium concentration. ROHG carbon (from −90.85 kJ mol−1 to −2.88 kJ mol−1) shows gradual change in the slope of enthalpy versus lithium ion concentration plot compared to graphite (−48.98 kJ mol−1 to 1.84 kJ mol−1). The study clearly shows that a lower amount of energy is required for the lithium ion intercalation into the ROHG structure compared to graphite structure. Randomly oriented graphene platelet cluster structure of ROHG carbon makes it easier for the intercalation or deintercalation of lithium ion. The ease of intercalation and the small cluster structure of ROHG as opposed to the long linear platelet structure of graphite lead to higher rates of the charge-discharge process for ROHG, when used as an electrode material in electrochemical applications.
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    Advanced Engine Flows and Combustion (2017)
    Hindawi
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    Publication Date: 2017-01-01
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    Topics: Energy, Environment Protection, Nuclear Power Engineering
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    An Experimental Insight into the Smoldering-Flaming Transition Phenomenon (2017)
    Hindawi
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    Publication Date: 2017-01-01
    Description: Transitional phenomena of smoldering combustion over thin solid fuels are investigated. An experimental setup was upraised and implications of both smoldering and flaming external heat sources are estimated. Incense sticks were used as potential fuel and external smoldering heat source along with a fixed candle flame. The role of key controlling parameters, namely, separation distance and number of external heat sources in horizontal and vertical direction, was extensively examined. The surfacing issues of enclosure effect and the external heat sources orientation are addressed. The study primarily aims at understanding the feasibility and spontaneity of transition owing to external heat sources (both flaming and smoldering). Forward heat transfer significantly deviates qualitatively and quantitatively with varying separation distance in both directions. Number of external heat sources intensifies the transition phenomenon in smoldering combustion. With practical considerations, external heat sources arrangement and orientation have substantial effect on the combustion process.
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    Experimental Study of the Combustion of Kerosene and Binary Surrogate in the Model Combustion Chamber (2017)
    Hindawi
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    Publication Date: 2017-01-01
    Description: The purpose of this paper is to conduct experimental research of hazardous substance emissions at the simulated combustion chamber output. The experiment was carried in a simulated combustion chamber. The combustion chamber included a burner device; a liquid fuel feed system; and a flame tube with two rows of mixing holes and one row of cooling holes. The combustion chamber operation mode was φ = 0.435, Tpreheat = 423 K, and the atmospheric pressure. The liquid fuel burn rate was 0.77 g/s. The pressure ratio in the combustion chamber remained constant at ΔP = 3%. Two types of fuel were used: aviation kerosene of Russia’s TS-1 brand and the fuel surrogate was n-decane mixture (C10H22) with benzene additions (C6H6). The benzene additions were 5% through 30% (n-decane/benzene: 95/5, 90/10, 85/15, 80/20, 75/25, and 70/30).
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    Numerical Investigation of Critical Velocity in Reduced Scale Tunnel Fire with Constant Heat Release Rate (2017)
    Hindawi
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    Publication Date: 2017-01-01
    Description: When a fire occurs in a tunnel in the absence of sufficient air supply, large quantities of smoke are generated, filling the vehicles and any space available around them. Hot gases and smoke produced by fire form layers flowing towards extremities of the tunnel which may interfere with person’s evacuation and firefighter’s intervention. This paper carries out a numerical simulation of an unexpected fire occurring in a one-way tunnel in order to investigate for the critical velocity of the ventilation airflow; this one is defined as the minimum velocity able to maintain the combustion products in the downstream side of tunnel. The computation is performed successively with two types of fuels representing a large and a small heat release rate, owing to an open source CFD code called ISIS, which is specific to fires in confined and nonconfined environments. It is indicated that, after several computations of full-scale fires of 43.103 and 19.103 kJ/kg as heat release rate, the velocities satisfying the criterion of healthy environment in the upstream side of the tunnel are 1.34 m/s and 1.12 m/s, respectively.
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    Small Engines as Bottoming Cycle Steam Expanders for Internal Combustion Engines (2017)
    Hindawi
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    Publication Date: 2017-01-01
    Description: Heat recovery bottoming cycles for internal combustion engines have opened new avenues for research into small steam expanders (Stobart and Weerasinghe, 2006). Dependable data for small steam expanders will allow us to predict their suitability as bottoming cycle engines and the fuel economy achieved by using them as bottoming cycles. Present paper is based on results of experiments carried out on small scale Wankel and two-stroke reciprocating engines as air expanders and as steam expanders. A test facility developed at Sussex used for measurements is comprised of a torque, power and speed measurements, electronic actuation of valves, synchronized data acquisition of pressure, and temperatures of steam and inside of the engines for steam and internal combustion cycles. Results are presented for four engine modes, namely, reciprocating engine in uniflow steam expansion mode and air expansion mode and rotary Wankel engine in steam expansion mode and air expansion mode. The air tests will provide base data for friction and motoring effects whereas steam tests will tell how effective the engines will be in this mode. Results for power, torque, and p-V diagrams are compared to determine the change in performance from air expansion mode to steam expansion mode.
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    Adiabatic Fixed-Bed Gasification of Colombian Coffee Husk Using Air-Steam Blends for Partial Oxidation (2017)
    Hindawi
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    Publication Date: 2017-01-01
    Description: The increasing energy consumption, mostly supplied by fossil fuels, has motivated the research and development of alternative fuel technologies to decrease the humanity’s dependence on fossil fuels, which leads to pollution of natural sources. Small-scale biomass gasification, using air-steam blends for partial oxidation, is a good alternative since biomass is a neutral carbon feedstock for sustainable energy generation. This research presents results obtained from an experimental study on coffee husk (CH) gasification, using air-steam blends for partial oxidation in a 10 kW fixed-bed gasifier. Parametric studies on equivalence ratio (ER) (1.53 〈 ER 〈 6.11) and steam-fuel (SF) ratio (0.23 〈 SF 〈 0.89) were carried out. The results show that increasing both SF and ER results in a syngas rich in CH4 and H2 but poor in CO. Also, decreased SF and ER decrease the peak temperature (Tpeak) at the gasifier combustion zone. The syngas high heating value (HHV) ranged from 3112 kJ/SATPm3 to 5085 kJ/SATPm3 and its maximum value was obtained at SF = 0.87 and ER = 4.09. The dry basis molar concentrations of the species, produced under those operating conditions (1.53 〈 ER 〈 6.11 and 0.23 〈 SF 〈 0.89), were between 1.12 and 4.1% for CH4, between 7.77 and 13.49% for CO, and between 7.54 and 19.07% for H2. Other species were in trace amount.
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    Study of the Radical Chain Mechanism of Hydrocarbon Oxidation for In Situ Combustion Process (2017)
    Hindawi
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    Publication Date: 2017-01-01
    Description: Despite the abundance of in situ combustion models of oil oxidation, many of the effects are still beyond consideration. For example, until now, initial stages of oxidation were not considered from a position of radical chain process. This is a serious difficulty for the simulation of oil recovery process that involves air injection. To investigate the initial stages of oxidation, the paper considers the sequence of chemical reactions, including intermediate short-living compounds and radicals. We have attempted to correlate the main stages of the reaction with areas of heat release observed in the experiments. The system of differential equations based on the equations of oxidation reactions was solved. Time dependence of peroxides formation and start of heat release is analytically derived for the initial stages. We have considered the inhibition of initial oxidation stages by aromatic oil compounds and have studied the induction time in dependence on temperature. Chain ignition criteria for paraffins and crude oil in presence of core samples were obtained. The calculation results are compared with the stages of oxidation that arise by high-pressure differential scanning calorimetry. According to experimental observations we have determined which reactions are important for the process and which can be omitted or combined into one as insignificant.
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    The Role of Liquid Fuels Channel Configuration on the Combustion inside Cylindrical Mesoscale Combustor (2017)
    Hindawi
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    Publication Date: 2017-01-01
    Description: This research intended to investigate combustion of liquid fuel in 3.5 mm inner diameter quartz glass tube mesocombustor, based on liquid film evaporation by using heat recirculation. The mesocombustor has a copper section for heating and evaporating the liquid fuel. In mesocombustor type A, the fuel was glided through the narrow canal in the copper wall while the air was glided through the axial of combustor. The flame could only be successfully stabilized in high-ratio equivalent ranging from ɸ  =1.1 to ɸ=1.6, due to the gap without combustion reaction caused by high air-fuel mixture over the limits of flame stability. Mesocombustor type B, which has annulus-shaped canal, could shift the flame stability from ɸ  =0.8 to ɸ  =1.2; however, it also narrowed the limits of flame stability due to the wall cooling. In mesocombustor type C, both liquid fuel and air were glided through the annulus-shaped canal in the copper wall to fix the fuel evaporation and air mixture. The flame of type C was successfully stabilized, from ɸ  =0.73 to ɸ  =1.48 wider than types A and B. The flame of type C mesocombustor is circle-shaped and fitted to cross section of mesocombustor, but it still has thin gap without any flames due to thermal quenching by the wall.
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    Effects of Injection Rate Profile on Combustion Process and Emissions in a Diesel Engine (2017)
    Hindawi
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    Publication Date: 2017-01-01
    Description: When multi-injection is implemented in diesel engine via high pressure common rail injection system, changed interval between injection pulses can induce variation of injection rate profile for sequential injection pulse, though other control parameters are the same. Variations of injection rate shape which influence the air-fuel mixing and combustion process will be important for designing injection strategy. In this research, CFD numerical simulations using KIVA-3V were conducted for examining the effects of injection rate shape on diesel combustion and emissions. After the model was validated by experimental results, five different shapes (including rectangle, slope, triangle, trapezoid, and wedge) of injection rate profiles were investigated. Modeling results demonstrate that injection rate shape can have obvious influence on heat release process and heat release traces which cause different combustion process and emissions. It is observed that the baseline, rectangle (flat), shape of injection rate can have better balance between NOx and soot emissions than the other investigated shapes. As wedge shape brings about the lowest NOx emissions due to retarded heat release, it produces the highest soot emissions among the five shapes. Trapezoid shape has the lowest soot emissions, while its NOx is not the highest one. The highest NOx emissions were produced by triangle shape due to higher peak injection rate.
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    Influence of Advanced Injection Timing and Fuel Additive on Combustion, Performance, and Emission Characteristics of a DI Diesel Engine Running on Plastic Pyrolysis Oil (2017)
    Hindawi
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    Publication Date: 2017-01-01
    Description: This paper presents the investigation of engine optimisation when plastic pyrolysis oil (PPO) is used as the primary fuel of a direct injection diesel engine. Our previous investigation revealed that PPO is a promising fuel; however the results suggested that control parameters should be optimised in order to obtain a better engine performance. In the present work, the injection timing was advanced, and fuel additives were utilised to overcome the issues experienced in the previous work. In addition, spray characteristics of PPO were investigated in comparison with diesel to provide in-depth understanding of the engine behaviour. The experimental results on advanced injection timing (AIT) showed reduced brake thermal efficiency and increased carbon monoxide, unburned hydrocarbons, and nitrogen oxides emissions in comparison to standard injection timing. On the other hand, the addition of fuel additive resulted in higher engine efficiency and lower exhaust emissions. Finally, the spray tests revealed that the spray tip penetration for PPO is faster than diesel. The results suggested that AIT is not a preferable option while fuel additive is a promising solution for long-term use of PPO in diesel engines.
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    Decomposition Characteristics and Kinetics of Microalgae in N2 and CO2 Atmospheres by a Thermogravimetry (2017)
    Hindawi
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    Publication Date: 2017-01-01
    Description: The thermal degradation characteristics of microalgae were investigated in highly purified N2 and CO2 atmospheres by a thermogravimetric analysis (TGA) under different heating rates (10, 20, and 40°C/min). The results indicated that the total residual mass in CO2 atmosphere (16.86%) was less than in N2 atmosphere (23.12%); in addition, the kinetics of microalgae in N2 and CO2 atmospheres could be described by the pseudo bicomponent separated state model (PBSM) and pseudo-multi-component overall model (PMOM), respectively. The kinetic parameters calculated by Coats-Redfern method showed that, in CO2 atmosphere, the apparent activation energy (E) of microalgae was between 9.863 and 309.381 kJ mol−1 and the reaction order (n) was varied from 1.1 to 7. The kinetic parameters (E,n) of the second stage in CO2 atmosphere were quite similar to those in N2 atmosphere.
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    Parametric Study to Improve Subpixel Accuracy of Nitric Oxide Tagging Velocimetry with Image Preprocessing (2017)
    Hindawi
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    Publication Date: 2017-01-01
    Description: Biacetyl phosphorescence has been the commonly used molecular tagging velocimetry (MTV) technique to investigate in-cylinder flow evolution and cycle-to-cycle variations in an optical engine. As the phosphorescence of biacetyl tracer deteriorates in the presence of oxygen, nitrogen was adopted as the working medium in the past. Recently, nitrous oxide MTV technique was employed to measure the velocity profile of an air jet. The authors here plan to investigate the potential application of this technique for engine flow studies. A possible experimental setup for this task indicated different permutations of image signal-to-noise ratio (SNR) and laser line width. In the current work, a numerical analysis is performed to study the effect of these two factors on displacement error in MTV image processing. Also, several image filtering techniques were evaluated and the performance of selected filters was analyzed in terms of enhancing the image quality and minimizing displacement errors. The flow displacement error without image preprocessing was observed to be inversely proportional to SNR and directly proportional to laser line width. The mean filter resulted in the smallest errors for line widths smaller than 9 pixels. The effect of filter size on subpixel accuracy showed that error levels increased as the filter size increased.
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    Reduction of the Electrode Overpotential of the Oxygen Evolution Reaction by Electrode Surface Modification (2017)
    Hindawi
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    Publication Date: 2017-01-01
    Description: Metal–air batteries exhibit high potential for grid-scale energy storage because of their high theoretical energy density, their abundance in the earth’s crust, and their low cost. In these batteries, the oxygen evolution reaction (OER) occurs on the air electrode during charging. This study proposes a method for improving the OER electrode performance. The method involves sequentially depositing a Ni underlayer, Sn whiskers, and a Ni protection layer on the metal mesh. Small and uniform gas bubbles form on the Ni/Sn/Ni mesh, leading to low overpotential and a decrease in the overall resistance of the OER electrode. The results of a simulated life cycle test indicate that the Ni/Sn/Ni mesh has a life cycle longer than 1,300 cycles when it is used as the OER electrode in 6 M KOH.
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    Removal of Pb, Cu, Cd, and Zn Present in Aqueous Solution Using Coupled Electrocoagulation-Phytoremediation Treatment (2017)
    Hindawi
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    Publication Date: 2017-01-01
    Description: This study presents the results of a coupled electrocoagulation-phytoremediation treatment for the reduction of copper, cadmium, lead, and zinc, present in aqueous solution. The electrocoagulation was carried out in a batch reactor using aluminum electrodes in parallel arrangement; the optimal conditions were current density of 8 mA/cm2 and operating time of 180 minutes. For phytoremediation the macrophytes, Typha latifolia L., were used during seven days of treatment. The results indicated that the coupled treatment reduced metal concentrations by 99.2% Cu, 81.3% Cd, and 99.4% Pb, while Zn increased due to the natural concentrations of the plant used.
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